Developing an accurate and visual sensing strategy for trace levels of fluoroquinolone residues that pose threat to food safety and human health is highly desired but remains challenging.Herein,a target selfcalibratio...Developing an accurate and visual sensing strategy for trace levels of fluoroquinolone residues that pose threat to food safety and human health is highly desired but remains challenging.Herein,a target selfcalibration ratiometric fluorescent sensing platform has been designed for sensitive visual detection of levofloxacin(LEV)based on fluorescent europium metal-organic framework(Eu-MOF)probe.Specifically,the Eu-MOF was facilely synthesized via directly mixing Eu^(3+)with 1,10-phenanthroline-2,9-dicarboxylic acid(PDA)ligand at room temperature,which exhibited well-stable red fluorescence at 612 nm.Upon the addition of target LEV,the significant fluorescence quenching from Eu^(3+)was observed owing to the inner filter effect between the Eu-MOF and LEV.While the intrinsic fluorescence for LEV at 462nm was gradually enhanced,thereby realizing the self-calibration ratiometric fluorescence responses to LEV.Through this strategy,LEV can be detected down to 27 nmol/L.Furthermore,a test paper-based Eu-MOF integrated with the smartphone assisted RGB color analysis was exploited for the quantitative monitoring of LEV through the multi-color changes from red to blue,thus achieved portable,convenient and visual detection of LEV in honey and milk samples.Therefore,the developed strategy could provide a useful tool for supporting the practical on-site test in food samples.展开更多
This work addresses the cut order planning(COP)problem for multi-color garment production,which is the first step in the clothing industry.First,a multi-objective optimization model of multicolor COP(MCOP)is establish...This work addresses the cut order planning(COP)problem for multi-color garment production,which is the first step in the clothing industry.First,a multi-objective optimization model of multicolor COP(MCOP)is established with production error and production cost as optimization objectives,combined with constraints such as the number of equipment and the number of layers.Second,a decoupled multi-objective optimization algorithm(DMOA)is proposed based on the linear programming decoupling strategy and non-dominated sorting in genetic algorithmsⅡ(NSGAII).The size-combination matrix and the fabric-layer matrix are decoupled to improve the accuracy of the algorithm.Meanwhile,an improved NSGAII algorithm is designed to obtain the optimal Pareto solution to the MCOP problem,thereby constructing a practical intelligent production optimization algorithm.Finally,the effectiveness and superiority of the proposed DMOA are verified through practical cases and comparative experiments,which can effectively optimize the production process for garment enterprises.展开更多
Conventional color-printing systems often use inks of three hues, such as CMY, CMYK and CMYKLcLm, but in order to obtain more realistic color reproductions, the ink set of more than three hues has been adopted by some...Conventional color-printing systems often use inks of three hues, such as CMY, CMYK and CMYKLcLm, but in order to obtain more realistic color reproductions, the ink set of more than three hues has been adopted by some color-printing systems. It is difficult, however, to model the composed color with the multiple inks when the number of the output ink hues exceeds three due to the none-unique mapping between the color spaces of the CIE Lab and the multi-color printing device. In this paper, we propose a fine color-printing method for multi-color printing device with the ink set of more than three hues. The proposed approach has good color expression ability and provides fine control of the printed color. By dividing the output color space into several subspaces, our method allows one-to-one mapping between the standard color space and the multi-color output color space. It has been proved effective when applied to the digital inkjet printer—Mutoh8000.展开更多
We study theoretically intense terahertz radiation from multi-color laser pulse with uncommon frequency ratios. Com- paring the two-color laser scheme, of which the uncommon frequency ratio should be set to be a speci...We study theoretically intense terahertz radiation from multi-color laser pulse with uncommon frequency ratios. Com- paring the two-color laser scheme, of which the uncommon frequency ratio should be set to be a specific value, we show that by using multi-color harmonic laser pulses as the first pump component, the lasers as the second pump component can be adjusted in a continuous frequency range. Moreover, these multi-color laser pulses can effectively modulate and enhance the terahertz radiation, and the terahertz yield increases with the increase of the wavelength of the uncommon pump com- ponent and is stable to the laser relative phase. Finally, we utilize the electron densities and velocities of ionization events to illustrate the physical mechanism of the intense terahertz generation.展开更多
Multi-color luminescence basing on amorphous Eu^3＋/Tb^3＋ co-doped Zn-A1 hydroxides and their annealed samples were studied in detail. Results suggest that excellent red emissions due to E^u3＋ and green emissions at...Multi-color luminescence basing on amorphous Eu^3＋/Tb^3＋ co-doped Zn-A1 hydroxides and their annealed samples were studied in detail. Results suggest that excellent red emissions due to E^u3＋ and green emissions attributed to Tb^3＋ appear under the excitation of favorable wavelength for all the as- prepared amorphous samples. Moreover, the emission intensity depends on the Eu^3＋/Tb^3＋ molar ratio. The samples annealed at 300, 500, and 700 ℃ still exhibit amorphous state, and multi-color lumi- nescence kept in the samples annealed at 300 ℃, while luminescence quenched for the samples annealed at 500 and 700 ℃. However, a broad emission ranging from 450 to 650 nm occurs in some samples annealed at 900 ℃. Further, the fluorescence decay and lifetimes for the as-prepared samples and the samples annealed at 300℃ were investigated. It is found that all the decay curves of emissions due to Tb^3＋ and Eu^3＋ present characteristic double exponential function despite their different lifetimes. The present work may be a good example for developing new multi-color even white light emitting materials.展开更多
Manipulating and real-time monitoring of neuronal activities with cell-type specificity and precise spatiotemporal resolution during animal behavior are fundamental technologies for exploring the functional connectivi...Manipulating and real-time monitoring of neuronal activities with cell-type specificity and precise spatiotemporal resolution during animal behavior are fundamental technologies for exploring the functional connectivity, information transmission, and physiological functions of neural circuits in vivo. However, current techniques for optogenetic stimulation and neuronal activity recording mostly operate independently. Here, we report an all-fiber-transmission photometry system for simultaneous optogenetic manipulation and multi-color recording of neuronal activities and the neurotransmitter release in a freely moving animal. We have designed and manufactured a wavelength-independent multi-branch fiber bundle to enable simultaneous optogenetic manipulation and multi-color recording at different wavelengths. Further, we combine a laser of narrow linewidth with the lock-in amplification method to suppress the optogenetic stimulation-induced artifacts and channel crosstalk. We show that the collection efficiency of our system outperforms a traditional epi-fluorescence system. Further, we demonstrate successful recording of dynamic dopamine(DA) responses to unexpected rewards in the nucleus accumbens(NAc) in a freely moving mouse. We also show simultaneous dual-color recording of neuronal Ca2+ signals and DA dynamics in the NAc upon delivering an unexpected reward and the simultaneous optogenetic activating at dopaminergic terminals in the same location. Thus, our multi-function fiber photometry system provides a compatible, efficient, and flexible solution for neuroscientists to study neural circuits and neurological diseases.展开更多
Mechano-luminescence(ML) has been found diverse applications such as stress sensing,3-D signature,energy harvesting,and anti-counterfeiting,due to the unique properties of the corresponding ML phosphors performing in-...Mechano-luminescence(ML) has been found diverse applications such as stress sensing,3-D signature,energy harvesting,and anti-counterfeiting,due to the unique properties of the corresponding ML phosphors performing in-situ and real-time response to mechanical stimulus.Trap-controlled ML materials realize reproducible,quantitative mechano-optical conversion resulting from the released carriers for the trap-mediated charge storage and release.Herein,modulating traps matters the controllable ML behavior for their promising applications.In this work,a deep trap distributed ranging from 0.9 to 1,3 eV is realized consecutively for the introduction of Sm^(3+)ions into LaGaO_(3) matrix,which contributes to the red emission at 600 nm under mechanical stimuli.Moreover,tunable ML emission modulated from 600to 545 nm is successfully achieved for the codopant of Tb^(3+)ions.It is unambiguously indicated that the released carriers from the trap sharing rather than an additional constructed trap contribute to the modulated ML color.Accordingly,multi-mode anti-counterfeiting and encryption are achieved with the as-explored Sm^(3+),Tb^(3+)co-activated ML phosphor.展开更多
BACKGROUND Near-infrared fluorescence imaging via using intravenous indocyanine green(ICG)has a wide range of applications in multiple surgical scenarios.In lapa-roscopic cholecystectomy(LC),it facilitates intraoperat...BACKGROUND Near-infrared fluorescence imaging via using intravenous indocyanine green(ICG)has a wide range of applications in multiple surgical scenarios.In lapa-roscopic cholecystectomy(LC),it facilitates intraoperative identification of the biliary system and reduces the risk of bile duct injury.However,the usual single color fluorescence imaging(SCFI)has limitations in manifesting the fluorescence signal of the target structure when its intensity is relatively low.Moreover,sur-geons often experience visual fatigue.We hypothesized that a novel imaging stra-tegy,named multi-color fluorescence imaging(MCFI),could potentially address these issues by decreasing hepatic and background fluorescence pollution and improving biliary visualization.AIM To investigate the novel imaging strategy MCFI in LC.METHODS This was a single-center retrospective study conducted at Peking Union Medical College Hospital,Beijing,China.Patients who underwent LC from June 2022 to March 2023 by the same surgical team were enrolled.Demographic features,clinical and surgical information were collected.The clarity,visual comfort,and effectiveness of different imaging strategies were subjectively evaluated by surgeons.RESULTS A total of 155 patients were included,60 patients were in the non-ICG group in which only bright light illuminance without ICG was applied,60 patients were in the SCFI group,and 35 patients were in the MCFI group.No statist-ically significant differences were found in demographics or clinical history.Post-surgical complications were minimal in all 3 groups with no significant differences observed.MCFI improved the clarity of imaging and visual comfort.Clarity of imaging and visual comfort were improved with MCFI.CONCLUSION MCFI improves biliary visualization and reduces liver fluorescence contamination,which supports its routine use in LC.MCFI may also be a better choice than SCFI in other clinical settings.展开更多
In an automatic bobbin management system that simultaneously detects bobbin color and residual yarn,a composite texture segmentation and recognition operation based on an odd partial Gabor filter and multi-color space...In an automatic bobbin management system that simultaneously detects bobbin color and residual yarn,a composite texture segmentation and recognition operation based on an odd partial Gabor filter and multi-color space hierarchical clustering are proposed.Firstly,the parameter-optimized odd partial Gabor filter is used to distinguish bobbin and yarn texture,to explore Garbor parameters for yarn bobbins,and to accurately discriminate frequency characteristics of yarns and texture.Secondly,multi-color clustering segmentation using color spaces such as red,green,blue(RGB)and CIELUV(LUV)solves the problems of over-segmentation and segmentation errors,which are caused by the difficulty of accurately representing the complex and variable color information of yarns in a single-color space and the low contrast between the target and background.Finally,the segmented bobbin is combined with the odd partial Gabor’s edge recognition operator to further distinguish bobbin texture from yarn texture and locate the position and size of the residual yarn.Experimental results show that the method is robust in identifying complex texture,damaged and dyed bobbins,and multi-color yarns.Residual yarn identification can distinguish texture features and residual yarns well and it can be transferred to the detection and differentiation of complex texture,which is significantly better than traditional methods.展开更多
For practical large-scale applications of computational fluid dynamics in the aero-space industry,implicit flow solvers are necessitated for efficient simulations.This paper presents the implementation of a solver tha...For practical large-scale applications of computational fluid dynamics in the aero-space industry,implicit flow solvers are necessitated for efficient simulations.This paper presents the implementation of a solver that employs an unstructured finite volume approach and a Multi-Colored Gauss-Seidel(MCGS)method for steady-state compressible flow simulations on a server equipped with multiple Graphics Process-ing Units(GPUs).The mesh partition process is completed with PyMetis,and Mes-sage Passing Interface(MPI)is utilized for communications between mesh partitions.A parallel coloring algorithm is employed in the pre-processing module.The code is developed using a hybrid programming approach,with the main framework writ-ten in Python and the GPU kernel source codes written in C.The transonic turbulent flows over the CHN-T1 transport aircraft model are simulated on unstructured hybrid meshes.The numerical results are compared with experimental data,and the perfor-mance of the developed flow simulation framework is analysed.展开更多
High-resolution organic arrays with diverse pixel types hold significant promise for various applications,such as full-color displays and photonic crystals.The direct growth of such arrays(e.g.,high-resolution multi-c...High-resolution organic arrays with diverse pixel types hold significant promise for various applications,such as full-color displays and photonic crystals.The direct growth of such arrays(e.g.,high-resolution multi-color patterns)cannot be achieved in a single step with conventional strategies.Here,we present a viable approach integrating a bottom-up solution strategy with phase-change materials(PCMs),specifically aggregation-induced emission(AIE)materials.Through intentional self-assembly,color-programmable organic micro-patterns featuring distinct phases or colors were created.Notably,manipulating the amount of involved substance for nucleation/crystallization was achieved by adjusting the sizes of pre-defined nucleation sites.This precise control resulted in varied phases and colors for each pixel.Thus,high-resolution organic micro-arrays with transfer-free multi-color pixels were directly achieved.These may open avenues for seamless,transfer-free growth of multifunctional micro-patterns using PCMs,holding immense potential for applications in high-resolution full-color imaging/displays,photonic crystals,information storage,and encryption,etc.展开更多
Purely organic single-component luminescent materials enabling multi-color photoluminescence are gaining significant interest,given their tunable optical properties,environmental friendliness,and cost-effectiveness.Ho...Purely organic single-component luminescent materials enabling multi-color photoluminescence are gaining significant interest,given their tunable optical properties,environmental friendliness,and cost-effectiveness.However,realizing multi-color electroluminescence from a single-component emitter for application in organic light-emitting diode(OLED)remains challenging,mainly due to the limitations in achieving distinct excited-state conformations in amorphous or solid states.In this study,we report two novel emitters(Bppy-PTZ and Bpph-PTZ)by incorporating a benzophenone acceptor and phenothiazine donor with pyridyl and phenylπ-bridging spacers.The introduction of a pyridine ring in Bppy-PTZ establishes intramolecular hydrogen bonding,stabilizing the quasi-axial(QA)conformation in the amorphous state,thereby facilitating multi-color and white-light emissions in thin-film and OLED devices.Photophysical and theoretical analyses reveal distinct emission behaviors from QA and quasi-equatorial conformations,with Bppy-PTZ exhibiting enhanced dual-emission and mechanochromic properties.Importantly,by adopting single-component Bppy-PTZ,the fabricated OLEDs realize color-tunable emissions,including blue,yellow,and adjustable white lights,reaching maximum external quantum efficiencies of up to 15.5%.This work provides valuable insights for the development of efficient single-component emitters affording multi-color OLEDs with high performances.展开更多
To identify alien chromosomes in recipient progenies and to analyze genome components in polyploidy, a genomic in situ hybridization （GISH） technique that is suitable for cotton was developed using increased stringe...To identify alien chromosomes in recipient progenies and to analyze genome components in polyploidy, a genomic in situ hybridization （GISH） technique that is suitable for cotton was developed using increased stringency conditions. The increased stringency conditions were a combination of the four factors in the following optimized state： 100：1 ratio of blocking DNA to probe, 60% formamide wash solution, 43 ℃ temperature wash and a 13 min wash. Under these specific conditions using gDNA from Gossypium sturtianum （C1 C1 ） as a probe, strong hybridization signals were only observed on chromosomes from the C1 genome in somatic cells of the hybrid F1 （G. hirsutum x G. sturtianum） （AtDtC1）. Therefore, GISH was able to discriminate parental chromosomes in the hybrid. Further, we developed a multi-color GISH to simultaneously discriminate the three genomes of the above hybrid. The results repeatedly displayed the three genomes, At, Dt, and C1, and each set of chromosomes with a unique color, making them easy to identify. The power of the multi-color GISH was proven by analysis of the hexaploid hybrid F1 （G. hirsutum x G. australe） （AtAtDtDtG2G2）. We believe that the powerful multi-color GISH technique could be applied extensively to analyze the genome component in polyploidy and to identify alien chromosomes in the recipient progenies.展开更多
Frequency conversion based on three-wave mixing is a critical nonlinear optic application,extending the frequency range of existing lasers and realizing frequency-transduced detectors in a wavelength range that lacks ...Frequency conversion based on three-wave mixing is a critical nonlinear optic application,extending the frequency range of existing lasers and realizing frequency-transduced detectors in a wavelength range that lacks an effective detector.Phase matching is vital for effective frequency conversion.The advantages of quasi-phase matching(QPM)over birefringent phase matching are a lack of walk-off effect,a maximum nonlinear coefficient,and phase matching in the entire transparency window.Herein,using different types and orders of QPM,four kinds of effective frequency doubling processes are realized in a periodically poled potassium titanyl phosphate(KTP)crystal with a single period,and three kinds of frequency doubling processes are experimentally verified.We also show a feasible way to construct an RGB color generator based on two different QPM processes.This study significantly expands the feasible frequency conversion of existing lasers to different wavelengths,providing an effective method for multi-color laser generation based on periodically poled KTP crystals.展开更多
Carbon dots(CDs)with aggregation-induced emission(AIE)have sparked significant interest in multidimensional anti-counterfeiting due to their exceptional fluorescence properties.However,the preparation of AIE CDs with ...Carbon dots(CDs)with aggregation-induced emission(AIE)have sparked significant interest in multidimensional anti-counterfeiting due to their exceptional fluorescence properties.However,the preparation of AIE CDs with multicolor solid-state fluorescence remains a formidable challenge due to its complicated construction.In the present work,a novel class of multicolor AIE CDs(M-CDs)were fabricated using selected precursor(salicylic acid,thiosalicylic acid,and 2,2'-dithiodibenzoic acid),with an eco-friendly,low-cost one-pot solvothermal method.In the dilute organic solution,M-CDs manifested blue emission,but upon aggregation in the presence of water,the red,yellow,green,and blue emissions were displayed due to the AIE effect.Structural analysis,coupled with theoretical calculations,revealed that the increase in the size of sp2 domains would lower the Eg and cause a red-shift emission wavelength.Significantly,the continuous emission of M-CDs from blue to red can be utilized as ink for multimode printing,enabling the creation of a variety of school badges and quick response codes.These findings hold promising implications for multi-information encryption applications.展开更多
Low-dimensional semiconductor nanostructures have attracted much interest for applications in integrated photonic and optoelectronic devices. Band gap engineering within single semiconductor nanoribbons helps to manip...Low-dimensional semiconductor nanostructures have attracted much interest for applications in integrated photonic and optoelectronic devices. Band gap engineering within single semiconductor nanoribbons helps to manipulate photon behavior in two different cavities （in the width and length directions） and realize new photonic phenomena and applications. In this work, lateral composition-graded semiconductor nanoribbons were grown for the first time through an improved source-moving vapor phase route. Along the width of the nanoribbon, the material can be gradually tuned from pure CdS to a highly Se-doped CdSSe alloy with a corresponding band gap modulation from 2.42 to 1.94 eV. The achieved alloy ribbons are overall high-quality crystals, and the position-dependent band-edge photoluminescence （PL） emission had a peak wavelength continuously tuned from -515 to -640 nm. These ribbons can realize multi-color lasing with three groups of lasing modes centered at 519, 557, and 623 run. It was confirmed that the red lasing was from optical resonance along the length direction, while the green and yellow lasing was from optical resonance along the width direction. These novel nanoribbon structures may be applied to many integrated photonic and optoelectronic devices.展开更多
Nanocarbon as an eco-friendly and abundant material has strong multi-color fluorescence, which makes it a promising candidate for healthy lighting and display. However, the low fluorescence efficiency and poor stabili...Nanocarbon as an eco-friendly and abundant material has strong multi-color fluorescence, which makes it a promising candidate for healthy lighting and display. However, the low fluorescence efficiency and poor stability of multi-color carbon nanoparticle（CNP） phosphors are main hurdles that hinder their applications. This work demonstrated efficient and stable multi-color CNP phosphors through synergy between inner polar groups and outer silica matrix. The polar groups in polyethylene glycol（PEG） 6,000 are favor of high fluorescence of the CNP phosphors, and the low melting point（64℃） of PEG 6,000 helps to improve the thermal stability of the phosphors, while the silica matrix provides protection to the phosphors. Based on this design,blue, green, yellow and red CNP phosphors with photoluminescence quantum yield of 53.1%, 47.4%, 43.8% and 42.3% have been achieved, all of which are the best values in ever reported multi-color CNP phosphors. Furthermore, the fluorescence of the CNP phosphors keeps almost unchanged at 100℃ and degrades little in one month, indicating their good thermal tolerance and temporal stability. In addition, multicolor devices including white light-emitting devices（LEDs）have been realized by coating the CNP phosphors onto UV chips. The luminous efficiency, correlated color temperature,Commission Internationale de L＇Eclairage and color rendering index of the white LED can reach 12 lm W^-1, 6,107 K,（0.32, 0.33） and 89, respectively, indicating the potential applications of the CNP phosphors in lighting and display.展开更多
Programming microscopic assembly mode to control macroscopic property is an attractive research objective.In particular,controlling molecular assembly to control fluorescence is of considerable interest for developing...Programming microscopic assembly mode to control macroscopic property is an attractive research objective.In particular,controlling molecular assembly to control fluorescence is of considerable interest for developing smart fluorescent materials.Herein,a color-tunable supramolecular emissive system was developed based on cucurbit[8]uril mediated host-vip assembly.Chemical designing for the molecular structures with minimized change resulted in different assembly modes and hence generating distinctive fluorescence,including green,yellow and orange with the addition of cucurbit[n]uril.Taking advantage of this feature,the advanced information encryption material(4D code)with multiple encryption levels and time-dependent encryption feature was developed.Such a code was dynamic on time scale,generating a series of 3D codes with time.The encrypted information only can be recognized by integrating time-coursed codes.This work provides a new insight for designing intelligent fluorescent materials for information encryption with high level of security.展开更多
A TiO_(2)-based multi-color photodetector with controlled photoelectric response to ultraviolet(UV)and visible light is developed by using band regulation technologies such as multi-junction synergy and surface adsorp...A TiO_(2)-based multi-color photodetector with controlled photoelectric response to ultraviolet(UV)and visible light is developed by using band regulation technologies such as multi-junction synergy and surface adsorption.This photodetector is manufactured via a continuous process including magnetron sputtering,hydrothermal growth,hydrogen annealing,spin coating and thermal evaporation assembly to form a structure of N-doped TiO_(2)/hydrogenated-TiO_(2)/p-Si heterojunction.These synergistic effects form electronic potential wells in the device to control the electrical transport and spectral response of photo-generated carriers.In the air,the device exhibits a controllable photodetection ability that responds to visible light at positive voltages and UV light at negative voltages.But in vacuum(<0.1 Pa),the photodetection ability of the device at negative voltages is greatly reduced due to the lack of barrier effect caused by surface adsorption.On the contrary,the photodetection ability at positive voltage(e.g.,4 V)has been greatly improved,and the quantum efficiency reaches 206.6%under the 480 nm wavelength light.The device has a controllable ability to detect UV and visible light depending on the environments,which is very useful in the fields of environmental detection,chemical sensing and multi-color communication,etc.展开更多
The identification of targets varies in different surge tests. A multi-color space threshold segmentation and self-learning k-nearest neighbor algorithm （k-NN） for equipment under test status identification was prop...The identification of targets varies in different surge tests. A multi-color space threshold segmentation and self-learning k-nearest neighbor algorithm （k-NN） for equipment under test status identification was proposed after using feature matching to identify equipment status had to train new patterns every time before testing. First, color space （L＊a＊b＊, hue saturation lightness （HSL）, hue saturation value （HSV）） to segment was selected according to the high luminance points ratio and white luminance points ratio of the image. Second, the unknown class sample Sr was classified by the k-NN algorithm with training set T~ according to the feature vector, which was formed from number ofpixels, eccentricity ratio, compact- ness ratio, and Euler＇s numbers. Last, while the classification confidence coefficient equaled k, made Sr as one sample ofpre-training set Tz＇. The training set Tz increased to Tz＋1 by Tz＇ if Tz＇ was saturated. In nine series of illuminant, indicator light, screen, and disturbances samples （a total of 21600 frames）, the algorithm had a 98.65% identification accuracy, also selected five groups of samples to enlarge the training set from To to T5 by itself. Keywords multi-color space, k-nearest neighbor algorithm （k-NN）, self-learning, surge test展开更多
基金supported by the National Natural Science Foundation of China(Nos.32260247 and 22064010)the Natural Science Foundation of Jiangxi Province(Nos.20232BAB215071 and 20224BAB213009).
文摘Developing an accurate and visual sensing strategy for trace levels of fluoroquinolone residues that pose threat to food safety and human health is highly desired but remains challenging.Herein,a target selfcalibration ratiometric fluorescent sensing platform has been designed for sensitive visual detection of levofloxacin(LEV)based on fluorescent europium metal-organic framework(Eu-MOF)probe.Specifically,the Eu-MOF was facilely synthesized via directly mixing Eu^(3+)with 1,10-phenanthroline-2,9-dicarboxylic acid(PDA)ligand at room temperature,which exhibited well-stable red fluorescence at 612 nm.Upon the addition of target LEV,the significant fluorescence quenching from Eu^(3+)was observed owing to the inner filter effect between the Eu-MOF and LEV.While the intrinsic fluorescence for LEV at 462nm was gradually enhanced,thereby realizing the self-calibration ratiometric fluorescence responses to LEV.Through this strategy,LEV can be detected down to 27 nmol/L.Furthermore,a test paper-based Eu-MOF integrated with the smartphone assisted RGB color analysis was exploited for the quantitative monitoring of LEV through the multi-color changes from red to blue,thus achieved portable,convenient and visual detection of LEV in honey and milk samples.Therefore,the developed strategy could provide a useful tool for supporting the practical on-site test in food samples.
基金Supported by the Natural Science Foundation of Zhejiang Province(No.LQ22F030015).
文摘This work addresses the cut order planning(COP)problem for multi-color garment production,which is the first step in the clothing industry.First,a multi-objective optimization model of multicolor COP(MCOP)is established with production error and production cost as optimization objectives,combined with constraints such as the number of equipment and the number of layers.Second,a decoupled multi-objective optimization algorithm(DMOA)is proposed based on the linear programming decoupling strategy and non-dominated sorting in genetic algorithmsⅡ(NSGAII).The size-combination matrix and the fabric-layer matrix are decoupled to improve the accuracy of the algorithm.Meanwhile,an improved NSGAII algorithm is designed to obtain the optimal Pareto solution to the MCOP problem,thereby constructing a practical intelligent production optimization algorithm.Finally,the effectiveness and superiority of the proposed DMOA are verified through practical cases and comparative experiments,which can effectively optimize the production process for garment enterprises.
基金Project (No. M603034) supported by the Natural Science Foundationof Zhejiang Province, China
文摘Conventional color-printing systems often use inks of three hues, such as CMY, CMYK and CMYKLcLm, but in order to obtain more realistic color reproductions, the ink set of more than three hues has been adopted by some color-printing systems. It is difficult, however, to model the composed color with the multiple inks when the number of the output ink hues exceeds three due to the none-unique mapping between the color spaces of the CIE Lab and the multi-color printing device. In this paper, we propose a fine color-printing method for multi-color printing device with the ink set of more than three hues. The proposed approach has good color expression ability and provides fine control of the printed color. By dividing the output color space into several subspaces, our method allows one-to-one mapping between the standard color space and the multi-color output color space. It has been proved effective when applied to the digital inkjet printer—Mutoh8000.
基金Project supported by the National Natural Science Foundation of China(Grant No.11604205)the Talent Program of Shanghai University of Engineering Science,China
文摘We study theoretically intense terahertz radiation from multi-color laser pulse with uncommon frequency ratios. Com- paring the two-color laser scheme, of which the uncommon frequency ratio should be set to be a specific value, we show that by using multi-color harmonic laser pulses as the first pump component, the lasers as the second pump component can be adjusted in a continuous frequency range. Moreover, these multi-color laser pulses can effectively modulate and enhance the terahertz radiation, and the terahertz yield increases with the increase of the wavelength of the uncommon pump com- ponent and is stable to the laser relative phase. Finally, we utilize the electron densities and velocities of ionization events to illustrate the physical mechanism of the intense terahertz generation.
基金Project supported by the National Natural Science Foundation of China(61564007)
文摘Multi-color luminescence basing on amorphous Eu^3＋/Tb^3＋ co-doped Zn-A1 hydroxides and their annealed samples were studied in detail. Results suggest that excellent red emissions due to E^u3＋ and green emissions attributed to Tb^3＋ appear under the excitation of favorable wavelength for all the as- prepared amorphous samples. Moreover, the emission intensity depends on the Eu^3＋/Tb^3＋ molar ratio. The samples annealed at 300, 500, and 700 ℃ still exhibit amorphous state, and multi-color lumi- nescence kept in the samples annealed at 300 ℃, while luminescence quenched for the samples annealed at 500 and 700 ℃. However, a broad emission ranging from 450 to 650 nm occurs in some samples annealed at 900 ℃. Further, the fluorescence decay and lifetimes for the as-prepared samples and the samples annealed at 300℃ were investigated. It is found that all the decay curves of emissions due to Tb^3＋ and Eu^3＋ present characteristic double exponential function despite their different lifetimes. The present work may be a good example for developing new multi-color even white light emitting materials.
基金supported by Beijing Municipal Governmentsupported by the National Natural Science Foundation of China(Grant Nos.61890952)the Director Fund of WNLO。
文摘Manipulating and real-time monitoring of neuronal activities with cell-type specificity and precise spatiotemporal resolution during animal behavior are fundamental technologies for exploring the functional connectivity, information transmission, and physiological functions of neural circuits in vivo. However, current techniques for optogenetic stimulation and neuronal activity recording mostly operate independently. Here, we report an all-fiber-transmission photometry system for simultaneous optogenetic manipulation and multi-color recording of neuronal activities and the neurotransmitter release in a freely moving animal. We have designed and manufactured a wavelength-independent multi-branch fiber bundle to enable simultaneous optogenetic manipulation and multi-color recording at different wavelengths. Further, we combine a laser of narrow linewidth with the lock-in amplification method to suppress the optogenetic stimulation-induced artifacts and channel crosstalk. We show that the collection efficiency of our system outperforms a traditional epi-fluorescence system. Further, we demonstrate successful recording of dynamic dopamine(DA) responses to unexpected rewards in the nucleus accumbens(NAc) in a freely moving mouse. We also show simultaneous dual-color recording of neuronal Ca2+ signals and DA dynamics in the NAc upon delivering an unexpected reward and the simultaneous optogenetic activating at dopaminergic terminals in the same location. Thus, our multi-function fiber photometry system provides a compatible, efficient, and flexible solution for neuroscientists to study neural circuits and neurological diseases.
基金Project supported by the Yunnan Provincial Natural Science Foundation (202101AT070126)the Research Start-up Fund of Chengdu University of Technology (10912-KYQD2020-08476)+1 种基金Fund of Hubei Key Laboratory of Plasma Chemistry,Advanced Materials (KF202103)Sichuan Natural Science Foundation (2022YFH0108,2022JDJQ0030)。
文摘Mechano-luminescence(ML) has been found diverse applications such as stress sensing,3-D signature,energy harvesting,and anti-counterfeiting,due to the unique properties of the corresponding ML phosphors performing in-situ and real-time response to mechanical stimulus.Trap-controlled ML materials realize reproducible,quantitative mechano-optical conversion resulting from the released carriers for the trap-mediated charge storage and release.Herein,modulating traps matters the controllable ML behavior for their promising applications.In this work,a deep trap distributed ranging from 0.9 to 1,3 eV is realized consecutively for the introduction of Sm^(3+)ions into LaGaO_(3) matrix,which contributes to the red emission at 600 nm under mechanical stimuli.Moreover,tunable ML emission modulated from 600to 545 nm is successfully achieved for the codopant of Tb^(3+)ions.It is unambiguously indicated that the released carriers from the trap sharing rather than an additional constructed trap contribute to the modulated ML color.Accordingly,multi-mode anti-counterfeiting and encryption are achieved with the as-explored Sm^(3+),Tb^(3+)co-activated ML phosphor.
基金Supported by the National High Level Hospital Clinical Research Funding,No.2022-PUMCH-B-003Beijing Technology Innovation Foundation for University or College Students,No.2022zglc06062.
文摘BACKGROUND Near-infrared fluorescence imaging via using intravenous indocyanine green(ICG)has a wide range of applications in multiple surgical scenarios.In lapa-roscopic cholecystectomy(LC),it facilitates intraoperative identification of the biliary system and reduces the risk of bile duct injury.However,the usual single color fluorescence imaging(SCFI)has limitations in manifesting the fluorescence signal of the target structure when its intensity is relatively low.Moreover,sur-geons often experience visual fatigue.We hypothesized that a novel imaging stra-tegy,named multi-color fluorescence imaging(MCFI),could potentially address these issues by decreasing hepatic and background fluorescence pollution and improving biliary visualization.AIM To investigate the novel imaging strategy MCFI in LC.METHODS This was a single-center retrospective study conducted at Peking Union Medical College Hospital,Beijing,China.Patients who underwent LC from June 2022 to March 2023 by the same surgical team were enrolled.Demographic features,clinical and surgical information were collected.The clarity,visual comfort,and effectiveness of different imaging strategies were subjectively evaluated by surgeons.RESULTS A total of 155 patients were included,60 patients were in the non-ICG group in which only bright light illuminance without ICG was applied,60 patients were in the SCFI group,and 35 patients were in the MCFI group.No statist-ically significant differences were found in demographics or clinical history.Post-surgical complications were minimal in all 3 groups with no significant differences observed.MCFI improved the clarity of imaging and visual comfort.Clarity of imaging and visual comfort were improved with MCFI.CONCLUSION MCFI improves biliary visualization and reduces liver fluorescence contamination,which supports its routine use in LC.MCFI may also be a better choice than SCFI in other clinical settings.
基金Key Research and Development Plan of Shaanxi Province,China(No.2023-YBGY-330)。
文摘In an automatic bobbin management system that simultaneously detects bobbin color and residual yarn,a composite texture segmentation and recognition operation based on an odd partial Gabor filter and multi-color space hierarchical clustering are proposed.Firstly,the parameter-optimized odd partial Gabor filter is used to distinguish bobbin and yarn texture,to explore Garbor parameters for yarn bobbins,and to accurately discriminate frequency characteristics of yarns and texture.Secondly,multi-color clustering segmentation using color spaces such as red,green,blue(RGB)and CIELUV(LUV)solves the problems of over-segmentation and segmentation errors,which are caused by the difficulty of accurately representing the complex and variable color information of yarns in a single-color space and the low contrast between the target and background.Finally,the segmented bobbin is combined with the odd partial Gabor’s edge recognition operator to further distinguish bobbin texture from yarn texture and locate the position and size of the residual yarn.Experimental results show that the method is robust in identifying complex texture,damaged and dyed bobbins,and multi-color yarns.Residual yarn identification can distinguish texture features and residual yarns well and it can be transferred to the detection and differentiation of complex texture,which is significantly better than traditional methods.
基金sponsored by Shanghai Pujiang Program(Grant No.22PJ1420200).
文摘For practical large-scale applications of computational fluid dynamics in the aero-space industry,implicit flow solvers are necessitated for efficient simulations.This paper presents the implementation of a solver that employs an unstructured finite volume approach and a Multi-Colored Gauss-Seidel(MCGS)method for steady-state compressible flow simulations on a server equipped with multiple Graphics Process-ing Units(GPUs).The mesh partition process is completed with PyMetis,and Mes-sage Passing Interface(MPI)is utilized for communications between mesh partitions.A parallel coloring algorithm is employed in the pre-processing module.The code is developed using a hybrid programming approach,with the main framework writ-ten in Python and the GPU kernel source codes written in C.The transonic turbulent flows over the CHN-T1 transport aircraft model are simulated on unstructured hybrid meshes.The numerical results are compared with experimental data,and the perfor-mance of the developed flow simulation framework is analysed.
基金supported by the National Natural Science Foundation of China (62074045, 62074040, 22309134)China Postdoctoral Science Foundation (2022M712402)Shanghai Rising-Star Program (23YF1449200)。
文摘High-resolution organic arrays with diverse pixel types hold significant promise for various applications,such as full-color displays and photonic crystals.The direct growth of such arrays(e.g.,high-resolution multi-color patterns)cannot be achieved in a single step with conventional strategies.Here,we present a viable approach integrating a bottom-up solution strategy with phase-change materials(PCMs),specifically aggregation-induced emission(AIE)materials.Through intentional self-assembly,color-programmable organic micro-patterns featuring distinct phases or colors were created.Notably,manipulating the amount of involved substance for nucleation/crystallization was achieved by adjusting the sizes of pre-defined nucleation sites.This precise control resulted in varied phases and colors for each pixel.Thus,high-resolution organic micro-arrays with transfer-free multi-color pixels were directly achieved.These may open avenues for seamless,transfer-free growth of multifunctional micro-patterns using PCMs,holding immense potential for applications in high-resolution full-color imaging/displays,photonic crystals,information storage,and encryption,etc.
基金the National Natural Science Foundation of China(NSFC:52473195,52303250,and 52073316)Guangdong Basic and Applied Basic Research Foundation(2022B1515020052)Research Foundation of the Department of Education of Guangdong Province(2024KCXTD009).
文摘Purely organic single-component luminescent materials enabling multi-color photoluminescence are gaining significant interest,given their tunable optical properties,environmental friendliness,and cost-effectiveness.However,realizing multi-color electroluminescence from a single-component emitter for application in organic light-emitting diode(OLED)remains challenging,mainly due to the limitations in achieving distinct excited-state conformations in amorphous or solid states.In this study,we report two novel emitters(Bppy-PTZ and Bpph-PTZ)by incorporating a benzophenone acceptor and phenothiazine donor with pyridyl and phenylπ-bridging spacers.The introduction of a pyridine ring in Bppy-PTZ establishes intramolecular hydrogen bonding,stabilizing the quasi-axial(QA)conformation in the amorphous state,thereby facilitating multi-color and white-light emissions in thin-film and OLED devices.Photophysical and theoretical analyses reveal distinct emission behaviors from QA and quasi-equatorial conformations,with Bppy-PTZ exhibiting enhanced dual-emission and mechanochromic properties.Importantly,by adopting single-component Bppy-PTZ,the fabricated OLEDs realize color-tunable emissions,including blue,yellow,and adjustable white lights,reaching maximum external quantum efficiencies of up to 15.5%.This work provides valuable insights for the development of efficient single-component emitters affording multi-color OLEDs with high performances.
基金the National Natural Science Foundation of China (30571184)Jiangsu Provincial Natural Science Foundation (BK2007166)+3 种基金the Tenth Five-year Plan of the National Key Program (2004BA525B05)the 111 Project(B08025) the Eleventh Five-year Plan of the National Sci-technologicalSupporting Program (2006BAD13B04-1-08)the Changjiang Scholars and Innovative Research Team in University and the Teaching and Research AwardProgram for Outstanding Young Teachers in Higher Education Institutions ofMinistry of Education (MOE), China.
文摘To identify alien chromosomes in recipient progenies and to analyze genome components in polyploidy, a genomic in situ hybridization （GISH） technique that is suitable for cotton was developed using increased stringency conditions. The increased stringency conditions were a combination of the four factors in the following optimized state： 100：1 ratio of blocking DNA to probe, 60% formamide wash solution, 43 ℃ temperature wash and a 13 min wash. Under these specific conditions using gDNA from Gossypium sturtianum （C1 C1 ） as a probe, strong hybridization signals were only observed on chromosomes from the C1 genome in somatic cells of the hybrid F1 （G. hirsutum x G. sturtianum） （AtDtC1）. Therefore, GISH was able to discriminate parental chromosomes in the hybrid. Further, we developed a multi-color GISH to simultaneously discriminate the three genomes of the above hybrid. The results repeatedly displayed the three genomes, At, Dt, and C1, and each set of chromosomes with a unique color, making them easy to identify. The power of the multi-color GISH was proven by analysis of the hexaploid hybrid F1 （G. hirsutum x G. australe） （AtAtDtDtG2G2）. We believe that the powerful multi-color GISH technique could be applied extensively to analyze the genome component in polyploidy and to identify alien chromosomes in the recipient progenies.
基金supported by the National Natural Science Foundation of China(Nos.92065101 and 11934013)the Space Debris Research Project of China(No.KJSP2020020202)。
文摘Frequency conversion based on three-wave mixing is a critical nonlinear optic application,extending the frequency range of existing lasers and realizing frequency-transduced detectors in a wavelength range that lacks an effective detector.Phase matching is vital for effective frequency conversion.The advantages of quasi-phase matching(QPM)over birefringent phase matching are a lack of walk-off effect,a maximum nonlinear coefficient,and phase matching in the entire transparency window.Herein,using different types and orders of QPM,four kinds of effective frequency doubling processes are realized in a periodically poled potassium titanyl phosphate(KTP)crystal with a single period,and three kinds of frequency doubling processes are experimentally verified.We also show a feasible way to construct an RGB color generator based on two different QPM processes.This study significantly expands the feasible frequency conversion of existing lasers to different wavelengths,providing an effective method for multi-color laser generation based on periodically poled KTP crystals.
基金the National Natural Science Foundation of China(No.21807085)the Natural Science Foundation Research Project of Shaanxi Province(No.2023-JCYB-087)+2 种基金the Technology Innovation Leading Program of Shaanxi(No.2020QFY07-05)the Innovation Capability Support Program of Shaanxi(No.2022KJXX-88)the fund of Education Department of Shaanxi Province(Program No.Z20230071).
文摘Carbon dots(CDs)with aggregation-induced emission(AIE)have sparked significant interest in multidimensional anti-counterfeiting due to their exceptional fluorescence properties.However,the preparation of AIE CDs with multicolor solid-state fluorescence remains a formidable challenge due to its complicated construction.In the present work,a novel class of multicolor AIE CDs(M-CDs)were fabricated using selected precursor(salicylic acid,thiosalicylic acid,and 2,2'-dithiodibenzoic acid),with an eco-friendly,low-cost one-pot solvothermal method.In the dilute organic solution,M-CDs manifested blue emission,but upon aggregation in the presence of water,the red,yellow,green,and blue emissions were displayed due to the AIE effect.Structural analysis,coupled with theoretical calculations,revealed that the increase in the size of sp2 domains would lower the Eg and cause a red-shift emission wavelength.Significantly,the continuous emission of M-CDs from blue to red can be utilized as ink for multimode printing,enabling the creation of a variety of school badges and quick response codes.These findings hold promising implications for multi-information encryption applications.
基金The authors are grateful to the National Natural Science Foundation of China （Nos. 11374092, 61474040, 61574054 and 61505051）, the National Basic Research Program of China （No. 2012CB933703）, the Aid Program for Science and Technology Innovative Research Team in Higher Educational Institutions of Hunan Province, the Hunan Provincial Science and Technology Depar- tment （Nos. 2014FJ2001, 2014GK3015 and 2014Tr1004）.
文摘Low-dimensional semiconductor nanostructures have attracted much interest for applications in integrated photonic and optoelectronic devices. Band gap engineering within single semiconductor nanoribbons helps to manipulate photon behavior in two different cavities （in the width and length directions） and realize new photonic phenomena and applications. In this work, lateral composition-graded semiconductor nanoribbons were grown for the first time through an improved source-moving vapor phase route. Along the width of the nanoribbon, the material can be gradually tuned from pure CdS to a highly Se-doped CdSSe alloy with a corresponding band gap modulation from 2.42 to 1.94 eV. The achieved alloy ribbons are overall high-quality crystals, and the position-dependent band-edge photoluminescence （PL） emission had a peak wavelength continuously tuned from -515 to -640 nm. These ribbons can realize multi-color lasing with three groups of lasing modes centered at 519, 557, and 623 run. It was confirmed that the red lasing was from optical resonance along the length direction, while the green and yellow lasing was from optical resonance along the width direction. These novel nanoribbon structures may be applied to many integrated photonic and optoelectronic devices.
基金supported by the National Natural Science Foundation of China (21601159, 61604132, 61505033, 11374296, 61404039)the National Science Fund for Distinguished Young Scholars (61425021)
文摘Nanocarbon as an eco-friendly and abundant material has strong multi-color fluorescence, which makes it a promising candidate for healthy lighting and display. However, the low fluorescence efficiency and poor stability of multi-color carbon nanoparticle（CNP） phosphors are main hurdles that hinder their applications. This work demonstrated efficient and stable multi-color CNP phosphors through synergy between inner polar groups and outer silica matrix. The polar groups in polyethylene glycol（PEG） 6,000 are favor of high fluorescence of the CNP phosphors, and the low melting point（64℃） of PEG 6,000 helps to improve the thermal stability of the phosphors, while the silica matrix provides protection to the phosphors. Based on this design,blue, green, yellow and red CNP phosphors with photoluminescence quantum yield of 53.1%, 47.4%, 43.8% and 42.3% have been achieved, all of which are the best values in ever reported multi-color CNP phosphors. Furthermore, the fluorescence of the CNP phosphors keeps almost unchanged at 100℃ and degrades little in one month, indicating their good thermal tolerance and temporal stability. In addition, multicolor devices including white light-emitting devices（LEDs）have been realized by coating the CNP phosphors onto UV chips. The luminous efficiency, correlated color temperature,Commission Internationale de L＇Eclairage and color rendering index of the white LED can reach 12 lm W^-1, 6,107 K,（0.32, 0.33） and 89, respectively, indicating the potential applications of the CNP phosphors in lighting and display.
基金supported by the National Natural Science Foundation of China(22025503,22220102004)the Shanghai Municipal Science and Technology Major Project(2018SHZDZX03)+3 种基金the Fundamental Research Funds for the Central Universitiesthe Programme of Introducing Talents of Discipline to Universities(B16017)the Science and Technology Commission of Shanghai Municipality(21JC1401700)the Starry Night Science Fund of Zhejiang University Shanghai Institute for Advanced Study(SN-ZJU-SIAS-006)。
文摘Programming microscopic assembly mode to control macroscopic property is an attractive research objective.In particular,controlling molecular assembly to control fluorescence is of considerable interest for developing smart fluorescent materials.Herein,a color-tunable supramolecular emissive system was developed based on cucurbit[8]uril mediated host-vip assembly.Chemical designing for the molecular structures with minimized change resulted in different assembly modes and hence generating distinctive fluorescence,including green,yellow and orange with the addition of cucurbit[n]uril.Taking advantage of this feature,the advanced information encryption material(4D code)with multiple encryption levels and time-dependent encryption feature was developed.Such a code was dynamic on time scale,generating a series of 3D codes with time.The encrypted information only can be recognized by integrating time-coursed codes.This work provides a new insight for designing intelligent fluorescent materials for information encryption with high level of security.
基金This work was financially supported by the National Natural Science Foundation of China(No.51972055)the Shenzhen Science and Technology Research Project(No.JCYJ20180508152903208)+5 种基金the Guangdong Basic and Applied Basic Research Foundation(No.2020A1515010258)the Stable Support Project for Shenzhen High Education Institutions(No.SZWD2021001)the Shenzhen Bay Laboratory Open Program(No.SZBL2020090501002)the Natural Science Foundation of Top Talent of SZTU(No.20200201)the Homemade Experimental Equipment Foundation of SZTU(No.2020XZY002)the Shenzhen Pengcheng Scholar Program.
文摘A TiO_(2)-based multi-color photodetector with controlled photoelectric response to ultraviolet(UV)and visible light is developed by using band regulation technologies such as multi-junction synergy and surface adsorption.This photodetector is manufactured via a continuous process including magnetron sputtering,hydrothermal growth,hydrogen annealing,spin coating and thermal evaporation assembly to form a structure of N-doped TiO_(2)/hydrogenated-TiO_(2)/p-Si heterojunction.These synergistic effects form electronic potential wells in the device to control the electrical transport and spectral response of photo-generated carriers.In the air,the device exhibits a controllable photodetection ability that responds to visible light at positive voltages and UV light at negative voltages.But in vacuum(<0.1 Pa),the photodetection ability of the device at negative voltages is greatly reduced due to the lack of barrier effect caused by surface adsorption.On the contrary,the photodetection ability at positive voltage(e.g.,4 V)has been greatly improved,and the quantum efficiency reaches 206.6%under the 480 nm wavelength light.The device has a controllable ability to detect UV and visible light depending on the environments,which is very useful in the fields of environmental detection,chemical sensing and multi-color communication,etc.
文摘The identification of targets varies in different surge tests. A multi-color space threshold segmentation and self-learning k-nearest neighbor algorithm （k-NN） for equipment under test status identification was proposed after using feature matching to identify equipment status had to train new patterns every time before testing. First, color space （L＊a＊b＊, hue saturation lightness （HSL）, hue saturation value （HSV）） to segment was selected according to the high luminance points ratio and white luminance points ratio of the image. Second, the unknown class sample Sr was classified by the k-NN algorithm with training set T~ according to the feature vector, which was formed from number ofpixels, eccentricity ratio, compact- ness ratio, and Euler＇s numbers. Last, while the classification confidence coefficient equaled k, made Sr as one sample ofpre-training set Tz＇. The training set Tz increased to Tz＋1 by Tz＇ if Tz＇ was saturated. In nine series of illuminant, indicator light, screen, and disturbances samples （a total of 21600 frames）, the algorithm had a 98.65% identification accuracy, also selected five groups of samples to enlarge the training set from To to T5 by itself. Keywords multi-color space, k-nearest neighbor algorithm （k-NN）, self-learning, surge test
