Coherent motion of particles in a plasma can imprint itself on radiation.The recent advent of high-power lasers—allowing the nonlinear inverse Compton-scattering regime to be reached—has opened the possibility of lo...Coherent motion of particles in a plasma can imprint itself on radiation.The recent advent of high-power lasers—allowing the nonlinear inverse Compton-scattering regime to be reached—has opened the possibility of looking at collective effects in laser–plasma interactions.Under certain conditions,the collective interaction of many electrons with a laser pulse can generate coherent radiation in the hard x-ray regime.This perspective paper explains the limitations under which such a regime might be attained.展开更多
In most collisional schemes of x-ray laser (XRL) experiments, a bow-like intensity distribution of XRL is often observed, and it is generally ascribed to the two-dimensional hydrodynamic behaviour of expanding plasm...In most collisional schemes of x-ray laser (XRL) experiments, a bow-like intensity distribution of XRL is often observed, and it is generally ascribed to the two-dimensional hydrodynamic behaviour of expanding plasma. In order to better understand its essence in physics, a newly developed two-dimensional non-equilibrium radiation hydrodynamic code XRL2D is used to simulate a quasi-steady state Ni-like Ag XRL experiment on ShenGuang-Ⅱfacility. The simulation results show that the bow-like distribution of Ni-like ions caused by over-ionization in the central area of plasma is responsible for the bow-like shape of the XRL intensity distribution observed.展开更多
For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer (several nm ...For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer (several nm depth) of silver is plated on the surface of some other materials. Furthermore, the Ni-like Ag 13.9 nm x-ray laser produced by three new kinds of two-layer target with CH, Al and Ge as foundation, was theoretically studied.展开更多
Based on the two-dimensional model, this paper compares the hydrodynamics of slab x-ray laser plasma produced by different nonuniform line focused irradiations. It finds that the average intensity and the duration of ...Based on the two-dimensional model, this paper compares the hydrodynamics of slab x-ray laser plasma produced by different nonuniform line focused irradiations. It finds that the average intensity and the duration of laser pulse and the overall shape of the intensity distribution in the focal line have different influences on the plasma. Calculations show that the evolution of temperature variation is more sensitive to the pulse duration and the electron density variation is more sensitive to the pulse intensity. Pulses with duration of 200 ps to 500 ps and with intensity of 0.2 TW/cm2 to 1.0 TW/cm2 are proved acceptable in slab x-ray lasers.展开更多
We investigate the Ne-like Cr x-ray laser at 28.6 nm by using a modified ID lagrangian hydrodynamic code MEDI03 coupled with an atomic physics data package and a 2D ray tracing code as a post-processor. The laser pump...We investigate the Ne-like Cr x-ray laser at 28.6 nm by using a modified ID lagrangian hydrodynamic code MEDI03 coupled with an atomic physics data package and a 2D ray tracing code as a post-processor. The laser pumping configuration includes two prepulses and one main pulse. The first prepulse normally irradiates the target, while the second prepulse and the main pulse irradiate the target at grazing-incident angles. We predict that saturation can be achieved for the Ne-like Cr x-ray lasers with a total pumping energy of 125mJ, Good beam qualities with no deflecting angle and a small divergence angle of 5 mrad are observed.展开更多
A method of studying a non-equilibrium x-ray laser plasma is developed by extending the existing one-dimensional similarity equations to the case of two-dimensional plasma study in the directions perpendicular to the ...A method of studying a non-equilibrium x-ray laser plasma is developed by extending the existing one-dimensional similarity equations to the case of two-dimensional plasma study in the directions perpendicular to the slab and along a focal line. With this method the characteristics of pre-plasma are optimized for transient neon-like Cr x-ray laser. It is found that when the duration and the intensity of 1.053μm pre-pulse are 1.2 ns and 6.5 TW/cm^2 respectively with a delay time of 1.5 ns, the temperature and the temperature discrepancy each approach a proper state, which will provide a uniform distribution of properly ionized neon-like Cr ions before the arrival of pumping pulse.展开更多
Using an X-ray free electron laser(XFEL)at 960 eV to photo-ionize the 1s electron in neutral neon followed by lasing on the 2p-1s transition in singly-ionized neon,an inner-shell X-ray laser was demonstrated at 849 eV...Using an X-ray free electron laser(XFEL)at 960 eV to photo-ionize the 1s electron in neutral neon followed by lasing on the 2p-1s transition in singly-ionized neon,an inner-shell X-ray laser was demonstrated at 849 eV in singly-ionized neon gas several years ago.It took decades to demonstrate this scheme,because it required a very strong X-ray source that could photo-ionize the 1s(K shell)electron in neon on a timescale comparable to the intrinsic Auger lifetime in neon of 2 fs.In this paper,we model the neon inner shell X-ray laser under similar conditions to those used in the XFEL experiments at the SLAC Linac Coherent Light Source(LCLS),and show how we can improve the efficiency of the neon laser and reduce the drive requirements by tuning the XFEL to the 1s-3p transition in neutral neon in order to create gain on the 2p-1s line in neutral neon.We also show how the XFEL could be used to photo-ionize L-shell electrons to drive gain on n=3-2 transitions in singlyionized Ar and Cu plasmas.These bright,coherent,and monochromatic X-ray lasers may prove very useful for doing high-resolution spectroscopy and for studying non-linear process in the X-ray regime.展开更多
A simple modified model is presented based on R. A. London's self-similarity model on time-independent ionization hydrodynamics of exploding foil X-ray lasers. In our model, the time-dependent ionization effect is un...A simple modified model is presented based on R. A. London's self-similarity model on time-independent ionization hydrodynamics of exploding foil X-ray lasers. In our model, the time-dependent ionization effect is under consideration and the average ion charge depends on the temperature. Then we obtain the new scaling laws for temperature, scale length and electron density, which have better agreement with experimental results.展开更多
Gain coefficients are calculated for neon-like gallium and germanium ions. Shorter wavelengths are calculated and predicted to be emitted. The gain coefficients are calculated among 457 energy levels of the neon-like ...Gain coefficients are calculated for neon-like gallium and germanium ions. Shorter wavelengths are calculated and predicted to be emitted. The gain coefficients are calculated among 457 energy levels of the neon-like ions. Collisional excitations were calculated through the distorted wave approximations through five electron temperatures T<sub>e</sub> = 300, 500, 700, 1000 and 1500 eV.展开更多
AmpliHcation of spontaneous emissions at 19.6,23.2 and 23.6 nm have been observed by a “ultiple-Target Series Coupling”design in Ge plasma,.The combined length for four targets is up to 56mm.The gain length product(...AmpliHcation of spontaneous emissions at 19.6,23.2 and 23.6 nm have been observed by a “ultiple-Target Series Coupling”design in Ge plasma,.The combined length for four targets is up to 56mm.The gain length product(GL)of small signal is up to 18 for both lines at 23.2 and 23.6 nmt and the effective GL is 16.4 and 15.7 for these two lines respectively.This two lines are obviously tending to saturation.The divergence of x-ray laser beam is about 4 mrad.展开更多
An x-ray laser shadowgraphy experiment was conducted on Xingguang-Ⅱ laser facility in 1996.A multi-layer spherical mirror was used as an imaging element and a high sensitivity CCD camera as a detector.We measured the...An x-ray laser shadowgraphy experiment was conducted on Xingguang-Ⅱ laser facility in 1996.A multi-layer spherical mirror was used as an imaging element and a high sensitivity CCD camera as a detector.We measured the near-field image of the Ti x-ray laser beam.With a Ti x-ray laser beam as a backlight source,we obtained a clear CU mesh image,demonstrating the potential as advanced diagnostic measurements to study high density plasmas in inertial confinement fusion research.展开更多
Advances in X-ray laser sources have paved the way to relativistic attosecond X-ray laser pulses and opened up the possibility of exploring highenergy-density physics with this technology.With particle-in-cell simulat...Advances in X-ray laser sources have paved the way to relativistic attosecond X-ray laser pulses and opened up the possibility of exploring highenergy-density physics with this technology.With particle-in-cell simulations,we investigate the interaction of realistic metal crystals with relativistic X-ray laser pulses of parameters that will be available in the near future.A wakefield of the order of TV/cm is excited in the crystal and accelerates trapped electrons stably even though the wakefield is locally modulated by the crystal lattice.Electron injection either occurs at the sharp crystal-vacuum boundary or is controlled by coating the crystal with a high-density film.High-repetition-rate attosecond(20 as)monoenergetic electron beams of energy 125 MeV,charge 100 fC,and emittance 1.6310−9mrad can be produced by shining MHz X-ray laser pulses of energy 2.1 mJ onto coated crystals several micrometers thick.Such a miniature crystal accelerator,which has high reproducibility and allows sufficient control of the parameters of the electron beams,greatly expands the applications of X-ray free electron lasers.For example,it could serve as an ideal electron source for ultrafast electron diffraction and ultrafast electron microscopy to achieve attosecond resolution.展开更多
Corrigendum text:There is a misprint in the text of Figs.3 and 4.The text on the bottom part of Figs.3 and 4 should be“100 fs pulse Photoexcitation”and“1 fs pulse Photoexcitation”respectively.This error does not a...Corrigendum text:There is a misprint in the text of Figs.3 and 4.The text on the bottom part of Figs.3 and 4 should be“100 fs pulse Photoexcitation”and“1 fs pulse Photoexcitation”respectively.This error does not affect any conclusions in this work,and it has been corrected in the printed version of the journal.展开更多
A new type of soft X-ray source, i.e. a plasma-based X-ray laser, is found to be promising to conduct transient measurement. By means of picosecond X-ray laser speckles, the dynamic microscopic polarization clusters w...A new type of soft X-ray source, i.e. a plasma-based X-ray laser, is found to be promising to conduct transient measurement. By means of picosecond X-ray laser speckles, the dynamic microscopic polarization clusters within cubic (paraelectric) BaTiO3 was directly observed and characterized in a microscopic scale for the first time. This opens a way to study this type of clusters, which usually manifest large external-field response for ferroelectric materials.展开更多
The lattice parameter,measured with sufficient accuracy,can be utilized to evaluate the quality of single crystals and to determine the equation of state for materials.We propose an iterative method for obtaining more...The lattice parameter,measured with sufficient accuracy,can be utilized to evaluate the quality of single crystals and to determine the equation of state for materials.We propose an iterative method for obtaining more precise lattice parameters using the interaction points for the pseudo-Kossel pattern obtained from laser-induced X-ray diffraction(XRD).This method has been validated by the analysis of an XRD experiment conducted on iron single crystals.Furthermore,the method was used to calculate the compression ratio and rotated angle of an LiF sample under high pressure loading.This technique provides a robust tool for in-situ characterization of structural changes in single crystals under extreme conditions.It has significant implications for studying the equation of state and phase transitions.展开更多
Synchrotron method of resonant X-ray reflectivity 2D mapping has been applied to study ultrathin epitaxial layers of WS_(2)grown by pulsed laser deposition on Al_(2)O_(3)(0001)substrates.The measurements were carried ...Synchrotron method of resonant X-ray reflectivity 2D mapping has been applied to study ultrathin epitaxial layers of WS_(2)grown by pulsed laser deposition on Al_(2)O_(3)(0001)substrates.The measurements were carried out across the L absorption edge of tungsten to perform depth-dependent element-selective analysis sensitive to potential chemical modification of the WS_(2)layer in ambient conditions.Despite the few monolayer thickness of the studied film,the experimentally measured maps of reflectance as a function of incident angle and photon energy turned out to be quite informative showing well-pronounced interference effects near W absorption edge at 10210 eV.The synchrotron studies were complemented with conventional non-resonant reflectance measurements carried out in the laboratory at a fixed photon energy corresponding to Cu Kαemission.The reconstruction of the depth and energy dependent scattering length density within the studied multilayers was carried out using the OpenCL empowered fitting software utilizing spectral shaping algorithm which does not rely on the pre-measured reference absorption spectra.A thin WO_(x) layer has been revealed at the surface of the WS_(2)layer pointing out to the effect of water assisted photo-oxidation reported in a number of works related to ultrathin layers of transition metal dichalcogenides.展开更多
The first experiments on laser-driven cylindrical gold foam hohlraums have been performed at the 100 kJ SG-Ⅲ laser facility.Measurements of the expanding plasma emission show that there is less expanding plasma fill ...The first experiments on laser-driven cylindrical gold foam hohlraums have been performed at the 100 kJ SG-Ⅲ laser facility.Measurements of the expanding plasma emission show that there is less expanding plasma fill in foam hohlraums with a wall density of 0.8 g/cm^(3) than in solid gold hohlraums.The radiation temperatures at different angles confirm these results.Simulation results show that the expanding plasma density in the foam hohlraums is lower than in the solid hohlraums,resulting in less expanding plasma emission and higher radiation temperature.Thus,foam gold hohlraums have advantages in reducing wall plasma filling and improving X-ray transmission,which has potential applications in achieving a higher fusion yield.展开更多
X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast scien...X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast science.Recently,there has been a growing demand for X-ray pulses with high photon energy,especially from developments in“diffraction-before-destruction”applications and in dynamic mesoscale materials science.Here,we propose utilizing the electron beams at XFELs to drive a meter-scale two-bunch plasma wakefield accelerator and double the energy of the accelerated beam in a compact and inexpensive way.Particle-in-cell simulations are performed to study the beam quality degradation under different beam loading scenarios and nonideal issues,and the results show that more than half of the accelerated beam can meet the requirements of XFELs.After its transport to the undulator,the accelerated beam can improve the photon energy to 22 keV by a factor of around four while maintaining the peak power,thus offering a promising pathway toward high-photon-energy XFELs.展开更多
The microstructural factors contributing to the high strength of additive-manufactured Al-Si alloys us-ing laser-beam powder bed fusion(PBF-LB)were identified by in-situ synchrotron X-ray diffraction in tensile deform...The microstructural factors contributing to the high strength of additive-manufactured Al-Si alloys us-ing laser-beam powder bed fusion(PBF-LB)were identified by in-situ synchrotron X-ray diffraction in tensile deformation and transmission electron microscopy.PBF-LB and heat treatment were employed to manufacture Al-12%Si binary alloy specimens with different microstructures.At an early stage of de-formation prior to macroscopic yielding,stress was dominantly partitioned into the α-Al matrix,rather than the Si phase in all specimens.Highly concentrated Si solute(~3%)in the α-Al matrix promoted the dynamic precipitation of nanoscale Si phase during loading,thereby increasing the yield strength.After macroscopic yielding,the partitioned stress in the Si phase monotonically increased in the strain-hardening regime with an increase in the dislocation density in the α-Al matrix.At a later stage of strain hardening,the flow curves of the partitioned stress in the Si phase yielded stress relaxation owing to plastic deformation.Therefore,Si-phase particles localized along the cell walls in the cellular-solidified microstructure play a significant role in dislocation obstacles for strain hardening.Compared with the results of the heat-treated specimens with different microstructural factors,the dominant strengthening factors of PBF-LB manufactured Al-Si alloys were discussed.展开更多
Laser powder bed fusion(LPBF)is a potential additive manufacturing process to manufacture Invar 36 alloy components with complicated geometry.Whereas it inevitably introduces specific microstructures and pore defects,...Laser powder bed fusion(LPBF)is a potential additive manufacturing process to manufacture Invar 36 alloy components with complicated geometry.Whereas it inevitably introduces specific microstructures and pore defects,which will further influence the mechanical properties.Hence,aiming at exploring the LPBF process-related microstructures and pore defects,and especially their influences on the damage mechanism and mechanical properties,Invar 36 alloy was manufactured by LPBF under designed different laser scanning speeds.The microstructure observations reveal that higher scanning speeds lead to equiaxed and short columnar grains with higher dislocation density,while lower scanning speeds result in elongated columnar grains with lower dislocation density.The pore defects analyzed by X-ray computed tomography(XCT)suggest that the high laser scanning speed gives rise to numerous lamellar and large lack-of-fusion(LOF)pores,and the excessively low laser scanning speed produces relatively small keyhole pores with high sphericity.Moreover,the insitu XCT tensile tests were originally performed to evaluate the damage evolution and failure mechanism.Specifically,high laser scanning speed causes brittle fracture due to the rapid growth and coalescence of initial lamellar LOF pores along the scan-ning direction.Low laser scanning speed induces ductile fracture originating from unstable depressions in the surfaces,while metallurgical and keyhole pores have little impact on damage evolution.Eventually,the process-structure-property correlation is established.The presence of high volume fraction of lamel-lar LOF pores,resulting from high scanning speed,leads to inferior yield strength and ductility.Besides,specimens without LOF pores exhibit larger grain sizes and lower dislocation density at decreased scanning speeds,slightly reducing yield strength while slightly enhancing ductility.This understanding lays the foundation for widespread applications of LPBF-processed Invar 36 alloy.展开更多
基金supported by the Czech Academy of Sciences(Mobility Plus Project No.CNRS-23-12)A.M.F.was supported by the Russian Science Foundation(Grant No.20-12-00077).
文摘Coherent motion of particles in a plasma can imprint itself on radiation.The recent advent of high-power lasers—allowing the nonlinear inverse Compton-scattering regime to be reached—has opened the possibility of looking at collective effects in laser–plasma interactions.Under certain conditions,the collective interaction of many electrons with a laser pulse can generate coherent radiation in the hard x-ray regime.This perspective paper explains the limitations under which such a regime might be attained.
文摘In most collisional schemes of x-ray laser (XRL) experiments, a bow-like intensity distribution of XRL is often observed, and it is generally ascribed to the two-dimensional hydrodynamic behaviour of expanding plasma. In order to better understand its essence in physics, a newly developed two-dimensional non-equilibrium radiation hydrodynamic code XRL2D is used to simulate a quasi-steady state Ni-like Ag XRL experiment on ShenGuang-Ⅱfacility. The simulation results show that the bow-like distribution of Ni-like ions caused by over-ionization in the central area of plasma is responsible for the bow-like shape of the XRL intensity distribution observed.
文摘For experiments such as on Ni-like Ag x-ray laser, driven by 1ω laser, the gain region is only several nm depth near the target surface, this paper proposes a new two-layer target, in which a thin layer (several nm depth) of silver is plated on the surface of some other materials. Furthermore, the Ni-like Ag 13.9 nm x-ray laser produced by three new kinds of two-layer target with CH, Al and Ge as foundation, was theoretically studied.
基金suported by the National Natural Science Foundation of China (Grant No. 10874242)the National Basic Research Program of China (973 Program) (Grant No. 2007CB815105)Research Fund for the Doctoral Program of Higher Education of China (Grant No. 20070290008)
文摘Based on the two-dimensional model, this paper compares the hydrodynamics of slab x-ray laser plasma produced by different nonuniform line focused irradiations. It finds that the average intensity and the duration of laser pulse and the overall shape of the intensity distribution in the focal line have different influences on the plasma. Calculations show that the evolution of temperature variation is more sensitive to the pulse duration and the electron density variation is more sensitive to the pulse intensity. Pulses with duration of 200 ps to 500 ps and with intensity of 0.2 TW/cm2 to 1.0 TW/cm2 are proved acceptable in slab x-ray lasers.
基金supported by the National Natural Science Foundation of China ( Grant Nos 60678007,60621063 and 10774184)the State Key Development Program for Basic Research of China (Grant No 2007CB815101)
文摘We investigate the Ne-like Cr x-ray laser at 28.6 nm by using a modified ID lagrangian hydrodynamic code MEDI03 coupled with an atomic physics data package and a 2D ray tracing code as a post-processor. The laser pumping configuration includes two prepulses and one main pulse. The first prepulse normally irradiates the target, while the second prepulse and the main pulse irradiate the target at grazing-incident angles. We predict that saturation can be achieved for the Ne-like Cr x-ray lasers with a total pumping energy of 125mJ, Good beam qualities with no deflecting angle and a small divergence angle of 5 mrad are observed.
基金Project supported by the National Natural Science Foundation of China (Grant Nos 10474137,10874242 and 10775018)the National Basic Research Program of China (Grant No 2007CB815105)the Specialized Research Fund for the DoctoralProgram of Higher Education of China (Grant No 20070290008)
文摘A method of studying a non-equilibrium x-ray laser plasma is developed by extending the existing one-dimensional similarity equations to the case of two-dimensional plasma study in the directions perpendicular to the slab and along a focal line. With this method the characteristics of pre-plasma are optimized for transient neon-like Cr x-ray laser. It is found that when the duration and the intensity of 1.053μm pre-pulse are 1.2 ns and 6.5 TW/cm^2 respectively with a delay time of 1.5 ns, the temperature and the temperature discrepancy each approach a proper state, which will provide a uniform distribution of properly ionized neon-like Cr ions before the arrival of pumping pulse.
基金performed under the auspices of the U.S.Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344。
文摘Using an X-ray free electron laser(XFEL)at 960 eV to photo-ionize the 1s electron in neutral neon followed by lasing on the 2p-1s transition in singly-ionized neon,an inner-shell X-ray laser was demonstrated at 849 eV in singly-ionized neon gas several years ago.It took decades to demonstrate this scheme,because it required a very strong X-ray source that could photo-ionize the 1s(K shell)electron in neon on a timescale comparable to the intrinsic Auger lifetime in neon of 2 fs.In this paper,we model the neon inner shell X-ray laser under similar conditions to those used in the XFEL experiments at the SLAC Linac Coherent Light Source(LCLS),and show how we can improve the efficiency of the neon laser and reduce the drive requirements by tuning the XFEL to the 1s-3p transition in neutral neon in order to create gain on the 2p-1s line in neutral neon.We also show how the XFEL could be used to photo-ionize L-shell electrons to drive gain on n=3-2 transitions in singlyionized Ar and Cu plasmas.These bright,coherent,and monochromatic X-ray lasers may prove very useful for doing high-resolution spectroscopy and for studying non-linear process in the X-ray regime.
基金supported by National Natural Science Foundation of China(Nos.11574390,11374360,41472130)the National Basic Research Program of China(No.2013CBA01504)
文摘A simple modified model is presented based on R. A. London's self-similarity model on time-independent ionization hydrodynamics of exploding foil X-ray lasers. In our model, the time-dependent ionization effect is under consideration and the average ion charge depends on the temperature. Then we obtain the new scaling laws for temperature, scale length and electron density, which have better agreement with experimental results.
文摘Gain coefficients are calculated for neon-like gallium and germanium ions. Shorter wavelengths are calculated and predicted to be emitted. The gain coefficients are calculated among 457 energy levels of the neon-like ions. Collisional excitations were calculated through the distorted wave approximations through five electron temperatures T<sub>e</sub> = 300, 500, 700, 1000 and 1500 eV.
基金Supported by the Laser Domain of the Chinese National High Technology Plan。
文摘AmpliHcation of spontaneous emissions at 19.6,23.2 and 23.6 nm have been observed by a “ultiple-Target Series Coupling”design in Ge plasma,.The combined length for four targets is up to 56mm.The gain length product(GL)of small signal is up to 18 for both lines at 23.2 and 23.6 nmt and the effective GL is 16.4 and 15.7 for these two lines respectively.This two lines are obviously tending to saturation.The divergence of x-ray laser beam is about 4 mrad.
基金Supported by the National High Technique 863-410 Project.
文摘An x-ray laser shadowgraphy experiment was conducted on Xingguang-Ⅱ laser facility in 1996.A multi-layer spherical mirror was used as an imaging element and a high sensitivity CCD camera as a detector.We measured the near-field image of the Ti x-ray laser beam.With a Ti x-ray laser beam as a backlight source,we obtained a clear CU mesh image,demonstrating the potential as advanced diagnostic measurements to study high density plasmas in inertial confinement fusion research.
基金This work was supported by the Ministry of Science and Technology of the People’s Republic of China(Grant Nos.2018YFA0404803 and 2016YFA0401102)the National Science Foundation of China(Grant No.11935008).
文摘Advances in X-ray laser sources have paved the way to relativistic attosecond X-ray laser pulses and opened up the possibility of exploring highenergy-density physics with this technology.With particle-in-cell simulations,we investigate the interaction of realistic metal crystals with relativistic X-ray laser pulses of parameters that will be available in the near future.A wakefield of the order of TV/cm is excited in the crystal and accelerates trapped electrons stably even though the wakefield is locally modulated by the crystal lattice.Electron injection either occurs at the sharp crystal-vacuum boundary or is controlled by coating the crystal with a high-density film.High-repetition-rate attosecond(20 as)monoenergetic electron beams of energy 125 MeV,charge 100 fC,and emittance 1.6310−9mrad can be produced by shining MHz X-ray laser pulses of energy 2.1 mJ onto coated crystals several micrometers thick.Such a miniature crystal accelerator,which has high reproducibility and allows sufficient control of the parameters of the electron beams,greatly expands the applications of X-ray free electron lasers.For example,it could serve as an ideal electron source for ultrafast electron diffraction and ultrafast electron microscopy to achieve attosecond resolution.
文摘Corrigendum text:There is a misprint in the text of Figs.3 and 4.The text on the bottom part of Figs.3 and 4 should be“100 fs pulse Photoexcitation”and“1 fs pulse Photoexcitation”respectively.This error does not affect any conclusions in this work,and it has been corrected in the printed version of the journal.
文摘A new type of soft X-ray source, i.e. a plasma-based X-ray laser, is found to be promising to conduct transient measurement. By means of picosecond X-ray laser speckles, the dynamic microscopic polarization clusters within cubic (paraelectric) BaTiO3 was directly observed and characterized in a microscopic scale for the first time. This opens a way to study this type of clusters, which usually manifest large external-field response for ferroelectric materials.
基金National Natural Science Foundation of China(12102410)Fund of National Key Laboratory of Shock Wave and Detonation Physics(JCKYS2022212005)。
文摘The lattice parameter,measured with sufficient accuracy,can be utilized to evaluate the quality of single crystals and to determine the equation of state for materials.We propose an iterative method for obtaining more precise lattice parameters using the interaction points for the pseudo-Kossel pattern obtained from laser-induced X-ray diffraction(XRD).This method has been validated by the analysis of an XRD experiment conducted on iron single crystals.Furthermore,the method was used to calculate the compression ratio and rotated angle of an LiF sample under high pressure loading.This technique provides a robust tool for in-situ characterization of structural changes in single crystals under extreme conditions.It has significant implications for studying the equation of state and phase transitions.
基金supported by the Ministry of Science and Higher Education of the Russian Federation(agreement No.075-15-2021-1349)。
文摘Synchrotron method of resonant X-ray reflectivity 2D mapping has been applied to study ultrathin epitaxial layers of WS_(2)grown by pulsed laser deposition on Al_(2)O_(3)(0001)substrates.The measurements were carried out across the L absorption edge of tungsten to perform depth-dependent element-selective analysis sensitive to potential chemical modification of the WS_(2)layer in ambient conditions.Despite the few monolayer thickness of the studied film,the experimentally measured maps of reflectance as a function of incident angle and photon energy turned out to be quite informative showing well-pronounced interference effects near W absorption edge at 10210 eV.The synchrotron studies were complemented with conventional non-resonant reflectance measurements carried out in the laboratory at a fixed photon energy corresponding to Cu Kαemission.The reconstruction of the depth and energy dependent scattering length density within the studied multilayers was carried out using the OpenCL empowered fitting software utilizing spectral shaping algorithm which does not rely on the pre-measured reference absorption spectra.A thin WO_(x) layer has been revealed at the surface of the WS_(2)layer pointing out to the effect of water assisted photo-oxidation reported in a number of works related to ultrathin layers of transition metal dichalcogenides.
基金support from the National Natural Science Foundation of China(Grant Nos.11775204 and 12105269)the Presidential Foundation of the China Academy of Engineering Physics(Grant No.YZJJLX2018011)。
文摘The first experiments on laser-driven cylindrical gold foam hohlraums have been performed at the 100 kJ SG-Ⅲ laser facility.Measurements of the expanding plasma emission show that there is less expanding plasma fill in foam hohlraums with a wall density of 0.8 g/cm^(3) than in solid gold hohlraums.The radiation temperatures at different angles confirm these results.Simulation results show that the expanding plasma density in the foam hohlraums is lower than in the solid hohlraums,resulting in less expanding plasma emission and higher radiation temperature.Thus,foam gold hohlraums have advantages in reducing wall plasma filling and improving X-ray transmission,which has potential applications in achieving a higher fusion yield.
基金supported by the National Grand Instrument Project No. SQ2019YFF01014400the Natural Science Foundation of China (Grant Nos. 12375147, 12435011, 12075030)+2 种基金the Beijing Outstanding Young Scientist Project, Project for Young Scientists in Basic Research of Chinese Academy of Sciences (YSBR-115)the Beijing Normal University Scientific Research Initiation Fund for Introducing Talents No. 310432104the Fundamental Research Funds for the Central Universities, Peking University
文摘X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast science.Recently,there has been a growing demand for X-ray pulses with high photon energy,especially from developments in“diffraction-before-destruction”applications and in dynamic mesoscale materials science.Here,we propose utilizing the electron beams at XFELs to drive a meter-scale two-bunch plasma wakefield accelerator and double the energy of the accelerated beam in a compact and inexpensive way.Particle-in-cell simulations are performed to study the beam quality degradation under different beam loading scenarios and nonideal issues,and the results show that more than half of the accelerated beam can meet the requirements of XFELs.After its transport to the undulator,the accelerated beam can improve the photon energy to 22 keV by a factor of around four while maintaining the peak power,thus offering a promising pathway toward high-photon-energy XFELs.
基金JST PRESTO(grant number JPMJPR22Q4)(Japan)The Light Metal Educational Foundation,Inc.(Japan),and“Knowledge Hub Aichi”Aichi Prefectural Government(Japan)The synchrotron radiation experiments were performed at BL46XUof SPring-8with the approval of the Japan Synchrotron Radiation Research Institute(JASRI)(Proposal No.2021A1663,2022A1001and 2022A1798).
文摘The microstructural factors contributing to the high strength of additive-manufactured Al-Si alloys us-ing laser-beam powder bed fusion(PBF-LB)were identified by in-situ synchrotron X-ray diffraction in tensile deformation and transmission electron microscopy.PBF-LB and heat treatment were employed to manufacture Al-12%Si binary alloy specimens with different microstructures.At an early stage of de-formation prior to macroscopic yielding,stress was dominantly partitioned into the α-Al matrix,rather than the Si phase in all specimens.Highly concentrated Si solute(~3%)in the α-Al matrix promoted the dynamic precipitation of nanoscale Si phase during loading,thereby increasing the yield strength.After macroscopic yielding,the partitioned stress in the Si phase monotonically increased in the strain-hardening regime with an increase in the dislocation density in the α-Al matrix.At a later stage of strain hardening,the flow curves of the partitioned stress in the Si phase yielded stress relaxation owing to plastic deformation.Therefore,Si-phase particles localized along the cell walls in the cellular-solidified microstructure play a significant role in dislocation obstacles for strain hardening.Compared with the results of the heat-treated specimens with different microstructural factors,the dominant strengthening factors of PBF-LB manufactured Al-Si alloys were discussed.
基金support of the National Natural Science Foundation of China(Grant Nos.12372133 and 12027901)supported by the Natural Science Foun-dation of Hunan Province(Grant No.2021JJ30085)+2 种基金the Science and Technology Innovation Program of Hunan Province(Grant No.2021RC30306)Open Research Fund of State Key Laboratory of Precision Manufacturing for Extreme Service Performance,Central South University(Grant No.Kfkt2021-01)the Fund of State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body(Grant No.52175012).
文摘Laser powder bed fusion(LPBF)is a potential additive manufacturing process to manufacture Invar 36 alloy components with complicated geometry.Whereas it inevitably introduces specific microstructures and pore defects,which will further influence the mechanical properties.Hence,aiming at exploring the LPBF process-related microstructures and pore defects,and especially their influences on the damage mechanism and mechanical properties,Invar 36 alloy was manufactured by LPBF under designed different laser scanning speeds.The microstructure observations reveal that higher scanning speeds lead to equiaxed and short columnar grains with higher dislocation density,while lower scanning speeds result in elongated columnar grains with lower dislocation density.The pore defects analyzed by X-ray computed tomography(XCT)suggest that the high laser scanning speed gives rise to numerous lamellar and large lack-of-fusion(LOF)pores,and the excessively low laser scanning speed produces relatively small keyhole pores with high sphericity.Moreover,the insitu XCT tensile tests were originally performed to evaluate the damage evolution and failure mechanism.Specifically,high laser scanning speed causes brittle fracture due to the rapid growth and coalescence of initial lamellar LOF pores along the scan-ning direction.Low laser scanning speed induces ductile fracture originating from unstable depressions in the surfaces,while metallurgical and keyhole pores have little impact on damage evolution.Eventually,the process-structure-property correlation is established.The presence of high volume fraction of lamel-lar LOF pores,resulting from high scanning speed,leads to inferior yield strength and ductility.Besides,specimens without LOF pores exhibit larger grain sizes and lower dislocation density at decreased scanning speeds,slightly reducing yield strength while slightly enhancing ductility.This understanding lays the foundation for widespread applications of LPBF-processed Invar 36 alloy.