A new dual-layer granular bed filter for hot gas cleanup was invented and studied experimentally. Fine sand,0.5-1 mm grain size and about 1350 kg/m3 bulk density,was used as the lower layer of the filter. Expanded per...A new dual-layer granular bed filter for hot gas cleanup was invented and studied experimentally. Fine sand,0.5-1 mm grain size and about 1350 kg/m3 bulk density,was used as the lower layer of the filter. Expanded perlite par-ticles,2-5 mm grain size and about 70 kg/m3 bulk density,was used for the upper layer of the filter in this study. It was confirmed that the sizes and densities of these two media matched well; the binary media remained in complete segre-gation during regeneration by fluidization. Test results show that the filtration of the expanded perlite particle layer was characterized as "deep bed filtration." Filtration of the fine sand layer was "surface cake filtration." The expanded per-lite particle layer contributed about 90% to the bed dust capacity,but only about 20% to the total bed pressure drop,which increased the bed dust capacity ten fold compared to a single-layer bed of the same sand and the same total bed pressure drop. The dust cake on the surface of the fine sand layer raised the collection efficiencies to over 99.99%.展开更多
A new gas clean-up process called 'integrated sintered metal screen moving granular bed' (ISMSMGB) for the integrated gasification combined cycle (IGCC) and pressured fluidized bed combustion (PFBC) was develo...A new gas clean-up process called 'integrated sintered metal screen moving granular bed' (ISMSMGB) for the integrated gasification combined cycle (IGCC) and pressured fluidized bed combustion (PFBC) was developed on the basis of a sintered metal candle filter and a cross-flow moving granular bed filter. This is a combination of the surface and deep bed filtering processes. A set of facilities was established and a series of cold model tests were carried out. The dust removal efficiency and the pressure drop of the filter were measured and analyzed. The results show that this process features the advantages of the moving bed for high capacity as well as high inlet dust load and the surface filter for high efficiency. Meanwhile, the granules moving downward cleans the cake on the screen surface, so that the system is operated at steady state.展开更多
Comparative experiments on the inactivation of Copepod were investigated in southern China. The 100% of inactivation effect may be attained by 3.0 mg/L of ozone for contacting time of 25 min, whereas 0.5 mg/L of dosag...Comparative experiments on the inactivation of Copepod were investigated in southern China. The 100% of inactivation effect may be attained by 3.0 mg/L of ozone for contacting time of 25 min, whereas 0.5 mg/L of dosage resulted in only 30% of inactivation rate. Copepod may not be completely inactivated by ozone oxidation for feasible dosage limited by higher bromide in raw water. The favorable environment of granular activated carbon （GAC） filter provided Copepod with conditions for excess propagation, The disinfection experimental results show that the inactivation rate is 90% by 2.0 mg/L of chloramines for contacting time of 30 min, whereas only 70% is attained with chlorine. The GC-MS examination indicates that the total organic substance is increased to 92 specie： inciuding 13 sorts of halogenated hydrocarbon by chlorine disnfection, which is more than that of chloramines. More products of bromiinated trihalomethanes occur in treated water by chlorine, disinfection and total amount of THMs is 3 times as high as that of chloramines.展开更多
Granular bed filter(GBF)has become one of the current research hot topics due to its excellent performance in removing fine particles.In this paper,a three-dimensional fixed bed GBF filtration model was established an...Granular bed filter(GBF)has become one of the current research hot topics due to its excellent performance in removing fine particles.In this paper,a three-dimensional fixed bed GBF filtration model was established and its accuracy was verified.Then,the GBF filtration performance at high temperature were studied.The results demonstrate that elevating the temperature diminishes the filtration efficiency,albeit to a limited extent.The increasing of inlet gas velocity can significantly improve pressure drop for GBF and the filtration efficiency for fine particles of sizes larger than 5μm.As the diameter of stacked granular particle diameter grows,the filtration efficiency and pressure drop drops.The density of fine particles almost does not affect the filtration efficiency for fine particles of 1∼7μm,but a higher density leads to a higher filtration efficiency for fine particles of sizes bigger than 9μm.Additionally,as the fine particles size increases,the change of the filtration efficiency roughly goes through three stages:Stage 1:the filtration efficiency is basically unchanged;Stage 2:the filtration efficiency increases rapidly;Stage 3:the filtration efficiency increases steadily,but the rate of increase slows down.With the increase of the fine particles Stokes number,the filtration efficiency of GBF will pass through two phases of stabilization and rapid increase.展开更多
The filtration performance of the moving bed granular filter with axial flow (MBGF-AF) is investigated through a large cold experiment. The effect of different operation parameters on the filtration performance (colle...The filtration performance of the moving bed granular filter with axial flow (MBGF-AF) is investigated through a large cold experiment. The effect of different operation parameters on the filtration performance (collection efficiency, pressure drop) of the axial-flow moving bed filter is investigated in combination with the dust deposition effect and the mechanism of trapping dust by the capturing particles. The results show that the collection efficiency of MBGF-AF is enhanced by decreasing the superficial gas velocity, increasing the inlet dust concentration properly, or decreasing the moving velocity of the capturing particles. A model covering the above operation parameters is established to calculate the collection efficiency of the moving bed granular filter. It is used in a wide range of operating parameters for the MBGFs.展开更多
The dual-layer granular bed filter packed with randomly arranged granules was simulated to study the effects of bed depth of the lower layer of fine granules and the inlet gas velocity on the collection mechanism.The ...The dual-layer granular bed filter packed with randomly arranged granules was simulated to study the effects of bed depth of the lower layer of fine granules and the inlet gas velocity on the collection mechanism.The computational results show that the collection efficiency is much better from this granular bed than a single-layer granular bed,especially for particle diameters of 1-10μm.The inlet gas velocity has less effect on the grade collection efficiency of the dual-layer granular bed than of the single-layer granular bed.The dual-layer granular bed provides a high collection efficiency and low pressure drop.The relationship between the grade collection efficiency and the Stokes number(St)based on the inlet gas velocity is obtained.If St is below a threshold,the grade collection efficiency remains stable;if St is in value above threshold,the grade collection efficiency increases linearly with lg(St).As the bed depth of the lower layer of fine granules increases,the threshold for St shifts forward.展开更多
The filtration of mixed dust that included a small number of melted(liquid)particles was studied in an experimental granular bed filter(GBF).Results show that the collection efficiency of dust containing melted partic...The filtration of mixed dust that included a small number of melted(liquid)particles was studied in an experimental granular bed filter(GBF).Results show that the collection efficiency of dust containing melted particles is higher than that of dust composed of solid particles but the pressure drop from the former is higher than that of the latter.The collection efficiency and pressure drop increase as the concentration of melted particles increases.A surface sliding GBF exhibits good comprehensive performance when filtering dust,especially dust containing a mix of solid and liquid particles.The effects of the gas temperature,gas velocity,sliding filter bed thickness,and sliding collector flux on filter performance were also examined.Based on the experimental results,correlations for the collection efficiency and pressure drop for mixed dust are presented.展开更多
Granular bed filters can effectively filter adhesive dust in high-temperature flue gas.In this study.polyvinyl chloride(PVC)powder was used as adhesive dust,and the mixture of PVC and ash powder was used to simulate s...Granular bed filters can effectively filter adhesive dust in high-temperature flue gas.In this study.polyvinyl chloride(PVC)powder was used as adhesive dust,and the mixture of PVC and ash powder was used to simulate solid and adhesive mixed dust.The effects of gas temperature,velocity,and inlet adhesive dust mass content on dust distribution in granular bed(GBF)were discussed.Results show that the mixed dust mainly accumulates on the upper part of the granular bed,and the mass of the collected dust decreases exponentially from the upper layer to the bottom layer in the GBF.The adhesive dust content collected in each layer differs from that of the incoming dust,and their deviation varies approximately linearly along with the depth of the bed.The total dust distribution and adhesive dust content deviation are influenced by gas temperature and inlet adhesive dust content but independent of gas velocity.The correlations of dust distribution of solid and adhesive mixed dust are presented based on the experimental results.展开更多
The coupled CFD-DEM method with the JKR(Johnson-Kendall-Roberts)model for describing the contact adhesion of dust to filter particles(FPs)is used to simulate the distribution pattern of dust particle deposition in the...The coupled CFD-DEM method with the JKR(Johnson-Kendall-Roberts)model for describing the contact adhesion of dust to filter particles(FPs)is used to simulate the distribution pattern of dust particle deposition in the granular bed filter(GBF)with multi-layer media.The minimum inlet flow velocity must meet the requirement that the contact probability between dust and FPs is in the high contact probability region.The air flow forms vortices on the leeward side of the FPs and changes abruptly at the intersection of different particle size FPs layers.Dust particles form large deposits at the intersection of the first and second layers and the different particle size filter layers.Dual element multilayer GBF can further optimize the bed structure by interlacing filter layers with different particle sizes.Compared with single particle size multi-layer GBF,the bed pressure drop is reduced by 40.24%-50.65%and the dust removal efficiency is increased by 21.93%-55.09%.展开更多
Shortcut nitrification-denitrification,anaerobic ammonium oxidation(ANAMMOX),and methanogenesis have been successfully coupled in an Expanded Granular Sludge Bed-Biological Aerated Filter(EGSB-BAF)integrated system.As...Shortcut nitrification-denitrification,anaerobic ammonium oxidation(ANAMMOX),and methanogenesis have been successfully coupled in an Expanded Granular Sludge Bed-Biological Aerated Filter(EGSB-BAF)integrated system.As fed different synthetic wastewater with chemical oxygen demand(COD)of 300-1200 mg·L^(-1)and NH_(4)^(+)-N of 30-120 mg·L^(-1)at the outer recycle ratio of 200%,the influence of influent on ANAMMOX in the integrated system was investigated in this paper.The experimental results showed that higher COD concentration caused an increase in denitrification and methanogenesis but a decrease in ANAMMOX;however,when an influent with the low concentration of COD was used,the opposite changes could be observed.Higher influent NH_(4)^(+)-N concentration favored ANAMMOX when the COD concentration of influent was fixed.Therefore,low COD=NH_(4)^(+)-N ratio would decrease competition for nitrite between ANAMMOX and denitrification,which was favorable for reducing the negative effect of organic COD on ANAMMOX.The good performance of the integrated system indicated that the bacterial community of denitrification,ANAMMOX,and methanogenesis could be dynamically maintained in the sludge of EGSB reactor for a certain range of influent.展开更多
Combustion-generated hydrogen chloride （HCl） is considered to be a very hazardous acid gaseous pollutant. This paper presents a laboratory study on the dry adsorption of HCl. The experiments were conducted in a dual...Combustion-generated hydrogen chloride （HCl） is considered to be a very hazardous acid gaseous pollutant. This paper presents a laboratory study on the dry adsorption of HCl. The experiments were conducted in a dual-layer granular bed filter, at gas temperatures of 500℃-700℃ and n（Ca）/n（Cl）molar ratios of 1.0-5.0 using the silver nitrate titration method by dry adsorbent powders Ca（OH）2. Mainly, the adsorption efficiency of HCI and utilization efficiency of Calcium were studied, by varying relevant factors including n（Ca）/n（Cl）, tempera- ture, feeding method, water vapor and CO2. With a relatively higher HCl concentration of 1000ppm, the experimental results revealed that 600℃ may be the optimum temperature for HCl adsorption when optimum n （Ca）/n（Cl） was 2.5 in our tests. The results also demonstrated that the feeding at a constant pressure was more effective, and the HCl adsorption efficiency could rapidly reach over 90% with n（Ca）/n（Cl） = 2.5 at 600℃. Furthermore, the HCl adsorption efficiency was found to be slightly promoted by water vapor, while could be impeded by CO2, and the utilization efficiency of calcium could be up to 74.4% without CO2, while was only 36.8% with CO2 when n（Ca）/n（Cl） was 2.5 at 600℃.展开更多
基金Projects 2006C23075 supported by the Key Research Project of Zhejiang Province02J20101-19 by the Science Foundation of Ningbo City
文摘A new dual-layer granular bed filter for hot gas cleanup was invented and studied experimentally. Fine sand,0.5-1 mm grain size and about 1350 kg/m3 bulk density,was used as the lower layer of the filter. Expanded perlite par-ticles,2-5 mm grain size and about 70 kg/m3 bulk density,was used for the upper layer of the filter in this study. It was confirmed that the sizes and densities of these two media matched well; the binary media remained in complete segre-gation during regeneration by fluidization. Test results show that the filtration of the expanded perlite particle layer was characterized as "deep bed filtration." Filtration of the fine sand layer was "surface cake filtration." The expanded per-lite particle layer contributed about 90% to the bed dust capacity,but only about 20% to the total bed pressure drop,which increased the bed dust capacity ten fold compared to a single-layer bed of the same sand and the same total bed pressure drop. The dust cake on the surface of the fine sand layer raised the collection efficiencies to over 99.99%.
基金Chinese Special Funds for Major State Basic Research Projects 973 (No. G1999022104).
文摘A new gas clean-up process called 'integrated sintered metal screen moving granular bed' (ISMSMGB) for the integrated gasification combined cycle (IGCC) and pressured fluidized bed combustion (PFBC) was developed on the basis of a sintered metal candle filter and a cross-flow moving granular bed filter. This is a combination of the surface and deep bed filtering processes. A set of facilities was established and a series of cold model tests were carried out. The dust removal efficiency and the pressure drop of the filter were measured and analyzed. The results show that this process features the advantages of the moving bed for high capacity as well as high inlet dust load and the surface filter for high efficiency. Meanwhile, the granules moving downward cleans the cake on the screen surface, so that the system is operated at steady state.
基金National Natural Science Foundation of China(No.50808065)National Key High-Tech Program(863) of China(No.2006AA06Z311)Key Laboratory of Integrated Regulation and Resource Development on Shallow Lakes Open Project,China(No.2006KJ006)
文摘Comparative experiments on the inactivation of Copepod were investigated in southern China. The 100% of inactivation effect may be attained by 3.0 mg/L of ozone for contacting time of 25 min, whereas 0.5 mg/L of dosage resulted in only 30% of inactivation rate. Copepod may not be completely inactivated by ozone oxidation for feasible dosage limited by higher bromide in raw water. The favorable environment of granular activated carbon （GAC） filter provided Copepod with conditions for excess propagation, The disinfection experimental results show that the inactivation rate is 90% by 2.0 mg/L of chloramines for contacting time of 30 min, whereas only 70% is attained with chlorine. The GC-MS examination indicates that the total organic substance is increased to 92 specie： inciuding 13 sorts of halogenated hydrocarbon by chlorine disnfection, which is more than that of chloramines. More products of bromiinated trihalomethanes occur in treated water by chlorine, disinfection and total amount of THMs is 3 times as high as that of chloramines.
基金support provided by the National Natural Science Foundation of China(grant No.51878356).
文摘Granular bed filter(GBF)has become one of the current research hot topics due to its excellent performance in removing fine particles.In this paper,a three-dimensional fixed bed GBF filtration model was established and its accuracy was verified.Then,the GBF filtration performance at high temperature were studied.The results demonstrate that elevating the temperature diminishes the filtration efficiency,albeit to a limited extent.The increasing of inlet gas velocity can significantly improve pressure drop for GBF and the filtration efficiency for fine particles of sizes larger than 5μm.As the diameter of stacked granular particle diameter grows,the filtration efficiency and pressure drop drops.The density of fine particles almost does not affect the filtration efficiency for fine particles of 1∼7μm,but a higher density leads to a higher filtration efficiency for fine particles of sizes bigger than 9μm.Additionally,as the fine particles size increases,the change of the filtration efficiency roughly goes through three stages:Stage 1:the filtration efficiency is basically unchanged;Stage 2:the filtration efficiency increases rapidly;Stage 3:the filtration efficiency increases steadily,but the rate of increase slows down.With the increase of the fine particles Stokes number,the filtration efficiency of GBF will pass through two phases of stabilization and rapid increase.
基金supported by National Natural Science Foundation of China(U1862202).
文摘The filtration performance of the moving bed granular filter with axial flow (MBGF-AF) is investigated through a large cold experiment. The effect of different operation parameters on the filtration performance (collection efficiency, pressure drop) of the axial-flow moving bed filter is investigated in combination with the dust deposition effect and the mechanism of trapping dust by the capturing particles. The results show that the collection efficiency of MBGF-AF is enhanced by decreasing the superficial gas velocity, increasing the inlet dust concentration properly, or decreasing the moving velocity of the capturing particles. A model covering the above operation parameters is established to calculate the collection efficiency of the moving bed granular filter. It is used in a wide range of operating parameters for the MBGFs.
基金This work was supported by the National Key R&D Program of China(Grant No.2016YFB0601101)the National Natural Sci-ence Foundation of China(Grant No.51576194).
文摘The dual-layer granular bed filter packed with randomly arranged granules was simulated to study the effects of bed depth of the lower layer of fine granules and the inlet gas velocity on the collection mechanism.The computational results show that the collection efficiency is much better from this granular bed than a single-layer granular bed,especially for particle diameters of 1-10μm.The inlet gas velocity has less effect on the grade collection efficiency of the dual-layer granular bed than of the single-layer granular bed.The dual-layer granular bed provides a high collection efficiency and low pressure drop.The relationship between the grade collection efficiency and the Stokes number(St)based on the inlet gas velocity is obtained.If St is below a threshold,the grade collection efficiency remains stable;if St is in value above threshold,the grade collection efficiency increases linearly with lg(St).As the bed depth of the lower layer of fine granules increases,the threshold for St shifts forward.
基金the support of the National Key Research and Development Program of China(2018YFB0605903)for this study.
文摘The filtration of mixed dust that included a small number of melted(liquid)particles was studied in an experimental granular bed filter(GBF).Results show that the collection efficiency of dust containing melted particles is higher than that of dust composed of solid particles but the pressure drop from the former is higher than that of the latter.The collection efficiency and pressure drop increase as the concentration of melted particles increases.A surface sliding GBF exhibits good comprehensive performance when filtering dust,especially dust containing a mix of solid and liquid particles.The effects of the gas temperature,gas velocity,sliding filter bed thickness,and sliding collector flux on filter performance were also examined.Based on the experimental results,correlations for the collection efficiency and pressure drop for mixed dust are presented.
基金support of the National Key Research and Development Program of China(grant No.2018YFB0605903)to this study.
文摘Granular bed filters can effectively filter adhesive dust in high-temperature flue gas.In this study.polyvinyl chloride(PVC)powder was used as adhesive dust,and the mixture of PVC and ash powder was used to simulate solid and adhesive mixed dust.The effects of gas temperature,velocity,and inlet adhesive dust mass content on dust distribution in granular bed(GBF)were discussed.Results show that the mixed dust mainly accumulates on the upper part of the granular bed,and the mass of the collected dust decreases exponentially from the upper layer to the bottom layer in the GBF.The adhesive dust content collected in each layer differs from that of the incoming dust,and their deviation varies approximately linearly along with the depth of the bed.The total dust distribution and adhesive dust content deviation are influenced by gas temperature and inlet adhesive dust content but independent of gas velocity.The correlations of dust distribution of solid and adhesive mixed dust are presented based on the experimental results.
基金supported by National Key Research and Development Program of China(No.2018YFB0606104).
文摘The coupled CFD-DEM method with the JKR(Johnson-Kendall-Roberts)model for describing the contact adhesion of dust to filter particles(FPs)is used to simulate the distribution pattern of dust particle deposition in the granular bed filter(GBF)with multi-layer media.The minimum inlet flow velocity must meet the requirement that the contact probability between dust and FPs is in the high contact probability region.The air flow forms vortices on the leeward side of the FPs and changes abruptly at the intersection of different particle size FPs layers.Dust particles form large deposits at the intersection of the first and second layers and the different particle size filter layers.Dual element multilayer GBF can further optimize the bed structure by interlacing filter layers with different particle sizes.Compared with single particle size multi-layer GBF,the bed pressure drop is reduced by 40.24%-50.65%and the dust removal efficiency is increased by 21.93%-55.09%.
基金This research was supported by the Natural Science Foundation of China(Grant No.50378094).
文摘Shortcut nitrification-denitrification,anaerobic ammonium oxidation(ANAMMOX),and methanogenesis have been successfully coupled in an Expanded Granular Sludge Bed-Biological Aerated Filter(EGSB-BAF)integrated system.As fed different synthetic wastewater with chemical oxygen demand(COD)of 300-1200 mg·L^(-1)and NH_(4)^(+)-N of 30-120 mg·L^(-1)at the outer recycle ratio of 200%,the influence of influent on ANAMMOX in the integrated system was investigated in this paper.The experimental results showed that higher COD concentration caused an increase in denitrification and methanogenesis but a decrease in ANAMMOX;however,when an influent with the low concentration of COD was used,the opposite changes could be observed.Higher influent NH_(4)^(+)-N concentration favored ANAMMOX when the COD concentration of influent was fixed.Therefore,low COD=NH_(4)^(+)-N ratio would decrease competition for nitrite between ANAMMOX and denitrification,which was favorable for reducing the negative effect of organic COD on ANAMMOX.The good performance of the integrated system indicated that the bacterial community of denitrification,ANAMMOX,and methanogenesis could be dynamically maintained in the sludge of EGSB reactor for a certain range of influent.
文摘Combustion-generated hydrogen chloride （HCl） is considered to be a very hazardous acid gaseous pollutant. This paper presents a laboratory study on the dry adsorption of HCl. The experiments were conducted in a dual-layer granular bed filter, at gas temperatures of 500℃-700℃ and n（Ca）/n（Cl）molar ratios of 1.0-5.0 using the silver nitrate titration method by dry adsorbent powders Ca（OH）2. Mainly, the adsorption efficiency of HCI and utilization efficiency of Calcium were studied, by varying relevant factors including n（Ca）/n（Cl）, tempera- ture, feeding method, water vapor and CO2. With a relatively higher HCl concentration of 1000ppm, the experimental results revealed that 600℃ may be the optimum temperature for HCl adsorption when optimum n （Ca）/n（Cl） was 2.5 in our tests. The results also demonstrated that the feeding at a constant pressure was more effective, and the HCl adsorption efficiency could rapidly reach over 90% with n（Ca）/n（Cl） = 2.5 at 600℃. Furthermore, the HCl adsorption efficiency was found to be slightly promoted by water vapor, while could be impeded by CO2, and the utilization efficiency of calcium could be up to 74.4% without CO2, while was only 36.8% with CO2 when n（Ca）/n（Cl） was 2.5 at 600℃.
