The particle concentration inside a cyclone separator at different operation parameters was simulated with the FLUENT software. The Advanced Reynolds Stress Model （ARSM） was used in gas phase turbulence modeling. St...The particle concentration inside a cyclone separator at different operation parameters was simulated with the FLUENT software. The Advanced Reynolds Stress Model （ARSM） was used in gas phase turbulence modeling. Stochastic Particle Tracking Model （SPTM） and the Particle-Source-In-Cell （PSIC） method were adopted for particles computing. The interaction between particles and the gas phase was also taken into account. The numerical simulation results were in agreement with the experimental data. The simulation revealed that an unsteady spiral dust strand appeared near the cyclone wall and a non-axi-symmetrical dust ring appeared in the annular space and under the cover plate of the cyclone. There were two regions in the radial particle concentration distribution, in which particle concentration was low in the inner region （r/R≤0.75） and increased greatly in the outer region （r/R〉0.75）. Large particles generally had higher concentration in the near-wall region and small particles had higher concentration in the inner swirling flow region. The axial distribution of particle concentration in the inner swirling flow （r/R≤0.3） region showed that there existed serious fine particle entrainment within the height of 0.SD above the dust discharge port and a short-cut flow at a distance of about 0.25D below the entrance of the vortex finder. The dimensionless concentration in the high-concentration region increased obviously in the upper part of the cyclone separation space when inlet particle loading was large. With increasing gas temperature, the particle separation ability of the cyclone was obviously weakened.展开更多
Adsorption/desorption in a new Zn（Ⅱ）-TiO2 adsorption system was investigated at different particle concentrations （Cp）. TEM, SEM and XRD analyses revealed that the TiO2 particles were an aggregation of nano-sized...Adsorption/desorption in a new Zn（Ⅱ）-TiO2 adsorption system was investigated at different particle concentrations （Cp）. TEM, SEM and XRD analyses revealed that the TiO2 particles were an aggregation of nano-sized （approximately 10 nm） pure anatase-type TiO2. Adsorption experiments were carried out with particle concentrations of 100, 400 and 1000 mg/L, and their adsorption isotherms were found to decline successively, showing an obvious Cp effect. Desorption experiments indicated that adsorption in this system was irreversible, and the irreversibility increased with increasing Cp. These phenomena could be explained by the MEA （metastable equilibrium adsorption） theory and the Cp effect could be modeled well with an MEA-Freundlich-type Cp effect isotherm equation. This study may heln understand environmental behavior of contaminants on ultrafine natural particles.展开更多
During the 2012 Lanzhou International Marathon, the local government made a significant effort to improve traffic conditions and air quality by implementing traffic restriction measures. To evaluate the direct effect ...During the 2012 Lanzhou International Marathon, the local government made a significant effort to improve traffic conditions and air quality by implementing traffic restriction measures. To evaluate the direct effect of these measures on urban air quality, especially particle concentrations and their size distributions, atmospheric particle size distributions （0.5-20μm） obtained using an aerodynamic particle sizer （model 3321, TSI, USA） in June 2012 were analyzed. It was found that the particle number, surface area and volume concentrations for size range 0.5-10 μm were （15.0±2.1） cm-3, （11.8±2.6） μm2/cm3 and （1.9±0.6） μm2/cm3, respectively, on the traffic-restricted day （Sunday）, which is 63.2%, 53.0% and 47.2% lower than those on a normal Sunday. For number and surface area concentrations, the most affected size range was 0.5-0.7 and 0.5-0.8 μm, respectively, while for volume concentration, the most affected size ranges were 0.5-0.8, 1.7-2.0 and 5.0-5.4 μm. Number and volume concentrations of particles in size range 0.5-1.0μm correlated well with the number of non-CNG （Compressed Natural Gas） powered vehicles, while their correlation with the number of CNG-powered vehicles was very low, suggesting that reasonable urban traffic controls along with vehicle technology improvements could play an important role in improving urban air quality.展开更多
The COVID-19 lockdown was a typical example of extreme emission reduction,providing an opportunity to study the impact of lockdown measures on air pollution.Particle number concentrations(PNC)originate from direct emi...The COVID-19 lockdown was a typical example of extreme emission reduction,providing an opportunity to study the impact of lockdown measures on air pollution.Particle number concentrations(PNC)originate from direct emissions or through new particle formation events.However,their variations during the lockdown period are under investigation.This study focuses on Luohe,a city on the southern edge of the North China Plain,analyzing the changes in PNC and its sources before,during,and after the COVID-19 lockdown.From March 25^(th)to May 31^(st),2022,real-time PNC measurements were conducted using a Scanning Mobility Particle Sizer for particle size.Results showed an 11.2%decrease in PNC during the lockdown compared to pre-lockdown and a 3.6%decrease compared to post-lockdown,indicating reduced local emissions and weakened regional transportation during the lockdown.Positive Matrix Factorization analysis identified six sources contributing to the total PNC,including photochemical nucleation,aged photochemical nucleation,gasoline vehicle emissions,diesel vehicle emissions,coal and biomass combustion,and secondary aerosols.The significant changes in source emissions indicate a substantially reduced traffic volume after the implementation of lockdown measures(2644.8#/cm^(3),2202.2#/cm^(3),2792.7#/cm^(3)).Concurrently,photochemical nucleation(310.1#/cm^(3),306.3#/cm^(3),393.1#/cm^(3))and photochemical nucleation aging(592.8#/cm^(3),744.1#/cm^(3),810.7#/cm^(3))exhibited increasing trends,while coal/biomass combustion(1656.6#/cm^(3),1586.2#/cm^(3),980.0#/cm^(3))and secondary sources(999.4#/cm^(3),791.1#/cm^(3),804.1#/cm^(3))showed decreasing trends.In summary,the contributions of traffic emissions to PNC highlight the potential for targeted traffic management strategies to improve urban air quality.展开更多
A cyclone dust collector is applied in many industries. Especially the axial flow cyclone is the mostsimple construction and it keeps high reliability for maintenance. On the other hand, the collectionefficiency of th...A cyclone dust collector is applied in many industries. Especially the axial flow cyclone is the mostsimple construction and it keeps high reliability for maintenance. On the other hand, the collectionefficiency of the cyclone depends not only on the inlet gas velocity but also on the feed particle concentration. The collection efficiency increases with increasing feed particle concentration. However untilnow the problem of how to estimate the collection efficiency depended on the feed particle concentrationis remained except the investigation by Muschelknautz & Brunner~[6]. Therefore in this paper one ofthe estimate method for the collection efficiency of the axial flow cyclones is proposed. The applicationto the geometrically similar type of cyclone of the body diameters D_1=30, 50, 69 and 99 mm showedin good agreement with the experimental results of the collection efficiencies which were described indetail in the paper by Ogawa & Sugiyama~[8].展开更多
The seasonal transport of the Saharan dust to the West African region, near the Gulf of Guinea, during northem winter has been studied over 12 years. Using an optical particle counter, the dust aerosols in the diamete...The seasonal transport of the Saharan dust to the West African region, near the Gulf of Guinea, during northem winter has been studied over 12 years. Using an optical particle counter, the dust aerosols in the diameter range 0.5-25 μm have been sampled at Kumasi （6040＇ N, l°34＇ W） in Ghana during the winter months of January-February from 1997 to 2009. The settling atmospheric dust particles observed during the peak Harmattan and the background Harmattan periods are analysed for the mean particle size, number and mass concentrations as well as the particle size-frequency. It is shown that the average daily particle diameter, number and mass concentrations obtained in the peak Harmattan periods are 1.57 ± 0.54 μm, 50 ± 25 particles/cm3 and 1,130 ± 994 μg/m3, respectively, while for the background Harmattan these values are correspondingly, 1.31 ±0.31 μm, 32 ±12 particles/cm3 and 576 ±429 μg/m3, respectively. These experimental results will be useful for the design of ambient air-filters and for understanding the West African climate change.展开更多
Ultrafine particles are associated with adverse health effects. Total Particle Number Concentration（TNC） of fine particles were measured during 2002 at the St. Louis — Midwest supersite. The time series showed over...Ultrafine particles are associated with adverse health effects. Total Particle Number Concentration（TNC） of fine particles were measured during 2002 at the St. Louis — Midwest supersite. The time series showed overall low level with frequent large peaks. The time series was analyzed alongside criteria pollutant measurements and meteorological observations. Multiple regression analysis was used to identify further contributing factors and to determine the association of different pollutants with TNC levels. This showed the strong contribution of sulfur dioxide（SO2） and nitrogen oxides（NO x） to high TNC levels. The analysis also suggested that increased dispersion resulting from faster winds and higher mixing heights led to higher TNC levels. Overall, the results show that there were intense particle nucleation events in a SO2 rich plume reaching the site which contributed around 29% of TNC. A further 40% was associated with primary emissions from mobile sources. By separating the remaining TNC by time of day and clear sky conditions,we suggest that most likely 8% of TNC are due to regional nucleation events and 23% are associated with the general urban background.展开更多
Particle size distribution of 12-500 nm was measured at Mt. Waliguan, China Global Atmosphere Watch Baseline Observatory, from Aug. in 2005 to May in 2007.72-hr back-trajectories at 100-m arrival height above ground l...Particle size distribution of 12-500 nm was measured at Mt. Waliguan, China Global Atmosphere Watch Baseline Observatory, from Aug. in 2005 to May in 2007.72-hr back-trajectories at 100-m arrival height above ground level for the same period were calculated at 6：00, 12：00, and 21：00 （Beijing Time） for each day using the Hybrid Single-Particle Lagrangian Integrated Trajectory （HYSPLIT-4） model developed by NOAA/ARL. It was found that air mass sources significantly impact particle number concentration and size distribution at Mt. Waliguan. Cluster analysis of back-trajectories show that higher Aitken mode particle number concentration was observed when air masses came from or passed by the northeastern section of Mt. Waliguan, with short trajectory length. High number concentration of nucleation mode was associated with air masses from clean regions, with long trajectory length.展开更多
The TSI-3321 APS was used to measure concentration of atmospheric particulates in Ranjiaba region of Yubei District in Chongqing City during March 21- 29,2014,and the temporal variations in the hourly average mass and...The TSI-3321 APS was used to measure concentration of atmospheric particulates in Ranjiaba region of Yubei District in Chongqing City during March 21- 29,2014,and the temporal variations in the hourly average mass and number concentration and median particle diameter of PM10 and PM2.5 as well as their correlation with relative humidity were analyzed. The results showed that the three indicators of PM10 and PM2.5 except for the mass concentration correlated with relative humidity,of which the correlation between the mass median particle diameter and relative humidity was the best. The correlation coefficient R^2 between the mass median particle diameter of PM10（ PM2.5） and relative humidity was up to 0. 943（ 0. 832）. Therefore,relative humidity and pressure are key impact factors of indicators of particles.展开更多
Direct measurement of slip length is based on the measured fluid velocity near solid boundary. However, previous micro particle image velocimetry/particle tracking velocimetry （microPIV/PTV） measurements have report...Direct measurement of slip length is based on the measured fluid velocity near solid boundary. However, previous micro particle image velocimetry/particle tracking velocimetry （microPIV/PTV） measurements have reported surprisingly large measured near-wall velocities of pressure-driven flow in apparent contradiction with the no-slip hy-pothesis and experimental results from other techniques. To better interpret the measured results of the microPIV/PTV, we performed velocity profile measurements near a hy-drophilic wall （z = 0.25-1.5 μm） with two sizes of tracer particles （φ 50 nm and φ200 nm）. The experimental results indicate that, at less than 1 μm from the wall, the deviations between the measured velocities and no-slip theoretical values obviously decrease from 93% of φ200 nm particles to 48% of φ50 nm particles. The Boltzmann-like exponential measured particle concentrations near wall were found. Based on the non linear Boltzmann distribution of particle concentration and the effective focus plane thickness, we illustrated the reason of the apparent velocity increase near wall and proposed a method to correct the measured velocity profile. By this method, the deviations between the corrected measured velocities and the no-slip theoretical velocity decrease from 45.8% to 10%, and the measured slip length on hy-drophilic glass is revised from 75 nm to 16 nm. These results indicated that the particle size and the biased particle concentration distribution can significantly affect near wall velocity measurement via microPIV/PTV, and result in larger measured velocity and slip length close to wall.展开更多
The Reynolds-averaged general dynamic equation(RAGDE)for the nanoparticle size distribution function is derived,including the contribution to particle coagulation resulting from the fluctuating concentration.The equat...The Reynolds-averaged general dynamic equation(RAGDE)for the nanoparticle size distribution function is derived,including the contribution to particle coagulation resulting from the fluctuating concentration.The equation together with that of a turbulent gas flow is solved numerically in the turbulent flow of a ventilation chamber with a jet on the wall based on the proposed model relating the fluctuating coagulation to the gradient of mean concentration.Some results are compared with the experimental data.The results show that the proposed model relating the fluctuating coagulation to the gradient of mean concentration is reasonable,and it is necessary to consider the contribution to coagulation resulting from the fluctuating concentration in such a flow.The changes of the particle number concentration M_(0) and the geometric mean diameter dg are more obvious in the core area of the jet,but less obvious in other areas.With the increase in the initial particle number concentration m00,the values of M_(0) and the standard deviation of the particle sizeσdecrease,but the value of d_(g) increases.The decrease in the initial particle diameter leads to the reduction of M_(0) andσand the increase in d_(g).With the increase in the Reynolds number,particles have few chances of collision,and hence the coagulation rate is reduced,leading to the increase in M_(0) andσand the decrease in d_(g).展开更多
Novel applications of nanotechnology may lead to the release of engineered nanoparticles（ENPs）, which result in concerns over their potential environmental hazardous impact. It is essential for the research workers ...Novel applications of nanotechnology may lead to the release of engineered nanoparticles（ENPs）, which result in concerns over their potential environmental hazardous impact. It is essential for the research workers to be able to quantitatively characterise ENPs in the environment and subsequently to assist the risk assessment of the ENPs. This study hence explored the application of nanoparticle tracking system（NTA） to quantitatively describe the behaviour of the ENPs in natural sediment-water systems. The NTA allows the measurement of both particle number concentration（PNC） and particle size distribution（PSD） of the ENPs. The developed NTA method was applied to a range of gold and magnetite ENPs with a selection of surface properties. The results showed that the positively-charged ENPs interacted more strongly with the sediment than neutral and negatively-charged ENPs. It was also found that the citrate coated Au ENPs had a higher distribution percentage（53%） than 11-mercaptoundecanoic acid coated Au ENPs（20%） and citrate coated magnetite ENPs（21%）. The principles of the electrostatic interactions between hard（and soft） acids and bases（HSAB） are used to explain such behaviours; the hard base coating（i.e. citrate ions） will interact more strongly with hard acid（i.e. magnetite） than soft acid（i.e. gold）.The results indicate that NTA is a complementary method to existing approaches to characterise the fate and behaviour of ENPs in natural sediment.展开更多
Particulate matter（PM） from cooking has caused seriously indoor air pollutant and aroused risk to human health.It is urged to get deep knowledge of their spatial-temporal distribution of source emission characterist...Particulate matter（PM） from cooking has caused seriously indoor air pollutant and aroused risk to human health.It is urged to get deep knowledge of their spatial-temporal distribution of source emission characteristics,especially ultrafine particles（UFP ＆lt; 100 nm） and accumulation mode particles（AMP 100-555 nm）.Four commercial cooking oils are auto dipped water to simulate cooking fume under heating to 255℃ to investigate PM emission and decay features between 0.03 and 10 μm size dimension by electrical low pressure impactor（ELPI） without ventilation.Rapeseed and sunflower produced high PM_（2.5） around5.1 mg/m^3,in comparison with those of soybean and corn（5.87 and 4.55 mg/m^3,respectively）at peak emission time between 340 and 450 sec since heating oil,but with the same level of particle numbers 6-9 × 10~5/cm^3.Mean values of PM_（1.0）/PM_（2.5） and PM_（2.5）/PM_（10） at peak emission time are around 0.51-0.55 and 0.23-0.29.After 15 min naturally deposition,decay rates of PM_（1.0）,PM_（2.5） and PM_（10） are 13.3%-29.8%,20.1%-33.9%and 41.2%-54.7%,which manifest that PM_（1.0） is quite hard to decay than larger particles,PM_（2.5） and PM_（1.0）.The majority of the particle emission locates at 43 nm with the largest decay rate at 75%,and shifts to a larger size between137 and 555 nm after 15 min decay.The decay rates of the particles are sensitive to the oil type.展开更多
During the Austral summer of 1996/1997, the First Chinese Antarctic Inland Expedition reached the inland area about 330 km along the direction around 76°E from Zhongshan Station, and collected 84 surface snow...During the Austral summer of 1996/1997, the First Chinese Antarctic Inland Expedition reached the inland area about 330 km along the direction around 76°E from Zhongshan Station, and collected 84 surface snow samples at an interval of 4 km . Micro particle analysis of the samples indicates that the micro particle concentration apparently decreases with the increasing of altitude, and the amplitudes of micro particle concentration is much larger in the lower altitude than in the higher altitude. Further analysis of grain size distributions of micro particle, percentage of micro particles from different sources and variations with altitude suggest that micro particles in this area are from a considerably dominant source. Although this area is controlled by polar easterly wind and katabatic wind, transportation and deposition of the micro particles are mainly influenced by marine transportation in coastal area.展开更多
The cyclone separator is an important separation device.This paper presents a new type of embedded two-stage cyclone,which includes a 2 nd-stage cyclone(internal traditional cyclone)with multiple inlets and a 1 st-sta...The cyclone separator is an important separation device.This paper presents a new type of embedded two-stage cyclone,which includes a 2 nd-stage cyclone(internal traditional cyclone)with multiple inlets and a 1 st-stage cyclone(outer cylinder)that unifies the 2 nd-stage cyclone inlets into one inlet.The Taguchi experimental method was used to study the two-stage cyclone separator’s inlet area on its performance.Studies have shown that the increase of the 1 st-stage cyclone inlet area and the increase in the number of 2 nd-stage cyclone inlets(N)positively affect reducing the pressure drop and a negative effect on efficiency.It is recommended to use 2 S(the original 1 st-stage cyclone inlet area)of the 1 st-stage cyclone inlet area and 2 N of the 2 nd-stage cyclone inlets when separating fine particles.Compared with a traditional cyclone,the pressure drop is reduced by 1303 Pa,the mass separation efficiency(Eq)is increased by 0.56%,and the number separation efficiency(En)is increased by 2.05%.When separating larger particles,it is recommended to use 2 S of the 1 st-stage cyclone inlet area and 4 N of the 2 nd-stage cyclone inlets.Compared with a traditional cyclone,although Endecreases slightly,the pressure drop is reduced by 3055 Pa,and the Eqis increased by 0.56%.The research results provide new insight into the design of the cyclone.展开更多
In order to solve the problem that the vulcanizing agent utilization rate is low and the dilution effect of copper slag is poor,the vortex stirring dilution method was used to improve the conditions of the dilution ki...In order to solve the problem that the vulcanizing agent utilization rate is low and the dilution effect of copper slag is poor,the vortex stirring dilution method was used to improve the conditions of the dilution kinetics and copper recovery.The water model was used to simulate the effect of copper slag dilution.Under the premise of keeping the Reynolds number consistent,silicone oil and glass beads were used instead of copper slag and vulcanizing agent.Based on the relationship between voltage and concentration,the PC6D dual-channel particle concentration measuring instrument was used to study the stirring speed and the insertion depth of the stirring paddle in model experiments,and the suitable conditions were speed 250 rpm and insertion depth 70 mm.The fire dilution of copper slag was done under the conditions.After stirring and sedimentation,the Fe_(3)O_(4) in slag decreased from 22.58% to 4.65%,and the copper content of the slag decreased from 2.94% to 0.34%.The copper recovery was 88.44%.展开更多
Based on the analysis of spectrum characteristics of intensity fluctuations while light beams pass through stack gas flow in an industrial setting, this paper puts emphasis upon discussing the spectrum of optical inte...Based on the analysis of spectrum characteristics of intensity fluctuations while light beams pass through stack gas flow in an industrial setting, this paper puts emphasis upon discussing the spectrum of optical intensity fluctuations by the variety of particle concentration in stack gas flow. This paper also gives the primary theoretical explanation of the measurement results in the stack of coal-fired utility boilers. Meanwhile, the cross-correlation formula is given as the theoretical basis of velocity measurement by using particle concentration scintillation.展开更多
Indoor environment separated with down-feed air curtain was numerically simulated and experimen-tally researched. Indoor airflow and temperature fields separated with air curtain were numerically simulated. Re-sults s...Indoor environment separated with down-feed air curtain was numerically simulated and experimen-tally researched. Indoor airflow and temperature fields separated with air curtain were numerically simulated. Re-sults show that both polluted airflow and thermal air current can be separated with a down-feed air curtain to pre-vent contaminants from spreading in the room space. In a test chamber, the smoke of burning Tibetan incense served as the source of contaminants, and the probe test shows that 1.0 μm is the prevailing diameter of the smoke particles. During the release of the smoke, the particle concentration of the indoor air was tested with a laser particle counter at the points of three different heights from the floor when the air curtain was running or not. Experimental results show that the higher the test point is located, the lower the particle concentration is, implying that the sepa-rating or isolating effect decreases as the air velocity of the curtain reduces along with the height descends. Accord-ing to both simulation and experimental results, down-feed air curtain can separate indoor environment effectively when the supply air velocity of air curtain is not less than 3 m/s. In order to strengthen separation effect, it is sug-gested that the supply air velocity be speeded up to 5 m/s.展开更多
The paper presents a simple model for outdoor air contaminant transmission into occupied rooms. In the model, several factors such as filtration, ventilation, deposition, re-emission, outdoor concentration and indoor ...The paper presents a simple model for outdoor air contaminant transmission into occupied rooms. In the model, several factors such as filtration, ventilation, deposition, re-emission, outdoor concentration and indoor sources are included. The model results show that the air exchange rate plays an important role in the transmission of outdoor contaminants into the indoor environment. The model shows that increasing the value of the filtration efficiency decreases the mass concentration of indoor particles. In addition, if outdoor aerosol particles have a periodic behaviour, indoor aerosol particles also behave periodically but smoother. Indoor sources are found to be able to increase indoor concentrations greatly and continuously.展开更多
基金Supported by the National Key Project of Basic Research of the Ministry for Science and Technology of P. R. China (Grant No. 2005CB22120103)
文摘The particle concentration inside a cyclone separator at different operation parameters was simulated with the FLUENT software. The Advanced Reynolds Stress Model （ARSM） was used in gas phase turbulence modeling. Stochastic Particle Tracking Model （SPTM） and the Particle-Source-In-Cell （PSIC） method were adopted for particles computing. The interaction between particles and the gas phase was also taken into account. The numerical simulation results were in agreement with the experimental data. The simulation revealed that an unsteady spiral dust strand appeared near the cyclone wall and a non-axi-symmetrical dust ring appeared in the annular space and under the cover plate of the cyclone. There were two regions in the radial particle concentration distribution, in which particle concentration was low in the inner region （r/R≤0.75） and increased greatly in the outer region （r/R〉0.75）. Large particles generally had higher concentration in the near-wall region and small particles had higher concentration in the inner swirling flow region. The axial distribution of particle concentration in the inner swirling flow （r/R≤0.3） region showed that there existed serious fine particle entrainment within the height of 0.SD above the dust discharge port and a short-cut flow at a distance of about 0.25D below the entrance of the vortex finder. The dimensionless concentration in the high-concentration region increased obviously in the upper part of the cyclone separation space when inlet particle loading was large. With increasing gas temperature, the particle separation ability of the cyclone was obviously weakened.
基金Project supported by the National Natural Science Foundation of China(No.20537020)the "Hundred Talent Scientist Program" of the Chinese Academy of Sciences.
文摘Adsorption/desorption in a new Zn（Ⅱ）-TiO2 adsorption system was investigated at different particle concentrations （Cp）. TEM, SEM and XRD analyses revealed that the TiO2 particles were an aggregation of nano-sized （approximately 10 nm） pure anatase-type TiO2. Adsorption experiments were carried out with particle concentrations of 100, 400 and 1000 mg/L, and their adsorption isotherms were found to decline successively, showing an obvious Cp effect. Desorption experiments indicated that adsorption in this system was irreversible, and the irreversibility increased with increasing Cp. These phenomena could be explained by the MEA （metastable equilibrium adsorption） theory and the Cp effect could be modeled well with an MEA-Freundlich-type Cp effect isotherm equation. This study may heln understand environmental behavior of contaminants on ultrafine natural particles.
基金supported by the Hundred Talents Program of Chinese Academy of Sciences (No. 29O827631)
文摘During the 2012 Lanzhou International Marathon, the local government made a significant effort to improve traffic conditions and air quality by implementing traffic restriction measures. To evaluate the direct effect of these measures on urban air quality, especially particle concentrations and their size distributions, atmospheric particle size distributions （0.5-20μm） obtained using an aerodynamic particle sizer （model 3321, TSI, USA） in June 2012 were analyzed. It was found that the particle number, surface area and volume concentrations for size range 0.5-10 μm were （15.0±2.1） cm-3, （11.8±2.6） μm2/cm3 and （1.9±0.6） μm2/cm3, respectively, on the traffic-restricted day （Sunday）, which is 63.2%, 53.0% and 47.2% lower than those on a normal Sunday. For number and surface area concentrations, the most affected size range was 0.5-0.7 and 0.5-0.8 μm, respectively, while for volume concentration, the most affected size ranges were 0.5-0.8, 1.7-2.0 and 5.0-5.4 μm. Number and volume concentrations of particles in size range 0.5-1.0μm correlated well with the number of non-CNG （Compressed Natural Gas） powered vehicles, while their correlation with the number of CNG-powered vehicles was very low, suggesting that reasonable urban traffic controls along with vehicle technology improvements could play an important role in improving urban air quality.
基金supported by the National Research Program for Key Issues in Air Pollution Control in China(No.DQGG202137)the National Natural Science Foundation of China(No.42277429)。
文摘The COVID-19 lockdown was a typical example of extreme emission reduction,providing an opportunity to study the impact of lockdown measures on air pollution.Particle number concentrations(PNC)originate from direct emissions or through new particle formation events.However,their variations during the lockdown period are under investigation.This study focuses on Luohe,a city on the southern edge of the North China Plain,analyzing the changes in PNC and its sources before,during,and after the COVID-19 lockdown.From March 25^(th)to May 31^(st),2022,real-time PNC measurements were conducted using a Scanning Mobility Particle Sizer for particle size.Results showed an 11.2%decrease in PNC during the lockdown compared to pre-lockdown and a 3.6%decrease compared to post-lockdown,indicating reduced local emissions and weakened regional transportation during the lockdown.Positive Matrix Factorization analysis identified six sources contributing to the total PNC,including photochemical nucleation,aged photochemical nucleation,gasoline vehicle emissions,diesel vehicle emissions,coal and biomass combustion,and secondary aerosols.The significant changes in source emissions indicate a substantially reduced traffic volume after the implementation of lockdown measures(2644.8#/cm^(3),2202.2#/cm^(3),2792.7#/cm^(3)).Concurrently,photochemical nucleation(310.1#/cm^(3),306.3#/cm^(3),393.1#/cm^(3))and photochemical nucleation aging(592.8#/cm^(3),744.1#/cm^(3),810.7#/cm^(3))exhibited increasing trends,while coal/biomass combustion(1656.6#/cm^(3),1586.2#/cm^(3),980.0#/cm^(3))and secondary sources(999.4#/cm^(3),791.1#/cm^(3),804.1#/cm^(3))showed decreasing trends.In summary,the contributions of traffic emissions to PNC highlight the potential for targeted traffic management strategies to improve urban air quality.
文摘A cyclone dust collector is applied in many industries. Especially the axial flow cyclone is the mostsimple construction and it keeps high reliability for maintenance. On the other hand, the collectionefficiency of the cyclone depends not only on the inlet gas velocity but also on the feed particle concentration. The collection efficiency increases with increasing feed particle concentration. However untilnow the problem of how to estimate the collection efficiency depended on the feed particle concentrationis remained except the investigation by Muschelknautz & Brunner~[6]. Therefore in this paper one ofthe estimate method for the collection efficiency of the axial flow cyclones is proposed. The applicationto the geometrically similar type of cyclone of the body diameters D_1=30, 50, 69 and 99 mm showedin good agreement with the experimental results of the collection efficiencies which were described indetail in the paper by Ogawa & Sugiyama~[8].
文摘The seasonal transport of the Saharan dust to the West African region, near the Gulf of Guinea, during northem winter has been studied over 12 years. Using an optical particle counter, the dust aerosols in the diameter range 0.5-25 μm have been sampled at Kumasi （6040＇ N, l°34＇ W） in Ghana during the winter months of January-February from 1997 to 2009. The settling atmospheric dust particles observed during the peak Harmattan and the background Harmattan periods are analysed for the mean particle size, number and mass concentrations as well as the particle size-frequency. It is shown that the average daily particle diameter, number and mass concentrations obtained in the peak Harmattan periods are 1.57 ± 0.54 μm, 50 ± 25 particles/cm3 and 1,130 ± 994 μg/m3, respectively, while for the background Harmattan these values are correspondingly, 1.31 ±0.31 μm, 32 ±12 particles/cm3 and 576 ±429 μg/m3, respectively. These experimental results will be useful for the design of ambient air-filters and for understanding the West African climate change.
基金funded the present analysis through grant number RD-83455701the original measurements through cooperative agreement R-82805901-0
文摘Ultrafine particles are associated with adverse health effects. Total Particle Number Concentration（TNC） of fine particles were measured during 2002 at the St. Louis — Midwest supersite. The time series showed overall low level with frequent large peaks. The time series was analyzed alongside criteria pollutant measurements and meteorological observations. Multiple regression analysis was used to identify further contributing factors and to determine the association of different pollutants with TNC levels. This showed the strong contribution of sulfur dioxide（SO2） and nitrogen oxides（NO x） to high TNC levels. The analysis also suggested that increased dispersion resulting from faster winds and higher mixing heights led to higher TNC levels. Overall, the results show that there were intense particle nucleation events in a SO2 rich plume reaching the site which contributed around 29% of TNC. A further 40% was associated with primary emissions from mobile sources. By separating the remaining TNC by time of day and clear sky conditions,we suggest that most likely 8% of TNC are due to regional nucleation events and 23% are associated with the general urban background.
基金sponsored by National Key Development Program for Fundamental Research (973 Program) Project(Nos.2006CB403703 and 2006CB403701)
文摘Particle size distribution of 12-500 nm was measured at Mt. Waliguan, China Global Atmosphere Watch Baseline Observatory, from Aug. in 2005 to May in 2007.72-hr back-trajectories at 100-m arrival height above ground level for the same period were calculated at 6：00, 12：00, and 21：00 （Beijing Time） for each day using the Hybrid Single-Particle Lagrangian Integrated Trajectory （HYSPLIT-4） model developed by NOAA/ARL. It was found that air mass sources significantly impact particle number concentration and size distribution at Mt. Waliguan. Cluster analysis of back-trajectories show that higher Aitken mode particle number concentration was observed when air masses came from or passed by the northeastern section of Mt. Waliguan, with short trajectory length. High number concentration of nucleation mode was associated with air masses from clean regions, with long trajectory length.
文摘The TSI-3321 APS was used to measure concentration of atmospheric particulates in Ranjiaba region of Yubei District in Chongqing City during March 21- 29,2014,and the temporal variations in the hourly average mass and number concentration and median particle diameter of PM10 and PM2.5 as well as their correlation with relative humidity were analyzed. The results showed that the three indicators of PM10 and PM2.5 except for the mass concentration correlated with relative humidity,of which the correlation between the mass median particle diameter and relative humidity was the best. The correlation coefficient R^2 between the mass median particle diameter of PM10（ PM2.5） and relative humidity was up to 0. 943（ 0. 832）. Therefore,relative humidity and pressure are key impact factors of indicators of particles.
基金supported by the National Natural Science Foundation of China (10872203)the National Basic Research Program(2007AC744701)the CAS Research and Development Program of China (KSCX2-YW-H18)
文摘Direct measurement of slip length is based on the measured fluid velocity near solid boundary. However, previous micro particle image velocimetry/particle tracking velocimetry （microPIV/PTV） measurements have reported surprisingly large measured near-wall velocities of pressure-driven flow in apparent contradiction with the no-slip hy-pothesis and experimental results from other techniques. To better interpret the measured results of the microPIV/PTV, we performed velocity profile measurements near a hy-drophilic wall （z = 0.25-1.5 μm） with two sizes of tracer particles （φ 50 nm and φ200 nm）. The experimental results indicate that, at less than 1 μm from the wall, the deviations between the measured velocities and no-slip theoretical values obviously decrease from 93% of φ200 nm particles to 48% of φ50 nm particles. The Boltzmann-like exponential measured particle concentrations near wall were found. Based on the non linear Boltzmann distribution of particle concentration and the effective focus plane thickness, we illustrated the reason of the apparent velocity increase near wall and proposed a method to correct the measured velocity profile. By this method, the deviations between the corrected measured velocities and the no-slip theoretical velocity decrease from 45.8% to 10%, and the measured slip length on hy-drophilic glass is revised from 75 nm to 16 nm. These results indicated that the particle size and the biased particle concentration distribution can significantly affect near wall velocity measurement via microPIV/PTV, and result in larger measured velocity and slip length close to wall.
基金Project supported by the Major Program of the National Natural Science Foundation of China(No.91852102)。
文摘The Reynolds-averaged general dynamic equation(RAGDE)for the nanoparticle size distribution function is derived,including the contribution to particle coagulation resulting from the fluctuating concentration.The equation together with that of a turbulent gas flow is solved numerically in the turbulent flow of a ventilation chamber with a jet on the wall based on the proposed model relating the fluctuating coagulation to the gradient of mean concentration.Some results are compared with the experimental data.The results show that the proposed model relating the fluctuating coagulation to the gradient of mean concentration is reasonable,and it is necessary to consider the contribution to coagulation resulting from the fluctuating concentration in such a flow.The changes of the particle number concentration M_(0) and the geometric mean diameter dg are more obvious in the core area of the jet,but less obvious in other areas.With the increase in the initial particle number concentration m00,the values of M_(0) and the standard deviation of the particle sizeσdecrease,but the value of d_(g) increases.The decrease in the initial particle diameter leads to the reduction of M_(0) andσand the increase in d_(g).With the increase in the Reynolds number,particles have few chances of collision,and hence the coagulation rate is reduced,leading to the increase in M_(0) andσand the decrease in d_(g).
基金CEFIC LRI,Natural Science Foundation of Jiangsu Province(No.BK20130186)the Fundamental Research Funds for the Central Universities(No.2013QNA18)for funding this project
文摘Novel applications of nanotechnology may lead to the release of engineered nanoparticles（ENPs）, which result in concerns over their potential environmental hazardous impact. It is essential for the research workers to be able to quantitatively characterise ENPs in the environment and subsequently to assist the risk assessment of the ENPs. This study hence explored the application of nanoparticle tracking system（NTA） to quantitatively describe the behaviour of the ENPs in natural sediment-water systems. The NTA allows the measurement of both particle number concentration（PNC） and particle size distribution（PSD） of the ENPs. The developed NTA method was applied to a range of gold and magnetite ENPs with a selection of surface properties. The results showed that the positively-charged ENPs interacted more strongly with the sediment than neutral and negatively-charged ENPs. It was also found that the citrate coated Au ENPs had a higher distribution percentage（53%） than 11-mercaptoundecanoic acid coated Au ENPs（20%） and citrate coated magnetite ENPs（21%）. The principles of the electrostatic interactions between hard（and soft） acids and bases（HSAB） are used to explain such behaviours; the hard base coating（i.e. citrate ions） will interact more strongly with hard acid（i.e. magnetite） than soft acid（i.e. gold）.The results indicate that NTA is a complementary method to existing approaches to characterise the fate and behaviour of ENPs in natural sediment.
基金supported by the strategic project of science and technology of Chinese Academy of Sciences(No.XDB05050000)
文摘Particulate matter（PM） from cooking has caused seriously indoor air pollutant and aroused risk to human health.It is urged to get deep knowledge of their spatial-temporal distribution of source emission characteristics,especially ultrafine particles（UFP ＆lt; 100 nm） and accumulation mode particles（AMP 100-555 nm）.Four commercial cooking oils are auto dipped water to simulate cooking fume under heating to 255℃ to investigate PM emission and decay features between 0.03 and 10 μm size dimension by electrical low pressure impactor（ELPI） without ventilation.Rapeseed and sunflower produced high PM_（2.5） around5.1 mg/m^3,in comparison with those of soybean and corn（5.87 and 4.55 mg/m^3,respectively）at peak emission time between 340 and 450 sec since heating oil,but with the same level of particle numbers 6-9 × 10~5/cm^3.Mean values of PM_（1.0）/PM_（2.5） and PM_（2.5）/PM_（10） at peak emission time are around 0.51-0.55 and 0.23-0.29.After 15 min naturally deposition,decay rates of PM_（1.0）,PM_（2.5） and PM_（10） are 13.3%-29.8%,20.1%-33.9%and 41.2%-54.7%,which manifest that PM_（1.0） is quite hard to decay than larger particles,PM_（2.5） and PM_（1.0）.The majority of the particle emission locates at 43 nm with the largest decay rate at 75%,and shifts to a larger size between137 and 555 nm after 15 min decay.The decay rates of the particles are sensitive to the oil type.
文摘During the Austral summer of 1996/1997, the First Chinese Antarctic Inland Expedition reached the inland area about 330 km along the direction around 76°E from Zhongshan Station, and collected 84 surface snow samples at an interval of 4 km . Micro particle analysis of the samples indicates that the micro particle concentration apparently decreases with the increasing of altitude, and the amplitudes of micro particle concentration is much larger in the lower altitude than in the higher altitude. Further analysis of grain size distributions of micro particle, percentage of micro particles from different sources and variations with altitude suggest that micro particles in this area are from a considerably dominant source. Although this area is controlled by polar easterly wind and katabatic wind, transportation and deposition of the micro particles are mainly influenced by marine transportation in coastal area.
基金financially supported by the National Key Research and Development Program of China(2016YFC0801700)the Project of the National Natural Science Foundation of China(51604018)the Basic Research Funding of the China Academy of Safety Science and Technology(2019JBKY11 and 2019JBKY04)。
文摘The cyclone separator is an important separation device.This paper presents a new type of embedded two-stage cyclone,which includes a 2 nd-stage cyclone(internal traditional cyclone)with multiple inlets and a 1 st-stage cyclone(outer cylinder)that unifies the 2 nd-stage cyclone inlets into one inlet.The Taguchi experimental method was used to study the two-stage cyclone separator’s inlet area on its performance.Studies have shown that the increase of the 1 st-stage cyclone inlet area and the increase in the number of 2 nd-stage cyclone inlets(N)positively affect reducing the pressure drop and a negative effect on efficiency.It is recommended to use 2 S(the original 1 st-stage cyclone inlet area)of the 1 st-stage cyclone inlet area and 2 N of the 2 nd-stage cyclone inlets when separating fine particles.Compared with a traditional cyclone,the pressure drop is reduced by 1303 Pa,the mass separation efficiency(Eq)is increased by 0.56%,and the number separation efficiency(En)is increased by 2.05%.When separating larger particles,it is recommended to use 2 S of the 1 st-stage cyclone inlet area and 4 N of the 2 nd-stage cyclone inlets.Compared with a traditional cyclone,although Endecreases slightly,the pressure drop is reduced by 3055 Pa,and the Eqis increased by 0.56%.The research results provide new insight into the design of the cyclone.
基金Funded by the National Natural Science Foundation of China(52004284)the Fundamental Research Funds from the Central University of the Ministry of Education of China(2020QN55)the China Postdoctoral Science Foundation(2019M661979)。
文摘In order to solve the problem that the vulcanizing agent utilization rate is low and the dilution effect of copper slag is poor,the vortex stirring dilution method was used to improve the conditions of the dilution kinetics and copper recovery.The water model was used to simulate the effect of copper slag dilution.Under the premise of keeping the Reynolds number consistent,silicone oil and glass beads were used instead of copper slag and vulcanizing agent.Based on the relationship between voltage and concentration,the PC6D dual-channel particle concentration measuring instrument was used to study the stirring speed and the insertion depth of the stirring paddle in model experiments,and the suitable conditions were speed 250 rpm and insertion depth 70 mm.The fire dilution of copper slag was done under the conditions.After stirring and sedimentation,the Fe_(3)O_(4) in slag decreased from 22.58% to 4.65%,and the copper content of the slag decreased from 2.94% to 0.34%.The copper recovery was 88.44%.
文摘Based on the analysis of spectrum characteristics of intensity fluctuations while light beams pass through stack gas flow in an industrial setting, this paper puts emphasis upon discussing the spectrum of optical intensity fluctuations by the variety of particle concentration in stack gas flow. This paper also gives the primary theoretical explanation of the measurement results in the stack of coal-fired utility boilers. Meanwhile, the cross-correlation formula is given as the theoretical basis of velocity measurement by using particle concentration scintillation.
基金Supported by Science Foundation of Tianjin Higher Educational Committee (No. 20031109).
文摘Indoor environment separated with down-feed air curtain was numerically simulated and experimen-tally researched. Indoor airflow and temperature fields separated with air curtain were numerically simulated. Re-sults show that both polluted airflow and thermal air current can be separated with a down-feed air curtain to pre-vent contaminants from spreading in the room space. In a test chamber, the smoke of burning Tibetan incense served as the source of contaminants, and the probe test shows that 1.0 μm is the prevailing diameter of the smoke particles. During the release of the smoke, the particle concentration of the indoor air was tested with a laser particle counter at the points of three different heights from the floor when the air curtain was running or not. Experimental results show that the higher the test point is located, the lower the particle concentration is, implying that the sepa-rating or isolating effect decreases as the air velocity of the curtain reduces along with the height descends. Accord-ing to both simulation and experimental results, down-feed air curtain can separate indoor environment effectively when the supply air velocity of air curtain is not less than 3 m/s. In order to strengthen separation effect, it is sug-gested that the supply air velocity be speeded up to 5 m/s.
基金Funded by Beijing Higher Education Young Elite Teacher Project(No.YETP0371)National Key Technologies R&D Program of China(No.2012BAJ02B02)
文摘The paper presents a simple model for outdoor air contaminant transmission into occupied rooms. In the model, several factors such as filtration, ventilation, deposition, re-emission, outdoor concentration and indoor sources are included. The model results show that the air exchange rate plays an important role in the transmission of outdoor contaminants into the indoor environment. The model shows that increasing the value of the filtration efficiency decreases the mass concentration of indoor particles. In addition, if outdoor aerosol particles have a periodic behaviour, indoor aerosol particles also behave periodically but smoother. Indoor sources are found to be able to increase indoor concentrations greatly and continuously.
