As an emerging member of the two-dimensional(2D)material family,V_(2)CT_(X)MXene shows great potential in the application of lithium-ion capacitors(LICs)due to its unique structure and excellent electrical conductivit...As an emerging member of the two-dimensional(2D)material family,V_(2)CT_(X)MXene shows great potential in the application of lithium-ion capacitors(LICs)due to its unique structure and excellent electrical conductivity.However,severe nanosheets stacking and intra-layer transport barriers have limited the further development of V_(2)CT_(X)MXene-based materials.Herein,we prepared Kions and–O functional group co-modified V_(2)CT_(X)MXene(VCT-K)and further incorporated it with single-walled carbon nanotube(SWCNT),obtaining freestanding V_(2)CT_(X)composite films(VCT-K@C)with the 3D conductive network.Significantly,K+ions were introduced into V_(2)CT_(X)MXene to stabilize the interlayer structure and prevent the aggregation of nanosheets,the terminal group of–O was controllably modified on the surface of MXene to improve the Li+ions storage reversible capacities and the SWCNT acted as the bridge between MXene nanosheets to opens up the channels for ion/electron transportation in the longitudinal direction.Benefited from the synergistic effect of VCT-K and SWCNT,the VCT-K@C exhibits superior reversible specific capacities of 671.8 mA h g^(-1)at 0.1 A g^(-1)and 318 mA h g^(-1)at 1.0 A g^(-1).Furthermore,the assembled LICs with VCT-K@C anode coupling activated carbon(AC)cathode deliver an outstanding power density of 19.0 kW kg^(-1)at 67.4 Wh kg^(-1),a high energy density of 140.5 Wh kg^(-1)at 94.8 W kg^(-1)and a stable capacitance retention of 86%after 6000 cycles at 10 A g^(-1).Such unique structures and excellent electrochemical properties are expected to pave the way for the large-scale application in LICs of MXene-based materials.展开更多
Twist,the very degree of freedom in van der Waals heterostructures,offers a compelling avenue to manipulate and tailor their electrical and optical characteristics.In particular,moirépatterns in twisted homobilay...Twist,the very degree of freedom in van der Waals heterostructures,offers a compelling avenue to manipulate and tailor their electrical and optical characteristics.In particular,moirépatterns in twisted homobilayer transition metal dichalcogenides(TMDs)lead to zone folding and miniband formation in the resulting electronic bands,holding the promise to exhibit inter-layer excitonic optical phenomena.Although some experiments have shown the existence of twist-angle-dependent intra-and inter-layer excitons in twisted MoSe2 homobilayers,electrical control of the interlayer excitons in MoSe_(2) is relatively under-explored.Here,we show the signatures of the moiréeffect on intralayer and interlayer excitons in 2H-stacked twisted MoSe2 homobilayers.Doping-and electric field-dependent photoluminescence mea-surements at low temperatures give evidence of the momentum-direct K-K intralayer excitons,and the momentum-indirect Г-K and Г-Q interlayer excitons.Our results suggest that twisted MoSe_(2) homobilayers are an intriguing platform for engineering interlayer exciton states,which may shed light on future atomically thin optoelectronic applications.展开更多
Dear editor,As of 2023,the domestic cat population in China reached 65 million,surpassing dogs to become the most numerous companion animal in the country.Feline calicivirus(FCV)infection,one of the three most prevale...Dear editor,As of 2023,the domestic cat population in China reached 65 million,surpassing dogs to become the most numerous companion animal in the country.Feline calicivirus(FCV)infection,one of the three most prevalent infectious diseases in cats,poses a severe threat to feline health.FCV,classified under the Caliciviridae family(genus Vesivirus).展开更多
Preterm birth and suboptimal fetal growth remain significant perinatal challenges worldwide.Recent data indicate that China's perinatal profile has improved due to reductions in preterm birth rates.However,the cou...Preterm birth and suboptimal fetal growth remain significant perinatal challenges worldwide.Recent data indicate that China's perinatal profile has improved due to reductions in preterm birth rates.However,the country has a 6.5%prevalence of small-for-gestational-age(SGA),ranking fifth globally in total SGA birth numbers^([1,2]).展开更多
Increasing the number of atoms that interact with microwave fields represents a promising strategy for enhancing the sensitivity of Rydberg atom-based superheterodyne receivers.Nevertheless,the practical implementatio...Increasing the number of atoms that interact with microwave fields represents a promising strategy for enhancing the sensitivity of Rydberg atom-based superheterodyne receivers.Nevertheless,the practical implementation of this approach is impeded by adverse effects such as excitation saturation of Rydberg atoms and power broadening.Here,we demonstrate enhanced microwave field measurements based on two specific velocity groups of atoms,simultaneously addressed by dual-channel probe beams in a Sagnac loop interferometer.The application of resonance detuning in two-photon excitation enables selective addressing of atoms moving along the beam direction,thereby significantly mitigating atomic transit noise.At 7.97 GHz,our method yields a 3 dB improvement in signal-to-noise ratio(SNR),achieving a sensitivity of 10.7 nV·cm^(−1)·Hz^(−1/2).This approach offers a viable pathway to further improve the sensitivity of Rydberg atom-based microwave electrometers.展开更多
Accessible communication based on sign language recognition(SLR)is the key to emergency medical assistance for the hearing-impaired community.Balancing the capture of both local and global information in SLR for emerg...Accessible communication based on sign language recognition(SLR)is the key to emergency medical assistance for the hearing-impaired community.Balancing the capture of both local and global information in SLR for emergency medicine poses a significant challenge.To address this,we propose a novel approach based on the inter-learning of visual features between global and local information.Specifically,our method enhances the perception capabilities of the visual feature extractor by strategically leveraging the strengths of convolutional neural network(CNN),which are adept at capturing local features,and visual transformers which perform well at perceiving global features.Furthermore,to mitigate the issue of overfitting caused by the limited availability of sign language data for emergency medical applications,we introduce an enhanced short temporal module for data augmentation through additional subsequences.Experimental results on three publicly available sign language datasets demonstrate the efficacy of the proposed approach.展开更多
Genetic relationships of eight species of genus Betula were evaluated using ISSR marks. A total of 236 loci were generated from 17 ISSR primers. Percentage of polymorphic bands (PPB) varied from 5.93 to 19.92. The hig...Genetic relationships of eight species of genus Betula were evaluated using ISSR marks. A total of 236 loci were generated from 17 ISSR primers. Percentage of polymorphic bands (PPB) varied from 5.93 to 19.92. The highest and the lowest level of genetic differentiation were detected in B. ovalifolia and B. maximowicziana Regel respectively. In these eight species, genetic diversity of birch (HT) was 24.38 %, and the genetic variation (GST ) interspecies was accounting for 79.36% of total genetic variation. According to the cluster results of genetic distance, the eight species were classified into three groups as B. davurica, B. ovalifolia, B. platyphylla and B. pendula for one group; B. schmidtii, B. costata and B. ermanii Cham. var. communis for one group, and B. maximowicziana Regel for another group. The result of cluster is consistent with traditional morphological classification.展开更多
基金funded by the National Natural Science Foundation of China(Grant Nos.22005167 and 21905152)the Shandong Provincial Natural Science Foundation of China(Grant Nos.ZR2020QB125 and ZR2020MB045)+1 种基金the China Postdoctoral Science Foundation(Grant Nos.2021M693256,2021T140687 and 2022M713249)the Qingdao Postdoctoral Applied Research Project and the Youth Innovation Team Project for Talent Introduction and Cultivation in Universities of Shandong Province。
文摘As an emerging member of the two-dimensional(2D)material family,V_(2)CT_(X)MXene shows great potential in the application of lithium-ion capacitors(LICs)due to its unique structure and excellent electrical conductivity.However,severe nanosheets stacking and intra-layer transport barriers have limited the further development of V_(2)CT_(X)MXene-based materials.Herein,we prepared Kions and–O functional group co-modified V_(2)CT_(X)MXene(VCT-K)and further incorporated it with single-walled carbon nanotube(SWCNT),obtaining freestanding V_(2)CT_(X)composite films(VCT-K@C)with the 3D conductive network.Significantly,K+ions were introduced into V_(2)CT_(X)MXene to stabilize the interlayer structure and prevent the aggregation of nanosheets,the terminal group of–O was controllably modified on the surface of MXene to improve the Li+ions storage reversible capacities and the SWCNT acted as the bridge between MXene nanosheets to opens up the channels for ion/electron transportation in the longitudinal direction.Benefited from the synergistic effect of VCT-K and SWCNT,the VCT-K@C exhibits superior reversible specific capacities of 671.8 mA h g^(-1)at 0.1 A g^(-1)and 318 mA h g^(-1)at 1.0 A g^(-1).Furthermore,the assembled LICs with VCT-K@C anode coupling activated carbon(AC)cathode deliver an outstanding power density of 19.0 kW kg^(-1)at 67.4 Wh kg^(-1),a high energy density of 140.5 Wh kg^(-1)at 94.8 W kg^(-1)and a stable capacitance retention of 86%after 6000 cycles at 10 A g^(-1).Such unique structures and excellent electrochemical properties are expected to pave the way for the large-scale application in LICs of MXene-based materials.
基金supported by the National Key R&D Program of China(No.2023YFF1500600)the National Natural Science Foun-dation of China(Nos.12004259,12204287)+3 种基金China Postdoc-toral Science Foundation(Grant No.2022M723215)Zheng Vitto Han acknowledges the support of the Fund for Shanxi“1331 Project”Key Subjects Construction,and the Innovation Program for Quantum Science and Technology(Grant No.2021ZD0302003)Kenji Watanabe and Takashi Taniguchi acknowledge support from the JSPS KAKENHI(Grant Nos.20H00354 and 23H02052)the World Premier International Research Center Initiative(WPI),MEXT,Japan.
文摘Twist,the very degree of freedom in van der Waals heterostructures,offers a compelling avenue to manipulate and tailor their electrical and optical characteristics.In particular,moirépatterns in twisted homobilayer transition metal dichalcogenides(TMDs)lead to zone folding and miniband formation in the resulting electronic bands,holding the promise to exhibit inter-layer excitonic optical phenomena.Although some experiments have shown the existence of twist-angle-dependent intra-and inter-layer excitons in twisted MoSe2 homobilayers,electrical control of the interlayer excitons in MoSe_(2) is relatively under-explored.Here,we show the signatures of the moiréeffect on intralayer and interlayer excitons in 2H-stacked twisted MoSe2 homobilayers.Doping-and electric field-dependent photoluminescence mea-surements at low temperatures give evidence of the momentum-direct K-K intralayer excitons,and the momentum-indirect Г-K and Г-Q interlayer excitons.Our results suggest that twisted MoSe_(2) homobilayers are an intriguing platform for engineering interlayer exciton states,which may shed light on future atomically thin optoelectronic applications.
基金supported by grants from the National Key Research and Development Program of China(Grant No.2022YFD1800100)National Natural Science Foundation of China(Grant No.32272982)Natural Science Foundation of Shanghai(Grant No.23ZR1477100).
文摘Dear editor,As of 2023,the domestic cat population in China reached 65 million,surpassing dogs to become the most numerous companion animal in the country.Feline calicivirus(FCV)infection,one of the three most prevalent infectious diseases in cats,poses a severe threat to feline health.FCV,classified under the Caliciviridae family(genus Vesivirus).
基金funded by the Natural Science Foundation of Hunan Province(grant number 2024JJ5283 to XH)。
文摘Preterm birth and suboptimal fetal growth remain significant perinatal challenges worldwide.Recent data indicate that China's perinatal profile has improved due to reductions in preterm birth rates.However,the country has a 6.5%prevalence of small-for-gestational-age(SGA),ranking fifth globally in total SGA birth numbers^([1,2]).
基金supported by the National Key R&D Program of China(Grant No.2022YFA1404003)the National Natural Science Foundation of China(Grant Nos.T2495252,12104279,and 123B2062)+2 种基金the Innovation Program for Quantum Science and Technology(Grant No.2021ZD0302100)the Fund for Shanxi“1331 Project”Key Subjects Constructionthe Bairen Project of Shanxi Province。
文摘Increasing the number of atoms that interact with microwave fields represents a promising strategy for enhancing the sensitivity of Rydberg atom-based superheterodyne receivers.Nevertheless,the practical implementation of this approach is impeded by adverse effects such as excitation saturation of Rydberg atoms and power broadening.Here,we demonstrate enhanced microwave field measurements based on two specific velocity groups of atoms,simultaneously addressed by dual-channel probe beams in a Sagnac loop interferometer.The application of resonance detuning in two-photon excitation enables selective addressing of atoms moving along the beam direction,thereby significantly mitigating atomic transit noise.At 7.97 GHz,our method yields a 3 dB improvement in signal-to-noise ratio(SNR),achieving a sensitivity of 10.7 nV·cm^(−1)·Hz^(−1/2).This approach offers a viable pathway to further improve the sensitivity of Rydberg atom-based microwave electrometers.
基金supported by the National Natural Science Foundation of China(No.62376197)the Tianjin Science and Technology Program(No.23JCYBJC00360)the Tianjin Health Research Project(No.TJWJ2025MS045).
文摘Accessible communication based on sign language recognition(SLR)is the key to emergency medical assistance for the hearing-impaired community.Balancing the capture of both local and global information in SLR for emergency medicine poses a significant challenge.To address this,we propose a novel approach based on the inter-learning of visual features between global and local information.Specifically,our method enhances the perception capabilities of the visual feature extractor by strategically leveraging the strengths of convolutional neural network(CNN),which are adept at capturing local features,and visual transformers which perform well at perceiving global features.Furthermore,to mitigate the issue of overfitting caused by the limited availability of sign language data for emergency medical applications,we introduce an enhanced short temporal module for data augmentation through additional subsequences.Experimental results on three publicly available sign language datasets demonstrate the efficacy of the proposed approach.
文摘目的比较Inter Tan和PFNA两种方法治疗老年股骨粗隆间骨折加压固定后的加压效果。方法 59例老年股骨粗隆间骨折患者随机分为2组,分别给予Inter Tan(n=39例)和PFNA(n=20例)治疗,X线随访2组患者术前、术后即时、术后4周和术后24周时骨折分离距离。结果 Inter Tan和PFNA两种方法治疗患者术前、术后即时和术后24周时骨折分离距离差异均无统计学意义(P>0.05),但是在术后4周时发现PFNA组有20.0%患者有骨折线增宽表现,而Inter Tan组仅为5.1%,组间比较差异有统计学意义(P<0.05)。结论 Inter Tan固定系统由于具有双螺钉交锁加压作用,在粗隆间骨折患者骨折复位后二次加压及持续维持加压作用方面,优于PFNA固定系统。
基金This paper was supported by Northeast Forestry University.
文摘Genetic relationships of eight species of genus Betula were evaluated using ISSR marks. A total of 236 loci were generated from 17 ISSR primers. Percentage of polymorphic bands (PPB) varied from 5.93 to 19.92. The highest and the lowest level of genetic differentiation were detected in B. ovalifolia and B. maximowicziana Regel respectively. In these eight species, genetic diversity of birch (HT) was 24.38 %, and the genetic variation (GST ) interspecies was accounting for 79.36% of total genetic variation. According to the cluster results of genetic distance, the eight species were classified into three groups as B. davurica, B. ovalifolia, B. platyphylla and B. pendula for one group; B. schmidtii, B. costata and B. ermanii Cham. var. communis for one group, and B. maximowicziana Regel for another group. The result of cluster is consistent with traditional morphological classification.
