The real-time and accurate calculation of electricity indirect carbon emissions is not only the critical component for quantifying the carbon emission levels of the power system but also an effective mean to guide ele...The real-time and accurate calculation of electricity indirect carbon emissions is not only the critical component for quantifying the carbon emission levels of the power system but also an effective mean to guide electricity users in carbon reduction and promote power industry low-carbon transformation.Fundamentally,calculating indirect carbon emissions involves allocating direct carbon emission data from the power source side,indicating that accurate indirect emission results rely on the precise measurement of power source emissions.However,existing research on indirect carbon emissions in large-scale power systems rarely accounts for variations in carbon emission characteristics under different operating conditions of power sources,such as rated/non-rated operating conditions and ramping up/down conditions,making it difficult to reflect source-side and load-side carbon emission information variation during providing ancillary services.Quadratic and exponential functions are proposed to characterize the energy consumption profiles of coal-fired and gas-fired power generation,respectively,to construct a refined carbon emission model for power sources.By leveraging the theory of power system carbon flow,we analyze how variable operating conditions of power sources impact indirect carbon emissions.Case studies demonstrate that changes in power source emissions under variable conditions have a significant effect on the indirect carbon emissions of power grids.展开更多
Carbon Capture,Utilization,and Storage(CCUS)technology has gained widespread attention in recent years as a critical strategy to combat global climate change,particularly in achieving carbon neutrality goals.The Guang...Carbon Capture,Utilization,and Storage(CCUS)technology has gained widespread attention in recent years as a critical strategy to combat global climate change,particularly in achieving carbon neutrality goals.The Guangdong-Hong Kong-Macao Greater Bay Area(GBA),as one of China's most economically active regions,serves as a key engine for economic growth while also facing considerable carbon emission challenges.This study analyzes the industrial emission volume and geographical distribution of key emitting enterprises in the GBA,summarizes their technological processes and main carbonemitting equipment,and provides scientific support for precise mitigation policies and low-carbon development.Based on data from 176 key emitting enterprises,the study reveals that Guangzhou and Dongguan host the largest number of such enterprises.Carbon emissions are primarily concentrated in the power sector,dominated by coal-and gas-fired power units,characterized by significant spatial dispersion and uneven distribution.Beyond the power sector,the paper industry has a high number of enterprises but lower emissions.Key facilities such as boilers,cogeneration systems,and production lines are predominantly located near tributaries rivers in Dongguan and Jiangmen.The building materials sector,primarily cement production,ranks as the second-largest emitter,with hightemperature kilns and grinding equipment,particularly rotary kilns and glass furnaces,as the main sources.The petrochemical and chemical sectors have fewer enterprises and lower emissions in the GBA,mainly located in suburban industrial clusters.Carbon emissions in the GBA exhibit distinct industry concentration and geographical distribution disparities.This study provides crucial data and theoretical insights for the development of targeted emission reduction strategies,optimization of source-sink matching,and the advancement of CCUS technologies in the region,particularly from the GBA to the northern South China Sea.展开更多
Micro light sources are crucial tools for studying the interactions between light and matter at the micro/nanoscale,encompassing diverse applications across multiple disciplines.Despite numerous studies on reducing th...Micro light sources are crucial tools for studying the interactions between light and matter at the micro/nanoscale,encompassing diverse applications across multiple disciplines.Despite numerous studies on reducing the size of micro light sources and enhancing optical resolution,the efficient and simple fabrication of ultra-high-resolution micro light sources remains challenging due to its reliance on precise micro-nano processing technology and advanced processing equipment.In this study,a simple approach for the efficient fabrication of submicron light sources is proposed,namely shadow-assisted sidewall emission(SASE)technology.The SASE utilizes the widely adopted UV photolithography process,employing metal shadow modulation to precisely control the emission of light from polymer sidewalls,thereby obtaining photoluminescent light sources with submicron line widths.The SASE eliminates the need for complex and cumbersome manufacturing procedures.The effects of process parameters,including exposure dose,development time,and metal film thickness,on the linewidth of sources are investigated on detail.It is successfully demonstrated red,green,and blue submicron light sources.Finally,their potential application in the field of optical anti-counterfeiting is also demonstrated.We believe that the SASE proposed in this work provides a novel approach for the preparation and application of micro light sources.展开更多
The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental result...The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental results have shown that in pp collisions,the size of the one-dimensional primordial source depends on the transverse mass(m_(T))of the hadron pairs,following a common scaling behavior similar to that observed in Pb-Pb collisions.In this study,a systematic analysis of the π-π source and correlation functions was performed using the multiphase transport model(AMPT)to understand the properties of the emitting source created in high-multiplicity pp collisions at√s=13 TeV.The mT-scaling behavior and pion emission source radii measured by the ALICE experiment can be described well by a model with a subnucleon structure.This work sheds new light on the effective size of the π-π emission source and the study of intensity interferometry in small systems using a transport model.展开更多
Acoustic waves in the pseudo-triaxial experiment system experience refraction phenomena.The conventional assumption that acoustic waves propagate along a straight line in traditional methods can lead to significant er...Acoustic waves in the pseudo-triaxial experiment system experience refraction phenomena.The conventional assumption that acoustic waves propagate along a straight line in traditional methods can lead to significant errors in localization results.To the end,this paper presents a method for locating acoustic emission(AE)sources in pseudo-triaxial experiments using shortest paths and orthogonal constraints.The approach consists of three main steps:(1)establishing control equations for refraction paths from AE sources to sensor locations;(2)calculating refraction point locations using the shortest travel principle and orthogonal constraints;(3)determining source coordinates using Taylor's first-order expansion.The results from laboratory AE experiments demonstrate that the average localization accuracy of the new method is only 6.5 mm,which is 66%more precise than the accuracy(19.4 mm)of the traditional method.Furthermore,simulation results indicate that the new method is not affected by the refraction ratio of the media and maintains the highest positioning accuracy across various arrival and velocity errors.展开更多
The Grey Wolf Optimization(GWO)algorithm is acknowledged as an effective method for rock acoustic emission localization.However,the conventional GWO algorithm encounters challenges related to solution accuracy and con...The Grey Wolf Optimization(GWO)algorithm is acknowledged as an effective method for rock acoustic emission localization.However,the conventional GWO algorithm encounters challenges related to solution accuracy and convergence speed.To address these concerns,this paper develops a Simplex Improved Grey Wolf Optimizer(SMIGWO)algorithm.The randomly generating initial populations are replaced with the iterative chaotic sequences.The search process is optimized using the convergence factor optimization algorithm based on the inverse incompleteГfunction.The simplex method is utilized to address issues related to poorly positioned grey wolves.Experimental results demonstrate that,compared to the conventional GWO algorithm-based AE localization algorithm,the proposed algorithm achieves a higher solution accuracy and showcases a shorter search time.Additionally,the algorithm demonstrates fewer convergence steps,indicating superior convergence efficiency.These findings highlight that the proposed SMIGWO algorithm offers enhanced solution accuracy,stability,and optimization performance.The benefits of the SMIGWO algorithm extend universally across various materials,such as aluminum,granite,and sandstone,showcasing consistent effectiveness irrespective of material type.Consequently,this algorithm emerges as a highly effective tool for identifying acoustic emission signals and improving the precision of rock acoustic emission localization.展开更多
Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory a...Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory and cardiovascular diseases.In this study,we assessed the oxidative potential(OP)of fresh and O_(3)-aged PM_(2.5)particles from various urban and rural emission sources using the dithiothreitol(DTT)method.Our results revealed variations in the OP of fresh PM_(2.5)among different emission sources,with biomass burning sources exhibiting the highest OP,followed by industrial areas,vehicular emissions,cooking emissions,and suburban areas,respectively.Water-soluble organics and transition metals might potentially exert significant influence on particle OP.O_(3)aging notably decreased the OP of PM_(2.5)particles,possibly due to the oxidation of highly DTT-active components into low redox-active small molecules.Moreover,the evolution of OP in different PM_(2.5)components,including methanol-soluble and insoluble fractions,exhibited distinct responses to O_(3)aging for source-oriented PM_(2.5).Additionally,differences in chemical composition between fresh and aged PM_(2.5)were further elucidated through measurements of component-dependent hygroscopic behaviors and phase transitions.This study systematically delineates variances in the toxic potential of fresh and O_(3)-aged PM_(2.5)from various anthropogenic sources.The findings highlight the intrinsic compositional dependence of particle OP and provide essential insights for assessing the health effects of source-oriented PM_(2.5),as well as for formulating human health protection policies.展开更多
Ultrafast electron sources, which enable high spatiotemporal resolution in time-resolved electron microscopy and scanning probe microscopy, are receiving increased attention. The most widely used method for achieving ...Ultrafast electron sources, which enable high spatiotemporal resolution in time-resolved electron microscopy and scanning probe microscopy, are receiving increased attention. The most widely used method for achieving ultrafast electron sources involves irradiating metal tips by ultrashort laser pulses, causing electron beam emission via the photoelectric effect [including photon-driven(quantum) or field-driven(classical) emission]. However, the thermionic electrons emission process due to the heating effect of ultrashort lasers, particularly its dynamic aspects, has rarely been addressed in previous studies. In this paper, we improved the signal-to-noise ratio of a two-pulse correlation measurement on the tip electron emission by nearly two orders of magnitude using a delay time modulation method. This allowed us to obtain information on the temperature evolution of hot electrons and phonons in a non-equilibrium state, and to extract characteristic time scales for electron-phonon and phonon-phonon scattering. Our findings indicate that the thermionic electrons emission, unlike the instantaneous photoelectric effect, causes electron emission to lag behind the laser pulse by tens of picoseconds, thus significantly affecting the detection of ultrafast dynamics of samples. Furthermore, such a lagging effect was found to be sensitive to the local structure of the metal tip, offering new insights into the improved design of ultrafast electron sources.展开更多
To find analytical solutions of nonlinear systems for locating the acoustic emission/microseismic（AE/MS） source without knowing the wave velocity of structures, the sensor location coordinates were simplified as a c...To find analytical solutions of nonlinear systems for locating the acoustic emission/microseismic（AE/MS） source without knowing the wave velocity of structures, the sensor location coordinates were simplified as a cuboid monitoring network. Different locations of sensors on upper and lower surfaces were considered and used to establish nonlinear equations. Based on the proposed functions of time difference of arrivals, the analytical solutions were obtained using five sensors under three networks. The proposed analytical solutions were validated using authentic data of numerical tests and experiments. The results show that located results are consistent with authentic data, and the outstanding characteristics of the new solution are that the solved process is not influenced by the wave velocity knowledge and iterated algorithms.展开更多
To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and...To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and plane location tests were carried out in the granite rod using two sensors and the cube of marble using four sensors, respectively. To compare the position accuracy between line and plane positions, the line poison test was also carried out on the marble surface. The results show that for line positioning, the maximum error of absolute distance is about 0.8 cm. With the speed difference of 200 m/s, the average value of absolute difference from the position error is about 0.4 cm. For the plane positioning, in the case of the sensor array of 30 cm, the absolute positioning distance is up to 8.7 cm. It can be seen that the sonic speed seriously impacts on the plane positioning accuracy. The plane positioning error is lager than the line positioning error, which means that when the line position can satisfy the need in practical engineering, it is better to use the line position instead of the plane location. The plane positioning error with the diagonal speed is the minimum one.展开更多
To find the analytical solution of the acoustic emission/microseismic(AE/MS) source location coordinates, the sensor location coordinates were optimized and simplified. A cube monitoring network of sensor location was...To find the analytical solution of the acoustic emission/microseismic(AE/MS) source location coordinates, the sensor location coordinates were optimized and simplified. A cube monitoring network of sensor location was selected, and the AE/MS source localization equations were established. A location method with P-wave velocity by analytical solutions (P-VAS) was obtained with these equations. The virtual location tests show that the relocation results of analytical method are fully consistent with the actual coordinates for events both inside and outside the monitoring network; whereas the location error of traditional time difference method is between 0.01 and 0.03 m for events inside the sensor array, and the location errors are larger, which is up to 1080986 m for events outside the sensor array. The broken pencil location tests were carried out in the cross section of 100 mm×98 mm, 350 mm-length granite rock specimen using five AE sensors. Five AE sources were relocated with the conventional method and the P-VAS method. For the four events outside monitoring network, the positioning accuracy by P-VAS method is higher than that by the traditional method, and the location accuracy of the larger one can be increased by 17.61 mm. The results of both virtual and broken pencil location tests show that the proposed analytical solution is effective to improve the positioning accuracy. It can locate the coordinates of AE/MS source only using simple four arithmetic operations, without determining the fitting initial value and iterative calculation, which can be solved by a conventional calculator or Microsoft Excel.展开更多
In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature...In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature extraction and the hierarchy support vector machine （H-SVM） classifier is proposed. After a four-level decomposition of the HWPT, the energy feature of AE signals in different frequency bands is extracted, which overcomes the shortcomings of the traditional wavelet packet including energy leakage, and inflexible frequency band selection and different frequency resolutions on different levels. The H-SVM classifier is trained with a subset of the experimental data for known AE source types and tested using the remaining set of data. The results of pressure-off experiments on the specimens of carbon fiber materials indicate that the proposed approach can effectively implement the AE source type identification, and has a better performance in terms of computational efficiency and identification accuracy than the wavelet packet （WPT） feature extraction.展开更多
The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of ...The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of 2007 were examined in a modeling study.The modeling system consisted of the Weather Research and Forecasting （WRF） model and the photochemical dispersion model,CAMx.The factor separation technique （FST） was used to quantify the effect of individual emission source types and the synergistic interactions among two or more types.Additionally,the effectiveness of emission reduction scenarios was explored.The industry,power plant,and transportation emission source types were found to be the most important in terms of their individual effects on O3DM.The key contributor to high surface O3 was power plant emissions,with a peak individual effect of 40 ppbv in the southwestern BTH area.The individual effect from the biogenic emission category was quite low.The synergistic effects from the combinations of each pair of anthropogenic emission types suppressed O3 formation,while the synergistic effects for combinations of three were favorable for O3 formation when the industrial and power plant emission source types coexisted.The quadruple synergistic effects were positive only with the combination of power plant,transportation,residential,and biogenic sources,while the quintuple synergistic effect showed only minor impacts on O3DM concentrations.A 30％ reduction in industrial and transportation sources produced the most effective impacts on O3 concentrations,with a maximum decrease of 20 ppbv.These results suggested that the synergistic impacts among emission source types should be considered when formulating emission control strategies for O3 reduction.展开更多
The methane(CH4) emissions from municipal solid waste(MSW) landfills in China in 2007 were estimated based on database of the three-dimensional emission factors matrix and point sources, by an IPCC recommended FOD(fir...The methane(CH4) emissions from municipal solid waste(MSW) landfills in China in 2007 were estimated based on database of the three-dimensional emission factors matrix and point sources, by an IPCC recommended FOD(firstorder decay) model. The location, capacity and age of landfills constitute the three dimensions of the emission factors matrix, which were obtained by laboratory analysis and in situ investigation. Key parameters such as waste composition,degradable organic carbon ratio, CH4 correction factor, oxidation factor and recovery rate, were carefully analyzed in terms of these three dimensions. The point sources database consists of 2,107 MSW landfills in cities and towns of China in 2007. The results show that the CH4 emissions from MSW landfills were 1.186 Mt in 2007. Compared with the CH4 emissions of 2.20 Mt in 2005, the significant discrepancy mainly comes from statistical data of landfills, e.g., number of landfills and amount of waste disposed in landfills. CH4 emissions were lower than 700 t for most of the landfills, whereas there were 279 landfills with emissions larger than 1,000 t, and only 10 landfills with emissions larger than 10,000 t.Jiangsu province ranks the largest emitter with 98,700 t while Tibet is the smallest emitter with 2,100 t. In general,the emissions from eastern provinces, such as Jiangsu, Guangdong and Zhejiang, were larger than those from western provinces, such as Ningxia, Tibet and Qinghai.展开更多
Particle breakage is a common occurrence in granular systems when the external stress exceeds the individual particle strength.A large number of experimental evidences suggested that particle breakage may significantl...Particle breakage is a common occurrence in granular systems when the external stress exceeds the individual particle strength.A large number of experimental evidences suggested that particle breakage may significantly influence the soil behavior.In the case of pile foundations,the subsoil below the pile tip experiences considerable high stress and consequently prone to break.Due to the lack of sufficient understanding on particle breakage mechanism,there is currently no consentaneous theoretical background for particle breakage analysis during the pile penetration process.This study aims to clarify the location of particle breakage and its evolving characteristics with the aid of acoustic emission(AE)source location method.The spatial distribution of AE hypocenters is interpreted to be associated with the mechanism of particle breakage.Results showed that the AE sources were not uniformly distributed,but concentrated within certain zones below the pile tip.This AE concentration zone was pushed downward with the advancing pile tip,and its distance from the real time pile tip position decreased after certain depth of pile penetration.The location of particle breakage interpreted from AE source location was verified with posttest excavations and the insights on the particle breakage evolution zone were further discussed.展开更多
The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire ...The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire more accurate results.First,the SEI of secondary component precursors(SO2,NOx,NH3,and VOCs)was compiled to acquire the emission ratios of these sources for the precursors.Then,a regular CMB simulation was executed to obtain the contributions of primary particle sources and secondary components(SO4^2-,NO3^-3,NH4^+,and SOC).Afterwards,the contributions of secondary components were apportioned into primary sources according to the source emission ratios.The final source apportionment results combined the contributions of primary sources by CMB and SEI.This integrated approach was carried out via a case study of three coastal cities(Zhoushan,Taizhou,and Wenzhou;abbreviated WZ,TZ,and ZS)in Zhejiang Province,China.The regular CMB simulation results showed that PM2.5 pollution was mainly affected by secondary components and mobile sources.The SEI results indicated that electricity,industrial production and mobile sources were the largest contributors to the emission of PM2.5 gaseous precursors.The simulation results of the CMB-SEI model showed that PM2.5 pollution in the coastal areas of Zhejiang Province presented complex pollution characteristics dominated by mobile sources,electricity production sources and industrial production sources.Compared to the results of the CMB and SEI models alone,the CMB-SEI model completely apportioned PM2.5 to primary sources and simultaneously made the results more accurate and reliable in accordance with local industrial characteristics.展开更多
To solve the problem that the existing acoustic emission(AE) source location algorithms cannot always obtain accurate results for multilayer cylindrical media,a new acoustic emission source location method considering...To solve the problem that the existing acoustic emission(AE) source location algorithms cannot always obtain accurate results for multilayer cylindrical media,a new acoustic emission source location method considering refraction was proposed.AE source coordinates were solved by the complex method.Pencil-lead-break experiments were used to verify this method.The absolute distance errors of location results are less than 3 mm,much less than those by the traditional method.The numerical experiments were used to further analyze factors that affect location accuracy.The results of numerical experiments show that the location accuracy of the proposed method is not affected by the ratio of wave velocities but affected by the measurement accuracy of wave velocity.These results show that new method can obtain accurate AE source location in the two-layered cylindrical surface media such as the triaxial compression test.展开更多
Acoustic emission(AE)localization plays an important role in the prediction and control of potential hazardous sources in complex structures.However,existing location methods have less discussion on the presence of un...Acoustic emission(AE)localization plays an important role in the prediction and control of potential hazardous sources in complex structures.However,existing location methods have less discussion on the presence of unknown empty areas.This paper proposes an AE source location method for structures containing unknown empty areas(SUEA).Firstly,this method identifies the shape,size,and location of empty areas in the unknown region by exciting the active AE sources and using the collected AE arrivals.Then,the unknown AE source can be located considering the identified empty areas.The lead break experiments were performed to verify the effectiveness and accuracy of the proposed method.Five specimens were selected containing empty areas with different positions,shapes,and sizes.Results show the average location accuracy of the SUEA increased by 78%compared to the results of the existing method.It can provide a more accurate solution for locating AE sources in complex structures containing unknown empty areas such as tunnels,bridges,railroads,and caves in practical engineering.展开更多
The effect of source size and emission time on the proton-proton(p-p)momentum correlation function(Cpp(q))has been studied systematically.Assuming a spherical Gaussian source with space and time profile according to t...The effect of source size and emission time on the proton-proton(p-p)momentum correlation function(Cpp(q))has been studied systematically.Assuming a spherical Gaussian source with space and time profile according to the function S(r,t)~exp(-r2/2 r02-t/τ)in the correlation function calculation code(CRAB),the results indicate that one Cpp(q)distribution corresponds to a unique combination of source size r0 and emission timeτ.Considering the possible nuclear deformation from a spherical nucleus,an ellipsoidal Gaussian source characterized by the deformation parameter∈=ΔR/R has been simulated.There is almost no difference of Cpp(q)between the results of spherically and ellipsoidally shaped sources with small deformation.These results indicate that a unique source size r0 and emission time could be extracted from the p-p momentum correlation function,which is especially important for identifying the mechanism of twoproton emission from proton-rich nuclei.Furthermore,considering the possible existence of cluster structures within a nucleus,the double Gaussian source is assumed.The results show that the p-p momentum correlation function for a source with or without cluster structures has large systematical differences with the variance of r0 andτ.This may provide a possible method for experimentally observing the cluster structures in proton-rich nuclei.展开更多
A comprehensive agricultural inventory of ammonia emissions for 2017 in Hefei was established on the basis of the specific emission factors and county-level activity data.The emissions over a 1 km×1 km grid and t...A comprehensive agricultural inventory of ammonia emissions for 2017 in Hefei was established on the basis of the specific emission factors and county-level activity data.The emissions over a 1 km×1 km grid and the associated monthly variations were distributed on the basis of land-use type and meteorological conditions,respectively.The total ammonia emissions were 27,242.7 t in 2017 in Hefei,to which livestock was the top contributor,accounting for 54.5%.Two major contributors to livestock waste were broilers and laying hens,which contributed 34.5%and 22.2%of the total emissions,respectively.Changfeng,Feixi,and Feidong counties,with more developed agriculture than other counties,accounted for a large proportion of the total ammonia emissions—as much as 28.5%,24.5%,and 21.0%,respectively.The average emissions density of the whole region was 2.4 t km−2,and the higher values were mostly in areas with denser populations.Seasonally,peak ammonia emissions occurred in summer.展开更多
基金supported by the Science and Technology Project of China Southern Power Grid Co.,Ltd.(ZBKTM20232244)the Project of National Natural of Science Foundation of China(52477103).
文摘The real-time and accurate calculation of electricity indirect carbon emissions is not only the critical component for quantifying the carbon emission levels of the power system but also an effective mean to guide electricity users in carbon reduction and promote power industry low-carbon transformation.Fundamentally,calculating indirect carbon emissions involves allocating direct carbon emission data from the power source side,indicating that accurate indirect emission results rely on the precise measurement of power source emissions.However,existing research on indirect carbon emissions in large-scale power systems rarely accounts for variations in carbon emission characteristics under different operating conditions of power sources,such as rated/non-rated operating conditions and ramping up/down conditions,making it difficult to reflect source-side and load-side carbon emission information variation during providing ancillary services.Quadratic and exponential functions are proposed to characterize the energy consumption profiles of coal-fired and gas-fired power generation,respectively,to construct a refined carbon emission model for power sources.By leveraging the theory of power system carbon flow,we analyze how variable operating conditions of power sources impact indirect carbon emissions.Case studies demonstrate that changes in power source emissions under variable conditions have a significant effect on the indirect carbon emissions of power grids.
基金supported by the National Natural Science Foundation of China(52304098,52106092,42376215,52474105)Shenzhen Science and Technology Program(JCYJ20220818095605012,JCYJ20220530113011027)+5 种基金Guangdong Basic and Applied Basic Research Foundation(2022A1515110338,2023A1515012316,2023A1515012761,2025A1515010748)Research Team Cultivation Program of Shenzhen University(2023QNT004)Shenzhen Key Laboratory of Natural Gas Hydrates(ZDSYS20200421111201738)the General Research Fund(No.12616222)Early Career Scheme(No.22611624)of Hong Kong Research Grants CouncilMajor Science and Technology Infrastructure Project of Material Genome Big–science Facilities Platform supported by the Municipal Development and Reform Commission of Shenzhen。
文摘Carbon Capture,Utilization,and Storage(CCUS)technology has gained widespread attention in recent years as a critical strategy to combat global climate change,particularly in achieving carbon neutrality goals.The Guangdong-Hong Kong-Macao Greater Bay Area(GBA),as one of China's most economically active regions,serves as a key engine for economic growth while also facing considerable carbon emission challenges.This study analyzes the industrial emission volume and geographical distribution of key emitting enterprises in the GBA,summarizes their technological processes and main carbonemitting equipment,and provides scientific support for precise mitigation policies and low-carbon development.Based on data from 176 key emitting enterprises,the study reveals that Guangzhou and Dongguan host the largest number of such enterprises.Carbon emissions are primarily concentrated in the power sector,dominated by coal-and gas-fired power units,characterized by significant spatial dispersion and uneven distribution.Beyond the power sector,the paper industry has a high number of enterprises but lower emissions.Key facilities such as boilers,cogeneration systems,and production lines are predominantly located near tributaries rivers in Dongguan and Jiangmen.The building materials sector,primarily cement production,ranks as the second-largest emitter,with hightemperature kilns and grinding equipment,particularly rotary kilns and glass furnaces,as the main sources.The petrochemical and chemical sectors have fewer enterprises and lower emissions in the GBA,mainly located in suburban industrial clusters.Carbon emissions in the GBA exhibit distinct industry concentration and geographical distribution disparities.This study provides crucial data and theoretical insights for the development of targeted emission reduction strategies,optimization of source-sink matching,and the advancement of CCUS technologies in the region,particularly from the GBA to the northern South China Sea.
基金supported by Natural Science Foundation of the Fujian Province,China(2024J010016)the National Key R&D Program of China(2021YFB3600400)Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Project(2020ZZ113,2021ZZ130)。
文摘Micro light sources are crucial tools for studying the interactions between light and matter at the micro/nanoscale,encompassing diverse applications across multiple disciplines.Despite numerous studies on reducing the size of micro light sources and enhancing optical resolution,the efficient and simple fabrication of ultra-high-resolution micro light sources remains challenging due to its reliance on precise micro-nano processing technology and advanced processing equipment.In this study,a simple approach for the efficient fabrication of submicron light sources is proposed,namely shadow-assisted sidewall emission(SASE)technology.The SASE utilizes the widely adopted UV photolithography process,employing metal shadow modulation to precisely control the emission of light from polymer sidewalls,thereby obtaining photoluminescent light sources with submicron line widths.The SASE eliminates the need for complex and cumbersome manufacturing procedures.The effects of process parameters,including exposure dose,development time,and metal film thickness,on the linewidth of sources are investigated on detail.It is successfully demonstrated red,green,and blue submicron light sources.Finally,their potential application in the field of optical anti-counterfeiting is also demonstrated.We believe that the SASE proposed in this work provides a novel approach for the preparation and application of micro light sources.
基金the National Natural Science Foundation of China(Nos.12061141008,12147101,and 12322508)the Science and Technology Commission of Shanghai Municipality(23590780100)+1 种基金LZ acknowledges the support of the Fundamental Research Funds for the Central UniversitiesChina University of Geosciences(Wuhan),with No.G1323523064.
文摘The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental results have shown that in pp collisions,the size of the one-dimensional primordial source depends on the transverse mass(m_(T))of the hadron pairs,following a common scaling behavior similar to that observed in Pb-Pb collisions.In this study,a systematic analysis of the π-π source and correlation functions was performed using the multiphase transport model(AMPT)to understand the properties of the emitting source created in high-multiplicity pp collisions at√s=13 TeV.The mT-scaling behavior and pion emission source radii measured by the ALICE experiment can be described well by a model with a subnucleon structure.This work sheds new light on the effective size of the π-π emission source and the study of intensity interferometry in small systems using a transport model.
基金the financial support provided by the National Key Research and Development Program for Young Scientists(Grant No.2021YFC2900400)the National Natural Science Foundation of China(Grant No.52304123)the China Postdoctoral Science Foundation(Grant No.2023M730412).
文摘Acoustic waves in the pseudo-triaxial experiment system experience refraction phenomena.The conventional assumption that acoustic waves propagate along a straight line in traditional methods can lead to significant errors in localization results.To the end,this paper presents a method for locating acoustic emission(AE)sources in pseudo-triaxial experiments using shortest paths and orthogonal constraints.The approach consists of three main steps:(1)establishing control equations for refraction paths from AE sources to sensor locations;(2)calculating refraction point locations using the shortest travel principle and orthogonal constraints;(3)determining source coordinates using Taylor's first-order expansion.The results from laboratory AE experiments demonstrate that the average localization accuracy of the new method is only 6.5 mm,which is 66%more precise than the accuracy(19.4 mm)of the traditional method.Furthermore,simulation results indicate that the new method is not affected by the refraction ratio of the media and maintains the highest positioning accuracy across various arrival and velocity errors.
基金support from the National Science Foundation of China(52304137,5192780752274124,52325403)Tiandi Science and Technology Co.,Ltd.(2022-2-TDMS012 and SKLIS202417)Sichuan University(SKHL2215).
文摘The Grey Wolf Optimization(GWO)algorithm is acknowledged as an effective method for rock acoustic emission localization.However,the conventional GWO algorithm encounters challenges related to solution accuracy and convergence speed.To address these concerns,this paper develops a Simplex Improved Grey Wolf Optimizer(SMIGWO)algorithm.The randomly generating initial populations are replaced with the iterative chaotic sequences.The search process is optimized using the convergence factor optimization algorithm based on the inverse incompleteГfunction.The simplex method is utilized to address issues related to poorly positioned grey wolves.Experimental results demonstrate that,compared to the conventional GWO algorithm-based AE localization algorithm,the proposed algorithm achieves a higher solution accuracy and showcases a shorter search time.Additionally,the algorithm demonstrates fewer convergence steps,indicating superior convergence efficiency.These findings highlight that the proposed SMIGWO algorithm offers enhanced solution accuracy,stability,and optimization performance.The benefits of the SMIGWO algorithm extend universally across various materials,such as aluminum,granite,and sandstone,showcasing consistent effectiveness irrespective of material type.Consequently,this algorithm emerges as a highly effective tool for identifying acoustic emission signals and improving the precision of rock acoustic emission localization.
基金supported by the National Natural Science Foundation of China(No.42305109)Quzhou Municipal Science and Technology Bureau(No.2023K222).
文摘Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory and cardiovascular diseases.In this study,we assessed the oxidative potential(OP)of fresh and O_(3)-aged PM_(2.5)particles from various urban and rural emission sources using the dithiothreitol(DTT)method.Our results revealed variations in the OP of fresh PM_(2.5)among different emission sources,with biomass burning sources exhibiting the highest OP,followed by industrial areas,vehicular emissions,cooking emissions,and suburban areas,respectively.Water-soluble organics and transition metals might potentially exert significant influence on particle OP.O_(3)aging notably decreased the OP of PM_(2.5)particles,possibly due to the oxidation of highly DTT-active components into low redox-active small molecules.Moreover,the evolution of OP in different PM_(2.5)components,including methanol-soluble and insoluble fractions,exhibited distinct responses to O_(3)aging for source-oriented PM_(2.5).Additionally,differences in chemical composition between fresh and aged PM_(2.5)were further elucidated through measurements of component-dependent hygroscopic behaviors and phase transitions.This study systematically delineates variances in the toxic potential of fresh and O_(3)-aged PM_(2.5)from various anthropogenic sources.The findings highlight the intrinsic compositional dependence of particle OP and provide essential insights for assessing the health effects of source-oriented PM_(2.5),as well as for formulating human health protection policies.
基金supported by the National Key R&D Program under Grant No.2021YFA1400500the National Natural Science Foundation of China under Grant No.22273029+1 种基金the New Cornerstone Science Foundation through the New Cornerstone Investigator Program under Grant No.NCI202303 and the XPLORER PRIZEthe Beijing Outstanding Young Scientist Program under Grant No.JWZQ20240101002。
文摘Ultrafast electron sources, which enable high spatiotemporal resolution in time-resolved electron microscopy and scanning probe microscopy, are receiving increased attention. The most widely used method for achieving ultrafast electron sources involves irradiating metal tips by ultrashort laser pulses, causing electron beam emission via the photoelectric effect [including photon-driven(quantum) or field-driven(classical) emission]. However, the thermionic electrons emission process due to the heating effect of ultrashort lasers, particularly its dynamic aspects, has rarely been addressed in previous studies. In this paper, we improved the signal-to-noise ratio of a two-pulse correlation measurement on the tip electron emission by nearly two orders of magnitude using a delay time modulation method. This allowed us to obtain information on the temperature evolution of hot electrons and phonons in a non-equilibrium state, and to extract characteristic time scales for electron-phonon and phonon-phonon scattering. Our findings indicate that the thermionic electrons emission, unlike the instantaneous photoelectric effect, causes electron emission to lag behind the laser pulse by tens of picoseconds, thus significantly affecting the detection of ultrafast dynamics of samples. Furthermore, such a lagging effect was found to be sensitive to the local structure of the metal tip, offering new insights into the improved design of ultrafast electron sources.
基金Projects(11447242,41272304,51209236,51274254)supported by the National Natural Science Foundation of ChinaProject(2015CB060200)supported by the National Basic Research Program of China
文摘To find analytical solutions of nonlinear systems for locating the acoustic emission/microseismic（AE/MS） source without knowing the wave velocity of structures, the sensor location coordinates were simplified as a cuboid monitoring network. Different locations of sensors on upper and lower surfaces were considered and used to establish nonlinear equations. Based on the proposed functions of time difference of arrivals, the analytical solutions were obtained using five sensors under three networks. The proposed analytical solutions were validated using authentic data of numerical tests and experiments. The results show that located results are consistent with authentic data, and the outstanding characteristics of the new solution are that the solved process is not influenced by the wave velocity knowledge and iterated algorithms.
基金Projects (50934006, 10872218) supported by the National Natural Science Foundation of ChinaProject (2010CB732004) supported by the National Basic Research Program of ChinaProject (kjdb2010-6) supported by Doctoral Candidate Innovation Research Support Program of Science & Technology Review, China
文摘To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and plane location tests were carried out in the granite rod using two sensors and the cube of marble using four sensors, respectively. To compare the position accuracy between line and plane positions, the line poison test was also carried out on the marble surface. The results show that for line positioning, the maximum error of absolute distance is about 0.8 cm. With the speed difference of 200 m/s, the average value of absolute difference from the position error is about 0.4 cm. For the plane positioning, in the case of the sensor array of 30 cm, the absolute positioning distance is up to 8.7 cm. It can be seen that the sonic speed seriously impacts on the plane positioning accuracy. The plane positioning error is lager than the line positioning error, which means that when the line position can satisfy the need in practical engineering, it is better to use the line position instead of the plane location. The plane positioning error with the diagonal speed is the minimum one.
基金Project (10872218) supported by the National Natural Science Foundation of ChinaProject (2010CB732004) supported by the National Basic Research Program of China+1 种基金Project (kjdb2010-6) supported by Doctoral Candidate Innovation Research Support Program of Science & Technology ReviewProject (201105) supported by Scholarship Award for Excellent Doctoral Student of Ministry of Education of China
文摘To find the analytical solution of the acoustic emission/microseismic(AE/MS) source location coordinates, the sensor location coordinates were optimized and simplified. A cube monitoring network of sensor location was selected, and the AE/MS source localization equations were established. A location method with P-wave velocity by analytical solutions (P-VAS) was obtained with these equations. The virtual location tests show that the relocation results of analytical method are fully consistent with the actual coordinates for events both inside and outside the monitoring network; whereas the location error of traditional time difference method is between 0.01 and 0.03 m for events inside the sensor array, and the location errors are larger, which is up to 1080986 m for events outside the sensor array. The broken pencil location tests were carried out in the cross section of 100 mm×98 mm, 350 mm-length granite rock specimen using five AE sensors. Five AE sources were relocated with the conventional method and the P-VAS method. For the four events outside monitoring network, the positioning accuracy by P-VAS method is higher than that by the traditional method, and the location accuracy of the larger one can be increased by 17.61 mm. The results of both virtual and broken pencil location tests show that the proposed analytical solution is effective to improve the positioning accuracy. It can locate the coordinates of AE/MS source only using simple four arithmetic operations, without determining the fitting initial value and iterative calculation, which can be solved by a conventional calculator or Microsoft Excel.
基金The Natural Science Foundation of Heilongjiang Province ( No. F201018)the National Natural Science Foundation of China( No. 60901042)
文摘In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature extraction and the hierarchy support vector machine （H-SVM） classifier is proposed. After a four-level decomposition of the HWPT, the energy feature of AE signals in different frequency bands is extracted, which overcomes the shortcomings of the traditional wavelet packet including energy leakage, and inflexible frequency band selection and different frequency resolutions on different levels. The H-SVM classifier is trained with a subset of the experimental data for known AE source types and tested using the remaining set of data. The results of pressure-off experiments on the specimens of carbon fiber materials indicate that the proposed approach can effectively implement the AE source type identification, and has a better performance in terms of computational efficiency and identification accuracy than the wavelet packet （WPT） feature extraction.
基金jointly supported by a key project of the Chinese Academy of Sciences (Grant No. XDB05030301)the National Natural Science Foundation of China (Grant Nos. 40905055 and 41175105)the special fund of the State Key Joint Laboratory of Environment Simulation and Pollution Control (Grant No. 13K04ESPCP)
文摘The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of 2007 were examined in a modeling study.The modeling system consisted of the Weather Research and Forecasting （WRF） model and the photochemical dispersion model,CAMx.The factor separation technique （FST） was used to quantify the effect of individual emission source types and the synergistic interactions among two or more types.Additionally,the effectiveness of emission reduction scenarios was explored.The industry,power plant,and transportation emission source types were found to be the most important in terms of their individual effects on O3DM.The key contributor to high surface O3 was power plant emissions,with a peak individual effect of 40 ppbv in the southwestern BTH area.The individual effect from the biogenic emission category was quite low.The synergistic effects from the combinations of each pair of anthropogenic emission types suppressed O3 formation,while the synergistic effects for combinations of three were favorable for O3 formation when the industrial and power plant emission source types coexisted.The quadruple synergistic effects were positive only with the combination of power plant,transportation,residential,and biogenic sources,while the quintuple synergistic effect showed only minor impacts on O3DM concentrations.A 30％ reduction in industrial and transportation sources produced the most effective impacts on O3 concentrations,with a maximum decrease of 20 ppbv.These results suggested that the synergistic impacts among emission source types should be considered when formulating emission control strategies for O3 reduction.
基金funded by the Project Study on Key Issues of China City Carbon Emission Inventory (No. 41101500)supported by National Natural Science Foundation of China
文摘The methane(CH4) emissions from municipal solid waste(MSW) landfills in China in 2007 were estimated based on database of the three-dimensional emission factors matrix and point sources, by an IPCC recommended FOD(firstorder decay) model. The location, capacity and age of landfills constitute the three dimensions of the emission factors matrix, which were obtained by laboratory analysis and in situ investigation. Key parameters such as waste composition,degradable organic carbon ratio, CH4 correction factor, oxidation factor and recovery rate, were carefully analyzed in terms of these three dimensions. The point sources database consists of 2,107 MSW landfills in cities and towns of China in 2007. The results show that the CH4 emissions from MSW landfills were 1.186 Mt in 2007. Compared with the CH4 emissions of 2.20 Mt in 2005, the significant discrepancy mainly comes from statistical data of landfills, e.g., number of landfills and amount of waste disposed in landfills. CH4 emissions were lower than 700 t for most of the landfills, whereas there were 279 landfills with emissions larger than 1,000 t, and only 10 landfills with emissions larger than 10,000 t.Jiangsu province ranks the largest emitter with 98,700 t while Tibet is the smallest emitter with 2,100 t. In general,the emissions from eastern provinces, such as Jiangsu, Guangdong and Zhejiang, were larger than those from western provinces, such as Ningxia, Tibet and Qinghai.
基金sponsored by the Shanghai Sailing Program (Grant No. 18YF1424000)Shanghai Education Commission (Peak Discipline Construction Program, Grant Nos. 0200121005/052 & 2019010206)
文摘Particle breakage is a common occurrence in granular systems when the external stress exceeds the individual particle strength.A large number of experimental evidences suggested that particle breakage may significantly influence the soil behavior.In the case of pile foundations,the subsoil below the pile tip experiences considerable high stress and consequently prone to break.Due to the lack of sufficient understanding on particle breakage mechanism,there is currently no consentaneous theoretical background for particle breakage analysis during the pile penetration process.This study aims to clarify the location of particle breakage and its evolving characteristics with the aid of acoustic emission(AE)source location method.The spatial distribution of AE hypocenters is interpreted to be associated with the mechanism of particle breakage.Results showed that the AE sources were not uniformly distributed,but concentrated within certain zones below the pile tip.This AE concentration zone was pushed downward with the advancing pile tip,and its distance from the real time pile tip position decreased after certain depth of pile penetration.The location of particle breakage interpreted from AE source location was verified with posttest excavations and the insights on the particle breakage evolution zone were further discussed.
基金supported by the National Key Research and Development Program of China(No.2018YFC0214102)。
文摘The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire more accurate results.First,the SEI of secondary component precursors(SO2,NOx,NH3,and VOCs)was compiled to acquire the emission ratios of these sources for the precursors.Then,a regular CMB simulation was executed to obtain the contributions of primary particle sources and secondary components(SO4^2-,NO3^-3,NH4^+,and SOC).Afterwards,the contributions of secondary components were apportioned into primary sources according to the source emission ratios.The final source apportionment results combined the contributions of primary sources by CMB and SEI.This integrated approach was carried out via a case study of three coastal cities(Zhoushan,Taizhou,and Wenzhou;abbreviated WZ,TZ,and ZS)in Zhejiang Province,China.The regular CMB simulation results showed that PM2.5 pollution was mainly affected by secondary components and mobile sources.The SEI results indicated that electricity,industrial production and mobile sources were the largest contributors to the emission of PM2.5 gaseous precursors.The simulation results of the CMB-SEI model showed that PM2.5 pollution in the coastal areas of Zhejiang Province presented complex pollution characteristics dominated by mobile sources,electricity production sources and industrial production sources.Compared to the results of the CMB and SEI models alone,the CMB-SEI model completely apportioned PM2.5 to primary sources and simultaneously made the results more accurate and reliable in accordance with local industrial characteristics.
基金Project(2015CB060200)supported by the National Basic Research Program of ChinaProject(41772313)supported by the National Natural Science Foundation of China+1 种基金Project(MDPC201803)supported by the Open Fund Research Program of State Key Laboratory of Mining Disaster Prevention and Control Co-founded by Shandong Province and the Ministry of Science and Technology,ChinaProject(2019zzts308)supported by the Fundamental Research Fund for the Central Universities of Central South University,China
文摘To solve the problem that the existing acoustic emission(AE) source location algorithms cannot always obtain accurate results for multilayer cylindrical media,a new acoustic emission source location method considering refraction was proposed.AE source coordinates were solved by the complex method.Pencil-lead-break experiments were used to verify this method.The absolute distance errors of location results are less than 3 mm,much less than those by the traditional method.The numerical experiments were used to further analyze factors that affect location accuracy.The results of numerical experiments show that the location accuracy of the proposed method is not affected by the ratio of wave velocities but affected by the measurement accuracy of wave velocity.These results show that new method can obtain accurate AE source location in the two-layered cylindrical surface media such as the triaxial compression test.
基金We are grateful for the financial support from the National Science Foundation for Excellent Young Scholars of China(51822407)the Natural Science Foundation of China(51774327)+1 种基金the Special Fund for Basic Scientific Research Operations in Universities(2282020cxqd055)the Fundamental Research Funds for the Central Universities of Central South University(2021zzts0875).
文摘Acoustic emission(AE)localization plays an important role in the prediction and control of potential hazardous sources in complex structures.However,existing location methods have less discussion on the presence of unknown empty areas.This paper proposes an AE source location method for structures containing unknown empty areas(SUEA).Firstly,this method identifies the shape,size,and location of empty areas in the unknown region by exciting the active AE sources and using the collected AE arrivals.Then,the unknown AE source can be located considering the identified empty areas.The lead break experiments were performed to verify the effectiveness and accuracy of the proposed method.Five specimens were selected containing empty areas with different positions,shapes,and sizes.Results show the average location accuracy of the SUEA increased by 78%compared to the results of the existing method.It can provide a more accurate solution for locating AE sources in complex structures containing unknown empty areas such as tunnels,bridges,railroads,and caves in practical engineering.
基金supported by the National Key R&D Program of China(No.2018YFA0404404)the National Natural Science Foundation of China(Nos.11925502,11935001,11961141003,11421505,11475244,and 11927901)+2 种基金the Shanghai Development Foundation for Science and Technology(No.19ZR1403100)the Strategic Priority Research Program of the CAS(No.XDB34030000)the Key Research Program of Frontier Sciences of the CAS(No.QYZDJ-SSW-SLH002).
文摘The effect of source size and emission time on the proton-proton(p-p)momentum correlation function(Cpp(q))has been studied systematically.Assuming a spherical Gaussian source with space and time profile according to the function S(r,t)~exp(-r2/2 r02-t/τ)in the correlation function calculation code(CRAB),the results indicate that one Cpp(q)distribution corresponds to a unique combination of source size r0 and emission timeτ.Considering the possible nuclear deformation from a spherical nucleus,an ellipsoidal Gaussian source characterized by the deformation parameter∈=ΔR/R has been simulated.There is almost no difference of Cpp(q)between the results of spherically and ellipsoidally shaped sources with small deformation.These results indicate that a unique source size r0 and emission time could be extracted from the p-p momentum correlation function,which is especially important for identifying the mechanism of twoproton emission from proton-rich nuclei.Furthermore,considering the possible existence of cluster structures within a nucleus,the double Gaussian source is assumed.The results show that the p-p momentum correlation function for a source with or without cluster structures has large systematical differences with the variance of r0 andτ.This may provide a possible method for experimentally observing the cluster structures in proton-rich nuclei.
基金This work was supported by the National Natural Science Foundation of China[grant number 41775154]the Six Talent Peaks Project in Jiangsu Province[grant number JNHB-057]the Postgraduate Practical Innovation Program of Jiangsu Province of China[grant number SJCX19_0301].
文摘A comprehensive agricultural inventory of ammonia emissions for 2017 in Hefei was established on the basis of the specific emission factors and county-level activity data.The emissions over a 1 km×1 km grid and the associated monthly variations were distributed on the basis of land-use type and meteorological conditions,respectively.The total ammonia emissions were 27,242.7 t in 2017 in Hefei,to which livestock was the top contributor,accounting for 54.5%.Two major contributors to livestock waste were broilers and laying hens,which contributed 34.5%and 22.2%of the total emissions,respectively.Changfeng,Feixi,and Feidong counties,with more developed agriculture than other counties,accounted for a large proportion of the total ammonia emissions—as much as 28.5%,24.5%,and 21.0%,respectively.The average emissions density of the whole region was 2.4 t km−2,and the higher values were mostly in areas with denser populations.Seasonally,peak ammonia emissions occurred in summer.
