The characteristics of summertime raindrop size distribution(DSD) and associated relations in the semi-arid region over the Inner Mongolian Plateau(IMP) were investigated,utilizing five-year continuous observations by...The characteristics of summertime raindrop size distribution(DSD) and associated relations in the semi-arid region over the Inner Mongolian Plateau(IMP) were investigated,utilizing five-year continuous observations by a PARSIVEL2disdrometer in East Ujimqin County(EUC),China.It is found that only 7.94% of the 15 664 one-min precipitation samples meet classification criteria as convective rain(CR),but its contribution to the total rainfall amount is 63.87%.Notably,40.72% of the rainfall comes from large-sized raindrops(D> 3 mm),despite the fact that large-sized raindrops account for only 1.73% of the CR total number concentration.Further results show that the mean value of mass-weighted mean diameters(Dm) is larger(2.43 mm) and generalized intercepts(lgN_(W)) is lower(3.19) in CR,aligning with a "continentallike" cluster,which is mainly influenced by the joint impact of in-cloud ice-based processes and the below-cloud environmental background.Also,the empirical relationships of shape-slope(μ-Λ),radar reflectivity-rain rate(Z-R),and rainfall kinetic energy(KE_(time)-Rand KE_(time)-Z) are localized.To quantitatively analyze the impact of DSD parameters on kinetic energy estimation,power-law KE_(time)-R and KE_(time)-Z relationships are derived based on the normalized gamma distribution.N_(W)takes precedence over μ in affecting variabilities of multiplicative coefficients,especially for KE_(time)-R relationship where the multiplicative coefficient is proportional to N_(W)^(-0.287).It should be noted that although the proportion of CR occurring throughout the summer is small,raindrops with lower N_(W) and larger Dmwill generate higher KE_(time),which will bring a higher potential risk of soil erosion in semi-arid regions over IMP.展开更多
Let I be the set of all infinitely divisible random variables with finite second moments,I_(0)={X∈I;Var(X)>0},P_(I)=inf_(x∈I)P{|X-E[X]|≤√Var(X)}and P_(I_(0))=inf P{|X-E[X]|<√Var(X)}.Firstly,we prove that P_...Let I be the set of all infinitely divisible random variables with finite second moments,I_(0)={X∈I;Var(X)>0},P_(I)=inf_(x∈I)P{|X-E[X]|≤√Var(X)}and P_(I_(0))=inf P{|X-E[X]|<√Var(X)}.Firstly,we prove that P_(I)≥P_(I_(0))>0.Secondly,we find_(x∈I_(0))the exact values of inf P{|X-E[X]|≤√Var(X)}and inf P{|X-E[X]|<√Var(X)}for the cases that J is the set of all geometric random variables,symmetric geometric random variables,Poisson random variables and symmetric Poisson random variables,respectively.As a consequence,we obtain that P_(I)≤e^(-1)^(∞)∑_(k=0)1/2^(2k)(k!)^(2)≈0.46576 and P_(I_(0))≤e^(-1)≈0.36788.展开更多
The distributions of light and nitrogen within a plant's canopy reflect the growth adaptation of crops to the environment and are conducive to improving the carbon assimilation ability.So can the yield in crop pro...The distributions of light and nitrogen within a plant's canopy reflect the growth adaptation of crops to the environment and are conducive to improving the carbon assimilation ability.So can the yield in crop production be maximized by improving the light and nitrogen distributions without adding any additional inputs?In this study,the effects of different nitrogen application rates and planting densities on the canopy light and nitrogen distributions of two highyielding maize cultivars(XY335 and DH618)and the regulatory effects of canopy physiological characteristics on radiation use efficiency(RUE)and yield were studied based on high-yield field experiments in Qitai,Xinjiang Uygur Autonomous Region,China,during 2019 and 2020.The results showed that the distribution of photosynthetically active photon flux density(PPFD)in the maize canopy decreased from top to bottom,while the vertical distribution of specific leaf nitrogen(SLN)initially increased and then decreased from top to bottom in the canopy.When SLN began to decrease,the PPDF values of XY335 and DH618 were 0.5 and 0.3,respectively,corresponding to 40.6 and49.3%of the total leaf area index(LAI).Nitrogen extinction coefficient(K_(N))/light extinction coefficient(K_(L))ratio in the middle and lower canopy of XY335(0.32)was 0.08 higher than that of DH618(0.24).The yield and RUE of XY335(17.2 t ha^(-1)and 1.8g MJ^(-1))were 7.0%(1.1 t ha^(-1))and 13.7%(0.2 g MJ^(-1))higher than those of DH618(16.1 t ha^(-1)and 1.6 g MJ^(-1)).Therefore,better light conditions(where the proportion of LAI in the upper and middle canopy was small)improved the light distribution when SLN started to decline,thus helping to mobilize the nitrogen distribution and maintain a high K_(N)and K_(N)/K_(L)ratio.In addition,K_(N)/K_(L)was a key parameter for yield improvement when the maize nutrient requirements were met at 360 kg N ha^(-1).At this level,an appropriately optimized high planting density could promote nitrogen utilization and produce higher yields and greater efficiency.The results of this study will be important for achieving high maize yields and the high efficiency cultivation and breeding of maize in the future.展开更多
The Chinese tree shrew has gained prominence as a model organism due to its phylogenetic proximity to primates,offering distinct advantages over traditional rodent models in biomedical research.However,the neuroanatom...The Chinese tree shrew has gained prominence as a model organism due to its phylogenetic proximity to primates,offering distinct advantages over traditional rodent models in biomedical research.However,the neuroanatomy of this species remains insufficiently defined,limiting its utility in neurophysiological and neuropathological studies.In this study,immunofluorescence microscopy was employed to comprehensively map the distribution of three calciumbinding proteins,parvalbumin,calbindin D-28k,and calretinin,across the tree shrew cerebrum.Serial brain sections in sagittal,coronal,and horizontal planes from 12 individuals generated a dataset of 3638 cellular-resolution images.This dataset,accessible via Science Data Bank(https://doi.org/10.57760/sciencedb.23471),provides detailed region-and laminar-selective distributions of calcium-binding proteins valuable for the cyto-and chemoarchitectural characterization of the tree shrew cerebrum.This resource will not only advance our understanding of brain organization and facilitate basic and translational neuroscience research in tree shrews but also enhance comparative and evolutionary analyses across species.展开更多
A double-moment cloud microphysics scheme requires an assumption for cloud droplet size distributions(DSDs).However,since observations of cloud DSDs are limited,default values for shape parameters and cloud condensati...A double-moment cloud microphysics scheme requires an assumption for cloud droplet size distributions(DSDs).However,since observations of cloud DSDs are limited,default values for shape parameters and cloud condensation nuclei activation parameters are often used in numerical simulations.In this study,the effects of cloud DSDs on numerical simulations of warm stratiform precipitation around Tokyo are investigated using the Japan Meteorological Agency's non-hydrostatic model,which incorporates a double-moment cloud microphysics scheme.Simulations using the default cloud DSD showed higher cloud droplet number concentrations and lower radar reflectivity than observed data,suggesting that the default cloud DSD is too narrow.Simulations with a cloud DSD based on in situ cloud observations corrected these errors.In addition,observation-based cloud DSDs affected rainfall amounts through the autoconversion rate of cloud water and improved the threat scores.These results suggest that realistic cloud DSDs should be provided for double-moment cloud microphysics schemes in scientific studies.展开更多
Geochemical surveys are essential for understanding the spatial distribution of ore-forming elements.However,these surveys often involve compositional data,the weight concentrations,which do not meet the requirements ...Geochemical surveys are essential for understanding the spatial distribution of ore-forming elements.However,these surveys often involve compositional data,the weight concentrations,which do not meet the requirements of statistical methods due to the closure effect.In this study,we applied an integrated approach combining compositional data,multifractal,and multivariate statistical analyses to identify the nonlinear complexity of the spatial distributions of elemental concentrations in the Er’renshan ore field.Initially,the raw concentrations were transformed into log-ratios following the principles of composition data theory to alleviate the impact of the closure effect.Multifractal analysis was then conducted to characterise the nonlinear complexity of the concentration distributions.Furthermore,principal component analysis(PCA)and factor analysis(FA)were applied to identify spurious correlations and the potential factors controlling the distribution patterns.The results demonstrate that:a)the raw data are biased,while the log-ratio data are unbiased and more reliable;b)the spatial distributions of elemental concentrations exhibit nonlinear complexity;and c)the elemental distribution in the study area is largely controlled by structural factors.展开更多
Using the ERA5 wave reanalysis,the distributions and trends of global available wave energy storage during 1980−2019 are analyzed.The results show that the available wave energy storage is not only related to total wa...Using the ERA5 wave reanalysis,the distributions and trends of global available wave energy storage during 1980−2019 are analyzed.The results show that the available wave energy storage is not only related to total wave energy storage but is also affected by the local available wave probability.Different distributions and trends between the available wave energy and total wave energy storage are observed.Larger values of total wave energy storage are concentrated in the high-latitude westerlies zone,whereas available wave energy storage exhibits greater concentration in the middle-low latitude regions.In each basin,there is a notable upward trend in both total wave energy storage and available wave energy storage.However,the northern Hemisphere(NH)exhibits an increasing trend in available wave probability,whereas the southern Hemisphere(SH)experiences a decreasing trend.This divergence contributes to the spatial distributions of available wave energy storage becoming increasingly uniform.These trends in wave energy are primarily influenced by changes in significant wave height.Although the increasing trend of significant wave height across all frequency ranges induces the growth of total wave energy storage,only the increasing of wave heights falling in 1.3−4 m can cause the growth of available wave energy storage.The consistent increasing rates of wave height under different mean levels contribute to the divergent trends in available wave probability.展开更多
The Yarlung Tsangpo River(YTR),located in the Himalayan orogenic belt,is renowned for its deep gorges and complex tectonic features,as well as its reputation as a landslide-prone region.However,less is known about the...The Yarlung Tsangpo River(YTR),located in the Himalayan orogenic belt,is renowned for its deep gorges and complex tectonic features,as well as its reputation as a landslide-prone region.However,less is known about the distribution of landslides across the entire river basin.To address this gap in knowledge,this study first established a comprehensive landslide inventory across the entire basin using remote sensing mapping and multiple field investigations.Then,a systematic analysis of the spatial and size distributions was conducted.The results indicated that the YTR basin features at least 2390 landslides with areas exceeding 104 m2,spanning a total area and volume of 1087.6 km^(2) and 48.4 km^(3),respectively.These landslides can be classified into eight types,and rockslides are the most common(53.1%).Their distributions are highly asymmetric,with the following notable patterns:(1)the Tsangpo suture zone(53.4%)contains a greater number of landslides than other tectonic units;(2)the landslide size is influenced by the relief and elevation conditions,with positive relationships observed between the local relief and landslide area,as well as between the elevation range and landslide area;and(3)the landslide distribution is not significantly correlated with rainfall,and seasonally frozen ground is associated with a greater concentration of landslides.Alternating slate and shale groups in the Tsangpo suture zone may be the factors responding to landslide concentration.A total of 20.6%of landslide-blocked rivers were observed,with some forming river knickpoints.Due to the limited data,spatial and size analyses are perhaps immature,and further systematic analysis remains necessary.展开更多
A new principle for grounding fault feeder detection based on negative sequence current variation and energy dissipated in the fault point is presented. It has high precision in both isolated systems and resonance ear...A new principle for grounding fault feeder detection based on negative sequence current variation and energy dissipated in the fault point is presented. It has high precision in both isolated systems and resonance earthed systems, even in full compensated systems. And it can be installed at the local control unit of feeder in distribution automation systems, such as field terminal unit (FTU). This principle is verified by EMTP simulator and experimentation.展开更多
The distributions and seasonal variations of total dissolved inorganic arsenic （TDIAs, [TDIAs] = [As^5＋]＋[As^3＋]） and arsenite （As3.） in the Yellow Sea and East China Sea are presented hero based on the observa...The distributions and seasonal variations of total dissolved inorganic arsenic （TDIAs, [TDIAs] = [As^5＋]＋[As^3＋]） and arsenite （As3.） in the Yellow Sea and East China Sea are presented hero based on the observations of 9 cruises carried out in 2000 - 2003. The study area covers a broad range of hydrographic and chemical properties. The emphasis is put on a southeast transect from Changjiang Estuary to the Ryukyu Islands （i.e. PN section） in the East China Sea to discuss the impact of terrestdal input on the marginal seas of China. Arsenic species （TDlAs and arsenite） are determined by selective hydride generation - atomic fluorescence spectrometry （HG-AFS）. TDIAs concentrations were high in the coastal area of Changjiang Estuary and decreased slightly towards the shelf region. High concentratiOns of TDIAs were also existed in the near bottom layer of shelf edge of the East China Sea which indicated another source of arsenic from the incursion of Kuroshio Waters. The seasonal variations of TDIAs in the study area depend on the hydrographic stages of Changjiang and the incursion intensity of Kuroshio Waters. Arsenite showed opposite distributions with TDIAs, with higher concentrations appeared at the surface layer of shelf region, which was positive correlated with the chlorophyll a. Biological conversion of arsenate into arsenite was hypothesized for the observed distribution pattern and its seasonal variations. The stoichoimetric ratios of As to P were estimated to be about 2×10^3 at PN Section in summer. The concentrations of dissolved arsenic in the Yellow Sea and East China Sea were comparable with other areas in the world.展开更多
A class of lifetime distributions, new better than equilibrium in expectation （NBEE）, and its dual, new worse than equilibrium in expectation （NWEE）, are studied based on the comparison of the expectations of life...A class of lifetime distributions, new better than equilibrium in expectation （NBEE）, and its dual, new worse than equilibrium in expectation （NWEE）, are studied based on the comparison of the expectations of lifetime X and its equilibrium Xo. The relationships of the NBEE （NWEE） and other lifetime distribution classes are discussed. It is proved that the NBEE is very large, and increasing failure rate （IFR）, new better than used （NBU） and the L class are its subclasses. The closure properties under two kinds of reliability operations, namely, convolution and mixture, are investigated. Furthermore, a Poisson shock model and a special cumulative model are also studied, in which the necessary and sufficient conditions for the NBEE （NWEE） lifetime distribution of the systems are established. In the homogenous Poisson shock model, the system lifetime belongs to NBEE（NWEE） if and only if the corresponding discrete failure distribution belongs to the discrete NBEE（NWEE）. While in the cumulative model, the system has an NBEE lifetime if and only if the stochastic threshold of accumulated damage is NBEE.展开更多
Value distributions of the general differential monomials is discussed.The following theorem is obtained:Let f be a transcendental meromorphic function in the plane,F=f n 0 (f (i) ) n i …(f (k) ) ...Value distributions of the general differential monomials is discussed.The following theorem is obtained:Let f be a transcendental meromorphic function in the plane,F=f n 0 (f (i) ) n i …(f (k) ) n k -c,n i≥1,c≠0 be a constant then (n 0-2)T(r,f)≤(r,1F)+S(r,f) when n 0】2;T(r,f)≤7(i+1)i( i) (r,1f)+(r,1F))+S(r,f) when n 0=1;T(r,f)≤7(N(r,1f)+(r,1F))+S(r,f) when n 0=0.展开更多
The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteri...The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.展开更多
Concentrations of polychlorinated biphenyls （PCBs） have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high res...Concentrations of polychlorinated biphenyls （PCBs） have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high resolution gas chromatography/high resolution mass spectrometry method. The concentration of PCBs ranged from 65.6 to 157 ng/g dry weight （dw）, with a mean value of 101 ng/g dw. The dioxin-like PCB WHO-TEQs （World Health Organization-Toxic Equivalents） of the sludge were lower than 1 pg /g dw. Consequently, all the concentrations of PCBs in sludge samples were below the upper limit for land application according to the Chinese legislation law for agriculture use. The PCB homologue profiles in sludge samples were dominated by tri-CBs and tetra- CBs. Similar distributions have been found in one of the Chinese PCB commercial products. The patterns of dioxin-like and indicator congeners observed in this study were quite similar in all samples. The predominant congener for dioxin-like and indicator PCBs were PCB-118 and PCB-28, respectively, while PCB-126 had the highest TEQ value.展开更多
The effects of neutral salt and alkali on the ion distribution were investigated in two alfalfa （Medicago sativa L.） cultivars, including Zhongmu 1, a high salt-tolerant cultivar, and Algonquin, a low salt-tolerant ...The effects of neutral salt and alkali on the ion distribution were investigated in two alfalfa （Medicago sativa L.） cultivars, including Zhongmu 1, a high salt-tolerant cultivar, and Algonquin, a low salt-tolerant cultivar. The alkali stress expressed more serious growth inhibition than the neutral salt stress at the same Na＋ concentration. Compared with Algonquin, Zhongmu 1 did not exhibit a higher alkali tolerance under the Na2CO3-NaHCO3 treatment with the low Na＋ concentration （50 mmol L-l）. The alkali increased the accumulation of Na＋, Ca2＋, and Mg2＋ in the root and changed the Ca2＋ and Mg2＋ balance in the entire alfalfa plant. The salt and alkali stresses decreased the K＋ and Fe3＋ contents of the roots and leaves, the root Mn2＋ content, and the shoot Zn2＋ content, but they increased the Fe3＋ accumulation of the shoots, the shoot and leaf Cu2＋ contents, and the leaf Zn2＋ content in both alfalfa cultivars. Based on the results obtained under the conditions of this experiment, we found that the salt and alkali stresses reduced the plant growth in both alfalfa cultivars, while the alkali caused a stronger stress than the neutral salt in alfalfa. Thus, we conclude that under hydroponic conditions, the deleterious effects of the alkali on plants are due to the distribution change of some trophic ion balance in the roots, shoots, and leaves of the plants by causing of Na＋, CO3^2-, and/or HCO3- stresses.展开更多
The effects of the component gradient distribution at interface and the fiber gradient distribution on the strength of cement-based materials were studied. The results show that the flexural strength and compressive s...The effects of the component gradient distribution at interface and the fiber gradient distribution on the strength of cement-based materials were studied. The results show that the flexural strength and compressive strength of the mortar and concrete with interface component and fiber gradient distributions are obviously improved. The strengthes of the fiber gradient distributed mortar and concrete (FGDM/C) are higher than those of fiber homogeneously distributed mortar and concrete (FHDM/C). To obtain the same strength, therefore, a smaller fiber volume content in FGDM/C is needed than that in FHDM/C. The results also show that the component gradient distribution of the concrete can be obtained by means of multi-layer vibrating formation.展开更多
Total suspended particulates （TSP） samples were collected using low pressure impactors （Andersen Series 20-800, USA） on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of ...Total suspended particulates （TSP） samples were collected using low pressure impactors （Andersen Series 20-800, USA） on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of size distributions and elemental compositions of particulate matter （PM） in different weather conditions. The concentrations of sixteen elements, including Na, Mg, Al, K, Ca, Mn, Fe, Ni, Cu, Zn, As, Se, Cd, Ba, T1 and Pb were detected using inductively coupled plasma mass spectrometry （ICP-MS）. The results showed that Ca, A1, Fe, Mg and Ba on foggy days were 2.0 2.6 times higher than on clear days, and 2.3-2.9 times higher than on hazy days. Concentrations of Cu, Zn, As, Se and Pb on foggy days were 163.5, 1186.7, 65.9, 32.0 and 708.2 ng m-3, respectively, in fine particles, and 68.1, 289.5, 19.8, 1.6 and 103.8 ng m-3, respectively, in coarse particles. This was 1.0~8.4 times higher and 1.4-7.4 times higher than on clear and hazy days, respectively. It is then shown that Mg, A1, Fe, Ca and Ba were mainly associated with coarse particles, peaking at 4.7~5.8 μm; that Cd, Se, Zn, As, T1 and Pb were most dominant in fine particles, peaking at 0.43-1.1 μm; and that Na, K, Ni, Cu and Mn had a multi-mode distribution, with peaks at 0.43-1.1 μm and 4.7-5.8 μm. The enrichment factors indicated that coal combustion along with vehicle and industry emissions may be the main sources of pollution elements.展开更多
Objective To determine the best statistical distribution of concentration data of major air pollutants in Shanghai. Methods Four types of theoretic distributions (lognormal, gamma, Pearson V and extreme value) were...Objective To determine the best statistical distribution of concentration data of major air pollutants in Shanghai. Methods Four types of theoretic distributions (lognormal, gamma, Pearson V and extreme value) were chosen to fit daily average concentration data of PM10, SO2 and NO2 from June 1, 2000 to May 31, 2003 in Shanghai by using the maximum likelihood method. The fit results were evaluated by Chi-square test. Results The best-fit distributions for PM10,SO2 and NO2 concentrations in Shanghai were lognormal, Pearson V, and extreme value distributions, respectively. Conclusion The results can be further applied to local air pollution prediction and control, e.g., the probabilities exceeding the air quality standard and emission source reduction of air pollutant concentration to meet the standard.展开更多
Aliphatic hydrocarbons （n-alkanes） associated with fine particulate matter were determined in the ambient air of urban, industrial and coastal areas in Tianjin, China, where intensive coal burning for industrial and...Aliphatic hydrocarbons （n-alkanes） associated with fine particulate matter were determined in the ambient air of urban, industrial and coastal areas in Tianjin, China, where intensive coal burning for industrial and domestic purpose takes place, n-Alkane homologues from C12 to C35 were quantifiable in all samples with C20-C31 being the most abundant species. Average concentrations of the total n-alkanes were 148.7, 250.1 and 842.0 ng/m3 in July, April and January, respectively. Seasonal variations were mainly attributed to ambient temperature changes and coal combustion for residential heating. Among the three studied areas, the highest levels of n-alkanes were observed in the industrial complex in winter and spring, but in summer the coastal alkane concentration moved up to the highest. A mono-modal distribution for n-alkanes was observed in spring and summer with odd carbon number predominance and a maximum centered at C27-C31, suggesting the release of plant wax into the atmosphere. The bimodal distribution with maxima at C22 and C26 observed in winter indicated a substantial influence of fossil fuel sources. All the CPIs （CPI1, CPI2, CPI3） values, varying between 0.64 and 1.97, indicated the influence of anthropogenic emissions on fine organic aerosols. The estimated contributions of plant wax to total n-alkanes were on average of 12.9%, 19.1% and 26.1% for winter, spring and summer, respectively.展开更多
For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide （SO2）, nitrogen oxides （NOx） and other pollutants to address the issues of poor air quality...For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide （SO2）, nitrogen oxides （NOx） and other pollutants to address the issues of poor air quality in Beijing. To investigate the effects of SO2 and NOx reductions on the particulate sulfate and nitrate concentrations as well as their size distributions, size-segregated aerosol samples were collected using micro-orifice uniform deposit impactors （MOUDIs） at urban and downwind rural sites in Beijing before and after full-scale controls. During the sampling period, the mass concentrations of fine particles （PMI.s） at the urban and rural sites were 94.0 and 85.9 p.g m-3, respectively. More than 90% of the sulfates and 60% of nitrates formed as fine particles. Benefiting from the advantageous meteorological conditions and the source controls, sulfates were observed in rather low concentrations and primarily in condensation mode during the Olympics. The effects of the control measures were separately analyzed for the northerly and the southerly air-mass-dominated days to account for any bias. After the control measures were implemented, PM, sulfates, and nitrates were significantly reduced when the northerly air masses prevailed, with a higher percentage of reduction in larger particles. The droplet mode particles, which dominated the sulfates and nitrates before the controls were implemented, were remarkably reduced in mass concentration after the control measures were implemented. Nevertheless, when the polluted southerly air masses prevailed, the local source control measures in Beijing did not effectively reduce the ambient sulfate concentration due to the enormous regional contribution from the North China Plain.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.42325503,42075063,42075066,and 42021004)the Hubei Provincial Natural Science Foundation and the Meteorological Innovation and Development Project of China(Grant No.2023AFD096)the Beijige Foundation of NJIAS(Grant No.BJG202304).
文摘The characteristics of summertime raindrop size distribution(DSD) and associated relations in the semi-arid region over the Inner Mongolian Plateau(IMP) were investigated,utilizing five-year continuous observations by a PARSIVEL2disdrometer in East Ujimqin County(EUC),China.It is found that only 7.94% of the 15 664 one-min precipitation samples meet classification criteria as convective rain(CR),but its contribution to the total rainfall amount is 63.87%.Notably,40.72% of the rainfall comes from large-sized raindrops(D> 3 mm),despite the fact that large-sized raindrops account for only 1.73% of the CR total number concentration.Further results show that the mean value of mass-weighted mean diameters(Dm) is larger(2.43 mm) and generalized intercepts(lgN_(W)) is lower(3.19) in CR,aligning with a "continentallike" cluster,which is mainly influenced by the joint impact of in-cloud ice-based processes and the below-cloud environmental background.Also,the empirical relationships of shape-slope(μ-Λ),radar reflectivity-rain rate(Z-R),and rainfall kinetic energy(KE_(time)-Rand KE_(time)-Z) are localized.To quantitatively analyze the impact of DSD parameters on kinetic energy estimation,power-law KE_(time)-R and KE_(time)-Z relationships are derived based on the normalized gamma distribution.N_(W)takes precedence over μ in affecting variabilities of multiplicative coefficients,especially for KE_(time)-R relationship where the multiplicative coefficient is proportional to N_(W)^(-0.287).It should be noted that although the proportion of CR occurring throughout the summer is small,raindrops with lower N_(W) and larger Dmwill generate higher KE_(time),which will bring a higher potential risk of soil erosion in semi-arid regions over IMP.
基金supported by the National Natural Science Foundation of China(12161029,12171335)the National Natural Science Foundation of Hainan Province(121RC149)+1 种基金the Science Development Project of Sichuan University(2020SCUNL201)the Natural Sciences and Engineering Research Council of Canada(4394-2018).
文摘Let I be the set of all infinitely divisible random variables with finite second moments,I_(0)={X∈I;Var(X)>0},P_(I)=inf_(x∈I)P{|X-E[X]|≤√Var(X)}and P_(I_(0))=inf P{|X-E[X]|<√Var(X)}.Firstly,we prove that P_(I)≥P_(I_(0))>0.Secondly,we find_(x∈I_(0))the exact values of inf P{|X-E[X]|≤√Var(X)}and inf P{|X-E[X]|<√Var(X)}for the cases that J is the set of all geometric random variables,symmetric geometric random variables,Poisson random variables and symmetric Poisson random variables,respectively.As a consequence,we obtain that P_(I)≤e^(-1)^(∞)∑_(k=0)1/2^(2k)(k!)^(2)≈0.46576 and P_(I_(0))≤e^(-1)≈0.36788.
基金supported by the National Natural Science Foundation of China(32172118)the National Key Research and Development Program of China(2016YFD0300110 and 2016YFD0300101)+1 种基金the Basic Scientific Research Fund of Chinese Academy of Agricultural Sciences,China(S2022ZD05)the Agricultural Science and Technology Innovation Program,China(CAAS-ZDRW202004)。
文摘The distributions of light and nitrogen within a plant's canopy reflect the growth adaptation of crops to the environment and are conducive to improving the carbon assimilation ability.So can the yield in crop production be maximized by improving the light and nitrogen distributions without adding any additional inputs?In this study,the effects of different nitrogen application rates and planting densities on the canopy light and nitrogen distributions of two highyielding maize cultivars(XY335 and DH618)and the regulatory effects of canopy physiological characteristics on radiation use efficiency(RUE)and yield were studied based on high-yield field experiments in Qitai,Xinjiang Uygur Autonomous Region,China,during 2019 and 2020.The results showed that the distribution of photosynthetically active photon flux density(PPFD)in the maize canopy decreased from top to bottom,while the vertical distribution of specific leaf nitrogen(SLN)initially increased and then decreased from top to bottom in the canopy.When SLN began to decrease,the PPDF values of XY335 and DH618 were 0.5 and 0.3,respectively,corresponding to 40.6 and49.3%of the total leaf area index(LAI).Nitrogen extinction coefficient(K_(N))/light extinction coefficient(K_(L))ratio in the middle and lower canopy of XY335(0.32)was 0.08 higher than that of DH618(0.24).The yield and RUE of XY335(17.2 t ha^(-1)and 1.8g MJ^(-1))were 7.0%(1.1 t ha^(-1))and 13.7%(0.2 g MJ^(-1))higher than those of DH618(16.1 t ha^(-1)and 1.6 g MJ^(-1)).Therefore,better light conditions(where the proportion of LAI in the upper and middle canopy was small)improved the light distribution when SLN started to decline,thus helping to mobilize the nitrogen distribution and maintain a high K_(N)and K_(N)/K_(L)ratio.In addition,K_(N)/K_(L)was a key parameter for yield improvement when the maize nutrient requirements were met at 360 kg N ha^(-1).At this level,an appropriately optimized high planting density could promote nitrogen utilization and produce higher yields and greater efficiency.The results of this study will be important for achieving high maize yields and the high efficiency cultivation and breeding of maize in the future.
基金supported by the Science and Technology Innovation(STI)2030-Major Projects(2022ZD0205000 to L.L.)CAS“Light of West China”Program(xbzg-zdsys-202404 to L.L.)+1 种基金Yunnan Revitalization Talent Support Program Yunling Scholar Project(to L.L.)Yunnan Fundamental Research Projects(202305AH340006,202301AS070060 to L.L.,202401AT070206 to X.C.)。
文摘The Chinese tree shrew has gained prominence as a model organism due to its phylogenetic proximity to primates,offering distinct advantages over traditional rodent models in biomedical research.However,the neuroanatomy of this species remains insufficiently defined,limiting its utility in neurophysiological and neuropathological studies.In this study,immunofluorescence microscopy was employed to comprehensively map the distribution of three calciumbinding proteins,parvalbumin,calbindin D-28k,and calretinin,across the tree shrew cerebrum.Serial brain sections in sagittal,coronal,and horizontal planes from 12 individuals generated a dataset of 3638 cellular-resolution images.This dataset,accessible via Science Data Bank(https://doi.org/10.57760/sciencedb.23471),provides detailed region-and laminar-selective distributions of calcium-binding proteins valuable for the cyto-and chemoarchitectural characterization of the tree shrew cerebrum.This resource will not only advance our understanding of brain organization and facilitate basic and translational neuroscience research in tree shrews but also enhance comparative and evolutionary analyses across species.
基金supported by Grants in Aid from the Japan Society for the Promotion of Science(JSPS)KAKENHI[grant numbers JP21H01163 and JP23H00149].
文摘A double-moment cloud microphysics scheme requires an assumption for cloud droplet size distributions(DSDs).However,since observations of cloud DSDs are limited,default values for shape parameters and cloud condensation nuclei activation parameters are often used in numerical simulations.In this study,the effects of cloud DSDs on numerical simulations of warm stratiform precipitation around Tokyo are investigated using the Japan Meteorological Agency's non-hydrostatic model,which incorporates a double-moment cloud microphysics scheme.Simulations using the default cloud DSD showed higher cloud droplet number concentrations and lower radar reflectivity than observed data,suggesting that the default cloud DSD is too narrow.Simulations with a cloud DSD based on in situ cloud observations corrected these errors.In addition,observation-based cloud DSDs affected rainfall amounts through the autoconversion rate of cloud water and improved the threat scores.These results suggest that realistic cloud DSDs should be provided for double-moment cloud microphysics schemes in scientific studies.
基金supported by the Doctoral Research Start-up Fund,East China University of Technology(DHBK2019313)the Open Research Fund Program of Key Laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring(Central South University),the Ministry of Education(2020YSJS10)+1 种基金the Open Research Fund Program of Shandong Provincial Engineering Laboratory of Application and Development of Big Data for Deep Gold Exploration(SDK202224)the Basic Scientific Research Fund of the Institute of Geophysical and Geochemical Exploration,Chinese Academy of Geological Sciences(AS2022P03).
文摘Geochemical surveys are essential for understanding the spatial distribution of ore-forming elements.However,these surveys often involve compositional data,the weight concentrations,which do not meet the requirements of statistical methods due to the closure effect.In this study,we applied an integrated approach combining compositional data,multifractal,and multivariate statistical analyses to identify the nonlinear complexity of the spatial distributions of elemental concentrations in the Er’renshan ore field.Initially,the raw concentrations were transformed into log-ratios following the principles of composition data theory to alleviate the impact of the closure effect.Multifractal analysis was then conducted to characterise the nonlinear complexity of the concentration distributions.Furthermore,principal component analysis(PCA)and factor analysis(FA)were applied to identify spurious correlations and the potential factors controlling the distribution patterns.The results demonstrate that:a)the raw data are biased,while the log-ratio data are unbiased and more reliable;b)the spatial distributions of elemental concentrations exhibit nonlinear complexity;and c)the elemental distribution in the study area is largely controlled by structural factors.
基金The National Key R&D Program of China under contract No.2023YFE0126300the National Natural Science Foundation of China under contract No.41930538the Open Fund of China Meteorological Administration Hydro-Meteorology Key Laboratory,Hohai University,under contract No.23SWQXM049.
文摘Using the ERA5 wave reanalysis,the distributions and trends of global available wave energy storage during 1980−2019 are analyzed.The results show that the available wave energy storage is not only related to total wave energy storage but is also affected by the local available wave probability.Different distributions and trends between the available wave energy and total wave energy storage are observed.Larger values of total wave energy storage are concentrated in the high-latitude westerlies zone,whereas available wave energy storage exhibits greater concentration in the middle-low latitude regions.In each basin,there is a notable upward trend in both total wave energy storage and available wave energy storage.However,the northern Hemisphere(NH)exhibits an increasing trend in available wave probability,whereas the southern Hemisphere(SH)experiences a decreasing trend.This divergence contributes to the spatial distributions of available wave energy storage becoming increasingly uniform.These trends in wave energy are primarily influenced by changes in significant wave height.Although the increasing trend of significant wave height across all frequency ranges induces the growth of total wave energy storage,only the increasing of wave heights falling in 1.3−4 m can cause the growth of available wave energy storage.The consistent increasing rates of wave height under different mean levels contribute to the divergent trends in available wave probability.
基金supported by the National Key R&D Program of China(Grant No.2023YFC3008300)the Science and Technology Research Program of the Institute of Mountain Hazards and Environment,Chinese Academy of Sciences,Chinese Academy of Sciences(Grant No.IMHE-ZYTS-03 and IMHE-ZDRW-03).
文摘The Yarlung Tsangpo River(YTR),located in the Himalayan orogenic belt,is renowned for its deep gorges and complex tectonic features,as well as its reputation as a landslide-prone region.However,less is known about the distribution of landslides across the entire river basin.To address this gap in knowledge,this study first established a comprehensive landslide inventory across the entire basin using remote sensing mapping and multiple field investigations.Then,a systematic analysis of the spatial and size distributions was conducted.The results indicated that the YTR basin features at least 2390 landslides with areas exceeding 104 m2,spanning a total area and volume of 1087.6 km^(2) and 48.4 km^(3),respectively.These landslides can be classified into eight types,and rockslides are the most common(53.1%).Their distributions are highly asymmetric,with the following notable patterns:(1)the Tsangpo suture zone(53.4%)contains a greater number of landslides than other tectonic units;(2)the landslide size is influenced by the relief and elevation conditions,with positive relationships observed between the local relief and landslide area,as well as between the elevation range and landslide area;and(3)the landslide distribution is not significantly correlated with rainfall,and seasonally frozen ground is associated with a greater concentration of landslides.Alternating slate and shale groups in the Tsangpo suture zone may be the factors responding to landslide concentration.A total of 20.6%of landslide-blocked rivers were observed,with some forming river knickpoints.Due to the limited data,spatial and size analyses are perhaps immature,and further systematic analysis remains necessary.
文摘A new principle for grounding fault feeder detection based on negative sequence current variation and energy dissipated in the fault point is presented. It has high precision in both isolated systems and resonance earthed systems, even in full compensated systems. And it can be installed at the local control unit of feeder in distribution automation systems, such as field terminal unit (FTU). This principle is verified by EMTP simulator and experimentation.
基金funded by National Science Foundation of China (No. 40606028)National Basic Research Programs of China (No. 2006CB400601and 2001CB409703)
文摘The distributions and seasonal variations of total dissolved inorganic arsenic （TDIAs, [TDIAs] = [As^5＋]＋[As^3＋]） and arsenite （As3.） in the Yellow Sea and East China Sea are presented hero based on the observations of 9 cruises carried out in 2000 - 2003. The study area covers a broad range of hydrographic and chemical properties. The emphasis is put on a southeast transect from Changjiang Estuary to the Ryukyu Islands （i.e. PN section） in the East China Sea to discuss the impact of terrestdal input on the marginal seas of China. Arsenic species （TDlAs and arsenite） are determined by selective hydride generation - atomic fluorescence spectrometry （HG-AFS）. TDIAs concentrations were high in the coastal area of Changjiang Estuary and decreased slightly towards the shelf region. High concentratiOns of TDIAs were also existed in the near bottom layer of shelf edge of the East China Sea which indicated another source of arsenic from the incursion of Kuroshio Waters. The seasonal variations of TDIAs in the study area depend on the hydrographic stages of Changjiang and the incursion intensity of Kuroshio Waters. Arsenite showed opposite distributions with TDIAs, with higher concentrations appeared at the surface layer of shelf region, which was positive correlated with the chlorophyll a. Biological conversion of arsenate into arsenite was hypothesized for the observed distribution pattern and its seasonal variations. The stoichoimetric ratios of As to P were estimated to be about 2×10^3 at PN Section in summer. The concentrations of dissolved arsenic in the Yellow Sea and East China Sea were comparable with other areas in the world.
基金The National Natural Science Foundation of China(No. 10801032)
文摘A class of lifetime distributions, new better than equilibrium in expectation （NBEE）, and its dual, new worse than equilibrium in expectation （NWEE）, are studied based on the comparison of the expectations of lifetime X and its equilibrium Xo. The relationships of the NBEE （NWEE） and other lifetime distribution classes are discussed. It is proved that the NBEE is very large, and increasing failure rate （IFR）, new better than used （NBU） and the L class are its subclasses. The closure properties under two kinds of reliability operations, namely, convolution and mixture, are investigated. Furthermore, a Poisson shock model and a special cumulative model are also studied, in which the necessary and sufficient conditions for the NBEE （NWEE） lifetime distribution of the systems are established. In the homogenous Poisson shock model, the system lifetime belongs to NBEE（NWEE） if and only if the corresponding discrete failure distribution belongs to the discrete NBEE（NWEE）. While in the cumulative model, the system has an NBEE lifetime if and only if the stochastic threshold of accumulated damage is NBEE.
文摘Value distributions of the general differential monomials is discussed.The following theorem is obtained:Let f be a transcendental meromorphic function in the plane,F=f n 0 (f (i) ) n i …(f (k) ) n k -c,n i≥1,c≠0 be a constant then (n 0-2)T(r,f)≤(r,1F)+S(r,f) when n 0】2;T(r,f)≤7(i+1)i( i) (r,1f)+(r,1F))+S(r,f) when n 0=1;T(r,f)≤7(N(r,1f)+(r,1F))+S(r,f) when n 0=0.
基金Project supported by the National Basic Research Project(973)of China(No.2005CB422203)the National Post-Doctor Foundation of China(No.20060390990).
文摘The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.
基金supported by the Key Project of Chinese Academy of Sciences (No. KZCX2-YW-420)the National Basic Research Program (973) of China (No.2009CB421606)the National Natural Science Foundation of China (No. 20621703)
文摘Concentrations of polychlorinated biphenyls （PCBs） have been measured in sewage sludge samples from 8 urban wastewater treatment plants in Beijing, China. The PCB congeners were analyzed by isotope dilution high resolution gas chromatography/high resolution mass spectrometry method. The concentration of PCBs ranged from 65.6 to 157 ng/g dry weight （dw）, with a mean value of 101 ng/g dw. The dioxin-like PCB WHO-TEQs （World Health Organization-Toxic Equivalents） of the sludge were lower than 1 pg /g dw. Consequently, all the concentrations of PCBs in sludge samples were below the upper limit for land application according to the Chinese legislation law for agriculture use. The PCB homologue profiles in sludge samples were dominated by tri-CBs and tetra- CBs. Similar distributions have been found in one of the Chinese PCB commercial products. The patterns of dioxin-like and indicator congeners observed in this study were quite similar in all samples. The predominant congener for dioxin-like and indicator PCBs were PCB-118 and PCB-28, respectively, while PCB-126 had the highest TEQ value.
基金supported financially by the Open Project of the National Key Laboratory for Grassland Agro-ecosytems hosted at Lanzhou University,Chinathe construction project of Key Discipline of Jiangsu Province for grass science,China
文摘The effects of neutral salt and alkali on the ion distribution were investigated in two alfalfa （Medicago sativa L.） cultivars, including Zhongmu 1, a high salt-tolerant cultivar, and Algonquin, a low salt-tolerant cultivar. The alkali stress expressed more serious growth inhibition than the neutral salt stress at the same Na＋ concentration. Compared with Algonquin, Zhongmu 1 did not exhibit a higher alkali tolerance under the Na2CO3-NaHCO3 treatment with the low Na＋ concentration （50 mmol L-l）. The alkali increased the accumulation of Na＋, Ca2＋, and Mg2＋ in the root and changed the Ca2＋ and Mg2＋ balance in the entire alfalfa plant. The salt and alkali stresses decreased the K＋ and Fe3＋ contents of the roots and leaves, the root Mn2＋ content, and the shoot Zn2＋ content, but they increased the Fe3＋ accumulation of the shoots, the shoot and leaf Cu2＋ contents, and the leaf Zn2＋ content in both alfalfa cultivars. Based on the results obtained under the conditions of this experiment, we found that the salt and alkali stresses reduced the plant growth in both alfalfa cultivars, while the alkali caused a stronger stress than the neutral salt in alfalfa. Thus, we conclude that under hydroponic conditions, the deleterious effects of the alkali on plants are due to the distribution change of some trophic ion balance in the roots, shoots, and leaves of the plants by causing of Na＋, CO3^2-, and/or HCO3- stresses.
文摘The effects of the component gradient distribution at interface and the fiber gradient distribution on the strength of cement-based materials were studied. The results show that the flexural strength and compressive strength of the mortar and concrete with interface component and fiber gradient distributions are obviously improved. The strengthes of the fiber gradient distributed mortar and concrete (FGDM/C) are higher than those of fiber homogeneously distributed mortar and concrete (FHDM/C). To obtain the same strength, therefore, a smaller fiber volume content in FGDM/C is needed than that in FHDM/C. The results also show that the component gradient distribution of the concrete can be obtained by means of multi-layer vibrating formation.
基金supported financially by the National Natural Science Foundation of China(40525016)the National Basic Research Program(2007CB407303 and 2006CB403702)
文摘Total suspended particulates （TSP） samples were collected using low pressure impactors （Andersen Series 20-800, USA） on typical clear, hazy and foggy days in Beijing in order to investigate the characteristics of size distributions and elemental compositions of particulate matter （PM） in different weather conditions. The concentrations of sixteen elements, including Na, Mg, Al, K, Ca, Mn, Fe, Ni, Cu, Zn, As, Se, Cd, Ba, T1 and Pb were detected using inductively coupled plasma mass spectrometry （ICP-MS）. The results showed that Ca, A1, Fe, Mg and Ba on foggy days were 2.0 2.6 times higher than on clear days, and 2.3-2.9 times higher than on hazy days. Concentrations of Cu, Zn, As, Se and Pb on foggy days were 163.5, 1186.7, 65.9, 32.0 and 708.2 ng m-3, respectively, in fine particles, and 68.1, 289.5, 19.8, 1.6 and 103.8 ng m-3, respectively, in coarse particles. This was 1.0~8.4 times higher and 1.4-7.4 times higher than on clear and hazy days, respectively. It is then shown that Mg, A1, Fe, Ca and Ba were mainly associated with coarse particles, peaking at 4.7~5.8 μm; that Cd, Se, Zn, As, T1 and Pb were most dominant in fine particles, peaking at 0.43-1.1 μm; and that Na, K, Ni, Cu and Mn had a multi-mode distribution, with peaks at 0.43-1.1 μm and 4.7-5.8 μm. The enrichment factors indicated that coal combustion along with vehicle and industry emissions may be the main sources of pollution elements.
基金This work was supported by Shanghai Municipal Committee of Science and Technology through grant 03DZ05052.
文摘Objective To determine the best statistical distribution of concentration data of major air pollutants in Shanghai. Methods Four types of theoretic distributions (lognormal, gamma, Pearson V and extreme value) were chosen to fit daily average concentration data of PM10, SO2 and NO2 from June 1, 2000 to May 31, 2003 in Shanghai by using the maximum likelihood method. The fit results were evaluated by Chi-square test. Results The best-fit distributions for PM10,SO2 and NO2 concentrations in Shanghai were lognormal, Pearson V, and extreme value distributions, respectively. Conclusion The results can be further applied to local air pollution prediction and control, e.g., the probabilities exceeding the air quality standard and emission source reduction of air pollutant concentration to meet the standard.
基金supported by the Commonweal Project of National Environment Protection(No.200709013 200709048)the National Basic Research Program (973)of China(No.2011CB503801)
文摘Aliphatic hydrocarbons （n-alkanes） associated with fine particulate matter were determined in the ambient air of urban, industrial and coastal areas in Tianjin, China, where intensive coal burning for industrial and domestic purpose takes place, n-Alkane homologues from C12 to C35 were quantifiable in all samples with C20-C31 being the most abundant species. Average concentrations of the total n-alkanes were 148.7, 250.1 and 842.0 ng/m3 in July, April and January, respectively. Seasonal variations were mainly attributed to ambient temperature changes and coal combustion for residential heating. Among the three studied areas, the highest levels of n-alkanes were observed in the industrial complex in winter and spring, but in summer the coastal alkane concentration moved up to the highest. A mono-modal distribution for n-alkanes was observed in spring and summer with odd carbon number predominance and a maximum centered at C27-C31, suggesting the release of plant wax into the atmosphere. The bimodal distribution with maxima at C22 and C26 observed in winter indicated a substantial influence of fossil fuel sources. All the CPIs （CPI1, CPI2, CPI3） values, varying between 0.64 and 1.97, indicated the influence of anthropogenic emissions on fine organic aerosols. The estimated contributions of plant wax to total n-alkanes were on average of 12.9%, 19.1% and 26.1% for winter, spring and summer, respectively.
基金the National Key Basic Research Program of China (973program)，a key project of the Shandong Provincial Environmental Protection Department，the Niche Area Development Scheme of the Hong Kong Polytechnic University，the Hong Kong Research Grants Council，the central level,scientific research institutes for basic R & D special fund business
文摘For the 2008 Olympic Games, drastic control measures were implemented on industrial and urban emissions of sulfur dioxide （SO2）, nitrogen oxides （NOx） and other pollutants to address the issues of poor air quality in Beijing. To investigate the effects of SO2 and NOx reductions on the particulate sulfate and nitrate concentrations as well as their size distributions, size-segregated aerosol samples were collected using micro-orifice uniform deposit impactors （MOUDIs） at urban and downwind rural sites in Beijing before and after full-scale controls. During the sampling period, the mass concentrations of fine particles （PMI.s） at the urban and rural sites were 94.0 and 85.9 p.g m-3, respectively. More than 90% of the sulfates and 60% of nitrates formed as fine particles. Benefiting from the advantageous meteorological conditions and the source controls, sulfates were observed in rather low concentrations and primarily in condensation mode during the Olympics. The effects of the control measures were separately analyzed for the northerly and the southerly air-mass-dominated days to account for any bias. After the control measures were implemented, PM, sulfates, and nitrates were significantly reduced when the northerly air masses prevailed, with a higher percentage of reduction in larger particles. The droplet mode particles, which dominated the sulfates and nitrates before the controls were implemented, were remarkably reduced in mass concentration after the control measures were implemented. Nevertheless, when the polluted southerly air masses prevailed, the local source control measures in Beijing did not effectively reduce the ambient sulfate concentration due to the enormous regional contribution from the North China Plain.
