With a three-dimensional semiclassical ensemble method, we theoretically investigated the nonsequential double ionization of Ar driven by the spatially inhomogeneous few-cycle negatively chirped laser pulses. Our resu...With a three-dimensional semiclassical ensemble method, we theoretically investigated the nonsequential double ionization of Ar driven by the spatially inhomogeneous few-cycle negatively chirped laser pulses. Our results show that the recollision time window can be precisely controlled within an isolated time interval of several hundred attoseconds, which is useful for understanding the subcycle correlated electron dynamics. More interestingly, the correlated electron momentum distribution (CEMD) exhibits a strong dependence on laser intensity. That is, at lower laser intensity, CEMD is located in the first quadrant. As the laser intensity increases,CEMD shifts almost completely to the second and fourth quadrants, and then gradually to the third quadrant.The underlying physics governing the CEMD's dependence on laser intensity is explained.展开更多
In this article, a modified version of the Differential Transform Method (DTM) is employed to examine soliton pulse propagation in a weakly non-local parabolic law medium and wave propagation in optical fibers. This s...In this article, a modified version of the Differential Transform Method (DTM) is employed to examine soliton pulse propagation in a weakly non-local parabolic law medium and wave propagation in optical fibers. This semi-analytic method has the advantage of overcoming the obstacle of the hardest nonlinear terms and is used to explain the origin of the bright and dark soliton solutions through the Schrödinger equation in its non-local form and the Radhakrishnan-Kundu-Laksmannan (RKL) equation. Numerical examples demonstrate the effectiveness of this method.展开更多
In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved ...In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved in two steps. The detailed analysis of computational results of a PDE with a single detonation tube and a PDE with five detonation tubes are given in this paper. Complex wave systems are observed inside and outside a PDE. For a PDE with 5 detonation tubes, there is a big bow shock produced from a number of little shocks near the open ends of tubes. A lot of vortexes interact with shocks and a large expansion wave propagates forward and backward with respect to the PDE in a semi-oval shape.展开更多
In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the sol...In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the soliton selffrequency shift is remarkable and the photonic crystal fibre (PCF) parameters vary with the frequency considerably. The precision of numerical simulation by using ASSFM is higher than that by using split-step Fourier method in the process of laser pulse propagation in PCFs due to the fact that the variation of fibre parameters with the peak frequency in the pulse spectrum can be taken into account fully.展开更多
The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an i...The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an initially big spiral can successfully transfer to several small spirals by applying a pulse array method. The impacts of several important factors, such as array density, controlling intensity and pulsing time, are investigated. This control approach may be useful for the control of 2D spatiotemporal patterns and has potential applications in the control of some realistic systems, such as meteorological and cardiac systems.展开更多
In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detect...In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detector following atmospheric transmission.To quantitatively analyze the effects of different satellite detection altitudes,burst heights,and transmission angles on the physical processes of X-ray transport and energy fluence,we developed an atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering correction.The proposed method is an improvement over the traditional analytical method that only computes direct-transmission X-rays.The traditional analytical method exhibits a maximum relative error of 67.79% compared with the Monte Carlo method.Our improved method reduces this error to within 10% under the same conditions,even reaching 1% in certain scenarios.Moreover,its computation time is 48,000 times faster than that of the Monte Carlo method.These results have important theoretical significance and engineering application value for designing satellite-borne nuclear detonation pulsed X-ray detectors,inverting nuclear detonation source terms,and assessing ionospheric effects.展开更多
Lherzolite is one of the most important components of the subcontinental mantle lithosphere, and the study of its heat transfer properties aids in understanding the thermal structure of the continental mantle lithosph...Lherzolite is one of the most important components of the subcontinental mantle lithosphere, and the study of its heat transfer properties aids in understanding the thermal structure of the continental mantle lithosphere. Currently, few studies have examined the heat transfer properties of lherzolite, and the experimental results remain controversial. This experiment utilized a pulse method to measure the thermal diffusivity of lherzolite at pressures ranging from 1.0 to 4.0 GPa and temperatures from 300 to 1 073 K on a cubic press apparatus. We obtained a thermal diffusivity for lherzolite of approximately 2.10 mm^2s^(-1) at ambient condition. The experimental pressure derivative of the thermal conductivity of lherzolite decreased with temperature, reaching approximately 10% at high temperature, a value higher than the previously reported 4%, which indicates that the temperature gradient of the upper mantle lithosphere is smaller than previously thought. Therefore, concerning calculation of the lithosphere thickness using the thermal conductivity of the lherzolite, the previous calculation using pressure derivative of the thermal conductivity of 4% may cause an underestimation of the upper mantle lithosphere thickness by approximately 6% in a first approximation.展开更多
In order to test the feasibility of a new thrust stand system based on impulse thrust mea- surement method, a liquid-fueled pulse detonation engine (PDE) is designed and built. Thrust per- formance of the engine is ...In order to test the feasibility of a new thrust stand system based on impulse thrust mea- surement method, a liquid-fueled pulse detonation engine (PDE) is designed and built. Thrust per- formance of the engine is obtained by direct thrust measurement with a force transducer and indirect thrust measurement with an eddy current displacement sensor (ECDS). These two sets of thrust data are compared with each other to verify the accuracy of the thrust performance. Then thrust data measured by the new thrust stand system are compared with the verified thrust data to test its feasibility. The results indicate that thrust data from the force transducer and ECDS system are consistent with each other within the range of measurement error. Though the thrust data from the impulse thrust measurement system is a litter lower than that from the force transducer due to the axial momentum losses of the detonation jet, the impulse thrust measurement method is valid when applied to measure the averaged thrust of PDE. Analytical models of PDE are also discussed in this paper. The analytical thrust performance is higher than the experimental data due to ignoring the losses during the deflagration to detonation transition process. Effect of equivalence ratio on the engine thrust performance is investigated by utilizing the modified analytical model. Thrust reaches maximum at the equivalence ratio of about 1.1.展开更多
A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite e...A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite element method (FEM) is used to solve Poisson's equation. In the proposed method, photoionization is considered by adopting an exact Helmholtz photoionization model. Furthermore, fully implicit discretization and variable time step are used to ensure the time-efficiency of the present method. Finally, the method is applied to a positive rod-plane corona problem. The numerical results are in agreement with the experimental results, and the validity of the proposed method is verified.展开更多
The pressing environmental concerns and the depletion of fossil fuel reserves necessitate a transition toward sustainable energy sources.Ethanol,a renewable biomass-derived fuel,is a promising alternative due to its a...The pressing environmental concerns and the depletion of fossil fuel reserves necessitate a transition toward sustainable energy sources.Ethanol,a renewable biomass-derived fuel,is a promising alternative due to its availability and high energy density.This study investigates the synthesis of gold nanoparticles(Au NPs)via a square-wave pulse deposition technique,aiming to enhance catalytic activity for ethanol electrooxidation.By varying pulse durations,we were able to exert precise control over Au NP size and distribution without stabilizing agents.Characterization using field emission scanning electron microscopy and X-ray diffraction techniques confirmed the formation of clustered nanoparticles of metallic gold phase.Electrochemical characteristics analyses revealed that Au NPs synthesized with a 900 ms pulse duration exhibited the lowest charge transfer resistance and the highest electrochemically active surface area.The electrocatalytic performance test of these Au NPs demonstrated an anodic current density of 2.5 mA cm^-(2)and a Tafel slope of 78 mV dec^(-1),indicating superior catalytic performance and reaction kinetics.Additionally,the Au NPs showed high resistance to poisoning,as evidenced by a low j_(b)/j_(f)ratio of 0.28 and stable chronoamperometric response.These findings underscore the potential of this synthesis method for producing high-performance electrocatalysts utilized in exploiting ethanol's potential as an environmentally friendly energy carrier.展开更多
Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit co...Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit correction. The algorithm can be acquired by z transform method which is easier for derivation. However, the baseline drift of trapezoidal pulse appears because the noise superimposes on the input signal. In this paper,two new methods based on convergence analysis and noise suppression are proposed to remove the baseline drift resulting from trapezoidal pulse shaping. Simulations and experimental tests are carried out to verify the methods. The results demonstrate that the proposed methods can remove baseline drift in trapezoidal pulse shaping.展开更多
A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-s...A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-stop curve of the pulse motor during the terminal guidance process is designed,along with its start-up logic.The effectiveness of the proposed guidance strategy is verified through simulation.展开更多
Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroac...Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroactivity of polyaniline were investigated. The results show that the electroactivity of polyaniline film strongly depends on the synthetic conditions, such as the ratio of “on time” to “off time”(ton/toff), frequency, monomer concentration, temperature and mean current density. Different electroactivities of polyaniline are caused by different morphologies of polyaniline. The nano-fibrous polyaniline has higher electroactivity than polyaniline with other morphologies. Under the following conditions: mean current density of pulse galvanostatic method 13mA·cm-2, ton/toff 1, frequency 200Hz, monomer concentration 0.3mol·L-1 and temperature 20℃, nano-fibrous polyaniline film with the highest electroactivity can be obtained.展开更多
In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigen...In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigenvalues and eigensolutions respectively.By the symplectic method,the solution of the local buckling of shells can be employed to the expansion series of symplectic eigensolutions in this system.As a result,relationships between critical buckling loads and other factors,such as length of pulse load,thickness of shells and circumferential orders,have been achieved.At the same time,symmetric and unsymmetric buckling modes have been discuss.Moreover,numerical results show that modes of post-buckling of shells can be Bamboo node-type,bending type,concave type and so on.Research in this paper provides analytical supports for ultimate load prediction and buckling failure assessment of cylindrical long shells under local axial pulse loads.展开更多
This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the...This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the three-pulse photon echo's amplitude and efficiency is analyzed with the Maxwell-Bloch equations solved by finite-difference timedomain method.We demonstrate that the amplitude of three-pulse echo will increase with the increasing of thickness and the optimum thickness to generate three-pulse photon echo is 0.3 cm for Tm^(3+):YAG when the attenuation of the input pulse is taken into account.Meanwhile,we find the expression 0.09 exp(α'L),which is previously employed to describe the relationship between echo's efficiency and thickness,should be modified as 1.3 · 0.09 exp(2.4 ·α'L) with the propagation of echo considered.展开更多
Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoerciviti...Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoercivities of the MnBi/Bi film are 1.5 T and 2.35 T at room temperature and at 373K, respectively, showing a positive temperature coefficient. Microstructural investigations show that the textured MnBi film results from the orientated growth induced by the textured Bi under-layer.展开更多
Pulsed tungsten inert gas (TIG) welding is widely used in industry due to its superior properties, so the measurement of arc telnperature is important to analyse welding process. Arc image of spectral line in 794.8 ...Pulsed tungsten inert gas (TIG) welding is widely used in industry due to its superior properties, so the measurement of arc telnperature is important to analyse welding process. Arc image of spectral line in 794.8 nm is captured by high speed camera; both the Abel inversion and the Fowler-Milne method are used to calculate the temperature distribution of the pulsed TIG welding. Characteristic of transient variation in arc intensity and temperature is analyzed. When the change of current happens, intensity and temperature of arc jump as well, it costs several millisoconds. The flirther the axial position from the tungsten is, the greater the intensity jumps, and the smaller the temperature changes.展开更多
We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to...We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to simultaneously measure the weak temporal phase and temporal profile of pulses, which are almost transform- limited. A detailed analysis shows that this iterative method has valuable potential applications in the charac- terization of pulses with weak temporal phase.展开更多
Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for ca...Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for calculating the transmission loss. Firstly, the transmission loss of the single-cavity element was simulated without any airflow, and the effects of different structural parameters on the acoustic performance were investigated comprehensively. Secondly, the static transmission loss of the perforated intake pipe was obtained by the rectangular-pulse method, which is proved to be accurate enough compared with the result by finite element method. Thirdly, under the different conditions of the mean airflow and the operating temperature, the specific transmission loss was acquired respectively. In general, the peaks of the transmission loss are shifted to the lower frequency range because of the reverse airflow, but the amplitudes are irregularly changed. Besides, when the operating temperature increases, the peaks are shifted to the higher frequencies. Finally, with the designed perforated pipe installed to the intake system, the road tests were proceeded to evaluate the actual acoustic performance, and the result indicates that the intake sound pressure level is greatly attenuated. Typically in the range of 600–1500 Hz, the insertion loss of the intake noise at the decelerating moment is almost 20 d B(A), and the overall noise is reduced more than 14.2 d B(A). In conclusion, the perforated intake pipe has been proved excellent in improving the acoustic performance of intake system and could provide the guidance for the automotive engineering application.展开更多
The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and no...The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and notch tensile strength. All these characteristics are considered together in the selection of process parameters by modified taguchi method to analyse the effect of each welding process parameter on tensile properties. Experimental results are furnished to illustrate the approach.展开更多
基金supported by the National Natural Science Foundation of China (Grant No. 12074329)Nanhu Scholars Program for Young Scholars of Xinyang Normal University。
文摘With a three-dimensional semiclassical ensemble method, we theoretically investigated the nonsequential double ionization of Ar driven by the spatially inhomogeneous few-cycle negatively chirped laser pulses. Our results show that the recollision time window can be precisely controlled within an isolated time interval of several hundred attoseconds, which is useful for understanding the subcycle correlated electron dynamics. More interestingly, the correlated electron momentum distribution (CEMD) exhibits a strong dependence on laser intensity. That is, at lower laser intensity, CEMD is located in the first quadrant. As the laser intensity increases,CEMD shifts almost completely to the second and fourth quadrants, and then gradually to the third quadrant.The underlying physics governing the CEMD's dependence on laser intensity is explained.
文摘In this article, a modified version of the Differential Transform Method (DTM) is employed to examine soliton pulse propagation in a weakly non-local parabolic law medium and wave propagation in optical fibers. This semi-analytic method has the advantage of overcoming the obstacle of the hardest nonlinear terms and is used to explain the origin of the bright and dark soliton solutions through the Schrödinger equation in its non-local form and the Radhakrishnan-Kundu-Laksmannan (RKL) equation. Numerical examples demonstrate the effectiveness of this method.
基金The project supported by the National Natural Science Foundation of China(59906005)the Teaching Research Award Program for Outstanding Young Teachers in High Education Institutions of MOE,China
文摘In this paper, the CE/SE method is developed to simulate the two- and three-dimensional flow-field of Pulse Detonation Engine (PDE). The conservation equations with stiff source terms for chemical reaction are solved in two steps. The detailed analysis of computational results of a PDE with a single detonation tube and a PDE with five detonation tubes are given in this paper. Complex wave systems are observed inside and outside a PDE. For a PDE with 5 detonation tubes, there is a big bow shock produced from a number of little shocks near the open ends of tubes. A lot of vortexes interact with shocks and a large expansion wave propagates forward and backward with respect to the PDE in a semi-oval shape.
文摘In this paper, the generalized nonlinear Schrodinger equation (GNLSE) is solved by an adaptive split-step Fourier method (ASSFM). It is found that ASSFM must be used to solve GNLSE to ensure precision when the soliton selffrequency shift is remarkable and the photonic crystal fibre (PCF) parameters vary with the frequency considerably. The precision of numerical simulation by using ASSFM is higher than that by using split-step Fourier method in the process of laser pulse propagation in PCFs due to the fact that the variation of fibre parameters with the peak frequency in the pulse spectrum can be taken into account fully.
文摘The domain size of spiral waves is an important issue in studies of two-dimensional (2D) spatiotemporal patterns. In this work, we use the 2D complex Ginzburg-Landau equation (CGLE) as our model and find that an initially big spiral can successfully transfer to several small spirals by applying a pulse array method. The impacts of several important factors, such as array density, controlling intensity and pulsing time, are investigated. This control approach may be useful for the control of 2D spatiotemporal patterns and has potential applications in the control of some realistic systems, such as meteorological and cardiac systems.
文摘In high-altitude nuclear detonations,the proportion of pulsed X-ray energy can exceed 70%,making it a specific monitoring signal for such events.These pulsed X-rays can be captured using a satellite-borne X-ray detector following atmospheric transmission.To quantitatively analyze the effects of different satellite detection altitudes,burst heights,and transmission angles on the physical processes of X-ray transport and energy fluence,we developed an atmospheric transmission algorithm for pulsed X-rays from high-altitude nuclear detonations based on scattering correction.The proposed method is an improvement over the traditional analytical method that only computes direct-transmission X-rays.The traditional analytical method exhibits a maximum relative error of 67.79% compared with the Monte Carlo method.Our improved method reduces this error to within 10% under the same conditions,even reaching 1% in certain scenarios.Moreover,its computation time is 48,000 times faster than that of the Monte Carlo method.These results have important theoretical significance and engineering application value for designing satellite-borne nuclear detonation pulsed X-ray detectors,inverting nuclear detonation source terms,and assessing ionospheric effects.
基金sponsored by the National Natural Science Foundation of China (No. 41504072)the "135" Program of Institute of Geochemistry, Chinese Academy of Sciences (CAS) and State Key Laboratory of Earthquake Dynamics
文摘Lherzolite is one of the most important components of the subcontinental mantle lithosphere, and the study of its heat transfer properties aids in understanding the thermal structure of the continental mantle lithosphere. Currently, few studies have examined the heat transfer properties of lherzolite, and the experimental results remain controversial. This experiment utilized a pulse method to measure the thermal diffusivity of lherzolite at pressures ranging from 1.0 to 4.0 GPa and temperatures from 300 to 1 073 K on a cubic press apparatus. We obtained a thermal diffusivity for lherzolite of approximately 2.10 mm^2s^(-1) at ambient condition. The experimental pressure derivative of the thermal conductivity of lherzolite decreased with temperature, reaching approximately 10% at high temperature, a value higher than the previously reported 4%, which indicates that the temperature gradient of the upper mantle lithosphere is smaller than previously thought. Therefore, concerning calculation of the lithosphere thickness using the thermal conductivity of the lherzolite, the previous calculation using pressure derivative of the thermal conductivity of 4% may cause an underestimation of the upper mantle lithosphere thickness by approximately 6% in a first approximation.
基金supported by the National Natural Science Foundation of China (No. 51306153)the Natural Science Foundation of Shanxi Province of China (No. 2010JQ7005)+1 种基金Doctoral Fund of Ministry of Education of China (No. 20116102120027)Northwestern Polytechnical University Foundation for Fundamental Research (No. NPU-FFRJCY20130129)
文摘In order to test the feasibility of a new thrust stand system based on impulse thrust mea- surement method, a liquid-fueled pulse detonation engine (PDE) is designed and built. Thrust per- formance of the engine is obtained by direct thrust measurement with a force transducer and indirect thrust measurement with an eddy current displacement sensor (ECDS). These two sets of thrust data are compared with each other to verify the accuracy of the thrust performance. Then thrust data measured by the new thrust stand system are compared with the verified thrust data to test its feasibility. The results indicate that thrust data from the force transducer and ECDS system are consistent with each other within the range of measurement error. Though the thrust data from the impulse thrust measurement system is a litter lower than that from the force transducer due to the axial momentum losses of the detonation jet, the impulse thrust measurement method is valid when applied to measure the averaged thrust of PDE. Analytical models of PDE are also discussed in this paper. The analytical thrust performance is higher than the experimental data due to ignoring the losses during the deflagration to detonation transition process. Effect of equivalence ratio on the engine thrust performance is investigated by utilizing the modified analytical model. Thrust reaches maximum at the equivalence ratio of about 1.1.
基金Project supported by the National Basic Research Program of China(Grant No.2011CB209402)the National Natural Science Foundation of China(Grant No.51177041)the Fundamental Research Funds for the Central Universities,China(Grant No.12QX01)
文摘A novel two-dimensional (2D) simulation method of positive corona current pulses is proposed. A control-volume- based finite element method (CV-FEM) is used to solve continuity equations, and the Galerkin finite element method (FEM) is used to solve Poisson's equation. In the proposed method, photoionization is considered by adopting an exact Helmholtz photoionization model. Furthermore, fully implicit discretization and variable time step are used to ensure the time-efficiency of the present method. Finally, the method is applied to a positive rod-plane corona problem. The numerical results are in agreement with the experimental results, and the validity of the proposed method is verified.
基金supported by the National Research and Innovation Agency(BRIN)and Lembaga Pengelola Dana Pendidikan(LPDP)Ministry of Finance,Republic of Indonesia through Riset dan Inovasi Untuk Indonesia Maju(RIIM)scheme batch 2 with contract number 1/PG.02.00.PT/LPPM/IV/2024(110/IV/KS/11/2022).
文摘The pressing environmental concerns and the depletion of fossil fuel reserves necessitate a transition toward sustainable energy sources.Ethanol,a renewable biomass-derived fuel,is a promising alternative due to its availability and high energy density.This study investigates the synthesis of gold nanoparticles(Au NPs)via a square-wave pulse deposition technique,aiming to enhance catalytic activity for ethanol electrooxidation.By varying pulse durations,we were able to exert precise control over Au NP size and distribution without stabilizing agents.Characterization using field emission scanning electron microscopy and X-ray diffraction techniques confirmed the formation of clustered nanoparticles of metallic gold phase.Electrochemical characteristics analyses revealed that Au NPs synthesized with a 900 ms pulse duration exhibited the lowest charge transfer resistance and the highest electrochemically active surface area.The electrocatalytic performance test of these Au NPs demonstrated an anodic current density of 2.5 mA cm^-(2)and a Tafel slope of 78 mV dec^(-1),indicating superior catalytic performance and reaction kinetics.Additionally,the Au NPs showed high resistance to poisoning,as evidenced by a low j_(b)/j_(f)ratio of 0.28 and stable chronoamperometric response.These findings underscore the potential of this synthesis method for producing high-performance electrocatalysts utilized in exploiting ethanol's potential as an environmentally friendly energy carrier.
基金Supported by National High Technology Research and Development Program of China(863 Program)(No.2012AA061804-03)
文摘Trapezoidal pulse shaping algorithm is widely applied to improve signal-to-noise ratio(SNR), throughput and energy resolution with the properties of noise suppression, pile-up pulse separation and ballistic deficit correction. The algorithm can be acquired by z transform method which is easier for derivation. However, the baseline drift of trapezoidal pulse appears because the noise superimposes on the input signal. In this paper,two new methods based on convergence analysis and noise suppression are proposed to remove the baseline drift resulting from trapezoidal pulse shaping. Simulations and experimental tests are carried out to verify the methods. The results demonstrate that the proposed methods can remove baseline drift in trapezoidal pulse shaping.
基金The National Natural Science Foundation of China(Project No.52102436)The Natural Science Foundation of Shanghai(Project No.23ZR1462700)+3 种基金The National Key Laboratory Open Fund for Strength and Structural Integrity(Project No.ASSIKFJJ202304006)The Shanghai Aerospace Science and Technology Innovation Fund(Project No.SAST2022-031)The National Key Laboratory of Space Intelligent Control(Project No.2023-JCJQ-LB-006-14)The Shanghai Key Laboratory of Spacecraft Mechanism(Project No.YY-F805202210025)。
文摘A new terminal guidance law is proposed based on a solid propellant pulse engine and an improved proportional navigation method to address the terminal guidance issue for kinetic interceptors.On this basis,the start-stop curve of the pulse motor during the terminal guidance process is designed,along with its start-up logic.The effectiveness of the proposed guidance strategy is verified through simulation.
基金Project(50473022) supported by the National Natural Science Foundation project supported by the State Key Laboratoryof Chemo/Biosensing and Chemometrics of China
文摘Nano-fibrous polyaniline was synthesized on stainless steel electrode in 0.5mol·L-1 H2SO4 solution by pulse galvanostatic method. The effects of synthetic conditions of pulse galvanostatic method on the electroactivity of polyaniline were investigated. The results show that the electroactivity of polyaniline film strongly depends on the synthetic conditions, such as the ratio of “on time” to “off time”(ton/toff), frequency, monomer concentration, temperature and mean current density. Different electroactivities of polyaniline are caused by different morphologies of polyaniline. The nano-fibrous polyaniline has higher electroactivity than polyaniline with other morphologies. Under the following conditions: mean current density of pulse galvanostatic method 13mA·cm-2, ton/toff 1, frequency 200Hz, monomer concentration 0.3mol·L-1 and temperature 20℃, nano-fibrous polyaniline film with the highest electroactivity can be obtained.
基金This research is funded by the grants from Dalian Project of Innovation Foundation of Science and Technology(No.2018J11CY005)Research Program of State Key Laboratory of Structural Analysis for Industrial Equipment(No.S18313).
文摘In this paper,the local buckling of cylindrical long shells is discussed under axial pulse loads in a Hamiltonian system.Using this system,critical loads and modes of buckling of shells are reduced to symplectic eigenvalues and eigensolutions respectively.By the symplectic method,the solution of the local buckling of shells can be employed to the expansion series of symplectic eigensolutions in this system.As a result,relationships between critical buckling loads and other factors,such as length of pulse load,thickness of shells and circumferential orders,have been achieved.At the same time,symmetric and unsymmetric buckling modes have been discuss.Moreover,numerical results show that modes of post-buckling of shells can be Bamboo node-type,bending type,concave type and so on.Research in this paper provides analytical supports for ultimate load prediction and buckling failure assessment of cylindrical long shells under local axial pulse loads.
基金Project supported by Tianjin Research Program Application Foundation and Advanced Technology,China(Grant No.15JCQNJC01100)
文摘This paper investigates the phenomenon of three-pulse photon echo in thick rare-earth ions doped crystal whose thickness is far larger than 0.002 cm which is adopted in previous works.The influence of thickness on the three-pulse photon echo's amplitude and efficiency is analyzed with the Maxwell-Bloch equations solved by finite-difference timedomain method.We demonstrate that the amplitude of three-pulse echo will increase with the increasing of thickness and the optimum thickness to generate three-pulse photon echo is 0.3 cm for Tm^(3+):YAG when the attenuation of the input pulse is taken into account.Meanwhile,we find the expression 0.09 exp(α'L),which is previously employed to describe the relationship between echo's efficiency and thickness,should be modified as 1.3 · 0.09 exp(2.4 ·α'L) with the propagation of echo considered.
基金Supported by the National Natural Science Foundation of China under Grant Nos 51171001,51371009 and 50971003the Foundation of Key Laboratory of Neutron Physics of CAEP under Grant No 2014BB02
文摘Textured Bi and MnBi/Bi thin films are prepared by the pulsed laser deposition method. The highly c-axis textured MnBi films are obtained by annealing the bilayer consisting of textured Bi and Mn films. The eoercivities of the MnBi/Bi film are 1.5 T and 2.35 T at room temperature and at 373K, respectively, showing a positive temperature coefficient. Microstructural investigations show that the textured MnBi film results from the orientated growth induced by the textured Bi under-layer.
基金the National Natural Science Foundation of China (No. 51275299)
文摘Pulsed tungsten inert gas (TIG) welding is widely used in industry due to its superior properties, so the measurement of arc telnperature is important to analyse welding process. Arc image of spectral line in 794.8 nm is captured by high speed camera; both the Abel inversion and the Fowler-Milne method are used to calculate the temperature distribution of the pulsed TIG welding. Characteristic of transient variation in arc intensity and temperature is analyzed. When the change of current happens, intensity and temperature of arc jump as well, it costs several millisoconds. The flirther the axial position from the tungsten is, the greater the intensity jumps, and the smaller the temperature changes.
基金Supported by the National Natural Science Foundation of China under Grant No 61205103
文摘We propose a simple iterative algorithm based on a temporally movable phase modulation process to retrieve the weak temporal phase of laser pulses. This unambiguous method can be used to achieve a high accuracy and to simultaneously measure the weak temporal phase and temporal profile of pulses, which are almost transform- limited. A detailed analysis shows that this iterative method has valuable potential applications in the charac- terization of pulses with weak temporal phase.
基金Project(51705454)supported by the National Natural Science Foundation of China
文摘Exact simulation of the acoustic performance is essential to the engineering application for a vehicle intake system. The rectangular-pulse method based on the computational fluid dynamics approach was employed for calculating the transmission loss. Firstly, the transmission loss of the single-cavity element was simulated without any airflow, and the effects of different structural parameters on the acoustic performance were investigated comprehensively. Secondly, the static transmission loss of the perforated intake pipe was obtained by the rectangular-pulse method, which is proved to be accurate enough compared with the result by finite element method. Thirdly, under the different conditions of the mean airflow and the operating temperature, the specific transmission loss was acquired respectively. In general, the peaks of the transmission loss are shifted to the lower frequency range because of the reverse airflow, but the amplitudes are irregularly changed. Besides, when the operating temperature increases, the peaks are shifted to the higher frequencies. Finally, with the designed perforated pipe installed to the intake system, the road tests were proceeded to evaluate the actual acoustic performance, and the result indicates that the intake sound pressure level is greatly attenuated. Typically in the range of 600–1500 Hz, the insertion loss of the intake noise at the decelerating moment is almost 20 d B(A), and the overall noise is reduced more than 14.2 d B(A). In conclusion, the perforated intake pipe has been proved excellent in improving the acoustic performance of intake system and could provide the guidance for the automotive engineering application.
文摘The selection of process parameters for obtaining optimal tensile properties in the pulsed current gas tungsten arc welding is presented. The tensile properties include ultimate tensile strength, yield strength and notch tensile strength. All these characteristics are considered together in the selection of process parameters by modified taguchi method to analyse the effect of each welding process parameter on tensile properties. Experimental results are furnished to illustrate the approach.