Perceiving harmonic information (especially weak harmonic information) in time series has important scientific and engineering significance. Fourier spectrum and time-frequency spectrum are commonly used tools for per...Perceiving harmonic information (especially weak harmonic information) in time series has important scientific and engineering significance. Fourier spectrum and time-frequency spectrum are commonly used tools for perceiving harmonic information, but they are often ineffective in perceiving weak harmonic signals because they are based on energy or amplitude analysis. Based on the theory of Normal time-frequency transform (NTFT) and complex correlation coefficient, a new type of spectrum, the Harmonicity Spectrum (HS), is developed to perceive harmonic information in time series. HS is based on the degree of signal harmony rather than energy or amplitude analysis, and can therefore perceive very weak harmonic information in signals sensitively. Simulation examples show that HS can detect harmonic information that cannot be detected by Fourier spectrum or time-frequency spectrum. Acoustic data analysis shows that HS has better resolution than traditional LOFAR spectrum.展开更多
Quantum nuclear effects and anharmonicity impact a wide range of functional materials and their properties.One of the most powerful techniques to model these effects is the Stochastic Self-Consistent Harmonic Approxim...Quantum nuclear effects and anharmonicity impact a wide range of functional materials and their properties.One of the most powerful techniques to model these effects is the Stochastic Self-Consistent Harmonic Approximation(SSCHA).Unfortunately,the SSCHA is extremely computationally expensive,prohibiting its routine use.We propose a protocol that pairs machine learning interatomic potentials,which can be tailored for the system at hand via active learning,with the SSCHA.Our method leverages an upscaling procedure that allows for the treatment of supercells of up to thousands of atoms with practically minimal computational effort.The protocol is applied to PdCuH_(x)(x=0−2)compounds,chosen because previous experimental studies have reported superconducting critical temperatures,Tcs,as high as 17 K at ambient pressures in an unknown hydrogenated PdCu phase.We identify a P4/mmm PdCuH_(2)structure,which is shown to be dynamically stable only upon the inclusion of quantum fluctuations,as being a key contributor to the measured superconductivity.For this system,our methodology is able to reduce the computational expense for the SSCHA calculations by~96%.The proposed protocol opens the door towards the routine inclusion of quantum nuclear motion and anharmonicity in materials discovery.展开更多
High harmonic generation(HHG)provides an experimental method for producing attosecond pulses and probing electron dynamics.Achieving precise dipole phase measurements is critical for tailoring the harmonic emission ph...High harmonic generation(HHG)provides an experimental method for producing attosecond pulses and probing electron dynamics.Achieving precise dipole phase measurements is critical for tailoring the harmonic emission phase and identifying the HHG mechanism.However,achieving this feature by applying traditional two-beam far-field interferometry to solid materials remains challenging.In this study,we present a novel interferometric approach that utilizes a single laser beam to excite two ZnO microwires(MWs)simultaneously,thereby generating coherent high-harmonic sources that form interference fringes in the far-field region.We leverage the diameter-dependent field-enhancement effect in MWs to measure the intensity-dependent fringe shift,revealing that the intraband current mechanism dominates the below-bandgap harmonic,whereas the interband polarization mechanism dominates the above-bandgap harmonic.This study offers a robust method for measuring the dipole phase of solid-state HHG and inspires intensity-modulated high-harmonic applications in coherent imaging and microdevice design.展开更多
The space gravitational wave detection aims to detect gravitational waves in the mHz band in order to study supermassive black hole mergers,galaxy evolution and the structure of the early universe.One of its core payl...The space gravitational wave detection aims to detect gravitational waves in the mHz band in order to study supermassive black hole mergers,galaxy evolution and the structure of the early universe.One of its core payloads is a transponder-type interstellar laser interferometer,designed to measure relative displacement changes at the pico-meter level.Among its components,phasemeter is tasked with extracting the phase and frequency of the interference signal.Currently,phase-locked loop(PLL)phasemeters are commonly employed.However,the second harmonic signal generated by the mixer can restrict both the dynamic range and phase measurement accuracy of the phasemeter.This paper analyzes the interstellar laser interferometer and the impact of the second harmonic signal on the phasemeter's performance.To address these challenges,a phasemeter incorporating a second harmonic signal filter is proposed.This new design mitigates second harmonic disturbances within the phasemeter's bandwidth by dynamically adjusting the filter's cutoff frequency to track the input signal frequency,thereby suppressing the second harmonic signal in real time.Theoretical and simulation analyses demonstrate that the proposed phasemeter with a second harmonic filter significantly enhances the dynamic range.Finally,experimental results verify that the phasemeter can achieve the tracking of sudden frequency changes up to4.8 MHz.展开更多
This paper presents a programmable frequency scan algorithm based on harmonic balance.The core idea involves treating systems under perturbation as nonlinear time-periodic(NTP)systems.Steady-state harmonics are first ...This paper presents a programmable frequency scan algorithm based on harmonic balance.The core idea involves treating systems under perturbation as nonlinear time-periodic(NTP)systems.Steady-state harmonics are first solved via Newton-Raphson iteration through a set of nonlinear equations,and then input-output variables are selected to estimate the linear transfer function of the original NTP system without perturbations.The applications and insights of the proposed algorithm are discussed,particularly in guiding existing frequency scan algorithms,which are restricted by time-domain signal generation or measurement.This improvement is achieved through linear stability analysis of NTP systems with perturbations.展开更多
With their intricate vectorial structures in space,optical skyrmions have significantly expanded the landscape of topological optics and light-matter interactions.We theoretically investigate high harmonic generation ...With their intricate vectorial structures in space,optical skyrmions have significantly expanded the landscape of topological optics and light-matter interactions.We theoretically investigate high harmonic generation in crystals driven by optical skyrmions.We find that although the skyrmion number is not conserved,the resulting high-order harmonics can exhibit a distinctive multi-vortex structure,whose features are shaped by both the topology of the optical skyrmions and the rotational symmetry of the crystal.The position of the vortex centers can be effectively tuned by employing different types of optical skyrmions.To elucidate the underlying physics,we develop a multi-absorption channel model based on the conservation laws of spin and orbital angular momentum.Our work explores the role of optical topology in extreme nonlinear light-matter interactions,offering new opportunities for the formation and manipulation of optical vortices and novel structured light fields in the visible and ultraviolet regimes.展开更多
In order to eliminate the meshing interference between the flexspline and circular spline after the taper deformation of the flexspline,the radial deformation difference method,major and minor axis fitting method,and ...In order to eliminate the meshing interference between the flexspline and circular spline after the taper deformation of the flexspline,the radial deformation difference method,major and minor axis fitting method,and ellipse fitting method are used to modify the tooth thickness of the flexspline and analyze the performance indexes such as the assembly stress,transmission error,and fatigue life.Firstly,the conjugate tooth profile is solved based on the quadruple-circular-arc tooth profile and modified kinematic method.Then,based on the finite element radial deformation of the flexspline,the principle and characteristics of three modification methods are analyzed,and the modification amount of each section of the flexspline tooth is calculated.Finally,the influence of the three modification methods on the performance of the harmonic drive is compared.The results show that the radial deformation difference method can initially determine the modification amount.The minimum static assembly stress is 406.22 MPa by the major and minor axis fitting method.The ellipse fitting method has the best dynamic performance,small transmission error fluctuation,a peak-to-peak value of 3.060",and a maximum fatigue life of 10^(7.558)cycles.展开更多
Harmonic mode-locking(HML)in soliton fiber lasers is crucial for generating high-repetition-rate pulse trains beyond the fundamental cavity frequency,enabling advanced applications in,for example,optical communication...Harmonic mode-locking(HML)in soliton fiber lasers is crucial for generating high-repetition-rate pulse trains beyond the fundamental cavity frequency,enabling advanced applications in,for example,optical communication and precision sensing.However,achieving HML in experiments is challenging,owing to its inherent instability and high sensitivity to laser parameters,resulting in complex and iterative adjustments.In this paper,a novel HML technique utilizing bidirectional adjustment of pump power is proposed,and it is experimentally demonstrated in an all-fiber hybrid mode-locked soliton laser.By first increasing the pump power to generate a soliton bunch with a certain number of pulses and then gradually decreasing it,HML can be achieved at an order corresponding to the number of pulses in the soliton bunch.Experimental results on the evolution of temporal pulse trains during bidirectional adjustment of the pump power enable a relationship to be established between pump power and soliton bunching with increasing pump power,and reveal the collapse of the soliton bunch and subsequent gradual uniform distribution of solitons into an HML state with decreasing pump power.Second-to sixth-order HML is successfully generated using the proposed technique,and an analysis of the results provides a deeper understanding of the observed pulse dynamics.展开更多
Quasi-periodic solutions with multiple base frequencies exhibit the feature of 2π-periodicity with respect to each of the hyper-time variables.However,it remains a challenge work,due to the lack of effective solution...Quasi-periodic solutions with multiple base frequencies exhibit the feature of 2π-periodicity with respect to each of the hyper-time variables.However,it remains a challenge work,due to the lack of effective solution methods,to solve and track the quasi-periodic solutions with multiple base frequencies until now.In this work,a multi-steps variable-coefficient formulation is proposed,which provides a unified framework to enable either harmonic balance method or collocation method or finite difference method to solve quasi-periodic solutions with multiple base frequencies.For this purpose,a method of alternating U and S domain is also developed to efficiently evaluate the nonlinear force terms.Furthermore,a new robust phase condition is presented for all of the three methods to make them track the quasi-periodic solutions with prior unknown multiple base frequencies,while the stability of the quasi-periodic solutions is assessed by mean of Lyapunov exponents.The feasibility of the constructed methods under the above framework is verified by application to three nonlinear systems.展开更多
Integration of renewable energy sources into power systems requires efficient multilevel inverters,capable of producing high-quality output voltage with low total harmonic distortion(THD).Conventional multilevel inver...Integration of renewable energy sources into power systems requires efficient multilevel inverters,capable of producing high-quality output voltage with low total harmonic distortion(THD).Conventional multilevel inverters often suffer from high component count,high switching stress,low voltage gain,and increased cost,limiting their practical application.This paper introduces a high-gain novel topology for multilevel inverters with reduced number of total components per level count,low voltage stress on power conductive devices,and minimizing a cost function,which depends on the number of components,standing voltage on switches and diodes,output voltage levels,and gain.The designed topology,which can be applied in photovoltaic(PV)systems,utilizes only one direct current(DC)input supply and a modular structure with the ability of capacitor’s voltage self-balancing.The high gain property and low THD of the proposed topology are two advantages that provide sine output waveform,with no need to a high DC input voltage source.Moreover,generalized topology,consisting of cascaded basic units,has been proposed.A comprehensive method has been proposed to determining the values of DC supplies in this configuration,aiming to minimize redundant switching modes and maximize the voltage levels count.The comparison with some other multilevel inverters confirms the desired performance of the basic version given inverter.A prototype has been also implemented and the experimental results have been obtained to verify the advantages of the proposed 25-level topology.展开更多
Hybrid MMC(Hy-MMC)has broad application prospects because of the negative level output ability in its bridge arm.A Hy-MMC topology with a high-modulation ratio is designed in this paper.A second-harmonic current injec...Hybrid MMC(Hy-MMC)has broad application prospects because of the negative level output ability in its bridge arm.A Hy-MMC topology with a high-modulation ratio is designed in this paper.A second-harmonic current injection(SHCI)strategy based on Hy-MMC in high-modulation operation is also proposed to improve the power density of Hy-MMC effectively in steady-state operation.The amplitude of SHCI is determined from the perspective of the root mean square(RMS)value of bridge arm current,and the optimal initial phase angle is determined from the multi-objective optimization(capacitor voltage ripple of sub-modules(SMs),power loss,and peak value of bridge arm current).The effectiveness and engineering practicability of the proposed SHCI strategy based on Hy-MMC in high-modulation operation is verified by the electromagnetic transient(EMT)simulation using PSCAD/EMTDC®.The simulation results show that the capacitor voltage ripple of SMs can be effectively decreased by 61.98%or the capacitance can be decreased by 40%.The power loss is also analyzed.In addition,little influence of low capacitance on multi-operation conditions of Hy-MMC is verified by EMT simulation.展开更多
High-precision optical frequency measurement serves as a cornerstone of modern science and technology,enabling advancements in fields ranging from fundamental physics to quantum information technologies.Obtaining prec...High-precision optical frequency measurement serves as a cornerstone of modern science and technology,enabling advancements in fields ranging from fundamental physics to quantum information technologies.Obtaining precise photon frequencies,especially in the ultraviolet or even extreme ultraviolet regimes,is a key goal in both light–matter interaction experiments and engineering applications.High-order harmonic generation(HHG)is an ideal light source for producing such photons.In this work,we propose an optical temporal interference model(OTIM)that establishes an analogy with multi-slit Fraunhofer diffraction(MSFD)to manipulate fine-frequency photon generation by exploiting the temporal coherence of HHG processes.Our model provides a unified physical framework for three distinct non-integer HHG generation schemes:single-pulse,shaped-pulse,and laser pulse train approaches,which correspond to single-MSFD-like,double-MSFD-like,and multi-MSFD-like processes,respectively.Arbitrary non-integer HHG photons can be obtained using our scheme.Our approach provides a new perspective for accurately measuring and controlling photon frequencies in fields such as frequency comb technology,interferometry,and atomic clocks.展开更多
A novel vibration isolation system designed for superior performance in low-frequency environments is proposed in this work.The isolator is based on a unique hexagonal arrangement of linear springs,allowing for an adj...A novel vibration isolation system designed for superior performance in low-frequency environments is proposed in this work.The isolator is based on a unique hexagonal arrangement of linear springs,allowing for an adjustable geometric configuration via the initial inclination angle.Based on the principle of Lagrangian mechanics,the equation of motion governing the structural dynamics is rigorously derived.The system is modeled as a strongly nonlinear single-degree-of-freedom dynamical system,loaded with a normalized payload and subject to harmonic base excitation.To analyze the steady-state response,the harmonic balance method is employed,providing accurate predictions of the payload's vibration amplitude and displacement transmissibility as functions of both the base excitation amplitude and frequency.The analysis reveals a direct relationship between the isolator's geometric and stiffness parameters and its load-bearing capacity,leading to the identification of three distinct operational regimes.Depending on the unloaded initial inclination angle,the equivalent stiffness ratio,and the payload design configuration,the system can exhibit one of three vibration isolation modes:(i)the quasizero stiffness(QZS)isolation mode,(ii)the zero linear stiffness with controllable nonlinear stiffness,and(iii)the full-band perfect zero stiffness.The vibration isolation performance of the proposed structure is thoroughly discussed for all three oscillation modes in terms of frequency response curves,displacement transmissibility,and time-domain responses.The key novel finding is that this structure can operate as a full-band,high-performance vibration isolator when the initial inclination angle is designed to be a right angle,enabling full isolation of the maximum possible payload.Moreover,the analytical results and numerical simulations demonstrate that the isolator's displacement transmissibility T with the unit dB tends to-∞as the air-damping coefficient approaches zero,enabling ideal vibration isolation across the entire excitation frequency range.These analytical insights are validated through comprehensive numerical simulations,which show excellent agreement with the theoretical predictions.展开更多
High-pressure hydrides have emerged as promising superconducting materials,attracting considerable attention in recent years.In this work,by combining the stochastic self-consistent harmonic approximation with first-p...High-pressure hydrides have emerged as promising superconducting materials,attracting considerable attention in recent years.In this work,by combining the stochastic self-consistent harmonic approximation with first-principles calculations,we elucidate crucial corrections to the vibrational and superconducting properties arising from quantum and anharmonic ionic vibrations of SnH4 in P63/mmc phase at 150–240 GPa.Compared with the classical harmonic approximation,inclusion of these effects results in a pronounced softening(over 500 cm^(−1))of hydrogen-derived optical phonon modes,and increases the superconducting critical temperature(Tc)from 65 K to 79 K(μ^(*)=0.1;isotropic Migdal–Eliashberg theory),corresponding to a 22%enhancement.For μ^(*)=0.13,the predicted Tc is approximately 70 K.Analysis of the Eliashberg spectral function confirms that hydrogen vibrational modes constitute the dominant tuning mechanism.These results provide quantitative insights into quantum ionic effects in hydride superconductors.展开更多
Conventional multilevel inverters often suffer from high harmonic distortion and increased design complexity due to the need for numerous power semiconductor components,particularly at elevated voltage levels.Addressi...Conventional multilevel inverters often suffer from high harmonic distortion and increased design complexity due to the need for numerous power semiconductor components,particularly at elevated voltage levels.Addressing these shortcomings,thiswork presents a robust 15-level PackedUCell(PUC)inverter topology designed for renewable energy and grid-connected applications.The proposed systemintegrates a sensor less proportional-resonant(PR)controller with an advanced carrier-based pulse width modulation scheme.This approach efficiently balances capacitor voltage,minimizes steady-state error,and strongly suppresses both zero and third-order harmonics resulting in reduced total harmonic distortion and enhanced voltage regulation.Additionally,a novel switching algorithm simplifies the design and implementation,further lowering voltage stress across switches.Extensive simulation results validate the performance under various resistive and resistive-inductive load conditions,demonstrating compliance with IEEE-519 THD standards and robust operation under dynamic changes.The proposed sensorless PR-controlled 15-PUC inverter thus offers a compelling,cost-effective solution for efficient power conversion in next-generation renewable energy systems.展开更多
Magnetically suspended rotor(MSR)systems have gained widespread industrial adoption owing to their frictionless operation and exceptional reliability.However,harmonic current generated by unbalanced mass and sensor ru...Magnetically suspended rotor(MSR)systems have gained widespread industrial adoption owing to their frictionless operation and exceptional reliability.However,harmonic current generated by unbalanced mass and sensor runout threatens the system stability.Repetitive control(RC)effectively suppresses harmonic current,but its parameter design relies on an accurate decoupling model of the system.The decoupling model for the MSR system is often simplified to a second-order linear system.Such a simplification,however,necessitates explicit consideration of system uncertainties caused by unmodeled nonlinearities during the RC design process.Especially under strong gyroscopic effects,the parameter uncertainty is further increased.In this article,an active disturbance rejection controller(ADRC)based on phase compensation(PC)is used to suppress coupling disturbances and improve the control performance of harmonic suppression.Firstly,the dynamic model of the MSR system is established,and both internal and external disturbances are thoroughly analyzed.Then,the RC-PCADRC scheme is designed,integrating the complementary strengths of RC and ADRC,with a particular emphasis on PC to improve stability margins.A comprehensive stability analysis is conducted,along with parameter optimization guidelines.Finally,the effectiveness and superiority of the proposed scheme are validated through both simulations and experiments.展开更多
We employ first-principles calculations combined with self-consistent phonon theory and Boltzmann transport equations to investigate the thermal transport and thermoelectric properties of full-Heusler compound Na_(2)T...We employ first-principles calculations combined with self-consistent phonon theory and Boltzmann transport equations to investigate the thermal transport and thermoelectric properties of full-Heusler compound Na_(2)TlSb.Our findings exhibit that the strong quartic anharmonicity and temperature dependence of the Tl atom with rattling behavior plays an important role in the lattice stability of Na_(2)TlSb.We find that soft Tl-Sb bonding and resonant bonding in the pseudocage composed of the Na and Sb atoms interaction is responsible for ultralowκL.Meanwhile,the multi-valley band structure increases the band degeneracy,results in a high power factor in p-type Na_(2)TlSb.The coexistence of ultralowκL and high power factor presents that Na_(2)TlSb is a potential candidate for thermoelectric applications.Moreover,these findings help to understand the origin of ultralowκL of full-Heusler compounds with strong quartic anharmonicity,leading to the rational design of full-Heusler compounds with high thermoelectric performance.展开更多
REMPI technique has been widely used to study the vibrational branching ratios of photoionization of excited states of molecules for the recent decades. It has been found out that the vibrational branching ratios of H...REMPI technique has been widely used to study the vibrational branching ratios of photoionization of excited states of molecules for the recent decades. It has been found out that the vibrational branching ratios of H<sub>2</sub> C<sup>l</sup>π<sub>u</sub> photoionization are strong non-Franck-Condon. The present letter, starting from the anharmonicity of H<sub>2</sub> and H<sub>2</sub><sup>+</sup>,展开更多
Atomic vibrations,in the form of phonons,are foundational in describing the thermal behavior of materials.The possible frequencies of phonons in materials are governed by the complex bonding between atoms,which is phy...Atomic vibrations,in the form of phonons,are foundational in describing the thermal behavior of materials.The possible frequencies of phonons in materials are governed by the complex bonding between atoms,which is physically represented by a spring-mass model that can account for interactions(spring forces)between the atoms(masses).The lowest-order,harmonic,approximation only considers linear forces between atoms and is thought incapable of explaining phenomena like thermal expansion and thermal conductivity,which are attributed to nonlinear,anharmonic,interactions.Here,we show that the kinetic energy of atoms in a solid produces a pressure much like the kinetic energy of atoms in a gas does.This vibrational or phonon pressure naturally increases with temperature,as it does in a gas and therefore results in a thermal expansion.Because thermal expansion thermodynamically defines a Grüneisen parameterγ,which is a typical metric of anharmonicity,we show that even a harmonic solid will necessarily have some anharmonicity.A consequence of this phonon pressure model is a harmonic estimation of the Grüneisen parameter asγ≈(3/2)(3−4x^(2))/(1+2x^(2)),where x=vt/vl is the ratio of the transverse and longitudinal speeds of sound.We demonstrate the immediate utility of this model by developing a high-throughput harmonic estimate of lattice thermal conductivity that is comparable to other state-of-the-art estimations.By linking harmonic and anharmonic properties explicitly,this study provokes new ideas about the fundamental nature of anharmonicity,while also providing a basis for new material engineering design metrics.展开更多
In this paper,we extend the equivalence of the analytic and probabilistic notions of harmonicity in the context of Hunt processes associated with non-symmetric Dirichlet forms on locally compact separable metric space...In this paper,we extend the equivalence of the analytic and probabilistic notions of harmonicity in the context of Hunt processes associated with non-symmetric Dirichlet forms on locally compact separable metric spaces.Extensions to the processes associated with semi-Dirichlet forms and nearly symmetric right processes on Lusin spaces including infinite dimensional spaces are mentioned at the end of this paper.展开更多
文摘Perceiving harmonic information (especially weak harmonic information) in time series has important scientific and engineering significance. Fourier spectrum and time-frequency spectrum are commonly used tools for perceiving harmonic information, but they are often ineffective in perceiving weak harmonic signals because they are based on energy or amplitude analysis. Based on the theory of Normal time-frequency transform (NTFT) and complex correlation coefficient, a new type of spectrum, the Harmonicity Spectrum (HS), is developed to perceive harmonic information in time series. HS is based on the degree of signal harmony rather than energy or amplitude analysis, and can therefore perceive very weak harmonic information in signals sensitively. Simulation examples show that HS can detect harmonic information that cannot be detected by Fourier spectrum or time-frequency spectrum. Acoustic data analysis shows that HS has better resolution than traditional LOFAR spectrum.
基金Funding for this research is provided by the National Science Foundation,under award DMR-2136038Calculations were performed at the Center for Computational Research at SUNY Buffalo(http://hdl.handle.net/10477/79221).
文摘Quantum nuclear effects and anharmonicity impact a wide range of functional materials and their properties.One of the most powerful techniques to model these effects is the Stochastic Self-Consistent Harmonic Approximation(SSCHA).Unfortunately,the SSCHA is extremely computationally expensive,prohibiting its routine use.We propose a protocol that pairs machine learning interatomic potentials,which can be tailored for the system at hand via active learning,with the SSCHA.Our method leverages an upscaling procedure that allows for the treatment of supercells of up to thousands of atoms with practically minimal computational effort.The protocol is applied to PdCuH_(x)(x=0−2)compounds,chosen because previous experimental studies have reported superconducting critical temperatures,Tcs,as high as 17 K at ambient pressures in an unknown hydrogenated PdCu phase.We identify a P4/mmm PdCuH_(2)structure,which is shown to be dynamically stable only upon the inclusion of quantum fluctuations,as being a key contributor to the measured superconductivity.For this system,our methodology is able to reduce the computational expense for the SSCHA calculations by~96%.The proposed protocol opens the door towards the routine inclusion of quantum nuclear motion and anharmonicity in materials discovery.
基金supported by the National Key R&D Program of China (Grant Nos.2023YFA1406801 and 2022YFA1604301)the National Natural Science Foundation of China (Grant Nos.12434013,12595343,12404393,and 12174011)。
文摘High harmonic generation(HHG)provides an experimental method for producing attosecond pulses and probing electron dynamics.Achieving precise dipole phase measurements is critical for tailoring the harmonic emission phase and identifying the HHG mechanism.However,achieving this feature by applying traditional two-beam far-field interferometry to solid materials remains challenging.In this study,we present a novel interferometric approach that utilizes a single laser beam to excite two ZnO microwires(MWs)simultaneously,thereby generating coherent high-harmonic sources that form interference fringes in the far-field region.We leverage the diameter-dependent field-enhancement effect in MWs to measure the intensity-dependent fringe shift,revealing that the intraband current mechanism dominates the below-bandgap harmonic,whereas the interband polarization mechanism dominates the above-bandgap harmonic.This study offers a robust method for measuring the dipole phase of solid-state HHG and inspires intensity-modulated high-harmonic applications in coherent imaging and microdevice design.
基金the National Key Research&Development Program of China(Grant No.2022YFC2203901)the State Key Laboratory of Spatial Datum(Grant No.SKLSD2025-KF-03)+1 种基金Fundamental Research Funds for the Central UniversitiesSun Yat-sen University for the support。
文摘The space gravitational wave detection aims to detect gravitational waves in the mHz band in order to study supermassive black hole mergers,galaxy evolution and the structure of the early universe.One of its core payloads is a transponder-type interstellar laser interferometer,designed to measure relative displacement changes at the pico-meter level.Among its components,phasemeter is tasked with extracting the phase and frequency of the interference signal.Currently,phase-locked loop(PLL)phasemeters are commonly employed.However,the second harmonic signal generated by the mixer can restrict both the dynamic range and phase measurement accuracy of the phasemeter.This paper analyzes the interstellar laser interferometer and the impact of the second harmonic signal on the phasemeter's performance.To address these challenges,a phasemeter incorporating a second harmonic signal filter is proposed.This new design mitigates second harmonic disturbances within the phasemeter's bandwidth by dynamically adjusting the filter's cutoff frequency to track the input signal frequency,thereby suppressing the second harmonic signal in real time.Theoretical and simulation analyses demonstrate that the proposed phasemeter with a second harmonic filter significantly enhances the dynamic range.Finally,experimental results verify that the phasemeter can achieve the tracking of sudden frequency changes up to4.8 MHz.
基金supported by China Southern Power Grid Corporation(036000KC23090005(GDKJXM20231027)).
文摘This paper presents a programmable frequency scan algorithm based on harmonic balance.The core idea involves treating systems under perturbation as nonlinear time-periodic(NTP)systems.Steady-state harmonics are first solved via Newton-Raphson iteration through a set of nonlinear equations,and then input-output variables are selected to estimate the linear transfer function of the original NTP system without perturbations.The applications and insights of the proposed algorithm are discussed,particularly in guiding existing frequency scan algorithms,which are restricted by time-domain signal generation or measurement.This improvement is achieved through linear stability analysis of NTP systems with perturbations.
基金supported by the National Natural Science Foundation of China (Grant Nos. 12234002, 92250303, 12474486, 12504301, and 12504396)the National Key Research and Development Program of China (Grant No. 2024YFA1612101)。
文摘With their intricate vectorial structures in space,optical skyrmions have significantly expanded the landscape of topological optics and light-matter interactions.We theoretically investigate high harmonic generation in crystals driven by optical skyrmions.We find that although the skyrmion number is not conserved,the resulting high-order harmonics can exhibit a distinctive multi-vortex structure,whose features are shaped by both the topology of the optical skyrmions and the rotational symmetry of the crystal.The position of the vortex centers can be effectively tuned by employing different types of optical skyrmions.To elucidate the underlying physics,we develop a multi-absorption channel model based on the conservation laws of spin and orbital angular momentum.Our work explores the role of optical topology in extreme nonlinear light-matter interactions,offering new opportunities for the formation and manipulation of optical vortices and novel structured light fields in the visible and ultraviolet regimes.
文摘In order to eliminate the meshing interference between the flexspline and circular spline after the taper deformation of the flexspline,the radial deformation difference method,major and minor axis fitting method,and ellipse fitting method are used to modify the tooth thickness of the flexspline and analyze the performance indexes such as the assembly stress,transmission error,and fatigue life.Firstly,the conjugate tooth profile is solved based on the quadruple-circular-arc tooth profile and modified kinematic method.Then,based on the finite element radial deformation of the flexspline,the principle and characteristics of three modification methods are analyzed,and the modification amount of each section of the flexspline tooth is calculated.Finally,the influence of the three modification methods on the performance of the harmonic drive is compared.The results show that the radial deformation difference method can initially determine the modification amount.The minimum static assembly stress is 406.22 MPa by the major and minor axis fitting method.The ellipse fitting method has the best dynamic performance,small transmission error fluctuation,a peak-to-peak value of 3.060",and a maximum fatigue life of 10^(7.558)cycles.
基金supported by the National Natural Science Foundation of China(Grant No.52475574).
文摘Harmonic mode-locking(HML)in soliton fiber lasers is crucial for generating high-repetition-rate pulse trains beyond the fundamental cavity frequency,enabling advanced applications in,for example,optical communication and precision sensing.However,achieving HML in experiments is challenging,owing to its inherent instability and high sensitivity to laser parameters,resulting in complex and iterative adjustments.In this paper,a novel HML technique utilizing bidirectional adjustment of pump power is proposed,and it is experimentally demonstrated in an all-fiber hybrid mode-locked soliton laser.By first increasing the pump power to generate a soliton bunch with a certain number of pulses and then gradually decreasing it,HML can be achieved at an order corresponding to the number of pulses in the soliton bunch.Experimental results on the evolution of temporal pulse trains during bidirectional adjustment of the pump power enable a relationship to be established between pump power and soliton bunching with increasing pump power,and reveal the collapse of the soliton bunch and subsequent gradual uniform distribution of solitons into an HML state with decreasing pump power.Second-to sixth-order HML is successfully generated using the proposed technique,and an analysis of the results provides a deeper understanding of the observed pulse dynamics.
基金supported by the National Natural Science Foundation of China(Grant Nos.12172267 and 12302014).
文摘Quasi-periodic solutions with multiple base frequencies exhibit the feature of 2π-periodicity with respect to each of the hyper-time variables.However,it remains a challenge work,due to the lack of effective solution methods,to solve and track the quasi-periodic solutions with multiple base frequencies until now.In this work,a multi-steps variable-coefficient formulation is proposed,which provides a unified framework to enable either harmonic balance method or collocation method or finite difference method to solve quasi-periodic solutions with multiple base frequencies.For this purpose,a method of alternating U and S domain is also developed to efficiently evaluate the nonlinear force terms.Furthermore,a new robust phase condition is presented for all of the three methods to make them track the quasi-periodic solutions with prior unknown multiple base frequencies,while the stability of the quasi-periodic solutions is assessed by mean of Lyapunov exponents.The feasibility of the constructed methods under the above framework is verified by application to three nonlinear systems.
文摘Integration of renewable energy sources into power systems requires efficient multilevel inverters,capable of producing high-quality output voltage with low total harmonic distortion(THD).Conventional multilevel inverters often suffer from high component count,high switching stress,low voltage gain,and increased cost,limiting their practical application.This paper introduces a high-gain novel topology for multilevel inverters with reduced number of total components per level count,low voltage stress on power conductive devices,and minimizing a cost function,which depends on the number of components,standing voltage on switches and diodes,output voltage levels,and gain.The designed topology,which can be applied in photovoltaic(PV)systems,utilizes only one direct current(DC)input supply and a modular structure with the ability of capacitor’s voltage self-balancing.The high gain property and low THD of the proposed topology are two advantages that provide sine output waveform,with no need to a high DC input voltage source.Moreover,generalized topology,consisting of cascaded basic units,has been proposed.A comprehensive method has been proposed to determining the values of DC supplies in this configuration,aiming to minimize redundant switching modes and maximize the voltage levels count.The comparison with some other multilevel inverters confirms the desired performance of the basic version given inverter.A prototype has been also implemented and the experimental results have been obtained to verify the advantages of the proposed 25-level topology.
基金supported by National Natural Science Foundation of China(52277094).
文摘Hybrid MMC(Hy-MMC)has broad application prospects because of the negative level output ability in its bridge arm.A Hy-MMC topology with a high-modulation ratio is designed in this paper.A second-harmonic current injection(SHCI)strategy based on Hy-MMC in high-modulation operation is also proposed to improve the power density of Hy-MMC effectively in steady-state operation.The amplitude of SHCI is determined from the perspective of the root mean square(RMS)value of bridge arm current,and the optimal initial phase angle is determined from the multi-objective optimization(capacitor voltage ripple of sub-modules(SMs),power loss,and peak value of bridge arm current).The effectiveness and engineering practicability of the proposed SHCI strategy based on Hy-MMC in high-modulation operation is verified by the electromagnetic transient(EMT)simulation using PSCAD/EMTDC®.The simulation results show that the capacitor voltage ripple of SMs can be effectively decreased by 61.98%or the capacitance can be decreased by 40%.The power loss is also analyzed.In addition,little influence of low capacitance on multi-operation conditions of Hy-MMC is verified by EMT simulation.
基金supported by the National Natural Science Foundation of China(Grant No.12304379)the Natural Science Foundation of Liaoning Province(Grant No.2024BS-269)the Guangdong Basic and Applied Basic Research Foundation(Grant No.025A1515011117)。
文摘High-precision optical frequency measurement serves as a cornerstone of modern science and technology,enabling advancements in fields ranging from fundamental physics to quantum information technologies.Obtaining precise photon frequencies,especially in the ultraviolet or even extreme ultraviolet regimes,is a key goal in both light–matter interaction experiments and engineering applications.High-order harmonic generation(HHG)is an ideal light source for producing such photons.In this work,we propose an optical temporal interference model(OTIM)that establishes an analogy with multi-slit Fraunhofer diffraction(MSFD)to manipulate fine-frequency photon generation by exploiting the temporal coherence of HHG processes.Our model provides a unified physical framework for three distinct non-integer HHG generation schemes:single-pulse,shaped-pulse,and laser pulse train approaches,which correspond to single-MSFD-like,double-MSFD-like,and multi-MSFD-like processes,respectively.Arbitrary non-integer HHG photons can be obtained using our scheme.Our approach provides a new perspective for accurately measuring and controlling photon frequencies in fields such as frequency comb technology,interferometry,and atomic clocks.
基金Project supported by the National Key R&D Program of China(No.2023YFE0125900)。
文摘A novel vibration isolation system designed for superior performance in low-frequency environments is proposed in this work.The isolator is based on a unique hexagonal arrangement of linear springs,allowing for an adjustable geometric configuration via the initial inclination angle.Based on the principle of Lagrangian mechanics,the equation of motion governing the structural dynamics is rigorously derived.The system is modeled as a strongly nonlinear single-degree-of-freedom dynamical system,loaded with a normalized payload and subject to harmonic base excitation.To analyze the steady-state response,the harmonic balance method is employed,providing accurate predictions of the payload's vibration amplitude and displacement transmissibility as functions of both the base excitation amplitude and frequency.The analysis reveals a direct relationship between the isolator's geometric and stiffness parameters and its load-bearing capacity,leading to the identification of three distinct operational regimes.Depending on the unloaded initial inclination angle,the equivalent stiffness ratio,and the payload design configuration,the system can exhibit one of three vibration isolation modes:(i)the quasizero stiffness(QZS)isolation mode,(ii)the zero linear stiffness with controllable nonlinear stiffness,and(iii)the full-band perfect zero stiffness.The vibration isolation performance of the proposed structure is thoroughly discussed for all three oscillation modes in terms of frequency response curves,displacement transmissibility,and time-domain responses.The key novel finding is that this structure can operate as a full-band,high-performance vibration isolator when the initial inclination angle is designed to be a right angle,enabling full isolation of the maximum possible payload.Moreover,the analytical results and numerical simulations demonstrate that the isolator's displacement transmissibility T with the unit dB tends to-∞as the air-damping coefficient approaches zero,enabling ideal vibration isolation across the entire excitation frequency range.These analytical insights are validated through comprehensive numerical simulations,which show excellent agreement with the theoretical predictions.
基金supported by the Scientific Research Program Funded by Shaanxi Provincial Education Department (Grant No.24JP126)the National Natural Science Foundation of China (Grant No.62174136)the Natural Science Basic Research Program of Shaanxi Province (Grant No.2025JC-YBMS-063)。
文摘High-pressure hydrides have emerged as promising superconducting materials,attracting considerable attention in recent years.In this work,by combining the stochastic self-consistent harmonic approximation with first-principles calculations,we elucidate crucial corrections to the vibrational and superconducting properties arising from quantum and anharmonic ionic vibrations of SnH4 in P63/mmc phase at 150–240 GPa.Compared with the classical harmonic approximation,inclusion of these effects results in a pronounced softening(over 500 cm^(−1))of hydrogen-derived optical phonon modes,and increases the superconducting critical temperature(Tc)from 65 K to 79 K(μ^(*)=0.1;isotropic Migdal–Eliashberg theory),corresponding to a 22%enhancement.For μ^(*)=0.13,the predicted Tc is approximately 70 K.Analysis of the Eliashberg spectral function confirms that hydrogen vibrational modes constitute the dominant tuning mechanism.These results provide quantitative insights into quantum ionic effects in hydride superconductors.
文摘Conventional multilevel inverters often suffer from high harmonic distortion and increased design complexity due to the need for numerous power semiconductor components,particularly at elevated voltage levels.Addressing these shortcomings,thiswork presents a robust 15-level PackedUCell(PUC)inverter topology designed for renewable energy and grid-connected applications.The proposed systemintegrates a sensor less proportional-resonant(PR)controller with an advanced carrier-based pulse width modulation scheme.This approach efficiently balances capacitor voltage,minimizes steady-state error,and strongly suppresses both zero and third-order harmonics resulting in reduced total harmonic distortion and enhanced voltage regulation.Additionally,a novel switching algorithm simplifies the design and implementation,further lowering voltage stress across switches.Extensive simulation results validate the performance under various resistive and resistive-inductive load conditions,demonstrating compliance with IEEE-519 THD standards and robust operation under dynamic changes.The proposed sensorless PR-controlled 15-PUC inverter thus offers a compelling,cost-effective solution for efficient power conversion in next-generation renewable energy systems.
基金supported by the Youth Innovation Promotion Association CAS under Grant 2023042the Major Science Facility Project of the Shandong Provincial Natural Science Foundation under Grant ZR2022DKX005。
文摘Magnetically suspended rotor(MSR)systems have gained widespread industrial adoption owing to their frictionless operation and exceptional reliability.However,harmonic current generated by unbalanced mass and sensor runout threatens the system stability.Repetitive control(RC)effectively suppresses harmonic current,but its parameter design relies on an accurate decoupling model of the system.The decoupling model for the MSR system is often simplified to a second-order linear system.Such a simplification,however,necessitates explicit consideration of system uncertainties caused by unmodeled nonlinearities during the RC design process.Especially under strong gyroscopic effects,the parameter uncertainty is further increased.In this article,an active disturbance rejection controller(ADRC)based on phase compensation(PC)is used to suppress coupling disturbances and improve the control performance of harmonic suppression.Firstly,the dynamic model of the MSR system is established,and both internal and external disturbances are thoroughly analyzed.Then,the RC-PCADRC scheme is designed,integrating the complementary strengths of RC and ADRC,with a particular emphasis on PC to improve stability margins.A comprehensive stability analysis is conducted,along with parameter optimization guidelines.Finally,the effectiveness and superiority of the proposed scheme are validated through both simulations and experiments.
基金This research were supported by the National Natural Science Foundation of China under Grant No.11974302,No.12174327,No.92270104the Graduate Innovation Foundation of Yantai University,GIFYTU under Grant No.KGIFYTU2213.
文摘We employ first-principles calculations combined with self-consistent phonon theory and Boltzmann transport equations to investigate the thermal transport and thermoelectric properties of full-Heusler compound Na_(2)TlSb.Our findings exhibit that the strong quartic anharmonicity and temperature dependence of the Tl atom with rattling behavior plays an important role in the lattice stability of Na_(2)TlSb.We find that soft Tl-Sb bonding and resonant bonding in the pseudocage composed of the Na and Sb atoms interaction is responsible for ultralowκL.Meanwhile,the multi-valley band structure increases the band degeneracy,results in a high power factor in p-type Na_(2)TlSb.The coexistence of ultralowκL and high power factor presents that Na_(2)TlSb is a potential candidate for thermoelectric applications.Moreover,these findings help to understand the origin of ultralowκL of full-Heusler compounds with strong quartic anharmonicity,leading to the rational design of full-Heusler compounds with high thermoelectric performance.
基金Project supported by the National Natural Science Foundation of China
文摘REMPI technique has been widely used to study the vibrational branching ratios of photoionization of excited states of molecules for the recent decades. It has been found out that the vibrational branching ratios of H<sub>2</sub> C<sup>l</sup>π<sub>u</sub> photoionization are strong non-Franck-Condon. The present letter, starting from the anharmonicity of H<sub>2</sub> and H<sub>2</sub><sup>+</sup>,
基金the U.S.Department of Energy,Office of Energy Efficiency and Renewable Energy(EERE)program“Accelerated Discovery of Compositionally Complex Alloys for Direct Thermal Energy Conversion”(DOE Award DE-AC02-76SF00515).
文摘Atomic vibrations,in the form of phonons,are foundational in describing the thermal behavior of materials.The possible frequencies of phonons in materials are governed by the complex bonding between atoms,which is physically represented by a spring-mass model that can account for interactions(spring forces)between the atoms(masses).The lowest-order,harmonic,approximation only considers linear forces between atoms and is thought incapable of explaining phenomena like thermal expansion and thermal conductivity,which are attributed to nonlinear,anharmonic,interactions.Here,we show that the kinetic energy of atoms in a solid produces a pressure much like the kinetic energy of atoms in a gas does.This vibrational or phonon pressure naturally increases with temperature,as it does in a gas and therefore results in a thermal expansion.Because thermal expansion thermodynamically defines a Grüneisen parameterγ,which is a typical metric of anharmonicity,we show that even a harmonic solid will necessarily have some anharmonicity.A consequence of this phonon pressure model is a harmonic estimation of the Grüneisen parameter asγ≈(3/2)(3−4x^(2))/(1+2x^(2)),where x=vt/vl is the ratio of the transverse and longitudinal speeds of sound.We demonstrate the immediate utility of this model by developing a high-throughput harmonic estimate of lattice thermal conductivity that is comparable to other state-of-the-art estimations.By linking harmonic and anharmonic properties explicitly,this study provokes new ideas about the fundamental nature of anharmonicity,while also providing a basis for new material engineering design metrics.
基金supported by National Natural Science Foundation of China(Grant No.10721101)National Basic Research Program of China(Grant No.2006CB805900)+1 种基金Key Lab of Random Complex Structures and Data Science,Chinese Academy of Sciences(Grant No.2008DP173182)Sino-Germany IGK Project
文摘In this paper,we extend the equivalence of the analytic and probabilistic notions of harmonicity in the context of Hunt processes associated with non-symmetric Dirichlet forms on locally compact separable metric spaces.Extensions to the processes associated with semi-Dirichlet forms and nearly symmetric right processes on Lusin spaces including infinite dimensional spaces are mentioned at the end of this paper.