Formamidinium lead iodide(FAPbI_(3))perovskite exhibits an impressive X-ray absorption coefficient and a large carrier mobility-lifetime product(μτ),making it as a highly promising candidate for X-ray detection appl...Formamidinium lead iodide(FAPbI_(3))perovskite exhibits an impressive X-ray absorption coefficient and a large carrier mobility-lifetime product(μτ),making it as a highly promising candidate for X-ray detection application.However,the presence of larger FA^(+)cation induces to an expansion of the Pb-I octahedral framework,which unfortunately affects both the stability and charge carrier mobility of the corresponding devices.To address this challenge,we develop a novel low-dimensional(HtrzT)PbI_(3) perovskite featuring a conjugated organic cation(1H-1,2,4-Triazole-3-thiol,HtrzT^(+))which matches well with theα-FAPbI_(3) lattices in two-dimensional plane.Benefiting from the matched lattice between(HtrzT)PbI_(3) andα-FAPbI_(3),the anchored lattice enhances the Pb-I bond strength and effectively mitigates the inherent tensile strain of theα-FAPbI_(3) crystal lattice.The X-ray detector based on(HtrzT)PbI_(3)(1.0)/FAPbI_(3) device achieves a remarkable sensitivity up to 1.83×10^(5)μC Gy_(air)^(−1) cm^(−2),along with a low detection limit of 27.6 nGy_(air) s^(−1),attributed to the release of residual stress,and the enhancement in carrier mobility-lifetime product.Furthermore,the detector exhibits outstanding stability under X-ray irradiation with tolerating doses equivalent to nearly 1.17×10^(6) chest imaging doses.展开更多
Soft X-ray detectors play a vital role in materials science,high-energy physics and medical imaging.Cs_(2)AgBiBr_(6),a lead-free double perovskite,has gained attention for its excellent optoelectronic properties,stabi...Soft X-ray detectors play a vital role in materials science,high-energy physics and medical imaging.Cs_(2)AgBiBr_(6),a lead-free double perovskite,has gained attention for its excellent optoelectronic properties,stability,and nontoxicity.However,its fast crystallization and requirement for high-temperature annealing(>250℃)often lead to inferior film quality,limiting its application in flexible devices.This study introduces an alloying strategy that significantly improves the quality of Cs_(2)AgBiBr_(6)thin films annealed at a reduced temperature of 150℃.Devices based on the alloyed thin films exhibit an ultra-low dark current of 0.32 nA·cm^(-2)and a quantum efficiency of 725%.Furthermore,the first successful integration of Cs_(2)AgBiBr_(6)with a thinfilm transistor backplane demonstrates its superior imaging performance,indicating that Cs_(2)AgBiBr_(6)is a promising material for next-generation soft X-ray sensors.展开更多
A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-d...A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-dimensional cusp boundary from a two-dimensional X-ray image because the detected X-ray signals will be integrated along the line of sight.In this work,a global magnetohydrodynamic code was used to simulate the X-ray images and photon count images,assuming an interplanetary magnetic field with a pure Bz component.The assumption of an elliptic cusp boundary at a given altitude was used to trace the equatorward and poleward boundaries of the cusp from a simulated X-ray image.The average discrepancy was less than 0.1 RE.To reduce the influence of instrument effects and cosmic X-ray backgrounds,image denoising was considered before applying the method above to SXI photon count images.The cusp boundaries were reasonably reconstructed from the noisy X-ray image.展开更多
This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the...This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the past 5 years.The photon energy range of the beamline is 8–72.5 keV.Several sets of X-ray imaging detectors with different pixel sizes(0.19–24 lm)are used to realize X-ray microcomputed tomography(X-ray micro-CT)and X-ray in-line phase-contrast imaging.To satisfy the requirements of user experiments,new X-ray imaging methods and image processing techniques are developed.In vivo dynamic micro-CT experiments with living insects are performed in 0.5 s(sampling rate of 2 Hz,2 tomograms/s)with a monochromatic beam from a wiggler source and in 40 ms(sampling rate of 25 Hz,25 tomograms/s)with a white beam from a bending magnet source.A new X-ray imaging method known as move contrast X-ray imaging is proposed,with which blood flow and moving tissues in raw images can be distinguished according to their moving frequencies in the time domain.Furthermore,X-ray speckle-tracking imaging with twice exposures to eliminate the edge enhancement effect is developed.A high-precision quantification method is realized to measure complex three-dimensional blood vessels obtained via X-ray micro-CT.X-ray imaging methods such as three-dimensional X-ray diffraction microscopy,small-angle X-ray scattering CT,and X-ray fluorescence CT are developed,in which the X-ray micro-CT imaging method is combined with other contrast mechanisms such as diffraction,scattering,and fluorescence contrasts respectively.Moreover,an X-ray nano-CT experiment is performed with a 100 nm spatial resolution.Typical user experimental results from the fields of material science,biomedicine,paleontology,physics,chemistry,and environmental science obtained on the beamline are provided.展开更多
In the exploration of celestial bodies,such as Mars,the Moon,and asteroids,X-ray fluorescence analysis has emerged as a critical tool for elemental analysis.However,the varying selection rules and excitation sources i...In the exploration of celestial bodies,such as Mars,the Moon,and asteroids,X-ray fluorescence analysis has emerged as a critical tool for elemental analysis.However,the varying selection rules and excitation sources introduce complexity.Specifically,these discrepancies can cause variations in the intensities of the characteristic spectral lines emitted by identical elements.These variations,compounded by the minimal energy spacing between these spectral lines,pose substantial challenges for conventional silicon drift detectors(SDD),hindering their ability to accurately differentiate these lines and provide detailed insights into the material structure.To overcome this challenge,a cryogenic X-ray spectrometer based on transition-edge sensor(TES)detector arrays is required to achieve precise measurements.This study measured and analyzed the K-edge characteristic lines of copper and the diverse L-edge characteristic lines of tungsten using a comparative analysis of the electron and X-ray excitation processes.For the electron excitation experiments,copper and tungsten targets were employed as X-ray sources,as they emit distinctive X-ray spectra upon electron-beam bombardment.In the photon excitation experiments,a molybdenum target was used to produce a continuous spectrum with the prominent Mo Kαlines to emit pure copper and tungsten samples.TES detectors were used for the comparative spectroscopic analysis.The initial comparison revealed no substantial differences in the Kαand Kβlines of copper across different excitation sources.Similarly,the Lαlines of tungsten exhibited uniformity under different excitation sources.However,this investigation revealed pronounced differences within the Lβline series.The study found that XRF spectra preferentially excite outer-shell electrons,in contrast to intrinsic spectra,owing to different photon and electron interaction mechanisms.Photon interactions are selection-ruledependent and involve a single electron,whereas electron interactions can involve multiple electrons without such limitations.This leads to varied excitation transitions,as evidenced in the observed Lβline series.展开更多
Nano-scale chemical inhomogeneity in surface oxide films formed on a V-and N-containing martensite stainless steel and tempering heating induced changes are investigated by a combination of synchrotron-based hard X-ra...Nano-scale chemical inhomogeneity in surface oxide films formed on a V-and N-containing martensite stainless steel and tempering heating induced changes are investigated by a combination of synchrotron-based hard X-ray Photoelectron emission spectroscopy(HAXPES)and microscopy(HAXPEEM)as well as microscopic X-ray absorption spectroscopy(μ-XAS)techniques.The results reveal the inhomogeneity in the oxide films on the micron-sized Cr_(2)N-and VN-type particles,while the inhomogeneity on the martensite matrix phase exists due to localised formation of nano-sized tempering nitride particles at 600℃.The oxide film formed on Cr_(2)N-type particles is rich in Cr_(2)O_(3) compared with that on the martensite matrix and VN-type particles.With the increase of tempering temperature,Cr_(2)O_(3) formation is faster for the oxidation of Cr in the martensite matrix than the oxidation of Cr nitride-rich particles.展开更多
Operando X-ray diffraction(XRD)is an important characterization tool for real-time monitoring of structural changes in materials under different reaction conditions.In this study,we developed a laboratory-based diffra...Operando X-ray diffraction(XRD)is an important characterization tool for real-time monitoring of structural changes in materials under different reaction conditions.In this study,we developed a laboratory-based diffractometer that could capture a full XRD spectrum within 10 s.The instrument has several advanced features.First,it uses a Ga–In alloy metal-jet X-ray source,thereby achieving high X-ray flux with a brightness of up to 3.0×10^(10) photons/(s·mm^(2)·mrad2).Second,it employs an ellipsoidal mirror with a multilayer coating to produce quasi-parallel monochromatic light characterized by a divergence of 0.6 mrad and an energy resolution of 5.9×10^(−3).Third,it is equipped with a high-efficiency,high-signal-to-noise-ratio Pilatus 3R 1M detector for collecting diffraction signals.These features make the developed instrument applicable in studying rapid phase transitions in lithium-ion batteries,especially under extremely fast charge–discharge conditions.The data quality was comparable to that of synchrotron radiation XRD.展开更多
This study describes the design and performance of a laboratory-based tender X-ray spectrometer for X-ray absorption spectroscopy.The system enables effective absorption spectra to be measured within the 2.0-9.0 keV r...This study describes the design and performance of a laboratory-based tender X-ray spectrometer for X-ray absorption spectroscopy.The system enables effective absorption spectra to be measured within the 2.0-9.0 keV range using Rowland circle geometry;it covers the K edge of 3d transition metals,the L edge of lanthanides,and the M edge of actinides.The spectrometer is configured with a Rowland circle with a diameter of 500 mm and integrates a 250 W liquid metal jet X-ray source,spherical bent crystal analyzer,and energy-resolving silicon drift detector.The X-ray source is installed outside the vacuum chamber and remains fixed,while the analyzer crystals and detector are adjusted to change the Bragg angle,maintaining the Rowland condition.The energy resolution is 0.36-1.30 eV at 2.0-9.0 keV,and the monochromatic flux is approximately 5×10^(5) counts/s at 7040 eV.This study highlights the primary characteristics of the spectrometer and demon-strates its capabilities using selected experimental examples.The successful development of this spectrometer can facilitate research on actinide elements,which are often constrained in synchrotron radiation experiments owing to their radioactivity,thus fostering advancements in related nuclear energy fields.展开更多
This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):B...This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):Bi,Eu phosphors were synthesized,with Bi enhancing X-ray-induced photochromic prop-erties.Under X-ray irradiation,the phosphors transfer from white to red in bright field conditions and emit red photoluminescence in dark field conditions.Exposure to 470 nm ultraviolet light induces rapid bleaching.The mechanisms of photochromism and photoluminescence,particularly Bi's role as a colorant,were systematically investigated.The Ba_(2)LaNbO_(6):Bi,Eu phosphors film achieves high resolution,high-lighting its potential for X-ray imaging and non-destructive testing.Furthermore,the flexible Ba_(2)LaNbO_(6):Bi,Eu film supports dual-mode imaging and detection,addressing the limitations of traditional flat dis-plays in 3D imaging.展开更多
A double-parabola monocapillary(DPM)was designed for laboratory x-ray sources,and its performance was evaluated through numerical simulations and experimental validation.A surface shape error model was developed to ch...A double-parabola monocapillary(DPM)was designed for laboratory x-ray sources,and its performance was evaluated through numerical simulations and experimental validation.A surface shape error model was developed to characterize the DPM surface profile,and ray-tracing methods were used to simulate key properties such as focal spot size,divergence,and transmission efficiency.The simulation results closely matched experimental measurements,validating the proposed model.This surface shape error simulation provides an efficient method for evaluating the impact of slope errors on DPM performance,offering insights for optimal design and precision manufacturing.展开更多
The increased use of rechargeable batteries in portable electronic devices and the continuous develop-ment of novel applications （e.g. transportation and large scale energy storage）, have raised a strong de-mand for...The increased use of rechargeable batteries in portable electronic devices and the continuous develop-ment of novel applications （e.g. transportation and large scale energy storage）, have raised a strong de-mand for high performance batteries with increased energy density, cycle and calendar life, safety andlower costs. This triggers significant efforts to reveal the fundamental mechanism determining batteryperformance with the use of advanced analytical techniques. However, the inherently complex character-istics of battery systems make the mechanism analysis sophisticated and difficult. Synchrotron radiationis an advanced collimated light source with high intensity and tunable energies. It has particular ad-vantages in electronic structure and geometric structure （both the short-range and long-range structure）analysis of materials on different length and time scales. In the past decades, synchrotron X-ray tech-niques have been widely used to understand the fundamental mechanism and guide the technologicaloptimization of batteries. In particular, in situ and operando techniques with high spatial and temporalresolution, enable the nondestructive, real time dynamic investigation of the electrochemical reaction,and lead to significant deep insights into the battery operation mechanism. This review gives a brief introduction of the application of synchrotron X-ray techniques to the inves-tigation of battery systems. The five widely implicated techniques, including X-ray diffraction （XRD）, PairDistribution Function （PDF）, Hard and Soft X-ray absorption spectroscopy （XAS） and X-ray photoelectronspectroscopy （XPS） will be reviewed, with the emphasis on their in situ studies of battery systems during cycling.展开更多
[目的/意义]苹果“冰糖心”又称水心病,是一种常见的果实病害,严重的水心病果会随着储藏时间的增加发生霉变,造成食品安全隐患。为实现不同等级水心病苹果快速无损检测,本研究旨在构建有效的分级与可溶性固形物(Soluble Solids Content,...[目的/意义]苹果“冰糖心”又称水心病,是一种常见的果实病害,严重的水心病果会随着储藏时间的增加发生霉变,造成食品安全隐患。为实现不同等级水心病苹果快速无损检测,本研究旨在构建有效的分级与可溶性固形物(Soluble Solids Content,SSC)预测模型。[方法]本研究选取了230个富士苹果,其中正常、轻度、中度、重度水心苹果数量分别为113、61、47和9个,分别采集了400~1000 nm范围的反射光谱和X射线计算机断层成像(X-ray Computed Tomography,X-ray CT)数据,并测定了SSC含量。[结果和讨论]SSC随水心程度加剧呈上升趋势,重度水心苹果呈现更高的光谱反射率,X-ray CT扫描成像观察到水心区域的组织体积平均密度高于健康组织,基于三维重建算法实现不同等级水心苹果内部水心组织可视化分布。基于偏最小二乘判别分析(Partial Least Squares Discriminant Analysis,PLSDA)构建的不同水心程度苹果果实分级模型建模集和测试集准确率分别为98.7%和95.9%;构建不同水心程度苹果果实SSC回归模型,校正集决定系数(Correlation Coefficient of Calibration,R_(C)^(2))为0.962,均方根误差(Root Mean Squares Error of Calibration,RMSEC)为0.264,测试集决定系数(Correlation Coefficient of Prediction,R_(P)^(2))为0.879,均方根误差(Root Mean Squares Error of Prediction,RMSEP)为0.435。[结论]该研究构建的不同水心程度苹果果实分级模型能够实现苹果不同等级水心病的预测,构建的不同水心程度苹果果实SSC回归模型能够较好地预测苹果果实的SSC,为苹果水心病无损检测和品质评估提供了有效方法。展开更多
Using the new soft X-ray data from the Macao Science Satellite-1,we studied a solar flare that occurred on 22 June 2023.We found that the centroids of the Ca(around 3.9 keV)and Fe(around 6.7 keV)line features exhibit ...Using the new soft X-ray data from the Macao Science Satellite-1,we studied a solar flare that occurred on 22 June 2023.We found that the centroids of the Ca(around 3.9 keV)and Fe(around 6.7 keV)line features exhibit a rapid shift toward higher energy channels during the flare's rising phase,followed by a gradual decrease during the decay phase.Through precise energy calibration,the centroids are determined with high accuracy.Temperature and velocity are then self-consistently derived by comparing the centroids with those calculated from the synthesized line features using the latest CHIANTI atomic database(ver.10.1).The calculated maximum velocity reaches up to 710±60 km s-1,which significantly exceeds the previously reported values.Our results suggest that the entire shift of soft X-ray lines may occur during the process of chromospheric evaporation.展开更多
BACKGROUND In pediatric age group patients(<18 years old)treated operatively for distal radius/both bone fractures extending imaging beyond the initial postoperative period-particularly in uncomplicated cases-appea...BACKGROUND In pediatric age group patients(<18 years old)treated operatively for distal radius/both bone fractures extending imaging beyond the initial postoperative period-particularly in uncomplicated cases-appears to provide limited additional benefit.AIM To determine the necessary number of follow-up X-rays to use resources efficiently.METHODS Participants included in this study are pediatric age group patients who were treated operatively for distal radius/both bone fractures and were identified from a prospected collected data from the operating room database between the years 2009 and 2017.The data in the study included patients who had distal radius fractures and underwent fixation surgery(n=88).RESULTS When assessing the difference in the odds of conducting 1 or less X-ray compared to 2 or more X-rays in regard to the type of fixation,the only significant difference is the closed reduction fixation method.Patients who underwent closed reduction method procedure have significantly lower odds of having 2 more X-rays compared to those who didn’t have closed reduction method.Open reduction,internal fixation,and other fixation methods(close reduction and internal fixation,debridement,or epiphysiodesis)have higher odds of having two or more X-rays compared to patients who did not receive these methods;however,these odds are not statistically significant.CONCLUSION The findings of this study reveal notable absence of a statistically significant association between the frequency of postoperative X-rays and the outcome of children with distal radius fractures.展开更多
The main scientific payload of Macao Science Satellite-1B is a solar soft X-ray detection unit.To obtain an accurate solar X-ray spectrum,we have designed low-noise,high-throughput electronics.Solar radiation is detec...The main scientific payload of Macao Science Satellite-1B is a solar soft X-ray detection unit.To obtain an accurate solar X-ray spectrum,we have designed low-noise,high-throughput electronics.Solar radiation is detected using a low-leakage silicon drift detector(SDD),which is cooled to-30℃.The SDD output is processed using two parallel shaping amplifiers with peaking times of 315 ns and 65 ns.The amplifiers are designed using two-pole multiple-feedback active low-pass filters optimized to achieve a Bessel response.The differential output of the shaping amplifier generates a bipolar signal.The phase of the differential stage is tuned to ensure zero crossing corresponding to the peak of the shaping amplifier.A high-speed switch is inserted between the shaping amplifier and the peak-hold capacitor,and the peak value is maintained by turning off the switch.Fast and slow peak-hold circuits share a common ADC via time-division multiplexing.Both peak values are sampled for space-background rejection.Traditional pile-up detection methods cannot distinguish pulses that overlap in a fast channel.In this study,the differential of the“fast shaping”is selected,enabling the distinction of events separated by as little as 65ns,which is crucial for solar flare detection.The energy resolution is measured to be 138 eV at 5.90 keV.The centroid drift is less than 3.6 eV between-5℃ and 20℃.Compared with other solar X-ray instruments,this study demonstrates improved energy resolution with a lower peaking time,indicating a higher solar flare detection capability.展开更多
X-ray detectors show potential applications in medical imaging,materials science,and nuclear energy.To achieve high detection efficiency and spatial resolution,many conventional semiconductor materials,such as amorpho...X-ray detectors show potential applications in medical imaging,materials science,and nuclear energy.To achieve high detection efficiency and spatial resolution,many conventional semiconductor materials,such as amorphous selenium,cadmium telluride zinc,and perovskites,have been utilized in direct conversion X-ray detectors.However,these semiconductor materials are susceptible to temperature-induced performance degradation,crystallization,delamination,uneven lattice growth,radiation damage,and high dark current.This study explores a new approach by coupling an FC40 electronic fluorinated liquid with a specialized high-resolution and high-readout-speed complementary metal-oxide-semiconductor(CMOS)pixel array,specifically the Topmetal II−chip,to fabricate a direct conversion X-ray detector.The fluorinated liquid FC40(molecular formula:C_(21)F_(48)N_(2))is an electronic medium that is minimally affected by temperature and displays no issues with uniform conductivity.It exhibits a low dark current and minimal radiation damage and enables customizable thickness in X-ray absorption.This addresses the limitations inherent in conventional semiconductor-based detectors.In this study,simple X-ray detector imaging tests were conducted,demonstrating the excellent coupling capability between FC40 electronic fluorinated liquid and CMOS chips by the X-ray detector.A spatial resolution of 4.0 lp/mm was measured using a striped line par card,and a relatively clear image of a cockroach was displayed in the digital radiography imaging results.Preliminary test results indicated the feasibility of fabricating an X-ray detector by combining FC40 electronic fluorinated liquid and CMOS chips.Owing to the absence of issues related to chip-material coupling,a high spatial resolution could be achieved by reducing the chip pixel size.This method presents a new avenue for studies on novel liquid-based direct conversion X-ray detectors.展开更多
Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image qual...Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image quality of the reconstruction is still difficult,which is particularly useful for scheme design of X-ray imaging systems,testing and improvement of imaging algorithms,and scientific research of X-ray sources.Currently,there is no specified method to quantitatively evaluate the quality of X-ray image reconstruction and the point-spread function(PSF)of an X-ray imager.In this paper,we propose percentage proximity degree(PPD)by considering the imaging characteristics of X-ray image reconstruction and in particular,sidelobes and their effects on imaging quality.After testing a variety of imaging quality assessments in six aspects,we utilized the technique for order preference by similarity to ideal solution to the indices that meet the requirements.Then we develop the final quality index for X-ray image reconstruction,QuIX,which consists of the selected indices and the new PPD.QuIX performs well in a series of tests,including assessment of instrument PSF and simulation tests under different grid configurations,as well as imaging tests with RHESSI data.It is also a useful tool for testing of imaging algorithms,and determination of imaging parameters for both RHESSI and ASO-S/Hard X-ray Imager,such as field of view,beam width factor,and detector selection.展开更多
Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method...Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method,an indirect imaging technique that requires algorithms to reconstruct and optimize images.During the last decade,a variety of algorithms have been developed and improved.However,it is difficult to quantitatively evaluate the image quality of different solutions without a true,reference image of observation.How to choose the values of imaging parameters for these algorithms to get the best performance is also an open question.In this study,we present a detailed test of the characteristics of these algorithms,imaging dynamic range and a crucial parameter for the CLEAN method,clean beam width factor(CBWF).We first used SDO/AIA EUV images to compute DEM maps and calculate thermal X-ray maps.Then these realistic sources and several types of simulated sources are used as the ground truth in the imaging simulations for both RHESSI and ASO-S/HXI.The different solutions are evaluated quantitatively by a number of means.The overall results suggest that EM,PIXON,and CLEAN are exceptional methods for sidelobe elimination,producing images with clear source details.Although MEM_GE,MEM_NJIT,VIS_WV and VIS_CS possess fast imaging processes and generate good images,they too possess associated imperfections unique to each method.The two forward fit algorithms,VF and FF,perform differently,and VF appears to be more robust and useful.We also demonstrated the imaging capability of HXI and available HXI algorithms.Furthermore,the effect of CBWF on image quality was investigated,and the optimal settings for both RHESSI and HXI were proposed.展开更多
During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a rest...During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.展开更多
The paper presents experimental investigation results of crack pattern change in cement pastes caused by external sulfate attack(ESA).To visualize the formation and development of cracks in cement pastes under ESA,an ...The paper presents experimental investigation results of crack pattern change in cement pastes caused by external sulfate attack(ESA).To visualize the formation and development of cracks in cement pastes under ESA,an X-ray computed tomography(X-ray CT)was used,i e,the tomography system of Zeiss Xradia 510 versa.The results indicate that X-CT can monitor the development process and distribution characteristics of the internal cracks of cement pastes under ESA with attack time.In addition,the C3A content in the cement significantly affects the damage mode of cement paste specimens during sulfate erosion.The damage of ordinary Portland cement(OPC)pastes subjected to sulfate attack with high C3A content are severe,while the damage of sulfate resistant Portland cement(SRPC)pastes is much smaller than that of OPC pastes.Furthermore,a quadratic function describes the correlation between the crack volume fraction and development depth for two cement pastes immermed in sulfate solution.展开更多
基金supports from the National Natural Science Foundation of China(22375220,U2001214,22471302)the Guangdong Basic and Applied Basic Research Foundation(2024B1515020101)Open Project Fund from State Key Laboratory of Optoelectronic Materials and Technologies(OEMT-2024-KF-08).
文摘Formamidinium lead iodide(FAPbI_(3))perovskite exhibits an impressive X-ray absorption coefficient and a large carrier mobility-lifetime product(μτ),making it as a highly promising candidate for X-ray detection application.However,the presence of larger FA^(+)cation induces to an expansion of the Pb-I octahedral framework,which unfortunately affects both the stability and charge carrier mobility of the corresponding devices.To address this challenge,we develop a novel low-dimensional(HtrzT)PbI_(3) perovskite featuring a conjugated organic cation(1H-1,2,4-Triazole-3-thiol,HtrzT^(+))which matches well with theα-FAPbI_(3) lattices in two-dimensional plane.Benefiting from the matched lattice between(HtrzT)PbI_(3) andα-FAPbI_(3),the anchored lattice enhances the Pb-I bond strength and effectively mitigates the inherent tensile strain of theα-FAPbI_(3) crystal lattice.The X-ray detector based on(HtrzT)PbI_(3)(1.0)/FAPbI_(3) device achieves a remarkable sensitivity up to 1.83×10^(5)μC Gy_(air)^(−1) cm^(−2),along with a low detection limit of 27.6 nGy_(air) s^(−1),attributed to the release of residual stress,and the enhancement in carrier mobility-lifetime product.Furthermore,the detector exhibits outstanding stability under X-ray irradiation with tolerating doses equivalent to nearly 1.17×10^(6) chest imaging doses.
基金supported by the NSFC under Grant No.62474169the National Key Research and Development Program of China under Grant No.2024YFB3212200the funding from USTC under Grant Nos.WK2100000025,KY2190000003,and KY2190000006。
文摘Soft X-ray detectors play a vital role in materials science,high-energy physics and medical imaging.Cs_(2)AgBiBr_(6),a lead-free double perovskite,has gained attention for its excellent optoelectronic properties,stability,and nontoxicity.However,its fast crystallization and requirement for high-temperature annealing(>250℃)often lead to inferior film quality,limiting its application in flexible devices.This study introduces an alloying strategy that significantly improves the quality of Cs_(2)AgBiBr_(6)thin films annealed at a reduced temperature of 150℃.Devices based on the alloyed thin films exhibit an ultra-low dark current of 0.32 nA·cm^(-2)and a quantum efficiency of 725%.Furthermore,the first successful integration of Cs_(2)AgBiBr_(6)with a thinfilm transistor backplane demonstrates its superior imaging performance,indicating that Cs_(2)AgBiBr_(6)is a promising material for next-generation soft X-ray sensors.
基金funded by the National Natural Science Foundation of China(NNSFC)under Grant Numbers 42322408,42188101,and 42441809Additional support was provided by the Climbing Program of the National Space Science Center(NSSC,Grant No.E4PD3005)as well as the Specialized Research Fund for State Key Laboratories of China.
文摘A large-scale view of the magnetospheric cusp is expected to be obtained by the Soft X-ray Imager(SXI)onboard the Solar wind Magnetosphere Ionosphere Link Explorer(SMILE).However,it is challenging to trace the three-dimensional cusp boundary from a two-dimensional X-ray image because the detected X-ray signals will be integrated along the line of sight.In this work,a global magnetohydrodynamic code was used to simulate the X-ray images and photon count images,assuming an interplanetary magnetic field with a pure Bz component.The assumption of an elliptic cusp boundary at a given altitude was used to trace the equatorward and poleward boundaries of the cusp from a simulated X-ray image.The average discrepancy was less than 0.1 RE.To reduce the influence of instrument effects and cosmic X-ray backgrounds,image denoising was considered before applying the method above to SXI photon count images.The cusp boundaries were reasonably reconstructed from the noisy X-ray image.
基金This work was supported by the National Key Research and Development Program of China(Nos.2017YFA0403801,2016YFA0401302,2017YFA0206004,2018YFC1200204)the National Major Scientific Instruments and Equipment Development Project of China(No.11627901).
文摘This paper introduces some latest developments regarding the X-ray imaging methodology and applications of the X-ray imaging and biomedical application beamline(BL13W1)at Shanghai Synchrotron Radiation Facility in the past 5 years.The photon energy range of the beamline is 8–72.5 keV.Several sets of X-ray imaging detectors with different pixel sizes(0.19–24 lm)are used to realize X-ray microcomputed tomography(X-ray micro-CT)and X-ray in-line phase-contrast imaging.To satisfy the requirements of user experiments,new X-ray imaging methods and image processing techniques are developed.In vivo dynamic micro-CT experiments with living insects are performed in 0.5 s(sampling rate of 2 Hz,2 tomograms/s)with a monochromatic beam from a wiggler source and in 40 ms(sampling rate of 25 Hz,25 tomograms/s)with a white beam from a bending magnet source.A new X-ray imaging method known as move contrast X-ray imaging is proposed,with which blood flow and moving tissues in raw images can be distinguished according to their moving frequencies in the time domain.Furthermore,X-ray speckle-tracking imaging with twice exposures to eliminate the edge enhancement effect is developed.A high-precision quantification method is realized to measure complex three-dimensional blood vessels obtained via X-ray micro-CT.X-ray imaging methods such as three-dimensional X-ray diffraction microscopy,small-angle X-ray scattering CT,and X-ray fluorescence CT are developed,in which the X-ray micro-CT imaging method is combined with other contrast mechanisms such as diffraction,scattering,and fluorescence contrasts respectively.Moreover,an X-ray nano-CT experiment is performed with a 100 nm spatial resolution.Typical user experimental results from the fields of material science,biomedicine,paleontology,physics,chemistry,and environmental science obtained on the beamline are provided.
基金supported by the National Key R&D Program of China(No.2022YFF0608303)the National Major Scientific Research Instrument Development Project(No.11927805)+4 种基金the NSFC Young Scientists Fund(No.12005134)the Shanghai-XFEL Beamline Project(SBP)(No.31011505505885920161A2101001)the Shanghai Municipal Science and Technology Major Project(No.2017SHZDZX02)the Open Fund of the Key Laboratory for Particle Astrophysics and CosmologyMinistry of Education of China。
文摘In the exploration of celestial bodies,such as Mars,the Moon,and asteroids,X-ray fluorescence analysis has emerged as a critical tool for elemental analysis.However,the varying selection rules and excitation sources introduce complexity.Specifically,these discrepancies can cause variations in the intensities of the characteristic spectral lines emitted by identical elements.These variations,compounded by the minimal energy spacing between these spectral lines,pose substantial challenges for conventional silicon drift detectors(SDD),hindering their ability to accurately differentiate these lines and provide detailed insights into the material structure.To overcome this challenge,a cryogenic X-ray spectrometer based on transition-edge sensor(TES)detector arrays is required to achieve precise measurements.This study measured and analyzed the K-edge characteristic lines of copper and the diverse L-edge characteristic lines of tungsten using a comparative analysis of the electron and X-ray excitation processes.For the electron excitation experiments,copper and tungsten targets were employed as X-ray sources,as they emit distinctive X-ray spectra upon electron-beam bombardment.In the photon excitation experiments,a molybdenum target was used to produce a continuous spectrum with the prominent Mo Kαlines to emit pure copper and tungsten samples.TES detectors were used for the comparative spectroscopic analysis.The initial comparison revealed no substantial differences in the Kαand Kβlines of copper across different excitation sources.Similarly,the Lαlines of tungsten exhibited uniformity under different excitation sources.However,this investigation revealed pronounced differences within the Lβline series.The study found that XRF spectra preferentially excite outer-shell electrons,in contrast to intrinsic spectra,owing to different photon and electron interaction mechanisms.Photon interactions are selection-ruledependent and involve a single electron,whereas electron interactions can involve multiple electrons without such limitations.This leads to varied excitation transitions,as evidenced in the observed Lβline series.
基金supported by the Vinnova(project number 2020-03778)supported by the Swedish Research Council(Vetenskapsradet,project number 2021-04157).
文摘Nano-scale chemical inhomogeneity in surface oxide films formed on a V-and N-containing martensite stainless steel and tempering heating induced changes are investigated by a combination of synchrotron-based hard X-ray Photoelectron emission spectroscopy(HAXPES)and microscopy(HAXPEEM)as well as microscopic X-ray absorption spectroscopy(μ-XAS)techniques.The results reveal the inhomogeneity in the oxide films on the micron-sized Cr_(2)N-and VN-type particles,while the inhomogeneity on the martensite matrix phase exists due to localised formation of nano-sized tempering nitride particles at 600℃.The oxide film formed on Cr_(2)N-type particles is rich in Cr_(2)O_(3) compared with that on the martensite matrix and VN-type particles.With the increase of tempering temperature,Cr_(2)O_(3) formation is faster for the oxidation of Cr in the martensite matrix than the oxidation of Cr nitride-rich particles.
基金supported by“2020 Special Fund for Key Technology and Equipment Development of Major Science and Technology Infrastructure”from the Development and Reform Commission of Shenzhensupport from National Natural Science Foundation of China(Grant No.52103365)Guangdong Innovative and Entrepreneurial Research Team Program(Grant No.2021ZT09L227).
文摘Operando X-ray diffraction(XRD)is an important characterization tool for real-time monitoring of structural changes in materials under different reaction conditions.In this study,we developed a laboratory-based diffractometer that could capture a full XRD spectrum within 10 s.The instrument has several advanced features.First,it uses a Ga–In alloy metal-jet X-ray source,thereby achieving high X-ray flux with a brightness of up to 3.0×10^(10) photons/(s·mm^(2)·mrad2).Second,it employs an ellipsoidal mirror with a multilayer coating to produce quasi-parallel monochromatic light characterized by a divergence of 0.6 mrad and an energy resolution of 5.9×10^(−3).Third,it is equipped with a high-efficiency,high-signal-to-noise-ratio Pilatus 3R 1M detector for collecting diffraction signals.These features make the developed instrument applicable in studying rapid phase transitions in lithium-ion batteries,especially under extremely fast charge–discharge conditions.The data quality was comparable to that of synchrotron radiation XRD.
基金supported by the Instrument and Equipment Development Program of the Chinese Academy of Science(Grant No.YJKYYQ20180066)the National Natural Science Foundation of China(No.22227809)+2 种基金the Shanghai Science and Technology Innovation Action Plan(No.22142200300)the Science and Technology Talents Program of the Shanghai Institute of Applied Physics(No.SINAP-KJZX-202204)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDA 0400000).
文摘This study describes the design and performance of a laboratory-based tender X-ray spectrometer for X-ray absorption spectroscopy.The system enables effective absorption spectra to be measured within the 2.0-9.0 keV range using Rowland circle geometry;it covers the K edge of 3d transition metals,the L edge of lanthanides,and the M edge of actinides.The spectrometer is configured with a Rowland circle with a diameter of 500 mm and integrates a 250 W liquid metal jet X-ray source,spherical bent crystal analyzer,and energy-resolving silicon drift detector.The X-ray source is installed outside the vacuum chamber and remains fixed,while the analyzer crystals and detector are adjusted to change the Bragg angle,maintaining the Rowland condition.The energy resolution is 0.36-1.30 eV at 2.0-9.0 keV,and the monochromatic flux is approximately 5×10^(5) counts/s at 7040 eV.This study highlights the primary characteristics of the spectrometer and demon-strates its capabilities using selected experimental examples.The successful development of this spectrometer can facilitate research on actinide elements,which are often constrained in synchrotron radiation experiments owing to their radioactivity,thus fostering advancements in related nuclear energy fields.
基金supported by the Key Project of the National Natural Science Foundation of China-Yunnan Joint Fund(No.U2102215)National Natural Science Foundation(No.52472002)+5 种基金Science and Technology Project of Southwest Joint Graduate School of Yunnan Province(No.202302A0370008)2024 Industrial Innovation Talent Support Project(Preparation of luminous materials,performance control and application in plateau agriculture,No.YFGRC202407)National Natural Science Foundation of High-End Foreign Expert Introduction Plan(No.G2022039008L)Academician Workstation of Cherkasova Tatiana in Yunnan Province(No.202305AF150099)Yunnan Province Major Science and Technology Special Plan(No.202302AB080005)and UTS Chancellor’s Research Fellowship Program(No.J.L.,PRO22-15457)the National Health and Medical Research Council(No.J.L.,2025442).
文摘This study explores the application of X-ray-induced photochromism and photoluminescence in optical storage,anti-counterfeiting,non-destructive testing,and high-resolution X-ray detection and imaging.Ba_(2)LaNbO_(6):Bi,Eu phosphors were synthesized,with Bi enhancing X-ray-induced photochromic prop-erties.Under X-ray irradiation,the phosphors transfer from white to red in bright field conditions and emit red photoluminescence in dark field conditions.Exposure to 470 nm ultraviolet light induces rapid bleaching.The mechanisms of photochromism and photoluminescence,particularly Bi's role as a colorant,were systematically investigated.The Ba_(2)LaNbO_(6):Bi,Eu phosphors film achieves high resolution,high-lighting its potential for X-ray imaging and non-destructive testing.Furthermore,the flexible Ba_(2)LaNbO_(6):Bi,Eu film supports dual-mode imaging and detection,addressing the limitations of traditional flat dis-plays in 3D imaging.
基金supported by project of Beijing Postdoctoral Research Fund(Grant No.2025-ZZ-86)the National Natural Science Foundation of China(Grant Nos.12105020 and 12075031)+3 种基金Shenzhen Science and Technology Program(Grant No.KJZD20230923114219040)the Natural Science Youth Foundation of Henan Province,China(Grant No.242300420637)the Open Fund of Key Laboratory of Beam Technology of the Ministry of Education,Beijing Normal University(Grant No.BEAM2024G02)the Innovation Cultivation of Beijing Academy of Science and Technology(Grant Nos.25CB007-01 and 25CB007-02)。
文摘A double-parabola monocapillary(DPM)was designed for laboratory x-ray sources,and its performance was evaluated through numerical simulations and experimental validation.A surface shape error model was developed to characterize the DPM surface profile,and ray-tracing methods were used to simulate key properties such as focal spot size,divergence,and transmission efficiency.The simulation results closely matched experimental measurements,validating the proposed model.This surface shape error simulation provides an efficient method for evaluating the impact of slope errors on DPM performance,offering insights for optimal design and precision manufacturing.
基金the National Natural Science Foundation of China (Grant nos.21233004,21303147 and 21473148,etc.)the National Key Research and Development Program (Grant no.2016YFB0901500)
文摘The increased use of rechargeable batteries in portable electronic devices and the continuous develop-ment of novel applications （e.g. transportation and large scale energy storage）, have raised a strong de-mand for high performance batteries with increased energy density, cycle and calendar life, safety andlower costs. This triggers significant efforts to reveal the fundamental mechanism determining batteryperformance with the use of advanced analytical techniques. However, the inherently complex character-istics of battery systems make the mechanism analysis sophisticated and difficult. Synchrotron radiationis an advanced collimated light source with high intensity and tunable energies. It has particular ad-vantages in electronic structure and geometric structure （both the short-range and long-range structure）analysis of materials on different length and time scales. In the past decades, synchrotron X-ray tech-niques have been widely used to understand the fundamental mechanism and guide the technologicaloptimization of batteries. In particular, in situ and operando techniques with high spatial and temporalresolution, enable the nondestructive, real time dynamic investigation of the electrochemical reaction,and lead to significant deep insights into the battery operation mechanism. This review gives a brief introduction of the application of synchrotron X-ray techniques to the inves-tigation of battery systems. The five widely implicated techniques, including X-ray diffraction （XRD）, PairDistribution Function （PDF）, Hard and Soft X-ray absorption spectroscopy （XAS） and X-ray photoelectronspectroscopy （XPS） will be reviewed, with the emphasis on their in situ studies of battery systems during cycling.
文摘[目的/意义]苹果“冰糖心”又称水心病,是一种常见的果实病害,严重的水心病果会随着储藏时间的增加发生霉变,造成食品安全隐患。为实现不同等级水心病苹果快速无损检测,本研究旨在构建有效的分级与可溶性固形物(Soluble Solids Content,SSC)预测模型。[方法]本研究选取了230个富士苹果,其中正常、轻度、中度、重度水心苹果数量分别为113、61、47和9个,分别采集了400~1000 nm范围的反射光谱和X射线计算机断层成像(X-ray Computed Tomography,X-ray CT)数据,并测定了SSC含量。[结果和讨论]SSC随水心程度加剧呈上升趋势,重度水心苹果呈现更高的光谱反射率,X-ray CT扫描成像观察到水心区域的组织体积平均密度高于健康组织,基于三维重建算法实现不同等级水心苹果内部水心组织可视化分布。基于偏最小二乘判别分析(Partial Least Squares Discriminant Analysis,PLSDA)构建的不同水心程度苹果果实分级模型建模集和测试集准确率分别为98.7%和95.9%;构建不同水心程度苹果果实SSC回归模型,校正集决定系数(Correlation Coefficient of Calibration,R_(C)^(2))为0.962,均方根误差(Root Mean Squares Error of Calibration,RMSEC)为0.264,测试集决定系数(Correlation Coefficient of Prediction,R_(P)^(2))为0.879,均方根误差(Root Mean Squares Error of Prediction,RMSEP)为0.435。[结论]该研究构建的不同水心程度苹果果实分级模型能够实现苹果不同等级水心病的预测,构建的不同水心程度苹果果实SSC回归模型能够较好地预测苹果果实的SSC,为苹果水心病无损检测和品质评估提供了有效方法。
文摘Using the new soft X-ray data from the Macao Science Satellite-1,we studied a solar flare that occurred on 22 June 2023.We found that the centroids of the Ca(around 3.9 keV)and Fe(around 6.7 keV)line features exhibit a rapid shift toward higher energy channels during the flare's rising phase,followed by a gradual decrease during the decay phase.Through precise energy calibration,the centroids are determined with high accuracy.Temperature and velocity are then self-consistently derived by comparing the centroids with those calculated from the synthesized line features using the latest CHIANTI atomic database(ver.10.1).The calculated maximum velocity reaches up to 710±60 km s-1,which significantly exceeds the previously reported values.Our results suggest that the entire shift of soft X-ray lines may occur during the process of chromospheric evaporation.
文摘BACKGROUND In pediatric age group patients(<18 years old)treated operatively for distal radius/both bone fractures extending imaging beyond the initial postoperative period-particularly in uncomplicated cases-appears to provide limited additional benefit.AIM To determine the necessary number of follow-up X-rays to use resources efficiently.METHODS Participants included in this study are pediatric age group patients who were treated operatively for distal radius/both bone fractures and were identified from a prospected collected data from the operating room database between the years 2009 and 2017.The data in the study included patients who had distal radius fractures and underwent fixation surgery(n=88).RESULTS When assessing the difference in the odds of conducting 1 or less X-ray compared to 2 or more X-rays in regard to the type of fixation,the only significant difference is the closed reduction fixation method.Patients who underwent closed reduction method procedure have significantly lower odds of having 2 more X-rays compared to those who didn’t have closed reduction method.Open reduction,internal fixation,and other fixation methods(close reduction and internal fixation,debridement,or epiphysiodesis)have higher odds of having two or more X-rays compared to patients who did not receive these methods;however,these odds are not statistically significant.CONCLUSION The findings of this study reveal notable absence of a statistically significant association between the frequency of postoperative X-rays and the outcome of children with distal radius fractures.
基金supported by the National Natural Science Foundation of China(No.12035020)National Key Scientific Instrument and Equipment Development Projects of China(No.42327802).
文摘The main scientific payload of Macao Science Satellite-1B is a solar soft X-ray detection unit.To obtain an accurate solar X-ray spectrum,we have designed low-noise,high-throughput electronics.Solar radiation is detected using a low-leakage silicon drift detector(SDD),which is cooled to-30℃.The SDD output is processed using two parallel shaping amplifiers with peaking times of 315 ns and 65 ns.The amplifiers are designed using two-pole multiple-feedback active low-pass filters optimized to achieve a Bessel response.The differential output of the shaping amplifier generates a bipolar signal.The phase of the differential stage is tuned to ensure zero crossing corresponding to the peak of the shaping amplifier.A high-speed switch is inserted between the shaping amplifier and the peak-hold capacitor,and the peak value is maintained by turning off the switch.Fast and slow peak-hold circuits share a common ADC via time-division multiplexing.Both peak values are sampled for space-background rejection.Traditional pile-up detection methods cannot distinguish pulses that overlap in a fast channel.In this study,the differential of the“fast shaping”is selected,enabling the distinction of events separated by as little as 65ns,which is crucial for solar flare detection.The energy resolution is measured to be 138 eV at 5.90 keV.The centroid drift is less than 3.6 eV between-5℃ and 20℃.Compared with other solar X-ray instruments,this study demonstrates improved energy resolution with a lower peaking time,indicating a higher solar flare detection capability.
基金supported by the National Natural Science Foundation of China(No.12235006)the National Key Research and Development Program of China(No.2020YFE0202002.
文摘X-ray detectors show potential applications in medical imaging,materials science,and nuclear energy.To achieve high detection efficiency and spatial resolution,many conventional semiconductor materials,such as amorphous selenium,cadmium telluride zinc,and perovskites,have been utilized in direct conversion X-ray detectors.However,these semiconductor materials are susceptible to temperature-induced performance degradation,crystallization,delamination,uneven lattice growth,radiation damage,and high dark current.This study explores a new approach by coupling an FC40 electronic fluorinated liquid with a specialized high-resolution and high-readout-speed complementary metal-oxide-semiconductor(CMOS)pixel array,specifically the Topmetal II−chip,to fabricate a direct conversion X-ray detector.The fluorinated liquid FC40(molecular formula:C_(21)F_(48)N_(2))is an electronic medium that is minimally affected by temperature and displays no issues with uniform conductivity.It exhibits a low dark current and minimal radiation damage and enables customizable thickness in X-ray absorption.This addresses the limitations inherent in conventional semiconductor-based detectors.In this study,simple X-ray detector imaging tests were conducted,demonstrating the excellent coupling capability between FC40 electronic fluorinated liquid and CMOS chips by the X-ray detector.A spatial resolution of 4.0 lp/mm was measured using a striped line par card,and a relatively clear image of a cockroach was displayed in the digital radiography imaging results.Preliminary test results indicated the feasibility of fabricating an X-ray detector by combining FC40 electronic fluorinated liquid and CMOS chips.Owing to the absence of issues related to chip-material coupling,a high spatial resolution could be achieved by reducing the chip pixel size.This method presents a new avenue for studies on novel liquid-based direct conversion X-ray detectors.
基金supported by the National Natural Science Foundation of China(NSFC)12333010the National Key R&D Program of China 2022YFF0503002+3 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(grant No.XDB0560000)the NSFC 11921003supported by the Prominent Postdoctoral Project of Jiangsu Province(2023ZB304)supported by the Strategic Priority Research Program on Space Science,the Chinese Academy of Sciences,grant No.XDA15320000.
文摘Indirect X-ray modulation imaging has been adopted in a number of solar missions and provided reconstructed X-ray images of solar flares that are of great scientific importance.However,the assessment of the image quality of the reconstruction is still difficult,which is particularly useful for scheme design of X-ray imaging systems,testing and improvement of imaging algorithms,and scientific research of X-ray sources.Currently,there is no specified method to quantitatively evaluate the quality of X-ray image reconstruction and the point-spread function(PSF)of an X-ray imager.In this paper,we propose percentage proximity degree(PPD)by considering the imaging characteristics of X-ray image reconstruction and in particular,sidelobes and their effects on imaging quality.After testing a variety of imaging quality assessments in six aspects,we utilized the technique for order preference by similarity to ideal solution to the indices that meet the requirements.Then we develop the final quality index for X-ray image reconstruction,QuIX,which consists of the selected indices and the new PPD.QuIX performs well in a series of tests,including assessment of instrument PSF and simulation tests under different grid configurations,as well as imaging tests with RHESSI data.It is also a useful tool for testing of imaging algorithms,and determination of imaging parameters for both RHESSI and ASO-S/Hard X-ray Imager,such as field of view,beam width factor,and detector selection.
基金supported by the National Key R&D Program of China 2022YFF0503002the National Natural Science Foundation of China(NSFC,Grant Nos.12333010 and 12233012)+2 种基金the Strategic Priority Research Program of the Chinese Academy of Sciences(grant No.XDB0560000)supported by the Prominent Postdoctoral Project of Jiangsu Province(2023ZB304)supported by the Strategic Priority Research Program on Space Science,the Chinese Academy of Sciences,grant No.XDA15320000.
文摘Imaging observations of solar X-ray bursts can reveal details of the energy release process and particle acceleration in flares.Most hard X-ray imagers make use of the modulation-based Fourier transform imaging method,an indirect imaging technique that requires algorithms to reconstruct and optimize images.During the last decade,a variety of algorithms have been developed and improved.However,it is difficult to quantitatively evaluate the image quality of different solutions without a true,reference image of observation.How to choose the values of imaging parameters for these algorithms to get the best performance is also an open question.In this study,we present a detailed test of the characteristics of these algorithms,imaging dynamic range and a crucial parameter for the CLEAN method,clean beam width factor(CBWF).We first used SDO/AIA EUV images to compute DEM maps and calculate thermal X-ray maps.Then these realistic sources and several types of simulated sources are used as the ground truth in the imaging simulations for both RHESSI and ASO-S/HXI.The different solutions are evaluated quantitatively by a number of means.The overall results suggest that EM,PIXON,and CLEAN are exceptional methods for sidelobe elimination,producing images with clear source details.Although MEM_GE,MEM_NJIT,VIS_WV and VIS_CS possess fast imaging processes and generate good images,they too possess associated imperfections unique to each method.The two forward fit algorithms,VF and FF,perform differently,and VF appears to be more robust and useful.We also demonstrated the imaging capability of HXI and available HXI algorithms.Furthermore,the effect of CBWF on image quality was investigated,and the optimal settings for both RHESSI and HXI were proposed.
基金financially supported by the National Natural Science Foundation of China(Nos.52274315 and 52374320)the Fundamental Research Funds for the Central Universities(Nos.FRF-TP-22-011A1 and FRF-DF22-16)。
文摘During the continuous casting process of high-Mn high-Al steels,various types of gases such as Ar need to escape through the top of the mold.In which,the behavior of bubbles traversing the liquid slag serves as a restrictive link,closely associated with viscosity and the thickness of liquid slag.In contrast to two-dimensional surface observation,three-dimensional(3D)analysis method can offer a more intuitive,accurate,and comprehensive information.Therefore,this study employs a 3D X-ray microscope(3D-XRM)to obtained spatial distribution and 3D morphological characteristics of residual bubbles in mold flux under different basicity of liquid slag,different temperatures,and different holding times.The results indicate that as basicity of slag increases from 0.52 to 1.03,temperature increases from 1423 to 1573 K,the viscosity of slag decreases,the floating rate of bubbles increases.In addition,when holding time increases from 10 to 30 s,the bubbles floating distance increases,and the volume fraction and average equivalent sphere diameter of the bubbles solidified in the mold flux gradually decreases.In one word,increasing the basicity,temperature,and holding time leading to an increase in the removal rate of bubbles especially for the large.These findings of bubbles escape behavior provide valuable insights into optimizing low basicity mold flux for high-Mn high-Al steels.
基金Funded by Chinese National Natural Science Foundation of China(No.U2006224)。
文摘The paper presents experimental investigation results of crack pattern change in cement pastes caused by external sulfate attack(ESA).To visualize the formation and development of cracks in cement pastes under ESA,an X-ray computed tomography(X-ray CT)was used,i e,the tomography system of Zeiss Xradia 510 versa.The results indicate that X-CT can monitor the development process and distribution characteristics of the internal cracks of cement pastes under ESA with attack time.In addition,the C3A content in the cement significantly affects the damage mode of cement paste specimens during sulfate erosion.The damage of ordinary Portland cement(OPC)pastes subjected to sulfate attack with high C3A content are severe,while the damage of sulfate resistant Portland cement(SRPC)pastes is much smaller than that of OPC pastes.Furthermore,a quadratic function describes the correlation between the crack volume fraction and development depth for two cement pastes immermed in sulfate solution.
