X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast scien...X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast science.Recently,there has been a growing demand for X-ray pulses with high photon energy,especially from developments in“diffraction-before-destruction”applications and in dynamic mesoscale materials science.Here,we propose utilizing the electron beams at XFELs to drive a meter-scale two-bunch plasma wakefield accelerator and double the energy of the accelerated beam in a compact and inexpensive way.Particle-in-cell simulations are performed to study the beam quality degradation under different beam loading scenarios and nonideal issues,and the results show that more than half of the accelerated beam can meet the requirements of XFELs.After its transport to the undulator,the accelerated beam can improve the photon energy to 22 keV by a factor of around four while maintaining the peak power,thus offering a promising pathway toward high-photon-energy XFELs.展开更多
Owing to their ultra-high accelerating gradients,combined with injection inside micrometer-scale accelerating wakefield buckets,plasma-based accelerators hold great potential to drive a new generation of free-electron...Owing to their ultra-high accelerating gradients,combined with injection inside micrometer-scale accelerating wakefield buckets,plasma-based accelerators hold great potential to drive a new generation of free-electron lasers(FELs).Indeed,the first demonstration of plasma-driven FEL gain was reported recently,representing a major milestone for the field.Several groups around the world are pursuing these novel light sources,with methodology varying in the use of wakefield driver(laser-driven or beam-driven),plasma structure,phase-space manipulation,beamline design,and undulator technology,among others.This paper presents our best attempt to provide a comprehensive overview of the global community efforts towards plasma-based FEL research and development.展开更多
A simple analysis is given for the optimum length of undulator in a self-seeding free electron laser （FEL）. The obtained relations show the correlation between the undulator length and the system parameters. The pow...A simple analysis is given for the optimum length of undulator in a self-seeding free electron laser （FEL）. The obtained relations show the correlation between the undulator length and the system parameters. The power required for the seeding in the second part of the undulator and the overall efficiency of monochromatizating the seeding determine the length of the first part of the undulator; the magnitude of seeding power dominates the length of the second part of the undulator; the whole length of the undulator in a self-seeding FEL is determined by the overall efficiency for getting coherent seed, and is about half as long again as that of SASE, not including the dispersion section. The requirement of the dispersion section strength is also analyzed.展开更多
The high temporal and spatial coherence of free electron lasers(FELs)reduces the uniformity of the illumination field,leading to scattering effects that blur the edges of patterns,resulting in diminished accuracy and ...The high temporal and spatial coherence of free electron lasers(FELs)reduces the uniformity of the illumination field,leading to scattering effects that blur the edges of patterns,resulting in diminished accuracy and clarity.Traditional imaging models regard the light source as fully incoherent,making it difficult to assess the impact of partially coherent light fields on imaging.If FELs are used in imaging systems,their coherence must be considered.To address this issue,this study explores the relationship between coherence,imaging quality and speckle contrast through a simulation method based on random phases.The method divides the light beam into temporal and spatial coherence cells,analyzes their interactions,and simulates imaging results under different coherence conditions.Additionally,speckle patterns for various illumination modes are calculated to evaluate their effects on speckle contrast and illumination uniformity.The results indicate that under different illumination modes,illumination uniformity decreases as coherence increases,while speckle contrast increases with higher coherence.In terms of imaging quality,higher coherence leads to an increase in both line edge roughness(LER)and line width roughness(LWR),thereby reducing the imaging quality.Additionally,the narrower the line width,the greater the impact of coherence on the imaging quality,resulting in poorer imaging performance.展开更多
A thermionic gun is endowed with a long bunch tail,which presents challenges for the compact terahertz free electron laser(FEL)facility at the Huazhong University of Science and Technology.Owing to a large energy spre...A thermionic gun is endowed with a long bunch tail,which presents challenges for the compact terahertz free electron laser(FEL)facility at the Huazhong University of Science and Technology.Owing to a large energy spread,the tail particles do not contribute to the radiation.In the original design,an x-direction slit is used in the dispersive section of the transport line to remove the tail particles.This paper presents an improved scheme to remove the tail by introducing an RF beam chopper system at the exit of the electron gun,to prevent a significant number of tail particles from entering the linac.The facility remains compact while effectively removing the tail of the bunch.The parameters of the beam chopper system are designed.Bunch parameters and radiation performance are analyzed via a start-to-end simulation.The findings indicate that 43%of the particles can pass through the beam chopper system for subsequent acceleration and transport,which saves the RF power,reduces beam loss in the linac,reduces background noise,and suppresses the sideband instability.Simultaneously,the beam chopper system causes an increase in beam emittance,energy spread,and an offset in the center of the bunch.These effects can be mitigated by a solenoid,linac,and steering coils.The simulation results for the FEL show that the micro-pulse energy is greater than 1.1μJ in the frequency range of 2.8-9.7 THz,and the maximum micro-pulse energy is 1.28μJ.展开更多
Attosecond soft X-ray pulses are of great importance for the study of ultrafast electronic phenomena.In this paper,a feasible method is proposed to generate isolated fully coherent attosecond soft X-ray free electron ...Attosecond soft X-ray pulses are of great importance for the study of ultrafast electronic phenomena.In this paper,a feasible method is proposed to generate isolated fully coherent attosecond soft X-ray free electron laser via optical frequency beating.Two optical lasers with the opposite frequency chirps are used to induce a gradient frequency energy modulation,which helps to generate a gradually varied spacing electron pulse train.Subsequently,the undulator sections with electron beam delay lines are used to amplify the target ultra-short radiation.Numerical start-to-end simulations have been performed and the results demonstrate that an isolated soft X-ray pulse with the peak power of 330 GW and pulse duration of 620 as can be achieved by the proposed technique.展开更多
A novel Smith-Purcell （S-P） free electron laser composed of an electron gun, a semi-elliptical resonator, a metallic reflecting grating and a collector, is presented for the first time. This paper studies the charac...A novel Smith-Purcell （S-P） free electron laser composed of an electron gun, a semi-elliptical resonator, a metallic reflecting grating and a collector, is presented for the first time. This paper studies the characteristics of this device by theoretical analysis and particle-in-cell simulation method. Results indicate that tunable coherent S-P radiation with a high output peak power at millimeter wavelengths can be generated by adjusting the length of the grating period, or adjusting the voltage of the electron beam. The present scheme has the following advantages： the semi-elliptical resonator can reflect all radiation with the emission angle {？ and random azimuthal angles, back onto the electron beam with same-phase and causes the electrons to be modulated, so the output power and efficiency are improved.展开更多
The Shanghai soft X-ray free-electron laser(SXFEL)user facility project started in 2016 and is expected to be open to users by 2022.It aims to deliver ultra-intense coherent femtosecond X-ray pulses to five endstation...The Shanghai soft X-ray free-electron laser(SXFEL)user facility project started in 2016 and is expected to be open to users by 2022.It aims to deliver ultra-intense coherent femtosecond X-ray pulses to five endstations covering a range of 100–620 eV for ultrafast X-ray science.Two undulator lines are designed and constructed,based on different lasing modes:self-amplified spontaneous emission and echo-enabled harmonic generation.The coherent scattering and imaging(CSI)endstation is the first of five endstations to be commissioned online.It focuses on high-resolution single-shot imaging and the study of ultrafast dynamic processes using coherent forward scattering techniques.Both the single-shot holograms and coherent diffraction patterns were recorded and reconstructed for nanoscale imaging,indicating the excellent coherence and high peak power of the SXFEL and the possibility of‘‘diffraction before destruction’’experiments at the CSI endstation.In this study,we report the first commissioning results of the CSI endstation.展开更多
Spectroscopic characterization of clusters is crucial to understanding the structures and reaction mechanisms at the microscopic level,but it has been proven to be a grand challenge for neutral clusters because the ab...Spectroscopic characterization of clusters is crucial to understanding the structures and reaction mechanisms at the microscopic level,but it has been proven to be a grand challenge for neutral clusters because the absence of a charge makes it di伍cult for the size selection and detection.Infrared(IR)spectroscopy based on threshold photoionization using a tunable vacuum ultraviolet free electron laser(VUV-FEL)has recently been developed in the lab.The IR-VUV depletion and IR+VUV enhancement spectroscopic techniques open new avenues for size-selected IR spectroscopies of a large variety of neutral clusters without confinement(i.e.,an ultraviolet chromophore,a messenger tag,or a host matrix).The spectroscopic principles have been demonstrated by investigations of some neutral water clusters and some metal carbonyls.Here,the spectroscopic principles and their applications for neutral clusters are reviewed.展开更多
Photodissociation of H2S in the VUV region plays an important role in the atmospheric chemistry and interstellar chemistry.To date,however,few studies have been focused on this topic.In this article,we have described ...Photodissociation of H2S in the VUV region plays an important role in the atmospheric chemistry and interstellar chemistry.To date,however,few studies have been focused on this topic.In this article,we have described a laser dispersion method applied in the apparatus combining the high-n H atom Rydberg tagging time-of-flight technique with the vacuum ultraviolet free electron laser(VUV FEL).The Lyman-αlaser beam(121.6 nm)used in the H-atom detection was generated by the difference frequency four-wave mixing schemes in a Kr/Ar gas cell.After passing through an off-axis biconvex LiF lens,the 121.6 nm beam was dispersed from the 212.6 nm and 845 nm beams due to the different deflection angles experienced by these laser beams at the surfaces of the biconvex lens.This method can eliminate the background signal from the 212.6 nm photolysis.Combined with the VUV FEL,photodissociation of H2S at 122.95 nm was studied successfully.The TOF spectrum was measured and the derived total kinetic energy release spectrum was displayed.The results suggest that the experimental setup is a powerful tool for investigating photodissociation dynamics of molecules in the VUV region which involves the H-atom elimination processes.展开更多
A theory for a two-stream free-electron laser （FEL） with an electromagnetic wiggler （EMW） and axial guide magnetic field is developed. In the analysis, the effects of self-fields are taken into account. The growth...A theory for a two-stream free-electron laser （FEL） with an electromagnetic wiggler （EMW） and axial guide magnetic field is developed. In the analysis, the effects of self-fields are taken into account. The growth rate is derived. The characteristics of the growth rate are studied numerically. The dependence of the normalized wave number, which corresponds to the maximum growth rate, on the cyclotron frequency is presented. The comparisons between the normalized maximum growth rate and its corresponding wave number normalized by employing the axial magnetic field, for the cases with and without self-fields in the two-stream FEL are studied numerically.展开更多
Cherenkov free electron laser(CFEL)is simulated numerically by using the single particle method to optimize the electron beam.The electron beam is assumed to be moving near the surface of a flat dielectric slab along ...Cherenkov free electron laser(CFEL)is simulated numerically by using the single particle method to optimize the electron beam.The electron beam is assumed to be moving near the surface of a flat dielectric slab along a growing radiation.The set of coupled nonlinear differential equations of motion is solved to study the electron dynamics.For three sets of parameters,in high power CFEL,it is found that an axial magnetic field is always necessary to keep the electron beam in the interaction region and its optimal strength is reported for each case.At the injection point,the electron beam’s distance above the dielectric surface is kept at a minimum value so that the electrons neither hit the dielectric nor move away from it to the weaker radiation fields and out of the interaction region.The optimal electron beam radius and current are thereby calculated.This analysis is in agreement with two previous numerical studies for a cylindrical waveguide but is at odds with analytical treatments of a flat dielectric that does not use an axial magnetic field.This is backed by an interesting physical reasoning.展开更多
Amplification of an electromagnetic wave by a free electron laser （FEL） with a helical wiggler and an ion channel with a periodically varying ion density is examined. The relativistic equation of motion for a single...Amplification of an electromagnetic wave by a free electron laser （FEL） with a helical wiggler and an ion channel with a periodically varying ion density is examined. The relativistic equation of motion for a single electron in the combined wiggler and the periodic ionbchannel fields is solved and the classes of possible trajectories in this configuration are discussed. The gain equation for the FEL in the low-gain-per-pass lirnit is obtained by adding the effect of the periodic ion channel. Numerical calculation is employed to analyse the gain induced by the effects of the non-uniform ion density. The variation of gain with ion-channel density is demonstrated. It is shown that there is a gain enhancement for group I orbits in the presence of a non-uniform ion-channel but not in a uniform one. It is also shown that periodic ion-channel guiding is used to reach the maximum peak gain in a low ion-channel frequency （low ion density）.展开更多
A theory for the two-stream free-electron laser with an electromagnetic wiggler （EMW） and an ion channel guiding is developed. In the analysis, the effects of self-fields have been taken into account. The electron t...A theory for the two-stream free-electron laser with an electromagnetic wiggler （EMW） and an ion channel guiding is developed. In the analysis, the effects of self-fields have been taken into account. The electron trajectories and the small signal gain are derived. The stability of the trajectories, the characteristics of the linear gain and the normalized maximum gain are studied numerically. The dependence of the normalized frequency ω corresponding to the maximum gain on the ion-channel frequency is presented. The results show that there are seven groups of orbits in the presence of the self-fields, which are similar to those reported in the absence of the self-fields. It is also shown that the normalized gains of 2 groups decrease while the rest increase with the increasing normalized ion-channel frequency. Furthermore, it is found that the two-stream instability and the self-field lead to a decrease in the maximum gain except for group 4.展开更多
A theory of a two-stream flee-electron laser in a combined electromagnetic wiggler （EMW） is developed, in which we use an axial-guide magnetic field and take into account the effects of the self-fields. The electron...A theory of a two-stream flee-electron laser in a combined electromagnetic wiggler （EMW） is developed, in which we use an axial-guide magnetic field and take into account the effects of the self-fields. The electron trajectories and the small signal gain are derived. The stability of the trajectories, the characteristics of the linear-gain, and the normalised maximum gain are studied numerically. The results show that there are nine stable groups of orbits in the presence of self-fields instead of seven groups reported in the absence of the self-field. It is also shown that the normalised gains of four groups of the orbits are decreasing and those for the rest of them are increasing with growing J20. Furthermore, it is found that the two-stream laser with seff-field enhances the maximum gain in comparison with the single stream case.展开更多
A theory for the two-stream free-electron laser（TSFEL） with a helical wiggler and an axial guide magnetic field is developed.In the analysis,the effects of self-fields are taken into account.An analysis of the two-s...A theory for the two-stream free-electron laser（TSFEL） with a helical wiggler and an axial guide magnetic field is developed.In the analysis,the effects of self-fields are taken into account.An analysis of the two-stream steady-state electron trajectories is given by solving the equation of motion.Numerical calculations show that there are seven groups of orbits in the presence of self-fields instead of two groups reported in the absence of self-fields.The stability of the trajectories is studied numerically.展开更多
The theory for the two-stream free electron laser （FEL） consisting of a relativistic electron beam transporting along the axis of a helical wiggler in the presence of an axial guiding magnetic field is proposed and ...The theory for the two-stream free electron laser （FEL） consisting of a relativistic electron beam transporting along the axis of a helical wiggler in the presence of an axial guiding magnetic field is proposed and investigated. In the analysis, the effects of self-fields are taken into account. The electron trajectories and the small signal gain are derived. The characteristics of the linear-gain and the normalized maximum gain are studied numerically. The results show that there are seven stable groups of orbits in the presence of self-fields instead of two groups reported in the absence of the self-fields. It is also shown that the normalized gains of three groups decrease while the rest increase with the increasing of normalized cyclotron frequency g20. Furthermore, it is found that the two-stream instability and the self-field lead to a decrease in the maximum gain except for group 3. The results show that the normalized maximum gain is enhanced in comparison with that of the single stream.展开更多
The cross-correlation method for temporal characterization is investigated using simulations of the two- color above threshold ionization （ATI） on He induced by a vacuum ultraviolet （VUV） free-electron laser （FEL...The cross-correlation method for temporal characterization is investigated using simulations of the two- color above threshold ionization （ATI） on He induced by a vacuum ultraviolet （VUV） free-electron laser （FEL） in the presence of an infrared （IR） field. Non-linear dependencies of the sideband structure pro- duced in the two-color ATI process are expressed as a function of IR laser intensity by considering the spatial distributions and temporal jitter of both lasers. The temporal properties of the FEL pulse can be characterized accurately using the cross-correlation method at a low IR laser intensity of ~3~101~ W/cm2 but with low cross-correlation signals. When the dynamic range of sidebands is increased to high IR intensity, the accuracy of the cross-correlation method becomes crucially dependent on the actual non- linear index. An approach of determining this index is proposed here to improve the accuracy of temporal characterizations.展开更多
The interaction between neon and x-ray free-electron lasers with different laser parameters is systematically studied by solving a set of coupled rate equations. As an example, the evolution of 1s^12 s^22 p^6 configur...The interaction between neon and x-ray free-electron lasers with different laser parameters is systematically studied by solving a set of coupled rate equations. As an example, the evolution of 1s^12 s^22 p^6 configuration is given under different incident photon numbers, pulse widths, and photon energies. We have also determined all of the charge-state populations as a function of three laser pulse parameters by averaging over time. The result shows that the variations of these charge-state populations demonstrate a pattern when the pulse width is shorter than 10 fs: some of the charge-states decrease rapidly,while the others rise but remain relatively constant for pulse width larger than 10 fs. The variation of the average charge with three parameters has also obtained. The average charge decreases for a pulse width shorter than 10 fs but remains basically unchanged for a pulse width longer than 10 fs.展开更多
FELiChEM is a new experimental facility under construction at the University of Science and Technology of China（USTC）. Its core device is two free electron laser oscillators generating middle-infrared and far-infrar...FELiChEM is a new experimental facility under construction at the University of Science and Technology of China（USTC）. Its core device is two free electron laser oscillators generating middle-infrared and far-infrared laser and covering the spectral range of 2.5–200 μm. It will be a dedicated infrared light source aiming at energy chemistry research. We present the brief design of the FEL oscillators, with the emphasis put on the middle-infrared oscillator.Most of the basic parameters are determined and the anticipated performance of the output radiation is given. The first light of FELiChEM is targeted for the end of 2017.展开更多
基金supported by the National Grand Instrument Project No. SQ2019YFF01014400the Natural Science Foundation of China (Grant Nos. 12375147, 12435011, 12075030)+2 种基金the Beijing Outstanding Young Scientist Project, Project for Young Scientists in Basic Research of Chinese Academy of Sciences (YSBR-115)the Beijing Normal University Scientific Research Initiation Fund for Introducing Talents No. 310432104the Fundamental Research Funds for the Central Universities, Peking University
文摘X-ray free-electron lasers(XFELs)can generate bright X-ray pulses with short durations and narrow bandwidths,leading to extensive applica-tions in many disciplines such as biology,materials science,and ultrafast science.Recently,there has been a growing demand for X-ray pulses with high photon energy,especially from developments in“diffraction-before-destruction”applications and in dynamic mesoscale materials science.Here,we propose utilizing the electron beams at XFELs to drive a meter-scale two-bunch plasma wakefield accelerator and double the energy of the accelerated beam in a compact and inexpensive way.Particle-in-cell simulations are performed to study the beam quality degradation under different beam loading scenarios and nonideal issues,and the results show that more than half of the accelerated beam can meet the requirements of XFELs.After its transport to the undulator,the accelerated beam can improve the photon energy to 22 keV by a factor of around four while maintaining the peak power,thus offering a promising pathway toward high-photon-energy XFELs.
文摘Owing to their ultra-high accelerating gradients,combined with injection inside micrometer-scale accelerating wakefield buckets,plasma-based accelerators hold great potential to drive a new generation of free-electron lasers(FELs).Indeed,the first demonstration of plasma-driven FEL gain was reported recently,representing a major milestone for the field.Several groups around the world are pursuing these novel light sources,with methodology varying in the use of wakefield driver(laser-driven or beam-driven),plasma structure,phase-space manipulation,beamline design,and undulator technology,among others.This paper presents our best attempt to provide a comprehensive overview of the global community efforts towards plasma-based FEL research and development.
基金Supported by Major State Basic Research Development Program(2011CB808301)National Natural Science Foundation of China(11375199)
文摘A simple analysis is given for the optimum length of undulator in a self-seeding free electron laser （FEL）. The obtained relations show the correlation between the undulator length and the system parameters. The power required for the seeding in the second part of the undulator and the overall efficiency of monochromatizating the seeding determine the length of the first part of the undulator; the magnitude of seeding power dominates the length of the second part of the undulator; the whole length of the undulator in a self-seeding FEL is determined by the overall efficiency for getting coherent seed, and is about half as long again as that of SASE, not including the dispersion section. The requirement of the dispersion section strength is also analyzed.
文摘The high temporal and spatial coherence of free electron lasers(FELs)reduces the uniformity of the illumination field,leading to scattering effects that blur the edges of patterns,resulting in diminished accuracy and clarity.Traditional imaging models regard the light source as fully incoherent,making it difficult to assess the impact of partially coherent light fields on imaging.If FELs are used in imaging systems,their coherence must be considered.To address this issue,this study explores the relationship between coherence,imaging quality and speckle contrast through a simulation method based on random phases.The method divides the light beam into temporal and spatial coherence cells,analyzes their interactions,and simulates imaging results under different coherence conditions.Additionally,speckle patterns for various illumination modes are calculated to evaluate their effects on speckle contrast and illumination uniformity.The results indicate that under different illumination modes,illumination uniformity decreases as coherence increases,while speckle contrast increases with higher coherence.In terms of imaging quality,higher coherence leads to an increase in both line edge roughness(LER)and line width roughness(LWR),thereby reducing the imaging quality.Additionally,the narrower the line width,the greater the impact of coherence on the imaging quality,resulting in poorer imaging performance.
基金supported by the National Natural Science Foundation of China(No.12175077).
文摘A thermionic gun is endowed with a long bunch tail,which presents challenges for the compact terahertz free electron laser(FEL)facility at the Huazhong University of Science and Technology.Owing to a large energy spread,the tail particles do not contribute to the radiation.In the original design,an x-direction slit is used in the dispersive section of the transport line to remove the tail particles.This paper presents an improved scheme to remove the tail by introducing an RF beam chopper system at the exit of the electron gun,to prevent a significant number of tail particles from entering the linac.The facility remains compact while effectively removing the tail of the bunch.The parameters of the beam chopper system are designed.Bunch parameters and radiation performance are analyzed via a start-to-end simulation.The findings indicate that 43%of the particles can pass through the beam chopper system for subsequent acceleration and transport,which saves the RF power,reduces beam loss in the linac,reduces background noise,and suppresses the sideband instability.Simultaneously,the beam chopper system causes an increase in beam emittance,energy spread,and an offset in the center of the bunch.These effects can be mitigated by a solenoid,linac,and steering coils.The simulation results for the FEL show that the micro-pulse energy is greater than 1.1μJ in the frequency range of 2.8-9.7 THz,and the maximum micro-pulse energy is 1.28μJ.
基金supported by the National Natural Science Foundation of China (Nos. 11905275, 11775294, 12122514, and 11975300)the Youth Innovation Promotion Association CAS
文摘Attosecond soft X-ray pulses are of great importance for the study of ultrafast electronic phenomena.In this paper,a feasible method is proposed to generate isolated fully coherent attosecond soft X-ray free electron laser via optical frequency beating.Two optical lasers with the opposite frequency chirps are used to induce a gradient frequency energy modulation,which helps to generate a gradually varied spacing electron pulse train.Subsequently,the undulator sections with electron beam delay lines are used to amplify the target ultra-short radiation.Numerical start-to-end simulations have been performed and the results demonstrate that an isolated soft X-ray pulse with the peak power of 330 GW and pulse duration of 620 as can be achieved by the proposed technique.
基金Project supported by the National Natural Science Foundation of China (Grant No. 60871047)the Natural Science Foundation of Liaocheng University of China (Grant No. X0810018)
文摘A novel Smith-Purcell （S-P） free electron laser composed of an electron gun, a semi-elliptical resonator, a metallic reflecting grating and a collector, is presented for the first time. This paper studies the characteristics of this device by theoretical analysis and particle-in-cell simulation method. Results indicate that tunable coherent S-P radiation with a high output peak power at millimeter wavelengths can be generated by adjusting the length of the grating period, or adjusting the voltage of the electron beam. The present scheme has the following advantages： the semi-elliptical resonator can reflect all radiation with the emission angle {？ and random azimuthal angles, back onto the electron beam with same-phase and causes the electrons to be modulated, so the output power and efficiency are improved.
基金the Shanghai Soft X-ray Free-Electron Laser Facility beamline projectionfunded by the Major State Basic Research Development Program of China(No.2017YFA0504802)+1 种基金Strategic Priority Research Program of the Chinese Academy of Sciences(No.XDB 37040303)National Natural Science Foundation of China(No.21727817).
文摘The Shanghai soft X-ray free-electron laser(SXFEL)user facility project started in 2016 and is expected to be open to users by 2022.It aims to deliver ultra-intense coherent femtosecond X-ray pulses to five endstations covering a range of 100–620 eV for ultrafast X-ray science.Two undulator lines are designed and constructed,based on different lasing modes:self-amplified spontaneous emission and echo-enabled harmonic generation.The coherent scattering and imaging(CSI)endstation is the first of five endstations to be commissioned online.It focuses on high-resolution single-shot imaging and the study of ultrafast dynamic processes using coherent forward scattering techniques.Both the single-shot holograms and coherent diffraction patterns were recorded and reconstructed for nanoscale imaging,indicating the excellent coherence and high peak power of the SXFEL and the possibility of‘‘diffraction before destruction’’experiments at the CSI endstation.In this study,we report the first commissioning results of the CSI endstation.
基金This work was supported by the National Natural Science Foundation of China(No.92061203 and No.21688102)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB17000000)+3 种基金International Partnership Program of Chinese Academy of Sciences(121421KYSB20170012)Chinese Academy of Sciences(GJJSTD20190002)K.C.Wong Education Foundation(GJTD-2018-06)Dalian Institute of Chemical Physics(DICP DCLS201702).
文摘Spectroscopic characterization of clusters is crucial to understanding the structures and reaction mechanisms at the microscopic level,but it has been proven to be a grand challenge for neutral clusters because the absence of a charge makes it di伍cult for the size selection and detection.Infrared(IR)spectroscopy based on threshold photoionization using a tunable vacuum ultraviolet free electron laser(VUV-FEL)has recently been developed in the lab.The IR-VUV depletion and IR+VUV enhancement spectroscopic techniques open new avenues for size-selected IR spectroscopies of a large variety of neutral clusters without confinement(i.e.,an ultraviolet chromophore,a messenger tag,or a host matrix).The spectroscopic principles have been demonstrated by investigations of some neutral water clusters and some metal carbonyls.Here,the spectroscopic principles and their applications for neutral clusters are reviewed.
基金supported by the Strategic Priority Research Program of the Chinese Academy of Sciences (No.XDB17000000)the National Natural Science Foundation of China (NSFC Center for Chemical Dynamics (No.21688102)+4 种基金the National Natural Science Foundation of China (No.21673232, No.21873099, No.21922306)the International Partnership Program of Chinese Academy of Sci-ences (No.121421KYSB20170012)supported by the National Natural Science Foundation of China (No.21973010)supported by the National Natural Science Foundation of China (No.21773236)supported by the Natural Science Research Project of Education Department of Anhui Province (No.KJ2019A0521).
文摘Photodissociation of H2S in the VUV region plays an important role in the atmospheric chemistry and interstellar chemistry.To date,however,few studies have been focused on this topic.In this article,we have described a laser dispersion method applied in the apparatus combining the high-n H atom Rydberg tagging time-of-flight technique with the vacuum ultraviolet free electron laser(VUV FEL).The Lyman-αlaser beam(121.6 nm)used in the H-atom detection was generated by the difference frequency four-wave mixing schemes in a Kr/Ar gas cell.After passing through an off-axis biconvex LiF lens,the 121.6 nm beam was dispersed from the 212.6 nm and 845 nm beams due to the different deflection angles experienced by these laser beams at the surfaces of the biconvex lens.This method can eliminate the background signal from the 212.6 nm photolysis.Combined with the VUV FEL,photodissociation of H2S at 122.95 nm was studied successfully.The TOF spectrum was measured and the derived total kinetic energy release spectrum was displayed.The results suggest that the experimental setup is a powerful tool for investigating photodissociation dynamics of molecules in the VUV region which involves the H-atom elimination processes.
文摘A theory for a two-stream free-electron laser （FEL） with an electromagnetic wiggler （EMW） and axial guide magnetic field is developed. In the analysis, the effects of self-fields are taken into account. The growth rate is derived. The characteristics of the growth rate are studied numerically. The dependence of the normalized wave number, which corresponds to the maximum growth rate, on the cyclotron frequency is presented. The comparisons between the normalized maximum growth rate and its corresponding wave number normalized by employing the axial magnetic field, for the cases with and without self-fields in the two-stream FEL are studied numerically.
文摘Cherenkov free electron laser(CFEL)is simulated numerically by using the single particle method to optimize the electron beam.The electron beam is assumed to be moving near the surface of a flat dielectric slab along a growing radiation.The set of coupled nonlinear differential equations of motion is solved to study the electron dynamics.For three sets of parameters,in high power CFEL,it is found that an axial magnetic field is always necessary to keep the electron beam in the interaction region and its optimal strength is reported for each case.At the injection point,the electron beam’s distance above the dielectric surface is kept at a minimum value so that the electrons neither hit the dielectric nor move away from it to the weaker radiation fields and out of the interaction region.The optimal electron beam radius and current are thereby calculated.This analysis is in agreement with two previous numerical studies for a cylindrical waveguide but is at odds with analytical treatments of a flat dielectric that does not use an axial magnetic field.This is backed by an interesting physical reasoning.
文摘Amplification of an electromagnetic wave by a free electron laser （FEL） with a helical wiggler and an ion channel with a periodically varying ion density is examined. The relativistic equation of motion for a single electron in the combined wiggler and the periodic ionbchannel fields is solved and the classes of possible trajectories in this configuration are discussed. The gain equation for the FEL in the low-gain-per-pass lirnit is obtained by adding the effect of the periodic ion channel. Numerical calculation is employed to analyse the gain induced by the effects of the non-uniform ion density. The variation of gain with ion-channel density is demonstrated. It is shown that there is a gain enhancement for group I orbits in the presence of a non-uniform ion-channel but not in a uniform one. It is also shown that periodic ion-channel guiding is used to reach the maximum peak gain in a low ion-channel frequency （low ion density）.
文摘A theory for the two-stream free-electron laser with an electromagnetic wiggler （EMW） and an ion channel guiding is developed. In the analysis, the effects of self-fields have been taken into account. The electron trajectories and the small signal gain are derived. The stability of the trajectories, the characteristics of the linear gain and the normalized maximum gain are studied numerically. The dependence of the normalized frequency ω corresponding to the maximum gain on the ion-channel frequency is presented. The results show that there are seven groups of orbits in the presence of the self-fields, which are similar to those reported in the absence of the self-fields. It is also shown that the normalized gains of 2 groups decrease while the rest increase with the increasing normalized ion-channel frequency. Furthermore, it is found that the two-stream instability and the self-field lead to a decrease in the maximum gain except for group 4.
文摘A theory of a two-stream flee-electron laser in a combined electromagnetic wiggler （EMW） is developed, in which we use an axial-guide magnetic field and take into account the effects of the self-fields. The electron trajectories and the small signal gain are derived. The stability of the trajectories, the characteristics of the linear-gain, and the normalised maximum gain are studied numerically. The results show that there are nine stable groups of orbits in the presence of self-fields instead of seven groups reported in the absence of the self-field. It is also shown that the normalised gains of four groups of the orbits are decreasing and those for the rest of them are increasing with growing J20. Furthermore, it is found that the two-stream laser with seff-field enhances the maximum gain in comparison with the single stream case.
基金Project supported by the Plasma Physics Research Center,Science and Research Branch,Islamic Azad University
文摘A theory for the two-stream free-electron laser（TSFEL） with a helical wiggler and an axial guide magnetic field is developed.In the analysis,the effects of self-fields are taken into account.An analysis of the two-stream steady-state electron trajectories is given by solving the equation of motion.Numerical calculations show that there are seven groups of orbits in the presence of self-fields instead of two groups reported in the absence of self-fields.The stability of the trajectories is studied numerically.
文摘The theory for the two-stream free electron laser （FEL） consisting of a relativistic electron beam transporting along the axis of a helical wiggler in the presence of an axial guiding magnetic field is proposed and investigated. In the analysis, the effects of self-fields are taken into account. The electron trajectories and the small signal gain are derived. The characteristics of the linear-gain and the normalized maximum gain are studied numerically. The results show that there are seven stable groups of orbits in the presence of self-fields instead of two groups reported in the absence of the self-fields. It is also shown that the normalized gains of three groups decrease while the rest increase with the increasing of normalized cyclotron frequency g20. Furthermore, it is found that the two-stream instability and the self-field lead to a decrease in the maximum gain except for group 3. The results show that the normalized maximum gain is enhanced in comparison with that of the single stream.
基金supported by the National Natural Science Foundation of China(No.11075118)the Specialized Research Fund for the Doctoral Program of Higher Education(No.20100072120036)
文摘The cross-correlation method for temporal characterization is investigated using simulations of the two- color above threshold ionization （ATI） on He induced by a vacuum ultraviolet （VUV） free-electron laser （FEL） in the presence of an infrared （IR） field. Non-linear dependencies of the sideband structure pro- duced in the two-color ATI process are expressed as a function of IR laser intensity by considering the spatial distributions and temporal jitter of both lasers. The temporal properties of the FEL pulse can be characterized accurately using the cross-correlation method at a low IR laser intensity of ~3~101~ W/cm2 but with low cross-correlation signals. When the dynamic range of sidebands is increased to high IR intensity, the accuracy of the cross-correlation method becomes crucially dependent on the actual non- linear index. An approach of determining this index is proposed here to improve the accuracy of temporal characterizations.
基金Project supported by the National Natural Science Foundation of China(Grant No.11474208)
文摘The interaction between neon and x-ray free-electron lasers with different laser parameters is systematically studied by solving a set of coupled rate equations. As an example, the evolution of 1s^12 s^22 p^6 configuration is given under different incident photon numbers, pulse widths, and photon energies. We have also determined all of the charge-state populations as a function of three laser pulse parameters by averaging over time. The result shows that the variations of these charge-state populations demonstrate a pattern when the pulse width is shorter than 10 fs: some of the charge-states decrease rapidly,while the others rise but remain relatively constant for pulse width larger than 10 fs. The variation of the average charge with three parameters has also obtained. The average charge decreases for a pulse width shorter than 10 fs but remains basically unchanged for a pulse width longer than 10 fs.
基金Supported by National Natural Science Foundation of China(21327901)
文摘FELiChEM is a new experimental facility under construction at the University of Science and Technology of China（USTC）. Its core device is two free electron laser oscillators generating middle-infrared and far-infrared laser and covering the spectral range of 2.5–200 μm. It will be a dedicated infrared light source aiming at energy chemistry research. We present the brief design of the FEL oscillators, with the emphasis put on the middle-infrared oscillator.Most of the basic parameters are determined and the anticipated performance of the output radiation is given. The first light of FELiChEM is targeted for the end of 2017.
