Cirrus clouds play a crucial role in the energy balance of the Earth-atmosphere system.We investigated the spatiotemporal variations of cirrus over the South China Sea(SCS)using satellite data(MOD08,MYD08,CALIPSO)and ...Cirrus clouds play a crucial role in the energy balance of the Earth-atmosphere system.We investigated the spatiotemporal variations of cirrus over the South China Sea(SCS)using satellite data(MOD08,MYD08,CALIPSO)and reanalysis data(MERRA-2)from March 2007 to February 2015(eight years).The horizontal distribution reveals lower cirrus fraction values in the northern SCS and higher values in the southern region,with minima observed in March and April and maxima sequentially occurring in August(northern SCS,NSCS),September(middle SCS,MSCS),and December(southern SCS,SSCS).Vertically,the cirrus fraction peaks in summer and reaches its lowest levels in spring.Opaque cirrus dominates during summer in the NSCS and MSCS,comprising 53.6%and 55.9%,respectively,while the SSCS exhibits a higher frequency of opaque cirrus relative to other cloud types.Subvisible cirrus clouds have the lowest frequency year-round,whereas thin cirrus is most prominent in winter in the NSCS(46.3%)and in spring in the MSCS(45.3%).A case study from September 2021 further explores the influence of ice crystal habits on brightness temperature(BT)over the SCS.Simulations utilizing five ice crystal shapes from the ARTS DDA(Atmospheric Radiative Transfer Simulator Discrete Dipole Approximation)database and the RTTOV 12.4 radiative transfer model reveal that the 8-column-aggregate shape best represents BT in the NSCS and SSCS,while the large-block-aggregate shape performs better in the SSCS.展开更多
Benzene,toluene,ethylbenzene,and xylene(BTEX)pollution poses a serious threat to public health and the environment because of its respiratory and neurological effects,carcinogenic properties,and adverse effects on air...Benzene,toluene,ethylbenzene,and xylene(BTEX)pollution poses a serious threat to public health and the environment because of its respiratory and neurological effects,carcinogenic properties,and adverse effects on air quality.BTEX exposure is a matter of grave concern in India owing to the growing vehicular and development activities,necessitating the assessment of atmospheric concentrations and their spatial variation.This paper presents a comprehensive assessment of ambient concentrations and spatiotemporal variations of BTEX in India.The study investigates the correlation of BTEX with other criteria pollutants andmeteorological parameters,aiming to identify interrelationships and diagnostic indicators for the source characterization of BTEX emissions.Additionally,the paper categorizes various regions in India according to the Air Quality Index(AQI)based on BTEX pollution levels.The results reveal that the northern zone of India exhibits the highest levels of BTEX pollution compared to central,eastern,and western regions.In contrast,the southern zone experiences the least pollution with BTEX.Seasonal analysis indicates that winter and postmonsoon periods,characterized by lower temperatures,are associated with higher BTEX levels due to the accumulation of localized emissions.When comparing the different zones in India,high traffic emissions and localized activities,such as solvent use and solvent evaporation,are found to be the primary sources of BTEX.The findings of the current study aid in source characterization and identification,and better understanding of the region’s air quality problems,which helps in the development of focused BTEX pollution reduction and control strategies.展开更多
To investigate the characteristics of water environmental pollution in the Nenjiang River Basin,five monitoring sections,including Zhenxi,Xianghai Reservoir,Baishatan,Yuelianghu Reservoir,and Da an,were selected.Utili...To investigate the characteristics of water environmental pollution in the Nenjiang River Basin,five monitoring sections,including Zhenxi,Xianghai Reservoir,Baishatan,Yuelianghu Reservoir,and Da an,were selected.Utilizing water quality monitoring data collected from 2013 to 2022,the fuzzy comprehensive evaluation method was employed to systematically analyze the spatiotemporal variation patterns of water quality,assess the current pollution status,and identify the influencing factors of non-point source pollution.The results indicated that the concentrations of representative pollutants at five sections in the lower reaches of the Nenjiang River generally exhibited a downward trend,accompanied by an overall improvement in water quality.However,the degree of improvement varied considerably among the different sections.Specifically,the water quality of the main stream of the Nenjiang River(Baishatan and Da an)improved from Class IV to Class III.In contrast,the Xianghai Reservoir consistently remained at Class V or below,primarily due to excessive fluoride levels.The water quality at Yuelianghu Reservoir and Heidimiao Section demonstrated a fluctuating but overall improving trend.Based on the analysis of pollution sources,targeted recommendations are proposed,including regulating the ecological water requirements of rivers,restoring wetland ecosystems,and enhancing the management of non-point source pollution.These measures offer scientific support for water quality management and ecological conservation in the river basins.展开更多
Methane(CH_(4))is the second greenhouse gas and has a profound impact on global climate change due to its high global warming potential and concentration.By 2022,the CH_(4)concentration was approximately 1.9 ppm,which...Methane(CH_(4))is the second greenhouse gas and has a profound impact on global climate change due to its high global warming potential and concentration.By 2022,the CH_(4)concentration was approximately 1.9 ppm,which was 264%of the pre-industrial level.The spatiotemporal distribution of CH_(4)was investigated by a portable CH_(4)detector on an unmanned aerial vehicle and electric bicycles in Shaoxing,a city situated in the Yangtze River Delta,China.The vertical distribution revealed CH_(4)concentration generally decreased slowly with height.However,the inversion condition and low atmospheric boundary layer height(ABLH)leaded to the enhancement of CH_(4)with height.The highest CH_(4)concentration(2.2±0.1 ppm,n=1428)was observed in winter and the lowest(2.0±0.2 ppm,n=1530)in spring.Regarding the daily variation,CH_(4)concentration peaked at 5:00 local time(LT)and reached its lowest level at 14:00 LT,which was attributed to the daily variation of ABLH,lowest in the early morning and highest in the noon.In urban areas,CH_(4)concentrations showed higher levels near restaurants,natural gas stations and sewerage well,with a maximum value of 13.1 ppm,which was caused by CH_(4)emission and natural gas leakage from these places.The annual CH_(4)emission in Shaoxing were estimated to be approximately 69 ton/(km^(2)·year)by the mass balance approach.Compared with other cities in the world,the CH_(4)emission is in higher level which imply some control measures should be conducted to reduce CH_(4)emission in Shaoxing.展开更多
As in-situ observations are sparse,targeted observations of a specific mesoscale eddy are rare.Therefore,it is difficult to study the three-dimensional structure of moving mesoscale eddies.From April to September 2014...As in-situ observations are sparse,targeted observations of a specific mesoscale eddy are rare.Therefore,it is difficult to study the three-dimensional structure of moving mesoscale eddies.From April to September 2014,an anticyclonic eddy located at 135°E-155°E,26°N-42°N was observed using 17 rapidsampling Argo floats,and the spatiotemporal variations in the three-dimensional structure were studied.The results are as follows:(1)the eddy was identified and tracked using satellite altimeter data.It had a lifetime of 269 days and an average radius of 91.5 km.The lifetime of the eddy can be divided into three phases,i.e.,the initiation,maturity,and termination phases.The depth of its influence reached 1000 m;(2)the Argo profiles were divided into seven periods(approximately 20 days in each)for composite analysis,and the composite Argo profiles and CARS2009(CSIRO Atlas of Regional Seas)climatology data were merged following the data-interpolating variational analysis(DIVA)method to reconstruct the three-dimensional structure.The temperature and salinity anomaly cores of the anticyclonic mesoscale eddy are located from 400 to 600 m.From 800 to 900 m,there is an area of low salinity at the center of the eddy.A high concentration anomaly of dissolved oxygen was located at approximately 250 m;(3)to better understand the features of the eddy and its interaction with the surroundings,we calculated the anomalous velocity of the geostrophic flow and the heat,salt,dissolved oxygen transport anomaly,and discussed the eddy's origin and its adjustments to topography.The maximum heat,salt,and oxygen transport caused by eddy were 9.37×10^11 W,3.08×10^3 kg/s,and 2.70×10^2 kg/s,which all occurred during the termination phase.This study highlights the applicability of using Argo floats to understand the three-dimensional structure thermohaline features of eddies in the North Pacific.展开更多
Photosynthetically active radiation （PAR） is the energy source of plant photosyn thesis, and the diffuse component can enhance canopy light use efficiency, thereby increasing the carbon uptake. Therefore, diffuse PA...Photosynthetically active radiation （PAR） is the energy source of plant photosyn thesis, and the diffuse component can enhance canopy light use efficiency, thereby increasing the carbon uptake. Therefore, diffuse PAR is an important driving factor of ecosystem productivity models. In this study, we estimated the diffuse PAR of over 700 meteorological sites in China from 1981 to 2010 using an empirical model based on observational data from Chinese Ecosystem Research Network （CERN） and China Meteorology Administration. Then we derived the spatial data set of 10 km monthly diffuse PAR using ANUSPLIN software, and analyzed the spatiotemporal variation characteristics of diffuse PAR through GIS and trend analysis techniques. The results showed that： （1） The spatial patterns of annual average diffuse PAR during 1981-2010 are heterogeneous across China, lower in the northeast and higher in the west and south. The nationwide average value for 30 years ranges from 6.66 mol m-2 d-1 to 15.27 mol m-2 d-1, and the value in summer is the biggest while the value in winter is the smallest. （2） There is an evident increasing trend of annual diffuse PAR during recent 30 years, with the increasing amplitude at 0.03 mol m-2 d-l/10a. But a significant declining trend is shown in the first 10 years, and obvious anomalies can be seen in 1982, 1983, 1991 and 1992. And there is a downtrend in spring and an uptrend in all the other seasons. （3） The spatial distribution of temporal variation rates of diffuse PAR is inhomogeneous across the country, generally decreasing in the north and increasing in the south.展开更多
Rapid industrialization and urbanization have led to the most serious habitat degradation in China,especially in the loess hilly area of the Yellow River Basin,where the ecological environment is relatively fragile.Th...Rapid industrialization and urbanization have led to the most serious habitat degradation in China,especially in the loess hilly area of the Yellow River Basin,where the ecological environment is relatively fragile.The contradiction between economic development and ecological environment protection has aroused widespread concern.In this study,we used the habitat quality of Integrated Valuation of Ecosystem Services and Tradeoffs(InVEST-HQ)model at different scales to evaluate the dynamic evolution characteristics of habitat quality in Lanzhou City,Gansu Province of China.The spatiotemporal variations of habitat quality were analyzed by spatial autocorrelation.A Geographical Detector(Geodetector)model was used to explore the driving factors that influencing the spatial differentiation of habitat quality,including natural factors,socio-economic factors,and ecological protection factors.The results showed that the habitat quality index of Lanzhou City decreased from 0.4638 to 0.4548 during 2000-2018.The areas with reduced the habitat quality index were mainly located in the Yellow River Basin and Qinwangchuan Basin,where are the main urban areas and the new economic development areas,respectively.The spatial distribution of habitat quality presented a trend of high in the surrounding areas and low in the middle,and showed a significant positive spatial autocorrelation.With the increase of study scale,the spatial distribution of habitat quality changed from concentrated to dispersed.The spatial differentiation of habitat quality in the study area was the result of multiple factors.Among them,topographic relief and slope were the key factors.The synergistic enhancement among these driving factors intensified the spatial differentiation of habitat quality.The findings of this study can provide a scientific basis for land resources utilization and ecosystem restoration in the arid and semi-arid land.展开更多
The process of habitat degradation varies in habitat type and driving force which shows certain spatial and temporal heterogeneity on regional scales. In the present study, a new diagnostic model for enclosed bay habi...The process of habitat degradation varies in habitat type and driving force which shows certain spatial and temporal heterogeneity on regional scales. In the present study, a new diagnostic model for enclosed bay habitat degradation was established, with which the spatial and temporal variation patterns of habitat degradation during 1991–2012 in Sansha Bay, Fujian, China was investigated. The results show that anthropogenic disturbance is the major controlling factor for the habitat degradation in large temporal heterogeneity in the bay. On the other hand, the habitat degradation experienced signifi cant spatial variations among six sub-bays. Under the joint action of temporal and spatial heterogeneity, the degradation trend in growing scale shows a more signifi cant correlation with the distribution of local leading industries along shorelines. Therefore, we quantifi ed the main characters of habitat degradation in Sansha Bay, and have understood the relationship between the status of habitats spatio-temporal variation value and the main controlling factor leading to the changes. However, a defi ciency of this research is the lack of or inaccessible to the detailed data, which shall be better solved in the future study for accessing more data from more sources.展开更多
Investigation on spatiotemporal variations of maximum seasonal freeze depth （MSFD） over the Heihe River Basin is of great importance for systematic understanding of regional climate and environmental change, ecologi...Investigation on spatiotemporal variations of maximum seasonal freeze depth （MSFD） over the Heihe River Basin is of great importance for systematic understanding of regional climate and environmental change, ecological-hydrological processes, water resources assessment, construction and resource development. Based on soil and air temperatures at the meteorological stations of the China Meteorological Administration （CMA） over the Heihe River Basin, MSFDs time series are structured into a composite time series over the 1960-2007 period. Evaluating the averaged MSFD time series for 1960 2007 reveals a statistically significant trend of 4.0 cm/decade or a net change of-19.2 cm for the 48-year period over the basin. The MSFD had significantly negative correlation with mean annual air temperature （MAAT）, winter air temperature, mean annual ground surface temperature （MAGST）, degree days of thawing for the air （DDTa） as well as for the surface （DDTs）, and degree days of freezing for the surface （DDFs）. While there was significantly positive correlation between DDF,. and MSFD time series, MSFD was deeper and changed greatly in the Heihe River source area. It was shallower in the east-central basin and gradually deepened in other sections of the basin. The MSFD distribution pattern in 2003-2005 is consistent with that of averaged degree days of freezing for air （DDFa） in 1960-2007. However, the maximum of MSFD may not be accurate, because there is no long term observation data in the deep seasonally frozen ground regions near the lower boundary of permafrost. With increasing elevation, averaged DDFa increased at a rate of 51.6 ℃-day/100m, therefore, the MSFG and the date reaching MSFG became deeper and later, respectively.展开更多
On the basis of the QSCAT/NCEP blended wind data and simple ocean data assimilation （SODA）, the wind-induced near-inertial energy flux （NIEF） in the mixed layer of the South China Sea （SCS） is estimated by a sla...On the basis of the QSCAT/NCEP blended wind data and simple ocean data assimilation （SODA）, the wind-induced near-inertial energy flux （NIEF） in the mixed layer of the South China Sea （SCS） is estimated by a slab model, and the model results are verified by observational data near the Xisha Islands in the SCS. Then, the spatial and temporal variations of the NIEF in the SCS are analyzed. It is found that, the monthly mean NIEF exhibits obvious spatial and temporal variabilities, i.e., it is large west of Luzon Island all the year, east of the Indo-China Peninsula all the year except in spring, and in the northern SCS from May to Septem- ber. The large monthly mean NIEF in the first two zones may be affected by the large local wind stress curl whilst that in the last zone is probably due to the shallow mixed layer depth. Moreover, the monthly mean NIEF is relatively large in summer and autumn due to the passage of typhoons. The spatial mean NIEF in the mixed layer of the SCS is estimated to be about 1.25 mW/m2 and the total wind energy input from wind is approximately 4.4 GW. Furthermore, the interannual variability of the spatial monthly mean NIEF and the Nifio3.4 index are negatively correlated.展开更多
As an important natural resource,forest land plays a key role in the maintenance of ecological security.However,variations of forest land in the agropastoral ecotone of northern China(AENC)have attracted little attent...As an important natural resource,forest land plays a key role in the maintenance of ecological security.However,variations of forest land in the agropastoral ecotone of northern China(AENC)have attracted little attention.Taking the AENC as an example and based on remote-sensing images from 2000,2010 to 2020,we explored the spatiotemporal variation of forest land and its driving factors using the land-use transfer matrix,spatial autocorrelation analysis and spatial error model.The results showed that from 2000 to 2020,the total area of forest land in the AENC increased from 75,547.52 to 77,359.96 km^(2) and the changes were dominated by the transformations among forest land,grassland and cropland,which occurred mainly in areas with the elevation of 500-2000 m and slope of 15°-25°.There was obvious spatial agglomeration of forest land in the AENC from 2000 to 2020,with hot spots of forest land gathered in the southern marginal areas of the Yanshan Mountains and the low mountainous and hilly areas of the Loess Plateau.The sub-hot spots around hot spots moved southward,the sub-cold spots spread to the surrounding areas and the cold spots disappeared.The spatiotemporal variation of forest land resulted from the interactions of natural environment,socioeconomic and policy factors from 2000 to 2020.The variables of average annual precipitation,slope,terrain relief,ecological conversion program and afforestation policy for barren mountains affected the spatial pattern of forest land positively,while those of annual average temperature,slope and road network density influenced it negatively.展开更多
The Los Alamos Sea-Ice Model(CICE)is one of the most popular sea-ice models.All versions of it have been the main sea-ice module coupled to climate system models.Therefore,evaluating their simulation capability is an ...The Los Alamos Sea-Ice Model(CICE)is one of the most popular sea-ice models.All versions of it have been the main sea-ice module coupled to climate system models.Therefore,evaluating their simulation capability is an important step in developing climate system models.Compared with observations and previous versions(CICE4.0 and CICE5.0),the advantages of CICE6.0(the latest version)are analyzed in this paper.It is found that CICE6.0 has the minimum interannual errors,and the seasonal cycle it simulates is the most consistent with observations.CICE4.0 overestimates winter sea-ice and underestimates summer sea-ice severely.Meanwhile,the errors of CICE5.0 in winter are larger than for the other versions.The main attention is paid to the perennial ice and the seasonal ice.The spatial distribution of root-mean-square errors indicates that the simulated errors are distributed in the Atlantic sector and the outer Arctic.Both CICE4.0 and CICE5.0 underestimate the concentration of the perennial ice and overestimate that of the seasonal ice in these areas.Meanwhile,CICE6.0 solves this problem commendably.Moreover,the decadal trends it simulates are comparatively the best,especially in the central Arctic sea.The other versions underestimate the decadal trend of the perennial ice and overestimate that of the seasonal ice.In addition,an index used to objectively describe the difference in the spatial distribution between the simulation and observation shows that CICE6.0 produces the best simulated spatial distribution.展开更多
River hydrogeochemistry offers necessary guidance for effective water environmental management.However,the influence of cascade reservoirs on river hydrogeochemistry remains unknown.In this study,the Jinsha River,the ...River hydrogeochemistry offers necessary guidance for effective water environmental management.However,the influence of cascade reservoirs on river hydrogeochemistry remains unknown.In this study,the Jinsha River,the headwaters of the Yangtze River of China,was selected to investigate the spatiotemporal variations of hydrogeochemistry after the construction of six cascade reservoirs.Major ions,total dissolved solids,electrical conductivity,and pH values of sampled water in the upper natural reaches and lower reservoir-regulated reaches were analyzed in both flood and dry seasons.The results of Piper diagram and Gibbs plots showed that the hydrogeochemistry of the Jinsha River was naturally controlled by both evaporation-crystallization and carbonate weathering processes,but it was also artificially affected by reservoirs.The impoundment of cascade reservoirs affected the hydrodynamic condition of the river.The river flow in the flood season was reduced by approximately 24.5%,altering the proportions of water sources and leading to notable hydrogeochemical alterations in reservoir-regulated reaches.Conversely,river hydrogeochemistry generally remained unchanged in the dry season,owing to the insignificant effect of cascade reservoirs on river flow.In contrast to what has been observed in previous studies of individual reservoirs,the cumulative influence of cascade reservoirs on the Jinsha River flow regime did not cause abrupt hydrogeochemical changes between the upstream and downstream areas of each reservoir.Moreover,the water quality assessments revealed that the impoundment of cascade reservoirs improved downstream irrigational water quality,with lower Naþratio values in the flood season.This study provides the earliest evaluation of cascade reservoir influence on the hydrogeochemistry of the Jinsha River.The findings of this study can be used as a reference for scientific guidelines for future environmental management of cascade reservoirs in large rivers.展开更多
Castanopsis fargesii is a good afforestation plants and various microorganisms play important roles in mediating the growth and ecological functions of this species.In this study,we evaluated changes in microbial comm...Castanopsis fargesii is a good afforestation plants and various microorganisms play important roles in mediating the growth and ecological functions of this species.In this study,we evaluated changes in microbial communities in soil samples from C.fargesii forests.The phospholipid fatty acid(PLFA)biomarker method was used to obtain bacteria,fungi,actinomycetes,gram-positive bacteria(G?),gram-negative bacteria(G-),aerobic bacteria,and anaerobic bacteria to investigate spatiotemporal changes in microbial communities during the growing season.The results show that soil microorganisms were mainly concentrated in the upper 20-cm layer,demonstrating an obvious surface aggregation(P<0.05).Large amounts of litter and heavy rainfall during the early growing season resulted in the highest PLFA contents for various microorganisms,whereas relatively low and stable levels were observed during other times.The dominant species during each period were bacteria.G+ or aerobic bacteria were the main bacterial populations,providing insights into the overall trends of soil bacterial PLFA contents.Due to the relative accumulation of refractory substances during the later stages of litter decomposition,the effects of fungi increased significantly.Overall,our findings demonstrate that the main factors influencing microbial communities were litter,rainfall,and soil field capacity.展开更多
The identities and concentrations of low-molecular-weight organic acids （LMWOAs） were determined by ion chromatography throughout a 20-m water column in Hongfeng Lake, China. The spatiotemporal variations of LMWOAs ...The identities and concentrations of low-molecular-weight organic acids （LMWOAs） were determined by ion chromatography throughout a 20-m water column in Hongfeng Lake, China. The spatiotemporal variations of LMWOAs and their contributions to dissolved organic matter （DOM） in a research period of 24 hr were also investigated. The results demonstrated that five LMWOAs （lactic, acetic, pyruvic, sorbic, oxalic acid） were detected, and their total concentration and proportion in DOC were 6.55 μmol/L and 7.47%. Their average levels were 2.50, 0.65, 2.35, 0.96 and 0.09 μmol/L, respectively. LMWOAs were higher during daytime （10：00-18：00 on Jun 13, 2008） than nighttime （21：00-6：00 the next morning）, in particular 4.99 μmol/L high in the epilimnion （ 1 m water depth）, reflecting the fact that direct import from terrigenous sources and photochemical production from humic materials were dominant during LMWOAs＇ origin and accumulation. The same factors caused LMWOAs to be 0.63 μmol/L in the epilimnion higher than in the hypolimnion. The rapid decrease of total organic acid （TOA） up until 18：00 mainly resulted from bio-uptake and mineralization in the hypolimnion （〉1 m water depth）. Pyruvic acid increased with time in the epilimnion and decreased in the hypolimnion, largely related to the two contrary processes of continuous degradation and synthesis of macromolecular organic matter during life materials＇ cycle mediated by organisms. Simultaneously, plankton behavior and thermal stratification played a pivotal role in LMWOAs＇ behavior in the water column, causing decreasing and increasing profiles. The distribution of LMWOAs represents an interesting resource for biogeochemical research of DOM in aquatic ecosystems.展开更多
Arsenic contamination from roxarsone in livestock manure is common,and livestock manure continuously accumulates in the open environment.Evaluations of the environmental processes of As mobilization and transformation...Arsenic contamination from roxarsone in livestock manure is common,and livestock manure continuously accumulates in the open environment.Evaluations of the environmental processes of As mobilization and transformation are critical for predicting the fate of As compounds after roxarsone degradation.In this study,spatiotemporal variations in As species and microbial community structure were characterized using laboratory column experiments with background soil collected from Yanggu County(northern Shandong Plain,China),a region of intense poultry production.Organic and inorganic arsenic were detected by high-performance liquid chromatography(HPLC)and HPLC with hydride generation atomic fluorescence spectrometry(HPLC-HG-AFS),respectively.High-throughput sequencing technology was used to describe microbial diversity.Results showed that roxarsone was transformed completely within 7 days,and A_(s)(Ⅲ)and As(Ⅴ)were the major degradation products.The concentration of A_(s)(Ⅲ)was much lower than that of As(Ⅴ).The A_(s)(Ⅲ)concentration increased significantly after Day 14,whereas the A_(s)(Ⅴ)concentration increased significantly after Day 84,indicating that A_(s)(Ⅲ)was initially produced.The microbial community structure changed significantly as roxarsone transformed into various As compounds.A critical and dominant bacterial strain,norank_f__Family_XVⅢ,was found to be related to the degradation of roxarsone into As(Ⅲ).This study improves our understanding of the fate of As species released from poultry litter to soil and groundwater,which is a threat to human health and environment.展开更多
Mangroves can not only provide multiple ecosystem service functions,but are also efficient carbon producers,capturers,and sinks.The estimation of the organic carbon accumulation rate(OCAR)in mangrove sediments is fund...Mangroves can not only provide multiple ecosystem service functions,but are also efficient carbon producers,capturers,and sinks.The estimation of the organic carbon accumulation rate(OCAR)in mangrove sediments is fundamental for elucidating the role of mangroves in the global carbon budget.In particular,understanding the past changes in the OCAR in mangrove sediments is vital for predicting the future role of mangroves in the rapidly changing environment.In this study,three dated sediment cores from interior and fringe of mangroves in the Yingluo Bay,China,were used to reconstruct the spatiotemporal variations of the calculated OCAR since 1900 in this area.The increasing OCAR in the mangrove interior was attributed to mangrove flourishment induced by climate change characterized by the rising temperature.However,in the mangrove fringe,the strengthening hydrodynamic conditions under the sea level rise were responsible for the decreasing OCAR,particularly after the1940 s.Furthermore,the duration of inundation by seawater was the primary factors controlling the spatial variability of the OCAR from the mangrove fringe to interior,while the strengthened hydrodynamic conditions after the 1940 s broke this original pattern.展开更多
The study of the heterogeneity of soil enzyme activities at different sampling locations in canopy gaps will help understand the influence mechanism of canopy gaps on soil ecological processes.In this paper,we analyze...The study of the heterogeneity of soil enzyme activities at different sampling locations in canopy gaps will help understand the influence mechanism of canopy gaps on soil ecological processes.In this paper,we analyzed the spatiotemporal variation of soil enzyme activities and soil physicochemical properties at different sampling locations(closed canopy,expanded edge,canopy edge,gap center)in different sampling time(December,February,April,June,August,and October)on the northern slope of the Tianshan Mountains,Northwest China.The results showed that soil catalase,cellulase,sucrase,and acid phosphatase activities were relatively high from June to October and low from December to April,and most of soil enzyme activities were higher at closed canopy than at gap center.Soil urease activity was high during December-February.The soil temperature reached the highest value during June-August and was relatively high at gap center in October,December,and February.Soil water content was significantly higher in December and April than in other months.Soil bulk density was higher at gap center than at closed canopy in December.Soil pH and soil electrical conductivity in most months were higher at closed canopy than at gap center.Soil organic carbon,soil total nitrogen,and soil total phosphorus were generally higher at gap center than at closed canopy.Furthermore,sampling time played a leading role in the dynamic change of soil enzyme activity.The key factors affecting soil enzyme activity were soil temperature and soil water content,which were governed by canopy gaps.These results provide important support for further understanding the influence mechanism of forest ecosystem management and conservation on the Tianshan Mountains.展开更多
In order to realize the spatiotemporal variations of benthic macrofaunal communities at the"Amphioxus Sand"habitat,six surveys including four seasons and three consecutive summers(i.e.,2014,2015 and 2016)wer...In order to realize the spatiotemporal variations of benthic macrofaunal communities at the"Amphioxus Sand"habitat,six surveys including four seasons and three consecutive summers(i.e.,2014,2015 and 2016)were conducted in two core sites,i.e.,Huangcuo(HC)and Nanxian-Shibaxian(NX),in the Xiamen Amphioxus Nature Reserve in China.A total of 155 species of macrofauna were recorded,therein,polychaetes were dominant in terms of species number and density.Significant spatiotemporal variations of macrofaunal communities were observed.The density of polychaetes and the biomass of molluscs in the HC site were higher than those in the NX site.Macrofauna were more diverse and abundant in the cold seasons(winter and spring)than that in the warm seasons(summer and autumn).The annual variations of macrofaunal communities may be attributed to the changes in sediment texture among the three years of the survey.The variations in macrofaunal communities were mainly related to the proportion of polychaetes within the community.In addition,the density of amphioxus(include Branchiostoma japonicum and B.belcheri)was negatively correlated to that of polychaetes,bivalves,and crustaceans.Amphioxus was less likely to be found in the sediments with higher silt and clay content.Five biotic indices including Margaref’s richness index(d),Peilou’s evenness index(J′),Shannon-Wiener diversity index(H′),AMBI and M-AMBI were calculated in the present study.AMBI seems suitable in assessing benthic health at the"Amphioxus Sand"habitat,and a potential risk of ecological health in Xiamen Amphioxus Nature Reserve should be aware.展开更多
Spatiotemporal variations of anthropogenic heat flux(AHF)is reported to be associated with global warming.However,confined to the low spatial resolution of energy consumption statistical data,details of AHF was not we...Spatiotemporal variations of anthropogenic heat flux(AHF)is reported to be associated with global warming.However,confined to the low spatial resolution of energy consumption statistical data,details of AHF was not well descripted.To obtain high spatial resolution data of AHF,Defense Meteorological Satellite Program/Operational Linescan System(DMSP/OLS)nighttime light time-series product and Moderate Resolution Imaging Spectroradiometer(MODIS)satellite monthly normalized difference vegetation index(NDVI)product were applied to construct the human settlement index.Based on the spatial regression relationship between human settlement index and energy consumption data.A 1-km resolution dataset of AHF of 12 selected cities in the eastern China was obtained.Ordinary least-squares(OLS)model was applied to detect the mechanism of spatial patterns of AHF.Results showed that industrial emission in selected cities of the eastern China was accountable for 63%of the total emission.AHF emission in megacities,such as Tianjin,Jinan,Qingdao,and Hangzhou,was most significant.AHF increasing speed in most areas in the chosen cities was quite low.High growth or extremely high growth of AHF were located in central downtown areas.In Beijing,Shanghai,Guangzhou,Jinan,Hangzhou,Changzhou,Zhaoqing,and Jiangmen,a single kernel of AHF was observed.Potential influencing factors showed that precipitation,temperature,elevation,normalized different vegetation index,gross domestic product,and urbanization level were positive with AHF.Overall,this investigation implied that urbanization level and economic development level might dominate the increasing of AHF and the spatial heterogeneousness of AHF.Higher urbanization level or economic development level resulted in high increasing speeds of AHF.These findings provide a novel way to reconstruct of AHF and scientific supports for energy management strategy development.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.42027804,41775026,and 41075012)。
文摘Cirrus clouds play a crucial role in the energy balance of the Earth-atmosphere system.We investigated the spatiotemporal variations of cirrus over the South China Sea(SCS)using satellite data(MOD08,MYD08,CALIPSO)and reanalysis data(MERRA-2)from March 2007 to February 2015(eight years).The horizontal distribution reveals lower cirrus fraction values in the northern SCS and higher values in the southern region,with minima observed in March and April and maxima sequentially occurring in August(northern SCS,NSCS),September(middle SCS,MSCS),and December(southern SCS,SSCS).Vertically,the cirrus fraction peaks in summer and reaches its lowest levels in spring.Opaque cirrus dominates during summer in the NSCS and MSCS,comprising 53.6%and 55.9%,respectively,while the SSCS exhibits a higher frequency of opaque cirrus relative to other cloud types.Subvisible cirrus clouds have the lowest frequency year-round,whereas thin cirrus is most prominent in winter in the NSCS(46.3%)and in spring in the MSCS(45.3%).A case study from September 2021 further explores the influence of ice crystal habits on brightness temperature(BT)over the SCS.Simulations utilizing five ice crystal shapes from the ARTS DDA(Atmospheric Radiative Transfer Simulator Discrete Dipole Approximation)database and the RTTOV 12.4 radiative transfer model reveal that the 8-column-aggregate shape best represents BT in the NSCS and SSCS,while the large-block-aggregate shape performs better in the SSCS.
文摘Benzene,toluene,ethylbenzene,and xylene(BTEX)pollution poses a serious threat to public health and the environment because of its respiratory and neurological effects,carcinogenic properties,and adverse effects on air quality.BTEX exposure is a matter of grave concern in India owing to the growing vehicular and development activities,necessitating the assessment of atmospheric concentrations and their spatial variation.This paper presents a comprehensive assessment of ambient concentrations and spatiotemporal variations of BTEX in India.The study investigates the correlation of BTEX with other criteria pollutants andmeteorological parameters,aiming to identify interrelationships and diagnostic indicators for the source characterization of BTEX emissions.Additionally,the paper categorizes various regions in India according to the Air Quality Index(AQI)based on BTEX pollution levels.The results reveal that the northern zone of India exhibits the highest levels of BTEX pollution compared to central,eastern,and western regions.In contrast,the southern zone experiences the least pollution with BTEX.Seasonal analysis indicates that winter and postmonsoon periods,characterized by lower temperatures,are associated with higher BTEX levels due to the accumulation of localized emissions.When comparing the different zones in India,high traffic emissions and localized activities,such as solvent use and solvent evaporation,are found to be the primary sources of BTEX.The findings of the current study aid in source characterization and identification,and better understanding of the region’s air quality problems,which helps in the development of focused BTEX pollution reduction and control strategies.
文摘To investigate the characteristics of water environmental pollution in the Nenjiang River Basin,five monitoring sections,including Zhenxi,Xianghai Reservoir,Baishatan,Yuelianghu Reservoir,and Da an,were selected.Utilizing water quality monitoring data collected from 2013 to 2022,the fuzzy comprehensive evaluation method was employed to systematically analyze the spatiotemporal variation patterns of water quality,assess the current pollution status,and identify the influencing factors of non-point source pollution.The results indicated that the concentrations of representative pollutants at five sections in the lower reaches of the Nenjiang River generally exhibited a downward trend,accompanied by an overall improvement in water quality.However,the degree of improvement varied considerably among the different sections.Specifically,the water quality of the main stream of the Nenjiang River(Baishatan and Da an)improved from Class IV to Class III.In contrast,the Xianghai Reservoir consistently remained at Class V or below,primarily due to excessive fluoride levels.The water quality at Yuelianghu Reservoir and Heidimiao Section demonstrated a fluctuating but overall improving trend.Based on the analysis of pollution sources,targeted recommendations are proposed,including regulating the ecological water requirements of rivers,restoring wetland ecosystems,and enhancing the management of non-point source pollution.These measures offer scientific support for water quality management and ecological conservation in the river basins.
基金supported by the National Natural Science Foundation of China(No.42327806)the National Key R&D Program of China(No.2022YFC3703500)+4 种基金Zhejiang Province“Lingyan”Research and Development Project(No.2022C03073)Zhejiang Provincial Natural Science Foundation of China(No.LQ23B070009)China Postdoctoral Science Foundation(No.2023M743763)Zhejiang Provincial Postdoctoral Research Excellence Funding Project(No.ZJ2023144)Shaoxing Science and Technology Plan Project(No.2022B41006).
文摘Methane(CH_(4))is the second greenhouse gas and has a profound impact on global climate change due to its high global warming potential and concentration.By 2022,the CH_(4)concentration was approximately 1.9 ppm,which was 264%of the pre-industrial level.The spatiotemporal distribution of CH_(4)was investigated by a portable CH_(4)detector on an unmanned aerial vehicle and electric bicycles in Shaoxing,a city situated in the Yangtze River Delta,China.The vertical distribution revealed CH_(4)concentration generally decreased slowly with height.However,the inversion condition and low atmospheric boundary layer height(ABLH)leaded to the enhancement of CH_(4)with height.The highest CH_(4)concentration(2.2±0.1 ppm,n=1428)was observed in winter and the lowest(2.0±0.2 ppm,n=1530)in spring.Regarding the daily variation,CH_(4)concentration peaked at 5:00 local time(LT)and reached its lowest level at 14:00 LT,which was attributed to the daily variation of ABLH,lowest in the early morning and highest in the noon.In urban areas,CH_(4)concentrations showed higher levels near restaurants,natural gas stations and sewerage well,with a maximum value of 13.1 ppm,which was caused by CH_(4)emission and natural gas leakage from these places.The annual CH_(4)emission in Shaoxing were estimated to be approximately 69 ton/(km^(2)·year)by the mass balance approach.Compared with other cities in the world,the CH_(4)emission is in higher level which imply some control measures should be conducted to reduce CH_(4)emission in Shaoxing.
基金Supported by the National Key R&D Program of China(No.2018YFC1406202)the National Natural Science Foundation of China(Nos.41830964,41976188,41605051)。
文摘As in-situ observations are sparse,targeted observations of a specific mesoscale eddy are rare.Therefore,it is difficult to study the three-dimensional structure of moving mesoscale eddies.From April to September 2014,an anticyclonic eddy located at 135°E-155°E,26°N-42°N was observed using 17 rapidsampling Argo floats,and the spatiotemporal variations in the three-dimensional structure were studied.The results are as follows:(1)the eddy was identified and tracked using satellite altimeter data.It had a lifetime of 269 days and an average radius of 91.5 km.The lifetime of the eddy can be divided into three phases,i.e.,the initiation,maturity,and termination phases.The depth of its influence reached 1000 m;(2)the Argo profiles were divided into seven periods(approximately 20 days in each)for composite analysis,and the composite Argo profiles and CARS2009(CSIRO Atlas of Regional Seas)climatology data were merged following the data-interpolating variational analysis(DIVA)method to reconstruct the three-dimensional structure.The temperature and salinity anomaly cores of the anticyclonic mesoscale eddy are located from 400 to 600 m.From 800 to 900 m,there is an area of low salinity at the center of the eddy.A high concentration anomaly of dissolved oxygen was located at approximately 250 m;(3)to better understand the features of the eddy and its interaction with the surroundings,we calculated the anomalous velocity of the geostrophic flow and the heat,salt,dissolved oxygen transport anomaly,and discussed the eddy's origin and its adjustments to topography.The maximum heat,salt,and oxygen transport caused by eddy were 9.37×10^11 W,3.08×10^3 kg/s,and 2.70×10^2 kg/s,which all occurred during the termination phase.This study highlights the applicability of using Argo floats to understand the three-dimensional structure thermohaline features of eddies in the North Pacific.
基金Research on the key technology of effectiveness evaluation and standardized construction of National Nature Reserve,No.201209028"Strategic Priority Research Program–Climate Change:Carbon Budget and Relevant Issues"of the Chinese Academy of Sciences,No.XDA05050600Key Projects in the National Science&Technology Pillar Program during the Twelve Five-year Plan Period,No.2013BAC03B03
文摘Photosynthetically active radiation （PAR） is the energy source of plant photosyn thesis, and the diffuse component can enhance canopy light use efficiency, thereby increasing the carbon uptake. Therefore, diffuse PAR is an important driving factor of ecosystem productivity models. In this study, we estimated the diffuse PAR of over 700 meteorological sites in China from 1981 to 2010 using an empirical model based on observational data from Chinese Ecosystem Research Network （CERN） and China Meteorology Administration. Then we derived the spatial data set of 10 km monthly diffuse PAR using ANUSPLIN software, and analyzed the spatiotemporal variation characteristics of diffuse PAR through GIS and trend analysis techniques. The results showed that： （1） The spatial patterns of annual average diffuse PAR during 1981-2010 are heterogeneous across China, lower in the northeast and higher in the west and south. The nationwide average value for 30 years ranges from 6.66 mol m-2 d-1 to 15.27 mol m-2 d-1, and the value in summer is the biggest while the value in winter is the smallest. （2） There is an evident increasing trend of annual diffuse PAR during recent 30 years, with the increasing amplitude at 0.03 mol m-2 d-l/10a. But a significant declining trend is shown in the first 10 years, and obvious anomalies can be seen in 1982, 1983, 1991 and 1992. And there is a downtrend in spring and an uptrend in all the other seasons. （3） The spatial distribution of temporal variation rates of diffuse PAR is inhomogeneous across the country, generally decreasing in the north and increasing in the south.
基金This research was supported by the National Natural Science Foundation of China(41961029)the Gansu Construction Science and Technology Soft Science Project of China(JK2022-16).
文摘Rapid industrialization and urbanization have led to the most serious habitat degradation in China,especially in the loess hilly area of the Yellow River Basin,where the ecological environment is relatively fragile.The contradiction between economic development and ecological environment protection has aroused widespread concern.In this study,we used the habitat quality of Integrated Valuation of Ecosystem Services and Tradeoffs(InVEST-HQ)model at different scales to evaluate the dynamic evolution characteristics of habitat quality in Lanzhou City,Gansu Province of China.The spatiotemporal variations of habitat quality were analyzed by spatial autocorrelation.A Geographical Detector(Geodetector)model was used to explore the driving factors that influencing the spatial differentiation of habitat quality,including natural factors,socio-economic factors,and ecological protection factors.The results showed that the habitat quality index of Lanzhou City decreased from 0.4638 to 0.4548 during 2000-2018.The areas with reduced the habitat quality index were mainly located in the Yellow River Basin and Qinwangchuan Basin,where are the main urban areas and the new economic development areas,respectively.The spatial distribution of habitat quality presented a trend of high in the surrounding areas and low in the middle,and showed a significant positive spatial autocorrelation.With the increase of study scale,the spatial distribution of habitat quality changed from concentrated to dispersed.The spatial differentiation of habitat quality in the study area was the result of multiple factors.Among them,topographic relief and slope were the key factors.The synergistic enhancement among these driving factors intensified the spatial differentiation of habitat quality.The findings of this study can provide a scientific basis for land resources utilization and ecosystem restoration in the arid and semi-arid land.
基金Supported by the Public Science and Technology Research Funds Projects of Ocean(No.201205009)
文摘The process of habitat degradation varies in habitat type and driving force which shows certain spatial and temporal heterogeneity on regional scales. In the present study, a new diagnostic model for enclosed bay habitat degradation was established, with which the spatial and temporal variation patterns of habitat degradation during 1991–2012 in Sansha Bay, Fujian, China was investigated. The results show that anthropogenic disturbance is the major controlling factor for the habitat degradation in large temporal heterogeneity in the bay. On the other hand, the habitat degradation experienced signifi cant spatial variations among six sub-bays. Under the joint action of temporal and spatial heterogeneity, the degradation trend in growing scale shows a more signifi cant correlation with the distribution of local leading industries along shorelines. Therefore, we quantifi ed the main characters of habitat degradation in Sansha Bay, and have understood the relationship between the status of habitats spatio-temporal variation value and the main controlling factor leading to the changes. However, a defi ciency of this research is the lack of or inaccessible to the detailed data, which shall be better solved in the future study for accessing more data from more sources.
基金supported by the Global Change Research Program of China (No. 2010CB951402)the Natural Science Foundation of China (Nos. 91025013, 91325202)+1 种基金the State Key Laboratory of Frozen Soil Engineering (No. SKLFSE-ZY-06), CAS, Chinathe Major Research Plan of the Natural Science Foundation of China (No. 2013CBA01802)
文摘Investigation on spatiotemporal variations of maximum seasonal freeze depth （MSFD） over the Heihe River Basin is of great importance for systematic understanding of regional climate and environmental change, ecological-hydrological processes, water resources assessment, construction and resource development. Based on soil and air temperatures at the meteorological stations of the China Meteorological Administration （CMA） over the Heihe River Basin, MSFDs time series are structured into a composite time series over the 1960-2007 period. Evaluating the averaged MSFD time series for 1960 2007 reveals a statistically significant trend of 4.0 cm/decade or a net change of-19.2 cm for the 48-year period over the basin. The MSFD had significantly negative correlation with mean annual air temperature （MAAT）, winter air temperature, mean annual ground surface temperature （MAGST）, degree days of thawing for the air （DDTa） as well as for the surface （DDTs）, and degree days of freezing for the surface （DDFs）. While there was significantly positive correlation between DDF,. and MSFD time series, MSFD was deeper and changed greatly in the Heihe River source area. It was shallower in the east-central basin and gradually deepened in other sections of the basin. The MSFD distribution pattern in 2003-2005 is consistent with that of averaged degree days of freezing for air （DDFa） in 1960-2007. However, the maximum of MSFD may not be accurate, because there is no long term observation data in the deep seasonally frozen ground regions near the lower boundary of permafrost. With increasing elevation, averaged DDFa increased at a rate of 51.6 ℃-day/100m, therefore, the MSFG and the date reaching MSFG became deeper and later, respectively.
基金The Strategic Priority Research Program of the Chinese Academy of Sciences under contract No.XDA11020201the National Basic Research Program of China under contract No.2013CB956101+2 种基金the Knowledge Innovation Program of the Chinese Academy of Sciences under con-tract No.SQ201302the National Science Foundation Council Grant of China under contract Nos 41430964,41406023 and 41025019the Chinese Academy of Sciences/State Administration of Foreign Experts Affairs International Partnership Program for Creative Research Teams and General Research Fund of Hong Kong Research Grants Council under contract No.CUHK402912
文摘On the basis of the QSCAT/NCEP blended wind data and simple ocean data assimilation （SODA）, the wind-induced near-inertial energy flux （NIEF） in the mixed layer of the South China Sea （SCS） is estimated by a slab model, and the model results are verified by observational data near the Xisha Islands in the SCS. Then, the spatial and temporal variations of the NIEF in the SCS are analyzed. It is found that, the monthly mean NIEF exhibits obvious spatial and temporal variabilities, i.e., it is large west of Luzon Island all the year, east of the Indo-China Peninsula all the year except in spring, and in the northern SCS from May to Septem- ber. The large monthly mean NIEF in the first two zones may be affected by the large local wind stress curl whilst that in the last zone is probably due to the shallow mixed layer depth. Moreover, the monthly mean NIEF is relatively large in summer and autumn due to the passage of typhoons. The spatial mean NIEF in the mixed layer of the SCS is estimated to be about 1.25 mW/m2 and the total wind energy input from wind is approximately 4.4 GW. Furthermore, the interannual variability of the spatial monthly mean NIEF and the Nifio3.4 index are negatively correlated.
基金funded by the National Natural Science Foundation of China(41971238)the Ministry of Education Humanities and Social Youth Foundation of China(19YJCZH144)+1 种基金the Natural Science Foundation of Shandong Province,China(ZR2019QD006)the National College Student Innovation Training Project(S202010446004).
文摘As an important natural resource,forest land plays a key role in the maintenance of ecological security.However,variations of forest land in the agropastoral ecotone of northern China(AENC)have attracted little attention.Taking the AENC as an example and based on remote-sensing images from 2000,2010 to 2020,we explored the spatiotemporal variation of forest land and its driving factors using the land-use transfer matrix,spatial autocorrelation analysis and spatial error model.The results showed that from 2000 to 2020,the total area of forest land in the AENC increased from 75,547.52 to 77,359.96 km^(2) and the changes were dominated by the transformations among forest land,grassland and cropland,which occurred mainly in areas with the elevation of 500-2000 m and slope of 15°-25°.There was obvious spatial agglomeration of forest land in the AENC from 2000 to 2020,with hot spots of forest land gathered in the southern marginal areas of the Yanshan Mountains and the low mountainous and hilly areas of the Loess Plateau.The sub-hot spots around hot spots moved southward,the sub-cold spots spread to the surrounding areas and the cold spots disappeared.The spatiotemporal variation of forest land resulted from the interactions of natural environment,socioeconomic and policy factors from 2000 to 2020.The variables of average annual precipitation,slope,terrain relief,ecological conversion program and afforestation policy for barren mountains affected the spatial pattern of forest land positively,while those of annual average temperature,slope and road network density influenced it negatively.
基金This research is supported jointly by the National Key R&D Program of China[grant numbers 2016YFA0602100 and 2018YFC1407104]the china Special Fund for Meteorological Research in the Public Interest[grant number GYHY201506011]the National Natural Science Foundation of China[grant number 41975134].
文摘The Los Alamos Sea-Ice Model(CICE)is one of the most popular sea-ice models.All versions of it have been the main sea-ice module coupled to climate system models.Therefore,evaluating their simulation capability is an important step in developing climate system models.Compared with observations and previous versions(CICE4.0 and CICE5.0),the advantages of CICE6.0(the latest version)are analyzed in this paper.It is found that CICE6.0 has the minimum interannual errors,and the seasonal cycle it simulates is the most consistent with observations.CICE4.0 overestimates winter sea-ice and underestimates summer sea-ice severely.Meanwhile,the errors of CICE5.0 in winter are larger than for the other versions.The main attention is paid to the perennial ice and the seasonal ice.The spatial distribution of root-mean-square errors indicates that the simulated errors are distributed in the Atlantic sector and the outer Arctic.Both CICE4.0 and CICE5.0 underestimate the concentration of the perennial ice and overestimate that of the seasonal ice in these areas.Meanwhile,CICE6.0 solves this problem commendably.Moreover,the decadal trends it simulates are comparatively the best,especially in the central Arctic sea.The other versions underestimate the decadal trend of the perennial ice and overestimate that of the seasonal ice.In addition,an index used to objectively describe the difference in the spatial distribution between the simulation and observation shows that CICE6.0 produces the best simulated spatial distribution.
基金This work was supported by the National Key Research and Development Program of China(Grant No.2016YFC0502203)the National Science Funds for Creative Research Groups of China(Grant No.51421006)the Key Program of the National Natural Science Foundation of China(Grant No.91647206).
文摘River hydrogeochemistry offers necessary guidance for effective water environmental management.However,the influence of cascade reservoirs on river hydrogeochemistry remains unknown.In this study,the Jinsha River,the headwaters of the Yangtze River of China,was selected to investigate the spatiotemporal variations of hydrogeochemistry after the construction of six cascade reservoirs.Major ions,total dissolved solids,electrical conductivity,and pH values of sampled water in the upper natural reaches and lower reservoir-regulated reaches were analyzed in both flood and dry seasons.The results of Piper diagram and Gibbs plots showed that the hydrogeochemistry of the Jinsha River was naturally controlled by both evaporation-crystallization and carbonate weathering processes,but it was also artificially affected by reservoirs.The impoundment of cascade reservoirs affected the hydrodynamic condition of the river.The river flow in the flood season was reduced by approximately 24.5%,altering the proportions of water sources and leading to notable hydrogeochemical alterations in reservoir-regulated reaches.Conversely,river hydrogeochemistry generally remained unchanged in the dry season,owing to the insignificant effect of cascade reservoirs on river flow.In contrast to what has been observed in previous studies of individual reservoirs,the cumulative influence of cascade reservoirs on the Jinsha River flow regime did not cause abrupt hydrogeochemical changes between the upstream and downstream areas of each reservoir.Moreover,the water quality assessments revealed that the impoundment of cascade reservoirs improved downstream irrigational water quality,with lower Naþratio values in the flood season.This study provides the earliest evaluation of cascade reservoir influence on the hydrogeochemistry of the Jinsha River.The findings of this study can be used as a reference for scientific guidelines for future environmental management of cascade reservoirs in large rivers.
基金This study was supported by the Science and Technology Basic Work Special(No 2014FY120700).
文摘Castanopsis fargesii is a good afforestation plants and various microorganisms play important roles in mediating the growth and ecological functions of this species.In this study,we evaluated changes in microbial communities in soil samples from C.fargesii forests.The phospholipid fatty acid(PLFA)biomarker method was used to obtain bacteria,fungi,actinomycetes,gram-positive bacteria(G?),gram-negative bacteria(G-),aerobic bacteria,and anaerobic bacteria to investigate spatiotemporal changes in microbial communities during the growing season.The results show that soil microorganisms were mainly concentrated in the upper 20-cm layer,demonstrating an obvious surface aggregation(P<0.05).Large amounts of litter and heavy rainfall during the early growing season resulted in the highest PLFA contents for various microorganisms,whereas relatively low and stable levels were observed during other times.The dominant species during each period were bacteria.G+ or aerobic bacteria were the main bacterial populations,providing insights into the overall trends of soil bacterial PLFA contents.Due to the relative accumulation of refractory substances during the later stages of litter decomposition,the effects of fungi increased significantly.Overall,our findings demonstrate that the main factors influencing microbial communities were litter,rainfall,and soil field capacity.
基金supported by the National Basic Research Program (973) of China (No.2008CB418200,2008CB418000)the National Natural Science Foundation of China (No.41003055, U0833603, 40632011,40873080)the Chinese Research Academy of Environmental Sciences (No.2007KYYW01)
文摘The identities and concentrations of low-molecular-weight organic acids （LMWOAs） were determined by ion chromatography throughout a 20-m water column in Hongfeng Lake, China. The spatiotemporal variations of LMWOAs and their contributions to dissolved organic matter （DOM） in a research period of 24 hr were also investigated. The results demonstrated that five LMWOAs （lactic, acetic, pyruvic, sorbic, oxalic acid） were detected, and their total concentration and proportion in DOC were 6.55 μmol/L and 7.47%. Their average levels were 2.50, 0.65, 2.35, 0.96 and 0.09 μmol/L, respectively. LMWOAs were higher during daytime （10：00-18：00 on Jun 13, 2008） than nighttime （21：00-6：00 the next morning）, in particular 4.99 μmol/L high in the epilimnion （ 1 m water depth）, reflecting the fact that direct import from terrigenous sources and photochemical production from humic materials were dominant during LMWOAs＇ origin and accumulation. The same factors caused LMWOAs to be 0.63 μmol/L in the epilimnion higher than in the hypolimnion. The rapid decrease of total organic acid （TOA） up until 18：00 mainly resulted from bio-uptake and mineralization in the hypolimnion （〉1 m water depth）. Pyruvic acid increased with time in the epilimnion and decreased in the hypolimnion, largely related to the two contrary processes of continuous degradation and synthesis of macromolecular organic matter during life materials＇ cycle mediated by organisms. Simultaneously, plankton behavior and thermal stratification played a pivotal role in LMWOAs＇ behavior in the water column, causing decreasing and increasing profiles. The distribution of LMWOAs represents an interesting resource for biogeochemical research of DOM in aquatic ecosystems.
基金This research was funded by National Natural Science Foundation of China(No.41907175 and 41902259)and China Geological Survey project(No.DD20190303).
文摘Arsenic contamination from roxarsone in livestock manure is common,and livestock manure continuously accumulates in the open environment.Evaluations of the environmental processes of As mobilization and transformation are critical for predicting the fate of As compounds after roxarsone degradation.In this study,spatiotemporal variations in As species and microbial community structure were characterized using laboratory column experiments with background soil collected from Yanggu County(northern Shandong Plain,China),a region of intense poultry production.Organic and inorganic arsenic were detected by high-performance liquid chromatography(HPLC)and HPLC with hydride generation atomic fluorescence spectrometry(HPLC-HG-AFS),respectively.High-throughput sequencing technology was used to describe microbial diversity.Results showed that roxarsone was transformed completely within 7 days,and A_(s)(Ⅲ)and As(Ⅴ)were the major degradation products.The concentration of A_(s)(Ⅲ)was much lower than that of As(Ⅴ).The A_(s)(Ⅲ)concentration increased significantly after Day 14,whereas the A_(s)(Ⅴ)concentration increased significantly after Day 84,indicating that A_(s)(Ⅲ)was initially produced.The microbial community structure changed significantly as roxarsone transformed into various As compounds.A critical and dominant bacterial strain,norank_f__Family_XVⅢ,was found to be related to the degradation of roxarsone into As(Ⅲ).This study improves our understanding of the fate of As species released from poultry litter to soil and groundwater,which is a threat to human health and environment.
基金The National Natural Science Foundation of China under contract Nos 41976068 and 41576061。
文摘Mangroves can not only provide multiple ecosystem service functions,but are also efficient carbon producers,capturers,and sinks.The estimation of the organic carbon accumulation rate(OCAR)in mangrove sediments is fundamental for elucidating the role of mangroves in the global carbon budget.In particular,understanding the past changes in the OCAR in mangrove sediments is vital for predicting the future role of mangroves in the rapidly changing environment.In this study,three dated sediment cores from interior and fringe of mangroves in the Yingluo Bay,China,were used to reconstruct the spatiotemporal variations of the calculated OCAR since 1900 in this area.The increasing OCAR in the mangrove interior was attributed to mangrove flourishment induced by climate change characterized by the rising temperature.However,in the mangrove fringe,the strengthening hydrodynamic conditions under the sea level rise were responsible for the decreasing OCAR,particularly after the1940 s.Furthermore,the duration of inundation by seawater was the primary factors controlling the spatial variability of the OCAR from the mangrove fringe to interior,while the strengthened hydrodynamic conditions after the 1940 s broke this original pattern.
基金supported by the National Natural Science Foundation of China (31760142)
文摘The study of the heterogeneity of soil enzyme activities at different sampling locations in canopy gaps will help understand the influence mechanism of canopy gaps on soil ecological processes.In this paper,we analyzed the spatiotemporal variation of soil enzyme activities and soil physicochemical properties at different sampling locations(closed canopy,expanded edge,canopy edge,gap center)in different sampling time(December,February,April,June,August,and October)on the northern slope of the Tianshan Mountains,Northwest China.The results showed that soil catalase,cellulase,sucrase,and acid phosphatase activities were relatively high from June to October and low from December to April,and most of soil enzyme activities were higher at closed canopy than at gap center.Soil urease activity was high during December-February.The soil temperature reached the highest value during June-August and was relatively high at gap center in October,December,and February.Soil water content was significantly higher in December and April than in other months.Soil bulk density was higher at gap center than at closed canopy in December.Soil pH and soil electrical conductivity in most months were higher at closed canopy than at gap center.Soil organic carbon,soil total nitrogen,and soil total phosphorus were generally higher at gap center than at closed canopy.Furthermore,sampling time played a leading role in the dynamic change of soil enzyme activity.The key factors affecting soil enzyme activity were soil temperature and soil water content,which were governed by canopy gaps.These results provide important support for further understanding the influence mechanism of forest ecosystem management and conservation on the Tianshan Mountains.
基金The National Key Research and Development Program of China under contract No.2016YFC0502904the Public Science and Technology Research Funds Projects of Oceans under contract No.201305030。
文摘In order to realize the spatiotemporal variations of benthic macrofaunal communities at the"Amphioxus Sand"habitat,six surveys including four seasons and three consecutive summers(i.e.,2014,2015 and 2016)were conducted in two core sites,i.e.,Huangcuo(HC)and Nanxian-Shibaxian(NX),in the Xiamen Amphioxus Nature Reserve in China.A total of 155 species of macrofauna were recorded,therein,polychaetes were dominant in terms of species number and density.Significant spatiotemporal variations of macrofaunal communities were observed.The density of polychaetes and the biomass of molluscs in the HC site were higher than those in the NX site.Macrofauna were more diverse and abundant in the cold seasons(winter and spring)than that in the warm seasons(summer and autumn).The annual variations of macrofaunal communities may be attributed to the changes in sediment texture among the three years of the survey.The variations in macrofaunal communities were mainly related to the proportion of polychaetes within the community.In addition,the density of amphioxus(include Branchiostoma japonicum and B.belcheri)was negatively correlated to that of polychaetes,bivalves,and crustaceans.Amphioxus was less likely to be found in the sediments with higher silt and clay content.Five biotic indices including Margaref’s richness index(d),Peilou’s evenness index(J′),Shannon-Wiener diversity index(H′),AMBI and M-AMBI were calculated in the present study.AMBI seems suitable in assessing benthic health at the"Amphioxus Sand"habitat,and a potential risk of ecological health in Xiamen Amphioxus Nature Reserve should be aware.
基金Under the auspices of National Natural Science Foundation of China(No.41901219,41671430,41801326)Key Special Project for Introduced Talents Team of Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou)(No.GML2019ZD0301)。
文摘Spatiotemporal variations of anthropogenic heat flux(AHF)is reported to be associated with global warming.However,confined to the low spatial resolution of energy consumption statistical data,details of AHF was not well descripted.To obtain high spatial resolution data of AHF,Defense Meteorological Satellite Program/Operational Linescan System(DMSP/OLS)nighttime light time-series product and Moderate Resolution Imaging Spectroradiometer(MODIS)satellite monthly normalized difference vegetation index(NDVI)product were applied to construct the human settlement index.Based on the spatial regression relationship between human settlement index and energy consumption data.A 1-km resolution dataset of AHF of 12 selected cities in the eastern China was obtained.Ordinary least-squares(OLS)model was applied to detect the mechanism of spatial patterns of AHF.Results showed that industrial emission in selected cities of the eastern China was accountable for 63%of the total emission.AHF emission in megacities,such as Tianjin,Jinan,Qingdao,and Hangzhou,was most significant.AHF increasing speed in most areas in the chosen cities was quite low.High growth or extremely high growth of AHF were located in central downtown areas.In Beijing,Shanghai,Guangzhou,Jinan,Hangzhou,Changzhou,Zhaoqing,and Jiangmen,a single kernel of AHF was observed.Potential influencing factors showed that precipitation,temperature,elevation,normalized different vegetation index,gross domestic product,and urbanization level were positive with AHF.Overall,this investigation implied that urbanization level and economic development level might dominate the increasing of AHF and the spatial heterogeneousness of AHF.Higher urbanization level or economic development level resulted in high increasing speeds of AHF.These findings provide a novel way to reconstruct of AHF and scientific supports for energy management strategy development.
