Ambient logics have been proposed to describe properties for mobile agentswhich may evolve over time as well as space. This paper takes a predicate-based approach toextending an ambient logic with recursion, yielding ...Ambient logics have been proposed to describe properties for mobile agentswhich may evolve over time as well as space. This paper takes a predicate-based approach toextending an ambient logic with recursion, yielding a predicate μ-calculus in which fixpointformulas are formed using predicate variables. An algorithm is developed for model checkingfinite-control mobile ambients against formulas of the logic, providing the first decidabilityresult for model checking a spatial logic with recursion.展开更多
Silica aerogel has broad applications in the field of high-temperature thermal insulation due to its low density,low thermal conductivity and high stability.However,its thermal insulation performance deteriorates sign...Silica aerogel has broad applications in the field of high-temperature thermal insulation due to its low density,low thermal conductivity and high stability.However,its thermal insulation performance deteriorates significantly at elevated temperatures exceeding 600℃,primarily due to the collapse of pore structure.Meanwhile,the shielding capacity of SiO_(2) aerogel to the infrared radiation at high temperature is rather low due to the intrinsic properties of SiO_(2).Herein,a strategy for improving the high-temperature stability and infrared shielding properties of SiO_(2) aerogel via Ca doping was explored.Calcium-doped silica aerogel(CSA)powders were prepared by Sol-Gel,hydrothermal,and ambient pressure drying(APD)techniques using water glass and anhydrous calcium chloride as precursors and trimethylchlorosilane as a hydrophobic modifier.The effects of Ca/Si molar ratio in the precursor and hydrothermal conditions(temperature and pH)on the crystalline properties,microscopic morphology and pore structure of CSAs were investigated.The results show that the Ca/Si molar ratio and hydrothermal treatment have significant effects on the microstructure and heat resistance of CSAs in the temperature range of 400-1000℃.The samples sintered at 1000℃have a high specific surface area of 100.1 m^(2)/g and a pore volume of 0.8705 cm^(3)/g,indicating that the CSA has good heat resistance.One-side insulation tests at temperatures up to 600℃show that the sample with a Ca/Si molar ratio of 1.0 has the best insulation performance,with a cold surface temperature of 450℃,which is 27℃lower than that of the pure silica aerogel.展开更多
Chinese strontium optical clocks help keep the world on time The new mandatory national standard GB 3095-2026,Ambient air quality standards,was jointly released by the Ministry of Ecology and Environment(MEE)and the S...Chinese strontium optical clocks help keep the world on time The new mandatory national standard GB 3095-2026,Ambient air quality standards,was jointly released by the Ministry of Ecology and Environment(MEE)and the State Administration for Market Regulation(SAMR).Two corresponding technical regulations,HJ 633-2026,Technical specifications on ambient air quality index,and HJ 663-2026,Technical specifications for ambient air quality assessment,were released as well.展开更多
Sound is considered an important aspect of an ecosystem and acoustic methods have emerged as effective tools for ecosystems research.Xincun Lagoon,Hainan Island,is an important ecosystem characterized by dense seagras...Sound is considered an important aspect of an ecosystem and acoustic methods have emerged as effective tools for ecosystems research.Xincun Lagoon,Hainan Island,is an important ecosystem characterized by dense seagrass,which has been declining due to increased human activities,raising great concerns.Previous studies have identified various threats to seagrass,including heavy metal pollution,poor quality water,and so on.In this study,we investigate sources and levels of noise in seagrass beds and attempt to point out potential threats from noise pollution.A line array of six hydrophones was deployed over a period of seven days,from January 15 to January 21,2024.The recordings captured various sounds from marine life,human activities,and natural processes.Biological sounds,such as fish sounds and whale calls,were the most prevalent.Low-frequency noise from wind and tide were often recorded.Xincun Bay hosts more than 1500 fishing vessels;however,due to bad weather conditions that kept most vessels docked during the recording period,only one segment of boat noise was recorded;it lasted for 7 minutes,exhibiting strong energy over a broad frequency band.This event underscores the necessity of long-term monitoring of noise to identify and evaluate not only boat noise but other noise sources,especially ones that are intermittent but strong,that were not encountered during the limited period of observation on which this report is based.展开更多
Prolonged exposure to n-butanol, a common hazardous volatile organic compound(VOC) in the environment, can lead to a broad range of adverse health effects. Therefore, detecting n-butanol safely and efficiently at low ...Prolonged exposure to n-butanol, a common hazardous volatile organic compound(VOC) in the environment, can lead to a broad range of adverse health effects. Therefore, detecting n-butanol safely and efficiently at low concentrations becomes critical for both environmental monitoring and human health. In this study, a novel Eu/Ce-codoped MOF-ZnO gas sensor was developed for the sensitive detection of n-butanol gas under ultraviolet activation at ambient temperature. A series of Eu/Ce-ZnO nanomaterials were synthesized via a simple co-precipitation route, by carefully designing the varied mass ratios of Eu and Ce incorporated into pristine ZnO derived from MOF precursors. The gas testing results revealed that introducing an appropriate amount of Eu and Ce would enlarge the specific surface area and enrich the oxygen vacancy content compared to pristine MOF-ZnO. Upon UV irradiation, the 0.03 wt% Eu 0.04 wt% Ce-ZnO sensor achieved a superior response of 611 for100 ppm n-butanol at room temperature, 15.28 times higher than that of pristine MOF-ZnO(40). Furthermore, the sensor presented rapid response/recovery times(15 s/28 s) and excellent selectivity. The above contributions pave the way for the promising development of highly sensitive, ultraviolet-enhanced gas sensors for ambient temperature detection of VOCs.展开更多
The Kumkol Basin,situated in the northern margin of the Qinghai-Xizang Plateau,provides a unique window into understanding the dynamic mechanisms driving the plateau’s northern expansion.However,its formation and tec...The Kumkol Basin,situated in the northern margin of the Qinghai-Xizang Plateau,provides a unique window into understanding the dynamic mechanisms driving the plateau’s northern expansion.However,its formation and tectonic evolution remain poorly understood due to limited geophysical data in this region.In this study,we computed cross-correlations for the TT components of station-pairs with high signal-to-noise ratios to extract Love wave waveforms and further performed Lovewave ambient noise tomography to image the upper crustal shear-wave velocity structure of the Kumkol basin down to 10 km depth.Our seismic velocity model reveals that the Kumkol Basin has a sedimentary thickness exceeding 8 km,with its center located near the Arka Mountain on the southern side.This suggests that the basin was likely formed as a foreland basin in response to the uplift of the Qiman Tagh Mountain to the north.Additionally,integrated with seismic reflection data,our seismic velocity model images a detachment fault at the basin basement depth.We inferred that the Kumkol Anticlinorium at the basin’s center have been produced by multiple thrust faults converging into this detachment fault at 8–10 km depth following the Early to Middle Miocene uplift of the Qiman Tagh Mountain.This structural configuration indicates pulsed basinward deformation since the late Miocene,likely reflecting a tectonic regime shift from extrusion to distributed shortening in the northern Qinghai-Xizang Plateau.Our findings provide a high-resolution velocity model of the Kumkol Basin,offering critical insights into its structural evolution and supporting future resource exploration in this underexplored region.展开更多
The Urumqi foreland thrust tectonic belt exhibits complex geological structures and strong seismicity.Imaging its shallow crustal structure is of great significance for understanding its tectonic mechanism and seismog...The Urumqi foreland thrust tectonic belt exhibits complex geological structures and strong seismicity.Imaging its shallow crustal structure is of great significance for understanding its tectonic mechanism and seismogenic environment.We obtained a high-resolution S-wave velocity model of the shallow crust at depths of 0–8 km using ambient noise tomography applied to data from a dense seismic array.Sediments are generally thinner in the southeast and thicker in the northwest,with a maximum thickness of more than 8 km.Variations in the velocity structure near the Xishan,Wanyaogou,and Yamalike faults indicate that their formation was related to differences in the physical properties on either side of the fault.In addition,the faults exhibit thrusting of the low-velocity sides towards the high-velocity sides.In the study area,earthquakes rarely occur at depths of less than 3 km and are mostly concentrated in the high-velocity zone in the southern part.Below 3 km depth,more earthquakes were observed,mainly distributed near faults or in relatively high-velocity areas in the southern part.This suggests that high-velocity structures are more prone to stress accumulation,resulting in earthquakes.At 6–8 km depth,the densely distributed earthquakes in the northwestern part of the Bogda mountains are well-aligned with the northwest-oriented low-velocity zone observed in this study,suggesting that this weak zone likely controls seismicity in this area.展开更多
The maximum rise-height,zero-buoyancy height,thickness of the spreading layer,minimum dilution and the height of the lower edge of the spreading layer are the important characteristic quantities of buoyant jets in str...The maximum rise-height,zero-buoyancy height,thickness of the spreading layer,minimum dilution and the height of the lower edge of the spreading layer are the important characteristic quantities of buoyant jets in stratified ambients.The scaling law is derived by the dimensional analysis of the influence factor on a buoyant jet.The characteristic quantities are found to converge to a single line under the unified scaling law.The correlation of the predicted results and experimental data is given.展开更多
Existing evidence suggests residential greenness is beneficial to human,while no research to date explored the associations of greenness with age-related macular degeneration(AMD).To evaluate the association of greenn...Existing evidence suggests residential greenness is beneficial to human,while no research to date explored the associations of greenness with age-related macular degeneration(AMD).To evaluate the association of greenness with AMD,modification and mediation effect of air pollution,we conducted this prospective study.We con-structed weighted quantile sum(WQS)index as co-exposure to nitrogen oxides(NO_(x)),particulate matter<2.5μm(PM_(2.5)),particulate matter<10μm(PM10).Stratified Cox regression models were applied to test the effect of exposure.Effect modification of air pollution was assessed.Stratified Cox models through the indirect method and Aalen additive risk models were used in mediation analysis.Over median follow-up of 11.67 years,4596 AMD events were ascertained.Hazard ratios(HRs)and 95%confidence intervals(95%CIs)of incident AMD for pollution per interquartile range(IQR)increment were 1.10(1.04–1.16)for nitrogen dioxide(NO_(2)),1.09(1.03–1.15)for NO_(x),1.14(1.05–1.24)for PM_(2.5),1.13(1.05–1.21)for PM10.The HR(95%CI)of AMD associated with greenness 1000 m buffer per IQR increment was 0.91(0.86–0.97),300 m buffer was 0.94(0.89–0.99).The as-sociation between greenness 1000 m and AMD was 28.59%,44.77%,35.59%,32.31%and 27.08%mediated by the decreased WQS index,NO_(2),NO_(x),PM_(2.5) and PM10,respectively.Increased greenness was associated with lower AMD incidence,and air pollution partly mediate it,which implies that interventions aimed at improving air quality and increasing greenness could have a dual benefit in mitigating AMD risk.展开更多
Underground carbon sequestration(CS)by solid waste backfill(SWB)offers an effective pathway for collaborative disposal of coal-based solid waste and CO_(2),where the amount of carbon sequestration is an important eval...Underground carbon sequestration(CS)by solid waste backfill(SWB)offers an effective pathway for collaborative disposal of coal-based solid waste and CO_(2),where the amount of carbon sequestration is an important evaluation parameter.In this study,the concept of whole-process carbon sequestration using coal-based solid waste and CO_(2),including sequential stirring and curing stages,was proposed to evaluate the performance evolution of CS.The results showed that CO_(2) pressure and ambient temperature positively correlated with the CS amount from coal-based SWB.In particular,CO_(2) pressure prevailed in the stirring stage,while the ambient temperature effect was more significant in the curing stage.The CS amounts obtained during the stirring stage alone,the curing stage alone,and two sequential stages ranged from 0.66%–3.10%,3.53%–5.09%,and 5.12%–6.02%,respectively.The functional group and micromorphology analyses revealed that the prevailing mechanism at the CS stirring stage was the stirringdriven gas dissolution-leaching-mineralization reaction,while that at the curing stage was the hydration-driven gas permeation-dissociation-CS reaction.Both were essentially solid-liquid-gas multiphase chemical reactions.The results are instrumental in substantiating the coal-based SWB carbon sequestration evolution patterns and mechanisms and providing data support for waste disposal and carbon emission reduction in the coal industry.展开更多
Superconducting elect rides have attracted growing attention for their potential to achieve high superconducting transition temperatures(T_(C))under pressure.However,many known elect rides are chemically reactive and ...Superconducting elect rides have attracted growing attention for their potential to achieve high superconducting transition temperatures(T_(C))under pressure.However,many known elect rides are chemically reactive and unstable,making high-quality single-crystal growth,characterization,and measurements difficult,and most do not exhibit superconductivity at ambient pressure.In contrast,La_(3) In stands out for its ambient-pressure superconductivity(T_(C)∼9.4 K)and the availability of high-quality single crystals.Here,we investigate its low-energy electronic structure using angle-resolved photoemission spectroscopy and first-principles calculations.The bands near the Fermi energy(E_(F))are mainly derived from La 5d and In 5p orbitals.A saddle point is directly observed at the Brillouin zone(BZ)boundary,while a three-dimensional Van Hove singularity crosses E_(F) at the BZ corner.First-principles calculations further reveal topological Dirac surface states within the bulk energy gap above E_(F).The coexistence of a high density of states and in-gap topological surface states near𝐸F suggests that La3In offers a promising platform for tuning superconductivity and exploring possible topological superconducting phases through doping or external pressure.展开更多
Inorganic materials can solve transportable and on-site hydrolytic hydrogen generation issues.CaH_(2)/(Al/Si)composites are preferable due to their notable chemical properties.However,these composites require pretreat...Inorganic materials can solve transportable and on-site hydrolytic hydrogen generation issues.CaH_(2)/(Al/Si)composites are preferable due to their notable chemical properties.However,these composites require pretreatments,an inert environment,and long hours of physical ball milling for high homogeneity and synergistic effects.CaH_(2)also inhibits the hydrolysis reaction by forming its products on the Al/Si surface,which hinders the direct utilization of composites.This work represents the first investigation of NaH-CaH_(2)(Al/Si)fuel composites,which greatly overcome these limitations and can be directly used for on-site hydrogen generation and proton exchange membrane(PEM)fuel cells.The NaH-CaH_(2)(Al/Si)fuel composites were prepared by using a straightforward mixing method with variable composition ratios,showing high H_(2)yield and fuel cell(FC)performance.NaH addition provides the bridge effect,which opens up a new way to enable efficient hydrolysis and greatly enhances the hydrolysis activity of CaH_(2)/(Al/Si)composites.The novel fuel composites(NaH-CaH_(2)/Al)have extraordinary FC performance and a 0.42 W/cm2 peak power density greater than commercial hydrogen generators.It provides high H_(2)yield 84.4%for NaH-CaH_(2)/Al and 82%for NaH-CaH_(2)/Si compared to NaOH-CaH_(2)(Al/Si),NaCl-CaH_(2)(Al/Si),and KCl-CaH_(2)(Al/Si)composites.The NaH bridge effect hinders the direct water contact and stops the formation of Ca(OH)2 around Al/Si,which provides adequate pathways for the CaH_(2)(Al/Si)hydrolysis.The impressive capabilities of novel fuel composites are anticipated to offer practical uses in fuel cells,automobile applications,and portable/on-board H_(2)generation.展开更多
Dense-array ambient noise tomography is a powerful tool for achieving high-resolution subsurface imag-ing,significantly impacting geohazard prevention and control.Conventional dense-array studies,how-ever,require simu...Dense-array ambient noise tomography is a powerful tool for achieving high-resolution subsurface imag-ing,significantly impacting geohazard prevention and control.Conventional dense-array studies,how-ever,require simultaneous observations of numerous stations for extensive coverage.To conduct a comprehensive karst feature investigation with limited stations,we designed a new synchronous-asyn-chronous observation system that facilitates dense array observations.We conducted two rounds of asynchronous observations,each lasting approximately 24 h,in combination with synchronous backbone stations.We achieved wide-ranging coverage of the study area utilizing 197 nodal receivers,with an average station spacing of 7 m.The beamforming results revealed distinct variations in the noise source distributions between day and night.We estimated the source strength in the stationary phase zone and used a weighting scheme for stacking the cross-correlation functions(C ^(1) functions)to suppress the influ-ence of nonuniform noise source distributions.The weights were derived from the similarity coefficients between multicomponent C^(1)functions related to Rayleigh waves.We employed the cross-correlation of C ^(1) functions(C^(2)methods)to obtain the empirical Green’s functions between asynchronous stations.To eliminate artifacts in C ^(2) functions from higher-mode surface waves in C^(1)functions,we filtered the C^(1)functions on the basis of different particle motions linked to multimode Rayleigh waves.The dispersion measurements of Rayleigh waves obtained from both the C^(1)and C^(2)functions were utilized in surface wave tomography.The inverted three-dimensional(3D)shear-wave(S-wave)velocity model reveals two significant low-velocity zones at depths ranging from 40 to 60 m,which align well with the karst caves found in the drilling data.The method of short-term synchronous-asynchronous ambient noise tomography shows promise as a cost-effective and efficient approach for urban geohazard investigations.展开更多
This study investigates the relationships between exposures to ambient air pollution—specifically particulate matter 2.5 (PM_(2.5)) and its metabolites—and the risk of depression.Nonlinear and linear regression,Baye...This study investigates the relationships between exposures to ambient air pollution—specifically particulate matter 2.5 (PM_(2.5)) and its metabolites—and the risk of depression.Nonlinear and linear regression,Bayesian kernel machine regression,and toxicogenomic analysis were key approaches.PM_(2.5)exposure was positively associated with the risk of developing depression,whereas phenylglyoxylic acid exposure was negatively associated with depression risk.We found a significant overall relationship between ambient air pollution and depression,particularly at the 55th and 60th percentiles.Although statistical significance was not reached at the 65th percentile,there was a noticeable upward trend,indicating a potential association.Interestingly,no significant connection was found between a combination of metabolites from ambient air pollution and depression.PM_(2.5)and phenylglyoxylic acid emerged as the most influential compounds in the models,respectively.PM_(2.5)exposure altered the expression of 42 specific targets associated with depression,especially POMC,SCL6A4,IL6,and SOD2.The study identified specific pathways related to insulin secretion,energy metabolism,blood circulation,tube diameter,and maintenance of blood vessel diameter,as well as key molecular mechanisms involving hsa-miR-124-3p,hsa-miR-155-5p,hsa-miR-16-5p,and SP1.These mechanisms were found to underlie the etiology of depression associated with PM_(2.5)exposure.In conclusions,PM_(2.5)and phenylglyoxylic acid were found to be associated with depression.Further work is needed to gain insight into the molecular mechanisms by which these chemicals affect depression,especially pathways related to insulin secretion and blood circulation.展开更多
The Tan-Lu Fault Zone is a large NNE-trending fault zone that has a substantial effect on the development of eastern China and its earthquake disaster prevention efforts. Aiming at the azimuthally anisotropic structur...The Tan-Lu Fault Zone is a large NNE-trending fault zone that has a substantial effect on the development of eastern China and its earthquake disaster prevention efforts. Aiming at the azimuthally anisotropic structure in the upper crust and seismogenic tectonics in the Hefei segment of this fault, we collected phase velocity dispersion data of fundamental mode Rayleigh waves from ambient noise cross-correlation functions of ~400 temporal seismographs in an area of approximately 80 × 70 km along the fault zone. The period band of the dispersion data was ~0.5–10 s. We inverted for the upper crustal three-dimensional(3-D) shear velocity model with azimuthal anisotropy from the surface to 10 km depth by using a 3-D direct azimuthal anisotropy inversion method. The inversion result shows the spatial distribution characteristics of the tectonic units in the upper crust. Additionally, the deformation of the Tan-Lu Fault Zone and its conjugated fault systems could be inferred from the anisotropy model. In particular, the faults that have remained active from the early and middle Pleistocene control the anisotropic characteristics of the upper crustal structure in this area. The direction of fast axes near the fault zone area in the upper crust is consistent with the strike of the faults, whereas for the region far away from the fault zone, the direction of fast axes is consistent with the direction of the regional principal stress caused by plate movement. Combined with the azimuthal anisotropy models in the deep crust and uppermost mantle from the surface wave and Pn wave, the different anisotropic patterns caused by the Tan-Lu Fault Zone and its conjugated fault system nearby are shown in the upper and lower crust. Furthermore,by using the double-difference method, we relocated the Lujiang earthquake series, which contained 32 earthquakes with a depth shallower than 10 km. Both the Vs model and earthquake relocation results indicate that earthquakes mostly occurred in the vicinity of structural boundaries with fractured media, with high-level development of cracks and small-scale faults jammed between more rigid areas.展开更多
The Anninghe–Zemuhe Fault and the Xiaojiang Fault are critical active faults along the middle-eastern boundary of the South Chuan–Dian Block. Many researchers have identified these faults as potential strong-earthqu...The Anninghe–Zemuhe Fault and the Xiaojiang Fault are critical active faults along the middle-eastern boundary of the South Chuan–Dian Block. Many researchers have identified these faults as potential strong-earthquake risk zones. In this study, we leveraged a dense seismic array to investigate the high-resolution shallow crust shear wave velocity(Vs) structure beneath the junction of the Zemuhe Fault Zone and the Xiaojiang Fault Zone, one of the most complex parts of the eastern boundary of the South Chuan–Dian Block. We analyzed the distribution of microseismic events detected between November 2022 and February 2023 based on the fine-scale Vs model obtained. The microseismicity in the study region was clustered into three groups, all spatially related to major faults in this region. These microseismic events indicate near-vertical fault planes, consistent with the fault geometry revealed by other researchers.Moreover, these microseismic events are influenced by the impoundment of the downstream Baihetan Reservoir and the complex tectonic stress near the junction of the Zemuhe Fault Zone and the Xiaojiang Fault Zone. The depths of these microseismic events are shallower in the junction zone, whereas moving south along the Xiaojiang Fault Zone, the microseismic events become deeper.Additionally, we compared our fine-scale local Vs model with velocity models obtained by other researchers and found that our model offers greater detail in characterizing subsurface heterogeneity while demonstrating improved reliability in delineating fault systems.展开更多
The Pamir Plateau,at the northwestern margin of the Tibetan Plateau,is a key region for investigating continental collision and plateau uplifting.To probe its deep structure,we collected seismic data from 263 stations...The Pamir Plateau,at the northwestern margin of the Tibetan Plateau,is a key region for investigating continental collision and plateau uplifting.To probe its deep structure,we collected seismic data from 263 stations across 11 research projects.We applied cross-correlation to noise data and extracted surface wave dispersion data from cross-correlation functions.The extracted dispersion data were subsequently inverted using a 3-D transdimensional Bayesian inversion method(rj-3 DMcMC).The inversion result reveals several crustal low-velocity zones(LVZs).Their formation is likely related to crustal thickening,the exposure of gneiss domes,and thicker sedimentary sequences compared to surrounding areas.In the lower crust and upper mantle,the LVZs in southern Pamir and southeastern Karakoram evolve into high-velocity zones,which expand northeastward with increasing depth.This suggests northward underthrusting of the Indian Plate.We also analyzed the Moho using both the standard deviation of S-wave velocity and the S-wave velocity structure.Results show that significant variations in velocity standard deviation reliably delineate the Moho interface.展开更多
High-energy-density lithium(Li)–air cells have been considered a promising energy-storage system,but the liquid electrolyte-related safety and side-reaction problems seriously hinder their development.To address thes...High-energy-density lithium(Li)–air cells have been considered a promising energy-storage system,but the liquid electrolyte-related safety and side-reaction problems seriously hinder their development.To address these above issues,solid-state Li–air batteries have been widely developed.However,many commonly-used solid electrolytes generally face huge interface impedance inLi–air cells and also showpoor stability towards ambient air/Li electrodes.Herein,we fabricate a differentiating surface-regulated ceramic-based composite electrolyte(DSCCE)by constructing disparately LiI-containing polymethyl methacrylate(PMMA)coating and Poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP)layer on both sides of Li_(1.5)Al_(0.5)Ge_(1.5)(PO_(4))_(3)(LAGP).The cathode-friendly LiI/PMMA layer displays excellent stability towards superoxide intermediates and also greatly reduces the decomposition voltage of discharge products in Li–air system.Additionally,the anode-friendly PVDF-HFP coating shows low-resistance properties towards anodes.Moreover,Li dendrite/passivation derived from liquid electrolyte-induced side reactions and air/I-attacking can be obviously suppressed by the uniformand compact composite framework.As a result,the DSCCE-based Li–air batteries possess high capacity/low voltage polarization(11,836mAh g^(-1)/1.45Vunder 500mAg^(-1)),good rate performance(capacity ratio under 1000mAg^(-1)/250mAg^(-1) is 68.2%)and longterm stable cell operation(~300 cycles at 750 mA g^(-1) with 750 mAh g^(-1))in ambient air.展开更多
文摘Ambient logics have been proposed to describe properties for mobile agentswhich may evolve over time as well as space. This paper takes a predicate-based approach toextending an ambient logic with recursion, yielding a predicate μ-calculus in which fixpointformulas are formed using predicate variables. An algorithm is developed for model checkingfinite-control mobile ambients against formulas of the logic, providing the first decidabilityresult for model checking a spatial logic with recursion.
文摘Silica aerogel has broad applications in the field of high-temperature thermal insulation due to its low density,low thermal conductivity and high stability.However,its thermal insulation performance deteriorates significantly at elevated temperatures exceeding 600℃,primarily due to the collapse of pore structure.Meanwhile,the shielding capacity of SiO_(2) aerogel to the infrared radiation at high temperature is rather low due to the intrinsic properties of SiO_(2).Herein,a strategy for improving the high-temperature stability and infrared shielding properties of SiO_(2) aerogel via Ca doping was explored.Calcium-doped silica aerogel(CSA)powders were prepared by Sol-Gel,hydrothermal,and ambient pressure drying(APD)techniques using water glass and anhydrous calcium chloride as precursors and trimethylchlorosilane as a hydrophobic modifier.The effects of Ca/Si molar ratio in the precursor and hydrothermal conditions(temperature and pH)on the crystalline properties,microscopic morphology and pore structure of CSAs were investigated.The results show that the Ca/Si molar ratio and hydrothermal treatment have significant effects on the microstructure and heat resistance of CSAs in the temperature range of 400-1000℃.The samples sintered at 1000℃have a high specific surface area of 100.1 m^(2)/g and a pore volume of 0.8705 cm^(3)/g,indicating that the CSA has good heat resistance.One-side insulation tests at temperatures up to 600℃show that the sample with a Ca/Si molar ratio of 1.0 has the best insulation performance,with a cold surface temperature of 450℃,which is 27℃lower than that of the pure silica aerogel.
文摘Chinese strontium optical clocks help keep the world on time The new mandatory national standard GB 3095-2026,Ambient air quality standards,was jointly released by the Ministry of Ecology and Environment(MEE)and the State Administration for Market Regulation(SAMR).Two corresponding technical regulations,HJ 633-2026,Technical specifications on ambient air quality index,and HJ 663-2026,Technical specifications for ambient air quality assessment,were released as well.
基金supported financially by the Director General’s Scientific Research Fund of Guangzhou Marine Geological Survey(Grant Number:2023GMGSJZJJ00029).
文摘Sound is considered an important aspect of an ecosystem and acoustic methods have emerged as effective tools for ecosystems research.Xincun Lagoon,Hainan Island,is an important ecosystem characterized by dense seagrass,which has been declining due to increased human activities,raising great concerns.Previous studies have identified various threats to seagrass,including heavy metal pollution,poor quality water,and so on.In this study,we investigate sources and levels of noise in seagrass beds and attempt to point out potential threats from noise pollution.A line array of six hydrophones was deployed over a period of seven days,from January 15 to January 21,2024.The recordings captured various sounds from marine life,human activities,and natural processes.Biological sounds,such as fish sounds and whale calls,were the most prevalent.Low-frequency noise from wind and tide were often recorded.Xincun Bay hosts more than 1500 fishing vessels;however,due to bad weather conditions that kept most vessels docked during the recording period,only one segment of boat noise was recorded;it lasted for 7 minutes,exhibiting strong energy over a broad frequency band.This event underscores the necessity of long-term monitoring of noise to identify and evaluate not only boat noise but other noise sources,especially ones that are intermittent but strong,that were not encountered during the limited period of observation on which this report is based.
基金supported by the National Natural Science Foundation of China (Grant No. 12304467)the China Postdoctoral Science Foundation (Grant No. 2023M732175)。
文摘Prolonged exposure to n-butanol, a common hazardous volatile organic compound(VOC) in the environment, can lead to a broad range of adverse health effects. Therefore, detecting n-butanol safely and efficiently at low concentrations becomes critical for both environmental monitoring and human health. In this study, a novel Eu/Ce-codoped MOF-ZnO gas sensor was developed for the sensitive detection of n-butanol gas under ultraviolet activation at ambient temperature. A series of Eu/Ce-ZnO nanomaterials were synthesized via a simple co-precipitation route, by carefully designing the varied mass ratios of Eu and Ce incorporated into pristine ZnO derived from MOF precursors. The gas testing results revealed that introducing an appropriate amount of Eu and Ce would enlarge the specific surface area and enrich the oxygen vacancy content compared to pristine MOF-ZnO. Upon UV irradiation, the 0.03 wt% Eu 0.04 wt% Ce-ZnO sensor achieved a superior response of 611 for100 ppm n-butanol at room temperature, 15.28 times higher than that of pristine MOF-ZnO(40). Furthermore, the sensor presented rapid response/recovery times(15 s/28 s) and excellent selectivity. The above contributions pave the way for the promising development of highly sensitive, ultraviolet-enhanced gas sensors for ambient temperature detection of VOCs.
基金funded by the National Natural Science Foundation of China(No.42274066),the Second Qinghai-Xizang Plateau Scientific Expedition and Research Program(STEP)(No.2019Q ZKK0701).
文摘The Kumkol Basin,situated in the northern margin of the Qinghai-Xizang Plateau,provides a unique window into understanding the dynamic mechanisms driving the plateau’s northern expansion.However,its formation and tectonic evolution remain poorly understood due to limited geophysical data in this region.In this study,we computed cross-correlations for the TT components of station-pairs with high signal-to-noise ratios to extract Love wave waveforms and further performed Lovewave ambient noise tomography to image the upper crustal shear-wave velocity structure of the Kumkol basin down to 10 km depth.Our seismic velocity model reveals that the Kumkol Basin has a sedimentary thickness exceeding 8 km,with its center located near the Arka Mountain on the southern side.This suggests that the basin was likely formed as a foreland basin in response to the uplift of the Qiman Tagh Mountain to the north.Additionally,integrated with seismic reflection data,our seismic velocity model images a detachment fault at the basin basement depth.We inferred that the Kumkol Anticlinorium at the basin’s center have been produced by multiple thrust faults converging into this detachment fault at 8–10 km depth following the Early to Middle Miocene uplift of the Qiman Tagh Mountain.This structural configuration indicates pulsed basinward deformation since the late Miocene,likely reflecting a tectonic regime shift from extrusion to distributed shortening in the northern Qinghai-Xizang Plateau.Our findings provide a high-resolution velocity model of the Kumkol Basin,offering critical insights into its structural evolution and supporting future resource exploration in this underexplored region.
基金supported by the Key Research and Development Program of the Xinjiang Uygur Autonomous Region(No.2020B03006-1)the National Natural Science Foundation of China(Nos.42304069,and 42102275).
文摘The Urumqi foreland thrust tectonic belt exhibits complex geological structures and strong seismicity.Imaging its shallow crustal structure is of great significance for understanding its tectonic mechanism and seismogenic environment.We obtained a high-resolution S-wave velocity model of the shallow crust at depths of 0–8 km using ambient noise tomography applied to data from a dense seismic array.Sediments are generally thinner in the southeast and thicker in the northwest,with a maximum thickness of more than 8 km.Variations in the velocity structure near the Xishan,Wanyaogou,and Yamalike faults indicate that their formation was related to differences in the physical properties on either side of the fault.In addition,the faults exhibit thrusting of the low-velocity sides towards the high-velocity sides.In the study area,earthquakes rarely occur at depths of less than 3 km and are mostly concentrated in the high-velocity zone in the southern part.Below 3 km depth,more earthquakes were observed,mainly distributed near faults or in relatively high-velocity areas in the southern part.This suggests that high-velocity structures are more prone to stress accumulation,resulting in earthquakes.At 6–8 km depth,the densely distributed earthquakes in the northwestern part of the Bogda mountains are well-aligned with the northwest-oriented low-velocity zone observed in this study,suggesting that this weak zone likely controls seismicity in this area.
文摘The maximum rise-height,zero-buoyancy height,thickness of the spreading layer,minimum dilution and the height of the lower edge of the spreading layer are the important characteristic quantities of buoyant jets in stratified ambients.The scaling law is derived by the dimensional analysis of the influence factor on a buoyant jet.The characteristic quantities are found to converge to a single line under the unified scaling law.The correlation of the predicted results and experimental data is given.
基金supported by the High-level Talents Introduction Plan from Central South University(No.502045003)the National Natural Science Foundation of China(No.42277438)Hunan Provincial Natural Science Foundation for Distinguished Young Scholars(No.2024JJ2082)to Fang Xiao,and the Postgraduate Independent Exploration and Innovation Project of Central South University,China(Nos.2024ZZTS0557 and 2023ZZTS0993)。
文摘Existing evidence suggests residential greenness is beneficial to human,while no research to date explored the associations of greenness with age-related macular degeneration(AMD).To evaluate the association of greenness with AMD,modification and mediation effect of air pollution,we conducted this prospective study.We con-structed weighted quantile sum(WQS)index as co-exposure to nitrogen oxides(NO_(x)),particulate matter<2.5μm(PM_(2.5)),particulate matter<10μm(PM10).Stratified Cox regression models were applied to test the effect of exposure.Effect modification of air pollution was assessed.Stratified Cox models through the indirect method and Aalen additive risk models were used in mediation analysis.Over median follow-up of 11.67 years,4596 AMD events were ascertained.Hazard ratios(HRs)and 95%confidence intervals(95%CIs)of incident AMD for pollution per interquartile range(IQR)increment were 1.10(1.04–1.16)for nitrogen dioxide(NO_(2)),1.09(1.03–1.15)for NO_(x),1.14(1.05–1.24)for PM_(2.5),1.13(1.05–1.21)for PM10.The HR(95%CI)of AMD associated with greenness 1000 m buffer per IQR increment was 0.91(0.86–0.97),300 m buffer was 0.94(0.89–0.99).The as-sociation between greenness 1000 m and AMD was 28.59%,44.77%,35.59%,32.31%and 27.08%mediated by the decreased WQS index,NO_(2),NO_(x),PM_(2.5) and PM10,respectively.Increased greenness was associated with lower AMD incidence,and air pollution partly mediate it,which implies that interventions aimed at improving air quality and increasing greenness could have a dual benefit in mitigating AMD risk.
基金supported by the National Key R&D Program of China(No.2023YFC3904304)the National Natural Science Foundation of China(No.52304158)Jiangsu Key Laboratory for Clean Utilization of Carbon Resources Research Project(No.BM2024007)。
文摘Underground carbon sequestration(CS)by solid waste backfill(SWB)offers an effective pathway for collaborative disposal of coal-based solid waste and CO_(2),where the amount of carbon sequestration is an important evaluation parameter.In this study,the concept of whole-process carbon sequestration using coal-based solid waste and CO_(2),including sequential stirring and curing stages,was proposed to evaluate the performance evolution of CS.The results showed that CO_(2) pressure and ambient temperature positively correlated with the CS amount from coal-based SWB.In particular,CO_(2) pressure prevailed in the stirring stage,while the ambient temperature effect was more significant in the curing stage.The CS amounts obtained during the stirring stage alone,the curing stage alone,and two sequential stages ranged from 0.66%–3.10%,3.53%–5.09%,and 5.12%–6.02%,respectively.The functional group and micromorphology analyses revealed that the prevailing mechanism at the CS stirring stage was the stirringdriven gas dissolution-leaching-mineralization reaction,while that at the curing stage was the hydration-driven gas permeation-dissociation-CS reaction.Both were essentially solid-liquid-gas multiphase chemical reactions.The results are instrumental in substantiating the coal-based SWB carbon sequestration evolution patterns and mechanisms and providing data support for waste disposal and carbon emission reduction in the coal industry.
基金supported by the National Natural Science Foundation of China(Grant Nos.12222413,12174443,12274459,and 12404266)the National Key R&D Program of China(Grant Nos.2023YFA1406500,2022YFA1403800,and 2022YFA1403103)+3 种基金the Natural Science Foundation of Shanghai (Grant No.23ZR1482200)the Natural Science Foundation of Ningbo (Grant No.2024J019)the Science Research Project of Hebei Education Department (Grant No.BJ2025060)the funding of Ningbo Yongjiang Talent Program。
文摘Superconducting elect rides have attracted growing attention for their potential to achieve high superconducting transition temperatures(T_(C))under pressure.However,many known elect rides are chemically reactive and unstable,making high-quality single-crystal growth,characterization,and measurements difficult,and most do not exhibit superconductivity at ambient pressure.In contrast,La_(3) In stands out for its ambient-pressure superconductivity(T_(C)∼9.4 K)and the availability of high-quality single crystals.Here,we investigate its low-energy electronic structure using angle-resolved photoemission spectroscopy and first-principles calculations.The bands near the Fermi energy(E_(F))are mainly derived from La 5d and In 5p orbitals.A saddle point is directly observed at the Brillouin zone(BZ)boundary,while a three-dimensional Van Hove singularity crosses E_(F) at the BZ corner.First-principles calculations further reveal topological Dirac surface states within the bulk energy gap above E_(F).The coexistence of a high density of states and in-gap topological surface states near𝐸F suggests that La3In offers a promising platform for tuning superconductivity and exploring possible topological superconducting phases through doping or external pressure.
基金financial support granted by the National Natural Science Foundation of China (No. 22402225)the Gusu Innovation and Entrepreneurship Leading Talent Plan(No. ZXL2023193)+2 种基金the Sinano Talents Plan (No. 2022000175)the Guangdong Basic and Applied Basic Research Foundation (No.2023A1515111133)the ANSO Scholarship for Young Talents
文摘Inorganic materials can solve transportable and on-site hydrolytic hydrogen generation issues.CaH_(2)/(Al/Si)composites are preferable due to their notable chemical properties.However,these composites require pretreatments,an inert environment,and long hours of physical ball milling for high homogeneity and synergistic effects.CaH_(2)also inhibits the hydrolysis reaction by forming its products on the Al/Si surface,which hinders the direct utilization of composites.This work represents the first investigation of NaH-CaH_(2)(Al/Si)fuel composites,which greatly overcome these limitations and can be directly used for on-site hydrogen generation and proton exchange membrane(PEM)fuel cells.The NaH-CaH_(2)(Al/Si)fuel composites were prepared by using a straightforward mixing method with variable composition ratios,showing high H_(2)yield and fuel cell(FC)performance.NaH addition provides the bridge effect,which opens up a new way to enable efficient hydrolysis and greatly enhances the hydrolysis activity of CaH_(2)/(Al/Si)composites.The novel fuel composites(NaH-CaH_(2)/Al)have extraordinary FC performance and a 0.42 W/cm2 peak power density greater than commercial hydrogen generators.It provides high H_(2)yield 84.4%for NaH-CaH_(2)/Al and 82%for NaH-CaH_(2)/Si compared to NaOH-CaH_(2)(Al/Si),NaCl-CaH_(2)(Al/Si),and KCl-CaH_(2)(Al/Si)composites.The NaH bridge effect hinders the direct water contact and stops the formation of Ca(OH)2 around Al/Si,which provides adequate pathways for the CaH_(2)(Al/Si)hydrolysis.The impressive capabilities of novel fuel composites are anticipated to offer practical uses in fuel cells,automobile applications,and portable/on-board H_(2)generation.
基金supported by the National Natural Science Foundation of China(41830103)the Project of Nanjing Center of China Geological Survey(DD20190281).
文摘Dense-array ambient noise tomography is a powerful tool for achieving high-resolution subsurface imag-ing,significantly impacting geohazard prevention and control.Conventional dense-array studies,how-ever,require simultaneous observations of numerous stations for extensive coverage.To conduct a comprehensive karst feature investigation with limited stations,we designed a new synchronous-asyn-chronous observation system that facilitates dense array observations.We conducted two rounds of asynchronous observations,each lasting approximately 24 h,in combination with synchronous backbone stations.We achieved wide-ranging coverage of the study area utilizing 197 nodal receivers,with an average station spacing of 7 m.The beamforming results revealed distinct variations in the noise source distributions between day and night.We estimated the source strength in the stationary phase zone and used a weighting scheme for stacking the cross-correlation functions(C ^(1) functions)to suppress the influ-ence of nonuniform noise source distributions.The weights were derived from the similarity coefficients between multicomponent C^(1)functions related to Rayleigh waves.We employed the cross-correlation of C ^(1) functions(C^(2)methods)to obtain the empirical Green’s functions between asynchronous stations.To eliminate artifacts in C ^(2) functions from higher-mode surface waves in C^(1)functions,we filtered the C^(1)functions on the basis of different particle motions linked to multimode Rayleigh waves.The dispersion measurements of Rayleigh waves obtained from both the C^(1)and C^(2)functions were utilized in surface wave tomography.The inverted three-dimensional(3D)shear-wave(S-wave)velocity model reveals two significant low-velocity zones at depths ranging from 40 to 60 m,which align well with the karst caves found in the drilling data.The method of short-term synchronous-asynchronous ambient noise tomography shows promise as a cost-effective and efficient approach for urban geohazard investigations.
文摘This study investigates the relationships between exposures to ambient air pollution—specifically particulate matter 2.5 (PM_(2.5)) and its metabolites—and the risk of depression.Nonlinear and linear regression,Bayesian kernel machine regression,and toxicogenomic analysis were key approaches.PM_(2.5)exposure was positively associated with the risk of developing depression,whereas phenylglyoxylic acid exposure was negatively associated with depression risk.We found a significant overall relationship between ambient air pollution and depression,particularly at the 55th and 60th percentiles.Although statistical significance was not reached at the 65th percentile,there was a noticeable upward trend,indicating a potential association.Interestingly,no significant connection was found between a combination of metabolites from ambient air pollution and depression.PM_(2.5)and phenylglyoxylic acid emerged as the most influential compounds in the models,respectively.PM_(2.5)exposure altered the expression of 42 specific targets associated with depression,especially POMC,SCL6A4,IL6,and SOD2.The study identified specific pathways related to insulin secretion,energy metabolism,blood circulation,tube diameter,and maintenance of blood vessel diameter,as well as key molecular mechanisms involving hsa-miR-124-3p,hsa-miR-155-5p,hsa-miR-16-5p,and SP1.These mechanisms were found to underlie the etiology of depression associated with PM_(2.5)exposure.In conclusions,PM_(2.5)and phenylglyoxylic acid were found to be associated with depression.Further work is needed to gain insight into the molecular mechanisms by which these chemicals affect depression,especially pathways related to insulin secretion and blood circulation.
基金financially supported by the National Key Research and Development Program of China (2022YFC3005600)the Foundation of the Anhui Educational Commission (2023AH051198)+1 种基金the National Natural Science Foundation of China (42125401 and 42104063)the Joint Open Fund of Mengcheng National Geophysical Observatory (MENGO-202201)。
文摘The Tan-Lu Fault Zone is a large NNE-trending fault zone that has a substantial effect on the development of eastern China and its earthquake disaster prevention efforts. Aiming at the azimuthally anisotropic structure in the upper crust and seismogenic tectonics in the Hefei segment of this fault, we collected phase velocity dispersion data of fundamental mode Rayleigh waves from ambient noise cross-correlation functions of ~400 temporal seismographs in an area of approximately 80 × 70 km along the fault zone. The period band of the dispersion data was ~0.5–10 s. We inverted for the upper crustal three-dimensional(3-D) shear velocity model with azimuthal anisotropy from the surface to 10 km depth by using a 3-D direct azimuthal anisotropy inversion method. The inversion result shows the spatial distribution characteristics of the tectonic units in the upper crust. Additionally, the deformation of the Tan-Lu Fault Zone and its conjugated fault systems could be inferred from the anisotropy model. In particular, the faults that have remained active from the early and middle Pleistocene control the anisotropic characteristics of the upper crustal structure in this area. The direction of fast axes near the fault zone area in the upper crust is consistent with the strike of the faults, whereas for the region far away from the fault zone, the direction of fast axes is consistent with the direction of the regional principal stress caused by plate movement. Combined with the azimuthal anisotropy models in the deep crust and uppermost mantle from the surface wave and Pn wave, the different anisotropic patterns caused by the Tan-Lu Fault Zone and its conjugated fault system nearby are shown in the upper and lower crust. Furthermore,by using the double-difference method, we relocated the Lujiang earthquake series, which contained 32 earthquakes with a depth shallower than 10 km. Both the Vs model and earthquake relocation results indicate that earthquakes mostly occurred in the vicinity of structural boundaries with fractured media, with high-level development of cracks and small-scale faults jammed between more rigid areas.
基金funded by the National Key R&D Program of China (Grant No. 2021YFC3000704)the National Natural Science Foundation of China (Grant No. 42125401)the Central Public-interest Scientific Institution Basal Research Fund (Grant No. CEAIEF20240401)。
文摘The Anninghe–Zemuhe Fault and the Xiaojiang Fault are critical active faults along the middle-eastern boundary of the South Chuan–Dian Block. Many researchers have identified these faults as potential strong-earthquake risk zones. In this study, we leveraged a dense seismic array to investigate the high-resolution shallow crust shear wave velocity(Vs) structure beneath the junction of the Zemuhe Fault Zone and the Xiaojiang Fault Zone, one of the most complex parts of the eastern boundary of the South Chuan–Dian Block. We analyzed the distribution of microseismic events detected between November 2022 and February 2023 based on the fine-scale Vs model obtained. The microseismicity in the study region was clustered into three groups, all spatially related to major faults in this region. These microseismic events indicate near-vertical fault planes, consistent with the fault geometry revealed by other researchers.Moreover, these microseismic events are influenced by the impoundment of the downstream Baihetan Reservoir and the complex tectonic stress near the junction of the Zemuhe Fault Zone and the Xiaojiang Fault Zone. The depths of these microseismic events are shallower in the junction zone, whereas moving south along the Xiaojiang Fault Zone, the microseismic events become deeper.Additionally, we compared our fine-scale local Vs model with velocity models obtained by other researchers and found that our model offers greater detail in characterizing subsurface heterogeneity while demonstrating improved reliability in delineating fault systems.
基金supported by the National Natural Science Foundation of China(Grant No.42174126)the Alliance of International Science Organizations(ANSO)Project(Grant No.ANSO-CR-PP2022-04)+1 种基金the Deep Earth Probe and Mineral Resources Exploration National Science and Technology Major Project(Grant Nos.2024ZD1002206,2024ZD1002201)Key R&D Program of Xinjiang Uyghur Autonomous Region(Grant No.2024B03013-2)。
文摘The Pamir Plateau,at the northwestern margin of the Tibetan Plateau,is a key region for investigating continental collision and plateau uplifting.To probe its deep structure,we collected seismic data from 263 stations across 11 research projects.We applied cross-correlation to noise data and extracted surface wave dispersion data from cross-correlation functions.The extracted dispersion data were subsequently inverted using a 3-D transdimensional Bayesian inversion method(rj-3 DMcMC).The inversion result reveals several crustal low-velocity zones(LVZs).Their formation is likely related to crustal thickening,the exposure of gneiss domes,and thicker sedimentary sequences compared to surrounding areas.In the lower crust and upper mantle,the LVZs in southern Pamir and southeastern Karakoram evolve into high-velocity zones,which expand northeastward with increasing depth.This suggests northward underthrusting of the Indian Plate.We also analyzed the Moho using both the standard deviation of S-wave velocity and the S-wave velocity structure.Results show that significant variations in velocity standard deviation reliably delineate the Moho interface.
基金supported by the National Natural Science Foundation of China(22379074)Young Science and Technology Talent Program of Inner Mongolia Province(NJYT24001)+4 种基金Natural Sciences and Engineering Research Council of Canada(NSERC)GLABAT Solid-State Battery Inc.,China Automotive Battery Research Institute Co.Ltd,Canada Research Chair Program(CRC)Canada Foundation for Innovation(CFI)Ontario Research Fundsupported by the Chinese Scholarship Council.
文摘High-energy-density lithium(Li)–air cells have been considered a promising energy-storage system,but the liquid electrolyte-related safety and side-reaction problems seriously hinder their development.To address these above issues,solid-state Li–air batteries have been widely developed.However,many commonly-used solid electrolytes generally face huge interface impedance inLi–air cells and also showpoor stability towards ambient air/Li electrodes.Herein,we fabricate a differentiating surface-regulated ceramic-based composite electrolyte(DSCCE)by constructing disparately LiI-containing polymethyl methacrylate(PMMA)coating and Poly(vinylidene fluoride-co-hexafluoropropylene)(PVDF-HFP)layer on both sides of Li_(1.5)Al_(0.5)Ge_(1.5)(PO_(4))_(3)(LAGP).The cathode-friendly LiI/PMMA layer displays excellent stability towards superoxide intermediates and also greatly reduces the decomposition voltage of discharge products in Li–air system.Additionally,the anode-friendly PVDF-HFP coating shows low-resistance properties towards anodes.Moreover,Li dendrite/passivation derived from liquid electrolyte-induced side reactions and air/I-attacking can be obviously suppressed by the uniformand compact composite framework.As a result,the DSCCE-based Li–air batteries possess high capacity/low voltage polarization(11,836mAh g^(-1)/1.45Vunder 500mAg^(-1)),good rate performance(capacity ratio under 1000mAg^(-1)/250mAg^(-1) is 68.2%)and longterm stable cell operation(~300 cycles at 750 mA g^(-1) with 750 mAh g^(-1))in ambient air.
