Soil erosion is one of the major global hazards threatening the food security of the world population.Soil erosion can be a result of both natural and anthropogenic processes.Field monitoring and models(numerical and ...Soil erosion is one of the major global hazards threatening the food security of the world population.Soil erosion can be a result of both natural and anthropogenic processes.Field monitoring and models(numerical and physical)are commonly used to quantify soil erosion.However,field methods are time-consuming and the models inherently work with a level of uncertainty.Soil erosion studies in the Himalayas have been mostly carried out using modelling but there is a lack of sufficient field data to validate the results.We quantified soil erosion in a small catchment(Pranmati)in the Himalayas using the fallout meteoric^(10)Be nuclide for the first time.Based on the^(10)Be flux delivery rates determined from global circulation models(GCM),we calculated the rates of soil erosion at discrete points in the hilltop and mid-slope regions of hillslopes.The erosion rates vary between 17 mm kyr^(-1)to 68 mm kyr^(-1).These rates were determined in pristine areas that are unaffected by anthropogenic activities,thus,indicate the background erosion rates in the region.We established empirical relationships with estimated erosion rates and topographic parameters to assess the sediment dynamics in the hillslopes.It was observed that the sediment redistribution process operates differently in the mid-slope region compared to the hilltop region,due to increasing complexity of the active processes in the mid-slope region.展开更多
In current neural network algorithms for nuclide identification in high-background,poor-resolution detectors,traditional network paradigms including back-propagation networks,convolutional neural networks,recurrent ne...In current neural network algorithms for nuclide identification in high-background,poor-resolution detectors,traditional network paradigms including back-propagation networks,convolutional neural networks,recurrent neural networks,etc.,have been limited in research on γ spectrum analysis because of their inherent mathematical mechanisms.It is difficult to make progress in terms of training data requirements and prediction accuracy.In contrast to traditional network paradigms,network models based on the transformer structure have the characteristics of parallel computing,position encoding,and deep stacking,which have enabled good performance in natural language processing tasks in recent years.Therefore,in this paper,a transformer-based neural network (TBNN) model is proposed to achieve nuclide identification for the first time.First,the Geant4 program was used to generate the basic single-nuclide energy spectrum through Monte Carlo simulations.A multi-nuclide energy spectrum database was established for neural network training using random matrices of γ-ray energy,activity,and noise.Based on the encoder–decoder structure,a network topology based on the transformer was built,transforming the 1024-channel energy spectrum data into a 32×32 energy spectrum sequence as the model input.Through experiments and adjustments of model parameters,including the learning rate of the TBNN model,number of attention heads,and number of network stacking layers,the overall recognition rate reached 98.7%.Additionally,this database was used for training AI models such as back-propagation networks,convolutional neural networks,residual networks,and long shortterm memory neural networks,with overall recognition rates of 92.8%,95.3%,96.3%,and 96.6%,respectively.This indicates that the TBNN model exhibited better nuclide identification among these AI models,providing an important reference and theoretical basis for the practical application of transformers in the qualitative and quantitative analysis of the γ spectrum.展开更多
Radiopharmaceuticals operate by combining radionuclides with carriers.The radiation energy emitted by radionuclides is utilized to selectively irradiate diseased tissues while minimizing damage to healthy tissues.In c...Radiopharmaceuticals operate by combining radionuclides with carriers.The radiation energy emitted by radionuclides is utilized to selectively irradiate diseased tissues while minimizing damage to healthy tissues.In comparison to external beam radiation therapy,radionuclide drugs demonstrate research potential due to their biological targeting capabilities and reduced normal tissue toxicity.This article reviews the applications and research progress of radiopharmaceuticals in cancer treatment.Several key radionuclides are examined,including^(223)Ra,^(90)Y,Lutetium-177(^(177)Lu),212 Pb,and Actinium-225(^(225)Ac).It also explores the current development trends of radiopharmaceuticals,encompassing the introduction of novel radionuclides,advancements in imaging technologies,integrated diagnosis and treatment approaches,and equipment-medication combinations.We review the progress in the development of new treatments,such as neutron capture therapy,proton therapy,and heavy ion therapy.Furthermore,we examine the challenges and breakthroughs associated with the clinical translation of radiopharmaceuticals and provide recommendations for the research and development of novel radionuclide drugs.展开更多
The multiple nuclides identification algorithm with low consumption and strong robustness is crucial for rapid radioactive source searching.This study investigates the design of a low-consumption multiple nuclides ide...The multiple nuclides identification algorithm with low consumption and strong robustness is crucial for rapid radioactive source searching.This study investigates the design of a low-consumption multiple nuclides identification algorithm for portable gamma spectrometers.First,the gamma spectra of 12 target nuclides(including the background case)were measured to create training datasets.The characteristic energies,obtained through energy calibration and full-energy peak addresses,are utilized as input features for a neural network.A large number of single-and multiple-nuclide training datasets are generated using random combinations and small-range drifting.Subsequently,a multi-label classification neural network based on a binary cross-entropy loss function is applied to export the existence probability of certain nuclides.The designed algorithm effectively reduces the computation time and storage space required by the neural network and has been successfully implemented in a portable gamma spectrometer with a running time of t_(r)<2 s.Results show that,in both validation and actual tests,the identification accuracy of the designed algorithm reaches 94.8%,for gamma spectra with a dose rate of d≈0.5μSv∕h and a measurement time t_(m)=60 s.This improves the ability to perform rapid on-site nuclide identification at important sites.展开更多
^(10)Be surface exposure dating is one of the methods most used in the dating of glacial landforms due to its well-understood dating mechanism,readily accessible materials.However,numerous dating studies have shown th...^(10)Be surface exposure dating is one of the methods most used in the dating of glacial landforms due to its well-understood dating mechanism,readily accessible materials.However,numerous dating studies have shown that nuclide inheritance may overestimate the age as a result of the nuclide concentrations accumulating in glacial deposits prior to their eventual exposure.As the concentration is challenging to measure directly,it is typically assumed to be zero.This study investigated the potential nuclide inheritance in the Hailuogou Glacier by measuring^(10)Be concentrations in modern moraines.The results showed that(1)in the glacier foreland,the exposure ages of two sub-angular boulders aligned with the timing of glacier retreat suggested minimal or potentially negligible nuclide inheritance,whereas two amalgamated samples exhibited^(10)Be exposure ages of 820±278 yr and 570±168 yr,indicating that multiple cobbles may contain inherited nuclides;and(2)the exposure ages of the angular boulder samples from the modern glacier surface ranged from 366±151 yr to 221±85 yr,the coarse-grained(CG)sand samples ranged from 470±129 yr to 178±103 yr in age,and the ages of the amalgamated samples ranged from 1,114±197 yr to 97±37 yr,which may reflecting the upper limits of inherited ages.展开更多
The utilization of a proton beam from the China Spallation Neutron Source(CSNS)for producing medical radioisotopes is appealing owing to its high current intensity and high energy.The medical isotope production based ...The utilization of a proton beam from the China Spallation Neutron Source(CSNS)for producing medical radioisotopes is appealing owing to its high current intensity and high energy.The medical isotope production based on the proton beam at the CSNS is significant for the development of future radiopharmaceuticals,particularly for theα-emitting radiopharmaceu-ticals.The production yield and activity of typical medical isotopes were estimated using the FLUKA simulation.The results indicate that the 300-MeV proton beam with a power of 100 kW at CSNS-II is highly suitable for proof-of-principle studies of most medical radioisotopes.In particular,this proton beam offers tremendous advantages for the large-scale production of alpha radioisotopes,such as 225Ac,whose theoretical production yield can reach approximately 57 Ci/week.Based on these results,we provide perspectives on the use of CSNS proton beams to produce radioisotopes for medical applications.展开更多
Topographic shielding(TS) is an important factor in cosmogenic nuclide surface exposure dating. The development of geographic information systems(GIS) and the availability of digital elevation models(DEMs) make it pos...Topographic shielding(TS) is an important factor in cosmogenic nuclide surface exposure dating. The development of geographic information systems(GIS) and the availability of digital elevation models(DEMs) make it possible to derive this factor directly from a DEM. Most available GIS models derive the TS factors for an area(all cells in a DEM) without the consideration of surface conditions of individual sites, such as the strike, dip,and height above ground, into the calculation. This paper presents a new GIS model to derive the TS factors for discrete sample sites. This model uses the Skyline and Skyline Graph functions in ArcGIS to extract the set of azimuth and elevation angles of topographic obstructions around each site from a DEM(considering the sample height above ground)and then incorporates the strike and dip information of the sample surface to derive the TS factor. All processing tools and steps are streamlined in ArcGIS modelbuilder and this model can be run like a standard ArcGIS geoprocessing tool. It provides an easy and user-friendly means to derive the TS factors for discrete samples based on a DEM and the measured strike, dip and sample height for each site.展开更多
Topographic shielding of cosmic radiation flux is a key parameter in using cosmogenic nuclides to determine surface exposure ages or erosion rates. Traditionally, this parameter is measured in the field and uncertaint...Topographic shielding of cosmic radiation flux is a key parameter in using cosmogenic nuclides to determine surface exposure ages or erosion rates. Traditionally, this parameter is measured in the field and uncertainty and/or inconsistency may exist among different investigators. This paper provides an ArcGIS python code to determine topographic shielding factors using digital elevation models （DEMs）. This code can be imported into ArcGIS as a geoprocessing tool with a user-friendly graphical interface. The DEM-derived parameters using this method were validated with field measurements in central Tian Shan. Results indicate that DEM-derived shielding factors are consistent with field-measured values. It provides a valuable tool to save fieldwork efforts and has the potential to provide consistent results for different regions in the world to facilitate the comparison of cosmogenie nuclide results.展开更多
The Luonan Basin is a key region of early human settlement in Central China with more than 300 discovered Paleolithic sites. Artifact layer 1 of the Liuwan site was dated to approximately 0.6 million years (Ma) based ...The Luonan Basin is a key region of early human settlement in Central China with more than 300 discovered Paleolithic sites. Artifact layer 1 of the Liuwan site was dated to approximately 0.6 million years (Ma) based on correlation with the well-dated loess-paleosol sequence of the central Chinese Loess Plateau. This study reassessed the age of the Liuwan artifact layer via an absolute dating method, namely, <sup>26</sup>Al/<sup>10</sup>Be burial dating. We determined the burial age of artifact layer 1, which was most likely at least 0.60 ± 0.12 Ma (1ơ), using three simple burial ages. The new burial age confirmed the previous estimated age and provided a considerably accurate age range. Therefore, we suggest the use of the <sup>26</sup>Al/<sup>10</sup>Be burial dating method in thin loess-covered Paleolithic sites around the Qinling Mountain Range is helpful to understand the early human behavior.展开更多
Offset geomorphic features and deformed late Quaternary strata indicate active deformation along the Langshan-Seertengshan piedmont fault （LSPF）, one of the most active faults in the Hetao fault zone in Inner Mongol...Offset geomorphic features and deformed late Quaternary strata indicate active deformation along the Langshan-Seertengshan piedmont fault （LSPF）, one of the most active faults in the Hetao fault zone in Inner Mongolia, North China. The widespread occurrence of bedrock fault scarps along the LSPF offers excellent opportunity to examine the faulting history. Using cosmogenic ^10Be exposure dating, we measured the exposure ages of the western Langshankou scarp, located in the middle segment of the LSPF. Our data revealed at least two earthquakes that occurred at 22.2±3.3 Ira and 7.2±2.4 ka, respectively. These events are consistent with previous paleoseismic trench studies. The regression of the relationship between the age and sampling height along the scarp yield a fault slip rate of 0.10 ±0.05/-0.06 mm/yr, which is significantly lower than the average post-late Pleistocene fault slip rate of ~1 mm/yr, as estimated from the offset of the T2 terraces by previous studies. This indicates that the slip of the LSPF may have been accommodated by other fault branches.展开更多
The rapid identification of radioactive substances in public areas is crucial.However,traditional nuclide identification methods only consider information regarding the full energy peaks of the gamma-ray spectrum and ...The rapid identification of radioactive substances in public areas is crucial.However,traditional nuclide identification methods only consider information regarding the full energy peaks of the gamma-ray spectrum and require long recording times,which lead to long response times.In this paper,a novel identification method using the event mode sequence(EMS)information of target radionuclides is proposed.The EMS of a target radionuclide and natural background radiation were established as two different probabilistic models and a decision function based on Bayesian inference and sequential testing was constructed.The proposed detection scheme individually processes each photon.When a photon is detected and accepted,the corresponding posterior probability distribution parameters are estimated using Bayesian inference and the decision function is updated.Then,value of the decision function is compared to preset detection thresholds to obtain a detection result.Experiments on different target radionuclides(137Cs and 60Co)were performed.The count rates of the regions of interest(ROI)in the backgrounds between[651,671],[1154,1186],and[1310,1350]keV were 2.35,5.14,and 0.57 CPS,respectively.The experimental results demonstrate that the average detection time was 6.0 s for 60Co(with an activity of 80400 Bq)at a distance of 60 cm from the detector.The average detection time was 7 s for 137Cs(with an activity of 131000 Bq)at a distance of 90 cm from the detector.The results demonstrate that the proposed method can detect radioactive substances with low activity.展开更多
The last deglaciation, a key period for understanding present and future climate changes, has long been the hot topic for palaeoclimatological study. The Qinghai-Tibetan Plateau（QTP） is often a target study area for...The last deglaciation, a key period for understanding present and future climate changes, has long been the hot topic for palaeoclimatological study. The Qinghai-Tibetan Plateau（QTP） is often a target study area for understanding hemispheric, or even global environment changes. The glacial landforms on the QTP provide a unique perspective for its climate change. In order to investigate the onset of the last deglaciation at the QTP and its regional correlation, the terrestrial cosmogenic nuclides（TCN） 10 Be and 26 Al surface exposure dating was chosen to date the roche moutonnée, the polished surface and the moraine debris located at the palaeo-Daocheng Ice Cap（pDIC）, southeastern QTP. Our results show that the onset of the last deglaciation is at about 19 ka, followed by another warming event occurring around 15 ka in the p-DIC area. These timings agree well with other records, e.g. equivalent with a rapid sea level rise at 19 ka and the onset of B？lling warming event at about 15 ka. Thus, our new data can provide good reveal constraint on the climate evolution at the QTP.展开更多
The glacial landforms of the Qinghai-Tibetan Plateau （QTP） provide a unique opportunity to research hemispheric and global environmental changes. In this study, we focus on the glacial history of the palaeo-Daocheng...The glacial landforms of the Qinghai-Tibetan Plateau （QTP） provide a unique opportunity to research hemispheric and global environmental changes. In this study, we focus on the glacial history of the palaeo-Daocheng Ice Cap （p-DIC） in the southeastern QTP during the last glacial cycle. Based on field investigations, morphostratigraphy, and surface exposure dating of roche moutonnée, polished surface and moraine debris through the terrestrial cosmogenic nuclides （TCN） ^10Be and ^26Al. We identify glacial deposits of the last deglaciation, with minimum ages of 14.9±1.3-18.7±1.7 ka, the Last Glacial Maximum （LGM） of 24.7±2.2 ka, and the early part of the last glacial period （marine oxygen isotope stage （MIS） 3） of 37.1±3.4-45.2±3.9 ka. Our results show that in this region, the extent of the glacial advance during MIS 3 was larger than that during the traditional LGM （MIS 2）. These ages are consistent with prior chronologies, and the ^10Be age is consistent with the ^26Al age for the same sample. Thus, these data provide reliable constraints on climate change in the QTP, during the last glaciation.展开更多
The novel pulsed liquid chromatography radionuclide separation method presented here provides a new and promising strategy for the extraction of uranium from seawater.In this study,a new chromatographic separation met...The novel pulsed liquid chromatography radionuclide separation method presented here provides a new and promising strategy for the extraction of uranium from seawater.In this study,a new chromatographic separation method was proposed,and a pulsed nuclide automated separation device was developed,alongside a new chromatographic column.The length of this chromatographic column was 10 m,with an internal warp of 3 mm and a packing size of 1 mm,while the total separation units of the column reached 12,250.The most favorable conditions for the separation of nuclides were then obtained through optimizing the separation conditions of the device:Sample pH in the column=2,sample injection flow rate=5.698 mL/min,chromatographic column heating temperature=60℃.Separation experiments were also carried out for uranium,europium,and sodium ions in mixed solutions;uranium and sodium ions in water samples from the Ganjiang River;and uranium,sodium,and magnesium ions from seawater samples.The separation factors between the different nuclei were then calculated based on the experimental data,and a formula for the separation level was derived.The experimental results showed that the separation factor in the mixed solution of uranium and europium(1:1)was 1.088,while achieving the initial separation of uranium and europium theoretically required a 47-stage separation.Considering the separation factor of 1.50for the uranium and sodium ions in water samples from the Ganjiang River,achieving the initial separation of uranium and sodium ions would have theoretically required at least a 21-stage separation.Furthermore,for the seawater sample separation experiments,the separation factor of uranium and sodium ions was 1.2885;therefore,more than 28 stages of sample separation would be required to achieve uranium extraction from seawater.The novel pulsed liquid chromatography method proposed in this study was innovative in terms of uranium separation and enrichment,while expanding the possibilities of extracting uranium from seawater through chromatography.展开更多
In situ terrestrial cosmogenic nuclide （TCN） exposure dating using 10Be is one of the most successful techniques used to determine the ages of Quaternary deposits and yields data that enable the reconstruction of th...In situ terrestrial cosmogenic nuclide （TCN） exposure dating using 10Be is one of the most successful techniques used to determine the ages of Quaternary deposits and yields data that enable the reconstruction of the Quaternary glacial history of the Tibetan Plateau and the surrounding mountain ranges. Statistical analysis of TCN 10Be exposure ages, helps to reconstruct the history of glacial fluctuations and past climate changes on the Tibetan Plateau, differences in the timing of glacier advances among different regions. However, different versions of the Cosmic-Ray-prOduced NUclide Systematics on Earth （CRONUS-Earth） online calculator, which calculates and corrects the TCN ages of Quaternary glacial landforms, yield different results. For convenience in establishing contrasts among regions, in this paper, we recalculate 1848 10Be exposure ages from the Tibetan Plateau that were published from 1999 to 2017 using version 2.3 of the CRONUS-Earth calculator. We also compare the results obtained for 1594 10Be exposure ages using different versions （2.2, 2.3 and 3.0） of the CRONUS- Earth calculator. The results are as follows. （1） Approximately 97% of the exposure ages are less than 200 ka. A probability density curve of the exposure ages suggests that greater numbers of oscillations emerge during the Holocene, and the peaks correspond to the Little Ice Age, the 8.2 ka and 9.3 ka cold events; the main peak covers the period between 12 and 18 ka. （2） In most areas, the newer versions of the calculator produce older 10Be exposure ages. When different versions of the CRONUS-Earth calculator are used, approximately 29% of the 10Be exposure ages display maximum differences greater than 10 ka, and the maximum age difference for a single sample is 181.1 ka.展开更多
Information on the decay process of nuclides in the superheavy region is critical in investigating new elements beyond oganesson and the island of stability.This paper presents the application of a random forest algor...Information on the decay process of nuclides in the superheavy region is critical in investigating new elements beyond oganesson and the island of stability.This paper presents the application of a random forest algorithm to examine the competition among different decay modes in the superheavy region,includingα decay,β^(-)decay,β^(+)decay,electron capture and spontaneous fission.The observed half-lives and dominant decay mode are well reproduced.The dominant decay mode of 96.9%of the nuclei beyond ^(212) Po is correctly obtained.Further,α decay is predicted to be the dominant decay mode for isotopes in new elements Z=119-122,except for spontaneous fission in certain even–even elements owing to the increased Coulomb repulsion and odd–even effect.The predicted half-lives demonstrate the existence of a long-lived spontaneous fission island southwest of ^(298) Fl caused by the competition between the fission barrier and Coulomb repulsion.A better understanding of spontaneous fission,particularly beyond ^(286)Fl,is crucial in the search for new elements and the island of stability.展开更多
In order to consider the influence of temperature and underground water movement, an elastoplastic model and a 2D FEM stress fields on the migration of radioactive nuclide with code for analysis of coupled thermo-hyd...In order to consider the influence of temperature and underground water movement, an elastoplastic model and a 2D FEM stress fields on the migration of radioactive nuclide with code for analysis of coupled thermo-hydro-mechanical （THM） processes in saturated and unsaturated porous media were extended and improved through introducing the percolation and migration equation, so that the code can be used for solving the temperature field, flow field, stress field and nuclide concentration field simultaneously. The states of temperatures, pore pressures and nuclide concentrations in the near field of a hypothetical nuclear waste repository were investigated. The influence of the half life of the radioactive nuclide on the temporal change of nuclide concentration was analyzed considering the thermo-hydro-mechanical-migratory coupling. The results show that, at the boundary of the vitrified waste, the concentration of radioactive nuclide with a half life of 10 a falls after a period of rising, with the maximum value of 0.182 mol/m3 and the minimum value of 0.181 mol/m^3 at the end of computation. For a half life of 1 000 a, the concentration of radioactive nuclide always increases with the increase of the time during the computation period; and the maximum value is 1.686 mol/m^3 at the end of the computation. Therefore, under the condition of THM coupling, the concentration of radioactive nuclide with a shorter half life will decrease more quickly with water flow; but for the radioactive nuclide with a longer half life, its concentration will keep at a higher level for a longer time in the migration process.展开更多
Cosmogenic Ne isotopes are stable and are routinely used for constraining the timing of events and the rate of surface change beyond the limit that can be studied with radionuclides ^10Be, ^26Al, and ^36Cl. Cosmogenic...Cosmogenic Ne isotopes are stable and are routinely used for constraining the timing of events and the rate of surface change beyond the limit that can be studied with radionuclides ^10Be, ^26Al, and ^36Cl. Cosmogenic Ne analysis can be used in quartz and in a range of other minerals. Analysis typically requires significantly less material than do cosmogenic ^10Be and ^26Al, opening up the technique for small samples--individual pebbles in fiver sediments, for example. Analysis is easier and faster than for radionuclides, not least because Ne measurements do not require significant chemical procedures. However, the presence of other sources of Ne in minerals tends to restrict the use of cosmogenic ^21Ne to old landscapes and long exposure durations. In this review we briefly outline the background of cosmogenic Ne production in rocks and minerals at the Earth＇s surface, then document the key uses of the technique by highlighting some earlier studies, and finish with a short perspective on the future of the technique.展开更多
Daluo Mountains lie at front of the arcuate tectonic belt at the northeastern margin of the Tibetan Plateau,and are the landform boundary zone between the active Tibetan Plateau and the stable North China Craton.Study...Daluo Mountains lie at front of the arcuate tectonic belt at the northeastern margin of the Tibetan Plateau,and are the landform boundary zone between the active Tibetan Plateau and the stable North China Craton.Studying of the late Cenozoic uplift evolution of Daluo Mountains is important for understanding the expansion mechanism of the northeastern margin of the Tibetan Plateau and its influence on the western North China Craton.In this study,the late Cenozoic uplift of Daluo Mountains is constructed from the development of the late Cenozoic alluvial fan around Daluo Mountains.The entire sedimentary sequence and framework of the fan was revealed by the newly obtained drilling core data.The cosmogenic nuclide,optically stimulated luminescence,and detrital zircon U-Pb dating results provide new evidences for discussion about the initial timing of the late Cenozoic uplift of Daluo Mountains and the key stages of uplift during the Pleistocene.The late Cenozoic alluvial fan at front of Daluo Mountains overlies a set of fluvial-facies strata;therefore,development of the alluvial-fan marks the start of late Cenozoic uplift of Daluo Mountains.The timing of this event can be constrained to~4.64 Ma.Two extensive gravel layers(dated to ca.0.76–0.6 Ma and~0.05 Ma)developed during the Pleistocene,indicating two episodes of considerable uplift.This study provides a new time scale for the uplift and expansion of the arcuate tectonic belt at the northeastern margin of the Tibetan Plateau.展开更多
基金financially supported by Council of Scientific and Industrial Research(CSIR)(grant no.09/045(1399)/2015-EMR-I)the Ministry of Earth Sciences(Mo ES),Government of India(grant no.Mo ES/P.O.(Geo)/95/2017)。
文摘Soil erosion is one of the major global hazards threatening the food security of the world population.Soil erosion can be a result of both natural and anthropogenic processes.Field monitoring and models(numerical and physical)are commonly used to quantify soil erosion.However,field methods are time-consuming and the models inherently work with a level of uncertainty.Soil erosion studies in the Himalayas have been mostly carried out using modelling but there is a lack of sufficient field data to validate the results.We quantified soil erosion in a small catchment(Pranmati)in the Himalayas using the fallout meteoric^(10)Be nuclide for the first time.Based on the^(10)Be flux delivery rates determined from global circulation models(GCM),we calculated the rates of soil erosion at discrete points in the hilltop and mid-slope regions of hillslopes.The erosion rates vary between 17 mm kyr^(-1)to 68 mm kyr^(-1).These rates were determined in pristine areas that are unaffected by anthropogenic activities,thus,indicate the background erosion rates in the region.We established empirical relationships with estimated erosion rates and topographic parameters to assess the sediment dynamics in the hillslopes.It was observed that the sediment redistribution process operates differently in the mid-slope region compared to the hilltop region,due to increasing complexity of the active processes in the mid-slope region.
基金supported by the National Natural Science Foundation of China(No.42127807)Natural Science Foundation of Sichuan Province(Nos.2024NSFSC0422,23NSFSCC0116)Nuclear Energy Development Project(No.[2021]-88).
文摘In current neural network algorithms for nuclide identification in high-background,poor-resolution detectors,traditional network paradigms including back-propagation networks,convolutional neural networks,recurrent neural networks,etc.,have been limited in research on γ spectrum analysis because of their inherent mathematical mechanisms.It is difficult to make progress in terms of training data requirements and prediction accuracy.In contrast to traditional network paradigms,network models based on the transformer structure have the characteristics of parallel computing,position encoding,and deep stacking,which have enabled good performance in natural language processing tasks in recent years.Therefore,in this paper,a transformer-based neural network (TBNN) model is proposed to achieve nuclide identification for the first time.First,the Geant4 program was used to generate the basic single-nuclide energy spectrum through Monte Carlo simulations.A multi-nuclide energy spectrum database was established for neural network training using random matrices of γ-ray energy,activity,and noise.Based on the encoder–decoder structure,a network topology based on the transformer was built,transforming the 1024-channel energy spectrum data into a 32×32 energy spectrum sequence as the model input.Through experiments and adjustments of model parameters,including the learning rate of the TBNN model,number of attention heads,and number of network stacking layers,the overall recognition rate reached 98.7%.Additionally,this database was used for training AI models such as back-propagation networks,convolutional neural networks,residual networks,and long shortterm memory neural networks,with overall recognition rates of 92.8%,95.3%,96.3%,and 96.6%,respectively.This indicates that the TBNN model exhibited better nuclide identification among these AI models,providing an important reference and theoretical basis for the practical application of transformers in the qualitative and quantitative analysis of the γ spectrum.
基金the National Key R&D Program of China(No.2023YFE0197700)the Fundamental Research Funds for the Central Universities(No.2632023TD04).
文摘Radiopharmaceuticals operate by combining radionuclides with carriers.The radiation energy emitted by radionuclides is utilized to selectively irradiate diseased tissues while minimizing damage to healthy tissues.In comparison to external beam radiation therapy,radionuclide drugs demonstrate research potential due to their biological targeting capabilities and reduced normal tissue toxicity.This article reviews the applications and research progress of radiopharmaceuticals in cancer treatment.Several key radionuclides are examined,including^(223)Ra,^(90)Y,Lutetium-177(^(177)Lu),212 Pb,and Actinium-225(^(225)Ac).It also explores the current development trends of radiopharmaceuticals,encompassing the introduction of novel radionuclides,advancements in imaging technologies,integrated diagnosis and treatment approaches,and equipment-medication combinations.We review the progress in the development of new treatments,such as neutron capture therapy,proton therapy,and heavy ion therapy.Furthermore,we examine the challenges and breakthroughs associated with the clinical translation of radiopharmaceuticals and provide recommendations for the research and development of novel radionuclide drugs.
文摘The multiple nuclides identification algorithm with low consumption and strong robustness is crucial for rapid radioactive source searching.This study investigates the design of a low-consumption multiple nuclides identification algorithm for portable gamma spectrometers.First,the gamma spectra of 12 target nuclides(including the background case)were measured to create training datasets.The characteristic energies,obtained through energy calibration and full-energy peak addresses,are utilized as input features for a neural network.A large number of single-and multiple-nuclide training datasets are generated using random combinations and small-range drifting.Subsequently,a multi-label classification neural network based on a binary cross-entropy loss function is applied to export the existence probability of certain nuclides.The designed algorithm effectively reduces the computation time and storage space required by the neural network and has been successfully implemented in a portable gamma spectrometer with a running time of t_(r)<2 s.Results show that,in both validation and actual tests,the identification accuracy of the designed algorithm reaches 94.8%,for gamma spectra with a dose rate of d≈0.5μSv∕h and a measurement time t_(m)=60 s.This improves the ability to perform rapid on-site nuclide identification at important sites.
基金supported by the National Natural Science Foundation of China(Grant Nos.41971009,41503054).
文摘^(10)Be surface exposure dating is one of the methods most used in the dating of glacial landforms due to its well-understood dating mechanism,readily accessible materials.However,numerous dating studies have shown that nuclide inheritance may overestimate the age as a result of the nuclide concentrations accumulating in glacial deposits prior to their eventual exposure.As the concentration is challenging to measure directly,it is typically assumed to be zero.This study investigated the potential nuclide inheritance in the Hailuogou Glacier by measuring^(10)Be concentrations in modern moraines.The results showed that(1)in the glacier foreland,the exposure ages of two sub-angular boulders aligned with the timing of glacier retreat suggested minimal or potentially negligible nuclide inheritance,whereas two amalgamated samples exhibited^(10)Be exposure ages of 820±278 yr and 570±168 yr,indicating that multiple cobbles may contain inherited nuclides;and(2)the exposure ages of the angular boulder samples from the modern glacier surface ranged from 366±151 yr to 221±85 yr,the coarse-grained(CG)sand samples ranged from 470±129 yr to 178±103 yr in age,and the ages of the amalgamated samples ranged from 1,114±197 yr to 97±37 yr,which may reflecting the upper limits of inherited ages.
基金the National Natural Science Foundation of China(No.12075135)the China Postdoctoral Science Foundation(No.2022M721908).
文摘The utilization of a proton beam from the China Spallation Neutron Source(CSNS)for producing medical radioisotopes is appealing owing to its high current intensity and high energy.The medical isotope production based on the proton beam at the CSNS is significant for the development of future radiopharmaceuticals,particularly for theα-emitting radiopharmaceu-ticals.The production yield and activity of typical medical isotopes were estimated using the FLUKA simulation.The results indicate that the 300-MeV proton beam with a power of 100 kW at CSNS-II is highly suitable for proof-of-principle studies of most medical radioisotopes.In particular,this proton beam offers tremendous advantages for the large-scale production of alpha radioisotopes,such as 225Ac,whose theoretical production yield can reach approximately 57 Ci/week.Based on these results,we provide perspectives on the use of CSNS proton beams to produce radioisotopes for medical applications.
基金support by the National Science Foundation of the United States(Grant No.BCS-1227018)the National Nature Science Foundation of China(Grant No.41328001)
文摘Topographic shielding(TS) is an important factor in cosmogenic nuclide surface exposure dating. The development of geographic information systems(GIS) and the availability of digital elevation models(DEMs) make it possible to derive this factor directly from a DEM. Most available GIS models derive the TS factors for an area(all cells in a DEM) without the consideration of surface conditions of individual sites, such as the strike, dip,and height above ground, into the calculation. This paper presents a new GIS model to derive the TS factors for discrete sample sites. This model uses the Skyline and Skyline Graph functions in ArcGIS to extract the set of azimuth and elevation angles of topographic obstructions around each site from a DEM(considering the sample height above ground)and then incorporates the strike and dip information of the sample surface to derive the TS factor. All processing tools and steps are streamlined in ArcGIS modelbuilder and this model can be run like a standard ArcGIS geoprocessing tool. It provides an easy and user-friendly means to derive the TS factors for discrete samples based on a DEM and the measured strike, dip and sample height for each site.
基金supported by the Professional Development Award of the University of Tennessee
文摘Topographic shielding of cosmic radiation flux is a key parameter in using cosmogenic nuclides to determine surface exposure ages or erosion rates. Traditionally, this parameter is measured in the field and uncertainty and/or inconsistency may exist among different investigators. This paper provides an ArcGIS python code to determine topographic shielding factors using digital elevation models （DEMs）. This code can be imported into ArcGIS as a geoprocessing tool with a user-friendly graphical interface. The DEM-derived parameters using this method were validated with field measurements in central Tian Shan. Results indicate that DEM-derived shielding factors are consistent with field-measured values. It provides a valuable tool to save fieldwork efforts and has the potential to provide consistent results for different regions in the world to facilitate the comparison of cosmogenie nuclide results.
基金National Natural Science Foundation of China,No.41572155,No.41690111The Global Change Program of the Ministry of Science and Technology of China,No.2016YFA0600503
文摘The Luonan Basin is a key region of early human settlement in Central China with more than 300 discovered Paleolithic sites. Artifact layer 1 of the Liuwan site was dated to approximately 0.6 million years (Ma) based on correlation with the well-dated loess-paleosol sequence of the central Chinese Loess Plateau. This study reassessed the age of the Liuwan artifact layer via an absolute dating method, namely, <sup>26</sup>Al/<sup>10</sup>Be burial dating. We determined the burial age of artifact layer 1, which was most likely at least 0.60 ± 0.12 Ma (1ơ), using three simple burial ages. The new burial age confirmed the previous estimated age and provided a considerably accurate age range. Therefore, we suggest the use of the <sup>26</sup>Al/<sup>10</sup>Be burial dating method in thin loess-covered Paleolithic sites around the Qinling Mountain Range is helpful to understand the early human behavior.
基金supported by the National Natural Science Foundation of China (Grant No.41171001)the 1:50000 Active Fault Mapping of Langshan Piedmont Fault (Grant No.201408023)the Basic Research Business Foundation of the China Earthquake Administration (Grant No.ZDJ2012-02)
文摘Offset geomorphic features and deformed late Quaternary strata indicate active deformation along the Langshan-Seertengshan piedmont fault （LSPF）, one of the most active faults in the Hetao fault zone in Inner Mongolia, North China. The widespread occurrence of bedrock fault scarps along the LSPF offers excellent opportunity to examine the faulting history. Using cosmogenic ^10Be exposure dating, we measured the exposure ages of the western Langshankou scarp, located in the middle segment of the LSPF. Our data revealed at least two earthquakes that occurred at 22.2±3.3 Ira and 7.2±2.4 ka, respectively. These events are consistent with previous paleoseismic trench studies. The regression of the relationship between the age and sampling height along the scarp yield a fault slip rate of 0.10 ±0.05/-0.06 mm/yr, which is significantly lower than the average post-late Pleistocene fault slip rate of ~1 mm/yr, as estimated from the offset of the T2 terraces by previous studies. This indicates that the slip of the LSPF may have been accommodated by other fault branches.
文摘The rapid identification of radioactive substances in public areas is crucial.However,traditional nuclide identification methods only consider information regarding the full energy peaks of the gamma-ray spectrum and require long recording times,which lead to long response times.In this paper,a novel identification method using the event mode sequence(EMS)information of target radionuclides is proposed.The EMS of a target radionuclide and natural background radiation were established as two different probabilistic models and a decision function based on Bayesian inference and sequential testing was constructed.The proposed detection scheme individually processes each photon.When a photon is detected and accepted,the corresponding posterior probability distribution parameters are estimated using Bayesian inference and the decision function is updated.Then,value of the decision function is compared to preset detection thresholds to obtain a detection result.Experiments on different target radionuclides(137Cs and 60Co)were performed.The count rates of the regions of interest(ROI)in the backgrounds between[651,671],[1154,1186],and[1310,1350]keV were 2.35,5.14,and 0.57 CPS,respectively.The experimental results demonstrate that the average detection time was 6.0 s for 60Co(with an activity of 80400 Bq)at a distance of 60 cm from the detector.The average detection time was 7 s for 137Cs(with an activity of 131000 Bq)at a distance of 90 cm from the detector.The results demonstrate that the proposed method can detect radioactive substances with low activity.
基金supported by the National Excellent Doctoral Dissertation cultivation project of Nanjing Normal University (Grant No. 2012BS0005)the National Natural Science Foundation of China (Grant No. 40572097)the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
文摘The last deglaciation, a key period for understanding present and future climate changes, has long been the hot topic for palaeoclimatological study. The Qinghai-Tibetan Plateau（QTP） is often a target study area for understanding hemispheric, or even global environment changes. The glacial landforms on the QTP provide a unique perspective for its climate change. In order to investigate the onset of the last deglaciation at the QTP and its regional correlation, the terrestrial cosmogenic nuclides（TCN） 10 Be and 26 Al surface exposure dating was chosen to date the roche moutonnée, the polished surface and the moraine debris located at the palaeo-Daocheng Ice Cap（pDIC）, southeastern QTP. Our results show that the onset of the last deglaciation is at about 19 ka, followed by another warming event occurring around 15 ka in the p-DIC area. These timings agree well with other records, e.g. equivalent with a rapid sea level rise at 19 ka and the onset of B？lling warming event at about 15 ka. Thus, our new data can provide good reveal constraint on the climate evolution at the QTP.
基金supported by the National Natural Science Foundation of China (Grant No.40572097)the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD) (Grant No.164320H116)by the Yulong Mountain tourism development and management committee special project
文摘The glacial landforms of the Qinghai-Tibetan Plateau （QTP） provide a unique opportunity to research hemispheric and global environmental changes. In this study, we focus on the glacial history of the palaeo-Daocheng Ice Cap （p-DIC） in the southeastern QTP during the last glacial cycle. Based on field investigations, morphostratigraphy, and surface exposure dating of roche moutonnée, polished surface and moraine debris through the terrestrial cosmogenic nuclides （TCN） ^10Be and ^26Al. We identify glacial deposits of the last deglaciation, with minimum ages of 14.9±1.3-18.7±1.7 ka, the Last Glacial Maximum （LGM） of 24.7±2.2 ka, and the early part of the last glacial period （marine oxygen isotope stage （MIS） 3） of 37.1±3.4-45.2±3.9 ka. Our results show that in this region, the extent of the glacial advance during MIS 3 was larger than that during the traditional LGM （MIS 2）. These ages are consistent with prior chronologies, and the ^10Be age is consistent with the ^26Al age for the same sample. Thus, these data provide reliable constraints on climate change in the QTP, during the last glaciation.
基金the Natural Science Foundation of Jiangxi Province,China(No.20202BABL203004)the Opening Project of the State Key Laboratory of Nuclear Resources and Environment(East China University of Technology)(No.2022NRE23)the Opening Project of Jiangxi Province Key Laboratory of Polymer Micro/Nano Manufacturing and Devices(No.PMND202101).
文摘The novel pulsed liquid chromatography radionuclide separation method presented here provides a new and promising strategy for the extraction of uranium from seawater.In this study,a new chromatographic separation method was proposed,and a pulsed nuclide automated separation device was developed,alongside a new chromatographic column.The length of this chromatographic column was 10 m,with an internal warp of 3 mm and a packing size of 1 mm,while the total separation units of the column reached 12,250.The most favorable conditions for the separation of nuclides were then obtained through optimizing the separation conditions of the device:Sample pH in the column=2,sample injection flow rate=5.698 mL/min,chromatographic column heating temperature=60℃.Separation experiments were also carried out for uranium,europium,and sodium ions in mixed solutions;uranium and sodium ions in water samples from the Ganjiang River;and uranium,sodium,and magnesium ions from seawater samples.The separation factors between the different nuclei were then calculated based on the experimental data,and a formula for the separation level was derived.The experimental results showed that the separation factor in the mixed solution of uranium and europium(1:1)was 1.088,while achieving the initial separation of uranium and europium theoretically required a 47-stage separation.Considering the separation factor of 1.50for the uranium and sodium ions in water samples from the Ganjiang River,achieving the initial separation of uranium and sodium ions would have theoretically required at least a 21-stage separation.Furthermore,for the seawater sample separation experiments,the separation factor of uranium and sodium ions was 1.2885;therefore,more than 28 stages of sample separation would be required to achieve uranium extraction from seawater.The novel pulsed liquid chromatography method proposed in this study was innovative in terms of uranium separation and enrichment,while expanding the possibilities of extracting uranium from seawater through chromatography.
基金supported by the National Natural Science Foundation of China(Grant No.41503054)the China Postdoctoral Science Foundation(2015M582728)+1 种基金the Priority Academic Program Development of Jiangsu Higher Education Institutions(PAPD)(Grant No.164320H116)the Yulong Mountain tourism development and management committee special project
文摘In situ terrestrial cosmogenic nuclide （TCN） exposure dating using 10Be is one of the most successful techniques used to determine the ages of Quaternary deposits and yields data that enable the reconstruction of the Quaternary glacial history of the Tibetan Plateau and the surrounding mountain ranges. Statistical analysis of TCN 10Be exposure ages, helps to reconstruct the history of glacial fluctuations and past climate changes on the Tibetan Plateau, differences in the timing of glacier advances among different regions. However, different versions of the Cosmic-Ray-prOduced NUclide Systematics on Earth （CRONUS-Earth） online calculator, which calculates and corrects the TCN ages of Quaternary glacial landforms, yield different results. For convenience in establishing contrasts among regions, in this paper, we recalculate 1848 10Be exposure ages from the Tibetan Plateau that were published from 1999 to 2017 using version 2.3 of the CRONUS-Earth calculator. We also compare the results obtained for 1594 10Be exposure ages using different versions （2.2, 2.3 and 3.0） of the CRONUS- Earth calculator. The results are as follows. （1） Approximately 97% of the exposure ages are less than 200 ka. A probability density curve of the exposure ages suggests that greater numbers of oscillations emerge during the Holocene, and the peaks correspond to the Little Ice Age, the 8.2 ka and 9.3 ka cold events; the main peak covers the period between 12 and 18 ka. （2） In most areas, the newer versions of the calculator produce older 10Be exposure ages. When different versions of the CRONUS-Earth calculator are used, approximately 29% of the 10Be exposure ages display maximum differences greater than 10 ka, and the maximum age difference for a single sample is 181.1 ka.
基金supported by the Guangdong Major Project of Basic and Applied Basic Research under Grant No. 2021B0301030006the computational resources from SYSU and the National Supercomputer Center in Guangzhou。
文摘Information on the decay process of nuclides in the superheavy region is critical in investigating new elements beyond oganesson and the island of stability.This paper presents the application of a random forest algorithm to examine the competition among different decay modes in the superheavy region,includingα decay,β^(-)decay,β^(+)decay,electron capture and spontaneous fission.The observed half-lives and dominant decay mode are well reproduced.The dominant decay mode of 96.9%of the nuclei beyond ^(212) Po is correctly obtained.Further,α decay is predicted to be the dominant decay mode for isotopes in new elements Z=119-122,except for spontaneous fission in certain even–even elements owing to the increased Coulomb repulsion and odd–even effect.The predicted half-lives demonstrate the existence of a long-lived spontaneous fission island southwest of ^(298) Fl caused by the competition between the fission barrier and Coulomb repulsion.A better understanding of spontaneous fission,particularly beyond ^(286)Fl,is crucial in the search for new elements and the island of stability.
基金Project(2010CB732101) supported by the National Basic Research Program of China Project(SKLQ 008) supported by the Research Fund of State Key Laboratory of Geomechanics and Geotechnical Engineering of China
文摘In order to consider the influence of temperature and underground water movement, an elastoplastic model and a 2D FEM stress fields on the migration of radioactive nuclide with code for analysis of coupled thermo-hydro-mechanical （THM） processes in saturated and unsaturated porous media were extended and improved through introducing the percolation and migration equation, so that the code can be used for solving the temperature field, flow field, stress field and nuclide concentration field simultaneously. The states of temperatures, pore pressures and nuclide concentrations in the near field of a hypothetical nuclear waste repository were investigated. The influence of the half life of the radioactive nuclide on the temporal change of nuclide concentration was analyzed considering the thermo-hydro-mechanical-migratory coupling. The results show that, at the boundary of the vitrified waste, the concentration of radioactive nuclide with a half life of 10 a falls after a period of rising, with the maximum value of 0.182 mol/m3 and the minimum value of 0.181 mol/m^3 at the end of computation. For a half life of 1 000 a, the concentration of radioactive nuclide always increases with the increase of the time during the computation period; and the maximum value is 1.686 mol/m^3 at the end of the computation. Therefore, under the condition of THM coupling, the concentration of radioactive nuclide with a shorter half life will decrease more quickly with water flow; but for the radioactive nuclide with a longer half life, its concentration will keep at a higher level for a longer time in the migration process.
基金supported by the basic scientific research fund, Institute of Geology, China Earthquake Administration (Grant Nos. IGCEA1504 and IGCEA1417)
文摘Cosmogenic Ne isotopes are stable and are routinely used for constraining the timing of events and the rate of surface change beyond the limit that can be studied with radionuclides ^10Be, ^26Al, and ^36Cl. Cosmogenic Ne analysis can be used in quartz and in a range of other minerals. Analysis typically requires significantly less material than do cosmogenic ^10Be and ^26Al, opening up the technique for small samples--individual pebbles in fiver sediments, for example. Analysis is easier and faster than for radionuclides, not least because Ne measurements do not require significant chemical procedures. However, the presence of other sources of Ne in minerals tends to restrict the use of cosmogenic ^21Ne to old landscapes and long exposure durations. In this review we briefly outline the background of cosmogenic Ne production in rocks and minerals at the Earth＇s surface, then document the key uses of the technique by highlighting some earlier studies, and finish with a short perspective on the future of the technique.
基金supported by the National Natural Science Foundation of China(41972119)the Foundation of Chinese Academy of Geological Sciences(DZLXJK202104)the Geological Investigation Project of the China Geological Survey(DD20160060,DD20190018).
文摘Daluo Mountains lie at front of the arcuate tectonic belt at the northeastern margin of the Tibetan Plateau,and are the landform boundary zone between the active Tibetan Plateau and the stable North China Craton.Studying of the late Cenozoic uplift evolution of Daluo Mountains is important for understanding the expansion mechanism of the northeastern margin of the Tibetan Plateau and its influence on the western North China Craton.In this study,the late Cenozoic uplift of Daluo Mountains is constructed from the development of the late Cenozoic alluvial fan around Daluo Mountains.The entire sedimentary sequence and framework of the fan was revealed by the newly obtained drilling core data.The cosmogenic nuclide,optically stimulated luminescence,and detrital zircon U-Pb dating results provide new evidences for discussion about the initial timing of the late Cenozoic uplift of Daluo Mountains and the key stages of uplift during the Pleistocene.The late Cenozoic alluvial fan at front of Daluo Mountains overlies a set of fluvial-facies strata;therefore,development of the alluvial-fan marks the start of late Cenozoic uplift of Daluo Mountains.The timing of this event can be constrained to~4.64 Ma.Two extensive gravel layers(dated to ca.0.76–0.6 Ma and~0.05 Ma)developed during the Pleistocene,indicating two episodes of considerable uplift.This study provides a new time scale for the uplift and expansion of the arcuate tectonic belt at the northeastern margin of the Tibetan Plateau.
