We systematically calculated the multinucleon transfer reactions of ^(208)Os,^(208)Pt,^(208)Hg,^(208)Pb,^(208)Po,^(208)Rn,^(208)Ra,and ^(132,136) Xe when bombarded on ^(232) Th and ^(248) Cm at Coulomb barrier energie...We systematically calculated the multinucleon transfer reactions of ^(208)Os,^(208)Pt,^(208)Hg,^(208)Pb,^(208)Po,^(208)Rn,^(208)Ra,and ^(132,136) Xe when bombarded on ^(232) Th and ^(248) Cm at Coulomb barrier energies within the dinuclear system model.These results are in good agreement with the available experimental data.The influence of Coulomb and shell effects on actinide production in these reactions has been rigorously studied.We calculated and analyzed the potential energy surface (PES) and total kinetic energy (TKE) mass distributions for the reactions involving ^(208)Hg,^(208)Pb,and ^(208) Po with ^(248) Cm and ^(232)Th.The PES and TKE spectra shed light on the fragment formation mechanisms in multinucleon transfer reactions,with clear indications of isospin and shell effects.The production cross sections for multinucleon transfer products show a strong dependence on isobar projectiles with a mass number A=208.Isobar projectiles with high N/Z ratios are advantageous for generating neutron-rich target-like fragments.Conversely,products induced by isobar projectiles with larger charge numbers tend to shift toward proton-rich regions.The intertwining of the Coulomb potential and shell effect is evident in the production cross sections of actinide isotopes.Drawing from reactions induced by radioactive projectiles,we anticipate the discovery of several new actinide isotopes near the nuclear drip lines,extending our reach into the superheavy nuclei domain.展开更多
The main progresses in the multinucleon transfer reactions at energies close to the Coulomb barrier are reviewed. After a short presentation of the experimental progress and theoretical progress, the predicted product...The main progresses in the multinucleon transfer reactions at energies close to the Coulomb barrier are reviewed. After a short presentation of the experimental progress and theoretical progress, the predicted production cross sections for unknown neutron-rich heavy nuclei and the trans-uranium nuclei are presented.展开更多
Within the framework of the dinuclear system model,the multinucleon transfer dynamics for nearly symmetric nuclear collisions has been investigated.The reaction mechanism in the systems of 198Pt+198Pt and 204Hg+198Pt ...Within the framework of the dinuclear system model,the multinucleon transfer dynamics for nearly symmetric nuclear collisions has been investigated.The reaction mechanism in the systems of 198Pt+198Pt and 204Hg+198Pt was investigated at beam energies around the Coulomb barrier.It was found that the isotopic yields are enhanced with increased incident energy in the domain of proton-rich nuclides.However,the production on the neutron-rich side weakly depends on the energy.The angular distribution with the beam energy was also analyzed in the multinucleon transfer reactions.Projectile-like fragments were produced toward the forward emission with increasing incident energy.The target-like fragments manifested the opposite trend in the transfer reactions.展开更多
The dinuclear system approach,coupled with the statistical decay model GEMINI++,was used to investigate multinucleon transfer reactions.Experimental production cross-sections in the reaction^(129)Xe+^(248)Cm were repr...The dinuclear system approach,coupled with the statistical decay model GEMINI++,was used to investigate multinucleon transfer reactions.Experimental production cross-sections in the reaction^(129)Xe+^(248)Cm were reproduced to assess the reliability of these theoretical models.The production of neutron-deficient transcalifornium nuclei with Z=99-106 was examined in multinucleon transfer reactions,including^(124)Xe+^(248)Cm,^(124)Xe+^(249)Cf,and^(129)Xe+^(249)Cf.Both the driving potential and the neutron-to-proton equilibration ratio were found to dominate the nucleon transfer process.The reaction^(124)Xe+^(249)Cf is proposed as a promising projectile-target combination for producing neutron-deficient isotopes with Z=99-106,with the optimal incident energy identified as E_(c.m.)=533.64 MeV.Production cross-sections of 25 unknown neutron-deficient trancalifornium isotopes with cross-sections greater than 1 pb were predicted.展开更多
A method based on the dinuclear system(DNS)is proposed to describe the angular distribution of products in multinucleon transfer(MNT)reactions.By considering fluctuation effects,the angular distributions of reactions ...A method based on the dinuclear system(DNS)is proposed to describe the angular distribution of products in multinucleon transfer(MNT)reactions.By considering fluctuation effects,the angular distributions of reactions involving^(136)Xe+^(208)Pb,^(136)Xe+^(209)Bi,^(86)Kr+^(166)Er,^(84)Kr+^(209)Bi,and^(84)Kr+^(208)Pb are examined,demonstrating good agreement with experimental data.Moreover,the double differential cross-sections(dσ^(2)/dl_(i)dΘand dσ^(2)/dZdΘ)of reactions^(136)Xe+^(208)Pb and^(136)Xe+^(209)Bi are analyzed to explore the mechanism of angular distribution in MNT reactions.Additionally,the optimal angles for detecting N=126 isotopes are determined via an analysis on the influence of proton and neutron numbers of the projectiles on the angular distribution of the N=126 isotopic line.The results of this study can provide valuable insights for experimental detection.展开更多
Multinucleon transfer reactions near the Coulomb barrier are investigated based on the improved dinuclear system(DNS)model,and the deexcitation process of primary fragments are described using the statistical model GE...Multinucleon transfer reactions near the Coulomb barrier are investigated based on the improved dinuclear system(DNS)model,and the deexcitation process of primary fragments are described using the statistical model GEMINI++.The production cross sections of^(40,48)Ca+^(124)Sn and^(64)Ni+^(130)Te based on the DNS model+GEMINI++are calculated and compared with experimental data.The calculated results reproduce experimental data.The cross sections of fusion-evaporation,fragmentation,and multinucleon transfer reactions in the region are also provided in this paper.The results show that in the region,fusion-evaporation and fragmentation reactions have good results in the relatively proton-rich region,but in the extreme proton-deficient region,the MNT reaction is still promising for synthesizing proton-rich nuclei.展开更多
Multinucleon transfer in low-energy heavy-ion collisions is increasingly considered a promising approach for generating exotic nuclei.Understanding the complex mechanisms involved in multinucleon transfer processes pr...Multinucleon transfer in low-energy heavy-ion collisions is increasingly considered a promising approach for generating exotic nuclei.Understanding the complex mechanisms involved in multinucleon transfer processes presents significant challenges for the theoretical investigation of nuclear reactions.A Langevin equation model was developed and employed to investigate multinucleon transfer processes.The^(40)Ar+^(232)Th reaction was simulated,and the calculated Wilczyński plot was used to verify the model.Additionally,to study the dynamics of multinucleon transfer reactions,the^(136)Xe+^(238)U and^(136)Xe+^(209)Bi reactions were simulated,and the corresponding TKE-mass and angular distributions were computed to analyze the energy dissipation and scattering angles.This investigation enhances our understanding of the dynamics involved in multinucleon transfer processes.展开更多
The improved quantum molecular dynamics model was employed to study the ^(238)U+^(238)U multinucleon transfer reaction at E_(c.m.)=833 Me V in this work.The influence of the orientation effect on the nuclear deformati...The improved quantum molecular dynamics model was employed to study the ^(238)U+^(238)U multinucleon transfer reaction at E_(c.m.)=833 Me V in this work.The influence of the orientation effect on the nuclear deformation at the contact moment,the composite system lifetime,the transfer rate and the fragment production mechanism are investigated.Statistical analysis reveals that at the contact moment,the orientation of the projectile and the target have less influence on each other and retain their respective initial characteristics to some extent.For collision parameters less than 6 fm,significant differences are observed in composite system lifetime and transfer rate under different orientation configurations;however,the orientation effect gradually diminishes with increasing collision parameters.Additionally,it is found that transfer reactions dominate when the collision parameter b≤6 fm,while elastic and inelastic scattering events increase rapidly as the collision parameter exceeds 6 fm.Within the range of 10≤b≤13 fm,the transfer probability for side–side collisions is significantly higher compared to other cases.展开更多
In this review article,we first briefty introduce the transport theory and quantum molecular dynamics model applied in the study of the heavy ion collisions from low to intermediate energies.The developments of improv...In this review article,we first briefty introduce the transport theory and quantum molecular dynamics model applied in the study of the heavy ion collisions from low to intermediate energies.The developments of improved quantum molecular dynamics model(ImQMD)and ultra-relativistic quantum molecular dynamics model(UrQMD),are reviewed.The reaction mechanism and phenomena related to the fusion,multinucleon transrer,fragmentation,collective flow and particle production are reviewed and discussed within the framework of the two models.The constraints on the isospin asymmetric muclear equation of state and in-medium nucleon nucleon cross sections by comparing the heavy ion collision data with transport models calculations in last decades are also discussed,and the uncertainties of these constraints are analyzed as well.Finally,we discuss the future direction of the development of the transport models for improving the understanding of the reaction mechanism,the descriptions of various observables,the constraint on the nuclear equation of state,as well as for the constraint on in-medium nucleon-nucleon cross sections.展开更多
197Au were irradiated with 47 MeV/u 12C ions. Iridium was produced via the multinucleon transfer reactions in bombardments of 197Au with 12C. and was separated radiochemically from Au and the mixture of the reaction p...197Au were irradiated with 47 MeV/u 12C ions. Iridium was produced via the multinucleon transfer reactions in bombardments of 197Au with 12C. and was separated radiochemically from Au and the mixture of the reaction products. The γ radioactivities of Ir isotopes were measured by using a HPGe detector. The production cross sections of Ir isotopes were determined from activities of Ir isotopes at the end of bombardment and the other relative data. It has been found that the cross sections for neutron-rich isotopes of iridium show an exponential dependence on the values of Qgg. Our experimental results also demonstrate lack of correlation between the cross sections and Qgg in the case of neutron-deficient isotopes of iridium. The fact can be explained from that neutron-rich isotopes of iridium were produced in the deep inelastic transfer reactions.展开更多
基金supported by National Natural Science Foundation of China (Nos. 12105241, 12175072)Natural Science Foundation of Jiangsu Province (No. BK20210788)+3 种基金Jiangsu Provincial Double-Innovation Doctoral Program (No. JSSCBS20211013)University Science Research Project of Jiangsu Province (No. 21KJB140026)Lv Yang Jin Feng (No. YZLYJFJH2021YXBS130)Key Laboratory of High-Precision Nuclear Spectroscopy,Institute of Modern Physics,Chinese Academy of Sciences (No. IMPKFKT2021001)。
文摘We systematically calculated the multinucleon transfer reactions of ^(208)Os,^(208)Pt,^(208)Hg,^(208)Pb,^(208)Po,^(208)Rn,^(208)Ra,and ^(132,136) Xe when bombarded on ^(232) Th and ^(248) Cm at Coulomb barrier energies within the dinuclear system model.These results are in good agreement with the available experimental data.The influence of Coulomb and shell effects on actinide production in these reactions has been rigorously studied.We calculated and analyzed the potential energy surface (PES) and total kinetic energy (TKE) mass distributions for the reactions involving ^(208)Hg,^(208)Pb,and ^(208) Po with ^(248) Cm and ^(232)Th.The PES and TKE spectra shed light on the fragment formation mechanisms in multinucleon transfer reactions,with clear indications of isospin and shell effects.The production cross sections for multinucleon transfer products show a strong dependence on isobar projectiles with a mass number A=208.Isobar projectiles with high N/Z ratios are advantageous for generating neutron-rich target-like fragments.Conversely,products induced by isobar projectiles with larger charge numbers tend to shift toward proton-rich regions.The intertwining of the Coulomb potential and shell effect is evident in the production cross sections of actinide isotopes.Drawing from reactions induced by radioactive projectiles,we anticipate the discovery of several new actinide isotopes near the nuclear drip lines,extending our reach into the superheavy nuclei domain.
文摘The main progresses in the multinucleon transfer reactions at energies close to the Coulomb barrier are reviewed. After a short presentation of the experimental progress and theoretical progress, the predicted production cross sections for unknown neutron-rich heavy nuclei and the trans-uranium nuclei are presented.
基金supported by the National Natural Science Foundation of China(Nos.11722546 and 11675226)the Talent Program of South China University of Technology。
文摘Within the framework of the dinuclear system model,the multinucleon transfer dynamics for nearly symmetric nuclear collisions has been investigated.The reaction mechanism in the systems of 198Pt+198Pt and 204Hg+198Pt was investigated at beam energies around the Coulomb barrier.It was found that the isotopic yields are enhanced with increased incident energy in the domain of proton-rich nuclides.However,the production on the neutron-rich side weakly depends on the energy.The angular distribution with the beam energy was also analyzed in the multinucleon transfer reactions.Projectile-like fragments were produced toward the forward emission with increasing incident energy.The target-like fragments manifested the opposite trend in the transfer reactions.
基金supported partly by the National Key R&D Program of China(No.2023YFA1606401)the National Natural Science Foundation of China(Nos.12135004,11635003,11961141004,12105019,and 12047513)+1 种基金the Open Project of Guangxi Key Laboratory of Nuclear Physics and Nuclear Technology(No.NLK2023-05)the Central Government Guidance Funds for Local Scientific and Technological Development,China(No.Guike ZY22096024)。
文摘The dinuclear system approach,coupled with the statistical decay model GEMINI++,was used to investigate multinucleon transfer reactions.Experimental production cross-sections in the reaction^(129)Xe+^(248)Cm were reproduced to assess the reliability of these theoretical models.The production of neutron-deficient transcalifornium nuclei with Z=99-106 was examined in multinucleon transfer reactions,including^(124)Xe+^(248)Cm,^(124)Xe+^(249)Cf,and^(129)Xe+^(249)Cf.Both the driving potential and the neutron-to-proton equilibration ratio were found to dominate the nucleon transfer process.The reaction^(124)Xe+^(249)Cf is proposed as a promising projectile-target combination for producing neutron-deficient isotopes with Z=99-106,with the optimal incident energy identified as E_(c.m.)=533.64 MeV.Production cross-sections of 25 unknown neutron-deficient trancalifornium isotopes with cross-sections greater than 1 pb were predicted.
基金Supported by the Guangdong Major Project of Basic and Applied Basic Research(2021B0301030006)the National Natural Science Foundation of China(12175151,12105181,11847235)the Steady Support Program for Higher Education Institutions of Shenzhen(20200817005440001)。
文摘A method based on the dinuclear system(DNS)is proposed to describe the angular distribution of products in multinucleon transfer(MNT)reactions.By considering fluctuation effects,the angular distributions of reactions involving^(136)Xe+^(208)Pb,^(136)Xe+^(209)Bi,^(86)Kr+^(166)Er,^(84)Kr+^(209)Bi,and^(84)Kr+^(208)Pb are examined,demonstrating good agreement with experimental data.Moreover,the double differential cross-sections(dσ^(2)/dl_(i)dΘand dσ^(2)/dZdΘ)of reactions^(136)Xe+^(208)Pb and^(136)Xe+^(209)Bi are analyzed to explore the mechanism of angular distribution in MNT reactions.Additionally,the optimal angles for detecting N=126 isotopes are determined via an analysis on the influence of proton and neutron numbers of the projectiles on the angular distribution of the N=126 isotopic line.The results of this study can provide valuable insights for experimental detection.
基金the ational Natural Science Foundation of China(12175064,U2167203)Hunan Provincial Education Department(Key project 20A290)。
文摘Multinucleon transfer reactions near the Coulomb barrier are investigated based on the improved dinuclear system(DNS)model,and the deexcitation process of primary fragments are described using the statistical model GEMINI++.The production cross sections of^(40,48)Ca+^(124)Sn and^(64)Ni+^(130)Te based on the DNS model+GEMINI++are calculated and compared with experimental data.The calculated results reproduce experimental data.The cross sections of fusion-evaporation,fragmentation,and multinucleon transfer reactions in the region are also provided in this paper.The results show that in the region,fusion-evaporation and fragmentation reactions have good results in the relatively proton-rich region,but in the extreme proton-deficient region,the MNT reaction is still promising for synthesizing proton-rich nuclei.
基金supported by the National Key R&D Program of China(No.2023YFA1606401)the National Natural Science Foundation of China(Nos.12135004,11635003 and 11961141004)。
文摘Multinucleon transfer in low-energy heavy-ion collisions is increasingly considered a promising approach for generating exotic nuclei.Understanding the complex mechanisms involved in multinucleon transfer processes presents significant challenges for the theoretical investigation of nuclear reactions.A Langevin equation model was developed and employed to investigate multinucleon transfer processes.The^(40)Ar+^(232)Th reaction was simulated,and the calculated Wilczyński plot was used to verify the model.Additionally,to study the dynamics of multinucleon transfer reactions,the^(136)Xe+^(238)U and^(136)Xe+^(209)Bi reactions were simulated,and the corresponding TKE-mass and angular distributions were computed to analyze the energy dissipation and scattering angles.This investigation enhances our understanding of the dynamics involved in multinucleon transfer processes.
基金supported by the Natural Science Foundation of Guangxi under Grant No.2024GXNSFBA010377,No.2022GXNSFBA035528,No.2023GXNSFBA026008Guangxi Science and Technology Base and Special Talent Program under Grant No.Guike AD22035060+2 种基金the Central Government Guides Local Scientific and Technological Development Fund Projects under Grant No.Guike ZY22096024the National Natural Science Foundation of China under Grant No.12135004,No.11635003 No.11961141004,No.12365016the Innovation Project of Guangxi Graduate Education Grant No.YCBZ2023060.
文摘The improved quantum molecular dynamics model was employed to study the ^(238)U+^(238)U multinucleon transfer reaction at E_(c.m.)=833 Me V in this work.The influence of the orientation effect on the nuclear deformation at the contact moment,the composite system lifetime,the transfer rate and the fragment production mechanism are investigated.Statistical analysis reveals that at the contact moment,the orientation of the projectile and the target have less influence on each other and retain their respective initial characteristics to some extent.For collision parameters less than 6 fm,significant differences are observed in composite system lifetime and transfer rate under different orientation configurations;however,the orientation effect gradually diminishes with increasing collision parameters.Additionally,it is found that transfer reactions dominate when the collision parameter b≤6 fm,while elastic and inelastic scattering events increase rapidly as the collision parameter exceeds 6 fm.Within the range of 10≤b≤13 fm,the transfer probability for side–side collisions is significantly higher compared to other cases.
基金Yingxun Zhang acknowledges the supports in part by the National Natural Science Foundation of China(Grant Nos.11875323,11875125,11475262,10675172,11075215,11475262,11790323,11790324,11790325,and 11961141003)the National Key R&D Program of China(Grant No.2018YFA0404404)+15 种基金the Continuous Basic Scientific Research Project(No.WDJC-2019-13)Ning Wang acknowledges the supports in part by the National Natural Science Foundation of China(Nos.U1867212 and 11422548)the Guangxi Natural Science Foundation(Nos.2015G XNSFDA139004,2017G XNSFG A198001)Qingfeng Li acknowledges the supports in part by the National Natural Science Foundation of China(Nos.11875125,11847315,11375062,11505057,11947410,and 11747312)the Zhejiang Provincial Natural Science Foundation of China(No.LY18A050002)the“Ten-Thousand Talent Program”of Zhejiang ProvinceJunlong Tian acknowledges the supports in part by the National Science Foundation of China(Nos.11961131010 and 11475004)Li Ou acknowledges the supports in part by the National Natural Science Foundation of China(No.11965004)the Natural Science Foundation of Guangxi Province(No.2016GXNSFFA380001)Foundation of Guangxi Innovative Team and Distinguished Scholar in Institutions of Higher EducationMin Liu acknowledges the supports in part by the National Natural Science Foundation of China(No.11875323)Kai Zhao acknowledges the supports in part by the National Natural Science Foundation of China(Nos.11675266,11005155,11475262,11275052,11375062,11547312,and 11275068)the National Key Basic Research Developm ent Program of China(Nos.2007CB209900 and 2013CB834404)Xizhen Wu acknowledges the supports in part by the National Natural Science Foundation of China(Nos.10235020,10979023,11005155,11365004,11475004,and 11675266)Zhuxia Li acknowledges the supports in part by the National Natural Science Foundation of China(Nos.19975073,10175093,10175089,10235030,11275052,11375062,11475262,11475004,11875323,and 11875125)the National Key Basic Research Development Program of China(Nos.G20000774 and 2007CB209900).
文摘In this review article,we first briefty introduce the transport theory and quantum molecular dynamics model applied in the study of the heavy ion collisions from low to intermediate energies.The developments of improved quantum molecular dynamics model(ImQMD)and ultra-relativistic quantum molecular dynamics model(UrQMD),are reviewed.The reaction mechanism and phenomena related to the fusion,multinucleon transrer,fragmentation,collective flow and particle production are reviewed and discussed within the framework of the two models.The constraints on the isospin asymmetric muclear equation of state and in-medium nucleon nucleon cross sections by comparing the heavy ion collision data with transport models calculations in last decades are also discussed,and the uncertainties of these constraints are analyzed as well.Finally,we discuss the future direction of the development of the transport models for improving the understanding of the reaction mechanism,the descriptions of various observables,the constraint on the nuclear equation of state,as well as for the constraint on in-medium nucleon-nucleon cross sections.
基金Supported by National Natural Science Foundation of China (10575118)
文摘197Au were irradiated with 47 MeV/u 12C ions. Iridium was produced via the multinucleon transfer reactions in bombardments of 197Au with 12C. and was separated radiochemically from Au and the mixture of the reaction products. The γ radioactivities of Ir isotopes were measured by using a HPGe detector. The production cross sections of Ir isotopes were determined from activities of Ir isotopes at the end of bombardment and the other relative data. It has been found that the cross sections for neutron-rich isotopes of iridium show an exponential dependence on the values of Qgg. Our experimental results also demonstrate lack of correlation between the cross sections and Qgg in the case of neutron-deficient isotopes of iridium. The fact can be explained from that neutron-rich isotopes of iridium were produced in the deep inelastic transfer reactions.
