Five cadmium naphthalene-diphosphonates,formulated as[Cd_(1.5)(1,4-ndpaH_(2))2(4,4'-bpyH)(4,4'-bpy)0.5(H_(2)O)_(2)]2(1),[Cd(1,4-ndpaH_(2))(1,4-bib)0.5(H_(2)O)](2),[Cd(1,4-ndpaH3)2(1,2-dpe)(H_(2)O)]·(1,2-d...Five cadmium naphthalene-diphosphonates,formulated as[Cd_(1.5)(1,4-ndpaH_(2))2(4,4'-bpyH)(4,4'-bpy)0.5(H_(2)O)_(2)]2(1),[Cd(1,4-ndpaH_(2))(1,4-bib)0.5(H_(2)O)](2),[Cd(1,4-ndpaH3)2(1,2-dpe)(H_(2)O)]·(1,2-dpe)·7H_(2)O(3),(1,2-bixH)[Cd3(1,4-ndpaH)(1,4-ndpaH_(2))2(H_(2)O)_(2)](4),and[Cd(1,4-ndpaH_(2))(H_(2)O)]·H_(2)O(5),have been synthesized from the selfassembly reactions of 1,4-naphthalenediphosphonic acid(1,4-ndpaH4)with Cd(NO3)2·4H_(2)O by introducing auxiliary ligands with variation of rigidity,such as 4,4'-bipyridine(4,4'-bpy),1,4-bis(1-imidazolyl)benzene(1,4-bib),1,2-di(4-pyridyl)ethylene(1,2-dpe),1,3-di(4-pyridyl)propane(1,3-dpp),and bis(imidazol-1-ylmethyl)benzene(1,2-bix),respectively.Structure resolution by single-crystal X-ray diffraction reveals that compound 1 possesses a layered framework,in which the{Cd3(PO2)2}trimers made up of corner-sharing two{CdO4N2}and one{CdO6}octahedra are connected by phosphonate groups,forming a ribbon,which are cross-linked by 4,4'-bipy ligands,forming a 2D layer.Compound 2 shows a 3D open-framework structure,where chains of corner-sharing{CdO4N}trigonal bipyramids and{PO3C}tetrahedra are cross-linked by 1,4-bib and/or phosphonate groups.A 1D ladder-like chain structure is found in compound 3,where the ladder-like chains made up of corner-sharing{CdO5N}octahedra and{PO3C}tetra hedra are connected by 1,4-ndpaH_(2)^(2-).Both compounds 4 and 5 obtained by the introduction of flexible ligands during the synthesis show a 2D layered structure,which is formed by ligand crosslinking double metal chains.Interestingly,In 4,flexible 1,2-bix was singly protonated,as vip molecules,filled between layer and layer,while flexible ligand 1,3-dpp is absent in 5.Photophysical measurements indicate that compounds 1-5 show ligand-centered emissions.展开更多
Piezocomposites with both flexibility and electromechanical conversion characteristics have been widely applied in various fields,including sensors,energy harvesting,catalysis,and biomedical treatment.In the compositi...Piezocomposites with both flexibility and electromechanical conversion characteristics have been widely applied in various fields,including sensors,energy harvesting,catalysis,and biomedical treatment.In the composition of piezocomposites or their preparation process,a category of materials is commonly employed that do not possess piezoelectric properties themselves but play a crucial role in performance enhancement.In this review,the concept of auxiliary phase is first proposed to define these materials,aiming to provide a new perspective for designing high-performance piezocomposites.Three different categories of modulation forms of auxiliary phase in piezocomposites are systematically summarized,including the modification of piezo-matrix,the modification of piezo-fillers,and the construction of special structures.Each category emphasizes the role of the auxiliary phase and systematically discusses the latest advancements and the physical mechanisms of the auxiliary phase enhanced flexible piezocomposites.Finally,a summary and future outlook of piezocomposites based on the auxiliary phase are provided.展开更多
Climate downscaling is used to transform large-scale meteorological data into small-scale data with enhanced detail,which finds wide applications in climate modeling,numerical weather forecasting,and renewable energy....Climate downscaling is used to transform large-scale meteorological data into small-scale data with enhanced detail,which finds wide applications in climate modeling,numerical weather forecasting,and renewable energy.Although deeplearning-based downscaling methods effectively capture the complex nonlinear mapping between meteorological data of varying scales,the supervised deep-learning-based downscaling methods suffer from insufficient high-resolution data in practice,and unsupervised methods struggle with accurately inferring small-scale specifics from limited large-scale inputs due to small-scale uncertainty.This article presents DualDS,a dual-learning framework utilizing a Generative Adversarial Network–based neural network and subgrid-scale auxiliary information for climate downscaling.Such a learning method is unified in a two-stream framework through up-and downsamplers,where the downsampler is used to simulate the information loss process during the upscaling,and the upsampler is used to reconstruct lost details and correct errors incurred during the upscaling.This dual learning strategy can eliminate the dependence on high-resolution ground truth data in the training process and refine the downscaling results by constraining the mapping process.Experimental findings demonstrate that DualDS is comparable to several state-of-the-art deep learning downscaling approaches,both qualitatively and quantitatively.Specifically,for a single surface-temperature data downscaling task,our method is comparable with other unsupervised algorithms with the same dataset,and we can achieve a 0.469 dB higher peak signal-to-noise ratio,0.017 higher structural similarity,0.08 lower RMSE,and the best correlation coefficient.In summary,this paper presents a novel approach to addressing small-scale uncertainty issues in unsupervised downscaling processes.展开更多
In wideband noncooperative interference cancellation,the reference signals obtained through auxiliary antennas are weighted to cancel with the interference signal.The correlation between the reference signal and the i...In wideband noncooperative interference cancellation,the reference signals obtained through auxiliary antennas are weighted to cancel with the interference signal.The correlation between the reference signal and the interference signal determines interference cancellation performance,while the auxiliary antenna array affects the correlation by influencing the amplitude and phase of the reference signals.This paper analyzes the effect of auxiliary antenna array on multiple performances of wideband noncooperative interference cancellation.Firstly,the array received signal model of wideband interference is established,and the weight vector coupled with the auxiliary antennas array manifold is solved by spectral analysis and eigen-subspace decomposition.Then,multiple performances which include cancellation resolution,grating null,wideband interference cancellation ratio(ICR),and convergence rate are quantitatively characterized with the auxiliary antenna array.It is obtained through analysis that the performances mutually restrict the auxiliary antenna array.Higher cancellation resolution requires larger array aperture,but when the number of auxiliary antennas is fixed,larger array aperture results in more grating nulls.When the auxiliary antennas are closer to the main antenna,the wideband ICR is improved,but the convergence rate is reduced.The conclusions are verified through simulation of one-dimensional uniform array and two-dimensional nonuniform array.The experiments of three arrays are compared,and the results conform well with simulation and support the theoretical analysis.展开更多
An efficient and accurate scalar auxiliary variable(SAV)scheme for numerically solving nonlinear parabolic integro-differential equation(PIDE)is developed in this paper.The original equation is first transformed into ...An efficient and accurate scalar auxiliary variable(SAV)scheme for numerically solving nonlinear parabolic integro-differential equation(PIDE)is developed in this paper.The original equation is first transformed into an equivalent system,and the k-order backward differentiation formula(BDF k)and central difference formula are used to discretize the temporal and spatial derivatives,respectively.Different from the traditional discrete method that adopts full implicit or full explicit for the nonlinear integral terms,the proposed scheme is based on the SAV idea and can be treated semi-implicitly,taking into account both accuracy and effectiveness.Numerical results are presented to demonstrate the high-order convergence(up to fourth-order)of the developed schemes and it is computationally efficient in long-time computations.展开更多
The Global Stratotype Section and Point(GSSP)of the base-Wuchiapingian Stage was formally ratified at the Penglaitan section in South China in 2005.However,the riverside GSSP section at Penglaitan and its auxiliary se...The Global Stratotype Section and Point(GSSP)of the base-Wuchiapingian Stage was formally ratified at the Penglaitan section in South China in 2005.However,the riverside GSSP section at Penglaitan and its auxiliary section at Tieqiao have been permanently flooded since 2020.We herein designate an excavated section at Penglaitan as the new GSSP and the Fengshan section as a new Standard Auxiliary Boundary Stratotype(SABS).In addition,we revised the original definition based on a detailed restudy of the conodont succession from the two sections.We define the GSSP of the base-Wuchiapingian by the First Appearance Datum(FAD)of Clarkina postbitteri within the lineage Jinogondolella granti→Clarkina postbitteri→C.dukouensis.It represents a major evolutionary turnover in conodonts from Jinogondolella to Clarkina and marks the end-Guadalupian extinction event.The U-Pb date of 259.51±0.21 Ma from the uppermost part of the Emeishan basalt is adopted for the GLB age.δ13Ccarb chemostratigraphy at the SABS exhibits several excursions between 3‰and 5‰across the GLB interval.Carbonate 87Sr/86Sr ratio is 0.707244 at the GLB.Remarkably,the SABS contains six normal and six reverse geomagnetic polarity zones in the uppermost Capitanian and three in the lowest Wuchiapingian.展开更多
The Ideale section(IS)at Montalbano Jonico,Italy,has been approved as a Standard Auxiliary Boundary Stratotype(SABS)for the Global boundary Stratotype Section and Point(GSSP)of the Middle Pleistocene Subseries/Subepoc...The Ideale section(IS)at Montalbano Jonico,Italy,has been approved as a Standard Auxiliary Boundary Stratotype(SABS)for the Global boundary Stratotype Section and Point(GSSP)of the Middle Pleistocene Subseries/Subepoch and Chibanian Stage/Age at the Chiba section,Japan.The proposal was submitted to the voting members of the International Commission on Stratigraphy’s Subcommission on Quaternary Stratigraphy(SQS)on May 4,2023,and following discussions was approved on July 8,2023.The 74 m thick IS continuously spans the Marine Isotope Stage(MIS)20–18 interval,and is part of the longer Montalbano Jonico succession(Basilicata,southern Italy in the Mediterranean region)encompassing MIS 37 to early MIS 16.The IS provides a detailed record based on multiple chronologically well constrained marine and terrestrial proxies,which are particularly useful for outlining the paleoclimatic evolution through the Lower–Middle Pleistocene transition.The high-resolution carbon and oxygen isotope stratigraphy outlines glacial–interglacial and stadial–interstadial phases as well as the sub-millennialscale features of Termination IX and the onset of MIS 19c.The sapropel layer equivalent to insolation cycle 74(784 ka)occurs in early MIS 19c.A prominent peak in the 10Be/9Be record at the MIS 19c–19b transition identifies the low geomagnetic dipole moment associated with the Matuyama–Brunhes boundary interval.Two tephra layers(V3 and V4)relevant to boundary interval are 40Ar/39Ar dated.The V4 layer,occurring at the MIS 19c–b transition and in the middle of the 10Be/9Be peak,has an age of 774.1±0.9 ka,corresponding to the age of the Middle Pleistocene GSSP.A high-resolution alkenone sea-surface temperature and several paleobiological records complement the rich chronological and paleoenvironmental dataset from MIS 20 to the inception of MIS 18.The GSSP boundary interval in the IS is represented from 35.50 to 39.50 m,which corresponds to the interval of the highest values of the 10Be/9Be ratio(~776.35–771.87 ka)and includes the V4 tephra layer and the MIS 19c–MIS 19b transition.This SABS extends the correlation potential of the Middle Pleistocene Subseries/Subepoch GSSP interval to the Mediterranean region.展开更多
Einstein–Podolsky–Rosen(EPR) steering is an example of nontrivial quantum nonlocality and characteristic in the non-classical world.The directivity(or asymmetry) is a fascinating trait of EPR steering,and it is diff...Einstein–Podolsky–Rosen(EPR) steering is an example of nontrivial quantum nonlocality and characteristic in the non-classical world.The directivity(or asymmetry) is a fascinating trait of EPR steering,and it is different from other quantum nonlocalities.Here,we consider the strategy in which two atoms compose a two-qubit X state,and the two atoms are owned by Alice and Bob,respectively.The atom of Alice suffers from a reservoir,and the atom of Bob couples with a bit flip channel.The influences of auxiliary qubits on EPR steering and its directions are revealed by means of the entropy uncertainty relation.The results indicate that EPR steering declines with growing time t when adding fewer auxiliary qubits.The EPR steering behaves as damped oscillation when introducing more auxiliary qubits in the strong coupling regime.In the weak coupling regime,the EPR steering monotonously decreases as t increases when coupling auxiliary qubits.The increases in auxiliary qubits are responsible for the fact that the steerability from Alice to Bob(or from Bob to Alice) can be more effectively revealed.Notably,the introductions of more auxiliary qubits can change the situation that steerability from Alice to Bob is certain to a situation in which steerability from Bob to Alice is certain.展开更多
With the boom of the communication systems on some independent platforms(such as satellites,space stations,airplanes,and vessels),co-site interference is becoming prominent.The adaptive interference cancellation metho...With the boom of the communication systems on some independent platforms(such as satellites,space stations,airplanes,and vessels),co-site interference is becoming prominent.The adaptive interference cancellation method has been adopted to solve the co-site interference problem.But the broadband interference cancellation performance of traditional Adaptive Co-site Interference Cancellation System(ACICS)with large delay mismatching and antenna sway is relatively poor.This study put forward an Adaptive Co-site Broadband Interference Cancellation System With Two Auxiliary Channels(ACBICS-2A).The system model was established,and the steady state weights and Interference Cancellation Ratio(ICR)were deduced by solving a time-varying differential equation.The relationship of ICR,system gain,modulation factor,interference signal bandwidth and delay mismatching degree was acquired through an in-depth analysis.Compared with traditional adaptive interference cancellation system,the proposed ACBICS-2A can improve broadband interference cancellation ability remarkably with large delay mismatching and antenna sway for the effect of auxiliary channel.The maximum improved ICR is more than 25 dB.Finally,the theoretical and simulation results were verified by experiments.展开更多
This paper develops a generalized scalar auxiliary variable(SAV)method for the time-dependent Ginzburg-Landau equations.The backward Euler method is used for discretizing the temporal derivative of the time-dependent ...This paper develops a generalized scalar auxiliary variable(SAV)method for the time-dependent Ginzburg-Landau equations.The backward Euler method is used for discretizing the temporal derivative of the time-dependent Ginzburg-Landau equations.In this method,the system is decoupled and linearized to avoid solving the non-linear equation at each step.The theoretical analysis proves that the generalized SAV method can preserve the maximum bound principle and energy stability,and this is confirmed by the numerical result,and also shows that the numerical algorithm is stable.展开更多
Purpose–Auxiliary power system is an indispensable part of the train;the auxiliary systems of both electric locomotives and EMUs mainly are powered by one of the two ways,which are either from auxiliary windings of t...Purpose–Auxiliary power system is an indispensable part of the train;the auxiliary systems of both electric locomotives and EMUs mainly are powered by one of the two ways,which are either from auxiliary windings of traction transformers or from DC-link voltage of traction converters.Powered by DC-link voltage of traction converters,the auxiliary systems were maintained of uninterruptable power supply with energy from electric braking.Meanwhile,powered by traction transformers,the auxiliary systems were always out of power while passing the neutral section of power supply grid and control system is powered by battery at this time.Design/methodology/approach–Uninterrupted power supply of auxiliary power system powered by auxiliary winding of traction transformer was studied.Failure reasons why previous solutions cannot be realized are analyzed.An uninterruptable power supply scheme for the auxiliary systems powered by auxiliary windings of traction transformers is proposed in this paper.The validity of the proposed scheme is verified by simulation and experimental results and on-site operation of an upgraded HXD3C type locomotive.This scheme is attractive for upgrading practical locomotives with the auxiliary systems powered by auxiliary windings of traction transformers.Findings–This scheme regenerates braking power supplied to auxiliary windings of traction transformers while a locomotive runs in the neutral section of the power supply grid.Control objectives of uninterrupted power supply technology are proposed,which are no overvoltage,no overcurrent and uninterrupted power supply.Originality/value–The control strategies of the scheme ensure both overvoltage free and inrush current free when a locomotive enters or leaves the neutral section.Furthermore,this scheme is cost low by employing updated control strategy of software and add both the two current sensors and two connection wires of hardware.展开更多
From July 16th to 19th,2024,2024 National Practical Technical Training on Textile Printing and Dyeing Auxiliary Preparation,organized by China Research Institute of Daily Chemical and National Engineering Research Cen...From July 16th to 19th,2024,2024 National Practical Technical Training on Textile Printing and Dyeing Auxiliary Preparation,organized by China Research Institute of Daily Chemical and National Engineering Research Center for Surfactants,and co-organized by the Dyeing and Finishing Technology Research Institute of Zhejiang Fashion Institute of Technology and the High Fastness Plant-based Dye Research Base of China Textile Engineering Society,was held successfully in Shangyu,Zhejiang Province,with 92 representatives from 64 work units from all over China.展开更多
The developed auxiliary software serves to simplify, standardize and facilitate the software loading of the structural organization of a complex technological system, as well as its further manipulation within the pro...The developed auxiliary software serves to simplify, standardize and facilitate the software loading of the structural organization of a complex technological system, as well as its further manipulation within the process of solving the considered technological system. Its help can be especially useful in the case of a complex structural organization of a technological system with a large number of different functional elements grouped into several technological subsystems. This paper presents the results of its application for a special complex technological system related to the reference steam block for the combined production of heat and electricity.展开更多
Constrained multi-objective optimization problems(CMOPs) include the optimization of objective functions and the satisfaction of constraint conditions, which challenge the solvers.To solve CMOPs, constrained multi-obj...Constrained multi-objective optimization problems(CMOPs) include the optimization of objective functions and the satisfaction of constraint conditions, which challenge the solvers.To solve CMOPs, constrained multi-objective evolutionary algorithms(CMOEAs) have been developed. However, most of them tend to converge into local areas due to the loss of diversity. Evolutionary multitasking(EMT) is new model of solving complex optimization problems, through the knowledge transfer between the source task and other related tasks. Inspired by EMT, this paper develops a new EMT-based CMOEA to solve CMOPs, in which the main task, a global auxiliary task, and a local auxiliary task are created and optimized by one specific population respectively. The main task focuses on finding the feasible Pareto front(PF), and global and local auxiliary tasks are used to respectively enhance global and local diversity. Moreover, the global auxiliary task is used to implement the global search by ignoring constraints, so as to help the population of the main task pass through infeasible obstacles. The local auxiliary task is used to provide local diversity around the population of the main task, so as to exploit promising regions. Through the knowledge transfer among the three tasks, the search ability of the population of the main task will be significantly improved. Compared with other state-of-the-art CMOEAs, the experimental results on three benchmark test suites demonstrate the superior or competitive performance of the proposed CMOEA.展开更多
In this paper, an efficient approximated method based upon the method of auxiliary sources （MAS） is proposed to solve the two-dimensional scattering problem of large, infinite dielectric cylinder. To reduce the size...In this paper, an efficient approximated method based upon the method of auxiliary sources （MAS） is proposed to solve the two-dimensional scattering problem of large, infinite dielectric cylinder. To reduce the size of the total computational cost, the formulation of the MAS is modified by minimizing the number of auxiliary sources considered to implement the solution. It is shown that the standard formulation of the method of auxiliary sources, based on placing a finite number of auxiliary sources in an interior cylinder and the same number in the exterior cylinder surrounding the physical boundary, can be replaced by a finite number of strips placed on the same interior and exterior cylinder. These strips, containing auxiliary sources, are separated by a constant angle. Thus, compared with the standard MAS, the number of auxiliary sources of the new approximated method is reduced; also the proposed method can greatly reduce the computational complexity and the memory requirement. The numerical results obtained in this paper reveal the validity of the proposed approximated method.展开更多
Only in the presence of sidelobe jamming （SLJ）, can the conventional adaptive monopulse technique null the jamming effectively and maintain the monopulse angle estimation accuracy simultaneously. While mainlobe jamm...Only in the presence of sidelobe jamming （SLJ）, can the conventional adaptive monopulse technique null the jamming effectively and maintain the monopulse angle estimation accuracy simultaneously. While mainlobe jamming （MLJ） exists, the mainlobe of adaptive pattern will subject to serious distortion, which results in a failure of detecting and tracking targets by monopulse technique. Therefore, a monopulse angle estimation algorithm based on combining sum-difference beam and auxiliary beam is presented. This algorithm utilizes both high gain difference beams and high gain auxiliary beams for cancelling the mainlobe jammer and multiple sidelobe jammers （SLJs） while keeping an adap- tive monopulse ratio. Theoretical analysis and simulation results indicate that the serious invalidation of monopulse technique in MLJ and SLJs scenarios is resolved well, which improves the monopulse angle accuracy greatly. Furthermore, the proposed algorithm is of simple implementation and low computational complexity.展开更多
A new procedure for the highly diastereoselective synthesis of （1S）-trans-cyclopropane derivatives using a fructose derivative as the chiral auxiliary was developed. Chloroacetylated 1,2;4,5-di-O-isopropylidene-D-fr...A new procedure for the highly diastereoselective synthesis of （1S）-trans-cyclopropane derivatives using a fructose derivative as the chiral auxiliary was developed. Chloroacetylated 1,2;4,5-di-O-isopropylidene-D-fructopyranose was reacted with a tertiary amine to form the ammonium salt, which was treated with cesium carbonate to give the cyclopropane derivative through ylide intermediate. The described procedure provides an efficient method to synthesize optically pure dior poly-substituded cyclopropanes.展开更多
The reliability of the on-wing aircraft Auxiliary Power Unit(APU)decides the cost and the comfort of flight to a large degree.The most important function of APU is to help start main engines by providing compressed ai...The reliability of the on-wing aircraft Auxiliary Power Unit(APU)decides the cost and the comfort of flight to a large degree.The most important function of APU is to help start main engines by providing compressed air.Especially on the condition of sudden shutdown in the air,APU can offer additional thrust for landing.Therefore,its condition monitoring has drawn much attention from the academic and industrial field.Among the on-wing sensing data which can reflect its condition,Exhaust Gas Temperature(EGT)is one of the most important parameters.To ensure the reliability of EGT,one kind of data-driven anomaly detection framework for EGT sensing data is proposed based on the Gaussian Process Regression and Kernel Principal Component Analysis.The situations of one-dimensional and two-dimensional input data for EGT anomaly detection are considered,respectively.The cross-validation experiments are carried out by utilizing the real condition data of APU,which are provided by China Southern Airlines Company Limited Shenyang Maintenance Base.The anomalous stuck condition of EGT sensing data is also detected.Experimental results show that the proposed EGT sensing data anomaly detection method can achieve better performance of false positive ratio,false negative ratio and accuracy.展开更多
A new hybrid welding process was successfully used to join aluminum alloy and stainless steel. In the MIG welding-brazing process, the lower thermal conductivity of steel can cause dramatic change of temperature gradi...A new hybrid welding process was successfully used to join aluminum alloy and stainless steel. In the MIG welding-brazing process, the lower thermal conductivity of steel can cause dramatic change of temperature gradient on steel surface, while the auxiliary TIG arc can change this phenomenon by heating the steel side. The auxiliary TIG improved the wettability of molten metal, resulting in the molten metal spreading fully on upper surfaces, front and back surface of steel, forming a sound brazing joint; the content of Cr and Ni elements in IMCs layer was increased, which can enhance the quality of the layer; and the microstructure of IMCs layer also was improved, increasing the bonding strength with the weld seam. The average tensile strength of the joint obtained with auxiliary TIG arc（146.7 MPa） was higher than that without auxiliary TIG arc（96.7 MPa）.展开更多
文摘Five cadmium naphthalene-diphosphonates,formulated as[Cd_(1.5)(1,4-ndpaH_(2))2(4,4'-bpyH)(4,4'-bpy)0.5(H_(2)O)_(2)]2(1),[Cd(1,4-ndpaH_(2))(1,4-bib)0.5(H_(2)O)](2),[Cd(1,4-ndpaH3)2(1,2-dpe)(H_(2)O)]·(1,2-dpe)·7H_(2)O(3),(1,2-bixH)[Cd3(1,4-ndpaH)(1,4-ndpaH_(2))2(H_(2)O)_(2)](4),and[Cd(1,4-ndpaH_(2))(H_(2)O)]·H_(2)O(5),have been synthesized from the selfassembly reactions of 1,4-naphthalenediphosphonic acid(1,4-ndpaH4)with Cd(NO3)2·4H_(2)O by introducing auxiliary ligands with variation of rigidity,such as 4,4'-bipyridine(4,4'-bpy),1,4-bis(1-imidazolyl)benzene(1,4-bib),1,2-di(4-pyridyl)ethylene(1,2-dpe),1,3-di(4-pyridyl)propane(1,3-dpp),and bis(imidazol-1-ylmethyl)benzene(1,2-bix),respectively.Structure resolution by single-crystal X-ray diffraction reveals that compound 1 possesses a layered framework,in which the{Cd3(PO2)2}trimers made up of corner-sharing two{CdO4N2}and one{CdO6}octahedra are connected by phosphonate groups,forming a ribbon,which are cross-linked by 4,4'-bipy ligands,forming a 2D layer.Compound 2 shows a 3D open-framework structure,where chains of corner-sharing{CdO4N}trigonal bipyramids and{PO3C}tetrahedra are cross-linked by 1,4-bib and/or phosphonate groups.A 1D ladder-like chain structure is found in compound 3,where the ladder-like chains made up of corner-sharing{CdO5N}octahedra and{PO3C}tetra hedra are connected by 1,4-ndpaH_(2)^(2-).Both compounds 4 and 5 obtained by the introduction of flexible ligands during the synthesis show a 2D layered structure,which is formed by ligand crosslinking double metal chains.Interestingly,In 4,flexible 1,2-bix was singly protonated,as vip molecules,filled between layer and layer,while flexible ligand 1,3-dpp is absent in 5.Photophysical measurements indicate that compounds 1-5 show ligand-centered emissions.
基金supported by the Beijing Natural Science Foundation(Grant No.JL23004)the National Natural Science Foundation of China(Grant Nos.52473120,52472117,52072010,51972005 and 52325204).
文摘Piezocomposites with both flexibility and electromechanical conversion characteristics have been widely applied in various fields,including sensors,energy harvesting,catalysis,and biomedical treatment.In the composition of piezocomposites or their preparation process,a category of materials is commonly employed that do not possess piezoelectric properties themselves but play a crucial role in performance enhancement.In this review,the concept of auxiliary phase is first proposed to define these materials,aiming to provide a new perspective for designing high-performance piezocomposites.Three different categories of modulation forms of auxiliary phase in piezocomposites are systematically summarized,including the modification of piezo-matrix,the modification of piezo-fillers,and the construction of special structures.Each category emphasizes the role of the auxiliary phase and systematically discusses the latest advancements and the physical mechanisms of the auxiliary phase enhanced flexible piezocomposites.Finally,a summary and future outlook of piezocomposites based on the auxiliary phase are provided.
基金supported by the following funding bodies:the National Key Research and Development Program of China(Grant No.2020YFA0608000)National Science Foundation of China(Grant Nos.42075142,42375148,42125503+2 种基金42130608)FY-APP-2022.0609,Sichuan Province Key Tech nology Research and Development project(Grant Nos.2024ZHCG0168,2024ZHCG0176,2023YFG0305,2023YFG-0124,and 23ZDYF0091)the CUIT Science and Technology Innovation Capacity Enhancement Program project(Grant No.KYQN202305)。
文摘Climate downscaling is used to transform large-scale meteorological data into small-scale data with enhanced detail,which finds wide applications in climate modeling,numerical weather forecasting,and renewable energy.Although deeplearning-based downscaling methods effectively capture the complex nonlinear mapping between meteorological data of varying scales,the supervised deep-learning-based downscaling methods suffer from insufficient high-resolution data in practice,and unsupervised methods struggle with accurately inferring small-scale specifics from limited large-scale inputs due to small-scale uncertainty.This article presents DualDS,a dual-learning framework utilizing a Generative Adversarial Network–based neural network and subgrid-scale auxiliary information for climate downscaling.Such a learning method is unified in a two-stream framework through up-and downsamplers,where the downsampler is used to simulate the information loss process during the upscaling,and the upsampler is used to reconstruct lost details and correct errors incurred during the upscaling.This dual learning strategy can eliminate the dependence on high-resolution ground truth data in the training process and refine the downscaling results by constraining the mapping process.Experimental findings demonstrate that DualDS is comparable to several state-of-the-art deep learning downscaling approaches,both qualitatively and quantitatively.Specifically,for a single surface-temperature data downscaling task,our method is comparable with other unsupervised algorithms with the same dataset,and we can achieve a 0.469 dB higher peak signal-to-noise ratio,0.017 higher structural similarity,0.08 lower RMSE,and the best correlation coefficient.In summary,this paper presents a novel approach to addressing small-scale uncertainty issues in unsupervised downscaling processes.
基金supported by the National Fund for Distinguished Young Scholars(52025072)the National Natural Science Foundation of China(52177012)the Foundation of National Key Laboratory of Science and Technology(614221722051301).
文摘In wideband noncooperative interference cancellation,the reference signals obtained through auxiliary antennas are weighted to cancel with the interference signal.The correlation between the reference signal and the interference signal determines interference cancellation performance,while the auxiliary antenna array affects the correlation by influencing the amplitude and phase of the reference signals.This paper analyzes the effect of auxiliary antenna array on multiple performances of wideband noncooperative interference cancellation.Firstly,the array received signal model of wideband interference is established,and the weight vector coupled with the auxiliary antennas array manifold is solved by spectral analysis and eigen-subspace decomposition.Then,multiple performances which include cancellation resolution,grating null,wideband interference cancellation ratio(ICR),and convergence rate are quantitatively characterized with the auxiliary antenna array.It is obtained through analysis that the performances mutually restrict the auxiliary antenna array.Higher cancellation resolution requires larger array aperture,but when the number of auxiliary antennas is fixed,larger array aperture results in more grating nulls.When the auxiliary antennas are closer to the main antenna,the wideband ICR is improved,but the convergence rate is reduced.The conclusions are verified through simulation of one-dimensional uniform array and two-dimensional nonuniform array.The experiments of three arrays are compared,and the results conform well with simulation and support the theoretical analysis.
基金Supported by the National Natural Science Foundation of China(Grant Nos.12001210 and 12261103)the Natural Science Foundation of Henan(Grant No.252300420308)the Yunnan Fundamental Research Projects(Grant No.202301AT070117).
文摘An efficient and accurate scalar auxiliary variable(SAV)scheme for numerically solving nonlinear parabolic integro-differential equation(PIDE)is developed in this paper.The original equation is first transformed into an equivalent system,and the k-order backward differentiation formula(BDF k)and central difference formula are used to discretize the temporal and spatial derivatives,respectively.Different from the traditional discrete method that adopts full implicit or full explicit for the nonlinear integral terms,the proposed scheme is based on the SAV idea and can be treated semi-implicitly,taking into account both accuracy and effectiveness.Numerical results are presented to demonstrate the high-order convergence(up to fourth-order)of the developed schemes and it is computationally efficient in long-time computations.
基金supported by the National Natural Science Foundation of China(42293280,42272031,42250104,42261144668)Strategic Priority Research Program(B)of the Chinese Academy of Sciences(XDB26000000).
文摘The Global Stratotype Section and Point(GSSP)of the base-Wuchiapingian Stage was formally ratified at the Penglaitan section in South China in 2005.However,the riverside GSSP section at Penglaitan and its auxiliary section at Tieqiao have been permanently flooded since 2020.We herein designate an excavated section at Penglaitan as the new GSSP and the Fengshan section as a new Standard Auxiliary Boundary Stratotype(SABS).In addition,we revised the original definition based on a detailed restudy of the conodont succession from the two sections.We define the GSSP of the base-Wuchiapingian by the First Appearance Datum(FAD)of Clarkina postbitteri within the lineage Jinogondolella granti→Clarkina postbitteri→C.dukouensis.It represents a major evolutionary turnover in conodonts from Jinogondolella to Clarkina and marks the end-Guadalupian extinction event.The U-Pb date of 259.51±0.21 Ma from the uppermost part of the Emeishan basalt is adopted for the GLB age.δ13Ccarb chemostratigraphy at the SABS exhibits several excursions between 3‰and 5‰across the GLB interval.Carbonate 87Sr/86Sr ratio is 0.707244 at the GLB.Remarkably,the SABS contains six normal and six reverse geomagnetic polarity zones in the uppermost Capitanian and three in the lowest Wuchiapingian.
文摘The Ideale section(IS)at Montalbano Jonico,Italy,has been approved as a Standard Auxiliary Boundary Stratotype(SABS)for the Global boundary Stratotype Section and Point(GSSP)of the Middle Pleistocene Subseries/Subepoch and Chibanian Stage/Age at the Chiba section,Japan.The proposal was submitted to the voting members of the International Commission on Stratigraphy’s Subcommission on Quaternary Stratigraphy(SQS)on May 4,2023,and following discussions was approved on July 8,2023.The 74 m thick IS continuously spans the Marine Isotope Stage(MIS)20–18 interval,and is part of the longer Montalbano Jonico succession(Basilicata,southern Italy in the Mediterranean region)encompassing MIS 37 to early MIS 16.The IS provides a detailed record based on multiple chronologically well constrained marine and terrestrial proxies,which are particularly useful for outlining the paleoclimatic evolution through the Lower–Middle Pleistocene transition.The high-resolution carbon and oxygen isotope stratigraphy outlines glacial–interglacial and stadial–interstadial phases as well as the sub-millennialscale features of Termination IX and the onset of MIS 19c.The sapropel layer equivalent to insolation cycle 74(784 ka)occurs in early MIS 19c.A prominent peak in the 10Be/9Be record at the MIS 19c–19b transition identifies the low geomagnetic dipole moment associated with the Matuyama–Brunhes boundary interval.Two tephra layers(V3 and V4)relevant to boundary interval are 40Ar/39Ar dated.The V4 layer,occurring at the MIS 19c–b transition and in the middle of the 10Be/9Be peak,has an age of 774.1±0.9 ka,corresponding to the age of the Middle Pleistocene GSSP.A high-resolution alkenone sea-surface temperature and several paleobiological records complement the rich chronological and paleoenvironmental dataset from MIS 20 to the inception of MIS 18.The GSSP boundary interval in the IS is represented from 35.50 to 39.50 m,which corresponds to the interval of the highest values of the 10Be/9Be ratio(~776.35–771.87 ka)and includes the V4 tephra layer and the MIS 19c–MIS 19b transition.This SABS extends the correlation potential of the Middle Pleistocene Subseries/Subepoch GSSP interval to the Mediterranean region.
基金Project supported by the National Natural Science Foundation of China(Grant No.12175001)the Key Project of Natural Science Research of West Anhui University(Grant No.WXZR202311)+7 种基金the Natural Science Research Key Project of Education Department of Anhui Province of China(Grant Nos.KJ2021A0943,2022AH051681,and 2023AH052648)the Open Fund of Anhui Undergrowth Crop Intelligent Equipment Engineering Research Center(Grant No.AUCIEERC-2022-01)Anhui Undergrowth Crop Intelligent Equipment Engineering Research Center(Grant No.2022AH010091)the University Synergy Innovation Program of Anhui Province(Grant No.GXXT-2021-026)the Anhui Provincial Natural Science Foundation(Grant Nos.2108085MA18 and 2008085MA20)Key Project of Program for Excellent Young Talents of Anhui Universities(Grant No.gxyq ZD2019042)the open project of the Key Laboratory of Functional Materials and Devices for Informatics of Anhui Higher Education Institutes(Grant No.FMDI202106)the research start-up funding project of High Level Talent of West Anhui University(Grant No.WGKQ2021048)。
文摘Einstein–Podolsky–Rosen(EPR) steering is an example of nontrivial quantum nonlocality and characteristic in the non-classical world.The directivity(or asymmetry) is a fascinating trait of EPR steering,and it is different from other quantum nonlocalities.Here,we consider the strategy in which two atoms compose a two-qubit X state,and the two atoms are owned by Alice and Bob,respectively.The atom of Alice suffers from a reservoir,and the atom of Bob couples with a bit flip channel.The influences of auxiliary qubits on EPR steering and its directions are revealed by means of the entropy uncertainty relation.The results indicate that EPR steering declines with growing time t when adding fewer auxiliary qubits.The EPR steering behaves as damped oscillation when introducing more auxiliary qubits in the strong coupling regime.In the weak coupling regime,the EPR steering monotonously decreases as t increases when coupling auxiliary qubits.The increases in auxiliary qubits are responsible for the fact that the steerability from Alice to Bob(or from Bob to Alice) can be more effectively revealed.Notably,the introductions of more auxiliary qubits can change the situation that steerability from Alice to Bob is certain to a situation in which steerability from Bob to Alice is certain.
基金supported by the National Natural Science Foundation of China[Grant No.61771187]the Natural Science Foundation of Hubei Province[Grant No.2016CFB396]+1 种基金the Hubei Provincial Technology Innovation Special Major Project[Grant No.2019AAA018]the Major Project of Hubei Collaborative Innovation Center for High-efficiency Utilization of Solar Energy[HBSKFZD2015002].
文摘With the boom of the communication systems on some independent platforms(such as satellites,space stations,airplanes,and vessels),co-site interference is becoming prominent.The adaptive interference cancellation method has been adopted to solve the co-site interference problem.But the broadband interference cancellation performance of traditional Adaptive Co-site Interference Cancellation System(ACICS)with large delay mismatching and antenna sway is relatively poor.This study put forward an Adaptive Co-site Broadband Interference Cancellation System With Two Auxiliary Channels(ACBICS-2A).The system model was established,and the steady state weights and Interference Cancellation Ratio(ICR)were deduced by solving a time-varying differential equation.The relationship of ICR,system gain,modulation factor,interference signal bandwidth and delay mismatching degree was acquired through an in-depth analysis.Compared with traditional adaptive interference cancellation system,the proposed ACBICS-2A can improve broadband interference cancellation ability remarkably with large delay mismatching and antenna sway for the effect of auxiliary channel.The maximum improved ICR is more than 25 dB.Finally,the theoretical and simulation results were verified by experiments.
基金supported by the National Natural Science Foundation of China(12126318,12126302).
文摘This paper develops a generalized scalar auxiliary variable(SAV)method for the time-dependent Ginzburg-Landau equations.The backward Euler method is used for discretizing the temporal derivative of the time-dependent Ginzburg-Landau equations.In this method,the system is decoupled and linearized to avoid solving the non-linear equation at each step.The theoretical analysis proves that the generalized SAV method can preserve the maximum bound principle and energy stability,and this is confirmed by the numerical result,and also shows that the numerical algorithm is stable.
文摘Purpose–Auxiliary power system is an indispensable part of the train;the auxiliary systems of both electric locomotives and EMUs mainly are powered by one of the two ways,which are either from auxiliary windings of traction transformers or from DC-link voltage of traction converters.Powered by DC-link voltage of traction converters,the auxiliary systems were maintained of uninterruptable power supply with energy from electric braking.Meanwhile,powered by traction transformers,the auxiliary systems were always out of power while passing the neutral section of power supply grid and control system is powered by battery at this time.Design/methodology/approach–Uninterrupted power supply of auxiliary power system powered by auxiliary winding of traction transformer was studied.Failure reasons why previous solutions cannot be realized are analyzed.An uninterruptable power supply scheme for the auxiliary systems powered by auxiliary windings of traction transformers is proposed in this paper.The validity of the proposed scheme is verified by simulation and experimental results and on-site operation of an upgraded HXD3C type locomotive.This scheme is attractive for upgrading practical locomotives with the auxiliary systems powered by auxiliary windings of traction transformers.Findings–This scheme regenerates braking power supplied to auxiliary windings of traction transformers while a locomotive runs in the neutral section of the power supply grid.Control objectives of uninterrupted power supply technology are proposed,which are no overvoltage,no overcurrent and uninterrupted power supply.Originality/value–The control strategies of the scheme ensure both overvoltage free and inrush current free when a locomotive enters or leaves the neutral section.Furthermore,this scheme is cost low by employing updated control strategy of software and add both the two current sensors and two connection wires of hardware.
文摘From July 16th to 19th,2024,2024 National Practical Technical Training on Textile Printing and Dyeing Auxiliary Preparation,organized by China Research Institute of Daily Chemical and National Engineering Research Center for Surfactants,and co-organized by the Dyeing and Finishing Technology Research Institute of Zhejiang Fashion Institute of Technology and the High Fastness Plant-based Dye Research Base of China Textile Engineering Society,was held successfully in Shangyu,Zhejiang Province,with 92 representatives from 64 work units from all over China.
文摘The developed auxiliary software serves to simplify, standardize and facilitate the software loading of the structural organization of a complex technological system, as well as its further manipulation within the process of solving the considered technological system. Its help can be especially useful in the case of a complex structural organization of a technological system with a large number of different functional elements grouped into several technological subsystems. This paper presents the results of its application for a special complex technological system related to the reference steam block for the combined production of heat and electricity.
基金supported in part by the National Natural Science Fund for Outstanding Young Scholars of China (61922072)the National Natural Science Foundation of China (62176238, 61806179, 61876169, 61976237)+2 种基金China Postdoctoral Science Foundation (2020M682347)the Training Program of Young Backbone Teachers in Colleges and Universities in Henan Province (2020GGJS006)Henan Provincial Young Talents Lifting Project (2021HYTP007)。
文摘Constrained multi-objective optimization problems(CMOPs) include the optimization of objective functions and the satisfaction of constraint conditions, which challenge the solvers.To solve CMOPs, constrained multi-objective evolutionary algorithms(CMOEAs) have been developed. However, most of them tend to converge into local areas due to the loss of diversity. Evolutionary multitasking(EMT) is new model of solving complex optimization problems, through the knowledge transfer between the source task and other related tasks. Inspired by EMT, this paper develops a new EMT-based CMOEA to solve CMOPs, in which the main task, a global auxiliary task, and a local auxiliary task are created and optimized by one specific population respectively. The main task focuses on finding the feasible Pareto front(PF), and global and local auxiliary tasks are used to respectively enhance global and local diversity. Moreover, the global auxiliary task is used to implement the global search by ignoring constraints, so as to help the population of the main task pass through infeasible obstacles. The local auxiliary task is used to provide local diversity around the population of the main task, so as to exploit promising regions. Through the knowledge transfer among the three tasks, the search ability of the population of the main task will be significantly improved. Compared with other state-of-the-art CMOEAs, the experimental results on three benchmark test suites demonstrate the superior or competitive performance of the proposed CMOEA.
文摘In this paper, an efficient approximated method based upon the method of auxiliary sources （MAS） is proposed to solve the two-dimensional scattering problem of large, infinite dielectric cylinder. To reduce the size of the total computational cost, the formulation of the MAS is modified by minimizing the number of auxiliary sources considered to implement the solution. It is shown that the standard formulation of the method of auxiliary sources, based on placing a finite number of auxiliary sources in an interior cylinder and the same number in the exterior cylinder surrounding the physical boundary, can be replaced by a finite number of strips placed on the same interior and exterior cylinder. These strips, containing auxiliary sources, are separated by a constant angle. Thus, compared with the standard MAS, the number of auxiliary sources of the new approximated method is reduced; also the proposed method can greatly reduce the computational complexity and the memory requirement. The numerical results obtained in this paper reveal the validity of the proposed approximated method.
基金supported by the National Natural Science Foundation of China(60925005)
文摘Only in the presence of sidelobe jamming （SLJ）, can the conventional adaptive monopulse technique null the jamming effectively and maintain the monopulse angle estimation accuracy simultaneously. While mainlobe jamming （MLJ） exists, the mainlobe of adaptive pattern will subject to serious distortion, which results in a failure of detecting and tracking targets by monopulse technique. Therefore, a monopulse angle estimation algorithm based on combining sum-difference beam and auxiliary beam is presented. This algorithm utilizes both high gain difference beams and high gain auxiliary beams for cancelling the mainlobe jammer and multiple sidelobe jammers （SLJs） while keeping an adap- tive monopulse ratio. Theoretical analysis and simulation results indicate that the serious invalidation of monopulse technique in MLJ and SLJs scenarios is resolved well, which improves the monopulse angle accuracy greatly. Furthermore, the proposed algorithm is of simple implementation and low computational complexity.
基金National Natural Science Foundation of China (Grant No. 20602001)
文摘A new procedure for the highly diastereoselective synthesis of （1S）-trans-cyclopropane derivatives using a fructose derivative as the chiral auxiliary was developed. Chloroacetylated 1,2;4,5-di-O-isopropylidene-D-fructopyranose was reacted with a tertiary amine to form the ammonium salt, which was treated with cesium carbonate to give the cyclopropane derivative through ylide intermediate. The described procedure provides an efficient method to synthesize optically pure dior poly-substituded cyclopropanes.
基金partially supported by the National Natural Science Foundation of China(No.61803121)China Postdoctoral Science Foundation(No.2019M651277).
文摘The reliability of the on-wing aircraft Auxiliary Power Unit(APU)decides the cost and the comfort of flight to a large degree.The most important function of APU is to help start main engines by providing compressed air.Especially on the condition of sudden shutdown in the air,APU can offer additional thrust for landing.Therefore,its condition monitoring has drawn much attention from the academic and industrial field.Among the on-wing sensing data which can reflect its condition,Exhaust Gas Temperature(EGT)is one of the most important parameters.To ensure the reliability of EGT,one kind of data-driven anomaly detection framework for EGT sensing data is proposed based on the Gaussian Process Regression and Kernel Principal Component Analysis.The situations of one-dimensional and two-dimensional input data for EGT anomaly detection are considered,respectively.The cross-validation experiments are carried out by utilizing the real condition data of APU,which are provided by China Southern Airlines Company Limited Shenyang Maintenance Base.The anomalous stuck condition of EGT sensing data is also detected.Experimental results show that the proposed EGT sensing data anomaly detection method can achieve better performance of false positive ratio,false negative ratio and accuracy.
文摘A new hybrid welding process was successfully used to join aluminum alloy and stainless steel. In the MIG welding-brazing process, the lower thermal conductivity of steel can cause dramatic change of temperature gradient on steel surface, while the auxiliary TIG arc can change this phenomenon by heating the steel side. The auxiliary TIG improved the wettability of molten metal, resulting in the molten metal spreading fully on upper surfaces, front and back surface of steel, forming a sound brazing joint; the content of Cr and Ni elements in IMCs layer was increased, which can enhance the quality of the layer; and the microstructure of IMCs layer also was improved, increasing the bonding strength with the weld seam. The average tensile strength of the joint obtained with auxiliary TIG arc（146.7 MPa） was higher than that without auxiliary TIG arc（96.7 MPa）.
