A modified internal-loop airlif reactor (MIALR) with a continuous slurry phase was studied to investigate the local hydrodynamic characteristics, including gas holdup, bubble size, bubble rise velocity and local mas...A modified internal-loop airlif reactor (MIALR) with a continuous slurry phase was studied to investigate the local hydrodynamic characteristics, including gas holdup, bubble size, bubble rise velocity and local mass transfer properties. Based on the analysis of geometrical construction and fluid properties of gas and slurry, MIALR was divided into six flow regions. In these flow regions, the local hydrodynamic characteristics were investigated over a wide range of operating variables. Furthermore, a new method was developed to measure the dissolved oxygen concentration. The volumetric mass-transfer coefficient in six flow regions was also calculated for comparison.展开更多
In this paper, the characteristics of fluid mixing time in a novel extra-loop fluidized bed were studied. The results showed that the mixing time was shortened with the increase of fluid velocity. All the discrete num...In this paper, the characteristics of fluid mixing time in a novel extra-loop fluidized bed were studied. The results showed that the mixing time was shortened with the increase of fluid velocity. All the discrete numbers of the reactor were above 0.2. The serial number n was 2.5 -3.0. It was judged accordingly that the reactor fluid state was continous stirred tank reactor (CSTR) mainly. When the inspiratory capacity increased the mixing time of the reactor was shortened. Thus the air input was beneficial for the fluid mixing. During the three phases mixing process, the mixing time of the reactor could be decreased by the n increase of carrier and air loading together, but the change was not significant. The parameters affecting the reactor fluid state were fluid velocity, inspiratory capacity and carrier. KLa could be increased with the air loading increase, and at the same gas/liquid ratio when the pressure drop was high, KL~ value was increased. The amount of carrier complex influence on KLa. As the carrier loading continued to increase, its value had been dropped but the changes was not significant, and optimization condition was found at above 800 1 000 g carrier loading (pouzzolane) or 600 g PVC. Under gas/liquid ratio of 0.8% -5.2%, KLa was (0.62-1.37)×10^-2· s^-1.展开更多
Artificial intelligence(AI)has undergone rapid development and has become increasingly involved in scientific explorations[1].It not only successfully facilitates the efficient completion of previous labor-intensive a...Artificial intelligence(AI)has undergone rapid development and has become increasingly involved in scientific explorations[1].It not only successfully facilitates the efficient completion of previous labor-intensive and time-consuming tasks,including literature review,compound screening,and data analysis,but also guides closed-loop experiments for target functions optimization[2].However,the potential of AI for uncovering new chemical knowledge remains largely untapped[3].展开更多
文摘A modified internal-loop airlif reactor (MIALR) with a continuous slurry phase was studied to investigate the local hydrodynamic characteristics, including gas holdup, bubble size, bubble rise velocity and local mass transfer properties. Based on the analysis of geometrical construction and fluid properties of gas and slurry, MIALR was divided into six flow regions. In these flow regions, the local hydrodynamic characteristics were investigated over a wide range of operating variables. Furthermore, a new method was developed to measure the dissolved oxygen concentration. The volumetric mass-transfer coefficient in six flow regions was also calculated for comparison.
基金Project supported by the Foundation Social European,Republoque Francaise
文摘In this paper, the characteristics of fluid mixing time in a novel extra-loop fluidized bed were studied. The results showed that the mixing time was shortened with the increase of fluid velocity. All the discrete numbers of the reactor were above 0.2. The serial number n was 2.5 -3.0. It was judged accordingly that the reactor fluid state was continous stirred tank reactor (CSTR) mainly. When the inspiratory capacity increased the mixing time of the reactor was shortened. Thus the air input was beneficial for the fluid mixing. During the three phases mixing process, the mixing time of the reactor could be decreased by the n increase of carrier and air loading together, but the change was not significant. The parameters affecting the reactor fluid state were fluid velocity, inspiratory capacity and carrier. KLa could be increased with the air loading increase, and at the same gas/liquid ratio when the pressure drop was high, KL~ value was increased. The amount of carrier complex influence on KLa. As the carrier loading continued to increase, its value had been dropped but the changes was not significant, and optimization condition was found at above 800 1 000 g carrier loading (pouzzolane) or 600 g PVC. Under gas/liquid ratio of 0.8% -5.2%, KLa was (0.62-1.37)×10^-2· s^-1.
基金supported by the Start-Up Research Fund of Southeast University(No.4012002405).
文摘Artificial intelligence(AI)has undergone rapid development and has become increasingly involved in scientific explorations[1].It not only successfully facilitates the efficient completion of previous labor-intensive and time-consuming tasks,including literature review,compound screening,and data analysis,but also guides closed-loop experiments for target functions optimization[2].However,the potential of AI for uncovering new chemical knowledge remains largely untapped[3].