Polyvinylpyrrolidone K-30(PVP) was introduced into the preparation of nanozero-valent iron(n ZVI) and the traditional liquid-phase reduction was improved. The introduction of PVP simplified the traditional method.The ...Polyvinylpyrrolidone K-30(PVP) was introduced into the preparation of nanozero-valent iron(n ZVI) and the traditional liquid-phase reduction was improved. The introduction of PVP simplified the traditional method.The n ZVI prepared with this new approach showed excellent surface characters and high performance on the removal of cadmium. TEM results showed that the aggregates of n ZVI can reach to several micrometers in length but less than 100 nm in diameter. The iron particles that were enclosed by a layer of oxide film that is less than10 nm, demonstrated that the n ZVI possesses a core–shell structure. BET results indicate that the specific surface area of the n ZVI was 20.3159 m^2g^(-1). A three factor and three level orthogonal experiment was employed to find out the dominant factor that affects the removal rate of cadmium by n ZVI. Based on the range values, the prominence order of each factor was: initial p H of the solution N initial concentration of cadmium N dosage of n ZVI, the range was 96.453, 3.294 and 1.747, respectively. A simulation was performed under the same condition and a same conclusion was derived, this consistence confirmed the validity of the conclusion that p H is the most significant factor that affects the adsorption efficiency.展开更多
Shock-timing experiments are indispensable to inertial confinement fusion mainly because the timing of multiple shock waves is crucial to understanding the processes of laser irradiation of targets. Investigations int...Shock-timing experiments are indispensable to inertial confinement fusion mainly because the timing of multiple shock waves is crucial to understanding the processes of laser irradiation of targets. Investigations into shock waves driven by a two-step radiation pulse in polystyrene（CH） capsule targets are experimentally conducted at the Shen Guang Ⅱ laser facility. Differing from the traditional shock-timing implementation in which one shock wave could catch up with another one in solid CH, in this experiment, the second shock front in a rarefaction CH layer is observed through velocity interferometry. This second shock could also be made to converge with rarefaction waves within only a few micrometers of the CH capsule by designing the two-shock coalescence time. A shock-timing diagnostic technique to tune the multi-shock convergence in the CH capsule can thereby be achieved.The experimental results in the CH layer are quasi-quantitatively interpreted using streamlines simulated with the Multi-1 D program. The experimental results are expected to offer important information for target structure and laser pulse design, both of which are important for realizing inertial confinement fusion.展开更多
基金Supported by the National Natural Science Foundation of China(51278147)the Funds for Creative Research Groups of China(51121062)State Key Laboratory of Urban Water Resource and Environment(Harbin Institute of Technology)(2014TS02)
文摘Polyvinylpyrrolidone K-30(PVP) was introduced into the preparation of nanozero-valent iron(n ZVI) and the traditional liquid-phase reduction was improved. The introduction of PVP simplified the traditional method.The n ZVI prepared with this new approach showed excellent surface characters and high performance on the removal of cadmium. TEM results showed that the aggregates of n ZVI can reach to several micrometers in length but less than 100 nm in diameter. The iron particles that were enclosed by a layer of oxide film that is less than10 nm, demonstrated that the n ZVI possesses a core–shell structure. BET results indicate that the specific surface area of the n ZVI was 20.3159 m^2g^(-1). A three factor and three level orthogonal experiment was employed to find out the dominant factor that affects the removal rate of cadmium by n ZVI. Based on the range values, the prominence order of each factor was: initial p H of the solution N initial concentration of cadmium N dosage of n ZVI, the range was 96.453, 3.294 and 1.747, respectively. A simulation was performed under the same condition and a same conclusion was derived, this consistence confirmed the validity of the conclusion that p H is the most significant factor that affects the adsorption efficiency.
基金Supported by the Science and Technology on Plasma Physics Laboratory under Grant No 9140C6801021001
文摘Shock-timing experiments are indispensable to inertial confinement fusion mainly because the timing of multiple shock waves is crucial to understanding the processes of laser irradiation of targets. Investigations into shock waves driven by a two-step radiation pulse in polystyrene（CH） capsule targets are experimentally conducted at the Shen Guang Ⅱ laser facility. Differing from the traditional shock-timing implementation in which one shock wave could catch up with another one in solid CH, in this experiment, the second shock front in a rarefaction CH layer is observed through velocity interferometry. This second shock could also be made to converge with rarefaction waves within only a few micrometers of the CH capsule by designing the two-shock coalescence time. A shock-timing diagnostic technique to tune the multi-shock convergence in the CH capsule can thereby be achieved.The experimental results in the CH layer are quasi-quantitatively interpreted using streamlines simulated with the Multi-1 D program. The experimental results are expected to offer important information for target structure and laser pulse design, both of which are important for realizing inertial confinement fusion.
