Conventional ignition methods are proving to be ineffective for low-sensitivity energetic materials,highlighting the need to investigate alternative ignition systems,such as laser-based techniques.Over the past decade...Conventional ignition methods are proving to be ineffective for low-sensitivity energetic materials,highlighting the need to investigate alternative ignition systems,such as laser-based techniques.Over the past decade,lasers have emerged as a promising solution,providing focused energy beams for controllable,efficient,and reliable ignition in the field of energetic materials.This study presents a comparative analysis of two state-of-the-art ignition approaches:direct laser ignition and laser-driven flyer ignition.Experiments were performed using a Neodymium-doped Yttrium Aluminum Garnet(Nd:YAG)laser at different energy beam levels to systematically evaluate ignition onset.In the direct laser ignition test setup,the laser beam was applied directly to the energetic tested material,while laserdriven flyer ignition utilized 40 and 100μm aluminum foils,propelled at velocities ranging from 300 to 1250 m/s.Comparative analysis with the Lawrence and Trott model substantiated the velocity data and provided insight into the ignition mechanisms.Experimental results indicate that the ignition time for the laser-driven flyer method was significantly shorter,with the pyrotechnic composition achieving complete combustion faster compared to direct laser ignition.Moreover,precise ignition thresholds were determined for both methods,providing critical parameters for optimizing ignition systems in energetic materials.This work elucidates the advantages and limitations of each technique while advancing next-generation ignition technology,enhancing the reliability and safety of propulsion systems.展开更多
Able to precisely control and manipulate materials'states at micro/nano-scale level,femtosecond(fs)laser micro/nano processing technology has undergone tremendous development over the past three decades.Free-formi...Able to precisely control and manipulate materials'states at micro/nano-scale level,femtosecond(fs)laser micro/nano processing technology has undergone tremendous development over the past three decades.Free-forming three-dimensional(3D)microscale functional devices and inducing fascinating and unique physical or chemical phenomena have granted this technology powerful versatility that no other technology can match.As this technology advances rapidly in various fields of application,some key challenges have emerged and remain to be urgently addressed.This review firstly introduces the fundamental principles for understanding how fs laser pulses interact with materials and the associated unique phenomena in section 2.Then micro/nano-fabrication in transparent materials by fs laser processing is presented in section 3.Thereafter,several high efficiency/throughput fabrication methods as well as pulse-shaping techniques are listed in sections 4 and 5 reviews four-dimensional(4D)and nanoscale printing realized by fs laser processing technology.Special attention is paid to the heterogeneous integration(HI)of functional materials enabled by fs laser processing in section 6.Several intriguing examples of 3D functional micro-devices created by fs laser-based manufacturing methods such as microfluidics,lab-on-chip,micro-optics,micro-mechanics,micro-electronics,micro-bots and micro-biodevices are reviewed in section 7.Finally,a summary of the review and a perspective are proposed to explore the challenges and future opportunities for further betterment of fs laser micro/nano processing technology.展开更多
AIM:To assess the effectiveness and safety of VISULAS®green laser selective laser trabeculoplasty(SLT)in lowering intraocular pressure(IOP)in patients with pseudoexfoliative syndrome glaucoma(PEXG)and pseudoexfol...AIM:To assess the effectiveness and safety of VISULAS®green laser selective laser trabeculoplasty(SLT)in lowering intraocular pressure(IOP)in patients with pseudoexfoliative syndrome glaucoma(PEXG)and pseudoexfoliative syndrome ocular hypertension(PEXS-OHT).METHODS:This prospective,single-center,interventional study included 20 eyes from 20 patients diagnosed with PEXG or PEXS-OHT.Patients underwent 180°SLT using the VISULAS®green laser,a diode-pumped,frequencydoubled Nd:YVO4 laser with a 532 nm wavelength.IOP was measured at baseline and post-treatment at 1,3,and 6mo.Medications regimen was stable through the study.Primary outcomes included mean IOP reduction,while secondary outcomes assessed visual and structural parameters,and safety.RESULTS:The mean age of participants was 72.2±6.6y,with 65%of the eyes being left eyes and 35%right eyes.At baseline,the mean IOP was 22.9±2.9 mm Hg.A significant reduction in IOP was observed at all follow-up intervals:18.5±3.1 mm Hg at 1mo(18.8%reduction,P=0.001),19.0±4.2 mm Hg at 3mo(16.7%reduction,P=0.002),and 18.2±4.5 mm Hg at 6mo(19.8%reduction,P=0.001).Subgroup analysis showed greater IOP reduction in patients with Shaffer grade 4 angles,phakic eyes,and those with PEXS-OHT compared to PEXG.No significant changes were detected in visual acuity,visual field index,mean deviation,or retinal nerve fiber layer thickness.At 1h post-procedure,20%of eyes showed an IOP spike>5 mm Hg that resolved without intervention except for one patient.CONCLUSION:SLT with the VISULAS®green laser is an effective and safe treatment for PEXG and PEXS-OHT,achieving significant IOP reduction without increasing medication burden or causing severe complications.These findings suggest its potential as an alternative or adjunct therapy in managing pseudoexfoliative glaucoma.展开更多
The effects of initial spin orientation on the final electron beam polarization in laser wakefield acceleration in a pre-polarized plasma are investigated theoretically and numerically.From the results of variation of...The effects of initial spin orientation on the final electron beam polarization in laser wakefield acceleration in a pre-polarized plasma are investigated theoretically and numerically.From the results of variation of the initial spin direction,the spin dynamics of the electron beam are found to depend on the self-injection mechanism.The effects of wakefields and laser fields are studied using test particle dynamics and particle-in-cell simulations based on the Thomas-Bargmann-Michel-Telegdi equation.Compared with transverse injection,longitudinal injection is found to be preferable for obtaining a highly polarized electron beam.展开更多
Laser remelting(LR)was used as an auxiliary post-treatment process for the Ti6Al4V titanium alloys fabricated by laser powder bed fusion(LPBF).Optical microscope(OM),scanning electron microscope(SEM)and electron back ...Laser remelting(LR)was used as an auxiliary post-treatment process for the Ti6Al4V titanium alloys fabricated by laser powder bed fusion(LPBF).Optical microscope(OM),scanning electron microscope(SEM)and electron back scattering diffraction(EBSD)observations showed that the grains in melted zone(MZ)transformed into equiaxial grains with an average size of 1.31μm,and the grains in heat affected zone(HAZ)were refined.Moreover,the texture intensity dropped significantly from 13.86 to 6.35 in MZ and 10.79 in HAZ.The temperature gradient(G)to solidification rate(R)ratio decreased when the laser scanning speed slowed down to a certain extent in the LR process,which effectively improved the highly preferred orientation and filled the hole defects in the surface of LPBF-Ti6Al4V.Furthermore,the hardness,wear resistance and corrosion resistance of the surface of the LPBF samples were improved by LR treatment.展开更多
The original online version of this article was revised:Several errors occurred in the published version of the article.These have now been corrected as follows:Page 2,section"2.2 Laser Texturing Procedure of Sur...The original online version of this article was revised:Several errors occurred in the published version of the article.These have now been corrected as follows:Page 2,section"2.2 Laser Texturing Procedure of Surfaces",line 2:The device name was corrected from"YDFLP-E-50-M8"to"YDFLP-50-M8."Page 3,Section 2.4:The phrase"95%confidence interval"has been corrected to"95%confidence level."Page 3,Figure 1 caption:The phrase"fandg"has been corrected to"f and g."The order"C4 and C12"has been reversed to"C12 and C4,"in accordance with the display order in the figure.Page 4,Figure reference:The phrase"Figs.4c and d"has been corrected to"Figs.5b and c."Page 5,paragraph starting with"The ANOVA results are presented...":The phrase"95%confidence interval"has been corrected to"95%confidence level."展开更多
The 193 nm deep-ultraviolet(DUV)laser plays a critical role in advanced semiconductor chip manufacturing[1,2],micro-nano material characterization[3,4]and biomedical analysis[5,6],due to its high spatial resolution an...The 193 nm deep-ultraviolet(DUV)laser plays a critical role in advanced semiconductor chip manufacturing[1,2],micro-nano material characterization[3,4]and biomedical analysis[5,6],due to its high spatial resolution and short wavelength.Efficient and compact 193 nm DUV laser source thus becomes a hot research area.Currently,193 nm Ar F excimer gas laser is widely employed in DUV lithography systems and serves as the enabling technology for 7 and 5 nm semiconductor fabrication.展开更多
Understanding the complex plasma dynamics in ultra-intense relativistic laser-solid interactions is of fundamental importance for applications of laser-plasma-based particle accelerators,the creation of high-energy-de...Understanding the complex plasma dynamics in ultra-intense relativistic laser-solid interactions is of fundamental importance for applications of laser-plasma-based particle accelerators,the creation of high-energy-density matter,understanding planetary science,and laser-driven fusion energy.However,experimental efforts in this regime have been limited by the lack of accessibility of over-critical densities and the poor spatiotemporal resolution of conventional diagnostics.Over the last decade,the advent of femtosecond brilliant hard X-ray free-electron lasers(XFELs)has opened new horizons to overcome these limitations.Here,for the first time,we present full-scale spatiotemporal measurements of solid-density plasma dynamics,including preplasma generation with tens of nanometer scale length driven by the leading edge of a relativistic laser pulse,ultrafast heating and ionization at the main pulse arrival,the laser-driven blast wave,and transient surface return current-induced compression dynamics up to hundreds of picoseconds after interaction.These observations are enabled by utilizing a novel combination of advanced X-ray diagnostics including small-angle X-ray scattering,resonant X-ray emission spectroscopy,and propagation-based X-ray phase-contrast imaging simultaneously at the European XFEL-HED beamline station.展开更多
Tunable mid-infrared and far-infrared laser output was demonstrated based on BaGa_(4)Se_(7)crystals and an optical parametric oscillator(OPO).With a 1.06μm Nd:YAG laser and a double-pass singly resonant OPO cavity,a ...Tunable mid-infrared and far-infrared laser output was demonstrated based on BaGa_(4)Se_(7)crystals and an optical parametric oscillator(OPO).With a 1.06μm Nd:YAG laser and a double-pass singly resonant OPO cavity,a laser energy output of 2.2 mJ at 10μm was obtained.By tuning the angle and temperature,a tunable laser output covering the wavelength range from 6μm to 17μm was obtained with a tuning precision better than 3 nm.The corresponding optical-to-optical conversion efficiency was 2.8%,and the slope efficiency was 4.4%.The damage effect of the output laser on detectors was also investigated,and point damage to the detector occurred at an output energy of 16.4μJ.The laser system has the advantages of miniaturization,a wide tuning range,high energy and high tuning resolution.Its broadband laser characteristics make it highly valuable for applications in atmospheric detection,infrared spectroscopy and electro-optical countermeasures.展开更多
Experiments with interacting high-velocity flows in a laser plasma can help answer fundamental questions in plasma physics and improve understanding of the mechanisms behind some astrophysical phenomena,such as the fo...Experiments with interacting high-velocity flows in a laser plasma can help answer fundamental questions in plasma physics and improve understanding of the mechanisms behind some astrophysical phenomena,such as the formation of collisionless shock waves,deceleration of accretion flows,and evolution of solar and stellar flares.This work presents the first direct experimental observations of stagnation and redirection of counterstreaming flows(jets)of laser plasma induced by intense laser pulses with intensity I~2×10^(18) W/cm^(2).Hybrid particlein-cell-fluid modeling,which takes into account the kinetic effects of ion motion and the evolution of the pressure tensor for electrons,demonstrates the compression of counterdirected toroidal self-generated magnetic fields embedded in counterstreaming plasma flows.The enhancement of the toroidal magnetic field in the interaction region results in plasma flow stagnation and redirection of the jets across the line of their initial propagation.展开更多
We investigate theoretically and experimentally the chaotic dynamics of visible-wavelength all-fiber ring laser.The100-m 630 HP fibers are used to ensure high non-linearity.A 4-m Pr^(3+)/Yb^(3+)-co-doped ZBLAN fiber p...We investigate theoretically and experimentally the chaotic dynamics of visible-wavelength all-fiber ring laser.The100-m 630 HP fibers are used to ensure high non-linearity.A 4-m Pr^(3+)/Yb^(3+)-co-doped ZBLAN fiber provides the gain.The chaotic laser was pumped by the laser diodes with the maximum power of 150 mW at the wavelength of 850 nm.The peak fluorescence spectrum of Pr^(3+)/Yb^(3+)-co-doped ZBLAN fiber at the wavelength of 635 nm shows that the visiblewavelength fiber laser can be achieved by synergistic energy transfer between Pr~(3+)and Yb^(3+)ions.The chaotic fiber laser is generated by adjusting the pump power,polarization controller and the auto-correlation,permutation entropy,skewness,and kurtosis were used to analyze the characteristics of chaotic laser.The noise-like time series and delta-like auto-correlation curve indicate the chaotic output.The complexity and randomness of time series are analyzed by the permutation entropy,skewness,and kurtosis.The result shows that chaotic dynamics is stable when the pump power exceeds a certain value.The visible chaotic all-fiber laser has high stability and can be applied for real-time monitoring and sensing.We believe that this approach may also be feasible for other materials for emission in the visible range.展开更多
We present a solid 226 nm deep ultraviolet laser system pumped by a Nd:YAG laser.A diamond Raman laser with a 1485 nm wavelength was generated up to 2.53 mJ pumped by a 9.7 mJ 1064 nm laser,which is the highest pulse ...We present a solid 226 nm deep ultraviolet laser system pumped by a Nd:YAG laser.A diamond Raman laser with a 1485 nm wavelength was generated up to 2.53 mJ pumped by a 9.7 mJ 1064 nm laser,which is the highest pulse energy of a second Stokes diamond Raman laser pumped by a 1064 nm laser as we know.Then,the Raman laser is mixed with the frequency-quadrupled 1064 nm laser to produce the 226 nm laser.The maximum output pulse energy at 226 nm reaches 0.49 mJ.The overall conversion efficiency from1064 to 226 nm is up to 1.14%,which is significantly higher than conventional optical parametric oscillator technology for the generation of 226 nm laser.The 226 nm laser system has been used in a laser-induced fluorescence(LIF)experiment of oxygen two-photon to demonstrate its potential for LIF measurements.展开更多
The suppression of ablative Rayleigh–Taylor instability(ARTI)by a spatially modulated laser in inertial confinement fusion(ICF)is studied through numerical simulations.The results show that in the acceleration phase ...The suppression of ablative Rayleigh–Taylor instability(ARTI)by a spatially modulated laser in inertial confinement fusion(ICF)is studied through numerical simulations.The results show that in the acceleration phase of ICF implosion,the growth of ARTI can be suppressed by using a short-wavelength spatially modulated laser.The ARTI growth rate decreases as the wavelength of the spatially modulated laser decreases,and ARTI is completely suppressed after a certain wavelength has been reached.A spatially uniform laser is introduced to keep the state of motion of the implosion fluid consistent,and it is found that the proportion of the spatially modulated laser required for complete suppression of ARTI decreases as the wavelength continues to decrease.We also optimize the spatial intensity distribution of the spatially modulated laser.In addition,as the duration of the spatially modulated laser decreases,the proportion required for completely suppressing ARTI increases,but the required energy decreases.When the perturbation wavenumber decreases,the wavelength of the spatially modulated laser required for complete suppression of ARTI becomes longer.In the case of multimode perturbation,ARTI can also be significantly suppressed by a spatially modulated laser,and the perturbation amplitude can be reduced to less than 10% of that without a spatially modulated laser.We believe that the conclusions drawn from our simulations can provide the basis for new approaches to control ARTI in ICF.展开更多
Additive and solvent-free direct printing is critical for many applications,including smart electronics,solar cells,healthcare,and electrochemical energy storage.Although a few green techniques for direct patterning o...Additive and solvent-free direct printing is critical for many applications,including smart electronics,solar cells,healthcare,and electrochemical energy storage.Although a few green techniques for direct patterning of inorganic functional materials have been developed,they operate at small scale and require long processing times,restricting their effective translation from laboratory to market.Here we report a fast,liquid-free,cost-effective,and environmentally friendly aerosol-based printing method for fabricating linear or planar structures at microscale dimensions.In situ and on-demand generation of dry aerosol via pulsed laser ablation,coupled with real-time aerodynamical focusing using a co-flowing sheath gas,allows the deposition of a wide variety of materials on various substrates at room temperature and atmospheric pressure.Using silver as a test material,we systematically characterized the laser-generated aerosol deposits in terms of microstructural morphology,sintering activity,mass yield,density,and electrical performance,to show the relationship between process variability and underlying mechanisms.The capacity of high-throughput printing of silver deposits,with thickness up to 160μm,in a single pass was demonstrated.This rapid,efficient,and inkless printing process opens new and exciting opportunities for future applications that require easy-to-integrate components in printed electronic devices.展开更多
A RadioFrequency Quadrupole(RFQ)cooler-buncher system was developed and implemented in a collinear laser spectroscopy setup.This system converts a continuous ion beam into short bunches while enhancing the beam qualit...A RadioFrequency Quadrupole(RFQ)cooler-buncher system was developed and implemented in a collinear laser spectroscopy setup.This system converts a continuous ion beam into short bunches while enhancing the beam quality and reducing the energy spread.The functionality of the RFQ cooler buncher was verified through offline tests with stable rubidium and indium beams delivered from a surface ion source and a laser ablation ion source,respectively.Bunched ion beams with a full width at half maximum of approximately 2μs in the time-of-flight spectrum were successfully achieved with a transmission efficiency exceeding 60%.The implementation of the RFQ cooler-buncher system also significantly improved the overall transmission efficiency of the collinear laser spectroscopy setup.展开更多
The combustion behavior of Ti-Al-Mo-Zr-Sn-W alloy(TC25G)was studied in a high-temperature and high-speed air flow environment using the laser ignition method combined with ultra-high temperature infrared thermometer,s...The combustion behavior of Ti-Al-Mo-Zr-Sn-W alloy(TC25G)was studied in a high-temperature and high-speed air flow environment using the laser ignition method combined with ultra-high temperature infrared thermometer,scanning electron microscope,X-ray diffractometer,and transmission electron microscope.The burn-resistant performance of TC25G and TC11 alloys was compared.Meanwhile,the microstructural characteristics,crystal structure,and formation mechanism of the combustion products of TC25G alloy were analyzed in detail.The results show that the high-temperature and high-speed air flow promotes combustion within the air flow temperature range of 200–400℃and the air flow velocity range of 0–100 m/s.The combustion path advances along the direction of the air flow.The combustion of TC25G alloy mainly relies on the diffusion of the oxygen and the expansion of the combustion area caused by the movement of the melt.Based on the microstructure and composition of combustion product,it can be divided into the combustion zone,the melting zone,and the heat affected zone.During combustion,the formation of microstructures is closely correlated with the behavior of alloying elements and their selective combination with O.The major oxidation products of Ti are TiO and TiO_(2).The oxides formed by Mo and W hinder the movement of the melt during the combustion.Al and Zr tend to undergo internal oxidation.Al_(2)O_(3)precipitates on the surface of ZrO_(2),forming a protective oxide layer that inhibits the inward diffusion of O.Moreover,the element enrichment at the interface between the melting zone and the heat affected zone increases the melting point on the solid side,hindering the migration of the solid-liquid interface.展开更多
We designed and investigated a passive synchronized mode-locked fiber laser.The device utilizes a dual-cavity structure driven by the nonlinear polarization rotation(NPR)mechanism.Stable mode-locking is attained by sy...We designed and investigated a passive synchronized mode-locked fiber laser.The device utilizes a dual-cavity structure driven by the nonlinear polarization rotation(NPR)mechanism.Stable mode-locking is attained by synergistically controlling gain,polarization state,and optical path length in two symmetric sub-cavities.Experiments proved that repetition rate of the sub-cavities can be adjusted via the time delay line(TDL)to achieve synchronized mode-locking.The system stably generates multi-wavelength pulses at a single repetition frequency,evidenced by multiple spectral peaks and equidistant pulse sequences.These findings facilitate the development of high-performance multi-wavelength ultrashort pulse sources,crucial for optical communications,spectral analysis,and remote sensing.展开更多
A dual-phase synergistic enhancement method was adopted to strengthen the Al-Mn-Mg-Sc-Zr alloy fabricated by laser powder bed fusion(LPBF)by leveraging the unique advantages of Er and TiB_(2).Spherical powders of 0.5w...A dual-phase synergistic enhancement method was adopted to strengthen the Al-Mn-Mg-Sc-Zr alloy fabricated by laser powder bed fusion(LPBF)by leveraging the unique advantages of Er and TiB_(2).Spherical powders of 0.5wt%Er-1wt%TiB_(2)/Al-Mn-Mg-Sc-Zr nanocomposite were prepared using vacuum homogenization technique,and the density of samples prepared through the LPBF process reached 99.8%.The strengthening and toughening mechanisms of Er-TiB_(2)were investigated.The results show that Al_(3)Er diffraction peaks are detected by X-ray diffraction analysis,and texture strength decreases according to electron backscatter diffraction results.The added Er and TiB_(2)nano-reinforcing phases act as heterogeneous nucleation sites during the LPBF forming process,hindering grain growth and effectively refining the grains.After incorporating the Er-TiB_(2)dual-phase nano-reinforcing phases,the tensile strength and elongation at break of the LPBF-deposited samples reach 550 MPa and 18.7%,which are 13.4%and 26.4%higher than those of the matrix material,respectively.展开更多
Quasi-two-dimensional(quasi-2d)perovskites are promising gain media for micro-nano lasers,yet their uncontrolled crystallization and abundant low-n phases often hinder optical gain and device performance.In this work,...Quasi-two-dimensional(quasi-2d)perovskites are promising gain media for micro-nano lasers,yet their uncontrolled crystallization and abundant low-n phases often hinder optical gain and device performance.In this work,we introduce ethyl acetate(EA)as a green antisolvent to fabricate high-quality quasi-2D PEA_(0.4)MAPbBr_(3)films.The EA-treated films exhibit superior morphology,enhanced crystallinity,and notably inhibited low n-phases.These improvements yield a prolonged photoluminescence lifetime of 26.3 ns and a substantially extended gain lifetime of 129 ps.Consequently,the optimized film exhibits a markedly reduced amplified spontaneous emission(ASE)threshold of 5.6μJ·cm^(-2)and a high net modal gain of 935 cm^(-1).Leveraging these enhanced gain properties,we successfully demonstrate a vertical-cavity surface-emitting laser(VCSEL)based on a dielectric Bragg reflector microcavity,which delivers single-mode lasing at 528.3 nm and a high quality factor of~5886.This work presents a green-solvent-engineering strategy for high-performance perovskite lasers,advancing their prospects for scalable photonic integration.展开更多
To explore the formation mechanism of anisotropy in Ti-6Al-4V alloy fabricated by selective laser melting(SLM),the compressive mechanical properties,microhardness,microstructure,and crystallographic orientation of the...To explore the formation mechanism of anisotropy in Ti-6Al-4V alloy fabricated by selective laser melting(SLM),the compressive mechanical properties,microhardness,microstructure,and crystallographic orientation of the alloy across different planes were investigated.The anisotropy of SLM-fabricated Ti-6Al-4V alloys was analyzed,and the electron backscatter diffraction technique was used to investigate the influence of different grain types and orientations on the stress-strain distribution at various scales.Results reveal that in room-temperature compression tests at a strain rate of 10^(-3) s^(-1),both the compressive yield strength and microhardness vary along the deposition direction,indicating a certain degree of mechanical property anisotropy.The alloy exhibits a columnar microstructure;along the deposition direction,the grains appear equiaxed,and they have internal hexagonal close-packed(hcp)α/α'martensitic structure.α'phase has a preferential orientation approximately along the<0001>direction.Anisotropy arises from the high aspect ratio of columnar grains,along with the weak texture of the microstructure and low symmetry of the hcp crystal structure.展开更多
文摘Conventional ignition methods are proving to be ineffective for low-sensitivity energetic materials,highlighting the need to investigate alternative ignition systems,such as laser-based techniques.Over the past decade,lasers have emerged as a promising solution,providing focused energy beams for controllable,efficient,and reliable ignition in the field of energetic materials.This study presents a comparative analysis of two state-of-the-art ignition approaches:direct laser ignition and laser-driven flyer ignition.Experiments were performed using a Neodymium-doped Yttrium Aluminum Garnet(Nd:YAG)laser at different energy beam levels to systematically evaluate ignition onset.In the direct laser ignition test setup,the laser beam was applied directly to the energetic tested material,while laserdriven flyer ignition utilized 40 and 100μm aluminum foils,propelled at velocities ranging from 300 to 1250 m/s.Comparative analysis with the Lawrence and Trott model substantiated the velocity data and provided insight into the ignition mechanisms.Experimental results indicate that the ignition time for the laser-driven flyer method was significantly shorter,with the pyrotechnic composition achieving complete combustion faster compared to direct laser ignition.Moreover,precise ignition thresholds were determined for both methods,providing critical parameters for optimizing ignition systems in energetic materials.This work elucidates the advantages and limitations of each technique while advancing next-generation ignition technology,enhancing the reliability and safety of propulsion systems.
基金supported by National Key R&D Program of China(Grant Nos.2021YFB2802000 and 2022YFB2804300)Science and Technology Commission of Shanghai Municipality(Grant No.21DZ1100500)+3 种基金Shanghai Municipal Science and Technology Major Projectthe Shanghai Frontiers Science Center Program(2021-2025 No.20)National Natural Science Foundation of China(Grant No.61975123)Shanghai Scienceand Technology Innovation Action Plan(Grant No.23JC1403100)。
文摘Able to precisely control and manipulate materials'states at micro/nano-scale level,femtosecond(fs)laser micro/nano processing technology has undergone tremendous development over the past three decades.Free-forming three-dimensional(3D)microscale functional devices and inducing fascinating and unique physical or chemical phenomena have granted this technology powerful versatility that no other technology can match.As this technology advances rapidly in various fields of application,some key challenges have emerged and remain to be urgently addressed.This review firstly introduces the fundamental principles for understanding how fs laser pulses interact with materials and the associated unique phenomena in section 2.Then micro/nano-fabrication in transparent materials by fs laser processing is presented in section 3.Thereafter,several high efficiency/throughput fabrication methods as well as pulse-shaping techniques are listed in sections 4 and 5 reviews four-dimensional(4D)and nanoscale printing realized by fs laser processing technology.Special attention is paid to the heterogeneous integration(HI)of functional materials enabled by fs laser processing in section 6.Several intriguing examples of 3D functional micro-devices created by fs laser-based manufacturing methods such as microfluidics,lab-on-chip,micro-optics,micro-mechanics,micro-electronics,micro-bots and micro-biodevices are reviewed in section 7.Finally,a summary of the review and a perspective are proposed to explore the challenges and future opportunities for further betterment of fs laser micro/nano processing technology.
文摘AIM:To assess the effectiveness and safety of VISULAS®green laser selective laser trabeculoplasty(SLT)in lowering intraocular pressure(IOP)in patients with pseudoexfoliative syndrome glaucoma(PEXG)and pseudoexfoliative syndrome ocular hypertension(PEXS-OHT).METHODS:This prospective,single-center,interventional study included 20 eyes from 20 patients diagnosed with PEXG or PEXS-OHT.Patients underwent 180°SLT using the VISULAS®green laser,a diode-pumped,frequencydoubled Nd:YVO4 laser with a 532 nm wavelength.IOP was measured at baseline and post-treatment at 1,3,and 6mo.Medications regimen was stable through the study.Primary outcomes included mean IOP reduction,while secondary outcomes assessed visual and structural parameters,and safety.RESULTS:The mean age of participants was 72.2±6.6y,with 65%of the eyes being left eyes and 35%right eyes.At baseline,the mean IOP was 22.9±2.9 mm Hg.A significant reduction in IOP was observed at all follow-up intervals:18.5±3.1 mm Hg at 1mo(18.8%reduction,P=0.001),19.0±4.2 mm Hg at 3mo(16.7%reduction,P=0.002),and 18.2±4.5 mm Hg at 6mo(19.8%reduction,P=0.001).Subgroup analysis showed greater IOP reduction in patients with Shaffer grade 4 angles,phakic eyes,and those with PEXS-OHT compared to PEXG.No significant changes were detected in visual acuity,visual field index,mean deviation,or retinal nerve fiber layer thickness.At 1h post-procedure,20%of eyes showed an IOP spike>5 mm Hg that resolved without intervention except for one patient.CONCLUSION:SLT with the VISULAS®green laser is an effective and safe treatment for PEXG and PEXS-OHT,achieving significant IOP reduction without increasing medication burden or causing severe complications.These findings suggest its potential as an alternative or adjunct therapy in managing pseudoexfoliative glaucoma.
基金supported by the National Natural Science Foundation of China(Grant Nos.11804348,11775056,11975154,12225505,and 12405281)the Science Challenge(Project No.TZ2018005)+2 种基金supported by the Shanghai Pujiang Program(Grant No.23PJ1414600)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0890203)supported by the Accelerator Technology Helmholtz Infrastructure consortium ATHENA.
文摘The effects of initial spin orientation on the final electron beam polarization in laser wakefield acceleration in a pre-polarized plasma are investigated theoretically and numerically.From the results of variation of the initial spin direction,the spin dynamics of the electron beam are found to depend on the self-injection mechanism.The effects of wakefields and laser fields are studied using test particle dynamics and particle-in-cell simulations based on the Thomas-Bargmann-Michel-Telegdi equation.Compared with transverse injection,longitudinal injection is found to be preferable for obtaining a highly polarized electron beam.
基金supported by the National Natural Science Foundation of China(No.51871243)the National Key Laboratory of Strength and Structural Integrity,China(No.ASSIKFJJ202304001)+3 种基金the State Key Laboratory of Precision Blasting and Hubei Key Laboratory of Blasting Engineering,China(No.PBSKL2022C01)the Guangdong-Hong Kong-Macao Joint Laboratory for Neutron Scattering Science and Technology,China(No.HT-CSNS-DG-CD-0092/2021)the Shock and Vibration of Engineering Materials and Structures Key Laboratory of Sichuan Province,China(No.22kfgk06)the Hubei Longzhong Laboratory,China(No.2022KF-08)。
文摘Laser remelting(LR)was used as an auxiliary post-treatment process for the Ti6Al4V titanium alloys fabricated by laser powder bed fusion(LPBF).Optical microscope(OM),scanning electron microscope(SEM)and electron back scattering diffraction(EBSD)observations showed that the grains in melted zone(MZ)transformed into equiaxial grains with an average size of 1.31μm,and the grains in heat affected zone(HAZ)were refined.Moreover,the texture intensity dropped significantly from 13.86 to 6.35 in MZ and 10.79 in HAZ.The temperature gradient(G)to solidification rate(R)ratio decreased when the laser scanning speed slowed down to a certain extent in the LR process,which effectively improved the highly preferred orientation and filled the hole defects in the surface of LPBF-Ti6Al4V.Furthermore,the hardness,wear resistance and corrosion resistance of the surface of the LPBF samples were improved by LR treatment.
文摘The original online version of this article was revised:Several errors occurred in the published version of the article.These have now been corrected as follows:Page 2,section"2.2 Laser Texturing Procedure of Surfaces",line 2:The device name was corrected from"YDFLP-E-50-M8"to"YDFLP-50-M8."Page 3,Section 2.4:The phrase"95%confidence interval"has been corrected to"95%confidence level."Page 3,Figure 1 caption:The phrase"fandg"has been corrected to"f and g."The order"C4 and C12"has been reversed to"C12 and C4,"in accordance with the display order in the figure.Page 4,Figure reference:The phrase"Figs.4c and d"has been corrected to"Figs.5b and c."Page 5,paragraph starting with"The ANOVA results are presented...":The phrase"95%confidence interval"has been corrected to"95%confidence level."
基金supported by the National Natural Science Foundation of China(Grant Nos.62450006,62304217,62274157,62127807,62234011,62034008,62074142,62074140)Tianshan Innovation Team Program(Grant No.2022TSYCTD0005)+1 种基金Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDB0880000)Youth Innovation Promotion Association of the Chinese Academy of Sciences(Grant Nos.2023124,Y2023032)。
文摘The 193 nm deep-ultraviolet(DUV)laser plays a critical role in advanced semiconductor chip manufacturing[1,2],micro-nano material characterization[3,4]and biomedical analysis[5,6],due to its high spatial resolution and short wavelength.Efficient and compact 193 nm DUV laser source thus becomes a hot research area.Currently,193 nm Ar F excimer gas laser is widely employed in DUV lithography systems and serves as the enabling technology for 7 and 5 nm semiconductor fabrication.
基金funding from Grant No. HIDSS-0002 DASHH (Data Science in Hamburg-Helmholtz Graduate School for the Structure of Matter)partially supported by the Helmholtz Imaging platform through the project “Smart Phase.”
文摘Understanding the complex plasma dynamics in ultra-intense relativistic laser-solid interactions is of fundamental importance for applications of laser-plasma-based particle accelerators,the creation of high-energy-density matter,understanding planetary science,and laser-driven fusion energy.However,experimental efforts in this regime have been limited by the lack of accessibility of over-critical densities and the poor spatiotemporal resolution of conventional diagnostics.Over the last decade,the advent of femtosecond brilliant hard X-ray free-electron lasers(XFELs)has opened new horizons to overcome these limitations.Here,for the first time,we present full-scale spatiotemporal measurements of solid-density plasma dynamics,including preplasma generation with tens of nanometer scale length driven by the leading edge of a relativistic laser pulse,ultrafast heating and ionization at the main pulse arrival,the laser-driven blast wave,and transient surface return current-induced compression dynamics up to hundreds of picoseconds after interaction.These observations are enabled by utilizing a novel combination of advanced X-ray diagnostics including small-angle X-ray scattering,resonant X-ray emission spectroscopy,and propagation-based X-ray phase-contrast imaging simultaneously at the European XFEL-HED beamline station.
基金supported by Independent Innovation Science Foundation of National University of Defense Technology(Grant No.23-ZZCX-JDZ-44)。
文摘Tunable mid-infrared and far-infrared laser output was demonstrated based on BaGa_(4)Se_(7)crystals and an optical parametric oscillator(OPO).With a 1.06μm Nd:YAG laser and a double-pass singly resonant OPO cavity,a laser energy output of 2.2 mJ at 10μm was obtained.By tuning the angle and temperature,a tunable laser output covering the wavelength range from 6μm to 17μm was obtained with a tuning precision better than 3 nm.The corresponding optical-to-optical conversion efficiency was 2.8%,and the slope efficiency was 4.4%.The damage effect of the output laser on detectors was also investigated,and point damage to the detector occurred at an output energy of 16.4μJ.The laser system has the advantages of miniaturization,a wide tuning range,high energy and high tuning resolution.Its broadband laser characteristics make it highly valuable for applications in atmospheric detection,infrared spectroscopy and electro-optical countermeasures.
基金supported by Russian Science Foundation Grant No.24-62-00032.
文摘Experiments with interacting high-velocity flows in a laser plasma can help answer fundamental questions in plasma physics and improve understanding of the mechanisms behind some astrophysical phenomena,such as the formation of collisionless shock waves,deceleration of accretion flows,and evolution of solar and stellar flares.This work presents the first direct experimental observations of stagnation and redirection of counterstreaming flows(jets)of laser plasma induced by intense laser pulses with intensity I~2×10^(18) W/cm^(2).Hybrid particlein-cell-fluid modeling,which takes into account the kinetic effects of ion motion and the evolution of the pressure tensor for electrons,demonstrates the compression of counterdirected toroidal self-generated magnetic fields embedded in counterstreaming plasma flows.The enhancement of the toroidal magnetic field in the interaction region results in plasma flow stagnation and redirection of the jets across the line of their initial propagation.
基金Project supported by the National Natural Science Foundation of China(Grant Nos.61975141,61575137,and61675144)。
文摘We investigate theoretically and experimentally the chaotic dynamics of visible-wavelength all-fiber ring laser.The100-m 630 HP fibers are used to ensure high non-linearity.A 4-m Pr^(3+)/Yb^(3+)-co-doped ZBLAN fiber provides the gain.The chaotic laser was pumped by the laser diodes with the maximum power of 150 mW at the wavelength of 850 nm.The peak fluorescence spectrum of Pr^(3+)/Yb^(3+)-co-doped ZBLAN fiber at the wavelength of 635 nm shows that the visiblewavelength fiber laser can be achieved by synergistic energy transfer between Pr~(3+)and Yb^(3+)ions.The chaotic fiber laser is generated by adjusting the pump power,polarization controller and the auto-correlation,permutation entropy,skewness,and kurtosis were used to analyze the characteristics of chaotic laser.The noise-like time series and delta-like auto-correlation curve indicate the chaotic output.The complexity and randomness of time series are analyzed by the permutation entropy,skewness,and kurtosis.The result shows that chaotic dynamics is stable when the pump power exceeds a certain value.The visible chaotic all-fiber laser has high stability and can be applied for real-time monitoring and sensing.We believe that this approach may also be feasible for other materials for emission in the visible range.
基金supported by the National Natural Science Foundation of China(Grant Nos.U2032136 and U2241288)the Shaanxi Fundamental Science Research Project for Mathematics and Physics(Grant No.23JSY012)。
文摘We present a solid 226 nm deep ultraviolet laser system pumped by a Nd:YAG laser.A diamond Raman laser with a 1485 nm wavelength was generated up to 2.53 mJ pumped by a 9.7 mJ 1064 nm laser,which is the highest pulse energy of a second Stokes diamond Raman laser pumped by a 1064 nm laser as we know.Then,the Raman laser is mixed with the frequency-quadrupled 1064 nm laser to produce the 226 nm laser.The maximum output pulse energy at 226 nm reaches 0.49 mJ.The overall conversion efficiency from1064 to 226 nm is up to 1.14%,which is significantly higher than conventional optical parametric oscillator technology for the generation of 226 nm laser.The 226 nm laser system has been used in a laser-induced fluorescence(LIF)experiment of oxygen two-photon to demonstrate its potential for LIF measurements.
基金supported by the National Natural Science Foundation of China(NSFC)(Nos.12074399,12204500,and 12004403)the Key Projects of Intergovernmental International Scientific and Technological Innovation Cooperation(No.2021YFE0116700)+1 种基金the Shanghai Natural Science Foundation(No.20ZR1464400)the Shanghai Sailing Program(No.22YF1455300).
文摘The suppression of ablative Rayleigh–Taylor instability(ARTI)by a spatially modulated laser in inertial confinement fusion(ICF)is studied through numerical simulations.The results show that in the acceleration phase of ICF implosion,the growth of ARTI can be suppressed by using a short-wavelength spatially modulated laser.The ARTI growth rate decreases as the wavelength of the spatially modulated laser decreases,and ARTI is completely suppressed after a certain wavelength has been reached.A spatially uniform laser is introduced to keep the state of motion of the implosion fluid consistent,and it is found that the proportion of the spatially modulated laser required for complete suppression of ARTI decreases as the wavelength continues to decrease.We also optimize the spatial intensity distribution of the spatially modulated laser.In addition,as the duration of the spatially modulated laser decreases,the proportion required for completely suppressing ARTI increases,but the required energy decreases.When the perturbation wavenumber decreases,the wavelength of the spatially modulated laser required for complete suppression of ARTI becomes longer.In the case of multimode perturbation,ARTI can also be significantly suppressed by a spatially modulated laser,and the perturbation amplitude can be reduced to less than 10% of that without a spatially modulated laser.We believe that the conclusions drawn from our simulations can provide the basis for new approaches to control ARTI in ICF.
基金financial support from the China Scholarship Council(No.202108220036)Advanced Microscopy Laboratory in Trinity College Dublin。
文摘Additive and solvent-free direct printing is critical for many applications,including smart electronics,solar cells,healthcare,and electrochemical energy storage.Although a few green techniques for direct patterning of inorganic functional materials have been developed,they operate at small scale and require long processing times,restricting their effective translation from laboratory to market.Here we report a fast,liquid-free,cost-effective,and environmentally friendly aerosol-based printing method for fabricating linear or planar structures at microscale dimensions.In situ and on-demand generation of dry aerosol via pulsed laser ablation,coupled with real-time aerodynamical focusing using a co-flowing sheath gas,allows the deposition of a wide variety of materials on various substrates at room temperature and atmospheric pressure.Using silver as a test material,we systematically characterized the laser-generated aerosol deposits in terms of microstructural morphology,sintering activity,mass yield,density,and electrical performance,to show the relationship between process variability and underlying mechanisms.The capacity of high-throughput printing of silver deposits,with thickness up to 160μm,in a single pass was demonstrated.This rapid,efficient,and inkless printing process opens new and exciting opportunities for future applications that require easy-to-integrate components in printed electronic devices.
基金supported by the National Natural Science Foundation of China(Nos.12027809,12350007)National Key R&D Program of China(Nos.2022YFA1605100,2023YFA1606403,and 2023YFE0101600)+1 种基金New Cornerstone Science Foundation through the XPLORER PRIZEfunding from the European Research Council(ERC)under the European Union’s Horizon 2020 research and innovation program under grant agreement No.679038.
文摘A RadioFrequency Quadrupole(RFQ)cooler-buncher system was developed and implemented in a collinear laser spectroscopy setup.This system converts a continuous ion beam into short bunches while enhancing the beam quality and reducing the energy spread.The functionality of the RFQ cooler buncher was verified through offline tests with stable rubidium and indium beams delivered from a surface ion source and a laser ablation ion source,respectively.Bunched ion beams with a full width at half maximum of approximately 2μs in the time-of-flight spectrum were successfully achieved with a transmission efficiency exceeding 60%.The implementation of the RFQ cooler-buncher system also significantly improved the overall transmission efficiency of the collinear laser spectroscopy setup.
基金China“Ye Qisun”Science Foundation Project of National Natural Science Foundation(U2141222)Innovation Fund(8F231527Z)。
文摘The combustion behavior of Ti-Al-Mo-Zr-Sn-W alloy(TC25G)was studied in a high-temperature and high-speed air flow environment using the laser ignition method combined with ultra-high temperature infrared thermometer,scanning electron microscope,X-ray diffractometer,and transmission electron microscope.The burn-resistant performance of TC25G and TC11 alloys was compared.Meanwhile,the microstructural characteristics,crystal structure,and formation mechanism of the combustion products of TC25G alloy were analyzed in detail.The results show that the high-temperature and high-speed air flow promotes combustion within the air flow temperature range of 200–400℃and the air flow velocity range of 0–100 m/s.The combustion path advances along the direction of the air flow.The combustion of TC25G alloy mainly relies on the diffusion of the oxygen and the expansion of the combustion area caused by the movement of the melt.Based on the microstructure and composition of combustion product,it can be divided into the combustion zone,the melting zone,and the heat affected zone.During combustion,the formation of microstructures is closely correlated with the behavior of alloying elements and their selective combination with O.The major oxidation products of Ti are TiO and TiO_(2).The oxides formed by Mo and W hinder the movement of the melt during the combustion.Al and Zr tend to undergo internal oxidation.Al_(2)O_(3)precipitates on the surface of ZrO_(2),forming a protective oxide layer that inhibits the inward diffusion of O.Moreover,the element enrichment at the interface between the melting zone and the heat affected zone increases the melting point on the solid side,hindering the migration of the solid-liquid interface.
文摘We designed and investigated a passive synchronized mode-locked fiber laser.The device utilizes a dual-cavity structure driven by the nonlinear polarization rotation(NPR)mechanism.Stable mode-locking is attained by synergistically controlling gain,polarization state,and optical path length in two symmetric sub-cavities.Experiments proved that repetition rate of the sub-cavities can be adjusted via the time delay line(TDL)to achieve synchronized mode-locking.The system stably generates multi-wavelength pulses at a single repetition frequency,evidenced by multiple spectral peaks and equidistant pulse sequences.These findings facilitate the development of high-performance multi-wavelength ultrashort pulse sources,crucial for optical communications,spectral analysis,and remote sensing.
基金Shaanxi Province Qin Chuangyuan“Scientist+Engineer”Team Construction Project(2022KXJ-071)2022 Qin Chuangyuan Achievement Transformation Incubation Capacity Improvement Project(2022JH-ZHFHTS-0012)+8 种基金Shaanxi Province Key Research and Development Plan-“Two Chains”Integration Key Project-Qin Chuangyuan General Window Industrial Cluster Project(2023QCY-LL-02)Xixian New Area Science and Technology Plan(2022-YXYJ-003,2022-XXCY-010)2024 Scientific Research Project of Shaanxi National Defense Industry Vocational and Technical College(Gfy24-07)Shaanxi Vocational and Technical Education Association 2024 Vocational Education Teaching Reform Research Topic(2024SZX354)National Natural Science Foundation of China(U24A20115)2024 Shaanxi Provincial Education Department Service Local Special Scientific Research Program Project-Industrialization Cultivation Project(24JC005,24JC063)Shaanxi Province“14th Five-Year Plan”Education Science Plan,2024 Project(SGH24Y3181)National Key Research and Development Program of China(2023YFB4606400)Longmen Laboratory Frontier Exploration Topics Project(LMQYTSKT003)。
文摘A dual-phase synergistic enhancement method was adopted to strengthen the Al-Mn-Mg-Sc-Zr alloy fabricated by laser powder bed fusion(LPBF)by leveraging the unique advantages of Er and TiB_(2).Spherical powders of 0.5wt%Er-1wt%TiB_(2)/Al-Mn-Mg-Sc-Zr nanocomposite were prepared using vacuum homogenization technique,and the density of samples prepared through the LPBF process reached 99.8%.The strengthening and toughening mechanisms of Er-TiB_(2)were investigated.The results show that Al_(3)Er diffraction peaks are detected by X-ray diffraction analysis,and texture strength decreases according to electron backscatter diffraction results.The added Er and TiB_(2)nano-reinforcing phases act as heterogeneous nucleation sites during the LPBF forming process,hindering grain growth and effectively refining the grains.After incorporating the Er-TiB_(2)dual-phase nano-reinforcing phases,the tensile strength and elongation at break of the LPBF-deposited samples reach 550 MPa and 18.7%,which are 13.4%and 26.4%higher than those of the matrix material,respectively.
文摘Quasi-two-dimensional(quasi-2d)perovskites are promising gain media for micro-nano lasers,yet their uncontrolled crystallization and abundant low-n phases often hinder optical gain and device performance.In this work,we introduce ethyl acetate(EA)as a green antisolvent to fabricate high-quality quasi-2D PEA_(0.4)MAPbBr_(3)films.The EA-treated films exhibit superior morphology,enhanced crystallinity,and notably inhibited low n-phases.These improvements yield a prolonged photoluminescence lifetime of 26.3 ns and a substantially extended gain lifetime of 129 ps.Consequently,the optimized film exhibits a markedly reduced amplified spontaneous emission(ASE)threshold of 5.6μJ·cm^(-2)and a high net modal gain of 935 cm^(-1).Leveraging these enhanced gain properties,we successfully demonstrate a vertical-cavity surface-emitting laser(VCSEL)based on a dielectric Bragg reflector microcavity,which delivers single-mode lasing at 528.3 nm and a high quality factor of~5886.This work presents a green-solvent-engineering strategy for high-performance perovskite lasers,advancing their prospects for scalable photonic integration.
基金National Natural Science Foundation of China(51504138,51674118,52271177)Hunan Provincial Natural Science Foundation of China(2023JJ50181)Supported by State Key Laboratory of Materials Processing and Die&Mould Technology,Huazhong University of Science and Technology(P2024-022)。
文摘To explore the formation mechanism of anisotropy in Ti-6Al-4V alloy fabricated by selective laser melting(SLM),the compressive mechanical properties,microhardness,microstructure,and crystallographic orientation of the alloy across different planes were investigated.The anisotropy of SLM-fabricated Ti-6Al-4V alloys was analyzed,and the electron backscatter diffraction technique was used to investigate the influence of different grain types and orientations on the stress-strain distribution at various scales.Results reveal that in room-temperature compression tests at a strain rate of 10^(-3) s^(-1),both the compressive yield strength and microhardness vary along the deposition direction,indicating a certain degree of mechanical property anisotropy.The alloy exhibits a columnar microstructure;along the deposition direction,the grains appear equiaxed,and they have internal hexagonal close-packed(hcp)α/α'martensitic structure.α'phase has a preferential orientation approximately along the<0001>direction.Anisotropy arises from the high aspect ratio of columnar grains,along with the weak texture of the microstructure and low symmetry of the hcp crystal structure.
