Succinonitrile(SN)-based polymer plastic crystal electrolytes(PPCEs)are regarded as promising candidates for lithium metal batteries but suffer from serious side reactions with Li metal.Herein,we propose a multi-dimen...Succinonitrile(SN)-based polymer plastic crystal electrolytes(PPCEs)are regarded as promising candidates for lithium metal batteries but suffer from serious side reactions with Li metal.Herein,we propose a multi-dimensional optimization strategy to alleviate the side reactions between SN and Li metal,and develop a highly stable poly-vinylethylene carbonate-based PPCE(PPCE-VEC).Moreover,we identify the intrinsic factors of multi-dimensional polymer structures on the electrolyte stability by three typical classes of polyesters.The PPCE-VEC constructed by in situ polymerization exhibits much better stability than poly-vinylene carbonate-based PPCE(PPCE-VCA)and poly-trifluoroethyl acrylate-based PPCE(PPCE-TFA),which is verified by its fewer SN-decomposition species in X-ray photoelectron spectroscopy(XPS)and outstanding full cell performance.The PPCE-VEC-enabled LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2)full cell achieve 73.7%capacity retention after 1400 cycles,which outperforms PPCE-VCA-and PPCE-TFA-enabled full cells(61.9%and 46.9%).Spectral analysis and theoretical calculation reveal that the high solvation ability of the carbonyl site,flexible polymer chain,and homogeneous electrolyte phase of PPCE-VEC are favorable to maximizing competition coordination with Li^(+)to weaken the Li^(+)–SN binding and shape an anion-rich solvation structure.This optimized polymer-involved Li^(+)solvation enhances SN stability and facilitates the formation of B/F enriched solid-electrolyte interphase(SEI),thus significantly improving PPCE stability.展开更多
A composite anti-disturbance predictive control strategy employing a Multi-dimensional Taylor Network(MTN)is presented for unmanned systems subject to time-delay and multi-source disturbances.First,the multi-source di...A composite anti-disturbance predictive control strategy employing a Multi-dimensional Taylor Network(MTN)is presented for unmanned systems subject to time-delay and multi-source disturbances.First,the multi-source disturbances are addressed according to their specific characteristics as follows:(A)an MTN data-driven model,which is used for uncertainty description,is designed accompanied with the mechanism model to represent the unmanned systems;(B)an adaptive MTN filter is used to remove the influence of the internal disturbance;(C)an MTN disturbance observer is constructed to estimate and compensate for the influence of the external disturbance;(D)the Extended Kalman Filter(EKF)algorithm is utilized as the learning mechanism for MTNs.Second,to address the time-delay effect,a recursiveτstep-ahead MTN predictive model is designed utilizing recursive technology,aiming to mitigate the impact of time-delay,and the EKF algorithm is employed as its learning mechanism.Then,the MTN predictive control law is designed based on the quadratic performance index.By implementing the proposed composite controller to unmanned systems,simultaneous feedforward compensation and feedback suppression to the multi-source disturbances are conducted.Finally,the convergence of the MTN and the stability of the closed-loop system are established utilizing the Lyapunov theorem.Two exemplary applications of unmanned systems involving unmanned vehicle and rigid spacecraft are presented to validate the effectiveness of the proposed approach.展开更多
Optical-resolution photoacoustic microscopy is a novel imaging technique that combines the advantages of optical and ultrasound imaging,enabling high-resolution visualization of biological tissues at the micrometer sc...Optical-resolution photoacoustic microscopy is a novel imaging technique that combines the advantages of optical and ultrasound imaging,enabling high-resolution visualization of biological tissues at the micrometer scale.However,the divergence of the excited Gaussian beam limits the depth-of-field of the system to less than 100μm,which hinders accurate three-dimensional imaging of living tissues and restrictsits applicability in biological research.Therefore,there is an urgent need for an effective method to enhance the depth-of-field without altering the hardware configuration.This paper presents a photoacoustic microscopy depth-of-field extension method and system based on three-dimensional continuity and sparsity deconvolution.This method utilizes a depth-varying point spread function and incorporates continuity and sparsity con-straints into the deconvolution process to mitigate the effect of background noise,enhancing the stability and accuracy of the depth-of-field extension.Experimental results using tungsten wire phantoms suggest that the depth-of-field of system can be extended to 650 pm,which is 7.2 times greater than conventional system,while improving the resolution of the defocused region by an average factor of 3.5.Furthermore,experiments on zebrafish and nude mouse ears with irregular topologies demonstrate that the proposed method successfully overcomes image blurring and the loss of structural information due to limited depth-of-field.All the results suggest that the system with higher lateral resolution and enhanced depth-of-field has significant potential for a wide range of practical biomedical applications.展开更多
The ancient tacit knowledge behind the logic system permeated the culture and promoted numerous impactful inventions throughout the history. Traditional Chinese medicine with its effectiveness should also have stemmed...The ancient tacit knowledge behind the logic system permeated the culture and promoted numerous impactful inventions throughout the history. Traditional Chinese medicine with its effectiveness should also have stemmed out from such logic system. This article aims to rearticulate the underlying lucid multi-dimensional logic system, which faded in obscurity only because of time-out loss of the mid-right concept. Retracing this past tacit but important concept could uncover a multi-dimensional system over a point relating to all matters while capturing the central core of the matter. The seemingly unmanageable multidimensional logic was strengthened by verification processes which affirmed its further extensions, and made up the language of the people, the concepts of yin-yang(阴阳), and the development of extensions of Ba Gua(八卦) derivatives, which furthered the interpretation of the space-time properties and Chinese medicine.展开更多
Stress accumulation is a key factor leading to sodium storage performance deterioration for NiSe_(2)-based anodes.Therefore,inhibiting the concentrated local stress during the sodiataion/desodiation process is crucial...Stress accumulation is a key factor leading to sodium storage performance deterioration for NiSe_(2)-based anodes.Therefore,inhibiting the concentrated local stress during the sodiataion/desodiation process is crucial for acquiring stable NiSe2-based materials for sodium-ion batteries(SIBs),Herein,a stress dissipation strategy driven by architecture engineering is proposed,which can achieve ultrafast and ultralong sodium storage properties.Different from the conventional sphere-like or rod-like architecture,the three-dimensional(3D)flower-like NiSe_(2)@C composite is delicately designed and assembled with onedimensional nanorods and carbon framework.More importantly,the fundamental mechanism of improved structure stability is unveiled by simulations and experimental results simultaneously.It demonstrates that this designed multidimensional flower-like architecture with dispersed nanorods can balance the structural mismatch,avoid concentrated local strain,and relax the internal stress,mainly induced by the unavoidable volume variation during the repeated conversion processes.Moreover,it can provide more Na^(+)-storage sites and multi-directional migration pathways,leading to a fast Na^(+)-migration channel with boosted reaction kinetic.As expected,it delivers superior rate performance(441 mA h g^(-1)at 5.0 A g^(-1))and long cycling stability(563 mA h g^(-1)at 1.0 A g^(-1)over 1000 cycles)for SIBs.This work provides useful insights for designing high-performance conversion-based anode materials for SIBs.展开更多
This paper explores whole-process engineering consulting,including its application models in public buildings and elderly-friendly projects,such as service integration and whole lifecycle management.It also addresses ...This paper explores whole-process engineering consulting,including its application models in public buildings and elderly-friendly projects,such as service integration and whole lifecycle management.It also addresses the construction of multi-dimensional collaborative theoretical models,public space streamline organization,and other aspects,emphasizing the importance of multi-dimensional collaboration.Additionally,it highlights the role of talent cultivation and digital transformation in enhancing project efficiency.展开更多
Traditional deconvolution methods based on single-channel inversion do not consider the spatial structural relation between channels,and hence,they yield high-resolution results with the existing transverse inconsiste...Traditional deconvolution methods based on single-channel inversion do not consider the spatial structural relation between channels,and hence,they yield high-resolution results with the existing transverse inconsistency or discontinuity.Therefore,in this study,the local dip angle was used to obtain the structural information and construct the spatial structurally constraint operator.This operator is then introduced into multichannel deconvolution as a regularization operator to improve the resolution and maintain the transverse continuity of seismic data.Model tests and actual seismic data processing have demonstrated the effectiveness and practicability of this method.展开更多
The multi-dimensional interactive teaching model significantly enhances the effectiveness of college English instruction by emphasizing dynamic engagement between teachers and students,as well as among students themse...The multi-dimensional interactive teaching model significantly enhances the effectiveness of college English instruction by emphasizing dynamic engagement between teachers and students,as well as among students themselves.This paper explores practical strategies for implementing this model,focusing on four key aspects:deepening teachers’understanding of the model through continuous learning,innovating interactive methods such as questioning techniques and practical activities,leveraging modern technology to integrate resources and track learning progress,and establishing a communication platform that centers on student participation.By adopting these approaches,the model fosters a student-centered classroom environment,improves comprehensive English application skills,and optimizes overall teaching quality.展开更多
During the critical transformation period of landscape architecture major after the adjustment of disciplinary structure and the changes in market demand,private colleges and universities,as important places for culti...During the critical transformation period of landscape architecture major after the adjustment of disciplinary structure and the changes in market demand,private colleges and universities,as important places for cultivating local talents,have pain points such as uneven quality of teachers and students and weak innovation and practice.The practice system with“multi-dimensional Integration”integrates four dimensions:interdisciplinary integration,spatial and temporal intersection,historical inheritance,and behavioral activity,deepens the disciplinary connotation,and integrates the three elements of nature,humanity,and technology,aiming to provide a new path for private colleges and universities to cultivate application-oriented and compound talents with innovative capabilities.In terms of optimizing talent cultivation and adapting to industry changes,this system provides thinking and reference for landscape architecture major,helping the major reshape its core competitiveness and promoting educational innovation and industry development.展开更多
This paper proposes a reliability evaluation model for a multi-dimensional network system,which has potential to be applied to the internet of things or other practical networks.A multi-dimensional network system with...This paper proposes a reliability evaluation model for a multi-dimensional network system,which has potential to be applied to the internet of things or other practical networks.A multi-dimensional network system with one source element and multiple sink elements is considered first.Each element can con-nect with other elements within a stochastic connection ranges.The system is regarded as successful as long as the source ele-ment remains connected with all sink elements.An importance measure is proposed to evaluate the performance of non-source elements.Furthermore,to calculate the system reliability and the element importance measure,a multi-valued decision diagram based approach is structured and its complexity is analyzed.Finally,a numerical example about the signal transfer station system is illustrated to analyze the system reliability and the ele-ment importance measure.展开更多
Constructing multi-dimensional hydrogen bond(H-bond)regulated single-molecule systems with multiemission remains a challenge.Herein,we report the design of a new excited-state intramolecular proton transfer(ESIPT)feat...Constructing multi-dimensional hydrogen bond(H-bond)regulated single-molecule systems with multiemission remains a challenge.Herein,we report the design of a new excited-state intramolecular proton transfer(ESIPT)featured chromophore(HBT-DPI)that shows flexible emission tunability via the multidimensional regulation of intra-and intermolecular H-bonds.The feature of switchable intramolecular Hbonds is induced via incorporating several hydrogen bond acceptors and donors into one single HBT-DPI molecule,allowing the“turn on/off”of ESIPT process by forming isomers with distinct intramolecular Hbonds configurations.In response to different external H-bonding environments,the obtained four types of crystal/cocrystals vary in the contents of isomers and the molecular packing modes,which are mainly guided by the intermolecular H-bonds,exhibiting non-emissive features or emissions ranging from green to orange.Utilizing the feature of intermolecular H-bond guided molecular packing,we demonstrate the utility of this fluorescent material for visualizing hydrophobic/hydrophilic areas on large-scale heterogeneous surfaces of modified poly(1,1-difluoroethylene)(PVDF)membranes and quantitatively estimating the surface hydrophobicity,providing a new approach for hydrophobicity/hydrophilicity monitoring and measurement.Overall,this study represents a new design strategy for constructing multi-dimensional hydrogen bond regulated ESIPT-based fluorescent materials that enable multiple emissions and unique applications.展开更多
To break the limitations of the multi-dimensional(M-D)vibration isolation(VI)platforms with the Stewart-Gough design,such as strongly coupling motions,excessive friction in connections,heavy weight,and limited workspa...To break the limitations of the multi-dimensional(M-D)vibration isolation(VI)platforms with the Stewart-Gough design,such as strongly coupling motions,excessive friction in connections,heavy weight,and limited workspace,this study processes a novel platform integrated by a stiffness-adjustable origami spring sub-structure and a parallel mechanism.The origami-based stiffness-adjustable spring realizes low-frequency VI,and the parallel mechanism symmetry design realizes motions decoupling.In the origami-based sub-leg,the parallel-stack-assembly(PSA)design mechanism with two Miura origami configurations is proposed to generate a symmetrical negative stiffness property.Paired with a linear positive stiffness spring,the origami-based sub-leg has wide-amplitude-high-static-low-dynamic stiffness(WA-HSLDS)characteristics in one direction.Then,with construction of the parallel mechanism connected with origami-based sub-legs,an M-D VI platform is achieved,whose motions in the vertical direction and yaw direction are decoupled with the motions in the other directions.Based on the dynamic model and incremental harmonic balance(IHB)with the arc-length continuation method,appropriate structural parameters in the parallel mechanism part are figured out,and the accurate transmissibility in different directions is defined,which gives the parametric influencing investigations for realization of low-frequency VI performances.Finally,experiments are conducted to validate the accuracy and feasibility of the theoretical methods,and to demonstrate the performance of M-D low-frequency isolation with load-carrying capacity of the proposed VI platform.The integration of the origami into the parallel mechanism results in a compact,efficient,and flexible platform with nonlinear adjustability,offering new possibilities for lightweight M-D VI,and developing the practical applications in high-precision platforms in ocean and aerospace environments.展开更多
In seismic data processing, blind deconvolution is a key technology. Introduced in this paper is a flow of one kind of blind deconvolution. The optimal precondition conjugate gradients (PCG) in Kyrlov subspace is als...In seismic data processing, blind deconvolution is a key technology. Introduced in this paper is a flow of one kind of blind deconvolution. The optimal precondition conjugate gradients (PCG) in Kyrlov subspace is also used to improve the stability of the algorithm. The computation amount is greatly decreased.展开更多
The conventional nonstationary convolutional model assumes that the seismic signal is recorded at normal incidence. Raw shot gathers are far from this assumption because of the effects of offsets. Because of such prob...The conventional nonstationary convolutional model assumes that the seismic signal is recorded at normal incidence. Raw shot gathers are far from this assumption because of the effects of offsets. Because of such problems, we propose a novel prestack nonstationary deconvolution approach. We introduce the radial trace （RT） transform to the nonstationary deconvolution, we estimate the nonstationary deconvolution factor with hyperbolic smoothing based on variable-step sampling （VSS） in the RT domain, and we obtain the high-resolution prestack nonstationary deconvolution data. The RT transform maps the shot record from the offset and traveltime coordinates to those of apparent velocity and traveltime. The ray paths of the traces in the RT better satisfy the assumptions of the convolutional model. The proposed method combines the advantages of stationary deconvolution and inverse Q filtering, without prior information for Q. The nonstationary deconvolution in the RT domain is more suitable than that in the space-time （XT） domain for prestack data because it is the generalized extension of normal incidence. Tests with synthetic and real data demonstrate that the proposed method is more effective in compensating for large-offset and deep data.展开更多
The Robinson convolution model is mainly restricted by three inappropriate assumptions, i.e., statistically white reflectivity, minimum-phase wavelet, and stationarity. Modern reflectivity inversion methods（e.g., spa...The Robinson convolution model is mainly restricted by three inappropriate assumptions, i.e., statistically white reflectivity, minimum-phase wavelet, and stationarity. Modern reflectivity inversion methods（e.g., sparsity-constrained deconvolution） generally attempt to suppress the problems associated with the first two assumptions but often ignore that seismic traces are nonstationary signals, which undermines the basic assumption of unchanging wavelet in reflectivity inversion. Through tests on reflectivity series, we confirm the effects of nonstationarity on reflectivity estimation and the loss of significant information, especially in deep layers. To overcome the problems caused by nonstationarity, we propose a nonstationary convolutional model, and then use the attenuation curve in log spectra to detect and correct the influences of nonstationarity. We use Gabor deconvolution to handle nonstationarity and sparsity-constrained deconvolution to separating reflectivity and wavelet. The combination of the two deconvolution methods effectively handles nonstationarity and greatly reduces the problems associated with the unreasonable assumptions regarding reflectivity and wavelet. Using marine seismic data, we show that correcting nonstationarity helps recover subtle reflectivity information and enhances the characterization of details with respect to the geological record.展开更多
Sparsity constrained deconvolution can improve the resolution of band-limited seismic data compared to conventional deconvolution. However, such deconvolution methods result in nonunique solutions and suppress weak re...Sparsity constrained deconvolution can improve the resolution of band-limited seismic data compared to conventional deconvolution. However, such deconvolution methods result in nonunique solutions and suppress weak reflections. The Cauchy function, modified Cauchy function, and Huber function are commonly used constraint criteria in sparse deconvolution. We used numerical experiments to analyze the ability of sparsity constrained deconvolution to restore reflectivity sequences and protect weak reflections under different constraint criteria. The experimental results demonstrate that the performance of sparsity constrained deconvolution depends on the agreement between the constraint criteria and the probability distribution of the reflectivity sequences; furthermore, the modified Cauchy- constrained criterion protects the weak reflections better than the other criteria. Based on the model experiments, the probability distribution of the reflectivity sequences of carbonate and clastic formations is statistically analyzed by using well-logging data and then the modified Cauchy-constrained deconvolution is applied to real seismic data much improving the resolution.展开更多
The predictive deconvolution algorithm （PD）, which is based on second-order statistics, assumes that the primaries and the multiples are implicitly orthogonal. However, the seismic data usually do not satisfy this a...The predictive deconvolution algorithm （PD）, which is based on second-order statistics, assumes that the primaries and the multiples are implicitly orthogonal. However, the seismic data usually do not satisfy this assumption in practice. Since the seismic data （primaries and multiples） have a non-Gaussian distribution, in this paper we present an improved predictive deconvolution algorithm （IPD） by maximizing the non-Gaussianity of the recovered primaries. Applications of the IPD method on synthetic and real seismic datasets show that the proposed method obtains promising results.展开更多
The study constructed a multi-dimensional feedback mode integrating teacher feedback, peer feedback and network feedback, and applied it in the teaching of College English Writing. After 16 weeks of teaching, the stud...The study constructed a multi-dimensional feedback mode integrating teacher feedback, peer feedback and network feedback, and applied it in the teaching of College English Writing. After 16 weeks of teaching, the students in the multi-dimen-sional feedback class had significantly better overall writing scores than those in the teacher-feedback class. In terms of individual scores, multi-dimensional feedback played a better role in improving vocabulary and grammar than the class using teacher feed-back. However, there were no significant differences in the responses of writing tasks, coherence and cohesion. The study showed that most students were satisfied with the mode, believing that it was helpful to relieve writing anxiety, stimulate writing interest and improve their writing level.展开更多
基金supported by the National Natural Science Foundation of China(22072048)the Guangdong Provincial Department of Science and Technology(2021A1515010128 and 2022A0505050013).
文摘Succinonitrile(SN)-based polymer plastic crystal electrolytes(PPCEs)are regarded as promising candidates for lithium metal batteries but suffer from serious side reactions with Li metal.Herein,we propose a multi-dimensional optimization strategy to alleviate the side reactions between SN and Li metal,and develop a highly stable poly-vinylethylene carbonate-based PPCE(PPCE-VEC).Moreover,we identify the intrinsic factors of multi-dimensional polymer structures on the electrolyte stability by three typical classes of polyesters.The PPCE-VEC constructed by in situ polymerization exhibits much better stability than poly-vinylene carbonate-based PPCE(PPCE-VCA)and poly-trifluoroethyl acrylate-based PPCE(PPCE-TFA),which is verified by its fewer SN-decomposition species in X-ray photoelectron spectroscopy(XPS)and outstanding full cell performance.The PPCE-VEC-enabled LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2)full cell achieve 73.7%capacity retention after 1400 cycles,which outperforms PPCE-VCA-and PPCE-TFA-enabled full cells(61.9%and 46.9%).Spectral analysis and theoretical calculation reveal that the high solvation ability of the carbonyl site,flexible polymer chain,and homogeneous electrolyte phase of PPCE-VEC are favorable to maximizing competition coordination with Li^(+)to weaken the Li^(+)–SN binding and shape an anion-rich solvation structure.This optimized polymer-involved Li^(+)solvation enhances SN stability and facilitates the formation of B/F enriched solid-electrolyte interphase(SEI),thus significantly improving PPCE stability.
基金co-supported by the National Key R&D Program of China(No.2023YFB4704400)the Zhejiang Provincial Natural Science Foundation of China(No.LQ24F030012)the National Natural Science Foundation of China General Project(No.62373033)。
文摘A composite anti-disturbance predictive control strategy employing a Multi-dimensional Taylor Network(MTN)is presented for unmanned systems subject to time-delay and multi-source disturbances.First,the multi-source disturbances are addressed according to their specific characteristics as follows:(A)an MTN data-driven model,which is used for uncertainty description,is designed accompanied with the mechanism model to represent the unmanned systems;(B)an adaptive MTN filter is used to remove the influence of the internal disturbance;(C)an MTN disturbance observer is constructed to estimate and compensate for the influence of the external disturbance;(D)the Extended Kalman Filter(EKF)algorithm is utilized as the learning mechanism for MTNs.Second,to address the time-delay effect,a recursiveτstep-ahead MTN predictive model is designed utilizing recursive technology,aiming to mitigate the impact of time-delay,and the EKF algorithm is employed as its learning mechanism.Then,the MTN predictive control law is designed based on the quadratic performance index.By implementing the proposed composite controller to unmanned systems,simultaneous feedforward compensation and feedback suppression to the multi-source disturbances are conducted.Finally,the convergence of the MTN and the stability of the closed-loop system are established utilizing the Lyapunov theorem.Two exemplary applications of unmanned systems involving unmanned vehicle and rigid spacecraft are presented to validate the effectiveness of the proposed approach.
基金supported by the National Key R&D Program of China[Grant No.2022YFC2402400]the National Natural Science Foundation of China[Grant No.62275062]+2 种基金Project of Shandong Innovation and Startup Community of High-end Medical Apparatus and Instruments[Grant Nos.2023-SGTTXM-002 and 2024-SGTTXM-005]the Shandong Province Technology Innovation Guidance Plan(Central Leading Local Science and Technology Development Fund)[Grant No.YDZX2023115]the Taishan Scholar Special Funding Project of Shandong Province,and the Shandong Laboratory of Advanced Biomaterials and Medical Devices in Weihai[Grant No.ZL202402].
文摘Optical-resolution photoacoustic microscopy is a novel imaging technique that combines the advantages of optical and ultrasound imaging,enabling high-resolution visualization of biological tissues at the micrometer scale.However,the divergence of the excited Gaussian beam limits the depth-of-field of the system to less than 100μm,which hinders accurate three-dimensional imaging of living tissues and restrictsits applicability in biological research.Therefore,there is an urgent need for an effective method to enhance the depth-of-field without altering the hardware configuration.This paper presents a photoacoustic microscopy depth-of-field extension method and system based on three-dimensional continuity and sparsity deconvolution.This method utilizes a depth-varying point spread function and incorporates continuity and sparsity con-straints into the deconvolution process to mitigate the effect of background noise,enhancing the stability and accuracy of the depth-of-field extension.Experimental results using tungsten wire phantoms suggest that the depth-of-field of system can be extended to 650 pm,which is 7.2 times greater than conventional system,while improving the resolution of the defocused region by an average factor of 3.5.Furthermore,experiments on zebrafish and nude mouse ears with irregular topologies demonstrate that the proposed method successfully overcomes image blurring and the loss of structural information due to limited depth-of-field.All the results suggest that the system with higher lateral resolution and enhanced depth-of-field has significant potential for a wide range of practical biomedical applications.
文摘The ancient tacit knowledge behind the logic system permeated the culture and promoted numerous impactful inventions throughout the history. Traditional Chinese medicine with its effectiveness should also have stemmed out from such logic system. This article aims to rearticulate the underlying lucid multi-dimensional logic system, which faded in obscurity only because of time-out loss of the mid-right concept. Retracing this past tacit but important concept could uncover a multi-dimensional system over a point relating to all matters while capturing the central core of the matter. The seemingly unmanageable multidimensional logic was strengthened by verification processes which affirmed its further extensions, and made up the language of the people, the concepts of yin-yang(阴阳), and the development of extensions of Ba Gua(八卦) derivatives, which furthered the interpretation of the space-time properties and Chinese medicine.
基金the financial support from the Guangxi Natural Science Foundation(grant no.2021GXNSFDA075012,2023GXNSFGA026002)National Natural Science Foundation of China(52104298,22075073,52362027,52462029)Fundamental Research Funds for the Central Universities(531107051077).
文摘Stress accumulation is a key factor leading to sodium storage performance deterioration for NiSe_(2)-based anodes.Therefore,inhibiting the concentrated local stress during the sodiataion/desodiation process is crucial for acquiring stable NiSe2-based materials for sodium-ion batteries(SIBs),Herein,a stress dissipation strategy driven by architecture engineering is proposed,which can achieve ultrafast and ultralong sodium storage properties.Different from the conventional sphere-like or rod-like architecture,the three-dimensional(3D)flower-like NiSe_(2)@C composite is delicately designed and assembled with onedimensional nanorods and carbon framework.More importantly,the fundamental mechanism of improved structure stability is unveiled by simulations and experimental results simultaneously.It demonstrates that this designed multidimensional flower-like architecture with dispersed nanorods can balance the structural mismatch,avoid concentrated local strain,and relax the internal stress,mainly induced by the unavoidable volume variation during the repeated conversion processes.Moreover,it can provide more Na^(+)-storage sites and multi-directional migration pathways,leading to a fast Na^(+)-migration channel with boosted reaction kinetic.As expected,it delivers superior rate performance(441 mA h g^(-1)at 5.0 A g^(-1))and long cycling stability(563 mA h g^(-1)at 1.0 A g^(-1)over 1000 cycles)for SIBs.This work provides useful insights for designing high-performance conversion-based anode materials for SIBs.
文摘This paper explores whole-process engineering consulting,including its application models in public buildings and elderly-friendly projects,such as service integration and whole lifecycle management.It also addresses the construction of multi-dimensional collaborative theoretical models,public space streamline organization,and other aspects,emphasizing the importance of multi-dimensional collaboration.Additionally,it highlights the role of talent cultivation and digital transformation in enhancing project efficiency.
基金supported by the basic and forward-looking project(No.2023YQX302)。
文摘Traditional deconvolution methods based on single-channel inversion do not consider the spatial structural relation between channels,and hence,they yield high-resolution results with the existing transverse inconsistency or discontinuity.Therefore,in this study,the local dip angle was used to obtain the structural information and construct the spatial structurally constraint operator.This operator is then introduced into multichannel deconvolution as a regularization operator to improve the resolution and maintain the transverse continuity of seismic data.Model tests and actual seismic data processing have demonstrated the effectiveness and practicability of this method.
文摘The multi-dimensional interactive teaching model significantly enhances the effectiveness of college English instruction by emphasizing dynamic engagement between teachers and students,as well as among students themselves.This paper explores practical strategies for implementing this model,focusing on four key aspects:deepening teachers’understanding of the model through continuous learning,innovating interactive methods such as questioning techniques and practical activities,leveraging modern technology to integrate resources and track learning progress,and establishing a communication platform that centers on student participation.By adopting these approaches,the model fosters a student-centered classroom environment,improves comprehensive English application skills,and optimizes overall teaching quality.
基金Sponsored by the Quality Engineering Project of Education Department of Anhui Province(2022jyxm671)Research Team Project of Anhui Xinhua University(kytd202202)+1 种基金Key Project of Scientific Research(Natural Science)of Higher Education Institutions in Anhui Province(2022AH051861)Teaching Reform Research and Practice Quality Engineering Project of Anhui Xinhua University(2024jy035).
文摘During the critical transformation period of landscape architecture major after the adjustment of disciplinary structure and the changes in market demand,private colleges and universities,as important places for cultivating local talents,have pain points such as uneven quality of teachers and students and weak innovation and practice.The practice system with“multi-dimensional Integration”integrates four dimensions:interdisciplinary integration,spatial and temporal intersection,historical inheritance,and behavioral activity,deepens the disciplinary connotation,and integrates the three elements of nature,humanity,and technology,aiming to provide a new path for private colleges and universities to cultivate application-oriented and compound talents with innovative capabilities.In terms of optimizing talent cultivation and adapting to industry changes,this system provides thinking and reference for landscape architecture major,helping the major reshape its core competitiveness and promoting educational innovation and industry development.
基金supported by the National Natural Science Foundation of China(72101025,72271049),the Interdisciplinary Research Project for Young Teachers of USTB(Fundamental Research Funds for the Central Universities,FRF-IDRY-24-024)the Hebei Natural Science Foundation(F2023501011)+1 种基金the Fundamental Research Funds for the Central Universities(FRF-TP-20-073A1)the R&D Program of Beijing Municipal Education Commission(KM202411232015).
文摘This paper proposes a reliability evaluation model for a multi-dimensional network system,which has potential to be applied to the internet of things or other practical networks.A multi-dimensional network system with one source element and multiple sink elements is considered first.Each element can con-nect with other elements within a stochastic connection ranges.The system is regarded as successful as long as the source ele-ment remains connected with all sink elements.An importance measure is proposed to evaluate the performance of non-source elements.Furthermore,to calculate the system reliability and the element importance measure,a multi-valued decision diagram based approach is structured and its complexity is analyzed.Finally,a numerical example about the signal transfer station system is illustrated to analyze the system reliability and the ele-ment importance measure.
基金supported by the National Key R&D Program of China(No.2021YFC2103600)the National Natural Science Foundation of China(Nos.21878156,21978131,22275085,and 22278224)+2 种基金the Natural Science Foundation of Jiangsu Province(Nos.BK20200089 and BK20200691)the Project of Priority Academic Program Development of Jiangsu Higher Education Institutions(PAPD)the State Key Laboratory of Materials-Oriented Chemical Engineering(No.KL21-08).
文摘Constructing multi-dimensional hydrogen bond(H-bond)regulated single-molecule systems with multiemission remains a challenge.Herein,we report the design of a new excited-state intramolecular proton transfer(ESIPT)featured chromophore(HBT-DPI)that shows flexible emission tunability via the multidimensional regulation of intra-and intermolecular H-bonds.The feature of switchable intramolecular Hbonds is induced via incorporating several hydrogen bond acceptors and donors into one single HBT-DPI molecule,allowing the“turn on/off”of ESIPT process by forming isomers with distinct intramolecular Hbonds configurations.In response to different external H-bonding environments,the obtained four types of crystal/cocrystals vary in the contents of isomers and the molecular packing modes,which are mainly guided by the intermolecular H-bonds,exhibiting non-emissive features or emissions ranging from green to orange.Utilizing the feature of intermolecular H-bond guided molecular packing,we demonstrate the utility of this fluorescent material for visualizing hydrophobic/hydrophilic areas on large-scale heterogeneous surfaces of modified poly(1,1-difluoroethylene)(PVDF)membranes and quantitatively estimating the surface hydrophobicity,providing a new approach for hydrophobicity/hydrophilicity monitoring and measurement.Overall,this study represents a new design strategy for constructing multi-dimensional hydrogen bond regulated ESIPT-based fluorescent materials that enable multiple emissions and unique applications.
基金Project supported by the National Natural Science Foundation of China(Nos.U2441202,12372043,and 12372022)the Fundamental Research Funds for Central Universities。
文摘To break the limitations of the multi-dimensional(M-D)vibration isolation(VI)platforms with the Stewart-Gough design,such as strongly coupling motions,excessive friction in connections,heavy weight,and limited workspace,this study processes a novel platform integrated by a stiffness-adjustable origami spring sub-structure and a parallel mechanism.The origami-based stiffness-adjustable spring realizes low-frequency VI,and the parallel mechanism symmetry design realizes motions decoupling.In the origami-based sub-leg,the parallel-stack-assembly(PSA)design mechanism with two Miura origami configurations is proposed to generate a symmetrical negative stiffness property.Paired with a linear positive stiffness spring,the origami-based sub-leg has wide-amplitude-high-static-low-dynamic stiffness(WA-HSLDS)characteristics in one direction.Then,with construction of the parallel mechanism connected with origami-based sub-legs,an M-D VI platform is achieved,whose motions in the vertical direction and yaw direction are decoupled with the motions in the other directions.Based on the dynamic model and incremental harmonic balance(IHB)with the arc-length continuation method,appropriate structural parameters in the parallel mechanism part are figured out,and the accurate transmissibility in different directions is defined,which gives the parametric influencing investigations for realization of low-frequency VI performances.Finally,experiments are conducted to validate the accuracy and feasibility of the theoretical methods,and to demonstrate the performance of M-D low-frequency isolation with load-carrying capacity of the proposed VI platform.The integration of the origami into the parallel mechanism results in a compact,efficient,and flexible platform with nonlinear adjustability,offering new possibilities for lightweight M-D VI,and developing the practical applications in high-precision platforms in ocean and aerospace environments.
基金With the support of the key project of Knowledge Innovation, CAS(KZCX1-y01, KZCX-SW-18), Fund of the China National Natural Sciences and the Daqing Oilfield with Grant No. 49894190
文摘In seismic data processing, blind deconvolution is a key technology. Introduced in this paper is a flow of one kind of blind deconvolution. The optimal precondition conjugate gradients (PCG) in Kyrlov subspace is also used to improve the stability of the algorithm. The computation amount is greatly decreased.
基金financially supported by the National Science and Technology Major Project of China(No.2011ZX05023-005-005)the National Natural Science Foundation of China(No.41274137)
文摘The conventional nonstationary convolutional model assumes that the seismic signal is recorded at normal incidence. Raw shot gathers are far from this assumption because of the effects of offsets. Because of such problems, we propose a novel prestack nonstationary deconvolution approach. We introduce the radial trace （RT） transform to the nonstationary deconvolution, we estimate the nonstationary deconvolution factor with hyperbolic smoothing based on variable-step sampling （VSS） in the RT domain, and we obtain the high-resolution prestack nonstationary deconvolution data. The RT transform maps the shot record from the offset and traveltime coordinates to those of apparent velocity and traveltime. The ray paths of the traces in the RT better satisfy the assumptions of the convolutional model. The proposed method combines the advantages of stationary deconvolution and inverse Q filtering, without prior information for Q. The nonstationary deconvolution in the RT domain is more suitable than that in the space-time （XT） domain for prestack data because it is the generalized extension of normal incidence. Tests with synthetic and real data demonstrate that the proposed method is more effective in compensating for large-offset and deep data.
基金funded by the National Basic Research Program of China(973 Program)(Grant No.2011CB201100)Major Program of the National Natural Science Foundation of China(Grant No.2011ZX05004003)
文摘The Robinson convolution model is mainly restricted by three inappropriate assumptions, i.e., statistically white reflectivity, minimum-phase wavelet, and stationarity. Modern reflectivity inversion methods（e.g., sparsity-constrained deconvolution） generally attempt to suppress the problems associated with the first two assumptions but often ignore that seismic traces are nonstationary signals, which undermines the basic assumption of unchanging wavelet in reflectivity inversion. Through tests on reflectivity series, we confirm the effects of nonstationarity on reflectivity estimation and the loss of significant information, especially in deep layers. To overcome the problems caused by nonstationarity, we propose a nonstationary convolutional model, and then use the attenuation curve in log spectra to detect and correct the influences of nonstationarity. We use Gabor deconvolution to handle nonstationarity and sparsity-constrained deconvolution to separating reflectivity and wavelet. The combination of the two deconvolution methods effectively handles nonstationarity and greatly reduces the problems associated with the unreasonable assumptions regarding reflectivity and wavelet. Using marine seismic data, we show that correcting nonstationarity helps recover subtle reflectivity information and enhances the characterization of details with respect to the geological record.
基金supported by the Major Basic Research Development Program of China (973 Program)(No.2013CB228606)the National Science foundation of China (No.41174117)+1 种基金the National Major Science-Technology Project (No.2011ZX05031-001)Innovation Fund of PetroChina (No.2010D-5006-0301)
文摘Sparsity constrained deconvolution can improve the resolution of band-limited seismic data compared to conventional deconvolution. However, such deconvolution methods result in nonunique solutions and suppress weak reflections. The Cauchy function, modified Cauchy function, and Huber function are commonly used constraint criteria in sparse deconvolution. We used numerical experiments to analyze the ability of sparsity constrained deconvolution to restore reflectivity sequences and protect weak reflections under different constraint criteria. The experimental results demonstrate that the performance of sparsity constrained deconvolution depends on the agreement between the constraint criteria and the probability distribution of the reflectivity sequences; furthermore, the modified Cauchy- constrained criterion protects the weak reflections better than the other criteria. Based on the model experiments, the probability distribution of the reflectivity sequences of carbonate and clastic formations is statistically analyzed by using well-logging data and then the modified Cauchy-constrained deconvolution is applied to real seismic data much improving the resolution.
基金National 863 Foundation of China(No.2006AA09A102-10)National Natural Science Foundation of China(No.40874056)NCET Fund
文摘The predictive deconvolution algorithm （PD）, which is based on second-order statistics, assumes that the primaries and the multiples are implicitly orthogonal. However, the seismic data usually do not satisfy this assumption in practice. Since the seismic data （primaries and multiples） have a non-Gaussian distribution, in this paper we present an improved predictive deconvolution algorithm （IPD） by maximizing the non-Gaussianity of the recovered primaries. Applications of the IPD method on synthetic and real seismic datasets show that the proposed method obtains promising results.
文摘The study constructed a multi-dimensional feedback mode integrating teacher feedback, peer feedback and network feedback, and applied it in the teaching of College English Writing. After 16 weeks of teaching, the students in the multi-dimen-sional feedback class had significantly better overall writing scores than those in the teacher-feedback class. In terms of individual scores, multi-dimensional feedback played a better role in improving vocabulary and grammar than the class using teacher feed-back. However, there were no significant differences in the responses of writing tasks, coherence and cohesion. The study showed that most students were satisfied with the mode, believing that it was helpful to relieve writing anxiety, stimulate writing interest and improve their writing level.
