The unique advantage of x-ray ghost imaging(XGI)is its potential in low dose radiology.One of the practical ways to reduce the radiation exposure is to reduce the measurements while remaining sufficient image quality....The unique advantage of x-ray ghost imaging(XGI)is its potential in low dose radiology.One of the practical ways to reduce the radiation exposure is to reduce the measurements while remaining sufficient image quality.Synthetic aperture x-ray ghost imaging(SAXGI)is invented to achieve megapixel XGI with limited measurements,which is expected to implement XGI simultaneously with large field of view and low radiation exposure.In this paper,we experimentally investigate the effect of measurements reduction on the spatial resolution and image quality of SAXGI with standard sample and biomedical specimen.The results with a resolution chart demonstrated that at 360 measurements,SAXGI successfully retrieved the sample image of 1960×1960 pixels with spatial resolution of 4μm.With measurement reduction,the spatial resolution deteriorates but the sparser structures are still discernable.Even with measurements reduced to 10,a spatial resolution of 10μm can still be achieved by SAXGI.A biomedical sample of a fish specimen is employed to evaluate the method and the fish image of 2000×1000 pixels with an SSIM of 0.962 is reconstructed by SAXGI with 770measurements,corresponding to an accumulative exposure reduction of more than 2 times.With the measurements reduced to 10 which corresponds to 1/160 of the accumulative radiation exposure for conventional radiology,bulky structure like the fish skeleton can still be definitely discerned and the SSIM for the reconstructed image still retained 0.9179.Results of this paper demonstrate that measurements reduction is practicable for the radiation exposure reduction of the sample,which implicates that SAXGI with limited measurements is an efficient solution for low dose radiology.展开更多
A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-d...A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-dimensional cusp boundary from a two-dimensional X-ray image because the detected X-ray signals will be integrated along the line of sight.In this work,a global magnetohydrodynamic code was used to simulate the X-ray images and photon count images,assuming an interplanetary magnetic field with a pure Bz component.The assumption of an elliptic cusp boundary at a given altitude was used to trace the equatorward and poleward boundaries of the cusp from a simulated X-ray image.The average discrepancy was less than 0.1 RE.To reduce the influence of instrument effects and cosmic X-ray backgrounds,image denoising was considered before applying the method above to SXI photon count images.The cusp boundaries were reasonably reconstructed from the noisy X-ray image.展开更多
Aqueous zinc metal batteries(AZMBs)face significant challenges in achieving reversibility and cycling stability,primarily due to hydrogen evolution reactions(HER)and zinc dendrite growth.In this study,by employing car...Aqueous zinc metal batteries(AZMBs)face significant challenges in achieving reversibility and cycling stability,primarily due to hydrogen evolution reactions(HER)and zinc dendrite growth.In this study,by employing carefully designed cells that approximate the structural characteristics of practical batteries,we revisit this widely held view through in-operando X-ray radiography to examine zinc dendrite formation and HER under nearpractical operating conditions.While conventional understanding emphasizes the severity of these processes,our findings suggest that zinc dendrites and HER are noticeably less pronounced in dense,real-operation configurations compared to modified cells,possibly due to a more uniform electric field and the suppression of triple-phase boundaries.This study indicates that other components,such as degradation at the cathode current collector interface and configuration mismatches within the full cell,may also represent important barriers to the practical application of AZMBs,particularly during the early stages of electrodeposition.展开更多
Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method...Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method,an indirect imaging technique that requires algorithms to reconstruct and optimize images.During the last decade,a variety of algorithms have been developed and improved.However,it is difficult to quantitatively evaluate the image quality of different solutions without a true,reference image of observation.How to choose the values of imaging parameters for these algorithms to get the best performance is also an open question.In this study,we present a detailed test of the characteristics of these algorithms,imaging dynamic range and a crucial parameter for the CLEAN method,clean beam width factor(CBWF).We first used SDO/AIA EUV images to compute DEM maps and calculate thermal X-ray maps.Then these realistic sources and several types of simulated sources are used as the ground truth in the imaging simulations for both RHESSI and ASO-S/HXI.The different solutions are evaluated quantitatively by a number of means.The overall results suggest that EM,PIXON,and CLEAN are exceptional methods for sidelobe elimination,producing images with clear source details.Although MEM_GE,MEM_NJIT,VIS_WV and VIS_CS possess fast imaging processes and generate good images,they too possess associated imperfections unique to each method.The two forward fit algorithms,VF and FF,perform differently,and VF appears to be more robust and useful.We also demonstrated the imaging capability of HXI and available HXI algorithms.Furthermore,the effect of CBWF on image quality was investigated,and the optimal settings for both RHESSI and HXI were proposed.展开更多
With the increasing demand for oil exploration and subsurface resource development,density imaging plays an increasingly important role in identifying thin layers.However,conventional density imaging tools are limited...With the increasing demand for oil exploration and subsurface resource development,density imaging plays an increasingly important role in identifying thin layers.However,conventional density imaging tools are limited by poor vertical resolution and therefore suffer from errors in accurately estimating the thickness and relative dip angle of thin layers.This affects the accurate evaluation of thin layer oil and gas reserves.To address this issue,this study evaluates the feasibility of employing novel methods based on advanced tool design.First,an electronically controllable X-ray source is selected to replace the traditional Cs-137 source,aiming to improve the tool's vertical resolution while reducing the radioactive risks commonly associated with chemical sources.Simulation results show that the X-ray tool provides sufficient depth of investigation with better vertical resolution while maintaining the same level of measurement sensitivity.Once the tool design is established,Fisher's optimal segmentation method is improved to enhance the estimation of thin layer thickness and relative dip angle.This is completed by transforming identifying thin layer interface into a mathematical clustering problem.The thin layer interface is fitted using the nonlinear least squares method,which enables the calculation of its parameters.The results demonstrate a 38.5%reduction in RMSE(root mean square error)for thin layer thickness and a 33.7%reduction in RMSE for relative dip angle,demonstrating the superior performance of enhanced X-ray tool in thin layer identification.This study provides a new perspective on the design of density imaging tools and assessment of thin layer,which can help in future thin layer hydrocarbon reserves evaluation and development decisions.展开更多
Organic-inorganic hybrid clusters with strong X-ray radioluminescence have exhibited great potential in scintillator field.However,fabricating the X-ray imaging screens of the clusters without sacrificing the scintill...Organic-inorganic hybrid clusters with strong X-ray radioluminescence have exhibited great potential in scintillator field.However,fabricating the X-ray imaging screens of the clusters without sacrificing the scintillation performance is challenging.Herein,we report an effective way to prepare high-quality scintillation films of two synthesized Cu(Ⅰ)clusters through vacuum evaporation deposition.The developed Cu(Ⅰ)clusters with rigid molecular structures show excellent scintillation performance with a high light yield of up to 19356.7 photons/MeV and a low detection limit of 158 nGy/s.The scintillation film based on the Cu(Ⅰ)clusters made by vacuum evaporation deposition is highly uniform with a small surface roughness value of 1.04 nm,which can be applied to X-ray imaging for various objects.These results not only provide important guidance to develop high-performance organic-inorganic hybrid scintillators,but also pave a straightforward way to prepare non-doped scintillation screens for remarkable X-ray imaging applications.展开更多
This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):B...This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):Bi,Eu phosphors were synthesized,with Bi enhancing X-ray-induced photochromic prop-erties.Under X-ray irradiation,the phosphors transfer from white to red in bright field conditions and emit red photoluminescence in dark field conditions.Exposure to 470 nm ultraviolet light induces rapid bleaching.The mechanisms of photochromism and photoluminescence,particularly Bi's role as a colorant,were systematically investigated.The Ba_(2)LaNbO_(6):Bi,Eu phosphors film achieves high resolution,high-lighting its potential for X-ray imaging and non-destructive testing.Furthermore,the flexible Ba_(2)LaNbO_(6):Bi,Eu film supports dual-mode imaging and detection,addressing the limitations of traditional flat dis-plays in 3D imaging.展开更多
In x-ray dark-field imaging using dual phase grating interferometer,multi-contrast signals are extracted from a set of acquired phase-stepping data by using the least-squares fitting algorithm.The extracted mean inten...In x-ray dark-field imaging using dual phase grating interferometer,multi-contrast signals are extracted from a set of acquired phase-stepping data by using the least-squares fitting algorithm.The extracted mean intensity,amplitude and visibility signals may be intrinsically biased.However,it is still unclear how large these biases are and how the data acquisition parameters influence the biases in the extracted signals.This work set out to address these questions.Analytical expressions of the biases of the extracted signals were theoretically derived by using a second-order Taylor series expansion.Extensive numerical simulations were performed to validate the theoretical results.It is illustrated that while the estimated mean intensity signal is always unbiased,the estimated amplitude and visibility signals are both positively biased.While the biases of the estimated amplitude signals are proportional to the inverse of the total number of phase steps,the biases of the estimated visibility signals are inversely proportional to the product of the total number of phase steps and the mean number of photons counted per phase step.Meanwhile,it is demonstrated that the dependence of the biases on the mean visibility is quite different from that of Talbot-Lau interferometer due to the difference in the intensity model.We expect that these results can be useful for data acquisition optimizations and interpretation of x-ray dark-field images.展开更多
BACKGROUND The objective of this study was to evaluate the use of combined parallax-free panoramic X-ray imaging during surgery by enabling the mobile C-arm with minimally invasive plate osteosynthesis(MIPO)in the man...BACKGROUND The objective of this study was to evaluate the use of combined parallax-free panoramic X-ray imaging during surgery by enabling the mobile C-arm with minimally invasive plate osteosynthesis(MIPO)in the management of proximal humeral shaft fractures.AIM To evaluate parallax-free panoramic X-ray images during surgery.METHODS A retrospective series of 17 proximal humeral shaft fractures were treated using combined parallax-free panoramic X-ray imaging during surgery by enabling the mobile C-arm with MIPO.The operating time and radiation exposure time were recorded,and early postoperative physical therapy and partial weight bearing were encouraged.Patients were followed at regular intervals and evaluated radiographically and clinically.RESULTS The mean operating time and radiation time were 73(range,49-95)minutes and 57(range:36-98)seconds,respectively.No complications occurred during the operation.All fractures healed at an average of 16.9(range:15-23)weeks.The average Constant-Murley score for all the patients was 89.5(range:75-100)points.None of the patients showed symptoms of vascular or nerve damage or wound infection.Three months after the operation,none of the patients developed subacromial impingement syndrome.No loosening or fracture of the implants occurred.The frontal and lateral radiographs showed good alignment.CONCLUSION We consider that MIPO with combined parallax-free panoramic X-ray imaging during surgery is an efficient method for treating proximal humeral shaft fractures,and could significantly reduce operative morbidity as well as lower the rate of intra-and postoperative complications.展开更多
This study presents an advanced method for post-mortem person identification using the segmentation of skeletal structures from chest X-ray images.The proposed approach employs the Attention U-Net architecture,enhance...This study presents an advanced method for post-mortem person identification using the segmentation of skeletal structures from chest X-ray images.The proposed approach employs the Attention U-Net architecture,enhanced with gated attention mechanisms,to refine segmentation by emphasizing spatially relevant anatomical features while suppressing irrelevant details.By isolating skeletal structures which remain stable over time compared to soft tissues,this method leverages bones as reliable biometric markers for identity verification.The model integrates custom-designed encoder and decoder blocks with attention gates,achieving high segmentation precision.To evaluate the impact of architectural choices,we conducted an ablation study comparing Attention U-Net with and without attentionmechanisms,alongside an analysis of data augmentation effects.Training and evaluation were performed on a curated chest X-ray dataset,with segmentation performance measured using Dice score,precision,and loss functions,achieving over 98% precision and 94% Dice score.The extracted bone structures were further processed to derive unique biometric patterns,enabling robust and privacy-preserving person identification.Our findings highlight the effectiveness of attentionmechanisms in improving segmentation accuracy and underscore the potential of chest bonebased biometrics in forensic and medical imaging.This work paves the way for integrating artificial intelligence into real-world forensic workflows,offering a non-invasive and reliable solution for post-mortem identification.展开更多
This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the...This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the past 5 years.The photon energy range of the beamline is 8–72.5 keV.Several sets of X-ray imaging detectors with different pixel sizes(0.19–24 lm)are used to realize X-ray microcomputed tomography(X-ray micro-CT)and X-ray in-line phase-contrast imaging.To satisfy the requirements of user experiments,new X-ray imaging methods and image processing techniques are developed.In vivo dynamic micro-CT experiments with living insects are performed in 0.5 s(sampling rate of 2 Hz,2 tomograms/s)with a monochromatic beam from a wiggler source and in 40 ms(sampling rate of 25 Hz,25 tomograms/s)with a white beam from a bending magnet source.A new X-ray imaging method known as move contrast X-ray imaging is proposed,with which blood flow and moving tissues in raw images can be distinguished according to their moving frequencies in the time domain.Furthermore,X-ray speckle-tracking imaging with twice exposures to eliminate the edge enhancement effect is developed.A high-precision quantification method is realized to measure complex three-dimensional blood vessels obtained via X-ray micro-CT.X-ray imaging methods such as three-dimensional X-ray diffraction microscopy,small-angle X-ray scattering CT,and X-ray fluorescence CT are developed,in which the X-ray micro-CT imaging method is combined with other contrast mechanisms such as diffraction,scattering,and fluorescence contrasts respectively.Moreover,an X-ray nano-CT experiment is performed with a 100 nm spatial resolution.Typical user experimental results from the fields of material science,biomedicine,paleontology,physics,chemistry,and environmental science obtained on the beamline are provided.展开更多
BACKGROUND Early-stage breast cancer patients often lack specific clinical manifestations,making diagnosis difficult.Molybdenum target X-ray and magnetic resonance imaging(MRI)examinations both have their own advantag...BACKGROUND Early-stage breast cancer patients often lack specific clinical manifestations,making diagnosis difficult.Molybdenum target X-ray and magnetic resonance imaging(MRI)examinations both have their own advantages.Thus,a combined examination methodology may improve early breast cancer diagnoses.AIM To explore the combined diagnostic efficacy of molybdenum target X-ray and MRI examinations in breast cancer.METHODS Patients diagnosed with breast cancer at our hospital from March 2019 to April 2021 were recruited,as were the same number of patients during the same period with benign breast tumors.Both groups underwent molybdenum target X-ray and MRI examinations,and diagnoses were given based on each exam.The single(i.e.,X-ray or MRI)and combined(i.e.,using both methods)diagnoses were counted,and the MRI-related examination parameters(e.g.,T-wave peak,peak and early enhancement rates,and apparent diffusion coefficient)were compared between the groups.RESULTS In total,63 breast cancer patients and 63 benign breast tumor patients were recruited.MRI detected 53 breast cancer cases and 61 benign breast tumor cases.Molybdenum target X-ray detected 50 breast cancer cases and 60 benign breast tumor cases.The combined methodology detected 61 breast cancer cases and 61 benign breast tumor cases.The sensitivity(96.83%)and accuracy(96.83%)of the combined methodology were higher than single-method MRI(84.13%and 90.48%,respectively)and molybdenum target X-ray(79.37%and 87.30%,respectively)(P<0.05).The combined methodology specificity(96.83%)did not differ from singlemethod MRI(96.83%)or molybdenum target X-ray(95.24%)(P>0.05).The Twave peak(169.43±32.05)and apparent diffusion coefficient(1.01±0.23)were lower in the breast cancer group than in the benign tumor group(228.86±46.51 and 1.41±0.35,respectively).However,the peak enhancement rate(1.08±0.24)and early enhancement rate(1.07±0.26)were significantly higher in the breast cancer group than in the benign tumor group(0.83±0.19 and 0.75±0.19,respectively)(P<0.05).CONCLUSION Combined molybdenum target X-ray and MRI examinations for diagnosing breast cancer improved the diagnostic sensitivity and accuracy,minimizing the missedand misdiagnoses risks and promoting timely treatment intervention.展开更多
Characterizing the microstructure and deformation mechanism associated with the performances and properties of metallic materials is of great importance in understanding the microstructure-property relationship.The pa...Characterizing the microstructure and deformation mechanism associated with the performances and properties of metallic materials is of great importance in understanding the microstructure-property relationship.The past few decades have witnessed the rapid development of characterization techniques from optical microscopy to electron microscopy,although these conventional methods are generally limited to the sample surface because of the intrinsic opaque nature of metallic materials.Advanced synchrotron radiation(SR)facilities can produce X-rays with strong penetrability and high spatiotemporal resolution,and thereby enabling the non-destructive visualization of full-field structural information in three dimensions.Tremendous endeavors were devoted to the 3 rd generation SR over the past three decades,in which X-ray beams have been focused down to 100 nm.In this paper,recent progresses on SR-related characterization technologies were reviewed,with particular emphases on the fundamentals of synchrotron X-ray imaging and synchrotron X-ray diffraction,as well as their applications in the in situ observations of material preparation(e.g.,in situ dendrite growth during solidification)and service under extreme environment(e.g.,in situ mechanics).Future innovations toward next-generation SR and newly emerging SRbased technologies such as dark-field X-ray microscopy and Bragg coherent X-ray diffraction imaging were also advocated.展开更多
Additive manufacturing(AM)is a rapid prototyping technology based on the idea of discrete accumulation which off ers an advantage of economically fabricating a component with complex geometries in a rapid design-to-ma...Additive manufacturing(AM)is a rapid prototyping technology based on the idea of discrete accumulation which off ers an advantage of economically fabricating a component with complex geometries in a rapid design-to-manufacture cycle.However,various internal defects,such as balling,cracks,residual stress and porosity,are inevitably occurred during AM due to the complexity of laser/electron beam-powder interaction,rapid melting and solidification process,and microstructure evolution.The existence of porosity defects can potentially deteriorate the mechanical properties of selective laser melting(SLM)components,such as material stiff ness,hardness,tensile strength,and fatigue resistance performance.Synchrotron X-ray imaging and diffraction are important non-destructive means to elaborately characterize the internal defect characteristics and mechanical properties of AM parts.This paper presents a review on the application of synchrotron X-ray in identifying and verifying the quality and requirement of AM parts.Defects,microstructures and mechanical properties of printed components characterized by synchrotron X-ray imaging and diffraction are summarized in this review.Subsequently,this paper also elaborates on the online characterization of the evolution of the microstructure during AM using synchrotron X-ray imaging,and introduces the method for measuring AM stress by X-ray diffraction(XRD).Finally,the future application of synchrotron X-ray characterization in the AM is prospected.展开更多
Wet chemistry methods,including hot-injection and precipitation methods,have emerged as major synthetic routes for high-quality perovskite nanocrystals in backlit display and scintillation applications.However,low che...Wet chemistry methods,including hot-injection and precipitation methods,have emerged as major synthetic routes for high-quality perovskite nanocrystals in backlit display and scintillation applications.However,low chemical yield hinders their upscale production for practical use.Meanwhile,the labile nature of halide-based perovskite poses a major challenge for long-term storage of perovskite nanocrystals.Herein,we report a green synthesis at room temperature for gram-scale production of CsPbBr3 nanosheets with minimum use of solvent,saving over 95% of the solvent for the unity mass nanocrystal production.The perovskite colloid exhibits record stability upon long-term storage for up to 8 months,preserving a photoluminescence quantum yield of 63% in solid state.Importantly,the colloidal nanosheets show self-assembly behavior upon slow solidification,generating a crack-free thin film in a large area.The uniform film was then demonstrated as an efficient scintillation screen for X-ray imaging.Our findings bring a scalable tool for synthesis of high-quality perovskite nanocrystals,which may inspire the industrial optoelectronic application of large-area perovskite film.展开更多
Doped elements in alloys significantly impact their performance.Conventional methods usually sputter the surface material of the sample,or their performance is limited to the surface of alloys owing to their poor pene...Doped elements in alloys significantly impact their performance.Conventional methods usually sputter the surface material of the sample,or their performance is limited to the surface of alloys owing to their poor penetration ability.The X-ray K-edge subtraction(KES)method exhibits great potential for the nondestructive in situ detection of element contents in alloys.However,the signal of doped elements usually deteriorates because of the strong absorption of the principal component and scattering of crystal grains.This in turn prevents the extensive application of X-ray KES imaging to alloys.In this study,methods were developed to calibrate the linearity between the grayscale of the KES image and element content.The methods were aimed at the sensitive analysis of elements in alloys.Furthermore,experiments with phantoms and alloys demonstrated that,after elaborate calibration,X-ray KES imaging is capable of nondestructive and sensitive analysis of doped elements in alloys.展开更多
Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image qual...Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image quality of the reconstruction is still difficult,which is particularly useful for scheme design of X-ray imaging systems,testing and improvement of imaging algorithms,and scientific research of X-ray sources.Currently,there is no specified method to quantitatively evaluate the quality of X-ray image reconstruction and the point-spread function(PSF)of an X-ray imager.In this paper,we propose percentage proximity degree(PPD)by considering the imaging characteristics of X-ray image reconstruction and in particular,sidelobes and their effects on imaging quality.After testing a variety of imaging quality assessments in six aspects,we utilized the technique for order preference by similarity to ideal solution to the indices that meet the requirements.Then we develop the final quality index for X-ray image reconstruction,QuIX,which consists of the selected indices and the new PPD.QuIX performs well in a series of tests,including assessment of instrument PSF and simulation tests under different grid configurations,as well as imaging tests with RHESSI data.It is also a useful tool for testing of imaging algorithms,and determination of imaging parameters for both RHESSI and ASO-S/Hard X-ray Imager,such as field of view,beam width factor,and detector selection.展开更多
A first and effective method is proposed to detect weld deject adaptively in various Dypes of real-time X-ray images obtained in different conditions. After weld extraction and noise reduction, a proper template of me...A first and effective method is proposed to detect weld deject adaptively in various Dypes of real-time X-ray images obtained in different conditions. After weld extraction and noise reduction, a proper template of median filter is used to estimate the weld background. After the weld background is subtracted from the original image, an adaptite threshold segmentation algorithm is proposed to obtain the binary image, and then the morphological close and open operation, labeling algorithm and fids＇e alarm eliminating algorithm are applied to pracess the binary image to obtain the defect, ct detection result. At last, a fast realization procedure jbr proposed method is developed. The proposed method is tested in real-time X-ray image,s obtairted in different X-ray imaging sutems. Experiment results show that the proposed method is effective to detect low contrast weld dejects with few .false alarms and is adaptive to various types of real-time X-ray imaging systems.展开更多
X-ray detection and imaging via scintillators has been utilized in missions worldwide within areas of scientific research,medical industry,military defense and homeland security.Commercial scintillators are costly wit...X-ray detection and imaging via scintillators has been utilized in missions worldwide within areas of scientific research,medical industry,military defense and homeland security.Commercial scintillators are costly with high energy consumption through the sintering.It is of great significance to seek alternative scintillating materials for sensitive X-ray detection in the next-generation.Herein,eight structure-defined Ln(Ⅲ)-based metal-organic frameworks(Ln-MOFs)were prepared,2D[Ln_(2)(1,4-ndc)_(3)(DMF)_(4)]_(n)·nH_(2)O(Ln=Sm 1,Eu 2,Dy 3,Tb 4)and 3D[Ln_(4)(2,6-ndc)_(6)(μ_(2)H_(2)O)2(H_(2)O)_(4)]n·2nH_(2)O(Ln=Sm 5,Eu 6,Dy 7,Tb 8),where 1,4-H_(2)ndc=1,4-naphthalene dicarboxylate acid,2,6-H_(2)ndc=2,6-napthalene dicarboxylate acid,DMF=N,N-dimethylformamide.Merely compounds 2 and 6 show remarkable X-ray scintillation performance via the characteristic red emissions of Eu(Ⅲ)ions,in which the absorbed energy from the triplet states of the organic moieties can be transferred more efficiently to the resonance emission levels of Eu(Ⅲ)ions than other lanthanide(Ⅲ)ions.The X-ray dosage rate detection limits of 2 and 6 are superior to the standard for the medical X-ray diagnosis dosage rate.As proofs-of-concepts,matrix-mixed membranes fabricated with 2 and 6 have achieved remarkable X-ray imaging with high resolution for practical object shooting.展开更多
In recent years,persistent luminescence materials(PLMs)excited by X-rays and emitting in biological windows have received extensive attention in the field of high-sensitivity bioimaging.Transition metal Mn^(2+)is an i...In recent years,persistent luminescence materials(PLMs)excited by X-rays and emitting in biological windows have received extensive attention in the field of high-sensitivity bioimaging.Transition metal Mn^(2+)is an ideal emission center,but few studies focus on Mn^(2+)-doped PLMs with X-ray excitation and biological window emission.Here,we report a Mn^(2+)-doped PLM,LiYGeO_(4):Mn^(2+)(LYGM),with excellent biological window persistent luminescence emission.After excitation by UV,LYGM produces a durable biological window of persistent luminescence emission at 660 nm for up to 20 h.More importantly.LYGM can be repeatedly excited by X-rays,resulting in long-term biological window persistent luminescence emission.In addition,we obtain LYGM around 200 nm in diameter by ball milling and centrifugation and improve its biocompatibility by surface modification to apply it to in vivo imaging in mice.After LYGM are injected into mice through the tail vein,in situ excitation of X-rays can be achieved.After the persistent luminescence decays,LYGM can be re-excited for repeated imaging.Therefore,LYGM shows potential prospects for in vivo deep tissue and long-term bioimaging.展开更多
基金Project supported by the National Key Research and Development Program of China(Grant Nos.2022YFA1603601,2021YFF0601203,and 2021YFA1600703)。
文摘The unique advantage of x-ray ghost imaging(XGI)is its potential in low dose radiology.One of the practical ways to reduce the radiation exposure is to reduce the measurements while remaining sufficient image quality.Synthetic aperture x-ray ghost imaging(SAXGI)is invented to achieve megapixel XGI with limited measurements,which is expected to implement XGI simultaneously with large field of view and low radiation exposure.In this paper,we experimentally investigate the effect of measurements reduction on the spatial resolution and image quality of SAXGI with standard sample and biomedical specimen.The results with a resolution chart demonstrated that at 360 measurements,SAXGI successfully retrieved the sample image of 1960×1960 pixels with spatial resolution of 4μm.With measurement reduction,the spatial resolution deteriorates but the sparser structures are still discernable.Even with measurements reduced to 10,a spatial resolution of 10μm can still be achieved by SAXGI.A biomedical sample of a fish specimen is employed to evaluate the method and the fish image of 2000×1000 pixels with an SSIM of 0.962 is reconstructed by SAXGI with 770measurements,corresponding to an accumulative exposure reduction of more than 2 times.With the measurements reduced to 10 which corresponds to 1/160 of the accumulative radiation exposure for conventional radiology,bulky structure like the fish skeleton can still be definitely discerned and the SSIM for the reconstructed image still retained 0.9179.Results of this paper demonstrate that measurements reduction is practicable for the radiation exposure reduction of the sample,which implicates that SAXGI with limited measurements is an efficient solution for low dose radiology.
基金funded by the National Natural Science Foundation of China(NNSFC)under Grant Numbers 42322408,42188101,and 42441809Additional support was provided by the Climbing Program of the National Space Science Center(NSSC,Grant No.E4PD3005)as well as the Specialized Research Fund for State Key Laboratories of China.
文摘A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-dimensional cusp boundary from a two-dimensional X-ray image because the detected X-ray signals will be integrated along the line of sight.In this work,a global magnetohydrodynamic code was used to simulate the X-ray images and photon count images,assuming an interplanetary magnetic field with a pure Bz component.The assumption of an elliptic cusp boundary at a given altitude was used to trace the equatorward and poleward boundaries of the cusp from a simulated X-ray image.The average discrepancy was less than 0.1 RE.To reduce the influence of instrument effects and cosmic X-ray backgrounds,image denoising was considered before applying the method above to SXI photon count images.The cusp boundaries were reasonably reconstructed from the noisy X-ray image.
基金the fundamental Research Funds for the central Universities(x2wjD2240360)for the funding supportMeanwhile,Engineering and Physical Sciences Research Council(EPSRC,EP/V027433/3)+2 种基金UK Research and Innovation(UKRI)under the UK government’s Horizon Europe funding(101077226,EP/Y008707/1)Faraday Institution(EP/S003053/1)Degradation project(FIRG001),Royal Society(IEC\NSFC\233361),QUB Agility Fund and Wright Technology and Research Centre(W-Tech,R5240MEE)Funding from UK aid from the UK Government through the Faraday Institution and the Transforming Energy Access Programme(Grant number FIRG050-Device engineering of Zn-based hybrid micro-flow batteries and by-product H2 collection for Emerging Economies)。
文摘Aqueous zinc metal batteries(AZMBs)face significant challenges in achieving reversibility and cycling stability,primarily due to hydrogen evolution reactions(HER)and zinc dendrite growth.In this study,by employing carefully designed cells that approximate the structural characteristics of practical batteries,we revisit this widely held view through in-operando X-ray radiography to examine zinc dendrite formation and HER under nearpractical operating conditions.While conventional understanding emphasizes the severity of these processes,our findings suggest that zinc dendrites and HER are noticeably less pronounced in dense,real-operation configurations compared to modified cells,possibly due to a more uniform electric field and the suppression of triple-phase boundaries.This study indicates that other components,such as degradation at the cathode current collector interface and configuration mismatches within the full cell,may also represent important barriers to the practical application of AZMBs,particularly during the early stages of electrodeposition.
基金supported by the National Key R&D Program of China 2022YFF0503002the National Natural Science Foundation of China(NSFC,Grant Nos.12333010 and 12233012)+2 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(grant No.XDB0560000)supported by the Prominent Postdoctoral Project of Jiangsu Province(2023ZB304)supported by the Strategic Priority Research Program on Space Science,the Chinese Academy of Sciences,grant No.XDA15320000.
文摘Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method,an indirect imaging technique that requires algorithms to reconstruct and optimize images.During the last decade,a variety of algorithms have been developed and improved.However,it is difficult to quantitatively evaluate the image quality of different solutions without a true,reference image of observation.How to choose the values of imaging parameters for these algorithms to get the best performance is also an open question.In this study,we present a detailed test of the characteristics of these algorithms,imaging dynamic range and a crucial parameter for the CLEAN method,clean beam width factor(CBWF).We first used SDO/AIA EUV images to compute DEM maps and calculate thermal X-ray maps.Then these realistic sources and several types of simulated sources are used as the ground truth in the imaging simulations for both RHESSI and ASO-S/HXI.The different solutions are evaluated quantitatively by a number of means.The overall results suggest that EM,PIXON,and CLEAN are exceptional methods for sidelobe elimination,producing images with clear source details.Although MEM_GE,MEM_NJIT,VIS_WV and VIS_CS possess fast imaging processes and generate good images,they too possess associated imperfections unique to each method.The two forward fit algorithms,VF and FF,perform differently,and VF appears to be more robust and useful.We also demonstrated the imaging capability of HXI and available HXI algorithms.Furthermore,the effect of CBWF on image quality was investigated,and the optimal settings for both RHESSI and HXI were proposed.
基金the support of theNational Natural Science Foundation of China(U23B20151 and52171253)。
文摘With the increasing demand for oil exploration and subsurface resource development,density imaging plays an increasingly important role in identifying thin layers.However,conventional density imaging tools are limited by poor vertical resolution and therefore suffer from errors in accurately estimating the thickness and relative dip angle of thin layers.This affects the accurate evaluation of thin layer oil and gas reserves.To address this issue,this study evaluates the feasibility of employing novel methods based on advanced tool design.First,an electronically controllable X-ray source is selected to replace the traditional Cs-137 source,aiming to improve the tool's vertical resolution while reducing the radioactive risks commonly associated with chemical sources.Simulation results show that the X-ray tool provides sufficient depth of investigation with better vertical resolution while maintaining the same level of measurement sensitivity.Once the tool design is established,Fisher's optimal segmentation method is improved to enhance the estimation of thin layer thickness and relative dip angle.This is completed by transforming identifying thin layer interface into a mathematical clustering problem.The thin layer interface is fitted using the nonlinear least squares method,which enables the calculation of its parameters.The results demonstrate a 38.5%reduction in RMSE(root mean square error)for thin layer thickness and a 33.7%reduction in RMSE for relative dip angle,demonstrating the superior performance of enhanced X-ray tool in thin layer identification.This study provides a new perspective on the design of density imaging tools and assessment of thin layer,which can help in future thin layer hydrocarbon reserves evaluation and development decisions.
文摘Organic-inorganic hybrid clusters with strong X-ray radioluminescence have exhibited great potential in scintillator field.However,fabricating the X-ray imaging screens of the clusters without sacrificing the scintillation performance is challenging.Herein,we report an effective way to prepare high-quality scintillation films of two synthesized Cu(Ⅰ)clusters through vacuum evaporation deposition.The developed Cu(Ⅰ)clusters with rigid molecular structures show excellent scintillation performance with a high light yield of up to 19356.7 photons/MeV and a low detection limit of 158 nGy/s.The scintillation film based on the Cu(Ⅰ)clusters made by vacuum evaporation deposition is highly uniform with a small surface roughness value of 1.04 nm,which can be applied to X-ray imaging for various objects.These results not only provide important guidance to develop high-performance organic-inorganic hybrid scintillators,but also pave a straightforward way to prepare non-doped scintillation screens for remarkable X-ray imaging applications.
基金supported by the Key Project of the National Natural Science Foundation of China-Yunnan Joint Fund(No.U2102215)National Natural Science Foundation(No.52472002)+5 种基金Science and Technology Project of Southwest Joint Graduate School of Yunnan Province(No.202302A0370008)2024 Industrial Innovation Talent Support Project(Preparation of luminous materials,performance control and application in plateau agriculture,No.YFGRC202407)National Natural Science Foundation of High-End Foreign Expert Introduction Plan(No.G2022039008L)Academician Workstation of Cherkasova Tatiana in Yunnan Province(No.202305AF150099)Yunnan Province Major Science and Technology Special Plan(No.202302AB080005)and UTS Chancellor’s Research Fellowship Program(No.J.L.,PRO22-15457)the National Health and Medical Research Council(No.J.L.,2025442).
文摘This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):Bi,Eu phosphors were synthesized,with Bi enhancing X-ray-induced photochromic prop-erties.Under X-ray irradiation,the phosphors transfer from white to red in bright field conditions and emit red photoluminescence in dark field conditions.Exposure to 470 nm ultraviolet light induces rapid bleaching.The mechanisms of photochromism and photoluminescence,particularly Bi's role as a colorant,were systematically investigated.The Ba_(2)LaNbO_(6):Bi,Eu phosphors film achieves high resolution,high-lighting its potential for X-ray imaging and non-destructive testing.Furthermore,the flexible Ba_(2)LaNbO_(6):Bi,Eu film supports dual-mode imaging and detection,addressing the limitations of traditional flat dis-plays in 3D imaging.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.U1532113,11475170,11905041)Anhui Provincial Natural Science Foundation(Grant No.2208085MA18)Fundamental Research Funds for the Central Universities(Grant No.JZ2022HGTB0244)。
文摘In x-ray dark-field imaging using dual phase grating interferometer,multi-contrast signals are extracted from a set of acquired phase-stepping data by using the least-squares fitting algorithm.The extracted mean intensity,amplitude and visibility signals may be intrinsically biased.However,it is still unclear how large these biases are and how the data acquisition parameters influence the biases in the extracted signals.This work set out to address these questions.Analytical expressions of the biases of the extracted signals were theoretically derived by using a second-order Taylor series expansion.Extensive numerical simulations were performed to validate the theoretical results.It is illustrated that while the estimated mean intensity signal is always unbiased,the estimated amplitude and visibility signals are both positively biased.While the biases of the estimated amplitude signals are proportional to the inverse of the total number of phase steps,the biases of the estimated visibility signals are inversely proportional to the product of the total number of phase steps and the mean number of photons counted per phase step.Meanwhile,it is demonstrated that the dependence of the biases on the mean visibility is quite different from that of Talbot-Lau interferometer due to the difference in the intensity model.We expect that these results can be useful for data acquisition optimizations and interpretation of x-ray dark-field images.
基金Supported by Wuhu Municipal Science and Technology Bureau of Anhui Province,No.2022cg43.
文摘BACKGROUND The objective of this study was to evaluate the use of combined parallax-free panoramic X-ray imaging during surgery by enabling the mobile C-arm with minimally invasive plate osteosynthesis(MIPO)in the management of proximal humeral shaft fractures.AIM To evaluate parallax-free panoramic X-ray images during surgery.METHODS A retrospective series of 17 proximal humeral shaft fractures were treated using combined parallax-free panoramic X-ray imaging during surgery by enabling the mobile C-arm with MIPO.The operating time and radiation exposure time were recorded,and early postoperative physical therapy and partial weight bearing were encouraged.Patients were followed at regular intervals and evaluated radiographically and clinically.RESULTS The mean operating time and radiation time were 73(range,49-95)minutes and 57(range:36-98)seconds,respectively.No complications occurred during the operation.All fractures healed at an average of 16.9(range:15-23)weeks.The average Constant-Murley score for all the patients was 89.5(range:75-100)points.None of the patients showed symptoms of vascular or nerve damage or wound infection.Three months after the operation,none of the patients developed subacromial impingement syndrome.No loosening or fracture of the implants occurred.The frontal and lateral radiographs showed good alignment.CONCLUSION We consider that MIPO with combined parallax-free panoramic X-ray imaging during surgery is an efficient method for treating proximal humeral shaft fractures,and could significantly reduce operative morbidity as well as lower the rate of intra-and postoperative complications.
基金funded by Umm Al-Qura University,Saudi Arabia under grant number:25UQU4300346GSSR08.
文摘This study presents an advanced method for post-mortem person identification using the segmentation of skeletal structures from chest X-ray images.The proposed approach employs the Attention U-Net architecture,enhanced with gated attention mechanisms,to refine segmentation by emphasizing spatially relevant anatomical features while suppressing irrelevant details.By isolating skeletal structures which remain stable over time compared to soft tissues,this method leverages bones as reliable biometric markers for identity verification.The model integrates custom-designed encoder and decoder blocks with attention gates,achieving high segmentation precision.To evaluate the impact of architectural choices,we conducted an ablation study comparing Attention U-Net with and without attentionmechanisms,alongside an analysis of data augmentation effects.Training and evaluation were performed on a curated chest X-ray dataset,with segmentation performance measured using Dice score,precision,and loss functions,achieving over 98% precision and 94% Dice score.The extracted bone structures were further processed to derive unique biometric patterns,enabling robust and privacy-preserving person identification.Our findings highlight the effectiveness of attentionmechanisms in improving segmentation accuracy and underscore the potential of chest bonebased biometrics in forensic and medical imaging.This work paves the way for integrating artificial intelligence into real-world forensic workflows,offering a non-invasive and reliable solution for post-mortem identification.
基金This work was supported by the National Key Research and Development Program of China(Nos.2017YFA0403801,2016YFA0401302,2017YFA0206004,2018YFC1200204)the National Major Scientific Instruments and Equipment Development Project of China(No.11627901).
文摘This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the past 5 years.The photon energy range of the beamline is 8–72.5 keV.Several sets of X-ray imaging detectors with different pixel sizes(0.19–24 lm)are used to realize X-ray microcomputed tomography(X-ray micro-CT)and X-ray in-line phase-contrast imaging.To satisfy the requirements of user experiments,new X-ray imaging methods and image processing techniques are developed.In vivo dynamic micro-CT experiments with living insects are performed in 0.5 s(sampling rate of 2 Hz,2 tomograms/s)with a monochromatic beam from a wiggler source and in 40 ms(sampling rate of 25 Hz,25 tomograms/s)with a white beam from a bending magnet source.A new X-ray imaging method known as move contrast X-ray imaging is proposed,with which blood flow and moving tissues in raw images can be distinguished according to their moving frequencies in the time domain.Furthermore,X-ray speckle-tracking imaging with twice exposures to eliminate the edge enhancement effect is developed.A high-precision quantification method is realized to measure complex three-dimensional blood vessels obtained via X-ray micro-CT.X-ray imaging methods such as three-dimensional X-ray diffraction microscopy,small-angle X-ray scattering CT,and X-ray fluorescence CT are developed,in which the X-ray micro-CT imaging method is combined with other contrast mechanisms such as diffraction,scattering,and fluorescence contrasts respectively.Moreover,an X-ray nano-CT experiment is performed with a 100 nm spatial resolution.Typical user experimental results from the fields of material science,biomedicine,paleontology,physics,chemistry,and environmental science obtained on the beamline are provided.
基金Supported by Clinical Plateau Department,Shanghai Pudong New Area Health Construction Commission,No.PWYgy2018-04.
文摘BACKGROUND Early-stage breast cancer patients often lack specific clinical manifestations,making diagnosis difficult.Molybdenum target X-ray and magnetic resonance imaging(MRI)examinations both have their own advantages.Thus,a combined examination methodology may improve early breast cancer diagnoses.AIM To explore the combined diagnostic efficacy of molybdenum target X-ray and MRI examinations in breast cancer.METHODS Patients diagnosed with breast cancer at our hospital from March 2019 to April 2021 were recruited,as were the same number of patients during the same period with benign breast tumors.Both groups underwent molybdenum target X-ray and MRI examinations,and diagnoses were given based on each exam.The single(i.e.,X-ray or MRI)and combined(i.e.,using both methods)diagnoses were counted,and the MRI-related examination parameters(e.g.,T-wave peak,peak and early enhancement rates,and apparent diffusion coefficient)were compared between the groups.RESULTS In total,63 breast cancer patients and 63 benign breast tumor patients were recruited.MRI detected 53 breast cancer cases and 61 benign breast tumor cases.Molybdenum target X-ray detected 50 breast cancer cases and 60 benign breast tumor cases.The combined methodology detected 61 breast cancer cases and 61 benign breast tumor cases.The sensitivity(96.83%)and accuracy(96.83%)of the combined methodology were higher than single-method MRI(84.13%and 90.48%,respectively)and molybdenum target X-ray(79.37%and 87.30%,respectively)(P<0.05).The combined methodology specificity(96.83%)did not differ from singlemethod MRI(96.83%)or molybdenum target X-ray(95.24%)(P>0.05).The Twave peak(169.43±32.05)and apparent diffusion coefficient(1.01±0.23)were lower in the breast cancer group than in the benign tumor group(228.86±46.51 and 1.41±0.35,respectively).However,the peak enhancement rate(1.08±0.24)and early enhancement rate(1.07±0.26)were significantly higher in the breast cancer group than in the benign tumor group(0.83±0.19 and 0.75±0.19,respectively)(P<0.05).CONCLUSION Combined molybdenum target X-ray and MRI examinations for diagnosing breast cancer improved the diagnostic sensitivity and accuracy,minimizing the missedand misdiagnoses risks and promoting timely treatment intervention.
基金financially supported by the National Key Research and Development Plan(Grant Nos.2020YFA0405900,2017YFA0403803)the National Natural Science Foundation of China(Grant No.51927801)the Natural Science Foundation of Jiangsu Province(Grant No.BK20202010)。
文摘Characterizing the microstructure and deformation mechanism associated with the performances and properties of metallic materials is of great importance in understanding the microstructure-property relationship.The past few decades have witnessed the rapid development of characterization techniques from optical microscopy to electron microscopy,although these conventional methods are generally limited to the sample surface because of the intrinsic opaque nature of metallic materials.Advanced synchrotron radiation(SR)facilities can produce X-rays with strong penetrability and high spatiotemporal resolution,and thereby enabling the non-destructive visualization of full-field structural information in three dimensions.Tremendous endeavors were devoted to the 3 rd generation SR over the past three decades,in which X-ray beams have been focused down to 100 nm.In this paper,recent progresses on SR-related characterization technologies were reviewed,with particular emphases on the fundamentals of synchrotron X-ray imaging and synchrotron X-ray diffraction,as well as their applications in the in situ observations of material preparation(e.g.,in situ dendrite growth during solidification)and service under extreme environment(e.g.,in situ mechanics).Future innovations toward next-generation SR and newly emerging SRbased technologies such as dark-field X-ray microscopy and Bragg coherent X-ray diffraction imaging were also advocated.
基金financially supported by the National Nature Science Foundation of China(No.51701112)the National Key Research and Development Program of China(No.2019YFA0705300)+2 种基金the Shanghai Rising-Star Program(Nos.20QA1403800 and 21QC1401500)the Shanghai Science and Technology Committee(No.19DZ1100704)the open fund of State Key Laboratory of Solidifi cation Processing in NWPU(Grant No.SKLSP202107)。
文摘Additive manufacturing(AM)is a rapid prototyping technology based on the idea of discrete accumulation which off ers an advantage of economically fabricating a component with complex geometries in a rapid design-to-manufacture cycle.However,various internal defects,such as balling,cracks,residual stress and porosity,are inevitably occurred during AM due to the complexity of laser/electron beam-powder interaction,rapid melting and solidification process,and microstructure evolution.The existence of porosity defects can potentially deteriorate the mechanical properties of selective laser melting(SLM)components,such as material stiff ness,hardness,tensile strength,and fatigue resistance performance.Synchrotron X-ray imaging and diffraction are important non-destructive means to elaborately characterize the internal defect characteristics and mechanical properties of AM parts.This paper presents a review on the application of synchrotron X-ray in identifying and verifying the quality and requirement of AM parts.Defects,microstructures and mechanical properties of printed components characterized by synchrotron X-ray imaging and diffraction are summarized in this review.Subsequently,this paper also elaborates on the online characterization of the evolution of the microstructure during AM using synchrotron X-ray imaging,and introduces the method for measuring AM stress by X-ray diffraction(XRD).Finally,the future application of synchrotron X-ray characterization in the AM is prospected.
基金supported by National Natural Science Foundation of China (Nos. 21805111 and 11405073)Taishan Scholar Fund
文摘Wet chemistry methods,including hot-injection and precipitation methods,have emerged as major synthetic routes for high-quality perovskite nanocrystals in backlit display and scintillation applications.However,low chemical yield hinders their upscale production for practical use.Meanwhile,the labile nature of halide-based perovskite poses a major challenge for long-term storage of perovskite nanocrystals.Herein,we report a green synthesis at room temperature for gram-scale production of CsPbBr3 nanosheets with minimum use of solvent,saving over 95% of the solvent for the unity mass nanocrystal production.The perovskite colloid exhibits record stability upon long-term storage for up to 8 months,preserving a photoluminescence quantum yield of 63% in solid state.Importantly,the colloidal nanosheets show self-assembly behavior upon slow solidification,generating a crack-free thin film in a large area.The uniform film was then demonstrated as an efficient scintillation screen for X-ray imaging.Our findings bring a scalable tool for synthesis of high-quality perovskite nanocrystals,which may inspire the industrial optoelectronic application of large-area perovskite film.
基金supported by the National Key Research and Development Program of China(Nos.2017YFA0403801,2017YFA0206004,2018YFC1200204)the National Natural Science Foundation of China(NSFC)(Nos.81430087,11775297,U1932205).
文摘Doped elements in alloys significantly impact their performance.Conventional methods usually sputter the surface material of the sample,or their performance is limited to the surface of alloys owing to their poor penetration ability.The X-ray K-edge subtraction(KES)method exhibits great potential for the nondestructive in situ detection of element contents in alloys.However,the signal of doped elements usually deteriorates because of the strong absorption of the principal component and scattering of crystal grains.This in turn prevents the extensive application of X-ray KES imaging to alloys.In this study,methods were developed to calibrate the linearity between the grayscale of the KES image and element content.The methods were aimed at the sensitive analysis of elements in alloys.Furthermore,experiments with phantoms and alloys demonstrated that,after elaborate calibration,X-ray KES imaging is capable of nondestructive and sensitive analysis of doped elements in alloys.
基金supported by the National Natural Science Foundation of China(NSFC)12333010the National Key R&D Program of China 2022YFF0503002+3 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(grant No.XDB0560000)the NSFC 11921003supported by the Prominent Postdoctoral Project of Jiangsu Province(2023ZB304)supported by the Strategic Priority Research Program on Space Science,the Chinese Academy of Sciences,grant No.XDA15320000.
文摘Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image quality of the reconstruction is still difficult,which is particularly useful for scheme design of X-ray imaging systems,testing and improvement of imaging algorithms,and scientific research of X-ray sources.Currently,there is no specified method to quantitatively evaluate the quality of X-ray image reconstruction and the point-spread function(PSF)of an X-ray imager.In this paper,we propose percentage proximity degree(PPD)by considering the imaging characteristics of X-ray image reconstruction and in particular,sidelobes and their effects on imaging quality.After testing a variety of imaging quality assessments in six aspects,we utilized the technique for order preference by similarity to ideal solution to the indices that meet the requirements.Then we develop the final quality index for X-ray image reconstruction,QuIX,which consists of the selected indices and the new PPD.QuIX performs well in a series of tests,including assessment of instrument PSF and simulation tests under different grid configurations,as well as imaging tests with RHESSI data.It is also a useful tool for testing of imaging algorithms,and determination of imaging parameters for both RHESSI and ASO-S/Hard X-ray Imager,such as field of view,beam width factor,and detector selection.
文摘A first and effective method is proposed to detect weld deject adaptively in various Dypes of real-time X-ray images obtained in different conditions. After weld extraction and noise reduction, a proper template of median filter is used to estimate the weld background. After the weld background is subtracted from the original image, an adaptite threshold segmentation algorithm is proposed to obtain the binary image, and then the morphological close and open operation, labeling algorithm and fids＇e alarm eliminating algorithm are applied to pracess the binary image to obtain the defect, ct detection result. At last, a fast realization procedure jbr proposed method is developed. The proposed method is tested in real-time X-ray image,s obtairted in different X-ray imaging sutems. Experiment results show that the proposed method is effective to detect low contrast weld dejects with few .false alarms and is adaptive to various types of real-time X-ray imaging systems.
基金supported by the National Natural Science Foundation of China(Nos.21971240 and 21827813)the National Key R&D Program of China(No.2017YFA0206802)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB20000000).
文摘X-ray detection and imaging via scintillators has been utilized in missions worldwide within areas of scientific research,medical industry,military defense and homeland security.Commercial scintillators are costly with high energy consumption through the sintering.It is of great significance to seek alternative scintillating materials for sensitive X-ray detection in the next-generation.Herein,eight structure-defined Ln(Ⅲ)-based metal-organic frameworks(Ln-MOFs)were prepared,2D[Ln_(2)(1,4-ndc)_(3)(DMF)_(4)]_(n)·nH_(2)O(Ln=Sm 1,Eu 2,Dy 3,Tb 4)and 3D[Ln_(4)(2,6-ndc)_(6)(μ_(2)H_(2)O)2(H_(2)O)_(4)]n·2nH_(2)O(Ln=Sm 5,Eu 6,Dy 7,Tb 8),where 1,4-H_(2)ndc=1,4-naphthalene dicarboxylate acid,2,6-H_(2)ndc=2,6-napthalene dicarboxylate acid,DMF=N,N-dimethylformamide.Merely compounds 2 and 6 show remarkable X-ray scintillation performance via the characteristic red emissions of Eu(Ⅲ)ions,in which the absorbed energy from the triplet states of the organic moieties can be transferred more efficiently to the resonance emission levels of Eu(Ⅲ)ions than other lanthanide(Ⅲ)ions.The X-ray dosage rate detection limits of 2 and 6 are superior to the standard for the medical X-ray diagnosis dosage rate.As proofs-of-concepts,matrix-mixed membranes fabricated with 2 and 6 have achieved remarkable X-ray imaging with high resolution for practical object shooting.
基金Project supported by the National Natural Science Foundation of China(62105333)the Key Research Program of the Chinese Academy of Sciences(ZDRW-CN-2021-3)+1 种基金Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China(2020ZZ114)the Xiamen Medical and Health Guidance Project,China(3502Z20209124)。
文摘In recent years,persistent luminescence materials(PLMs)excited by X-rays and emitting in biological windows have received extensive attention in the field of high-sensitivity bioimaging.Transition metal Mn^(2+)is an ideal emission center,but few studies focus on Mn^(2+)-doped PLMs with X-ray excitation and biological window emission.Here,we report a Mn^(2+)-doped PLM,LiYGeO_(4):Mn^(2+)(LYGM),with excellent biological window persistent luminescence emission.After excitation by UV,LYGM produces a durable biological window of persistent luminescence emission at 660 nm for up to 20 h.More importantly.LYGM can be repeatedly excited by X-rays,resulting in long-term biological window persistent luminescence emission.In addition,we obtain LYGM around 200 nm in diameter by ball milling and centrifugation and improve its biocompatibility by surface modification to apply it to in vivo imaging in mice.After LYGM are injected into mice through the tail vein,in situ excitation of X-rays can be achieved.After the persistent luminescence decays,LYGM can be re-excited for repeated imaging.Therefore,LYGM shows potential prospects for in vivo deep tissue and long-term bioimaging.
