The development of advanced magnetoelectric(ME)composites necessitates high-performance materials that arecapable of achieving high levels of ME coupling,minimal magnetic loss,and absence or limited reliance on extern...The development of advanced magnetoelectric(ME)composites necessitates high-performance materials that arecapable of achieving high levels of ME coupling,minimal magnetic loss,and absence or limited reliance on externalexcitation sources.In this paper,a(2-2)connectivity ME laminate integrates multiple layers of FeSiB alloy(Metglas)andPb(Mg,Nb)O_(3)-PbTiO_(3)(PMN-PT)single crystal,achieving a remarkable ME coupling coefficient of 2033.4 V/Oe·cm(sevenfold rise)by laser thermal annealing treatment.Here,the laser-induced nanostructures on Metglas,with anoxidized insulation layer and soft and hard magnetic dipole layer improve the Magneto-electric-mechanical couplingwith a mechanical quality factor(Q_(m))exceeding 350.More importantly,the interaction between amorphous andnanocrystalline dipoles triggers an Exchange Bias(EB)effect,leading to a self-biasing performance of 67.45 V/Oe·cm.Furthermore,the composite exhibits an excellent passive DC magnetic detection limit of 22 nT,and an improved weakAC magnetic detection limit down to 383 fT.These explorations offer the potential to enhance passive currentmeasurement,and underwater communication,extend weak magnetic positioning and brain magnetic detection.展开更多
基金supported by the National Key Research and Development Program(Grant No.2021YFB3201800)the Natural Science Foundation of China(Grants 62131017,U22A2019)the Key R&D Project of Shaanxi Province-University Joint Project(2023GXLH-020).
文摘The development of advanced magnetoelectric(ME)composites necessitates high-performance materials that arecapable of achieving high levels of ME coupling,minimal magnetic loss,and absence or limited reliance on externalexcitation sources.In this paper,a(2-2)connectivity ME laminate integrates multiple layers of FeSiB alloy(Metglas)andPb(Mg,Nb)O_(3)-PbTiO_(3)(PMN-PT)single crystal,achieving a remarkable ME coupling coefficient of 2033.4 V/Oe·cm(sevenfold rise)by laser thermal annealing treatment.Here,the laser-induced nanostructures on Metglas,with anoxidized insulation layer and soft and hard magnetic dipole layer improve the Magneto-electric-mechanical couplingwith a mechanical quality factor(Q_(m))exceeding 350.More importantly,the interaction between amorphous andnanocrystalline dipoles triggers an Exchange Bias(EB)effect,leading to a self-biasing performance of 67.45 V/Oe·cm.Furthermore,the composite exhibits an excellent passive DC magnetic detection limit of 22 nT,and an improved weakAC magnetic detection limit down to 383 fT.These explorations offer the potential to enhance passive currentmeasurement,and underwater communication,extend weak magnetic positioning and brain magnetic detection.
