In high-temperature gas-cooled reactors,graphite dust particles within the reactor core and the heat transfer equipment experience large temperature gradients.Under such conditions,thermophoresis may play an important...In high-temperature gas-cooled reactors,graphite dust particles within the reactor core and the heat transfer equipment experience large temperature gradients.Under such conditions,thermophoresis may play an important role in determining aerosol evolution.This study presents a theoretical and numerical analysis of the thermophoretic effects on aerosol coagulation within these reactors.The coagulation rates for Brownian versus thermophoretic coagulation are calculated and compared for various temperature gradients.Our results show that thermophoretic coagulation dominates over Brownian coagulation for large temperature gradients.We defined an enhancement factor to evaluate the role of thermophoretic coagulation under various reactor conditions.The enhancement factor increased dramatically with increasing temperature gradient,decreasing pressure and increasing particle diameter,but was not very sensitive to temperature change.The time evolution of the particle size distribution related to combined Brownian and thermophoretic coagulation was simulated using a log-skew-normal method of moments.The simulation results indicate that aerosol evolution can be strongly accelerated by thermophoretic coagulation under large temperature gradients.展开更多
基金supported in part by the Novel Bio-statistical and Epidemiologic Methodology grants from the University of Rochester Medical Center Clinical and Translational Science Institute Pilot Awards Program
基金This work was supported by the National Natural Science Foundation of China(Grant No.51676112)the National Key Research&Development Program of China(Grant No.2016YFC0202700)+1 种基金the National Science&Technology Major Project(Grant No.ZX069)Key Laboratory of Advanced Reactor Engineering and Safety of Ministry of Education.We also thank Prof.David Christopher for editing the English.
文摘In high-temperature gas-cooled reactors,graphite dust particles within the reactor core and the heat transfer equipment experience large temperature gradients.Under such conditions,thermophoresis may play an important role in determining aerosol evolution.This study presents a theoretical and numerical analysis of the thermophoretic effects on aerosol coagulation within these reactors.The coagulation rates for Brownian versus thermophoretic coagulation are calculated and compared for various temperature gradients.Our results show that thermophoretic coagulation dominates over Brownian coagulation for large temperature gradients.We defined an enhancement factor to evaluate the role of thermophoretic coagulation under various reactor conditions.The enhancement factor increased dramatically with increasing temperature gradient,decreasing pressure and increasing particle diameter,but was not very sensitive to temperature change.The time evolution of the particle size distribution related to combined Brownian and thermophoretic coagulation was simulated using a log-skew-normal method of moments.The simulation results indicate that aerosol evolution can be strongly accelerated by thermophoretic coagulation under large temperature gradients.
