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NUMERICAL ANALYSIS OF TWO-DIMENSIONAL MULTI-OBJECT SCATTERING SYSTEMS WITH ARBITRARY STRUCTURE
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作者 樊德森 《Journal of Electronics(China)》 1992年第3期253-260,共8页
A general analysis approach to multi-object(M-object)scattering systems of ar-bitrary structure is presented.Through the system scattering equation(SSE),the M-objectproblems are first transformed into a series of sing... A general analysis approach to multi-object(M-object)scattering systems of ar-bitrary structure is presented.Through the system scattering equation(SSE),the M-objectproblems are first transformed into a series of single-object(S-object)problems and then arethey solved,one-object by one-object,to determine the unknown coefficients of SSE.Finally theSSE is solved to yield the global solutions of original M-object problems.As to the solution ofS-object problems concerned,we use the global numerical boundary condition(GNBC)basedfinite element method(FEM)for complex scatterers,or the moment method(MM)for conduct-ing scatterers.For clarity we will confine ourself in two-dimensional(2-D)cases,and show somecalculation examples of M-object scattering systems for demonstration. 展开更多
关键词 Electromagnetic scattering multi-object scattering system FINITE element METHOD MOMENT METHOD
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Tip-enhanced Raman scattering of glucose molecules 被引量:3
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作者 Zhonglin Xie Chao Meng +3 位作者 Donghua Yue Lei Xu Ting Mei Wending Zhang 《Opto-Electronic Science》 2025年第5期2-9,共8页
Glucose molecules are of great significance being one of the most important molecules in metabolic chain.However,due to the small Raman scattering cross-section and weak/non-adsorption on bare metals,accurately obtain... Glucose molecules are of great significance being one of the most important molecules in metabolic chain.However,due to the small Raman scattering cross-section and weak/non-adsorption on bare metals,accurately obtaining their"fingerprint information"remains a huge obstacle.Herein,we developed a tip-enhanced Raman scattering(TERS)technique to address this challenge.Adopting an optical fiber radial vector mode internally illuminates the plasmonic fiber tip to effectively suppress the background noise while generating a strong electric-field enhanced tip hotspot.Furthermore,the tip hotspot approaching the glucose molecules was manipulated via the shear-force feedback to provide more freedom for selecting substrates.Consequently,our TERS technique achieves the visualization of all Raman modes of glucose molecules within spectral window of 400-3200 cm^(-1),which is not achievable through the far-field/surface-enhanced Raman,or the existing TERS techniques.Our TERS technique offers a powerful tool for accurately identifying Raman scattering of molecules,paving the way for biomolecular analysis. 展开更多
关键词 tip-enhanced Raman scattering scanning near-field optical microscope fiber vector light field tip nanofocusing light source
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Single-beam optical trap-based surfaceenhanced raman scattering optofluidic molecular fingerprint spectroscopy detection system 被引量:1
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作者 Ning Sun Yuan Gan +4 位作者 Yujie Wu Xing Wang Shen Shen Yong Zhu Jie Zhang 《Opto-Electronic Advances》 2025年第2期16-27,共12页
In this study,we developed a single-beam optical trap-based surface-enhanced Raman scattering(SERS)optofluidic molecular fingerprint spectroscopy detection system.This system utilizes a single-beam optical trap to con... In this study,we developed a single-beam optical trap-based surface-enhanced Raman scattering(SERS)optofluidic molecular fingerprint spectroscopy detection system.This system utilizes a single-beam optical trap to concentrate free silver nanoparticles(AgNPs)within an optofluidic chip,significantly enhancing SERS performance.We investigated the optical field distribution characteristics within the tapered fiber using COMSOL simulation software and established a MATLAB simulation model to validate the single-beam optical trap's effectiveness in capturing AgNPs,demonstrating the theoretical feasibility of our approach.To verify the particle capture efficacy of the system,we experimentally controlled the optical trap's on-off state to manage the capture and release of particles precisely.The experimental results indicated that the Raman signal intensity in the capture state was significantly higher than in the non-capture state,confirming that the single-beam optical trap effectively enhances the SERS detection capability of the optofluidic detection system.Furthermore,we employed Raman mapping techniques to investigate the impact of the capture area on the SERS effect,revealing that the spectral intensity of molecular fingerprints in the laser-trapping region is significantly improved.We successfully detected the Raman spectrum of crystal violet at a concentration of 10^(−9)mol/L and pesticide thiram at a concentration of 10^(−5)mol/L,further demonstrating the ability of the single-beam optical trap in enhancing the molecular fingerprint spectrum identification capability of the SERS optofluidic chips.The optical trapping SERS optofluidic detection system developed in this study,as a key component of an integrated optoelectronic sensing system,holds the potential for integration with portable high-power lasers and high-performance Raman spectrometers.This integration is expected to advance highly integrated technologies and significantly enhance the overall performance and portability of optoelectronic sensing systems. 展开更多
关键词 surface-enhanced Raman scattering optofluidic single-beam optical trap tapered optical fibers
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Quantitative detection of trace nanoplastics (down to 50 nm) via surface-enhanced Raman scattering based on the multiplex-feature coffee ring 被引量:1
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作者 Xinao Lin Fengcai Lei +5 位作者 Xiu Liang Yang Jiao Xiaofei Zhao Zhen Li Chao Zhang Jing Yu 《Opto-Electronic Advances》 2025年第6期27-39,共13页
Quantitative detection of trace small-sized nanoplastics(<100 nm)remains a significant challenge in surface-enhanced Raman scattering(SERS).To tackle this issue,we developed a hydrophobic CuO@Ag nanowire substrate ... Quantitative detection of trace small-sized nanoplastics(<100 nm)remains a significant challenge in surface-enhanced Raman scattering(SERS).To tackle this issue,we developed a hydrophobic CuO@Ag nanowire substrate and introduced a multiplex-feature analysis strategy based on the coffee ring effect.This substrate not only offers high Raman enhancement but also exhibits a high probability of detection(POD),enabling rapid and accurate identification of 50 nm polystyrene nanoplastics over a broad concentration range(1–10−10 wt%).Importantly,experimental results reveal a strong correlation between the coffee ring formation and the concentration of nanoplastic dispersion.By incorporating Raman signal intensity,coffee ring diameter,and POD as combined features,we established a machine learning-based mapping between nanoplastic concentration and coffee ring characteristics,allowing precise predictions of dispersion concentration.The mean squared error of these predictions is remarkably low,ranging from 0.21 to 0.54,representing a 19 fold improvement in accuracy compared to traditional linear regression-based methods.This strategy effectively integrates SERS with wettability modification techniques,ensuring high sensitivity and fingerprinting capabilities,while addressing the limitations of Raman signal intensity in accurately reflecting concentration changes at ultra-low levels,providing a new idea for precise SERS measurements of nanoplastics. 展开更多
关键词 quantitative detection of trace nanoplastics surface-enhanced Raman scattering coffee ring multiplexfeature analysis machine learning
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Electron dynamics in neutron scattering with hydrogen atoms
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作者 Mingzhao Xing Libin Fu 《Communications in Theoretical Physics》 2025年第1期158-163,共6页
Gas targets have been used to measure the scattering length in neutron-proton(n-p)scattering experiments.Changes in electron dynamics within the gas target have a negligible effect on the dynamics of nucleons.However,... Gas targets have been used to measure the scattering length in neutron-proton(n-p)scattering experiments.Changes in electron dynamics within the gas target have a negligible effect on the dynamics of nucleons.However,electron dynamics are sensitively related to the specific form of the n-p interaction during the scattering process.We propose a theoretical approach to explore electron dynamics and determine the parameters of the n-p interaction.This approach is based on a three-body scattering process involving a neutron,a proton and an electron.Numerical results indicate significant differences in electron dynamics with varying values of n-p interaction parameters,providing additional information beyond scattering cross-sections to accurately determine these parameters. 展开更多
关键词 neutron scattering three-body scattering electron dynamics momentum spectrum
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Enhanced Spin-Orbit Torque Induced by Interfacial Scattering in Ir/Pt Superlattice
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作者 Jiahui Li Jing Dong +19 位作者 Yuqiang Wang Mingtong Zhu Yang Yao Ying Meng Jiyang Ou Guibin Lan Xuming Luo Jihao Xia Hongjun Xu Yizhan Wang Jiafeng Feng Hongxiang Wei Congli He Richeng Yu Junwei Zhang Yong Peng Nianpeng Lu Caihua Wan Xiufeng Han Guoqiang Yu 《Chinese Physics Letters》 2025年第5期140-150,共11页
The mechanisms of enhancing spin-orbit torque(SOT) have attracted significant attention, particularly regarding the influence of extrinsic scattering mechanisms on SOT efficiency, as they complement intrinsic contribu... The mechanisms of enhancing spin-orbit torque(SOT) have attracted significant attention, particularly regarding the influence of extrinsic scattering mechanisms on SOT efficiency, as they complement intrinsic contributions. In multilayer systems, extrinsic interfacial scattering, along with scattering from defects or impurities inside the materials, plays a crucial role in affecting the SOT efficiency. In this study, we successfully fabricated high-quality epitaxially grown [Ir/Pt]N superlattices with an increasing number of interfaces using a magnetron sputtering system to investigate the contribution of extrinsic interfacial scattering to SOT efficiency. We measured SOT efficiency through spin-torque ferromagnetic resonance methods and determined the spin Hall angle using the spin pumping technique. Additionally, we calculated spin transparency based on the SOT efficiency and spin Hall angle. Our findings indicate that the values of SOT efficiency, spin Hall angle, and spin transparency are enhanced in the superlattice structure compared to Pt, which we attribute to the increase in interfacial scattering.This research offers an effective strategy for designing and fabricating advanced spintronic devices. 展开更多
关键词 interfacial scattering spin transparency spin Hall angle extrinsic scattering mechanisms extrinsic interfacial scattering spin tronic devices ir pt superlattice spin orbit torque
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Quantitative Measurement of Temperature-Dependent Quasiparticle Scattering of the Topological Surface States in Bi_(2)Se_(3)
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作者 Shengyue Lu Yeqinbo Zhang +3 位作者 Xueyan Ma Jingze Li Yongkai Deng Yunquan Liu 《Chinese Physics Letters》 2025年第1期153-162,共10页
The quasiparticle scattering processes of the topological surface state(TSS)in three-dimensional topological insulators(TIs)have a vital effect on the many-body interactions and potential applications of topological m... The quasiparticle scattering processes of the topological surface state(TSS)in three-dimensional topological insulators(TIs)have a vital effect on the many-body interactions and potential applications of topological materials.In this study,we performed high-resolution temperature-dependent angle-resolved photoemission spectroscopy analysis of the 3D strong TI Bi_(2)Se_(3).Using an ab initio simulation,we analyzed the temperature dependence of the electronic structure and lifetime broadening of the TSS,which are closely associated with the quasiparticle scattering process,i.e.,electron–phonon coupling and spin-dependent scattering.We show that,at a low temperature(7 K),the spin-dependent electron scattering facilitates the anisotropic scattering rate of the TSS.Conversely,at room temperature(300 K),the electron–phonon coupling dominates the contribution to the scattering rate.The scattering rate increases with temperature and becomes uniform in momentum space owing to the temperature dependence of quasiparticle scattering.The quantitative study of temperature-dependent scattering rates in TSS is crucial to understanding the topological property and transport mobility of Dirac fermions for fundamental studies and potential applications. 展开更多
关键词 scattering materials TOPOLOGICAL
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Ultraviolet spectral broadening by stimulated rotational Raman scattering on nitrogen pumped with signal laser injection
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作者 Xiangbing Wang Xiangxu Chai +10 位作者 Ping Li Bo Zhang Qihua Zhu Xiaocheng Tian Ju Wang Zhaoyu Zong Song Zhou Ke Yao Sen Li Junpu Zhao Zhitao Peng 《Matter and Radiation at Extremes》 2025年第1期33-38,共6页
We present experimental results on kilojoule ultraviolet laser output with 1%spectral broadening.Through stimulated rotational Raman scattering(SRRS)with signal laser injection,we achieve effective spectral broadening... We present experimental results on kilojoule ultraviolet laser output with 1%spectral broadening.Through stimulated rotational Raman scattering(SRRS)with signal laser injection,we achieve effective spectral broadening in short-range propagation,with good retention of the original near-field distribution and time waveform.Theoretical calculations show that 2%bandwidth spectral broadening can be achieved by injecting 20 kW/cm^(2) signal light at 2.2 GW/cm^(2) flux of the pump laser.In addition,high-frequency modulation in the near field can be effectively avoided through replacement of the original random noise signal light by the controllable signal light.The SRRS in the atmospheric environment excited with signal laser injection can provide wide-band light output with controllable beam quality without long-distance propagation,representing an important potential route to realization of broadband laser drivers. 展开更多
关键词 scattering PUMPED PUMP
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Coherent Compton scattering using a stretched off-axis paraboloid
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作者 Kai Zhao Chang-Bo Fu +1 位作者 Xiang-Jin Kong Yu-Gang Ma 《Nuclear Science and Techniques》 2025年第8期270-277,共8页
Extreme ultraviolet(EUV)lithography is crucial for advancing semiconductor manufacturing;however,current EUV light sources,such as laser-produced plasma(LPP),have significant limitations,including low energy-conversio... Extreme ultraviolet(EUV)lithography is crucial for advancing semiconductor manufacturing;however,current EUV light sources,such as laser-produced plasma(LPP),have significant limitations,including low energy-conversion efficiency and debris contamination.Various schemes,including optical free-electron laser undulators,have been studied to generate coherent EUV light.However,optical undulators suffer from limited focal lengths,which pose a significant challenge to achieving a higher gain.In this study,a novel approach is proposed that employs a stretched off-axis paraboloid(sOAP)mirror,thus extending the focus distance to the centimeter range while achieving a well-controlled periodic light field.This enables high-intensity 92-eV EUV sources to exceed 1016/s,as demonstrated in the simulations.The proposed setup provides an efficient and powerful solution for advanced applications including semiconductor lithography. 展开更多
关键词 Laser Compton scattering(LCS) Coherent scattering Free-electron laser(FEL)
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Elastic scattering of metastable positronium from antihydrogen
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作者 Yi Zhang Jun-Yi Zhang 《Communications in Theoretical Physics》 2025年第7期187-192,共6页
The study of collision between metastable positronium(Ps)and antihydrogen(H)is crucial for precision experiments involving H.In this paper,we investigate the elastic scattering between H and Ps(2s)by combining the con... The study of collision between metastable positronium(Ps)and antihydrogen(H)is crucial for precision experiments involving H.In this paper,we investigate the elastic scattering between H and Ps(2s)by combining the confined variational method with the projection method,for scattering energies from 0.0245 eV to 0.068 eV.Our calculations provide accurate phase shifts and cross sections for the 1,3S and 1,3P symmetries.Near the binding threshold,the rapid increase in the total cross section may be attributed to the P-wave resonance effect.Additionally,we determined the S-wave scattering lengths to be 9.34 a_(0)and 5.81 a_(0)for singlet and triplet elastic scattering,respectively. 展开更多
关键词 elastic scattering POSITRONIUM ANTIHYDROGEN
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Some regularity properties of scattering data for the derivative nonlinear Schrödinger equation
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作者 Weifang Weng Zhenya Yan 《Communications in Theoretical Physics》 2025年第5期1-20,共20页
In this paper,we present some properties of scattering data for the derivative nonlinear Schrödinger equation in H^(S)(R)(s≥1/2)starting from the Lax pair.We show that the reciprocal of the transmission coeffici... In this paper,we present some properties of scattering data for the derivative nonlinear Schrödinger equation in H^(S)(R)(s≥1/2)starting from the Lax pair.We show that the reciprocal of the transmission coefficient can be expressed as the sum of some iterative integrals,and its logarithm can be written as the sum of some connected iterative integrals.We provide the asymptotic properties of the first few iterative integrals of the reciprocal of the transmission coefficient.Moreover,we provide some regularity properties of the reciprocal of the transmission coefficient related to scattering data in H^(S)(R). 展开更多
关键词 derivative nonlinear Schrödinger equation modified Zakharov-Shabat spectral problem scattering data inverse scattering transform ASYMPTOTICS
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Semiclassical Coulomb-scattering model for strong-field tunneling ionization
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作者 Qing Zhao Yigen Peng +4 位作者 Jiayin Che Chao Chen Shang Wang Guoguo Xin Yanjun Chen 《Chinese Physics B》 2025年第9期160-167,共8页
This study analytically examines the ionization of atoms in strong near-circular laser fields.The classic Keldysh-Rutherford(KR)Coulomb-scattering(CS)model[Phys.Rev.Lett.121123201(2018)]successfully explained the atto... This study analytically examines the ionization of atoms in strong near-circular laser fields.The classic Keldysh-Rutherford(KR)Coulomb-scattering(CS)model[Phys.Rev.Lett.121123201(2018)]successfully explained the attoclock experimental curve for the H atom at lower laser intensities.Here,we develop a semiclassical model that includes the initial conditions related to the quantum properties of tunneling in the KR model at the beginning of the scattering process.This model is able to explain recent attoclock experimental curves over a wider range of laser and atomic parameters.Our results show the importance of system symmetry and quantum effects in attoclock measurements,suggesting the complex role of the Coulomb potential in strong-field ionization. 展开更多
关键词 tunneling ionization Coulomb scattering attoclock
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Experimental research on stimulated Raman scattering under a hybrid-drive ignition path
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作者 Kaiqiang Pan Zhanjun Liu +8 位作者 Xuelong Qin Jiwei Li Tao Gong Qing Wang Ji Yan Zhichao Li Dong Yang Yonggang Liu Xiantu He 《Matter and Radiation at Extremes》 2025年第5期45-53,共9页
Stimulated Raman scattering(SRS)under a new ignition path that combines the advantages of direct-drive(DD)and indirect-drive(ID)schemes is investigated experimentally at the Shenguang-100 kJ facility.The results show ... Stimulated Raman scattering(SRS)under a new ignition path that combines the advantages of direct-drive(DD)and indirect-drive(ID)schemes is investigated experimentally at the Shenguang-100 kJ facility.The results show that collective SRS in the plasma produced by ablating a polyimide film is detected for the ID beams,but is suppressed by adding a toe before the main pulse of the ID beams.The toe also strongly influences SRS of both the ID and DD beams excited in the plasma generated in the hohlraum.When a toe is used,the SRS spectra of the DD beams show that SRS tends to be excited in lower plasma density,which will result in a lower risk of super-hot electrons.Measurements of hot electrons support this conclusion.This research will help us produce a better pulse design for this new ignition path. 展开更多
关键词 stimulated raman scattering srs ignition path Direct Drive Stimulated Raman scattering ablating polyimide film Plasma Density Indirect Drive id dd beams
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Modeling the electronic band-structure of strained long-wavelength Type-Ⅱsuperlattices using the scattering matrix method
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作者 Abbas Haddadi Gail Brown Manijeh Razeghi 《红外与毫米波学报》 北大核心 2025年第3期346-351,共6页
This study introduces a comprehensive theoretical framework for accurately calculating the electronic band-structure of strained long-wavelength InAs/GaSb type-Ⅱsuperlattices.Utilizing an eight-band k·p Hamilto⁃... This study introduces a comprehensive theoretical framework for accurately calculating the electronic band-structure of strained long-wavelength InAs/GaSb type-Ⅱsuperlattices.Utilizing an eight-band k·p Hamilto⁃nian in conjunction with a scattering matrix method,the model effectively incorporates quantum confinement,strain effects,and interface states.This robust and numerically stable approach achieves exceptional agreement with experimental data,offering a reliable tool for analyzing and engineering the band structure of complex multi⁃layer systems. 展开更多
关键词 type-Ⅱsuperlattices long-wavelength infrared(LWIR) scattering matrix method electronic band-structure modeling InAs/GaSb heterostructures infrared photodetectors bandgap engineering
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Optimization of transverse unidirectional scattering by morphology modification of irregular V-shaped silicon nanoantennas
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作者 ZENG Ming ZHAO Feng WANG Xianghui 《Optoelectronics Letters》 2025年第3期129-135,共7页
A scheme based on irregular V-shaped silicon nanoantennas is proposed to optimize transverse unidirectional scattering under plane wave irradiation.Traditional methods of designing regular shapes offer fewer parameter... A scheme based on irregular V-shaped silicon nanoantennas is proposed to optimize transverse unidirectional scattering under plane wave irradiation.Traditional methods of designing regular shapes offer fewer parameters and higher search efficiency.However,due to the limitations of regular shapes,it is challenging to meet high-precision design requirements.Irregular shape design allows for a broader range of adjustments,but the complexity of shape parameters leads to lower search efficiency and a higher likelihood of converging to local optima. 展开更多
关键词 irregular v shaped silicon nanoantennas plane wave irradiation design efficiency plane wave irradiationtraditional optimize transverse unidirectional scattering morphology modification transverse unidirectional scattering search efficiency
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Single photon scattering with the giant and small atom interplay in a one-dimensional coupled resonator waveguide
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作者 Xi Tian Xiaojun Zhang +3 位作者 Wei Zhao Jingcheng Hou Zhihai Wang Tian Tian 《Communications in Theoretical Physics》 2025年第2期64-69,共6页
We study single photon scattering in a one-dimensional coupled resonator waveguide,which is dressed by a small and a giant artificial atom simultaneously.Here,we have set the small atom to be a neighbor to one leg of ... We study single photon scattering in a one-dimensional coupled resonator waveguide,which is dressed by a small and a giant artificial atom simultaneously.Here,we have set the small atom to be a neighbor to one leg of the giant atom,and the giant atom couples to the waveguide via two distant sites.When the small and giant atoms are both resonant with the bare resonator in the waveguide,we observe the perfect reflection of the resonant incident photon.On the other hand,when the small atom is detuned from the giant atom,the single photon reflection is characterized by a wide window and Fano line shape.We hope our work will pave the way for the potential application of small and giant atom hybrid systems in the study of photonic control in the lowdimensional waveguide structure. 展开更多
关键词 giant atom single-photon scattering fano shape
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Active polarization high-resolution imaging through complex scattering media
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作者 Meng Xiang Xue Dong +6 位作者 Tianyu Wang Sen Wang Jingjing Ge Jinpeng Liu Qianqian Liu Fei Liu Xiaopeng Shao 《Advanced Photonics Nexus》 2025年第1期127-137,共11页
High-resolution seeing through complex scattering media such as turbid water,biological tissues,and mist is a significant challenge because the strong scattering scrambles the light paths and forms the scattering wall... High-resolution seeing through complex scattering media such as turbid water,biological tissues,and mist is a significant challenge because the strong scattering scrambles the light paths and forms the scattering wall.We propose an active polarized iterative optimization approach for high-resolution imaging through complex scattering media.By acquiring a series of sub-polarized images,we can capture the diverse pattern-illuminated images with various high-frequency component information caused by the Brownian motion of complex scattering materials,which are processed using the common-mode rejection of polarization characteristics to extract target information from scattering medium information.Following that,our computational reconstruction technique employs an iterative optimization algorithm that commences with patternilluminated Fourier ptychography for reconstructing the high-resolution scene.It is extremely important that our approach for high-resolution imaging through complex scattering media is not limited by priori information and optical memory effect.The proposed approach is suitable for not only dynamic but also static scattering media,which may find applications in the biomedicine field,such as skin abnormalities,non-invasive blood flow,and superficial tumors. 展开更多
关键词 complex scattering media iterative optimization POLARIZATION Fourier ptychography.
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Four-wave mixing Bragg scattering for small frequency shift from silicon coupled microrings
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作者 Chang Zhao Chao Wu +5 位作者 Pingyu Zhu Yuxing Du Yan Wang Miaomiao Yu Kaikai Zhang Ping Xu 《Chinese Physics B》 2025年第1期351-355,共5页
Frequency conversion is pivotal in nonlinear optics and quantum optics for manipulating and translating light signals across different wavelength regimes.Achieving frequency conversion between two light beams with a s... Frequency conversion is pivotal in nonlinear optics and quantum optics for manipulating and translating light signals across different wavelength regimes.Achieving frequency conversion between two light beams with a small frequency interval is a central challenge.In this work,we design a pair of coupled silicon microrings wherein coupled-induced modesplitting exists to achieve a small frequency shift by the process of four-wave mixing Bragg scattering.As an example,the signal can be up or down converted to the idler which is 15.5 GHz spaced when two pumps align with another pair of split resonances.The results unveil the potential of coupled microring resonators for small interval frequency conversion in a high-fidelity,all-optical,and signal processing quantum frequency interface. 展开更多
关键词 four-wave mixing Bragg scattering silicon coupled microrings
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Unravel the Spinodal Decomposition Kinetics in(FeCoCrNi)85(AlCu)15 Alloy through Small-Angle Neutron Scattering
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作者 Shun-Fu Xie Han-Qiu Jiang +2 位作者 Zhen-Hua Xie Wei-Wen Zhang Yu-Bin Ke 《Acta Metallurgica Sinica(English Letters)》 2025年第1期86-92,共7页
High entropy alloys(HEAs)constituted of single solid solution phase,but remains chemical inhomogeneity in nature due to its multi-principal composition.Currently,existence of nanoscale spinodal decomposition(SD)phase ... High entropy alloys(HEAs)constituted of single solid solution phase,but remains chemical inhomogeneity in nature due to its multi-principal composition.Currently,existence of nanoscale spinodal decomposition(SD)phase in matrix was found to have significant impact on the properties of HEAs.Nevertheless,the morphology evolution and the kinetics of SD is not clear,which hinders in-depth understanding of the structure-property relationship.In this study,we examine the spinodal structures in(FeCoCrNi)85(AlCu)15 HEAs at different states using in-situ small-angle neutron scattering(SANS),in conjunction with transmission electron microscopy technique.The result demonstrates that SD occurred when aging the HEA samples at temperatures ranging from 500 to 800℃,which leads to the phase constitution of NiAlCu-rich and FeCoCr-rich spinodal phases,L1_(2)ordered phases,and FCC matrix.The characteristic wavelength of SD(λ_(SD))grows from 5.31 to 51.26 nm when aging temperature rises from 500 to 800℃,which explains the enhancement of the alloy’s microhardness.The SD kinetics was unraveled by fitting the time-dependentλ_(SD)through in-situ SANS measurement at 700℃.During isothermal treatment at 700℃,theλ_(SD)increases from 10.42 to 17.43 nm with prolonged time,and SD is in the late stage from the exponential trend of theλ_(SD)over time.Moreover,comparing with aging temperature,the aging time has a relatively minor impact on the coarsening of SD. 展开更多
关键词 High entropy alloys Spinodal decomposition Small-angle neutron scattering KINETICS
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Transparent and Flexible Surface-enhanced Raman Scattering (SERS) Substrates with High SERS Performance and Stability
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作者 Jian-Ping Peng Pei-Jiang Liu +3 位作者 Yu-Tao Song Shan-Zheng Zhao Xin-Yue Deng Zhen-Kai Huang 《Chinese Journal of Polymer Science》 2025年第9期1584-1591,I0009,共9页
This paper presents a polymer-brush-guided templating strategy for fabricating ordered gold plasmonic architectures.The synthesized nanostructures featuring densely packed Au nanoparticles(NPs)exhibited strong surface... This paper presents a polymer-brush-guided templating strategy for fabricating ordered gold plasmonic architectures.The synthesized nanostructures featuring densely packed Au nanoparticles(NPs)exhibited strong surface-enhanced Raman scattering(SERS)activity.Using a simple mechanical transfer technique,these assemblies were integrated into flexible polydimethylsiloxane(PDMS)films.Polymer encapsulation during synthesis ensures structural integrity during processing,resulting in a mechanically robust SERS substrate with exceptional analytical performance.This platform achieved 4-mercaptobenzoic acid(4-MBA)detection at 100 pmol/L(10-10 mol/L)with high reproducibility(RSD=6.8%).Environmental and mechanical stability tests demonstrated 95%signal retention over 30 days and sustained functionality after 100 bending/twisting cycles.Combined with a non-destructive adhesion-transfer protocol,the substrate enabled on-site thiram detection on apple surfaces(1μmol/L limit).This study provides a scalable approach for developing flexible SERS devices for food safety monitoring and environmental analysis. 展开更多
关键词 Flexible sensors Patterned Au nanostructures POLYDIMETHYLSILOXANE Surface-enhanced Raman scattering
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