Chemical short-range order(SRO),a phenomenon at the atomic scale resulting from inhomogeneities in the local chemical environment,is usually studied using machine learning force field-based molecular dynamics simulati...Chemical short-range order(SRO),a phenomenon at the atomic scale resulting from inhomogeneities in the local chemical environment,is usually studied using machine learning force field-based molecular dynamics simulations due to the limitations of experimental methods.To promote the reliable application of machine potentials in high-entropy alloy simulations,first,this work uses NEP models trained on two different datasets to predict the SRO coefficients of NbMoTaW.The results show that within the same machine learning framework,there are significant differences in the prediction of SRO coefficients for the Nb-Nb atomic pair.Subsequently,this work predicts the SRO coefficients of NbMoTaW using the NEP model and the SNAP model,both of which are trained on the same dataset.The results reveal significant discrepancies in SRO predictions for like-element pairs(e.g.,Nb-Nb and W-W)between the two potentials,despite the identical training data.The findings of this study indicate that discrepancies in the prediction results of SRO coefficients can arise from either the same machine learning framework trained on different datasets or different learning frameworks trained on the same dataset.This reflects possible incompleteness in the current training set's coverage of local chemical environments at the atomic scale.Future research should establish unified evaluation standards to assess the capability of training sets to accurately describe complex atomic-scale behaviors such as SRO.展开更多
Missile-borne short-range infrared detection(SIRD)technology is commonly used in military ground target detection.In complex battlefield environments,achieving precise strike on ground target is a challenging task.How...Missile-borne short-range infrared detection(SIRD)technology is commonly used in military ground target detection.In complex battlefield environments,achieving precise strike on ground target is a challenging task.However,real battlefield data is limited,and equivalent experiments are costly.Currently,there is a lack of comprehensive physical modeling and numerical simulation methods for SIRD.To this end,this study proposes a SIRD simulation framework incorporating full-link physical response,which is integrated through the radiative transfer layer,the sensor response layer,and the model-driven layer.In the radiative transfer layer,a coupled dynamic detection model is established to describe the external optical channel response of the SIRD system by combining the infrared radiation model and the geometric measurement model.In the sensor response layer,considering photoelectric conversion and signal processing,the internal signal response model of the SIRD system is established by a hybrid mode of parametric modeling and analog circuit analysis.In the model-driven layer,a cosimulation application based on a three-dimensional virtual environment is proposed to drive the full-link physical model,and a parallel ray tracing method is employed for real-time synchronous simulation.The proposed simulation framework can provide pixel-level signal output and is verified by the measured data.The evaluation results of the root mean square error(RMSE)and the Pearson correlation coefficient(PCC)show that the simulated data and the measured data achieve good consistency,and the evaluation results of the waveform eigenvalues indicate that the simulated signals exhibit low errors compared to the measured signals.The proposed simulation framework has the potential to acquire large sample datasets of SIRD under various complex battlefield environments and can provide an effective data source for SIRD application research.展开更多
Chemical short-range orders(CSROs),as the built-in sub-nanoscale entities in a high-/medium-entropy alloy(H/MEA),have aroused an ever-increasing interest.With multi-principal elements in an H/MEA to form a complex con...Chemical short-range orders(CSROs),as the built-in sub-nanoscale entities in a high-/medium-entropy alloy(H/MEA),have aroused an ever-increasing interest.With multi-principal elements in an H/MEA to form a complex concentrated solution,a variety of sub-systems of species exist to induce the metastable ordered compounds as candidates for ultimate CSROs.The issues remain pending on the origin of CSROs as to how to judge if CSRO will form in an H/MEA and particularly,what kind of CSROs would be stably produced if there were multiple possibilities.Here,the first-principles method,along with the proposed local formation energy calculation in allusion to the atomic-scale chemical heterogeneities,is used to predict the CSRO formation based on the mechanical stability,thermodynamic formation energy,and electronic characteristics.The simulations are detailed in an equiatomic ternary VCoNi MEA with three kinds of potential compounds,i.e.,L1_(1),L1_(2),and B2,in the face-centered cubic matrix.It turns out that L1_(1)is stable but hard to grow up so as to become the final CSRO.L1_(1)is further predicted as CSROs in CrCoNi,but unable to form in FeCoNi and CrMnFeCoNi alloys.These predictions are consistent with the experimental observations.Our findings shed light on understanding the formation of CSROs.This method is applicable to other H/MEAs to design and tailor CSROs by tuning chemical species/contents and thermal processing for high performance.展开更多
The immerging three dimensional(3D) metal-organic framework(MOF)-reinforced composite solid-state electrolytes have attracted great interest because of the enhanced ionic conductivity and mechanical properties. Howeve...The immerging three dimensional(3D) metal-organic framework(MOF)-reinforced composite solid-state electrolytes have attracted great interest because of the enhanced ionic conductivity and mechanical properties. However, the defective spatial arrangement of MOFs restricted by fabrication methodology leads to insufficient lithium ion transport in electrolytes. Herein, a 3D interconnected MOF framework tailored for all-solid-state electrolytes is rationally designed by a universal polydopamine(PDA)-engineered "double-sided tape" strategy. The PDA serves as a double-sided tape, firmly adhering on the special single-layer Nylon grid as well as offering uniform nucleation sites to anchor the metal nodes to ensure continuous growth of well-ordered MOFs. Benefiting from the Lewis acid feature of MOFs and its cage effect toward TFSI^(-), a fast and homogeneous lithium ion transport can be achieved through the internal channels within neighboring MOFs and the continuous MOFs/polymer interfaces both along the short-range circumferential boundary of Nylon fiber. The resultant composite electrolytes exhibit high lithium ion conductivity and prominent mechanical properties, rendering excellent cyclic stability whether used in coin or pouch cells. This work demonstrates a widely applicable "double-sided tape"strategy for controllable spatial arrangement of MOF nanoparticles on optional substrates, which provides a scalable approach to rationally construct desired lithium ion pathways within composite electrolytes.展开更多
High/medium entropy alloys(H/MEAs)are generally possible to exhibit chemical short-range order(SRO).However,the complex role of SRO on mechanical properties from nano-scale to meso-scale is still challenging so far.He...High/medium entropy alloys(H/MEAs)are generally possible to exhibit chemical short-range order(SRO).However,the complex role of SRO on mechanical properties from nano-scale to meso-scale is still challenging so far.Here,we study the strengthening mechanism and deformation behavior in a model body-centered-cubic HfNbTa MEA by using atomic-scale molecular dynamics,micro-scale dislocation dynamics,and meso-scale crystal plasticity finite element.The SRO inhibits dislocation nucleation at the atomic scale,improving the flow stress.The SRO-induced ultrastrong local stress fluctuation greatly improves the micro-scale dislocation-based strength by the significant dislocation forest strengthening.Moreover,the Ta-rich locally ordered structure leads to an obvious heterogeneous strain and stress partitioning,which forms a strong strain gradient in the adjacent grain interiors and contributes to the strong back-stress-induced strain hardening.展开更多
Three dimensional(3-D)imaging algorithms with irregular planar multiple-input-multiple-output(MIMO)arrays are discussed and compared with each other.Based on the same MIMO array,a modified back projection algorithm(MB...Three dimensional(3-D)imaging algorithms with irregular planar multiple-input-multiple-output(MIMO)arrays are discussed and compared with each other.Based on the same MIMO array,a modified back projection algorithm(MBPA)is accordingly proposed and four imaging algorithms are used for comparison,back-projection method(BP),back-projection one in time domain(BP-TD),modified back-projection one and fast Fourier transform(FFT)-based MIMO range migration algorithm(FFT-based MIMO RMA).All of the algorithms have been implemented in practical application scenarios by use of the proposed imaging system.Back to the practical applications,MIMO array-based imaging system with wide-bandwidth properties provides an efficient tool to detect objects hidden behind a wall.An MIMO imaging radar system,composed of a vector network analyzer(VNA),a set of switches,and an array of Vivaldi antennas,have been designed,fabricated,and tested.Then,these algorithms have been applied to measured data collected in different scenarios constituted by five metallic spheres in the absence and in the presence of a wall between the antennas and the targets in simulation and pliers in free space for experimental test.Finally,the focusing properties and time consumption of the above algorithms are compared.展开更多
The short-range order(SRO)in multi-principal element alloys(MPEAs)is an intriguing topic in advanced alloy research.The crucial question related to this topic lies in the effect of the local chemical fluctu-ations on ...The short-range order(SRO)in multi-principal element alloys(MPEAs)is an intriguing topic in advanced alloy research.The crucial question related to this topic lies in the effect of the local chemical fluctu-ations on the deformation behavior of MPEAs.In this study,the large-scale molecular dynamics(MD)simulation is used to investigate the dislocation glide behavior and mechanical performance of CoCrNi medium-entropy alloy(MEA)with respect to the SRO and lattice distortion(LD)effects.The slip plane softening and dislocation glide competition are found in the models with SRO.The change of energy barrier caused by SRO degeneration is the dominant reason for the slip plane softening,while the combi-nation of dislocation pinning and slip plane softening leads to the dislocation glide competition,which is the primary mechanism for the shear localization in the CoCrNi MEA with SRO.Moreover,the dislocation glide competition compensates for the strength loss induced by slip plane softening.The results provide a new proposition for the conflicting simulation and experimental results on the topic of the SRO effect in MPEAs.展开更多
Enormous progresses to understand the jamming transition have been driven via simulating purely repulsive particles which were somehow idealized in the past two decades. While the attractive systems are both theoretic...Enormous progresses to understand the jamming transition have been driven via simulating purely repulsive particles which were somehow idealized in the past two decades. While the attractive systems are both theoretical and practical compared with repulsive systems. By studying the statistics of rigid clusters, we find that the critical packing fraction φ_(c) varies linearly with attraction μ for different system sizes when the range of attraction is short. While for systems with long-range attractions, however, the slope of φ_(c) appears significantly different, which means that there are two distinct jamming scenarios. In this paper, we focus our main attention on short-range attractions scenario and define a new quantity named "short-range attraction susceptibility" χ_(p), which describes the degree of response of the probability of finding jammed states pjto short-range attraction strength μ. Our central results are that χ_(p) diverges in the thermodynamic limit as χ_(p) ∝|φ-φ_(c)^(∞)|^(-γ_(p)), where φ_(c)^(∞) is the packing fraction at the jamming transition for the infinite system in the absence of attraction. χ_(p) obeys scaling collapse with a scaling function in both two and three dimensions, illuminating that the jamming transition can be considered as a phase transition as proposed in previous work.展开更多
In this letter,we briefly summarize experimental and theoretical findings of fo rmation and characterization of short-range orderings(SROs)as well as their effects on the defo rmation behavior of high-entropy alloys(H...In this letter,we briefly summarize experimental and theoretical findings of fo rmation and characterization of short-range orderings(SROs)as well as their effects on the defo rmation behavior of high-entropy alloys(HEAs).We show that existence of SROs is a common yet key structural feature of HEAs,and tuning the degree of SROs is an effective way for optimizing mechanical properties of HEAs.In additional,the challenges concerning about formation mechanism and characterization of SROs in HEAs are discussed,and future research activities in this regard are also proposed.展开更多
High(or medium)-entropy alloys(H/MEAs)are complex concentrated solid solutions prone to develop the chemical short-range orders(CSROs),as an indispensable structural constituent to make H/MEAs essentially different fr...High(or medium)-entropy alloys(H/MEAs)are complex concentrated solid solutions prone to develop the chemical short-range orders(CSROs),as an indispensable structural constituent to make H/MEAs essentially different from the traditional alloys.The CSROs are predicted to play roles in dislocation behaviors and mechanical properties.So far,the image of CSROs is built up by the theoretical modeling and computational simulations in terms of the conventional concept,i.e.,the preference/avoidance of elemental species to satisfy the short-ranged ordering in the first and the next couple of nearest-neighbor atomic shells.In these simulated CSROs,however,the structural image is missing on the atomic scale,even though the lattice periodicity does not exist in the CSROs.Further,it is pending as to the issues if and what kind of CSRO may be formed in a specific H/MEA.All these are ascribed to the challenge of experimentally seeing the CSROs.Until recently,the breakthrough does not appear to convincingly identify the CSROs in the H/MEAs by using the state-of-the-art transmission electron microscope.To be specific,the electron diffractions provide solid evidence to doubtlessly ascertain CSROs.The structure motif of CSROs is then constructed,showing both the lattice structure and species ordering occupation,along with the stereoscopic topography of the CSRO.It is suggested that the CSROs,as the first landscape along the path of development of the local chemical ordering,offer one more route to substantially develop the ordered structure on the atomic scale in the H/MEAs,parallel to the existing grain-leveled microstructure.The findings of CSROs make a step forward to understand the CSROs-oriented relationship between the microstructure and mechanical properties.This review focuses on the recent progress mainly in the experimental aspects of the identification,structure motif,and mechanical stability in CSROs,along with the chemical medium-range orders as the growing CSROs。展开更多
A scheme of assimilating radar-retrieved water vapor is adopted to improve the quality of NWP initial field for improvement of the accuracy of short-range precipitation prediction. To reveal the impact of the assimila...A scheme of assimilating radar-retrieved water vapor is adopted to improve the quality of NWP initial field for improvement of the accuracy of short-range precipitation prediction. To reveal the impact of the assimilation of radar-retrieved water vapor on short-term precipitation forecast, three parallel experiments, cold start, hot start and hot start plus the assimilation of radar-retrieved water vapor, are designed to simulate the 31 days of May, 2013 with a fine numerical model for South China. Furthermore, a case of heavy rain that occurred from 8-9 May 2013 over the region from the southwest of Guangdong province to Pearl River Delta is analyzed in detail. Results show that the cold start experiment is not conducive to precipitation 12 hours ahead; the hot start experiment is able to reproduce well the first6 hours of precipitation, but badly for subsequent prediction; the experiment of assimilating radar-retrieved water vapor is not only able to simulate well the precipitation 6 hours ahead, but also able to correctly predict the evolution of rain bands from 6 to 12 hours in advance.展开更多
Owing to the lack of a direct link with the operations in short-range air combat,conventional aircraft flying qualities criteria are inappropriate to guide the design of a task-tailored flight control law.By applying ...Owing to the lack of a direct link with the operations in short-range air combat,conventional aircraft flying qualities criteria are inappropriate to guide the design of a task-tailored flight control law.By applying the mission-oriented flying qualities evaluation approach,various aircraft with different control law parameters are evaluated on a ground-based simulator.This paper compares the evaluation results with several conventional flying qualities criteria,and discusses the appropriate parameter combination to reflect the flying qualities requirements of short-range air combat.The comparison and analysis show that a short-range air combat mission requires a higher minimum short period mode natural frequency and a smaller maximum roll mode time constant,and allows a lower minimum pitch attitude bandwidth and a higher maximum short period mode damp ratio than those of conventional flying qualities criteria.Furthermore,a combination of the pitch attitude bandwidth,the pitch attitude magnitude at the bandwidth frequency,and the pitch attitude transfer function gain can define the flying qualities requirements of short-range air combat.The new metric can successfully predict the flying quality levels of aircraft in a short-range air combat mission.展开更多
A running mean bias （RMB） correction ap- proach was applied to the forecasts of near-surface variables in a seasonal short-range ensemble forecasting experiment with 57 consecutive cases during summer 2010 in the no...A running mean bias （RMB） correction ap- proach was applied to the forecasts of near-surface variables in a seasonal short-range ensemble forecasting experiment with 57 consecutive cases during summer 2010 in the northern China region. To determine a proper training window length for calculating RMB, window lengths from 2 to 20 days were evaluated, and 16 days was taken as an optimal window length, since it receives most of the benefit from extending the window length. The raw and 16-day RMB corrected ensembles were then evaluated for their ensemble mean forecast skills. The results show that the raw ensemble has obvious bias in all near-surface variables. The RMB correction can remove the bias reasonably well, and generate an unbiased ensemble. The bias correction not only reduces the ensemble mean forecast error, but also results in a better spreaderror relationship. Moreover, two methods for computing calibrated probabilistic forecast （PF） were also evaluated through the 57 case dates： 1） using the relative frequency from the RMB-eorrected ensemble; 2） computing the forecasting probabilities based on a historical rank histogram. The first method outperforms the second one, as it can improve both the reliability and the resolution of the PFs, while the second method only has a small effect on the reliability, indicating the necessity and importance of removing the systematic errors from the ensemble.展开更多
[ Objective] The study aimed to discuss the temporal-spatial distribution and short-range prediction indicators of hail weather in east central Haixi Prefecture of Qinghai Province. [Method] Using hail data of six sta...[ Objective] The study aimed to discuss the temporal-spatial distribution and short-range prediction indicators of hail weather in east central Haixi Prefecture of Qinghai Province. [Method] Using hail data of six stations in east central Haixi Prefecture from 1960 to 2010, the temporal and spatial distribution of hail weather was analyzed firstly. Afterwards, based on the high-altitude factual data of 30 case studies of hail during 2006 -2010, its high-altitude and ground weather situation and physical quantity field were studied to summarize short-term circulation pattern and shod- range prediction characteristics of hail weather. [ Result] In east central Haixi, hail appeared from April to September, and it was most frequently from May to August. Meanwhile, hail was frequent from 14：00 to 20：00. Among the six stations, hail was most frequent in Tianjun but least frequent in Wulan. Moreover, hail disaster mainly occurred in Wulan and Tianjun. In addition, there were three typos of circulation pattern of hail weather at 500 hPa. Hail mainly occurred under the effect of northwest airflow, and it had shortwave trough, cold center or trough, jet stream core or one of the three. Hail appeared frequently under the situation of upper-level divergence and low-level convergence, and abundant water vapor and water vapor flux convergence at low levels were important conditions for hailing. [ Conclusion] The research could provide scientific references for improving the accuracy of hail forecast.展开更多
Uniaxial tensile tests were carried out at room temperature(RT)and 250℃,respectively,to investigate the effect of shortrange ordering(SRO)on the mechanical properties and deformation micromechanism of fine-grained(FG...Uniaxial tensile tests were carried out at room temperature(RT)and 250℃,respectively,to investigate the effect of shortrange ordering(SRO)on the mechanical properties and deformation micromechanism of fine-grained(FG)Cu–Mn alloys with high stacking fault energy.The results show that at RT,with the increase in SRO degree,the strength of FG Cu–Mn alloys is improved without a loss of ductility,and corresponding deformation micromechanism is mainly manifested by a decrease in the size of dislocation cells.In contrast,at a high temperature of 250℃,the SRO degree becomes violently enhanced with increasing Mn content,and the deformation microstructures thus transform from dislocation cells to planar slip bands and even to deformation twins,significantly enhancing the work hardening capacity of the alloys and thus achieving a better strength-ductility synergy of FG Cu–Mn alloys.展开更多
The airborne conformal array(CFA)radar's clutter ridges are range-modulated,which result in a bias in the estimation of the clutter covariance matrix(CCM)of the cell under test(CUT),further,reducing the clutter su...The airborne conformal array(CFA)radar's clutter ridges are range-modulated,which result in a bias in the estimation of the clutter covariance matrix(CCM)of the cell under test(CUT),further,reducing the clutter suppression performance of the airborne CFA radar.The clutter ridges can be effectively compensated by the space-time separation interpolation(STSINT)method,which costs less computation than the space-time interpolation(STINT)method,but the performance of interpolation algorithms is seriously affected by the short-range clutter,especially near the platform height.Location distributions of CFA are free,which yields serious impact that range spaces of steering vector matrices are non-orthogonal complement and even no longer disjoint.Further,a new method is proposed that the shortrange clutter is pre-processed by oblique projection with the intersected range spaces(OPIRS),and then clutter data after being pre-processed are compensated to the desired range bin through the STSINT method.The OPIRS also has good compatibility and can be used in combination with many existing methods.At the same time,oblique projectors of OPIRS can be obtained in advance,so the proposed method has almost the same computational load as the traditional compensation method.In addition,the proposed method can perform well when the channel error exists.Computer simulation results verify the effectiveness of the proposed method.展开更多
Using the asymptotic iteration method, we obtain the S-wave solution for a short-range three-parameter central potential with 1/r singularity and with a non-orbital barrier. To the best of our knowledge, this is the f...Using the asymptotic iteration method, we obtain the S-wave solution for a short-range three-parameter central potential with 1/r singularity and with a non-orbital barrier. To the best of our knowledge, this is the first attempt at calculating the energy spectrum for this potential, which was introduced by H. Bahlouli and A. D. Alhaidari and for which they obtained the “potential parameter spectrum”. Our results are also independently verified using a direct method of diagonalizing the Hamiltonian matrix in the J-matrix basis.展开更多
With the high-speed development of numerical weather prediction, since the later 1980's, the prediction of short-range climate anomalies has attracted worldwide meteorologists' attention . What the so called s...With the high-speed development of numerical weather prediction, since the later 1980's, the prediction of short-range climate anomalies has attracted worldwide meteorologists' attention . What the so called short-range refers to the time scale from one month to one season or more. In dealing with the problem of short-range climate prediction, two points are needed noticing: one is the basic research to explore or investigate the mechanism of variability of the slow varying components which mainly include internal dynamics of extratropics, external forcings and tropical dynamics, and the other is the modeling efforts to simulate the process of the long-term evolution of the signal which include the improvement of model quality, stochastic prediction and the air-sea-coupled model (Miyakoda et al.,1986). Previous researches on the numerical prediction of short-term climate anomalies are mostly concentrated in the analysis of variables with global spatial scale, especially the global general atmospheric circulation analysis.As to the simulation or prediction of regional short-term climate anomalies, there exist many difficulties and problems. Though some meteorologists are devoting themself to this field, up to now, they have not reached satisfactory results. As a primary effort, by using the 2-level general atmospheric circulation model developed in the Institute of Atmospheric Physics, Chinese Academy of Sciences (IAP-AGCM) (Zeng et al., 1989), and taking the year of 1985 as a case, a numerical simulation of regional short-term climate change is completed. We pay high attention to the predictant of anomalous summer rainfall in the Yangtze River and Yellow River valleys, especially its month to month variation.展开更多
A biased sampling algorithm for the restricted Boltzmann machine(RBM) is proposed, which allows generating configurations with a conserved quantity. To validate the method, a study of the short-range order in binary a...A biased sampling algorithm for the restricted Boltzmann machine(RBM) is proposed, which allows generating configurations with a conserved quantity. To validate the method, a study of the short-range order in binary alloys with positive and negative exchange interactions is carried out. The network is trained on the data collected by Monte–Carlo simulations for a simple Ising-like binary alloy model and used to calculate the Warren–Cowley short-range order parameter and other thermodynamic properties. We demonstrate that the proposed method allows us not only to correctly reproduce the order parameters for the alloy concentration at which the network was trained, but can also predict them for any other concentrations.展开更多
The development of a Ni-based superalloy that consists of only theγ-solid-solution phase is highly desired for some applications such as high-temperature gas-cooled reactors in power plants.In this study,the temperat...The development of a Ni-based superalloy that consists of only theγ-solid-solution phase is highly desired for some applications such as high-temperature gas-cooled reactors in power plants.In this study,the temperature dependence of the plastic deformation behavior of Ni-22Cr-8W(at%)alloy was examined for the first time by using a single crystal,focusing on the influence of the short-range order(SRO),especially upon high-temperature deformation behavior.The critical resolved shear stress(CRSS)for(111)[10¯1]slip exhibited a rapid decrease as the temperature increased at low temperatures but an almost constant value of∼45 MPa between 500 and 900℃.In addition,a slight yield stress anomaly(YSA)was observed,reaching a maximum value at 1000℃.To clarify the influence of the SRO on the YSA behavior,the mechanical properties of Ni-8W and Ni-5Re single crystals were also examined.Similar temperature dependence for the CRSS,including the occurrence of slight YSA,was observed for Ni-8W,in which SRO developed.In the Ni-5Re single crystal in which SRO did not significantly develop,however,the CRSS monotonically decreased as the temperature increased.The results suggest that the presence of SRO in a Ni-Cr-W alloy contributes to the strengthening of the alloy not only at low temperatures but also at high temperatures up to∼1000℃.The results strongly suggested that the pseudo-PLC effect is related to the origin of YSA appearing in Ni-basedγ-solid-solution alloys at high temperatures.展开更多
基金Project supported by the Hunan Provincial Natural Science Foundation(Grant Nos.2024JJ6190 and 2024JK2007-1)。
文摘Chemical short-range order(SRO),a phenomenon at the atomic scale resulting from inhomogeneities in the local chemical environment,is usually studied using machine learning force field-based molecular dynamics simulations due to the limitations of experimental methods.To promote the reliable application of machine potentials in high-entropy alloy simulations,first,this work uses NEP models trained on two different datasets to predict the SRO coefficients of NbMoTaW.The results show that within the same machine learning framework,there are significant differences in the prediction of SRO coefficients for the Nb-Nb atomic pair.Subsequently,this work predicts the SRO coefficients of NbMoTaW using the NEP model and the SNAP model,both of which are trained on the same dataset.The results reveal significant discrepancies in SRO predictions for like-element pairs(e.g.,Nb-Nb and W-W)between the two potentials,despite the identical training data.The findings of this study indicate that discrepancies in the prediction results of SRO coefficients can arise from either the same machine learning framework trained on different datasets or different learning frameworks trained on the same dataset.This reflects possible incompleteness in the current training set's coverage of local chemical environments at the atomic scale.Future research should establish unified evaluation standards to assess the capability of training sets to accurately describe complex atomic-scale behaviors such as SRO.
基金supported by the Foundation of Equipment Preresearch Area(Grant No.80919010303).
文摘Missile-borne short-range infrared detection(SIRD)technology is commonly used in military ground target detection.In complex battlefield environments,achieving precise strike on ground target is a challenging task.However,real battlefield data is limited,and equivalent experiments are costly.Currently,there is a lack of comprehensive physical modeling and numerical simulation methods for SIRD.To this end,this study proposes a SIRD simulation framework incorporating full-link physical response,which is integrated through the radiative transfer layer,the sensor response layer,and the model-driven layer.In the radiative transfer layer,a coupled dynamic detection model is established to describe the external optical channel response of the SIRD system by combining the infrared radiation model and the geometric measurement model.In the sensor response layer,considering photoelectric conversion and signal processing,the internal signal response model of the SIRD system is established by a hybrid mode of parametric modeling and analog circuit analysis.In the model-driven layer,a cosimulation application based on a three-dimensional virtual environment is proposed to drive the full-link physical model,and a parallel ray tracing method is employed for real-time synchronous simulation.The proposed simulation framework can provide pixel-level signal output and is verified by the measured data.The evaluation results of the root mean square error(RMSE)and the Pearson correlation coefficient(PCC)show that the simulated data and the measured data achieve good consistency,and the evaluation results of the waveform eigenvalues indicate that the simulated signals exhibit low errors compared to the measured signals.The proposed simulation framework has the potential to acquire large sample datasets of SIRD under various complex battlefield environments and can provide an effective data source for SIRD application research.
基金supported by the National Key Re-search and Development Program of the Ministry of Science and Technology of China(No.2019YFA0209902)the Natural Sci-ence Foundation of China(Nos.11988102 and 11972350).
文摘Chemical short-range orders(CSROs),as the built-in sub-nanoscale entities in a high-/medium-entropy alloy(H/MEA),have aroused an ever-increasing interest.With multi-principal elements in an H/MEA to form a complex concentrated solution,a variety of sub-systems of species exist to induce the metastable ordered compounds as candidates for ultimate CSROs.The issues remain pending on the origin of CSROs as to how to judge if CSRO will form in an H/MEA and particularly,what kind of CSROs would be stably produced if there were multiple possibilities.Here,the first-principles method,along with the proposed local formation energy calculation in allusion to the atomic-scale chemical heterogeneities,is used to predict the CSRO formation based on the mechanical stability,thermodynamic formation energy,and electronic characteristics.The simulations are detailed in an equiatomic ternary VCoNi MEA with three kinds of potential compounds,i.e.,L1_(1),L1_(2),and B2,in the face-centered cubic matrix.It turns out that L1_(1)is stable but hard to grow up so as to become the final CSRO.L1_(1)is further predicted as CSROs in CrCoNi,but unable to form in FeCoNi and CrMnFeCoNi alloys.These predictions are consistent with the experimental observations.Our findings shed light on understanding the formation of CSROs.This method is applicable to other H/MEAs to design and tailor CSROs by tuning chemical species/contents and thermal processing for high performance.
基金supported by the Anhui Provincial Natural Science Foundation (2308085MB58)the National Natural Science Foundation of China (NSFC, 21908037, 22278107)the Anhui Provincial Development and Reform Commission (2021-442)。
文摘The immerging three dimensional(3D) metal-organic framework(MOF)-reinforced composite solid-state electrolytes have attracted great interest because of the enhanced ionic conductivity and mechanical properties. However, the defective spatial arrangement of MOFs restricted by fabrication methodology leads to insufficient lithium ion transport in electrolytes. Herein, a 3D interconnected MOF framework tailored for all-solid-state electrolytes is rationally designed by a universal polydopamine(PDA)-engineered "double-sided tape" strategy. The PDA serves as a double-sided tape, firmly adhering on the special single-layer Nylon grid as well as offering uniform nucleation sites to anchor the metal nodes to ensure continuous growth of well-ordered MOFs. Benefiting from the Lewis acid feature of MOFs and its cage effect toward TFSI^(-), a fast and homogeneous lithium ion transport can be achieved through the internal channels within neighboring MOFs and the continuous MOFs/polymer interfaces both along the short-range circumferential boundary of Nylon fiber. The resultant composite electrolytes exhibit high lithium ion conductivity and prominent mechanical properties, rendering excellent cyclic stability whether used in coin or pouch cells. This work demonstrates a widely applicable "double-sided tape"strategy for controllable spatial arrangement of MOF nanoparticles on optional substrates, which provides a scalable approach to rationally construct desired lithium ion pathways within composite electrolytes.
基金supported by the National Natural Science Foundation of China(Grant Nos.12372069,12302083,and 12172123)China Postdoctoral Science Foundation(Grant Nos.2023M731061 and BX20230109)+2 种基金the Natural Science Foundation of Hunan Province(Grant No.2022JJ20001)Hunan Provincial Innovation Foundation for Postgraduate(Grant No.CX20220378)Peter K.Liaw very much appreciates the support from the National Science Foundation(Grant Nos.DMR-1611180,1809640,and 2226508).
文摘High/medium entropy alloys(H/MEAs)are generally possible to exhibit chemical short-range order(SRO).However,the complex role of SRO on mechanical properties from nano-scale to meso-scale is still challenging so far.Here,we study the strengthening mechanism and deformation behavior in a model body-centered-cubic HfNbTa MEA by using atomic-scale molecular dynamics,micro-scale dislocation dynamics,and meso-scale crystal plasticity finite element.The SRO inhibits dislocation nucleation at the atomic scale,improving the flow stress.The SRO-induced ultrastrong local stress fluctuation greatly improves the micro-scale dislocation-based strength by the significant dislocation forest strengthening.Moreover,the Ta-rich locally ordered structure leads to an obvious heterogeneous strain and stress partitioning,which forms a strong strain gradient in the adjacent grain interiors and contributes to the strong back-stress-induced strain hardening.
基金National Natural Science Foundation of China(No.62293493)。
文摘Three dimensional(3-D)imaging algorithms with irregular planar multiple-input-multiple-output(MIMO)arrays are discussed and compared with each other.Based on the same MIMO array,a modified back projection algorithm(MBPA)is accordingly proposed and four imaging algorithms are used for comparison,back-projection method(BP),back-projection one in time domain(BP-TD),modified back-projection one and fast Fourier transform(FFT)-based MIMO range migration algorithm(FFT-based MIMO RMA).All of the algorithms have been implemented in practical application scenarios by use of the proposed imaging system.Back to the practical applications,MIMO array-based imaging system with wide-bandwidth properties provides an efficient tool to detect objects hidden behind a wall.An MIMO imaging radar system,composed of a vector network analyzer(VNA),a set of switches,and an array of Vivaldi antennas,have been designed,fabricated,and tested.Then,these algorithms have been applied to measured data collected in different scenarios constituted by five metallic spheres in the absence and in the presence of a wall between the antennas and the targets in simulation and pliers in free space for experimental test.Finally,the focusing properties and time consumption of the above algorithms are compared.
基金supported by the National Science Fund for Distinguished Young Scholar(No.11925203)the National Natural Science Foundation of China(No.12232006)+2 种基金the Guang-dong Basic and the Applied Basic Research Foundation(No.2022B1515120044)Xiaohu Yao also acknowledges support from National Key Laboratory of Shock Wave and Detonation Physics(No.JCKYS2023212002)Zhuocheng Xie gratefully acknowledges support from the China Scholarship Council(No.202106150123).
文摘The short-range order(SRO)in multi-principal element alloys(MPEAs)is an intriguing topic in advanced alloy research.The crucial question related to this topic lies in the effect of the local chemical fluctu-ations on the deformation behavior of MPEAs.In this study,the large-scale molecular dynamics(MD)simulation is used to investigate the dislocation glide behavior and mechanical performance of CoCrNi medium-entropy alloy(MEA)with respect to the SRO and lattice distortion(LD)effects.The slip plane softening and dislocation glide competition are found in the models with SRO.The change of energy barrier caused by SRO degeneration is the dominant reason for the slip plane softening,while the combi-nation of dislocation pinning and slip plane softening leads to the dislocation glide competition,which is the primary mechanism for the shear localization in the CoCrNi MEA with SRO.Moreover,the dislocation glide competition compensates for the strength loss induced by slip plane softening.The results provide a new proposition for the conflicting simulation and experimental results on the topic of the SRO effect in MPEAs.
基金supported by the National Natural Science Foundation of China (Grant No. 11702289)Key Core Technology and Generic Technology Research and Development Project of Shanxi Province,China (Grant No. 2020XXX013)the National Key Research and Development Project of China。
文摘Enormous progresses to understand the jamming transition have been driven via simulating purely repulsive particles which were somehow idealized in the past two decades. While the attractive systems are both theoretical and practical compared with repulsive systems. By studying the statistics of rigid clusters, we find that the critical packing fraction φ_(c) varies linearly with attraction μ for different system sizes when the range of attraction is short. While for systems with long-range attractions, however, the slope of φ_(c) appears significantly different, which means that there are two distinct jamming scenarios. In this paper, we focus our main attention on short-range attractions scenario and define a new quantity named "short-range attraction susceptibility" χ_(p), which describes the degree of response of the probability of finding jammed states pjto short-range attraction strength μ. Our central results are that χ_(p) diverges in the thermodynamic limit as χ_(p) ∝|φ-φ_(c)^(∞)|^(-γ_(p)), where φ_(c)^(∞) is the packing fraction at the jamming transition for the infinite system in the absence of attraction. χ_(p) obeys scaling collapse with a scaling function in both two and three dimensions, illuminating that the jamming transition can be considered as a phase transition as proposed in previous work.
基金supported by the National Natural Science Foundation of China(Nos.51921001,51871016,51971017,51531001,51901013,and 51671021)111 Project(B07003)+3 种基金Program for Changjiang Scholars and Innovative Research Team in University of China(IRT-14R05)the Projects of SKLAMM-USTBthe financial support from the Fundamental Research Fund for the Central Universities(No.FRF-BD-19002B)National Key Basic Research Program,China(No.2016YFB0300502)。
文摘In this letter,we briefly summarize experimental and theoretical findings of fo rmation and characterization of short-range orderings(SROs)as well as their effects on the defo rmation behavior of high-entropy alloys(HEAs).We show that existence of SROs is a common yet key structural feature of HEAs,and tuning the degree of SROs is an effective way for optimizing mechanical properties of HEAs.In additional,the challenges concerning about formation mechanism and characterization of SROs in HEAs are discussed,and future research activities in this regard are also proposed.
基金supported by the National Key Research and Development Program of the Ministry of Science and Technology of China(No.2019YFA0209902)the National Natural Science Foundation of China(Nos.11998102,11972350,and 11790293)the Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB22040503).
文摘High(or medium)-entropy alloys(H/MEAs)are complex concentrated solid solutions prone to develop the chemical short-range orders(CSROs),as an indispensable structural constituent to make H/MEAs essentially different from the traditional alloys.The CSROs are predicted to play roles in dislocation behaviors and mechanical properties.So far,the image of CSROs is built up by the theoretical modeling and computational simulations in terms of the conventional concept,i.e.,the preference/avoidance of elemental species to satisfy the short-ranged ordering in the first and the next couple of nearest-neighbor atomic shells.In these simulated CSROs,however,the structural image is missing on the atomic scale,even though the lattice periodicity does not exist in the CSROs.Further,it is pending as to the issues if and what kind of CSRO may be formed in a specific H/MEA.All these are ascribed to the challenge of experimentally seeing the CSROs.Until recently,the breakthrough does not appear to convincingly identify the CSROs in the H/MEAs by using the state-of-the-art transmission electron microscope.To be specific,the electron diffractions provide solid evidence to doubtlessly ascertain CSROs.The structure motif of CSROs is then constructed,showing both the lattice structure and species ordering occupation,along with the stereoscopic topography of the CSRO.It is suggested that the CSROs,as the first landscape along the path of development of the local chemical ordering,offer one more route to substantially develop the ordered structure on the atomic scale in the H/MEAs,parallel to the existing grain-leveled microstructure.The findings of CSROs make a step forward to understand the CSROs-oriented relationship between the microstructure and mechanical properties.This review focuses on the recent progress mainly in the experimental aspects of the identification,structure motif,and mechanical stability in CSROs,along with the chemical medium-range orders as the growing CSROs。
基金National Natural Science Foundation of China(41075040,41475102)"973"project for typhoon(2015CB452802)+1 种基金CMA Special Welfare Research Fund(GYHY201406009)Public Welfare(Meteorological Sector)Research Fund(GYHY201406003)
文摘A scheme of assimilating radar-retrieved water vapor is adopted to improve the quality of NWP initial field for improvement of the accuracy of short-range precipitation prediction. To reveal the impact of the assimilation of radar-retrieved water vapor on short-term precipitation forecast, three parallel experiments, cold start, hot start and hot start plus the assimilation of radar-retrieved water vapor, are designed to simulate the 31 days of May, 2013 with a fine numerical model for South China. Furthermore, a case of heavy rain that occurred from 8-9 May 2013 over the region from the southwest of Guangdong province to Pearl River Delta is analyzed in detail. Results show that the cold start experiment is not conducive to precipitation 12 hours ahead; the hot start experiment is able to reproduce well the first6 hours of precipitation, but badly for subsequent prediction; the experiment of assimilating radar-retrieved water vapor is not only able to simulate well the precipitation 6 hours ahead, but also able to correctly predict the evolution of rain bands from 6 to 12 hours in advance.
文摘Owing to the lack of a direct link with the operations in short-range air combat,conventional aircraft flying qualities criteria are inappropriate to guide the design of a task-tailored flight control law.By applying the mission-oriented flying qualities evaluation approach,various aircraft with different control law parameters are evaluated on a ground-based simulator.This paper compares the evaluation results with several conventional flying qualities criteria,and discusses the appropriate parameter combination to reflect the flying qualities requirements of short-range air combat.The comparison and analysis show that a short-range air combat mission requires a higher minimum short period mode natural frequency and a smaller maximum roll mode time constant,and allows a lower minimum pitch attitude bandwidth and a higher maximum short period mode damp ratio than those of conventional flying qualities criteria.Furthermore,a combination of the pitch attitude bandwidth,the pitch attitude magnitude at the bandwidth frequency,and the pitch attitude transfer function gain can define the flying qualities requirements of short-range air combat.The new metric can successfully predict the flying quality levels of aircraft in a short-range air combat mission.
基金supported by a project of the National Natural Science Foundation of China (Grant No. 41305099)
文摘A running mean bias （RMB） correction ap- proach was applied to the forecasts of near-surface variables in a seasonal short-range ensemble forecasting experiment with 57 consecutive cases during summer 2010 in the northern China region. To determine a proper training window length for calculating RMB, window lengths from 2 to 20 days were evaluated, and 16 days was taken as an optimal window length, since it receives most of the benefit from extending the window length. The raw and 16-day RMB corrected ensembles were then evaluated for their ensemble mean forecast skills. The results show that the raw ensemble has obvious bias in all near-surface variables. The RMB correction can remove the bias reasonably well, and generate an unbiased ensemble. The bias correction not only reduces the ensemble mean forecast error, but also results in a better spreaderror relationship. Moreover, two methods for computing calibrated probabilistic forecast （PF） were also evaluated through the 57 case dates： 1） using the relative frequency from the RMB-eorrected ensemble; 2） computing the forecasting probabilities based on a historical rank histogram. The first method outperforms the second one, as it can improve both the reliability and the resolution of the PFs, while the second method only has a small effect on the reliability, indicating the necessity and importance of removing the systematic errors from the ensemble.
文摘[ Objective] The study aimed to discuss the temporal-spatial distribution and short-range prediction indicators of hail weather in east central Haixi Prefecture of Qinghai Province. [Method] Using hail data of six stations in east central Haixi Prefecture from 1960 to 2010, the temporal and spatial distribution of hail weather was analyzed firstly. Afterwards, based on the high-altitude factual data of 30 case studies of hail during 2006 -2010, its high-altitude and ground weather situation and physical quantity field were studied to summarize short-term circulation pattern and shod- range prediction characteristics of hail weather. [ Result] In east central Haixi, hail appeared from April to September, and it was most frequently from May to August. Meanwhile, hail was frequent from 14：00 to 20：00. Among the six stations, hail was most frequent in Tianjun but least frequent in Wulan. Moreover, hail disaster mainly occurred in Wulan and Tianjun. In addition, there were three typos of circulation pattern of hail weather at 500 hPa. Hail mainly occurred under the effect of northwest airflow, and it had shortwave trough, cold center or trough, jet stream core or one of the three. Hail appeared frequently under the situation of upper-level divergence and low-level convergence, and abundant water vapor and water vapor flux convergence at low levels were important conditions for hailing. [ Conclusion] The research could provide scientific references for improving the accuracy of hail forecast.
基金supported by the National Natural Science Foundation of China(NSFC)under Grant Nos.51571058 and 51871048。
文摘Uniaxial tensile tests were carried out at room temperature(RT)and 250℃,respectively,to investigate the effect of shortrange ordering(SRO)on the mechanical properties and deformation micromechanism of fine-grained(FG)Cu–Mn alloys with high stacking fault energy.The results show that at RT,with the increase in SRO degree,the strength of FG Cu–Mn alloys is improved without a loss of ductility,and corresponding deformation micromechanism is mainly manifested by a decrease in the size of dislocation cells.In contrast,at a high temperature of 250℃,the SRO degree becomes violently enhanced with increasing Mn content,and the deformation microstructures thus transform from dislocation cells to planar slip bands and even to deformation twins,significantly enhancing the work hardening capacity of the alloys and thus achieving a better strength-ductility synergy of FG Cu–Mn alloys.
基金supported by the Fund for Foreign Scholars in University Research and Teaching Programs(the 111 Project)(B18039)。
文摘The airborne conformal array(CFA)radar's clutter ridges are range-modulated,which result in a bias in the estimation of the clutter covariance matrix(CCM)of the cell under test(CUT),further,reducing the clutter suppression performance of the airborne CFA radar.The clutter ridges can be effectively compensated by the space-time separation interpolation(STSINT)method,which costs less computation than the space-time interpolation(STINT)method,but the performance of interpolation algorithms is seriously affected by the short-range clutter,especially near the platform height.Location distributions of CFA are free,which yields serious impact that range spaces of steering vector matrices are non-orthogonal complement and even no longer disjoint.Further,a new method is proposed that the shortrange clutter is pre-processed by oblique projection with the intersected range spaces(OPIRS),and then clutter data after being pre-processed are compensated to the desired range bin through the STSINT method.The OPIRS also has good compatibility and can be used in combination with many existing methods.At the same time,oblique projectors of OPIRS can be obtained in advance,so the proposed method has almost the same computational load as the traditional compensation method.In addition,the proposed method can perform well when the channel error exists.Computer simulation results verify the effectiveness of the proposed method.
文摘Using the asymptotic iteration method, we obtain the S-wave solution for a short-range three-parameter central potential with 1/r singularity and with a non-orbital barrier. To the best of our knowledge, this is the first attempt at calculating the energy spectrum for this potential, which was introduced by H. Bahlouli and A. D. Alhaidari and for which they obtained the “potential parameter spectrum”. Our results are also independently verified using a direct method of diagonalizing the Hamiltonian matrix in the J-matrix basis.
基金This work was supported by the National Natural Science Foundation, Chinese Academy of Sciences, the Key Projects of National Foundamental Researches and LASG.
文摘With the high-speed development of numerical weather prediction, since the later 1980's, the prediction of short-range climate anomalies has attracted worldwide meteorologists' attention . What the so called short-range refers to the time scale from one month to one season or more. In dealing with the problem of short-range climate prediction, two points are needed noticing: one is the basic research to explore or investigate the mechanism of variability of the slow varying components which mainly include internal dynamics of extratropics, external forcings and tropical dynamics, and the other is the modeling efforts to simulate the process of the long-term evolution of the signal which include the improvement of model quality, stochastic prediction and the air-sea-coupled model (Miyakoda et al.,1986). Previous researches on the numerical prediction of short-term climate anomalies are mostly concentrated in the analysis of variables with global spatial scale, especially the global general atmospheric circulation analysis.As to the simulation or prediction of regional short-term climate anomalies, there exist many difficulties and problems. Though some meteorologists are devoting themself to this field, up to now, they have not reached satisfactory results. As a primary effort, by using the 2-level general atmospheric circulation model developed in the Institute of Atmospheric Physics, Chinese Academy of Sciences (IAP-AGCM) (Zeng et al., 1989), and taking the year of 1985 as a case, a numerical simulation of regional short-term climate change is completed. We pay high attention to the predictant of anomalous summer rainfall in the Yangtze River and Yellow River valleys, especially its month to month variation.
基金supported by the financing program AAAA-A16-116021010082-8。
文摘A biased sampling algorithm for the restricted Boltzmann machine(RBM) is proposed, which allows generating configurations with a conserved quantity. To validate the method, a study of the short-range order in binary alloys with positive and negative exchange interactions is carried out. The network is trained on the data collected by Monte–Carlo simulations for a simple Ising-like binary alloy model and used to calculate the Warren–Cowley short-range order parameter and other thermodynamic properties. We demonstrate that the proposed method allows us not only to correctly reproduce the order parameters for the alloy concentration at which the network was trained, but can also predict them for any other concentrations.
基金Iketani Science and Technology Foundation,Japan(No.0221044-A)Grant-in-Aid for Young Scientist(B)from the Japan Society for the Promotion of Science(JSPSgrant number:22760540).
文摘The development of a Ni-based superalloy that consists of only theγ-solid-solution phase is highly desired for some applications such as high-temperature gas-cooled reactors in power plants.In this study,the temperature dependence of the plastic deformation behavior of Ni-22Cr-8W(at%)alloy was examined for the first time by using a single crystal,focusing on the influence of the short-range order(SRO),especially upon high-temperature deformation behavior.The critical resolved shear stress(CRSS)for(111)[10¯1]slip exhibited a rapid decrease as the temperature increased at low temperatures but an almost constant value of∼45 MPa between 500 and 900℃.In addition,a slight yield stress anomaly(YSA)was observed,reaching a maximum value at 1000℃.To clarify the influence of the SRO on the YSA behavior,the mechanical properties of Ni-8W and Ni-5Re single crystals were also examined.Similar temperature dependence for the CRSS,including the occurrence of slight YSA,was observed for Ni-8W,in which SRO developed.In the Ni-5Re single crystal in which SRO did not significantly develop,however,the CRSS monotonically decreased as the temperature increased.The results suggest that the presence of SRO in a Ni-Cr-W alloy contributes to the strengthening of the alloy not only at low temperatures but also at high temperatures up to∼1000℃.The results strongly suggested that the pseudo-PLC effect is related to the origin of YSA appearing in Ni-basedγ-solid-solution alloys at high temperatures.
