Palladium-modified nitrogen-doped titanium oxide(TiON/PdO) thin film was synthesized by the ion-beamassisted deposition technique,which enabled a heavy nitrogen doping and the subsequent light absorption extension to7...Palladium-modified nitrogen-doped titanium oxide(TiON/PdO) thin film was synthesized by the ion-beamassisted deposition technique,which enabled a heavy nitrogen doping and the subsequent light absorption extension to700 nm for a better usage of the solar spectrum.Based on TiON/PdO thin film and a phase contrast microscope,a micro-reaction chamber was developed,which allowed the simultaneous optical excitation of the photocatalytic thin film and the phase contrast image observation of cells in it.The real time,in situ observation of the photocatalytic destruction of Saccharomyces cerevisiae(S.cerevisiae),an essential eukaryotic unicellular model of living cells,was conducted with this new observation technique,which demonstrated clearly that the photocatalytic destruction effect was much stronger than the photodamage effect caused by the visible light irradiation alone in the disinfection process.展开更多
基金supported by the National Natural Science Foundation of China (Grant No. 51102246)the Knowledge Innovation Program of Institute of Metal Research, Chinese Academy of Sciences (Grant No. Y0N5A111A1)+1 种基金the Youth Innovation Promotion Association, Chinese Academy of Sciences (Grant No. Y2N5711171)the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry, China
文摘Palladium-modified nitrogen-doped titanium oxide(TiON/PdO) thin film was synthesized by the ion-beamassisted deposition technique,which enabled a heavy nitrogen doping and the subsequent light absorption extension to700 nm for a better usage of the solar spectrum.Based on TiON/PdO thin film and a phase contrast microscope,a micro-reaction chamber was developed,which allowed the simultaneous optical excitation of the photocatalytic thin film and the phase contrast image observation of cells in it.The real time,in situ observation of the photocatalytic destruction of Saccharomyces cerevisiae(S.cerevisiae),an essential eukaryotic unicellular model of living cells,was conducted with this new observation technique,which demonstrated clearly that the photocatalytic destruction effect was much stronger than the photodamage effect caused by the visible light irradiation alone in the disinfection process.