In this study,we theoretically investigate the feasibility of using laser-wakefield accelerated(LWFA)electrons for the photonuclear measurement of nuclear isomers according to the characteristics of the electrons obta...In this study,we theoretically investigate the feasibility of using laser-wakefield accelerated(LWFA)electrons for the photonuclear measurement of nuclear isomers according to the characteristics of the electrons obtained from LWFA experiments conducted at the Compact Laser-Plasma Accelerator(CLAPA)laboratory.The experiments at the CLAPA show that a stable electron beam with an energy of 78-135 MeV and a charge of 300-600 pC can be obtained.The bremsstrahlung spectra were simulated using Geant4,which suggests that a bremsstrahlung source with a peak intensity of 10^(19) photons/s can be generated.Theoretical calculations of isomer production cross sections from the photonuclear reactions on six target nuclei,^(197)Au,^(180)Hf,^(159)Tb,^(115)In,^(103)Rh,and ^(90)Zr,were performed and compared with the available experimental data in EXFOR,which suggest that further experiments are required for a series of photonuclear reaction channels.Flux-averaged cross sections and isomer ratios(IR)resulting from such bremsstrahlung sources are theoretically deduced.The results suggest that IR measurements can be used to constrain nuclear components,such asγstrength function and optical model potential.In addition,the detection of the decay characteristics was evaluated with Geant4 simulations.The use of the LWFA electron beam and its bremsstrahlung for photonuclear studies involving nuclear isomers is anticipated.展开更多
The photoneutron reaction^(18)Ta(y,3m)(178m,g)Ta was investigated with the beam from the NSC KIPT electron linear accelerator LUE-40.The measurements were performed using the residual y-activity method.The bremsstrahl...The photoneutron reaction^(18)Ta(y,3m)(178m,g)Ta was investigated with the beam from the NSC KIPT electron linear accelerator LUE-40.The measurements were performed using the residual y-activity method.The bremsstrahlung flux-averaged cross sections((E_(γmax))>.(r(E_(γmax))>m.<r(E_(γmax))g and the isomerie ratio of the re-action products d(E_(γmax))were measured.The theoretical values of the averaged cross-sections and isomeric ratio were calculated using the partial cross-sections from the TALYS1.95 code for different level density models LD 1-6..The obtained experimental d(E_(γmax))agree with the data in the lterature,but differ from the theoretical values in ab-solute magnitude and the behavior of the energy dependence.A comparison of the determined averaged cross-sec-tions with the calculated cross sections showed the best agreement for the case of the LD 5 model.展开更多
The flux-averaged cross-sections<σ(E_(γmax))>for the reactions^(65)Cu(γ,n)^(64)Cu,^(63)Cu(γ,n)^(62)Cu,^(63)Cu(γ,2n)^(61)Cu,and^(63)Cu(γ,3n)^(60)Cu have been measured within the bremsstrahlung end-point ene...The flux-averaged cross-sections<σ(E_(γmax))>for the reactions^(65)Cu(γ,n)^(64)Cu,^(63)Cu(γ,n)^(62)Cu,^(63)Cu(γ,2n)^(61)Cu,and^(63)Cu(γ,3n)^(60)Cu have been measured within the bremsstrahlung end-point energy E_(γmax)range of 35–94 MeV.The experiments were performed with the electron beam from the NSC KIPT linear accelerator LUE-40 with the use of the activation and off-lineγ-ray spectrometric techniques.Theoretical calculation of the flux-average cross-sections<σ(E_(γmax))>_(th)was conducted using the cross-sectionσ(E)values from the TALYS1.95 code,run with default options.It is shown that the experimental average cross-sections for the reactions^(65)Cu(γ,n)^(64)Cu,^(63)Cu(γ,n)^(62)Cu,and^(63)Cu(γ,2n)^(61)Cu are systematically higher than the theoretical estimates based on the TALYS1.95 code.The obtained<σ(E_(γmax))values supplement the data of different laboratories for the(γ,n)and(γ,2n)reactions of^(63)Cu and^(65)Cu.For the reaction^(63)Cu(γ,3n)^(60)Cu,the values of<σ(E_(γmax))>were measured for the first time.展开更多
The bremsstrahlung flux-averaged cross-sections(σ(Eγmax))and the cross-sections per equivalent photon(σ(Eγmax)Q)were first measured for the photonuclear multichannel reaction ^(27)Al(γ,x)22 Na at end-point bremss...The bremsstrahlung flux-averaged cross-sections(σ(Eγmax))and the cross-sections per equivalent photon(σ(Eγmax)Q)were first measured for the photonuclear multichannel reaction ^(27)Al(γ,x)22 Na at end-point bremsstrahlung gamma energies ranging from 35 MeV to 95 MeV.The experiments were performed with the beam from the NSC KIPT electron linear accelerator LUE-40 using theγ-activation technique.The bremsstrahlung quantum flux was calculated with the GEANT4.9.2 program and was also monitored via the ^(100)Mo(γ,n)^(99)Mo reaction.The flux-averaged cross-sections were calculated using the partial cross-sectionσ(E)values computed with the TALYS1.95 code for different level density models.Consideration is given to special features of calculating the cross-sections<σ(Eγmax)>and<σ(Eγmax)Q>for the case of the final nucleus ^(22)Na via several partial channels x:nα+dt+npt+2 n^(3) He+n2d+2 npd+2 p3 n.展开更多
基金supported by the National Natural Science Foundation of China (Nos.11921006,U2230133)Beijing Outstanding Young Scientists Program+2 种基金National Grand Instrument Project (No.2019YFF01014400)National Key R&D Program of China (No.2022YFA1603303)Open Foundation of Key Laboratory of High Power Laser and Physics,Chinese Academy of Sciences (No.SGKF202104)。
文摘In this study,we theoretically investigate the feasibility of using laser-wakefield accelerated(LWFA)electrons for the photonuclear measurement of nuclear isomers according to the characteristics of the electrons obtained from LWFA experiments conducted at the Compact Laser-Plasma Accelerator(CLAPA)laboratory.The experiments at the CLAPA show that a stable electron beam with an energy of 78-135 MeV and a charge of 300-600 pC can be obtained.The bremsstrahlung spectra were simulated using Geant4,which suggests that a bremsstrahlung source with a peak intensity of 10^(19) photons/s can be generated.Theoretical calculations of isomer production cross sections from the photonuclear reactions on six target nuclei,^(197)Au,^(180)Hf,^(159)Tb,^(115)In,^(103)Rh,and ^(90)Zr,were performed and compared with the available experimental data in EXFOR,which suggest that further experiments are required for a series of photonuclear reaction channels.Flux-averaged cross sections and isomer ratios(IR)resulting from such bremsstrahlung sources are theoretically deduced.The results suggest that IR measurements can be used to constrain nuclear components,such asγstrength function and optical model potential.In addition,the detection of the decay characteristics was evaluated with Geant4 simulations.The use of the LWFA electron beam and its bremsstrahlung for photonuclear studies involving nuclear isomers is anticipated.
文摘The photoneutron reaction^(18)Ta(y,3m)(178m,g)Ta was investigated with the beam from the NSC KIPT electron linear accelerator LUE-40.The measurements were performed using the residual y-activity method.The bremsstrahlung flux-averaged cross sections((E_(γmax))>.(r(E_(γmax))>m.<r(E_(γmax))g and the isomerie ratio of the re-action products d(E_(γmax))were measured.The theoretical values of the averaged cross-sections and isomeric ratio were calculated using the partial cross-sections from the TALYS1.95 code for different level density models LD 1-6..The obtained experimental d(E_(γmax))agree with the data in the lterature,but differ from the theoretical values in ab-solute magnitude and the behavior of the energy dependence.A comparison of the determined averaged cross-sec-tions with the calculated cross sections showed the best agreement for the case of the LD 5 model.
文摘The flux-averaged cross-sections<σ(E_(γmax))>for the reactions^(65)Cu(γ,n)^(64)Cu,^(63)Cu(γ,n)^(62)Cu,^(63)Cu(γ,2n)^(61)Cu,and^(63)Cu(γ,3n)^(60)Cu have been measured within the bremsstrahlung end-point energy E_(γmax)range of 35–94 MeV.The experiments were performed with the electron beam from the NSC KIPT linear accelerator LUE-40 with the use of the activation and off-lineγ-ray spectrometric techniques.Theoretical calculation of the flux-average cross-sections<σ(E_(γmax))>_(th)was conducted using the cross-sectionσ(E)values from the TALYS1.95 code,run with default options.It is shown that the experimental average cross-sections for the reactions^(65)Cu(γ,n)^(64)Cu,^(63)Cu(γ,n)^(62)Cu,and^(63)Cu(γ,2n)^(61)Cu are systematically higher than the theoretical estimates based on the TALYS1.95 code.The obtained<σ(E_(γmax))values supplement the data of different laboratories for the(γ,n)and(γ,2n)reactions of^(63)Cu and^(65)Cu.For the reaction^(63)Cu(γ,3n)^(60)Cu,the values of<σ(E_(γmax))>were measured for the first time.
文摘The bremsstrahlung flux-averaged cross-sections(σ(Eγmax))and the cross-sections per equivalent photon(σ(Eγmax)Q)were first measured for the photonuclear multichannel reaction ^(27)Al(γ,x)22 Na at end-point bremsstrahlung gamma energies ranging from 35 MeV to 95 MeV.The experiments were performed with the beam from the NSC KIPT electron linear accelerator LUE-40 using theγ-activation technique.The bremsstrahlung quantum flux was calculated with the GEANT4.9.2 program and was also monitored via the ^(100)Mo(γ,n)^(99)Mo reaction.The flux-averaged cross-sections were calculated using the partial cross-sectionσ(E)values computed with the TALYS1.95 code for different level density models.Consideration is given to special features of calculating the cross-sections<σ(Eγmax)>and<σ(Eγmax)Q>for the case of the final nucleus ^(22)Na via several partial channels x:nα+dt+npt+2 n^(3) He+n2d+2 npd+2 p3 n.
