Laser-induced aerosols,predominantly submicron in size,pose significant environmental and health risks during the decommissioning of nuclear reactors.This study experimentally investigated the removal of laser-generat...Laser-induced aerosols,predominantly submicron in size,pose significant environmental and health risks during the decommissioning of nuclear reactors.This study experimentally investigated the removal of laser-generated aerosol particles using a water spray system integrated with an innovative system for pre-injecting electrically charged mist in our facility.To simulate aerosol generation in reactor decommissioning,a high-power laser was used to irradiate various materials(including stainless steel,carbon steel,and concrete),generating aerosol particles that were agglomerated with injected water mist and subsequently scavenged by water spray.Experimental results demonstrate enhanced aerosol removal via aerosol-mist agglomeration,with charged mist significantly improving particle capture by increasing wettability and size.The average improvements for the stainless steel,carbon steel,and concrete were 40%,44%,and 21%,respectively.The results of experiments using charged mist with different polarities(both positive and negative)and different surface coatings reveal that the dominant polarity of aerosols varies with the irradiated materials,influenced by their crystal structure and electron emission properties.Notably,surface coatings such as ZrO_(2)and CeO_(2)were found to possibly alter aerosol charging characteristics,thereby affecting aerosol removal efficiency with charged mist configurations.The innovative aerosol-mist agglomeration approach shows promise in mitigating radiation exposure,ensuring environmental safety,and reducing contaminated water during reactor dismantling.This study contributes critical knowledge for the development of advanced aerosol management strategies for nuclear reactor decommissioning.The understanding obtained in this work is also expected to be useful for various environmental and chemical engineering applications such as gas decontamination,air purification,and pollution control.展开更多
The radiological characterization is to determine the type, the distribution and the radioactivity of the radionuclide in the reactor by investigation of the information, instrumentation detection, sampling analyses a...The radiological characterization is to determine the type, the distribution and the radioactivity of the radionuclide in the reactor by investigation of the information, instrumentation detection, sampling analyses and theoretical calculation. It is used for determination of the decommissioning implementation option and radiological protection measure of the workers. After completion of the decommissioning it is used for determination of the site release. The radiological characterization should go through whole decommissioning process, which includes： the collection and review of historical file, the performing calculation of radionuclide inventory in the reactor, in situ measurement, sampling analyses, the review and evaluation of the data obtained and the comparison of calculated result with measured date etc.. The special attention should be paid to the radiological characterization information from the key part of reactor in decommissioning end state. The sampling from the ＂hot spot＂ should not be lost; the number of the sampling should be reasonable based on reliable statistics. The radioactivity density for site release should comply with the guide, standard and regulation of International Atomic Energy Agency and China.展开更多
In Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, the fuel debris formed in the Reactor Pressure Vessel (RPV) and Primary Containment Vessel (PCV) at Unit 1</span><span style="font-family:Verdan...In Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, the fuel debris formed in the Reactor Pressure Vessel (RPV) and Primary Containment Vessel (PCV) at Unit 1</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">-</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">3. To accelerate and decide further decommissioning steps of the FDNPP, it is crucial to obtain realistic information of the debris and localize contaminated water leakage from PCV. Due to high radiation and dark environment inside the PCV, investigating instruments and techniques should necessarily to meet specification of radiation resistance, waterproofness, dust resistance and so on. This study focuses on development of ultrasonic measurement system using a couple of sectorial array sensors to localize contaminated water leakage and visualize shape of object that repre</span><span style="font-family:Verdana;">- </span><span style="font-family:Verdana;">senting fuel debris, simultaneously. In this study, Total Focusing Method</span><span style="font-family:Verdana;"> (TFM) and Ultrasonic Velocity Profiler (UVP) methods are considered to visualize object shape and flow pattern around it, respectively. To demonstrate applicability and reliability of developed measurement system with sectorial array sensors, a mock-up experiment result</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">of simulated water leakage and fuel debris shape were discussed in this paper.展开更多
基金financial support from the Nuclear Energy Science&Technology and Human Resource Development Project of the Japan Atomic Energy Agency/Collaborative Laboratories for Advanced Decommissioning Science(No.R04I034)The author Ruicong Xu appreciates the scholarship(financial support)from the China Scholarship Council(CSC,No.202106380073).
文摘Laser-induced aerosols,predominantly submicron in size,pose significant environmental and health risks during the decommissioning of nuclear reactors.This study experimentally investigated the removal of laser-generated aerosol particles using a water spray system integrated with an innovative system for pre-injecting electrically charged mist in our facility.To simulate aerosol generation in reactor decommissioning,a high-power laser was used to irradiate various materials(including stainless steel,carbon steel,and concrete),generating aerosol particles that were agglomerated with injected water mist and subsequently scavenged by water spray.Experimental results demonstrate enhanced aerosol removal via aerosol-mist agglomeration,with charged mist significantly improving particle capture by increasing wettability and size.The average improvements for the stainless steel,carbon steel,and concrete were 40%,44%,and 21%,respectively.The results of experiments using charged mist with different polarities(both positive and negative)and different surface coatings reveal that the dominant polarity of aerosols varies with the irradiated materials,influenced by their crystal structure and electron emission properties.Notably,surface coatings such as ZrO_(2)and CeO_(2)were found to possibly alter aerosol charging characteristics,thereby affecting aerosol removal efficiency with charged mist configurations.The innovative aerosol-mist agglomeration approach shows promise in mitigating radiation exposure,ensuring environmental safety,and reducing contaminated water during reactor dismantling.This study contributes critical knowledge for the development of advanced aerosol management strategies for nuclear reactor decommissioning.The understanding obtained in this work is also expected to be useful for various environmental and chemical engineering applications such as gas decontamination,air purification,and pollution control.
文摘The radiological characterization is to determine the type, the distribution and the radioactivity of the radionuclide in the reactor by investigation of the information, instrumentation detection, sampling analyses and theoretical calculation. It is used for determination of the decommissioning implementation option and radiological protection measure of the workers. After completion of the decommissioning it is used for determination of the site release. The radiological characterization should go through whole decommissioning process, which includes： the collection and review of historical file, the performing calculation of radionuclide inventory in the reactor, in situ measurement, sampling analyses, the review and evaluation of the data obtained and the comparison of calculated result with measured date etc.. The special attention should be paid to the radiological characterization information from the key part of reactor in decommissioning end state. The sampling from the ＂hot spot＂ should not be lost; the number of the sampling should be reasonable based on reliable statistics. The radioactivity density for site release should comply with the guide, standard and regulation of International Atomic Energy Agency and China.
文摘In Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, the fuel debris formed in the Reactor Pressure Vessel (RPV) and Primary Containment Vessel (PCV) at Unit 1</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">-</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">3. To accelerate and decide further decommissioning steps of the FDNPP, it is crucial to obtain realistic information of the debris and localize contaminated water leakage from PCV. Due to high radiation and dark environment inside the PCV, investigating instruments and techniques should necessarily to meet specification of radiation resistance, waterproofness, dust resistance and so on. This study focuses on development of ultrasonic measurement system using a couple of sectorial array sensors to localize contaminated water leakage and visualize shape of object that repre</span><span style="font-family:Verdana;">- </span><span style="font-family:Verdana;">senting fuel debris, simultaneously. In this study, Total Focusing Method</span><span style="font-family:Verdana;"> (TFM) and Ultrasonic Velocity Profiler (UVP) methods are considered to visualize object shape and flow pattern around it, respectively. To demonstrate applicability and reliability of developed measurement system with sectorial array sensors, a mock-up experiment result</span><span style="font-family:Verdana;"> </span><span style="font-family:Verdana;">of simulated water leakage and fuel debris shape were discussed in this paper.
