As part of“The Earth Summit Mission-2022”during the second Tibetan Plateau Scientific Expedition and Research(STEP)in April and May 2022,we conducted the ozone sounding experiment(an ozonesonde mated to a radiosonde...As part of“The Earth Summit Mission-2022”during the second Tibetan Plateau Scientific Expedition and Research(STEP)in April and May 2022,we conducted the ozone sounding experiment(an ozonesonde mated to a radiosonde)at Mt.Qomolangma Base Camp(MQBC;86.85°E,28.14°N;5200 m),a location at an extremely high altitude.A total of ten sounding profiles were obtained between April 30 and May 06,2022,of which seven profiles were above35 km in altitude,with a maximum detection altitude up to 39.0 km.This study presents the temporal variation and vertical distributions of atmospheric temperature,humidity,and ozone during the MQBC campaign.The averaged ozone concentration was high(68.3 ppbv)at the surface and then increased smoothly until peaking(~110 ppbv)in the middle troposphere(approximately 10 km),and afterward,the ozone concentration increased rapidly from the upper troposphere to a maximum of~10 ppmv at~30 km.The enhanced ozone concentration in the middle troposphere was associated with the blocking high pressure,and transport from the southern flank of the Himalayas occurred during the campaign period.The average total ozone column was 291.9±21.4 DU for the seven profiles exceeding 35km in altitude.The ozonesonde measurements were also compared with the vertical ozone profiles retrieved from the space-borne ozone products from the Microwave Limb Sounder(MLS)onboard the Aura satellite and the Atmospheric Infrared Sounder(AIRS)onboard the Aqua satellite.展开更多
The first shipborne ozone soundings(0–30 km) campaign in the South China Sea was conducted from 22 May to 15 June 2023, aiming to better investigate the ozone vertical structure over the South China Sea. Results show...The first shipborne ozone soundings(0–30 km) campaign in the South China Sea was conducted from 22 May to 15 June 2023, aiming to better investigate the ozone vertical structure over the South China Sea. Results show that ozone concentrations in the boundary layer over the South China Sea are higher than those at tropical marine sites. Balloon measurements revealed finer ozone lamina structures that satellite and reanalysis data could not reproduce. Notably, ozone in the upper troposphere(~13.5 km) decreased significantly due to transport by a tropical cyclone, while it increased slightly in the middle troposphere. These measurements provide valuable insights into ozone's chemical structure and support the need for long-term monitoring of the vertical evolution of ozone from the surface to the middle stratosphere over oceanic regions.展开更多
基金supported by the second Tibetan Plateau Scientific Expedition and Research Program(STEP,2019QZKK0606,2019QZKK0604)the National Natural Science Foundation of China(Grant No.41875183)。
文摘As part of“The Earth Summit Mission-2022”during the second Tibetan Plateau Scientific Expedition and Research(STEP)in April and May 2022,we conducted the ozone sounding experiment(an ozonesonde mated to a radiosonde)at Mt.Qomolangma Base Camp(MQBC;86.85°E,28.14°N;5200 m),a location at an extremely high altitude.A total of ten sounding profiles were obtained between April 30 and May 06,2022,of which seven profiles were above35 km in altitude,with a maximum detection altitude up to 39.0 km.This study presents the temporal variation and vertical distributions of atmospheric temperature,humidity,and ozone during the MQBC campaign.The averaged ozone concentration was high(68.3 ppbv)at the surface and then increased smoothly until peaking(~110 ppbv)in the middle troposphere(approximately 10 km),and afterward,the ozone concentration increased rapidly from the upper troposphere to a maximum of~10 ppmv at~30 km.The enhanced ozone concentration in the middle troposphere was associated with the blocking high pressure,and transport from the southern flank of the Himalayas occurred during the campaign period.The average total ozone column was 291.9±21.4 DU for the seven profiles exceeding 35km in altitude.The ozonesonde measurements were also compared with the vertical ozone profiles retrieved from the space-borne ozone products from the Microwave Limb Sounder(MLS)onboard the Aura satellite and the Atmospheric Infrared Sounder(AIRS)onboard the Aqua satellite.
基金supported by the National Natural Science Foundation of China (Grant Nos.42394121,41675040)the Guangzhou Science and Technology Planning Program (202201010482)。
文摘The first shipborne ozone soundings(0–30 km) campaign in the South China Sea was conducted from 22 May to 15 June 2023, aiming to better investigate the ozone vertical structure over the South China Sea. Results show that ozone concentrations in the boundary layer over the South China Sea are higher than those at tropical marine sites. Balloon measurements revealed finer ozone lamina structures that satellite and reanalysis data could not reproduce. Notably, ozone in the upper troposphere(~13.5 km) decreased significantly due to transport by a tropical cyclone, while it increased slightly in the middle troposphere. These measurements provide valuable insights into ozone's chemical structure and support the need for long-term monitoring of the vertical evolution of ozone from the surface to the middle stratosphere over oceanic regions.
