Based on the Holstein model Hamiltonian of one-dimensional molecular crystals, by making use of the expansion approach of the correlated squeezed-coherent states of phonon instead of the two-phonon coherent state expa...Based on the Holstein model Hamiltonian of one-dimensional molecular crystals, by making use of the expansion approach of the correlated squeezed-coherent states of phonon instead of the two-phonon coherent state expansion scheme, the properties of the ground state and the anomalous quantum fluctuations are investigated in a strongly coupled electron-phonon system with special consideration of the electron-two-phonon interaction. The effective renormalization （ai） of the displacement of the squeezed phonons with the effect of the squeezed-coherent states of phonon and both the electron-displaced pbonon and the polaron-squeezed phonon correlations have been combined to obtain the anomalous quantum fluctuations for the corrections of the coherent state. Due to these non-adiabatic correlations, the effective displacement parameter ai is larger than the ordinary parameter ai （0） In comparison with the electron-one-phonon interaction （g） corrected as oig, we have found the electron-two-phonon interaction （gl） corrected as ai2gi is enhanced significantly. For this reason, the ground state energy （E（2）） contributed by the electron-two-phonon interaction is more negative than the single-phonon case （E01）） and the soliton solution is more stable. At the same time, the effects of the electron-two-phonon interaction greatly increase the polaron energy and the quantum fluctuations. Furthermore, in a deeper level, we have considered the effect of the polaron-squeezed phonon correlation （f-correlation）. Since this correlation parameter f 〉 1, this effect will strengthen the electron-one and two-phonon interactions by fai9 and f2ai2g1, respectively. The final results show that the ground state energy and the polaron energy will appear more negative further and the quantum fluctuations will gain further improvement.展开更多
Employing the Geilikman-Kresin (GK) theory, we address the experimental data obtained by Bauer et al., and by Schneider et al., on the thermal conductivity (κ) of superconducting MgB2. The two gaps of this compound h...Employing the Geilikman-Kresin (GK) theory, we address the experimental data obtained by Bauer et al., and by Schneider et al., on the thermal conductivity (κ) of superconducting MgB2. The two gaps of this compound have qualitatively been understood via the well-known Suhl, Matthias, and Walker’s (SMW) approach to multigap superconductivity. Since this approach is based on one-phonon exchange mechanism for the formation of Cooper pairs, it cannot give a quantitative account of the values of Tc and the multiple gaps that characterize MgB2 and other high-Tc superconductors (SCs). Despite this fact and some rather ambiguous features, it has been pointed out in a recent critical review by Malik and Llano (ML) that the SMW approach provides an important clue to deal with an SC the two gaps of which close at the same Tc: consider the possibility of the interaction parameters in the theory to be temperature-dependent. Guided by this clue, ML gave a complete summary of parameters that quantitatively account for the Tc and the gaps of MgB2 via the generalized BCS equations (GBCSEs). GBCSEs which we recall, invoke multi-phonon exchange mechanism for the formation of Cooper pairs and multiple Debye temperatures to deal with composite SCs. The parameter-values given in ML are used here to calculate the temperature-dependent gaps, which are an essential input for the GK theory. Notable features of this work are: 1)?kMgB2 is calculated for both—the scenario in which the two gaps of MgB2 close/do not close at the same temperature whence it is found that 2) the latter scenario yields results in better agreement with experiment.展开更多
We address the Tc (s) and multiple gaps of La2CuO4 (LCO) via generalized BCS equations incorporating chemical potential. Appealing to the structure of the unit cell of LCO, which comprises sub- lattices with LaO and O...We address the Tc (s) and multiple gaps of La2CuO4 (LCO) via generalized BCS equations incorporating chemical potential. Appealing to the structure of the unit cell of LCO, which comprises sub- lattices with LaO and OLa layers and brings into play two Debye temperatures, the concept of itinerancy of electrons, and an insight provided by Tacon et al.’s recent experimental work concerned with YBa2Cu3O6.6 which reveals that very large electron-phonon coupling can occur in a very narrow region of phonon wavelengths, we are enabled to account for all values of its gap-to-Tc ratio (2Δ0/kBTc), i.e., 4.3, 7.1, ≈8 and 9.3, which were reported by Bednorz and Müller in their Nobel lecture. Our study predicts carrier concentrations corresponding to these gap values to lie in the range 1.3 × 1021 - 5.6 × 1021 cm-3, and values of 0.27 - 0.29 and 1.12 for the gap-to-Tc ratios of the smaller gaps.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No. 10574163)
文摘Based on the Holstein model Hamiltonian of one-dimensional molecular crystals, by making use of the expansion approach of the correlated squeezed-coherent states of phonon instead of the two-phonon coherent state expansion scheme, the properties of the ground state and the anomalous quantum fluctuations are investigated in a strongly coupled electron-phonon system with special consideration of the electron-two-phonon interaction. The effective renormalization （ai） of the displacement of the squeezed phonons with the effect of the squeezed-coherent states of phonon and both the electron-displaced pbonon and the polaron-squeezed phonon correlations have been combined to obtain the anomalous quantum fluctuations for the corrections of the coherent state. Due to these non-adiabatic correlations, the effective displacement parameter ai is larger than the ordinary parameter ai （0） In comparison with the electron-one-phonon interaction （g） corrected as oig, we have found the electron-two-phonon interaction （gl） corrected as ai2gi is enhanced significantly. For this reason, the ground state energy （E（2）） contributed by the electron-two-phonon interaction is more negative than the single-phonon case （E01）） and the soliton solution is more stable. At the same time, the effects of the electron-two-phonon interaction greatly increase the polaron energy and the quantum fluctuations. Furthermore, in a deeper level, we have considered the effect of the polaron-squeezed phonon correlation （f-correlation）. Since this correlation parameter f 〉 1, this effect will strengthen the electron-one and two-phonon interactions by fai9 and f2ai2g1, respectively. The final results show that the ground state energy and the polaron energy will appear more negative further and the quantum fluctuations will gain further improvement.
文摘Employing the Geilikman-Kresin (GK) theory, we address the experimental data obtained by Bauer et al., and by Schneider et al., on the thermal conductivity (κ) of superconducting MgB2. The two gaps of this compound have qualitatively been understood via the well-known Suhl, Matthias, and Walker’s (SMW) approach to multigap superconductivity. Since this approach is based on one-phonon exchange mechanism for the formation of Cooper pairs, it cannot give a quantitative account of the values of Tc and the multiple gaps that characterize MgB2 and other high-Tc superconductors (SCs). Despite this fact and some rather ambiguous features, it has been pointed out in a recent critical review by Malik and Llano (ML) that the SMW approach provides an important clue to deal with an SC the two gaps of which close at the same Tc: consider the possibility of the interaction parameters in the theory to be temperature-dependent. Guided by this clue, ML gave a complete summary of parameters that quantitatively account for the Tc and the gaps of MgB2 via the generalized BCS equations (GBCSEs). GBCSEs which we recall, invoke multi-phonon exchange mechanism for the formation of Cooper pairs and multiple Debye temperatures to deal with composite SCs. The parameter-values given in ML are used here to calculate the temperature-dependent gaps, which are an essential input for the GK theory. Notable features of this work are: 1)?kMgB2 is calculated for both—the scenario in which the two gaps of MgB2 close/do not close at the same temperature whence it is found that 2) the latter scenario yields results in better agreement with experiment.
文摘We address the Tc (s) and multiple gaps of La2CuO4 (LCO) via generalized BCS equations incorporating chemical potential. Appealing to the structure of the unit cell of LCO, which comprises sub- lattices with LaO and OLa layers and brings into play two Debye temperatures, the concept of itinerancy of electrons, and an insight provided by Tacon et al.’s recent experimental work concerned with YBa2Cu3O6.6 which reveals that very large electron-phonon coupling can occur in a very narrow region of phonon wavelengths, we are enabled to account for all values of its gap-to-Tc ratio (2Δ0/kBTc), i.e., 4.3, 7.1, ≈8 and 9.3, which were reported by Bednorz and Müller in their Nobel lecture. Our study predicts carrier concentrations corresponding to these gap values to lie in the range 1.3 × 1021 - 5.6 × 1021 cm-3, and values of 0.27 - 0.29 and 1.12 for the gap-to-Tc ratios of the smaller gaps.
