High-resolution multi-color printing relies upon pixelated optical nanostructures,which is crucial to promote color display by producing nonbleaching colors,yet requires simplicity in fabrication and dynamic switching...High-resolution multi-color printing relies upon pixelated optical nanostructures,which is crucial to promote color display by producing nonbleaching colors,yet requires simplicity in fabrication and dynamic switching.Antimony trisulfide(Sb_(2)S_(3))is a newly rising chalcogenide material that possesses prompt and significant transition of its optical characteristics in the visible region between amorphous and crystalline phases,which holds the key to color-varying devices.Herein,we proposed a dynamically switchable color printing method using Sb_(2)S_(3)-based stepwise pixelated Fabry-Pérot(FP)cavities with various cavity lengths.The device was fabricated by employing a direct laser patterning that is a less timeconsuming,more approachable,and low-cost technique.As switching the state of Sb_(2)S_(3) between amorphous and crystalline,the multi-color of stepwise pixelated FP cavities can be actively changed.The color variation is due to the profound change in the refractive index of Sb_(2)S_(3) over the visible spectrum during its phase transition.Moreover,we directly fabricated sub-50 nm nano-grating on ultrathin Sb_(2)S_(3) laminate via microsphere 800-nm femtosecond laser irradiation in far field.The minimum feature size can be further decreased down to~45 nm(λ/17)by varying the thickness of Sb_(2)S_(3) film.Ultrafast switchable Sb_(2)S_(3) photonic devices can take one step toward the next generation of inkless erasable papers or displays and enable information encryption,camouflaging surfaces,anticounterfeiting,etc.Importantly,our work explores the prospects of rapid and rewritable fabrication of periodic structures with nano-scale resolution and can serve as a guideline for further development of chalcogenide-based photonics components.展开更多
Color filters are produced using semiconductor production techniques although problems with low yield remain to be addressed. This study presents a new means of selective removal using excimer irradiation, chemical et...Color filters are produced using semiconductor production techniques although problems with low yield remain to be addressed. This study presents a new means of selective removal using excimer irradiation, chemical etching, or electrochemical machining on the fifth generation TFT LCDs. The selective removal of microstructure layers from the color filter surface of an optoelectronic flat panel display, as well as complete removal of the ITO thin-films, RGB layer, or resin black matrix (BM) layer from the substrate is possible. Individual defective film layers can be removed, or all films down to the Cr layer or bare glass can be completely eliminated. Experimental results demonstrate that defective ITO thin-films, RGB layers, or the resin BM layer can now be recycled with a great precision. When the ITO or RGB layer proves difficult to remove, excimer light can be used to help with removal. During this recycling process, the use of 225 nm excimer irradiation before chemical etching, or electrochemical machining, makes removal of stubborn film residues easy, effectively improving the quality of recycled color filters and reducing fabrication cost.展开更多
Tamm plasmon polaritons(TPPs)are localized photonic states at the interface between a metal layer and one-dimensional(1D)photonic crystal substrate.Unlike surface plasmon polaritons(SPPs),TPPs can be excited by both t...Tamm plasmon polaritons(TPPs)are localized photonic states at the interface between a metal layer and one-dimensional(1D)photonic crystal substrate.Unlike surface plasmon polaritons(SPPs),TPPs can be excited by both transverse magnetic and electric waves without requiring additional coupling optics.TPPs offer robust color filtering,making them ideal for applications such as complementary metal oxide semiconductor(CMOS)image detectors.However,obtaining a large-area,reversible,and reconfigurable filter remains challenging.This study demonstrates a dynamically reconfigurable reflective color filter by integrating an ultrathin antimony trisulfide(Sb_(2)S_(3))layer with Tamm plasmonic photonic crystals.Reconfigurable tuning was achieved by inducing Sb_(2)S_(3) crystallization and reamorphization via thermal and optical activation,respectively.The material exhibited good stability after multiple switching cycles.The reflectance spectrum can be tuned across the visible range,with a shift of approximately 50 nm by switching Sb_(2)S_(3) between its amorphous and crystalline phases.This phase transition is nonvolatile and substantially minimizes the energy consumption,enhancing efficiency for practical applications.Tamm plasmonic photonic crystals are low-cost and large-scale production,offering a platform for compact color display systems and customizable photonic crystal filters for realistic system integration.展开更多
A multiplexed holographic display video has been achieved by using a passive azo-dye-doped liquid crystal （LC） cell. Holograms formed in this cell can be refreshed in the order of several milliseconds. By angular mu...A multiplexed holographic display video has been achieved by using a passive azo-dye-doped liquid crystal （LC） cell. Holograms formed in this cell can be refreshed in the order of several milliseconds. By angular multiplexing technique, dynamically multiplexed holographic videos are realized. Moreover, the reconstructed RGB images are merged into a color image, which illustrates the possibility of a color holographic three-dimensional （3D） display by holographic multiplexing of the LC cell.展开更多
A method of drawing color spectrogram of speech by using microcomputer is described in this paper , and referred to the metod of drawing spectrogram by computer . With the software and no addition any other aqripment....A method of drawing color spectrogram of speech by using microcomputer is described in this paper , and referred to the metod of drawing spectrogram by computer . With the software and no addition any other aqripment., we can draw color three - dimension spectrogram ( or black -white spectrogram without color monitor ), and it is similar to spectrogram of sonagrapher .展开更多
Vacuum-deposited perovskite light-emitting diodes(PeLEDs)have demonstrated significant potential for high-colorgamut active-matrix displays.Despite the rapid advance of green PeLEDs,red ones remain a considerable chal...Vacuum-deposited perovskite light-emitting diodes(PeLEDs)have demonstrated significant potential for high-colorgamut active-matrix displays.Despite the rapid advance of green PeLEDs,red ones remain a considerable challenge because of the inferior photophysical properties of vacuum-deposited red-light-emitting materials.Here,a rationally designed fluorine-modified phosphine oxide additive was introduced to in-situ passivate vacuum-deposited perovskites.The highly polar 2-F-TPPO incorporated perovskite films demonstrated enhanced photoluminescence quantum yield(PLQY),suppressed defects,and improved crystallinity.When implemented as active layers in PeLEDs,an external quantum efficiency(EQE)of 12.6%with an emission wavelength of 640 nm is achieved,which was 6 times higher compared to the previously reported most efficient vacuum-deposited red PeLEDs(EQE below 2%).Our findings lay the foundations for the further exploration of high-performance vacuum-deposited PeLEDs toward fullcolor perovskite displays.展开更多
Dynamic plasmonics with the real-time active control capability of plasmonic resonances attracts much interest in the communities of physics,chemistry,and material science.Among versatile reconfigurable strategies for...Dynamic plasmonics with the real-time active control capability of plasmonic resonances attracts much interest in the communities of physics,chemistry,and material science.Among versatile reconfigurable strategies for dynamic plasmonics,electrochemically driven strategies have garnered most of the attention.We summarize three primary strategies to enable electrochemically dynamic plasmonics,including structural transformation,carrier-density modulation,and electrochemically active surrounding-media manipulation.The reconfigurable microstructures,optical properties,and underlying physical mechanisms are discussed in detail.We also summarize the most promising applications of dynamic plasmonics,including smart windows,structural color displays,and chemical sensors.We suggest more research efforts toward the widespread applications of dynamic plasmonics.展开更多
We propose a simple gradation representation method using a binary-weighted computer-generated hologram（CGH） to be displayed on a high-speed spatial light modulator that can be controlled by the pulse-width modulati...We propose a simple gradation representation method using a binary-weighted computer-generated hologram（CGH） to be displayed on a high-speed spatial light modulator that can be controlled by the pulse-width modulation technique. The proposed method uses multiple bit planes comprising binary-weighted CGHs with various pulse widths. The object points of a three-dimensional（3D） object are assigned to multiple bit planes according to their gray levels. The bit planes are sequentially displayed in a time-division-multiplexed manner.Consequently, the proposed method realizes a gradation representation of a reconstructed 3D object.展开更多
基金support from the National Key Research and Development Program of China (2020YFA0714504,2019YFA0709100).
文摘High-resolution multi-color printing relies upon pixelated optical nanostructures,which is crucial to promote color display by producing nonbleaching colors,yet requires simplicity in fabrication and dynamic switching.Antimony trisulfide(Sb_(2)S_(3))is a newly rising chalcogenide material that possesses prompt and significant transition of its optical characteristics in the visible region between amorphous and crystalline phases,which holds the key to color-varying devices.Herein,we proposed a dynamically switchable color printing method using Sb_(2)S_(3)-based stepwise pixelated Fabry-Pérot(FP)cavities with various cavity lengths.The device was fabricated by employing a direct laser patterning that is a less timeconsuming,more approachable,and low-cost technique.As switching the state of Sb_(2)S_(3) between amorphous and crystalline,the multi-color of stepwise pixelated FP cavities can be actively changed.The color variation is due to the profound change in the refractive index of Sb_(2)S_(3) over the visible spectrum during its phase transition.Moreover,we directly fabricated sub-50 nm nano-grating on ultrathin Sb_(2)S_(3) laminate via microsphere 800-nm femtosecond laser irradiation in far field.The minimum feature size can be further decreased down to~45 nm(λ/17)by varying the thickness of Sb_(2)S_(3) film.Ultrafast switchable Sb_(2)S_(3) photonic devices can take one step toward the next generation of inkless erasable papers or displays and enable information encryption,camouflaging surfaces,anticounterfeiting,etc.Importantly,our work explores the prospects of rapid and rewritable fabrication of periodic structures with nano-scale resolution and can serve as a guideline for further development of chalcogenide-based photonics components.
基金supported by the BEN TEN CO., and National Science Council contracts 98-2221-E-152-001 and 99-2221-E-152-001
文摘Color filters are produced using semiconductor production techniques although problems with low yield remain to be addressed. This study presents a new means of selective removal using excimer irradiation, chemical etching, or electrochemical machining on the fifth generation TFT LCDs. The selective removal of microstructure layers from the color filter surface of an optoelectronic flat panel display, as well as complete removal of the ITO thin-films, RGB layer, or resin black matrix (BM) layer from the substrate is possible. Individual defective film layers can be removed, or all films down to the Cr layer or bare glass can be completely eliminated. Experimental results demonstrate that defective ITO thin-films, RGB layers, or the resin BM layer can now be recycled with a great precision. When the ITO or RGB layer proves difficult to remove, excimer light can be used to help with removal. During this recycling process, the use of 225 nm excimer irradiation before chemical etching, or electrochemical machining, makes removal of stubborn film residues easy, effectively improving the quality of recycled color filters and reducing fabrication cost.
文摘Tamm plasmon polaritons(TPPs)are localized photonic states at the interface between a metal layer and one-dimensional(1D)photonic crystal substrate.Unlike surface plasmon polaritons(SPPs),TPPs can be excited by both transverse magnetic and electric waves without requiring additional coupling optics.TPPs offer robust color filtering,making them ideal for applications such as complementary metal oxide semiconductor(CMOS)image detectors.However,obtaining a large-area,reversible,and reconfigurable filter remains challenging.This study demonstrates a dynamically reconfigurable reflective color filter by integrating an ultrathin antimony trisulfide(Sb_(2)S_(3))layer with Tamm plasmonic photonic crystals.Reconfigurable tuning was achieved by inducing Sb_(2)S_(3) crystallization and reamorphization via thermal and optical activation,respectively.The material exhibited good stability after multiple switching cycles.The reflectance spectrum can be tuned across the visible range,with a shift of approximately 50 nm by switching Sb_(2)S_(3) between its amorphous and crystalline phases.This phase transition is nonvolatile and substantially minimizes the energy consumption,enhancing efficiency for practical applications.Tamm plasmonic photonic crystals are low-cost and large-scale production,offering a platform for compact color display systems and customizable photonic crystal filters for realistic system integration.
基金sponsored by the National"973"Program of China(No.2013CB328804)the National Natural Science Foundation of China(No.61307028)the Science & Technology Commission of Shanghai Municipality(Nos.13ZR1420000 and 11JC1405300)
文摘A multiplexed holographic display video has been achieved by using a passive azo-dye-doped liquid crystal （LC） cell. Holograms formed in this cell can be refreshed in the order of several milliseconds. By angular multiplexing technique, dynamically multiplexed holographic videos are realized. Moreover, the reconstructed RGB images are merged into a color image, which illustrates the possibility of a color holographic three-dimensional （3D） display by holographic multiplexing of the LC cell.
文摘A method of drawing color spectrogram of speech by using microcomputer is described in this paper , and referred to the metod of drawing spectrogram by computer . With the software and no addition any other aqripment., we can draw color three - dimension spectrogram ( or black -white spectrogram without color monitor ), and it is similar to spectrogram of sonagrapher .
基金supported by the National Natural Science Foundation of China(62322505,62425502,62374069,62375060,62375276,U23A6002,and 62104077)Shanghai Pilot Program for Basic Research(22JC1403200)+2 种基金“Pioneer”and“Leading Goose”R&D Program of Zhejiang(2024C01192)the Natural Science Foundation of Hubei Province(2024AFB423 and 2023BAB102)the National Key Research and Development Program of China(2021YFB3501800,2023YFB3608903,2024YFA1209503).
文摘Vacuum-deposited perovskite light-emitting diodes(PeLEDs)have demonstrated significant potential for high-colorgamut active-matrix displays.Despite the rapid advance of green PeLEDs,red ones remain a considerable challenge because of the inferior photophysical properties of vacuum-deposited red-light-emitting materials.Here,a rationally designed fluorine-modified phosphine oxide additive was introduced to in-situ passivate vacuum-deposited perovskites.The highly polar 2-F-TPPO incorporated perovskite films demonstrated enhanced photoluminescence quantum yield(PLQY),suppressed defects,and improved crystallinity.When implemented as active layers in PeLEDs,an external quantum efficiency(EQE)of 12.6%with an emission wavelength of 640 nm is achieved,which was 6 times higher compared to the previously reported most efficient vacuum-deposited red PeLEDs(EQE below 2%).Our findings lay the foundations for the further exploration of high-performance vacuum-deposited PeLEDs toward fullcolor perovskite displays.
基金jointly supported by the National Natural Science Foundation of China(Nos.12022403,61735008,51925204,and 11874211)Key Science and Technology Innovation Program of Shandong Province(No.2019JZZY020704)the Fundamental Research Funds for the Central Universities(Nos.021314380140 and 021314380150)。
文摘Dynamic plasmonics with the real-time active control capability of plasmonic resonances attracts much interest in the communities of physics,chemistry,and material science.Among versatile reconfigurable strategies for dynamic plasmonics,electrochemically driven strategies have garnered most of the attention.We summarize three primary strategies to enable electrochemically dynamic plasmonics,including structural transformation,carrier-density modulation,and electrochemically active surrounding-media manipulation.The reconfigurable microstructures,optical properties,and underlying physical mechanisms are discussed in detail.We also summarize the most promising applications of dynamic plasmonics,including smart windows,structural color displays,and chemical sensors.We suggest more research efforts toward the widespread applications of dynamic plasmonics.
基金supported by the Japan Society for the Promotion of Science through a Grantin-Aid for Scientific Research(C)15K00153+1 种基金a Grant-in-Aid for Scientific Research(A)25240015
文摘We propose a simple gradation representation method using a binary-weighted computer-generated hologram（CGH） to be displayed on a high-speed spatial light modulator that can be controlled by the pulse-width modulation technique. The proposed method uses multiple bit planes comprising binary-weighted CGHs with various pulse widths. The object points of a three-dimensional（3D） object are assigned to multiple bit planes according to their gray levels. The bit planes are sequentially displayed in a time-division-multiplexed manner.Consequently, the proposed method realizes a gradation representation of a reconstructed 3D object.
