Lithium metal batteries (LMBs) show great potential in delivering high energy density (>500 Wh/kg) with cycling [1]. The cycling life of LMBs is mainly improved by regulating the composition and structure of solid/...Lithium metal batteries (LMBs) show great potential in delivering high energy density (>500 Wh/kg) with cycling [1]. The cycling life of LMBs is mainly improved by regulating the composition and structure of solid/cathode electrolyte interphase(SEI/CEI) with electrolytes [2]. However, both Li anode and transition metal oxide cathode have high interfacial reactivity at extreme voltages, which highly needs compatible electrolytes.Recently, localized high-concentration electrolytes (LHCEs) have promisingly stabilized the dual electrodes of high-voltage LMBs[3].展开更多
文摘Lithium metal batteries (LMBs) show great potential in delivering high energy density (>500 Wh/kg) with cycling [1]. The cycling life of LMBs is mainly improved by regulating the composition and structure of solid/cathode electrolyte interphase(SEI/CEI) with electrolytes [2]. However, both Li anode and transition metal oxide cathode have high interfacial reactivity at extreme voltages, which highly needs compatible electrolytes.Recently, localized high-concentration electrolytes (LHCEs) have promisingly stabilized the dual electrodes of high-voltage LMBs[3].