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What decarbonized the residential building operation worldwide since the 2000s
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作者 Min-Da Ma Min-Xia Chen +1 位作者 Wei Feng Jing-Wen Huo 《Petroleum Science》 SCIE CAS CSCD 2022年第6期3194-3208,共15页
Decarbonization in operational residential buildings worldwide has become critical in achieving the carbon neutral target due to the growing household energy demand.To accelerate the pace of global carbon neutrality,t... Decarbonization in operational residential buildings worldwide has become critical in achieving the carbon neutral target due to the growing household energy demand.To accelerate the pace of global carbon neutrality,this study explores the operational carbon change in global residential buildings through the generalized Divisia index method and decoupling analysis,considering the decarbonization levels of residential buildings at different scales.The results show that(1)most of the samples showed a decrease in the total emissions from 2000 to 2019.Except for China and the United States(US),the carbon emissions in global residential building operations decreased by 7.95 million tons of carbon dioxide(MtCO_(2))per year over the study period.Emissions per gross domestic product(GDP)was the most positive driver causing the decarbonization of residential buildings,while GDP was the most negative driver.(2)Carbon intensity was essential to achieving a strong decoupling of economic development and carbon emissions.The US almost consistently presented strong decoupling,while China showed weak decoupling over the last two decades.(3)The pace of decarbonization in global residential building operations is gradually slowing down.From 2000 to 2019,decarbonization from residential buildings across 30 countries was 2094.3 MtCO_(2),with a decarbonization efficiency of 3.4%.Overall,this study addresses gaps in evaluating global decarbonization from operational residential buildings and provides a reference for evaluating building decarbonization by other emitters. 展开更多
关键词 Global residential building Operational decarbonization Generalized divisia index method Decoupling elasticity Building decarbonization strategies
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Toward a sustainable and decarbonized grid:Zimbabwe’s readiness in adopting nuclear and green hydrogen energies
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作者 Anesu Nicholas Charamba 《Clean Energy》 2025年第4期80-97,共18页
A shift toward a sustainable and decarbonized power grid is one of Zimbabwe’s main goals in the energy sector.This study comprehensively analyzes the country’s readiness to implement green hydrogen and nuclear energ... A shift toward a sustainable and decarbonized power grid is one of Zimbabwe’s main goals in the energy sector.This study comprehensively analyzes the country’s readiness to implement green hydrogen and nuclear energy generation.Despite the extensive energy studies available in literature,the question of whether the country is ready to adopt these two technologies remains unanswered.The literature lacks information on how well the country is prepared for green hydrogen production for its industrial applications.Therefore,this paper begins with a synopsis of current electricity generation and consumption trends,followed by overviews of nuclear energy and green hydrogen generation,respectively.The country’s readiness to adopt the technologies under study is then examined by considering the available infrastructure,economic status of the country,supporting policies,regulatory frameworks already in place,social acceptance,and the potential positive and negative impacts.An analysis of strengths,weaknesses,opportunities,and threats analysis is implemented,emphasizing the critical factors that must be considered.Recommendations are outlined to enable a strategic and seamless adoption of green hydrogen and nuclear energy,specifically small modular reactors.The main findings indicate that Zimbabwe currently relies on thermal and hydroelectric energies,with an increasing demand for electricity,particularly in the mining sector.In addition,adopting green hydrogen and nuclear energy primarily results in improved grid resilience,reduced electricity supply-demand gap,economic growth through increased investments,and mitigation of poverty.However,insufficient policies and regulatory frameworks,as well as increased safety concerns,can hinder the implementation of these projects.However,these limitations can be effectively minimized by technological advances or international and regional collaborations.Hence,comprehensive economic reforms,supporting policies,and regulations are required,along with capacity-building investments.The study provides policymakers,investors,and stakeholders with insights into the substantial benefits of considering these energy sources for a decarbonized and sustainable energy future. 展开更多
关键词 renewable energy decarbonized grid nuclear energy green hydrogen sustainable development small modular reactors
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Mapping regional disparities in the global shift toward decarbonized power systems
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作者 Binbin Ju Zhujun Chen +4 位作者 Yong Geng Peixue Xing Linbo Han Lili Wang Wendong Wei 《Carbon Neutrality》 2025年第1期284-297,共14页
Global efforts to transform power systems are accelerating,yet the localized patterns and trajectories of this transition-crucial for equitable and regionally tailored policy-making-remain insufficiently explored.This... Global efforts to transform power systems are accelerating,yet the localized patterns and trajectories of this transition-crucial for equitable and regionally tailored policy-making-remain insufficiently explored.This study introduces a comprehensive subnational dataset of global power plants,encompassing nine energy types and spanning the years 2015 to 2020.Through spatial statistics,clustering,and cross-regional comparisons,we identify distinct trajectories of power capacity change across energy types and regions.While decarbonization remains a clear global trend,structurally disadvantaged or over-averaged regions are still at risk of being overlooked.To better understand these transition dynamics,we conducted a machine learning-based driver analysis,which highlights the dominant influence of development-related factors such as electricity demand and economic growth.The openly accessible dataset fills a critical gap in global energy data and offers a standardized,robust framework for analyzing regional power infrastructure development.Its design enables fine-grained,dynamic assessments of transition pathways and facilitates interdisciplinary research across energy,climate,and policy domains. 展开更多
关键词 Energy transition Power plant Renewable energy Decarbonization Subnational dataset
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GREENING THE ENGINE ROOM China's new initiative to decarbonize its industrial parks
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作者 Li Nan 《Beijing Review》 2026年第4期16-17,共2页
On December 26,2025 China announced plans to begin the zero-carbon transformation of 52 industrial parks across the country.This first batch of parks span sectors such as new energy,advanced manufactur-ing and computi... On December 26,2025 China announced plans to begin the zero-carbon transformation of 52 industrial parks across the country.This first batch of parks span sectors such as new energy,advanced manufactur-ing and computing.The list ensures every province,autonomous region,and municipality has at least one designated park,with transforma-tion set for completion by 2030. 展开更多
关键词 industrial parks zero carbon transformation China new energyadvanced decarbonization
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Shipping decarbonization governance in Arctic waters:theoretic logic and implementation pathways 被引量:1
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作者 LI Wenwen HU Zhengliang 《Advances in Polar Science》 2025年第2期152-166,共15页
The accelerated decline of Arctic sea ice since the 1980s has paradoxically amplified greenhouse gas(GHG)emissions through increased shipping activities in this ecologically vulnerable region.This study investigates h... The accelerated decline of Arctic sea ice since the 1980s has paradoxically amplified greenhouse gas(GHG)emissions through increased shipping activities in this ecologically vulnerable region.This study investigates how to reconcile the decarbonization of Arctic shipping with conflicting environmental,economic,and geopolitical interests.Through systematic literature review and interest-balancing analysis,our findings identify three systemic barriers:(1)inadequate adaptation of International Maritime Organization(IMO)regulations to Arctic-specific environmental risks,(2)fragmented enforcement mechanisms among Arctic and non-Arctic States,and(3)technological limitations in clean fuel adoption for ice-class vessels.To address these challenges,a tripartite governance framework is proposed.First,legally binding amendments to International Convention for the Prevention of Pollution from Ships(MARPOL)Annex VI introducing Arctic-specific Energy Efficiency eXisting ship Index(EEXI)standards and extending energy efficiency regulations to fishing vessels.Second,a phased fuel transition prioritizing liquefied natural gas(LNG)and methanol,followed by hydrogen-ammonia synthetics.Third,enhanced multilateral cooperation through an Arctic Climate Shipping Alliance to coordinate joint research and development in cold-adapted technologies and ice-route optimization.By integrating United Nations Convention on the Law of the Sea(UNCLOS)obligations with IMO Polar Code implementation,this study advances a dynamic interest-balancing framework for policymakers,offering actionable pathways to achieve Paris Agreement targets while safeguarding Arctic ecosystems. 展开更多
关键词 SHIPPING decarbonization Arctic waters GHG emission IMO
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Erratum to:Life cycle assessment of hydrogen production pathways to support hydrogen decarbonization policies in a Canadian context
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作者 Giovanna Gonzales-Calienes Miyuru Kannangara +6 位作者 Jianjun Yang Jalil Shadbahr FaridBensebaa Anton Alvarez-Majmutov Jinwen Chen Nima Ghavidel Mehr Marzouk Benali 《Frontiers in Energy》 2025年第6期1143-1143,共1页
The article“Life cycle assessment of hydrogen production pathways to support hydrogen decarbonization policies in a Canadian context”written by Giovanna Gonzales-Calienes,Miyuru Kannangara,Jianjun Yang,Jalil Shadbah... The article“Life cycle assessment of hydrogen production pathways to support hydrogen decarbonization policies in a Canadian context”written by Giovanna Gonzales-Calienes,Miyuru Kannangara,Jianjun Yang,Jalil Shadbahr,Farid Bensebaa,Anton Alvarez-Majmutov,Jinwen Chen,Nima Ghavidel Mehr and Marzouk Benali,was originally published electronically without Open Access due to an unfortunate error.The article should be published Open Access under the terms of CC BY license.Therefore,the copyright of the article has been changed to©The Author(s)2025. 展开更多
关键词 open access cycle assessment hydrogen production canadian context life cycle assessment hydrogen decarbonization policies decarbonization policies
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Recent progress and prospects of ammonia combustion for gas turbines
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作者 Yitong ZHAO Ye TIAN 《Chinese Journal of Aeronautics》 2025年第10期286-287,共2页
1.Introduction and background Global warming demands low-carbon energy.Ammonia(NH_(3)),a carbon-free hydrogen carrier,offers CO_(2)reduction potential,aligning with decarbonization,per the work of Zhang et al.2.NH_(3)... 1.Introduction and background Global warming demands low-carbon energy.Ammonia(NH_(3)),a carbon-free hydrogen carrier,offers CO_(2)reduction potential,aligning with decarbonization,per the work of Zhang et al.2.NH_(3)as a fuel Advantages:NH_(3)offers high hydrogen content ease of storage,cost-effectiveness in large-scale transport,and technological maturity in synthesis. 展开更多
关键词 global warming hydrogen carrier gas turbines CO reduction AMMONIA decarbonization COMBUSTION low carbon energy
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Environmental impact of patient travel for cataract surgery
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作者 Matthias Fritz Uhrmann Holger Repp Christian Gissel 《International Journal of Ophthalmology(English edition)》 2025年第11期2155-2159,共5页
AIM:To analyze the environmental impact of patient travel for cataract surgery at a German ophthalmology center.METHODS:All cataract surgeries performed between October 23 and October 27,2023,were analyzed,and all pat... AIM:To analyze the environmental impact of patient travel for cataract surgery at a German ophthalmology center.METHODS:All cataract surgeries performed between October 23 and October 27,2023,were analyzed,and all patient records were reviewed for follow-up visits.All travel distances were calculated,and the associated emissions were quantified.Additionally,patients’utilization of geographically closer branch practices for follow-up care was evaluated,along with the corresponding effects on travel-related emissions.RESULTS:A total of 69 patients underwent unilateral cataract surgery.The average one-way travel distance was 40.1 km(24.9 mi;SD=23.6 km).Corresponding emissions were 1284.8 kg of greenhouse gas(GHG),2.477 kg of nitrogen oxides,and 0.101 kg of particulates.All patients attended at least two follow-up visits.Conducting followup visits at branch practices reduced travel distance by 49.1%.The associated GHG emissions from all travel were 1984.3 kg.Emissions from follow-up visits were 54.4%higher than those from the surgery itself.Total GHG emissions amounted to 3269.1 kg,with an average of 47.4 kg of GHG per patient for all travel associated with cataract surgery.CONCLUSION:A dense network of branch practices contributes to reducing the carbon footprint of cataract surgery-related patient travel;however,the development of digital health approaches for follow-up care is necessary to further optimize the environmental sustainability of cataract surgery. 展开更多
关键词 CATARACT decarbonization digital health health policy sustainable healthcare
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Simultaneous Denitrification and Decarbonization of Wastewater over In Situ Generation of·ClO Radicals Through a Fast,High-Performance Electro-Filtration Process
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作者 Bin Zhao Jialin Yang +2 位作者 Ruiping Liu Jiuhui Qu Meng Sun 《Engineering》 2025年第12期217-228,共12页
The contamination of wastewater with organic pollutants and nitrogen compounds poses significant environmental challenges.The primary objective of wastewater treatment is the simultaneous denitrification and decarboni... The contamination of wastewater with organic pollutants and nitrogen compounds poses significant environmental challenges.The primary objective of wastewater treatment is the simultaneous denitrification and decarbonization of ammonia nitrogen and organics into harmless by-products.This study presents a novel method for the directional generation of chlorine radical species like·ClO and·Cl using electro-reactive membranes(EMs)known as RuO_(2)@PbO_(2)-M,which were fabricated using an electro-deposition coupled template approach.This method facilitates the rapid and efficient conversion of ammonia to nitrogen and concurrently reduces the chemical oxygen demand in the effluent.Our system achieved ultra-efficient simultaneous denitrification and decarbonization with minimal energy consumption in single-filtration mode,thereby eliminating the need for chemical precursors.We elucidate the formation pathway of·ClO and·Cl during the electrochemical oxidation process involving RuO_(2)@PbO_(2)-M,where·Cl generated from RuO_(2)reacts with·OH from PbO_(2)under hypochlorous acid conditions,thereby enhancing nitrogen and carbon removal.These findings highlight a novel electro-filtration and an innovative reactive membrane design for·ClO synthesis,which provides a new research framework for the concurrent removal of nitrogen and carbon,and offers a promising solution to enhance wastewater treatment efficiency. 展开更多
关键词 Wastewater treatment DENITRIFICATION Decarbonization Chlorine oxide radical Electro-reactive membranes
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Enhancing energy security through efficient decarbonization:Impact of China’s“Constructing Large Units and Restricting Small Ones”policy on thermal power productivity
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作者 Jinsong Zhao Chin-Hsien Yu Xinghao Li 《Chinese Journal of Population,Resources and Environment》 2025年第2期168-180,共13页
Developing low-carbon and efficient power systems is critical for energy security in the global warming context.We address this issue by focusing on the productivity impact of a decarbonization policy in China’s ther... Developing low-carbon and efficient power systems is critical for energy security in the global warming context.We address this issue by focusing on the productivity impact of a decarbonization policy in China’s thermal power sector—namely,the“Constructing Large Units and Restricting Small Ones”(CLRS)initiative.Utilizing a resource misallocation model,we construct a new theoretical framework to distinguish between technical and allocative efficiency and analyze productivity using plant-level data.The results indicate that the CLRS policy has significantly improved the allocative and technical efficiency of China’s coal-fired power sector,thereby ensuring power security.The closure of outdated and highly distorted small coal-fired units,which have been replaced by technologically advanced large units,primarily drives the enhanced efficiency.The policy’s effects are most pronounced in large-scale power plants and those with high coal combustion efficiency.Furthermore,a comparison of power plants’productivity distribution before and after policy implementation reveals that the CLRS policy not only enhances capital productivity in the coal-fired power sector but also increases rational labor allocation.Our findings have important policy implications for developing countries vis-à-vis building efficient and stable power systems amid climate change. 展开更多
关键词 Decarbonization policy Energy security Thermal power Technical efficiency Resource allocative efficiency
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Decarbonizing Marine Logistics:Multi-Echelon Green Supply Chain Models for Offshore Vessel Networks
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作者 Suleiman Ibrahim Mohammad Badrea Al Qraini +3 位作者 Sultan Alaswad Alenazi Asokan Vasudevan Anber Abraheem Shelash Imad Ali 《Sustainable Marine Structures》 2025年第3期227-247,共21页
This study addresses the critical need for decarbonization in offshore marine logistics by developing an integrated modeling framework to support low-emission operations across complex,multi-echelon vessel networks.It... This study addresses the critical need for decarbonization in offshore marine logistics by developing an integrated modeling framework to support low-emission operations across complex,multi-echelon vessel networks.It focuses on port-to-platform supply chains serving offshore wind farms,oil rigs,and floating logistics hubs.A hybrid analytical approach was adopted,combining Mixed-Integer Linear Programming(MILP)for optimizing emission-minimizing routing,Discrete-Event Simulation(DES)to evaluate offshore scheduling performance under variability,and a Multi-Criteria Decision Analysis(MCDA)model using AHP-TOPSIS to rank alternative marine fuel types.Monte Carlo simulation was also employed to assess cost and delivery fluctuations across uncertain operational scenarios.Data inputs were compiled from real-world offshore fleet specifications,port emissions records,and marine fuel technology benchmarks.MILP-based network flow optimization reduced CO₂emissions by 22%while maintaining service reliability across all demand points.DES simulations revealed congestion-driven scheduling delays during peak vessel utilization.MCDA analysis ranked bio-LNG and hydrogen propulsion systems as optimal choices based on emission,cost,and availability trade-offs.Hypothesis testing confirmed significant relationships between fuel type,network structure,and emission performance.The study demonstrates how multi-echelon logistics planning,integrated with emissions-based modeling,can facilitate environmentally responsible marine supply chain design.The framework offers practical guidance for offshore fleet managers,port authorities,and policy regulators aiming to align operational efficiency with decarbonization objectives under IMO and EU directives. 展开更多
关键词 Decarbonization Offshore Logistics Multi-Echelon Supply Chain Emission Optimization Marine Fuel Alternatives
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Japan’s Critical Mineral Strategy and Its Implications for China
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作者 Shu Biquan 《China International Studies》 2025年第2期162-188,共27页
With the global economy undergoing decarbonization and a new wave of technological revolution and industrial transformation,supply chain security risks have become increasingly prominent.Major countries are shifting t... With the global economy undergoing decarbonization and a new wave of technological revolution and industrial transformation,supply chain security risks have become increasingly prominent.Major countries are shifting their focus toward critical minerals,beyond traditional common minerals such as iron and copper.The trend is especially notable regarding minerals considered essential for strategically important emerging industries. 展开更多
关键词 global economy technological revolution critical minerals industrial transformationsupply chain security China decarbonization JAPAN industrial transformation
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SCIENCE AND TECHNOLOGY
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《China Today》 2025年第8期63-63,共1页
World’s First Ammonia-Fueled Vessel Sets Sail The world's first pure ammonia-powered demonstration vessel,the Anhui,successfully completed its maiden voyage in Hefei,east China's Anhui Province,on June 28,mar... World’s First Ammonia-Fueled Vessel Sets Sail The world's first pure ammonia-powered demonstration vessel,the Anhui,successfully completed its maiden voyage in Hefei,east China's Anhui Province,on June 28,marking a major step forward for green shipping.Ammonia,a major chemical industry feedstock,has a high energy density and due to its carbon-free nature,produces only water and nitrogen when fully combusted.This makes it a highly promising fuel for decarbonizing shipping. 展开更多
关键词 chemical industry feedstockhas green shipping decarbonizing shipping FUEL green shippingammoniaa AMMONIA chemical industry VESSEL
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Carbon Input and Output at Subduction Zones:Review and Prospect
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作者 CHEN Wei ZHANG Guoliang 《Journal of Ocean University of China》 2025年第3期657-671,共15页
Subduction zones,linking the surface and deep carbon reservoirs,significantly affect the Earth’s long-term climate change and habitability.The subducting slabs undergo decarbonation with increasing pressure and tempe... Subduction zones,linking the surface and deep carbon reservoirs,significantly affect the Earth’s long-term climate change and habitability.The subducting slabs undergo decarbonation with increasing pressure and temperature,during which partial carbon mobilizes out of the slab and returns to the surface by arc volcanism or degassing,while the residual carbon continues to descend to greater depths in the mantle.The estimated carbon influx at subduction zones depends strongly on the calculation model,with contributions from sediments ranging from 15 to 60 Mt C/yr,altered ocean basalts from 18 to 61 Mt C/yr,and serpentinized perdotites from 1.3 to 36 Mt C/yr.The carbon influx varies in space and time.Carbon removal from subducting slab occurs through metamorphic reactions,carbonate dissolution,diapirism,hydrocarbon formation and melting.Among these decarbonation mechanisms,diapirism and slab meting play a decisive role in dictating the depth at which surface carbonates can subduct.Specifically,diapirism may restrict sedimentary carbonates at shallow depths(<200 km),while slab melting exhausts all carbonates from the altered ocean crust near transition zones(410–660 km).Consequently,a mechanism enabling surface carbonates to reach the lower mantle,i.e.,ultra-deep carbon cycle,is required to be in accordance with observations by natural samples. 展开更多
关键词 deep carbon cycle subduction zones carbon flux slab decarbonation
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Oil Companies Face both Opportunities and Challenges in CCUS Industry Development
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作者 Hou Mingyang Wang Rui 《China Oil & Gas》 2025年第5期33-38,共6页
As decarbonization pressure on traditional fossil fuel-related industries gradually intensifies,CCUS has been increasingly incorporated into energy transition strategies by various oil companies.From a development opp... As decarbonization pressure on traditional fossil fuel-related industries gradually intensifies,CCUS has been increasingly incorporated into energy transition strategies by various oil companies.From a development opportunity perspective,oil companies possess four key advantages in developing the CCUS industry:exploration and development technology advantages;geological resource advantages;capital advantages;source-sink matching advantages.In terms of challenges,oil companies face numerous issues in developing the CCUS industry,including technological development,economic viability,and policy and legal aspects.At the national level,China’s oil companies should advocate for improving and optimizing relevant laws and regulations,enhancing the policy support system,incorporating CCUS into the carbon trading market,and strengthening top-level design and medium-to long-term planning;at the enterprise level,they should continuously advance full industrial chain technologies and reduce CCUS project operating costs,selectively participate in industrial segments that suit their capabilities,strengthen CCUS full industrial chain operational capabilities,and enhance talent development and strengthen international exchange and cooperation. 展开更多
关键词 geological resources source sink matching development technology CCUS industry decarbonization capital advantages oil companies exploration development technology
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Strategic Global Deployment of Photovoltaic Technology:Balancing Economic Capacity and Decarbonization Potential
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作者 Ian Marius PETERS 《Advances in Atmospheric Sciences》 2025年第2期261-268,共8页
This study investigates the disparities in the deployment of photovoltaic(PV)technology for carbon emissions reduction across different nations,highlighting the mismatch between countries with high economic capacity a... This study investigates the disparities in the deployment of photovoltaic(PV)technology for carbon emissions reduction across different nations,highlighting the mismatch between countries with high economic capacity and those where PV installation would maximize global decarbonization benefits.This mismatch is discussed based on three key factors influencing decarbonization via PV technology:per capita gross domestic product;carbon intensity of the energy system;and solar resource availability.Current PV deployment is predominantly concentrated in economically advanced countries,and does not coincide with regions where the environmental and economic impact of such installations would be most significant.Through a series of thought experiments,it is demonstrated how alternative prioritization strategies could significantly reduce global carbon emissions.Argument is put forward for a globally coordinated approach to PV deployment,particularly targeting high-impact sunbelt regions,to enhance the efficacy of decarbonization efforts and promote equitable energy access.The study underscores the need for international policies that support sustainable energy transitions in economically less developed regions through workforce development and assistance with the activation of capital. 展开更多
关键词 photovoltaic deployment decarbonization strategies solar resource availability global energy equity carbon emission reductions
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A preliminary evaluation of carbon dioxide sequestration in coal seams at the Mae Moh mine,northern Thailand:A review
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作者 Piyaphong Chenrai 《Energy Geoscience》 2025年第4期1-11,共11页
The Mae Moh lignite-fired power plant is the only lignite-fired power plant and is the main point source of CO_(2)emissions in Thailand.This power plant uses lignite supplied from the Mae Moh lignite open-pit mine in ... The Mae Moh lignite-fired power plant is the only lignite-fired power plant and is the main point source of CO_(2)emissions in Thailand.This power plant uses lignite supplied from the Mae Moh lignite open-pit mine in the same vicinity.Carbon dioxide sequestration technologies can play a crucial role in reducing carbon emissions in the energy sector,particularly in coal-fired power plants.This case study provides the first assessment of the potential for geological CO_(2)storage in coal seams at the Mae Moh coal mine in northern Thailand based on literature reviews.The Mae Moh Basin is a rift basin with a complex normal fault and contains coal seams at different depths separated by claystones.The geological setting potentially offers favorable conditions for the geological storage of CO_(2)in the coal seams through a combination of physical and chemical trapping mechanisms.The findings suggest that the Mae Moh coal mine is suitable for geological CO_(2)storage,especially in K and Q coal seams.However,leakage risks,storage capacity,and CO_(2)-water-coal reactions could be problematic.Thus,more subsurface studies should be carried out,and more detailed criteria should be considered before CO_(2)sequestration is undertaken in the Mae Moh coal mine. 展开更多
关键词 Carbon storage Coal seam Coal-fired power plant Geological CO_(2)storage Decarbonization
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Theoretical High-Throughput Screening of Single-Atom CO_(2)Electroreduction Catalysts to Methanol Using Active Learning
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作者 Honghao Chen Jun Yin +1 位作者 Jiali Li Xiaonan Wang 《Engineering》 2025年第9期172-182,共11页
Industrial decarbonization is critical for achieving net-zero goals.The carbon dioxide electrochemical reduction reaction(CO_(2)RR)is a promising approach for converting CO_(2)into high-value chemicals,offering the po... Industrial decarbonization is critical for achieving net-zero goals.The carbon dioxide electrochemical reduction reaction(CO_(2)RR)is a promising approach for converting CO_(2)into high-value chemicals,offering the potential for decarbonizing industrial processes toward a sustainable,carbon-neutral future.However,developing CO_(2)RR catalysts with high selectivity and activity remains a challenge due to the complexity of finding such catalysts and the inefficiency of traditional computational or experimental approaches.Here,we present a methodology integrating density functional theory(DFT)calculations,deep learning models,and an active learning strategy to rapidly screen high-performance catalysts.The proposed methodology is then demonstrated on graphene-based single-atom catalysts for selective CO_(2)electroreduction to methanol.First,we conduct systematic binding energy calculations for 3045 single-atom catalysts to identify thermodynamically stable catalysts as the design space.We then use a graph neural network,fine-tuned with a specialized adsorption energy database,to predict the relative activity and selectivity of the candidate catalysts.An autonomous active learning framework is used to facilitate the exploration of designs.After six learning cycles and 2180 adsorption calculations across 15 intermediates,we develop a surrogate model that identifies four novel catalysts on the Pareto front of activity and selectivity.Our work demonstrates the effectiveness of leveraging a domain foundation model with an active learning framework and holds potential to significantly accelerate the discovery of high-performance CO_(2)RR catalysts. 展开更多
关键词 CO_(2)electrochemical reduction Machine learning Active learning Catalyst Decarbonization
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Electro-reforming for green hydrogen:Technological frontiers and systemic challenges
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作者 Zhiwen Lu Zhenhai Wen 《Journal of Energy Chemistry》 2025年第10期528-530,共3页
In the grand tapestry of the global energy transition,the quest for scalable hydrogen economies emerges as a pivotal thread,weaving together the dual imperatives of decarbonization and industrial pragmatism.Yet,in its... In the grand tapestry of the global energy transition,the quest for scalable hydrogen economies emerges as a pivotal thread,weaving together the dual imperatives of decarbonization and industrial pragmatism.Yet,in its present form,hydrogen production remains deeply entwined with carbon emissions. 展开更多
关键词 technological frontiers global energy transitionthe green hydrogen global energy transition carbon emissions electro reforming systemic challenges decarbonization
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A STUDY OF THE PROPERTIES OF S25C-SUS405 STEEL JOINTS BY VAOUUM DIFFUSION WELDING
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作者 杜则裕 菊地靖志 +1 位作者 池内建二 堀之内力 《Transactions of Tianjin University》 EI CAS 1995年第2期114+111-114,共5页
In this paper, the properties of S25C-SUS405 steel joints by vacuum diffusion welding are discussed, and the specific deformation, tensile strength and hardness of the joints made of those two kinds of steel are intro... In this paper, the properties of S25C-SUS405 steel joints by vacuum diffusion welding are discussed, and the specific deformation, tensile strength and hardness of the joints made of those two kinds of steel are introduced. Through metallographic examination and microanalysis, it can be observed that at the weld interface of the joints there is a decarbonized layer on the S25C steel side and a carburized layer on the SUS405 steel side. This is the main cause giving rise to the heterogeneity of microstructure distribution and the nonuniformity of hardness distribution in weldment. In addition, with the help of electronic probe microanalysis the element distribution, such as carbon and chrome, is reported in this paper. 展开更多
关键词 VDW carburized layer decarbonized layer
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