We numerically investigate the formation and interaction of a parabolic-shaped pulse pair in a passively mode-locked Yb-doped fiber laser. Based on a lumped model, the parabolic-shaped pulse pair is obtained by contro...We numerically investigate the formation and interaction of a parabolic-shaped pulse pair in a passively mode-locked Yb-doped fiber laser. Based on a lumped model, the parabolic-shaped pulse pair is obtained by controlling the intercavity average dispersion and gain saturation energy, Moreover, pulse repulsive and attractive motion are also achieved with different pulse separations. Simulation results show that the phase shift plays an important role in pulse interaction, and the interaction is determined by the inter-cavity average dispersion and gain saturation energy, i.e., the strength of the interaction is proportional to the gain saturation energy, a stronger gain saturation energy will result in a higher interaction intensity. On the contrary, the increase of the inter-cavity dispersion will counterbalance some interaction force. The results also show that the interaction of a parabolic-shaped pulse pair has a larger interaction distance compared to conventional solitons.展开更多
Amplifying the attosecond pulse by the chirp pulse amplification method is impossible. Furthermore, the intensity of attosecond pulse is low in the interaction of laser pulse and underdense plasma. This motivates us t...Amplifying the attosecond pulse by the chirp pulse amplification method is impossible. Furthermore, the intensity of attosecond pulse is low in the interaction of laser pulse and underdense plasma. This motivates us to propose using a multi-color pulse to produce the high intense attosecond pulse. In the present study, the relativistic interaction of a three-color linearly-polarized laser-pulse with highly overdense plasma is studied. We show that the combination of ω1, ω2 and ω3 frequencies decreases the instance full width at half maximum reflected attosecond pulse train from the overdense plasma surface. Moreover, we show that the three-color pulse increases the intensity of generated harmonics, which is explained by the relativistic oscillating mirror model. The obtained results demonstrate that if the three-color laser pulse interacts with overdense plasma, it will enhance two orders of magnitude of intensity of ultra short attosecond pulses in comparison with monochromatic pulse.展开更多
Self-injection and acceleration of monoenergetic electron beams from laser wakefield accelerators are first investigated in the highly relativistic regime, using 100 TW class, 27 fs laser pulses. Quasi-monoenergetic m...Self-injection and acceleration of monoenergetic electron beams from laser wakefield accelerators are first investigated in the highly relativistic regime, using 100 TW class, 27 fs laser pulses. Quasi-monoenergetic multi- bunched beams with energies as high as multi-hundredMeV are observed with simultaneous measurements of side-scattering emissions that indicate the formation of self-channelfing and self-injection of electrons into a plasma wake, referred to as a ＇bubble＇. The three-dimensional particle-in-cell simulations confirmed multiple self-injection of electron bunches into the bubble and their beam acceleration with gradient of 1.5 GeV/cm.展开更多
A scheme of generating energetic ions by the interaction of an ultrahigh-intensity laser pulse and a thin solid foil is studied. The combination of the effects of radiation pressure and Coulomb explosion makes the ion...A scheme of generating energetic ions by the interaction of an ultrahigh-intensity laser pulse and a thin solid foil is studied. The combination of the effects of radiation pressure and Coulomb explosion makes the ion acceleration more effective. The maximum ion velocity variation with time is predicted theoretically while the temporal evolution of the electrostatic field due to the Coulomb explosion is taken into consideration. Two-dimensional particle-in-cell simulations are done to verify the theory.展开更多
In one-dimensional particle-in-cell simulations, this paper shows that the formation of multiple ion bunches is disadvantageous to the generation of monoenergetic ion beams and can be suppressed by choosing an optimum...In one-dimensional particle-in-cell simulations, this paper shows that the formation of multiple ion bunches is disadvantageous to the generation of monoenergetic ion beams and can be suppressed by choosing an optimum target thickness in the radiation pressure acceleration mechanism by a circularly polarised laser pulse. As the laser pulse becomes intense, the optimum target thickness obtained by a non-relativistic treatment is no longer adequate. Considering the relativistic Doppler-shifted pressure, it proposes a relativistic formulation to determine the optimum target thickness. The theoretical predictions agree with the simulation results well. The model is also valid for two-dimensional cases. The accelerated ion beams can be compelled to be more stable by choosing the optimum target thickness when they exhibit some unstable behaviours.展开更多
Spectral-broadening of the APOLLON PW-class laser pulses using a thin-film compression technique within the longfocal-area interaction chamber of the APOLLON laser facility is reported,demonstrating the delivery of th...Spectral-broadening of the APOLLON PW-class laser pulses using a thin-film compression technique within the longfocal-area interaction chamber of the APOLLON laser facility is reported,demonstrating the delivery of the full energy pulse to the target interaction area.The laser pulse at 7 J passing through large aperture,thin glass wafers is spectrally broadened to a bandwidth that is compatible with a 15-fs pulse,indicating also the possibility to achieve sub-10-fs pulses using 14 J.Placing the post-compressor near the interaction makes for an economical method to produce the shortest pulses by limiting the need for high damage,broadband optics close to the final target rather than throughout the entire laser transport system.展开更多
The post-compression technique based on self-phase modulation of high-energy pulses leads to an increase in achievable peak power and intensity.Typically,the pulses considered in experiments have been less than 100 fs...The post-compression technique based on self-phase modulation of high-energy pulses leads to an increase in achievable peak power and intensity.Typically,the pulses considered in experiments have been less than 100 fs in duration.Here,the method is applied to the ELFIE laser system at the LULI facility,for a pulse of 7 J energy and an initial measured duration of 350 fs.A 5-mm-thick fused silica window and a 2 mm cyclic-olefin polymer were used as optical nonlinear materials.The 9 cm diameter beam was spectrally broadened to a bandwidth corresponding to 124 fs Fourier-limited pulse duration,and then it was partly post-compressed to 200 fs.After measuring the spatial spectra of the beam fluence,a uniform gain factor of 4 increase in the fluctuations over the studied range of frequencies is observed,due to small-scale self-focusing.展开更多
The interactions between the new organometallic complexes, ferrocenesubstituted dithioocarborane conjugates （denoted as FcSB1, FcSB2 and FcSBCO） and hemoglobin （Hb） are investigated by electrochemistry, fluorescen...The interactions between the new organometallic complexes, ferrocenesubstituted dithioocarborane conjugates （denoted as FcSB1, FcSB2 and FcSBCO） and hemoglobin （Hb） are investigated by electrochemistry, fluorescence and UVvis absorption spectroscopy. The results demonstrate that FcSB1, FcSB2 and FcSBCO can bind to the heme iron center through the replacement of the weakly bound H20/02 in the distal heme pocket of Hb by their sulfur donor atoms, inducing the allosteric change from the R state （oxygenated conformation, relax） to T state （deoxygenated conformation, tense）. The binding affinity is in the order of FcSBCO〉FeSB2〉FeSB1. Moreover, the fluorescence study illustrates that the three ferrocenecarborane conjugates differently affect the quarterly and tertiary structures as well as the polarity in the surrounding of the Trp and Tyr residues in Hb. Typically, FcSB2 mainly induces alterations of the microenvironment around the 1337Trp residue which is located on the cql32 interface of Hb. Such distinct influences are attributed to the structural features of FcSB1, FcSB2 and FcSBCO containing hydrophobic ferrocenyl and carboranyl units as well as C=O group. Screening the proteinbinding behavior can signify the potential bioactivity of such molecules and may be helpful in the future development of promising multifunctional metallodrugs.展开更多
The collective response of electrons in an ultrathin foil target irradiated by an ultraintense(~6×10^(20)W cm^(-2)) laser pulse is investigated experimentally and via 3D particle-in-cell simulations. It is shown ...The collective response of electrons in an ultrathin foil target irradiated by an ultraintense(~6×10^(20)W cm^(-2)) laser pulse is investigated experimentally and via 3D particle-in-cell simulations. It is shown that if the target is sufficiently thin that the laser induces significant radiation pressure, but not thin enough to become relativistically transparent to the laser light, the resulting relativistic electron beam is elliptical, with the major axis of the ellipse directed along the laser polarization axis. When the target thickness is decreased such that it becomes relativistically transparent early in the interaction with the laser pulse, diffraction of the transmitted laser light occurs through a so called ‘relativistic plasma aperture', inducing structure in the spatial-intensity profile of the beam of energetic electrons. It is shown that the electron beam profile can be modified by variation of the target thickness and degree of ellipticity in the laser polarization.展开更多
A new crystal spectrometer for application in X-ray opacity experiments is proposed. The conditions necessary to yield broad spectral coverage with a resolution >500, strong rejection of hard X-ray backgrounds and ...A new crystal spectrometer for application in X-ray opacity experiments is proposed. The conditions necessary to yield broad spectral coverage with a resolution >500, strong rejection of hard X-ray backgrounds and negligible source broadening for extended sources are formulated. In addition, the design, response modeling and reporting of an elliptical crystal spectrometer in conjunction with a linear detector are presented. The measured results demonstrate the performance of the new crystal spectrometer with a broad energy coverage range, high spectral resolution, and high luminosity(good collection efficiency). This spectrometer can be used in combination with point-projection backlighting techniques as utilized in X-ray opacity experiments. Specifically, the X-ray source, transmission and self-emission spectra of the sample can be measured simultaneously in a single shot, which can reduce the experimental uncertainties from shot-to-shot fluctuations. The new crystal spectrometer has been used in the X-ray opacity experiment to precisely measure the aluminum K-absorption edge shift in the energy range around 1.560 keV in strongly compressed matter. It is demonstrated that the spectrometer can be used to realize measurements of new and unpredictable physical interactions of interest, as well as basic and applied high-energy-density science.展开更多
Modern chirped pulse amplification laser systems with continuously improving controllability and increasing power are about to reach intensities of up to 10^(22) W cm^(-2) and have proven their potential to accelerate...Modern chirped pulse amplification laser systems with continuously improving controllability and increasing power are about to reach intensities of up to 10^(22) W cm^(-2) and have proven their potential to accelerate ions out of plasma to several tens percent of the speed of light. For enabling application, one important step is to increase the repetition rate at which ion bunches are at the disposal. In particular, techniques used so far for thin foil target production can require several days of preparing reasonable amounts for a single campaign. In this paper we describe the reasonably droplet method which we have tested and improved so that the emerging foils with thicknesses of a few nanometres up to micrometre can be used as targets for laser ion acceleration. Their quality and performance can compete with so far employed techniques thereby enabling the production of hundreds of targets per day.展开更多
The application of laser pulses with psec or shorter duration enables nonthermal efficient ultrahigh acceleration of plasma blocks with homogeneous high ion energies exceeding ion current densities of 10^(12) A cm^(-2...The application of laser pulses with psec or shorter duration enables nonthermal efficient ultrahigh acceleration of plasma blocks with homogeneous high ion energies exceeding ion current densities of 10^(12) A cm^(-2). The effects of ultrahigh acceleration of plasma blocks with high energy proton beams are proposed for muon production in a compact magnetic fusion device. The proposed new scheme consists of an ignition fusion spark by muon catalyzed fusion(μCF) in a small mirror-like configuration where low temperature D–T plasma is trapped for a duration of 1 μs. This initial fusion spark produces sufficient alpha heating in order to initiate the fusion process in the main device. The use of a multi-fluid global particle and energy balance code allows us to follow the temporal evolution of the reaction rate of the fusion process in the device. Recent progress on the ICAN and IZEST projects for high efficient high power and high repetition rate laser systems allows development of the proposed device for clean energy production. With the proposed approaches,experiments on fusion nuclear reactions and μCF process can be performed in magnetized plasmas in existing kJ/PW laser facilities as the GEKKO-LFEX, the PETAL and the ORION or in the near future laser facilities as the ELI-NP Romanian pillar.展开更多
基金Project supported by the National Natural Science Foundation of China (Grant No. 60372061)the Scientific Forefront and Interdisciplinary Innovation Project of Jilin University, China (Grant No. 200903296)
文摘We numerically investigate the formation and interaction of a parabolic-shaped pulse pair in a passively mode-locked Yb-doped fiber laser. Based on a lumped model, the parabolic-shaped pulse pair is obtained by controlling the intercavity average dispersion and gain saturation energy, Moreover, pulse repulsive and attractive motion are also achieved with different pulse separations. Simulation results show that the phase shift plays an important role in pulse interaction, and the interaction is determined by the inter-cavity average dispersion and gain saturation energy, i.e., the strength of the interaction is proportional to the gain saturation energy, a stronger gain saturation energy will result in a higher interaction intensity. On the contrary, the increase of the inter-cavity dispersion will counterbalance some interaction force. The results also show that the interaction of a parabolic-shaped pulse pair has a larger interaction distance compared to conventional solitons.
文摘Amplifying the attosecond pulse by the chirp pulse amplification method is impossible. Furthermore, the intensity of attosecond pulse is low in the interaction of laser pulse and underdense plasma. This motivates us to propose using a multi-color pulse to produce the high intense attosecond pulse. In the present study, the relativistic interaction of a three-color linearly-polarized laser-pulse with highly overdense plasma is studied. We show that the combination of ω1, ω2 and ω3 frequencies decreases the instance full width at half maximum reflected attosecond pulse train from the overdense plasma surface. Moreover, we show that the three-color pulse increases the intensity of generated harmonics, which is explained by the relativistic oscillating mirror model. The obtained results demonstrate that if the three-color laser pulse interacts with overdense plasma, it will enhance two orders of magnitude of intensity of ultra short attosecond pulses in comparison with monochromatic pulse.
文摘Self-injection and acceleration of monoenergetic electron beams from laser wakefield accelerators are first investigated in the highly relativistic regime, using 100 TW class, 27 fs laser pulses. Quasi-monoenergetic multi- bunched beams with energies as high as multi-hundredMeV are observed with simultaneous measurements of side-scattering emissions that indicate the formation of self-channelfing and self-injection of electrons into a plasma wake, referred to as a ＇bubble＇. The three-dimensional particle-in-cell simulations confirmed multiple self-injection of electron bunches into the bubble and their beam acceleration with gradient of 1.5 GeV/cm.
基金Project supported by National Natural Science Foundation of China (Grant Nos 10675155 and 10834008)the 973 Program (GrantNo 2006CB806004)Japan-Korea-China Cooperative Project on High Energy Density Sciences for Laser Fusion Energy
文摘A scheme of generating energetic ions by the interaction of an ultrahigh-intensity laser pulse and a thin solid foil is studied. The combination of the effects of radiation pressure and Coulomb explosion makes the ion acceleration more effective. The maximum ion velocity variation with time is predicted theoretically while the temporal evolution of the electrostatic field due to the Coulomb explosion is taken into consideration. Two-dimensional particle-in-cell simulations are done to verify the theory.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.10875015,10725521 and 10834008)the National Basic Research Program of China(Grant No.2006CB806004)
文摘In one-dimensional particle-in-cell simulations, this paper shows that the formation of multiple ion bunches is disadvantageous to the generation of monoenergetic ion beams and can be suppressed by choosing an optimum target thickness in the radiation pressure acceleration mechanism by a circularly polarised laser pulse. As the laser pulse becomes intense, the optimum target thickness obtained by a non-relativistic treatment is no longer adequate. Considering the relativistic Doppler-shifted pressure, it proposes a relativistic formulation to determine the optimum target thickness. The theoretical predictions agree with the simulation results well. The model is also valid for two-dimensional cases. The accelerated ion beams can be compelled to be more stable by choosing the optimum target thickness when they exhibit some unstable behaviours.
基金the support in this work provided through the project SBUF (ELI-RO 16/2020)
文摘Spectral-broadening of the APOLLON PW-class laser pulses using a thin-film compression technique within the longfocal-area interaction chamber of the APOLLON laser facility is reported,demonstrating the delivery of the full energy pulse to the target interaction area.The laser pulse at 7 J passing through large aperture,thin glass wafers is spectrally broadened to a bandwidth that is compatible with a 15-fs pulse,indicating also the possibility to achieve sub-10-fs pulses using 14 J.Placing the post-compressor near the interaction makes for an economical method to produce the shortest pulses by limiting the need for high damage,broadband optics close to the final target rather than throughout the entire laser transport system.
基金This work was supported by the Center of Excellence‘Center of Photonics’,Ministry of Science and Higher Education of the Russian Federation(contract No.075-15-2020-906)Project ELI-RO 16/2020 SBUF funded by the Institute for Atomic Physics(IFA)and by the Council for Doctoral Studies(CSUD),University of Bucharest.
文摘The post-compression technique based on self-phase modulation of high-energy pulses leads to an increase in achievable peak power and intensity.Typically,the pulses considered in experiments have been less than 100 fs in duration.Here,the method is applied to the ELFIE laser system at the LULI facility,for a pulse of 7 J energy and an initial measured duration of 350 fs.A 5-mm-thick fused silica window and a 2 mm cyclic-olefin polymer were used as optical nonlinear materials.The 9 cm diameter beam was spectrally broadened to a bandwidth corresponding to 124 fs Fourier-limited pulse duration,and then it was partly post-compressed to 200 fs.After measuring the spatial spectra of the beam fluence,a uniform gain factor of 4 increase in the fluctuations over the studied range of frequencies is observed,due to small-scale self-focusing.
基金supported by the National Basic Research Program of China (2010CB732404, 2010CB923303)the National Natural Science Foundation of China (21175020, 90713023, 20925104)+4 种基金the Project of High Technology Research and Development Program of China (2007AA022007)Gongdong Province (2011B090400357)the Natural Science Foundation of Jiangsu Province (BK2008149, BK2010052)C. W. acknowledges the Fundamental Research Funds for the Central Universities (ZYGX2011J099)the support by the Open Research Fund of State Key Laboratory of Bioelectronics, Southeast University (2011E09)
文摘The interactions between the new organometallic complexes, ferrocenesubstituted dithioocarborane conjugates （denoted as FcSB1, FcSB2 and FcSBCO） and hemoglobin （Hb） are investigated by electrochemistry, fluorescence and UVvis absorption spectroscopy. The results demonstrate that FcSB1, FcSB2 and FcSBCO can bind to the heme iron center through the replacement of the weakly bound H20/02 in the distal heme pocket of Hb by their sulfur donor atoms, inducing the allosteric change from the R state （oxygenated conformation, relax） to T state （deoxygenated conformation, tense）. The binding affinity is in the order of FcSBCO〉FeSB2〉FeSB1. Moreover, the fluorescence study illustrates that the three ferrocenecarborane conjugates differently affect the quarterly and tertiary structures as well as the polarity in the surrounding of the Trp and Tyr residues in Hb. Typically, FcSB2 mainly induces alterations of the microenvironment around the 1337Trp residue which is located on the cql32 interface of Hb. Such distinct influences are attributed to the structural features of FcSB1, FcSB2 and FcSBCO containing hydrophobic ferrocenyl and carboranyl units as well as C=O group. Screening the proteinbinding behavior can signify the potential bioactivity of such molecules and may be helpful in the future development of promising multifunctional metallodrugs.
基金supported by EPSRC (grants:EP/J003832/1,EP/M018091/1,EP/L001357/1,EP/K022415/1 and EP/L000237/1)EPSRC grant EP/G054940/1+2 种基金STFC (grant number ST/K502340/1)the US Air Force Office of Scientific Research (grant:FA8655-13-1-3008)the European Unions Horizon 2020 research and innovation programme (grant agreement No 654148 Laserlab-Europe)
文摘The collective response of electrons in an ultrathin foil target irradiated by an ultraintense(~6×10^(20)W cm^(-2)) laser pulse is investigated experimentally and via 3D particle-in-cell simulations. It is shown that if the target is sufficiently thin that the laser induces significant radiation pressure, but not thin enough to become relativistically transparent to the laser light, the resulting relativistic electron beam is elliptical, with the major axis of the ellipse directed along the laser polarization axis. When the target thickness is decreased such that it becomes relativistically transparent early in the interaction with the laser pulse, diffraction of the transmitted laser light occurs through a so called ‘relativistic plasma aperture', inducing structure in the spatial-intensity profile of the beam of energetic electrons. It is shown that the electron beam profile can be modified by variation of the target thickness and degree of ellipticity in the laser polarization.
基金supported by the National Natural Science Foundation of China (Nos. 11575168 and 61475146)the funding through IFSA Collaborative Innovation Center, Shanghai Jiao Tong University, Shanghai 200240, China
文摘A new crystal spectrometer for application in X-ray opacity experiments is proposed. The conditions necessary to yield broad spectral coverage with a resolution >500, strong rejection of hard X-ray backgrounds and negligible source broadening for extended sources are formulated. In addition, the design, response modeling and reporting of an elliptical crystal spectrometer in conjunction with a linear detector are presented. The measured results demonstrate the performance of the new crystal spectrometer with a broad energy coverage range, high spectral resolution, and high luminosity(good collection efficiency). This spectrometer can be used in combination with point-projection backlighting techniques as utilized in X-ray opacity experiments. Specifically, the X-ray source, transmission and self-emission spectra of the sample can be measured simultaneously in a single shot, which can reduce the experimental uncertainties from shot-to-shot fluctuations. The new crystal spectrometer has been used in the X-ray opacity experiment to precisely measure the aluminum K-absorption edge shift in the energy range around 1.560 keV in strongly compressed matter. It is demonstrated that the spectrometer can be used to realize measurements of new and unpredictable physical interactions of interest, as well as basic and applied high-energy-density science.
基金supported by the DFG funded Cluster of Excellence Munich Centre for Advanced Photonics and the Transregio 18
文摘Modern chirped pulse amplification laser systems with continuously improving controllability and increasing power are about to reach intensities of up to 10^(22) W cm^(-2) and have proven their potential to accelerate ions out of plasma to several tens percent of the speed of light. For enabling application, one important step is to increase the repetition rate at which ion bunches are at the disposal. In particular, techniques used so far for thin foil target production can require several days of preparing reasonable amounts for a single campaign. In this paper we describe the reasonably droplet method which we have tested and improved so that the emerging foils with thicknesses of a few nanometres up to micrometre can be used as targets for laser ion acceleration. Their quality and performance can compete with so far employed techniques thereby enabling the production of hundreds of targets per day.
文摘The application of laser pulses with psec or shorter duration enables nonthermal efficient ultrahigh acceleration of plasma blocks with homogeneous high ion energies exceeding ion current densities of 10^(12) A cm^(-2). The effects of ultrahigh acceleration of plasma blocks with high energy proton beams are proposed for muon production in a compact magnetic fusion device. The proposed new scheme consists of an ignition fusion spark by muon catalyzed fusion(μCF) in a small mirror-like configuration where low temperature D–T plasma is trapped for a duration of 1 μs. This initial fusion spark produces sufficient alpha heating in order to initiate the fusion process in the main device. The use of a multi-fluid global particle and energy balance code allows us to follow the temporal evolution of the reaction rate of the fusion process in the device. Recent progress on the ICAN and IZEST projects for high efficient high power and high repetition rate laser systems allows development of the proposed device for clean energy production. With the proposed approaches,experiments on fusion nuclear reactions and μCF process can be performed in magnetized plasmas in existing kJ/PW laser facilities as the GEKKO-LFEX, the PETAL and the ORION or in the near future laser facilities as the ELI-NP Romanian pillar.
