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Enhancing sensitivity,selectivity,and intelligence of gas detection based on field-effect transistors:Principle,process,and materials
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作者 Rabia Sultana Song Wang +6 位作者 Misbah Sehar Abbasi Kamran Ahmad Shah Muhammad Mubeen Luxi Yang Qiyu Zhang Zepeng Li Yinghui Han 《Journal of Environmental Sciences》 2025年第8期174-199,共26页
A sensor,serving as a transducer,produces a quantifiable output in response to a predetermined input stimulus,which may be of a chemical or physical nature.The field of gas detection has experienced a substantial surg... A sensor,serving as a transducer,produces a quantifiable output in response to a predetermined input stimulus,which may be of a chemical or physical nature.The field of gas detection has experienced a substantial surge in research activity,attributable to the diverse functionalities and enhanced accessibility of advanced active materials.In this work,recent advances in gas sensors,specifically those utilizing Field Effect Transistors(FETs),are summarized,including device configurations,response characteristics,sensor materials,and application domains.In pursuing high-performance artificial olfactory systems,the evolution of FET gas sensors necessitates their synchronization with material advancements.These materials should have large surface areas to enhance gas adsorption,efficient conversion of gas input to detectable signals,and strong mechanical qualities.The exploration of gas-sensitive materials has covered diverse categories,such as organic semiconductor polymers,conductive organic compounds and polymers,metal oxides,metal-organic frameworks,and low-dimensional materials.The application of gas sensing technology holds significant promise in domains such as industrial safety,environmental monitoring,and medical diagnostics.This comprehensive review thoroughly examines recent progress,identifies prevailing technical challenges,and outlines prospects for gas detection technology utilizing field effect transistors.The primary aim is to provide a valuable reference for driving the development of the next generation of gas-sensitive monitoring and detection systems characterized by improved sensitivity,selectivity,and intelligence. 展开更多
关键词 gas detection Field Effect Transistor(FET)gas sensors Adsorption gas sensitivematerials Applications Technical advancements
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Preparation of(111)-Orientation NiO Epitaxial Films and their High Selectivity for H_(2)S Gas Detection
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作者 Lingling Kuang Tao Xiang +10 位作者 Jiangxiao Li Siyu Wu Yongqi Dong Qingyu He Jiawei Xue Xinyan Chen Yajun Tao Yuting Wang Han Jin Jianxin Yi Zhenlin Luo 《Chinese Journal of Chemical Physics》 2025年第3期272-280,I0011-I0013,I0108,共13页
Nickel oxide(NiO)based gas sensors have at-tracted intense attention due to its high re-sponse to hydrogen sulfide(H_(2)S)gas.It has been demonstrated that the NiO sensors with exposed(111)facet exhibit excellent perf... Nickel oxide(NiO)based gas sensors have at-tracted intense attention due to its high re-sponse to hydrogen sulfide(H_(2)S)gas.It has been demonstrated that the NiO sensors with exposed(111)facet exhibit excellent perfor-mance,but the single-orientation NiO sensors with exposed(111)facet have rarely been studied.In this work,high quality(111)-ori-ented NiO epitaxial films were fabricated by pulsed laser deposition.Detailed crystalline structural information was revealed by using synchrotron based X-ray diffraction(XRD)technology.These NiO thin films show good se-lectivity for H_(2)S gas detection.Without further modification,the highest response to 100 ppm H_(2)S was measured to be 13.07 at 300℃,and limit of detection(LOD)could be as low as 186 ppb.Fitting of the electrical response curves during adsorption and desorption of H_(2)S gas indicates the two-site Langmuir kinetic processes.Combining with XPS and XAS measure-ments,the mechanism was discussed.Density functional theory(DFT)calculations show that NiO with exposed(111)facets has the most negative adsorption energy,indicating more sen-sitive to H_(2)S.These results could inspire more studies of metal oxide semiconductor-based gas sensors with specific surface. 展开更多
关键词 NIO Epitaxial film H_(2)S gas detection gas sensing
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Preparation of CeO_(2)/NiO Ammonia Gas Sensor and Its Application in Breath Detection
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作者 DING Pengfei ZHANG Hongyan +3 位作者 YANG Chen ZHANG Haiyang MA Xiujuan LI Xudong 《新疆大学学报(自然科学版中英文)》 2025年第5期550-560,共11页
A high-performance ammonia(NH3)sensor is prepared based on CeO_(2)/NiO composite,using a hydrothermal method.Experimental findings confirm that the CeO_(2)/NiO composite significantly enhances the performance of the N... A high-performance ammonia(NH3)sensor is prepared based on CeO_(2)/NiO composite,using a hydrothermal method.Experimental findings confirm that the CeO_(2)/NiO composite significantly enhances the performance of the NiO-based NH3 sensor.This improvement is primarily due to the increase in oxygen vacancies(Ov),chemically adsorbed oxygen(Oc),and the proportion of Ni3+on the surface of the CeO_(2)/NiO.The CeO_(2)/NiO sensor shows a high response to NH3,exhibiting response/recovery times of 1.8 s/0.9 s at the NH3 concentration of 5×10^(−6)mL/m^(3),with the theoretical lowest detection limit of 98.651×10^(−9)mL/m^(3).Additionally,the CeO_(2)/NiO sensor has been successfully applied in the simulated detection of Helicobacter pylori infection,highlighting its significant research value and potential application prospects in biomedical diagnostics. 展开更多
关键词 gas sensor NH3 detection CeO_(2)/NiO breath detection
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Multimodal Gas Detection Using E-Nose and Thermal Images:An Approach Utilizing SRGAN and Sparse Autoencoder
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作者 Pratik Jadhav Vuppala Adithya Sairam +5 位作者 Niranjan Bhojane Abhyuday Singh Shilpa Gite Biswajeet Pradhan Mrinal Bachute Abdullah Alamri 《Computers, Materials & Continua》 2025年第5期3493-3517,共25页
Electronic nose and thermal images are effective ways to diagnose the presence of gases in real-time realtime.Multimodal fusion of these modalities can result in the development of highly accurate diagnostic systems.T... Electronic nose and thermal images are effective ways to diagnose the presence of gases in real-time realtime.Multimodal fusion of these modalities can result in the development of highly accurate diagnostic systems.The low-cost thermal imaging software produces low-resolution thermal images in grayscale format,hence necessitating methods for improving the resolution and colorizing the images.The objective of this paper is to develop and train a super-resolution generative adversarial network for improving the resolution of the thermal images,followed by a sparse autoencoder for colorization of thermal images and amultimodal convolutional neural network for gas detection using electronic nose and thermal images.The dataset used comprises 6400 thermal images and electronic nose measurements for four classes.A multimodal Convolutional Neural Network(CNN)comprising an EfficientNetB2 pre-trainedmodel was developed using both early and late feature fusion.The Super Resolution Generative Adversarial Network(SRGAN)model was developed and trained on low and high-resolution thermal images.Asparse autoencoder was trained on the grayscale and colorized thermal images.The SRGAN was trained on lowand high-resolution thermal images,achieving a Structural Similarity Index(SSIM)of 90.28,a Peak Signal-to-Noise Ratio(PSNR)of 68.74,and a Mean Absolute Error(MAE)of 0.066.The autoencoder model produced an MAE of 0.035,a Mean Squared Error(MSE)of 0.006,and a Root Mean Squared Error(RMSE)of 0.0705.The multimodal CNN,trained on these images and electronic nose measurements using both early and late fusion techniques,achieved accuracies of 97.89% and 98.55%,respectively.Hence,the proposed framework can be of great aid for the integration with low-cost software to generate high quality thermal camera images and highly accurate detection of gases in real-time. 展开更多
关键词 Thermal imaging gas detection multimodal learning generative models autoencoders
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Hydrate Blockage in Subsea Oil/Gas Pipelines:Characterization,Detection,and Engineering Solutions
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作者 Yang Meng Bingyue Han +6 位作者 Jiguang Wang Jiawei Chu Haiyuan Yao Jiafei Zhao Lunxiang Zhang Qingping Li Yongchen Song 《Engineering》 2025年第3期363-382,共20页
With the development of offshore oil and gas resources,hydrates pose a significant challenge to flow assurance.Hydrates can form,accumulate,and settle in pipelines,causing blockages,reducing transport capacity,and lea... With the development of offshore oil and gas resources,hydrates pose a significant challenge to flow assurance.Hydrates can form,accumulate,and settle in pipelines,causing blockages,reducing transport capacity,and leading to significant economic losses and fatalities.As oil and gas exploration moves deeper into the ocean,the issue of hydrate blockages has become more severe.It is essential to take adequate measures promptly to mitigate the hazards of hydrate blockages after they form.However,a prerequisite for effective mitigation is accurately detecting the location and amount of hydrate formation.This article summarizes the temperature–pressure,acoustic,electrical,instrumental–response,and flow characteristics of hydrate formation and blocking under various conditions.It also analyzes the principles,limitations,and applicability of various blockage detection methods,including acoustic,transient,and fiber-optic-based methods.Finally,it lists the results of field experiments and commercially used products.Given their advantages of accuracy and a wide detection range,acoustic pulse reflectometry and transient-based methods are considered effective for detecting hydrate blockages in future underwater pipelines.Using strict backpressure warnings combined with accurate detection via acoustic pulse reflectometry or transient-based methods,efficient and timely diagnosis of hydrate blockages can be achieved.The use of a hydrate model combined with fiber optics could prove to be an effective method for detecting blockages in newly laid pipelines in the future. 展开更多
关键词 Oil and gas pipeline Flow assurance Hydrate blockage detection ACOUSTIC TRANSIENT
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Metal-organic framework as a multi-component sensor for detection of Fe^(3+),ascorbic acid and acid phosphatase 被引量:5
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作者 Hao Wang Xiuli Wang +2 位作者 Rong-Mei Kong Lian Xia Fengli Qu 《Chinese Chemical Letters》 SCIE CAS CSCD 2021年第1期198-202,共5页
In this research,a hydroxyl group functionalized metal-organic framework(MOF),UiO-66-(OH)_(2),was synthesized as a "on-off-on" fluore scent switching nanoprobe for highly sensitive and selective detection of... In this research,a hydroxyl group functionalized metal-organic framework(MOF),UiO-66-(OH)_(2),was synthesized as a "on-off-on" fluore scent switching nanoprobe for highly sensitive and selective detection of Fe^(3+),ascorbic acid(AA) and acid phosphatase(ACP).UiO-66-(OH)_(2) emits yellow-green light under ultraviolet light,when Fe^(3+) was added,Fe^(3+) was chelated with hydroxyl group,the electrons in the excited state S_1 of the MOF transferred to the half-filled 3 d orbits of Fe^(3+),resulting in fluorescence quenching because of the nonradiative electron/hole recombination annihilation.AA could reduce Fe^(3+) to Fe^(2+),which can destroy the electron transfer between UiO-66-(OH)_(2) and Fe^(3+) after AA adding,resulted in nonoccurrence of the nonradiative electron transfer,leading to the recovery of UiO-66-(OH)_(2) fluorescence intensity.The probe can also be used to detect ACP based on the enzymolysis of 2-phospho-L-ascorbic acid(AAP) to produce AA.Benefitting from the hydroxyl group and the characteristics of UiO-66,including the high porosity and large surface area,the developed UiO-66-(OH)_(2) showed extensive advantages as a fluorescent probe for detection of multi-component,such as high sensitivity and selectivity,colorimetric detection,fast response kinetics and easy to operate,economical and secure.This is the first time to use active group functionalized MOFs as a multicomponent sensor for these three substances detection. 展开更多
关键词 Metal-organic frameworks Hydroxyl functionalization UiO-66-(OH)_(2) multi-component detection
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Quantitative Detection Model of Pernicious Gases in Pig House Based on BP Neural Network
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作者 俞守华 张洁芳 区晶莹 《Animal Husbandry and Feed Science》 CAS 2009年第3期40-43,48,共5页
To find a neural network model suitable to identify the concentration of mixed pernicious gases in pig house, the quantitative detection model of pernicious gases in pig house was set up based on BP ( Back propagatio... To find a neural network model suitable to identify the concentration of mixed pernicious gases in pig house, the quantitative detection model of pernicious gases in pig house was set up based on BP ( Back propagation) neural network. The BP neural network was trained separately by the three functions, trainbr, traingdm and trainlm, in order to identify the concentration of mixed pernicious gases composed of ammonia gas and hepatic gas. The neural network toolbox in MATLAB software was used to simulate the detection. The results showed that the neural network trained by trainbr function has high average identification accuracy and faster detection speed, and it is also insensitive to noise; therefore, it is suitable to identify the concentration of pemidous gases in pig house. These data provide a reference for intelligent monitoring of pemicious gases in pigsty. 展开更多
关键词 BP neural network pig house -Quantitative detection of gas
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Fretting Wear Behavior of Medium Carbon Steel Modified by Low Temperature Gas Multi-component Thermo-chemical Treatment 被引量:3
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作者 LUO Jun ZHENG Jianfeng PENG Jinfang HE Liping ZHU Minhao 《Chinese Journal of Mechanical Engineering》 SCIE EI CAS CSCD 2010年第3期288-296,共9页
The introduction of surface engineering is expected to be an effective strategy against fretting damage. A large number of studies show that the low gas multi-component (such as carbon, nitrogen, sulphur and oxygen, ... The introduction of surface engineering is expected to be an effective strategy against fretting damage. A large number of studies show that the low gas multi-component (such as carbon, nitrogen, sulphur and oxygen, etc) thermo-chemical treatment(LTGMTT) can overcome the brittleness of nitriding process, and upgrade the surface hardness and improve the wear resistance and fatigue properties of the work-pieces significantly. However, there are few reports on the anti-fretting properties of the LTGMTT modified layer up to now, which limits the applications of fretting. So this paper discusses the fretting wear behavior of modified layer on the surface of LZ50 (0.48%C) steel prepared by low temperature gas multi-component thermo-chemical treatment (LTGMTT) technology. The fretting wear tests of the modified layer flat specimens and its substrate (LZ50 steel) against 52100 steel balls with diameter of 40 mm are carried out under normal load of 150 N and displacement amplitudes varied from 2 μm to 40 μm. Characterization of the modified layer and dynamic analyses in combination with microscopic examinations were performed through the means of scanning electron microscope(SEM), optical microscope(OM), X-ray diffraction(XRD) and surface profilometer. The experimental results showed that the modified layer with a total thickness of 60 μm was consisted of three parts, i.e., loose layer, compound layer and diffusion layer. Compared with the substrate, the range of the mixed fretting regime(MFR) of the LTGMTT modified layer diminished, and the slip regime(SR) of the modified layer shifted to the direction of smaller displacement amplitude. The coefficient of friction(COF) of the modified layer was lower than that of the substrate in the initial stage. For the modified layer, the damage in partial slip regime(PSR) was very slight. The fretting wear mechanism of the modified layer both in MFR and SR was abrasive wear and delamination. The modified layer presented better wear resistance than the substrate in PSR and MFR; however, in SR, the wear resistance of the modified layer decreased with the increase of the displacement amplitudes. The experimental results can provide some experimental bases for promoting industrial application of LTGMTT modified layer in anti-fretting wear. 展开更多
关键词 fretting wear fretting regimes low temperature gas multi-component thermo-chemical treatment(LTGMTT) modified layer medium carbon steel
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Predicting gas-bearing distribution using DNN based on multi-component seismic data: Quality evaluation using structural and fracture factors 被引量:4
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作者 Kai Zhang Nian-Tian Lin +3 位作者 Jiu-Qiang Yang Zhi-Wei Jin Gui-Hua Li Ren-Wei Ding 《Petroleum Science》 SCIE CAS CSCD 2022年第4期1566-1581,共16页
The tight-fractured gas reservoir of the Upper Triassic Xujiahe Formation in the Western Sichuan Depression has low porosity and permeability. This study presents a DNN-based method for identifying gas-bearing strata ... The tight-fractured gas reservoir of the Upper Triassic Xujiahe Formation in the Western Sichuan Depression has low porosity and permeability. This study presents a DNN-based method for identifying gas-bearing strata in tight sandstone. First, multi-component composite seismic attributes are obtained.The strong nonlinear relationships between multi-component composite attributes and gas-bearing reservoirs can be constrained through a DNN. Therefore, we identify and predict the gas-bearing strata using a DNN. Then, sample data are fed into the DNN for training and testing. After optimized network parameters are determined by the performance curves and empirical formulas, the best deep learning gas-bearing prediction model is determined. The composite seismic attributes can then be fed into the model to extrapolate the hydrocarbon-bearing characteristics from known drilling areas to the entire region for predicting the gas reservoir distribution. Finally, we assess the proposed method in terms of the structure and fracture characteristics and predict favorable exploration areas for identifying gas reservoirs. 展开更多
关键词 multi-component seismic exploration Tight sandstone gas reservoir prediction Deep neural network(DNN) Reservoir quality evaluation Fracture prediction Structural characteristics
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Wide dynamic detection range of methane gas based on enhanced cavity absorption spectroscopy 被引量:2
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作者 Yu Wang Bo-Kun Ding +4 位作者 Kun-Yang Wang Jiao-Xu Mei Ze-Lin Han Tu Tan Xiao-Ming Gao 《Chinese Physics B》 SCIE EI CAS CSCD 2022年第4期244-248,共5页
Integrated cavity output spectroscopy(ICOS) is an effective technique in trace gase detection.The strong absorption due to the long optical path of this method makes it challenging in the application scenes that have ... Integrated cavity output spectroscopy(ICOS) is an effective technique in trace gase detection.The strong absorption due to the long optical path of this method makes it challenging in the application scenes that have large gas concentration fluctuation,especially when the gas concentration is high.In this paper,we demonstrate an extension of the dynamic range of ICOS by using a detuned laser combined with an off-axis integrating cavity.With this,we improve the upper limit of the dynamic detection range from 0.1%(1000 ppm) to 20% of the gas concentration.This method provides a way of using ICOS in the applications with unpredictable gas concentrations such as gas leak detection,ocean acidification,carbon sequestration,etc. 展开更多
关键词 integrated cavity output spectroscopy(ICOS) trace gas wide dynamic detection absorption positions
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A visible-light-assisted Pd/TiO_(2)gas sensor with carbon nanotubes electrodes for trace formaldehyde detection 被引量:2
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作者 Can Liu Qiao-Qiao Zou +1 位作者 Bin Liu Yong Zhang 《Rare Metals》 SCIE EI CAS CSCD 2024年第1期257-266,共10页
Owing to the ppb-level detection standard toward the toxic and harmful gas,the detection of trace gases has become an important subject in the field of indoor environment management.However,the traditional resistive g... Owing to the ppb-level detection standard toward the toxic and harmful gas,the detection of trace gases has become an important subject in the field of indoor environment management.However,the traditional resistive gas sensors hardly meet the requirement due to the weak signal generated by trace gas molecules that are difficult to capture.Herein,a visible-light-assisted Pd/TiO_(2)gas sensor is proposed to endow the effective detection of trace formaldehyde(HCHO)gas without heating temperature.Benefiting from the enhanced photocatalytic properties of TiO_(2)by Pd decoration,the visible-light-assisted Pd/TiO_(2)gas sensor can detect the HCHO gas as low as80×10^(–9)at room temperature.The successful preparation of nanoscale TiO_(2)sensing layer is facilitated by the ultrathin carbon nanotube interdigital electrode in the gas sensor,which avoids the discontinuity of the sensing layer caused by the excessive thickness of the traditional metal electrode.In addition,the whole preparation process of the Pd/TiO_(2)gas sensor with carbon nanotube electrodes is compatible with mainstream CMOS fabrication technology,which is expected to realize the batch fabrication and micro-integrated application of gas sensors.It is expected that our work can provide a new strategy for the batch preparation of high-performance trace HCHO gas sensors and their future applications in portable electronic devices such as smartphones. 展开更多
关键词 Visible-light-assisted gas sensor Pd/TiO_(2) Trace HCHO detection Carbon nanotubes electrodes
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Preparation of polythiophene/WO_3 organic-inorganic hybrids and their gas sensing properties for NO_2 detection at low temperature 被引量:2
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作者 Jing Huan~ Yanfei Kang +2 位作者 Taili Yang Yao Wang Shurong Wang 《Journal of Natural Gas Chemistry》 EI CAS CSCD 2011年第4期403-407,共5页
Polythiophene/WO3(PTP/WO3)organic-inorganic hybrids were synthesized by an in situ chemical oxidative polymerization method,and char- acterized by X-ray diffraction(XRD),transmission electron microscopy(TEM)and ... Polythiophene/WO3(PTP/WO3)organic-inorganic hybrids were synthesized by an in situ chemical oxidative polymerization method,and char- acterized by X-ray diffraction(XRD),transmission electron microscopy(TEM)and thermo-gravimetric analysis(TGA).The Polythiophene/ WO3 hybrids have higher thermal stability than pure polythiophene,which is beneficial to potential application as chemical sensors.Gas sensing measurements demonstrate that the gas sensor based on the Polythiophene/WO3 hybrids has high response and good selectivity for de- tecting NO2 of ppm level at low temperature.Both the operating temperature and PTP contents have an influence on the response of PTP/WO3 hybrids to NO2.The 10 wt%PTP/WO3 hybrid showed the highest response at low operating temperature of 70-C.It is expected that the PTP/WO3 hybrids can be potentially used as gas sensor material for detecting the low concentration of NO2 at low temperature. 展开更多
关键词 polythiophene/WO3 organic-inorganic hybrids gas sensing properties NO2 detection low temperature
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MOF/Polymer-Integrated Multi-Hotspot Mid-Infrared Nanoantennas for Sensitive Detection of CO_(2) Gas 被引量:1
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作者 Hong Zhou Zhihao Ren +2 位作者 Cheng Xu Liangge Xu Chengkuo Lee 《Nano-Micro Letters》 SCIE EI CAS CSCD 2022年第12期352-372,共21页
Metal-organic frameworks(MOFs)have been extensively used for gas sorption,storage and separation owing to ultrahigh porosity,exceptional thermal stability,and wide structural diversity.However,when it comes to ultra-l... Metal-organic frameworks(MOFs)have been extensively used for gas sorption,storage and separation owing to ultrahigh porosity,exceptional thermal stability,and wide structural diversity.However,when it comes to ultra-low concentration gas detection,technical bottlenecks of MOFs appear due to the poor adsorption capacity at ppm-/ppblevel concentration and the limited sensitivity for signal transduction.Here,we present hybrid MOF-polymer physi-chemisorption mechanisms integrated with infrared(IR)nanoantennas for highly selective and ultrasensitive CO_(2) detection.To improve the adsorption capacity for trace amounts of gas molecules,MOFs are decorated with amino groups to introduce the chemisorption while maintaining the structural integrity for physisorption.Additionally,leveraging all major optimization methods,a multi-hotspot strategy is proposed to improve the sensitivity of nanoantennas by enhancing the near field and engineering the radiative and absorptive loss.As a benefit,we demonstrate the competitive advantages of our strategy against the state-of-the-art miniaturized IR CO_(2) sensors,including low detection limit,high sensitivity(0.18%/ppm),excellent reversibility(variation within 2%),and high selectivity(against C_(2)H_(5)OH,CH_(3)OH,N_(2)).This work provides valuable insights into the integration of advanced porous materials and nanophotonic devices,which can be further adopted in ultra-low concentration gas monitoring in industry and environmental applications. 展开更多
关键词 Metal-organic framework gas detection Mid-infrared nanoantennas Multi-hotspot Loss engineering
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Gas concentration monitoring system for small and medium-sized coal mines based on gas-sensing detection and single-chip control 被引量:1
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作者 Bin Guangfu Huang Zhenyu +1 位作者 Zhu Guanghui Li Xuejun 《Engineering Sciences》 EI 2010年第4期47-51,共5页
This paper is aimed at the actual conditions of disaster caused by gas in small and medium-sized coal mines. A new gas concentration monitoring system for coal mines is developed on the basis of gas-sensing detection ... This paper is aimed at the actual conditions of disaster caused by gas in small and medium-sized coal mines. A new gas concentration monitoring system for coal mines is developed on the basis of gas-sensing detection and single-chip control. The monitoring system uses the tin oxide as the main material of N-type semiconductor gas sensors, be- cause it has good sensitive characteristics for the flammable and explosive gas ( such as methane, carbon monoxide). The QM-N5-semiconductor gas sensor is adopted to detect the output values of the resistance under the different gas con- centrations. The system, designedly, takes the AT89C51 digital chip as the core of the circuit processing hardware structure to analyze and judge the input values of the resistance, and then achieve the control and alarm for going beyond the limit of gas concentration. The gas concentration monitoring system has man), advantages including simple in struc- ture, fast response time, stable performance and low cost. Thus, it can be widely used to monitor gas concentration and provide early wamings in small and medium-sized coal mines. 展开更多
关键词 gas concentration monitoring gas-sensing detection single-chip control small and medium-sized coal
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A Novel Method of Detecting Methanol in Transformer Oil Based on Methanol Gas Sensor With Solid-Phase Extraction Technology
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作者 Song Cheng Guokai Huang +2 位作者 Liang Zhang Wei Sun Qingguo Chen 《High Voltage》 2025年第5期1293-1301,共9页
As a novel chemical marker,methanol has been widely applied to evaluate the ageing state of insulating paper in recent years.Methanol gas sensor(MGS)could be applied to detect the methanol content in transformer oil f... As a novel chemical marker,methanol has been widely applied to evaluate the ageing state of insulating paper in recent years.Methanol gas sensor(MGS)could be applied to detect the methanol content in transformer oil for its high portability and stability.However,it has the defects of a high limit of detection(LOD)and poor anti-interference performance.Therefore,a novel method of detecting methanol in transformer oil based on MGS with the solid-phase extraction(SPE)technology was investigated in this paper.A detection platform for methanol in transformer oil based on SPE was established,and the SPE experimental process and the crucial parameters were optimised.The results show that the SPE decreased the LOD of MGS from 0.4 to 0.2 ppm and effectively eliminated the interfering substances in oil.Although a part of methanol would be lost during the SPE process,the regression correction coefficient was proposed to correct the evaluation errors.The results indicate that the average relative errors decreased from 17.09%to 4.38%,and the proposed method has good applicability. 展开更多
关键词 insulating paper chemical markermethanol evaluate ageing state gas sensor mgs could transformer oil METHANOL detecting methanol gas sensor
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Development of a ceramic gas-electron-multiplier neutron detector prototype with a large sensitive area
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作者 Lin Zhu Jianrong Zhou +13 位作者 Xiaojuan Zhou Lixin Zeng Liang Xiao Hong Xu Fei Jia Chaoyue Zhang Yezhao Yang Dingfu Li Hao Xiong Yuguang Xie Yubin Zhao Yadong Wei Zhijia Sun Yuanbo Chen 《Chinese Physics B》 2025年第9期135-141,共7页
The rapid growth of neutron flux has driven the development of^(3)He-free neutron detectors to satisfy the requirements of the neutron scattering instruments under construction or planned at the China Spallation Neutr... The rapid growth of neutron flux has driven the development of^(3)He-free neutron detectors to satisfy the requirements of the neutron scattering instruments under construction or planned at the China Spallation Neutron Source(CSNS).Position-sensitive neutron detectors with a high counting rate and large area play an important role in the instruments performing neutron measurements in or close to the direct beam.The ceramic gas-electron-multiplier(GEM)detector serves as a promising solution,and considerable work has been done using the small-area GEM neutron detectors.In this article,we designed and constructed a detector prototype utilizing ceramic GEM foils with an effective area of about307 mm×307 mm.To evaluate and investigate their basic characteristics,the Monte Carlo(MC)tool FLUKA was employed and several neutron beam tests were conducted at CSNS.The simulated spatial resolution was basically in agreement with the measured value of 2.50±0.01 mm(FWHM).The wavelength spectra measurement was verified through comparisons with a commercial beam monitor.In addition,a detection efficiency of 4.7±0.1%was achieved for monoenergetic neutrons of 1.59 A wavelength.This is consistent with the simulated result.The results indicate that the large-area ceramic GEM detector is a good candidate to implement neutron beam measurements.Its efficiency can be improved in a cascading manner to approach that reached by traditional^(3)He detectors. 展开更多
关键词 neutron detector counting rate gas electron multiplier spatial resolution detection efficiency
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Specific Sn–O–Fe Active Sites from Atomically Sn‑Doping Porous Fe_(2)O_(3)for Ultrasensitive NO_(2)Detection
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作者 Yihong Zhong Guotao Yuan +8 位作者 Dequan Bao Yi Tao Zhenqiu Gao Wei Zhao Shuo Li Yuting Yang Pingping Zhang Hao Zhang Xuhui Sun 《Nano-Micro Letters》 2025年第11期362-375,共14页
Conventional gas sensing materials(e.g.,metal oxides)suffer from deficient sensitivity and serve cross-sensitivity issues due to the lack of efficient adsorption sites.Herein,the heteroatom atomically doping strategy ... Conventional gas sensing materials(e.g.,metal oxides)suffer from deficient sensitivity and serve cross-sensitivity issues due to the lack of efficient adsorption sites.Herein,the heteroatom atomically doping strategy is demonstrated to significantly enhance the sensing performance of metal oxides-based gas sensing materials.Specifically,the Sn atoms were incorporated into porous Fe_(2)O_(3)in the form of atomically dispersed sites.As revealed by X-ray absorption spectroscopy and atomic-resolution scanning transmission electron microscopy,these Sn atoms successfully occupy the Fe sites in the Fe_(2)O_(3)lattice,forming the unique Sn-O-Fe sites.Compared to Fe-O-Fe sites(from bare Fe_(2)O_(3))and Sn-O-Sn sites(from SnO_(2)/Fe_(2)O_(3)with high Sn loading),the Sn-O-Fe sites on porous Fe_(2)O_(3)exhibit a superior sensitivity(Rg/Ra=2646.6)to 1 ppm NO_(2),along with dramatically increased selectivity and ultra-low limits of detection(10 ppb).Further theoretical calculations suggest that the strong adsorption of NO_(2)on Sn-O-Fe sites(N atom on Sn site,O atom on Fe site)contributes a more efficient gas response,compared to NO_(2)on Fe-O-Fe sites and other gases on Sn-O-Fe sites.Moreover,the incorporated Sn atoms reduce the bandgap of Fe_(2)O_(3),not only facilitating the electron release but also increasing the NO_(2)adsorption at a low working temperature(150°C).This work introduces an effective strategy to construct effective adsorption sites that show a unique response to specific gas molecules,potentially promoting the rational design of atomically modified gas sensing materials with high sensitivity and high selectivity. 展开更多
关键词 Atomically doping Specific Sn-O-Fe sites NO_(2)detection gas sensor Specific adsorption
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Application of multi-component joint inversion in oil and gas exploration:A case study of reservoir and gas saturation prediction of the Xujiahe formation in the PLN area of the central Sichuan Basin
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作者 Wang Dong He Zhen-Hua +4 位作者 Wang Xu-Ben Li Le Yang Hai-Tao Fu Zhi-Guo Wang Hong-Yan 《Applied Geophysics》 SCIE CSCD 2020年第5期879-889,905,共12页
Multi-component seismic exploration is an important technique in the utilization of P-waves and converted S-waves for oil and gas exploration.It has unique advantages in the structural imaging of gas zones,reservoir p... Multi-component seismic exploration is an important technique in the utilization of P-waves and converted S-waves for oil and gas exploration.It has unique advantages in the structural imaging of gas zones,reservoir prediction,lithology,and gas-water identifi cation,and the development direction and degree of fractures.Multi-component joint inversion is one of the most important steps in multi-component exploration.In this paper,starting from the basic principle of multi-component joint inversion,the diff erences between the method and single P-wave inversion are introduced.Next,the technique is applied to the PLN area of the Sichuan Basin,and the P-wave impedance,S-wave impedance,and density are obtained based on multi-component joint inversion.Through the velocity and lithology,porosity,and gas saturation fi tting formulas,prediction results are calculated,and the results are analyzed.Finally,multi-component joint inversion and single P-wave inversion are compared in eff ective reservoir prediction.The results show that multi-component joint inversion increases the constraints on the inversion conditions,reduces the multi-solution of a single P-wave inversion,and is more objective and reliable for the identification of reservoirs,effectively improving the accuracy of oil and gas reservoir prediction and development. 展开更多
关键词 multi-component joint inversion lithology identifi cation POROSITY gas saturation reservoir prediction
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Hydrocarbon detections using multi-attributes based quantum neural networks in a tight sandstone gas reservoir in the Sichuan Basin, China 被引量:1
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作者 Ya-juan Xue Xing-jian Wang +1 位作者 Jun-xing Cao Xiao-Fang Liao 《Artificial Intelligence in Geosciences》 2021年第1期107-114,共8页
A direct hydrocarbon detection is performed by using multi-attributes based quantum neural networks with gas fields.The proposed multi-attributes based quantum neural networks for hydrocarbon detection use data cluste... A direct hydrocarbon detection is performed by using multi-attributes based quantum neural networks with gas fields.The proposed multi-attributes based quantum neural networks for hydrocarbon detection use data clustering and local wave decomposition based seismic attenuation characteristics,relative wave impedance features of prestack seismic data as the selected multiple attributes for one tight sandstone gas reservoir and further employ principal component analysis combined with quantum neural networks for giving the distinguishing results of the weak responses of the gas reservoir,which is hard to detect by using the conventional technologies.For the seismic data from a tight sandstone gas reservoir in the Sichuan basin,China,we found that multiattributes based quantum neural networks can effectively capture the weak seismic responses features associated with gas saturation in the gas reservoir.This study is hoped to be useful as an aid for hydrocarbon detections for the gas reservoir with the characteristics of the weak seismic responses by the complement of the multiattributes based quantum neural networks. 展开更多
关键词 Hydrocarbon detection Multi-attributes Quantum neural networks Tight sandstone gas reservoir Weak seismic responses
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