Transforming a scattering medium into a lens for imaging very simple binary objects is possible;however,it remains challenging to image complex grayscale objects,let alone measure 3D continuous distribution objects.He...Transforming a scattering medium into a lens for imaging very simple binary objects is possible;however,it remains challenging to image complex grayscale objects,let alone measure 3D continuous distribution objects.Here,we propose and demonstrate the use of a ground glass diffuser as a scattering lens for imaging complex grayscale fringes,and we employ it to achieve microscopic structured light 3D imaging(MSL3DI).The ubiquitous property of the speckle patterns permits the exploitation of the scattering medium as an ultra-thin scattering lens with a variable focal length and a flexible working distance for microscale object measurement.The method provides a light,flexible,and cost-effective imaging device as an alternative to microscope objectives or telecentric lenses in conventional MSL3DI systems.We experimentally demonstrate that employing a scattering lens allows us to achieve relatively good phase information and robust 3D imaging from depth measurements,yielding measurement accuracy only marginally lower than that of a telecentric lens,typically within approximately 10μm.Furthermore,the scattering lens demonstrates robust performance even when the imaging distance exceeds the typical working distance of a telecentric lens.The proposed method facilitates the application of scattering imaging techniques,providing a more flexible solution for MSL3DI.展开更多
The indirect boundary element method is used to study the 3D dynamic response of an infinitely long alluvial valley embedded in a saturated layered half-space for obli- quely incident SV waves. A wave-number transform...The indirect boundary element method is used to study the 3D dynamic response of an infinitely long alluvial valley embedded in a saturated layered half-space for obli- quely incident SV waves. A wave-number transform is first applied along the valley's axis to reduce a 3D problem to a 2D plane strain problem. The problem is then solved in the section perpendicular to the axis of the valley. Finally, the 3D dynamic responses of the valley are obtained by an inverse wave-number transform. The validity of the method is con- firmed by comparison with relevant results. The differences between the responses around the valley embedded in dry and in saturated poroelastic medium are studied, and the effects of drainage conditions, porosity, soil layer stiffness, and soil layer thickness on the dynamic response are dis- cussed in detail resulting in some conclusions.展开更多
In this paper,a new M3Y-type effective nucleon–nucleon interaction,derived based on the lowest order constrained variational approach(LOCV)and termed B3Y-Fetal,has been used in DDM3Y1,BDM3Y1,BDM3Y2,and BDM3Y3 density...In this paper,a new M3Y-type effective nucleon–nucleon interaction,derived based on the lowest order constrained variational approach(LOCV)and termed B3Y-Fetal,has been used in DDM3Y1,BDM3Y1,BDM3Y2,and BDM3Y3 density-dependent versions in a heavy ion(HI)optical potential based on four types of a real folded potential and a phenomenological Woods–Saxon imaginary potential to study the elastic scattering of the^(16)O+^(16)O nuclear system within the framework of the optical model(OM)by computing the associated differential cross sections at various incident energies.The results of the folding analyses have shown the DDB3Y1-Fetal and BDB3Y1-Fetal,out of the four folded potentials,give a reasonably better description of the elastic data of the nuclear system.These best-fit folded potentials are followed,in performance,by the BDB3Y2-Fetal,with the BDB3Y3-Fetal potential coming last.This performance trend was also demonstrated by the optical potentials based on the M3Y-Reid interaction.Furthermore,the best-fit folded potentials,renormalized by a factor NRof approximately 0.9,have been shown to reproduce the energy dependence of the real optical potential for^(16)O scattering found in previous optical model analyses creditably well.In excellent agreement with previous works,they have also been identified in this work to belong to the family of deep refractive potentials because they have been able to reproduce and consistently describe the evolution of Airylike structures,at large scattering angles,observed in the^(16)O scattering data at different energies.Finally,a comparison of the performances of B3Y-Fetal and M3Y-Reid effective interactions undertaken in this work has shown impressive agreement between them.展开更多
In this paper, a generalized three-dimensional(3D) scattering channel model for macrocellular land mobile environments is considered. This model simultaneously describes angular arrival of multi-path signals in the az...In this paper, a generalized three-dimensional(3D) scattering channel model for macrocellular land mobile environments is considered. This model simultaneously describes angular arrival of multi-path signals in the azimuth and elevation planes in an environment where uniformly distributed scatterers are assumed to be present in hemispheroids around the base station(BS) and mobile station(MS). Using this channel model, we first derive the closed-form expression for the joint and marginal probability density functions of the angle-of-arrival and time-of-arrival measured at the BS and the MS corresponding to the azimuth and elevation angles. Next, we derive an expression for the Doppler spectral distribution caused by motion of the MSs. Furthermore, we analyze the performance of multiple-input multiple-output antenna systems numerically. The results show that the proposed 3D scattering channel model performs better than previously proposed two-dimensional(2D) models for indoor and outdoor environments. We compare the results with previous scattering channel models and measurement results to validate the generalizability of our model.展开更多
The indirect boundary element method(IBEM) was established to solve the problem of 3-D seismic responses of 2-D topographies,by calculating the free-field responses with the direct-stiffness method and simulating the ...The indirect boundary element method(IBEM) was established to solve the problem of 3-D seismic responses of 2-D topographies,by calculating the free-field responses with the direct-stiffness method and simulating the scattering wave fields with the dynamic Green's functions of moving distributed loads.The proposed method yields accurate results,because the 3-D dynamic stiffness matrixes used are exact and the fictitious moving distributed loads can be acted directly on the interface between the alluvial valley and the layered half-space without singularity.The comparison with the published methods verifies the validity of the proposed method.And the numerical analyses are performed to give some beneficial conclusions.The study shows that 3-D scattering by an alluvial valley is essentially different from the 2-D case,and that the presence of soil layer affects not only the amplitude value of surface displacements but also the distribution of surface displacements.展开更多
Obtaining the ground truth for imaging through the scattering objects is always a challenging task.Furthermore,the scattering process caused by complex media is too intricate to be accurately modeled by either traditi...Obtaining the ground truth for imaging through the scattering objects is always a challenging task.Furthermore,the scattering process caused by complex media is too intricate to be accurately modeled by either traditional physical models or neural networks.To address this issue,we present a learning from better simulation(LBS)method.Utilizing the physical information from a single experimentally captured image through an optimization-based approach,the LBS method bypasses the multiple-scattering process and directly creates highly realistic synthetic data.The data can then be used to train downstream models.As a proof of concept,we train a simple U-Net solely on the synthetic data and demonstrate that it generalizes well to experimental data without requiring any manual labeling.3D holographic particle field monitoring is chosen as the testing bed,and simulation and experimental results are presented to demonstrate the effectiveness and robustness of the proposed technique for imaging of complex scattering media.The proposed method lays the groundwork for reliable particle field imaging in high concentration.The concept of utilizing realistic synthetic data for training can be significantly beneficial in various deep learningbased imaging tasks,especially those involving complex scattering media.展开更多
This paper reports that La-doped BiFeO3 (Bil-xLaxFeO3, x = 0, 0.1, 0.2, 0.3, 0.6, 0.8 and 1.0) were studied by using micro-Raman spectroscopy and x-ray diffraction (XRD). The XRD patterns indicate that the structu...This paper reports that La-doped BiFeO3 (Bil-xLaxFeO3, x = 0, 0.1, 0.2, 0.3, 0.6, 0.8 and 1.0) were studied by using micro-Raman spectroscopy and x-ray diffraction (XRD). The XRD patterns indicate that the structure of Bi1-xLaxFeO3 changes from rhombohedral BiFeO3 to orthorhombic LaFeO3. The results of Raman spectroscopy show good agreement with the XRD results. Strikingly, the phonon peak at around 610 cm^-1 and the two-phonon peaks in the high frequency range exist in all compounds and enhance with increasing La substitution. The increasing intensity of the 610 cm-1 peak is attributed to the changes in the FeO6 octahedron during the rhombohedral-orthorhombic phase transition. The enhancements of the two-phonon peaks are associated with the breakdown of the cycloid spin configuration with the appearance of the orthorhombic structure. These results indicate the existence of strong spin phonon coupling in Bi1-xLaxFeO3, which may provide useful information for understanding the effects of La content on the structural and magnetic properties of Bi1 -xLaxFeO3.展开更多
A combined study examining the temperature dependencies of Raman scattering and photoluminescence(PL)of a YBa2 Cu3 O7(YBCO)matrix doped with SiO2(12 nm;0.01 wt%.,0.10 wt%)and Zn0.95Mn0.05O(20 nm;0.02 wt%,0.10 wt%)nano...A combined study examining the temperature dependencies of Raman scattering and photoluminescence(PL)of a YBa2 Cu3 O7(YBCO)matrix doped with SiO2(12 nm;0.01 wt%.,0.10 wt%)and Zn0.95Mn0.05O(20 nm;0.02 wt%,0.10 wt%)nanoparticles was presented.X-ray diffraction(XRD)analysis confirms that both YBCO types exhibit aperovskite structure with the orthorhombic Pmmm phase.The microstructure was examined using environmental scanning electron microscopy(ESEM).Raman scattering and photoluminescence measurements as functions of temperature were conducted in the 77-837 K range.The photoluminescence intensity is observed to decrease for the doped YBCO than for the pure YBCO,because of localized defects.The photoluminescence spectrum is primarily composed of three bands at 1.60,1.88,and 2.40 eV.A clearly pronounced correlation is observed between electronic and structural changes in the doped YBCO,which is due to the temperature,illumination,added oxygen or metal ions,and spectral parameters.The PL integrated intensity as a function of the inverse temperature was simulated using the Arrhenius model.This analysis reveals that the energy exchange between the different levels in the pure and doped YBCO was conducted via two vibration modes only,which are strongly linked to the oxygen and copper atoms in the YBCO matrix.The temperature dependencies of the modes at 340 and 500 cm-1 exhibit softening with temperature increase,resulting from microstructure control,which may be due to small concentrations of Si,Zn,and Mn substitutions at the chain Cu(1)and plane Cu(2)sites.展开更多
From the sound velocity measured using the Brillouin scattering technique, the elastic, piezoelectric, and dielectric constants of a high-quality monodomain tetragonal Rh:BaTiO3 single crystal are determined at room ...From the sound velocity measured using the Brillouin scattering technique, the elastic, piezoelectric, and dielectric constants of a high-quality monodomain tetragonal Rh:BaTiO3 single crystal are determined at room temperature. The elastic constants are in fairly good agreement with those of the BaTiO3 single crystal, measured previously by Brillouin scattering and the low-frequency equivalent circuit methods. However, their electromeehanical properties are significantly different. Based on the sound propagation equations and these results, the directional dependence of the compressional modulus and the shear modulus of Rh:BaTiO3 in the (010) plane is investigated. Some properties of sound propagation and electromechanical coupling in the crystal are discussed.展开更多
Regulation of optical properties and electronic structure of graphitic carbon nitride (g-C3N4 ) via external strain has attracted much attention due to its potential in photocatalyst and electronic devices. However,...Regulation of optical properties and electronic structure of graphitic carbon nitride (g-C3N4 ) via external strain has attracted much attention due to its potential in photocatalyst and electronic devices. However, the identifi- cation of g-C3N4 structure transformation induced by strain is greatly lacking. In this work, the Raman spectra of g-C3N4 with external strain are determined theoretically based on the density function theory. Deformation induced by external strain not only regulates the Raman mode positions but also leads to a I^aman mode split- ting, which can be ascribed to crystal symmetry destruction by strain engineering. Our results suggest the use of Raman scattering in structural identification in deformed 9-C3N4 structure.展开更多
The soft measurement technology of flame temperature field is an efficient method to learn the combustion status in furnace. Generally, it reconstructs the temperature field in furnace through the image of flame, whic...The soft measurement technology of flame temperature field is an efficient method to learn the combustion status in furnace. Generally, it reconstructs the temperature field in furnace through the image of flame, which is a process to solve radiative inverse problem. In this paper, the flame of pulverized coal is considered as 3-D, absorbing, emitting, and anisotropically scattering non-gray medium. Through the study on inverse problem of radiative heat transfer, the temperature field in this kind of medium has been reconstructed. The mechanism of 3-D radiative heat transfer in a rectangular media, which is 2 m×3 m× 5 m and full of CO2, N2 and carbon particles, is studied with Monte Carlo method. The 3-D temperature field in this rectangular space is reconstructed and the influence of particles density profile is discussed.展开更多
We present a theoretical investigation of the scattering of high frequency S0 Lamb mode from a circular blind hole defect in a plate based on the 3D theory. The SO wave is incident at the frequency above the A1 mode c...We present a theoretical investigation of the scattering of high frequency S0 Lamb mode from a circular blind hole defect in a plate based on the 3D theory. The SO wave is incident at the frequency above the A1 mode cut-off frequency, in which the popular approximate plate theories are inapplicable. Due to the non-symmetric blind hole defect, the scattered fields will contain higher order converted modes in addition to the fundamental SO and AO modes. The far-field scattering amplitudes of various propagating Lamb modes for different hole sizes are inspected. The results are compared with those of lower frequencies and some different phenomena are found. Two-dimensional Fourier transform (2DFT) results of transient scattered Lamb and SH wave signals agree well with the analytical dispersion curves, which check the validity of the solutions from another point of view.展开更多
Gold nanoparticle arrays fabricated via layerby-layer technique were investigated using grazing-incidence small-angle X-ray scattering(GISAXS) method.Samples containing two gold nanoparticle layers that were separated...Gold nanoparticle arrays fabricated via layerby-layer technique were investigated using grazing-incidence small-angle X-ray scattering(GISAXS) method.Samples containing two gold nanoparticle layers that were separated by 5,11,15 and 21 poly electrolyte(PE) interlayers were studied.By using different X-ray incident angles,correlations of gold nanoparticles(GNPs) in the same layer and in two different layers were investigated.It is found that both sideway correlations between GNPs in the same layer and vertical correlation between two gold nanoparticle layers depend on the thickness of PE interlayers.According to sideway correlation,the size of GNPs is determined to be(13.0±0.5) nm in all of the four samples,which was also proved by scanning electron microscopy(SEM) and theoretical calculation of form factor of spherical particles.From vertical correlation,distance between two gold nanoparticle layers was determined for sample with 11,15 and 21 PE layers.These distances can be reasonably explained with the number of PE layers and the thickness of single PE layer.These results indicate that by repeated depositing of oppositely charged PE layers,a true three-dimensional(3 D) nanostructure can eventually be designed.展开更多
To solve seismic wave scattering by a large-scale three-dimensional(3-D) hill topography, a fast parallel indirect boundary element method(IBEM) is developed by proposing a new construction method for the wave field, ...To solve seismic wave scattering by a large-scale three-dimensional(3-D) hill topography, a fast parallel indirect boundary element method(IBEM) is developed by proposing a new construction method for the wave field, modifying the generalized minimum residual(GMRES) algorithm and constructing an Open MP plus MPI parallel model. The validations of accuracy and efficiency show that this method can solve 3-D seismic response of a large-scale hill topography for broadband waves, and overcome the weakness of large storage and low efficiency of the traditional IBEM. Based on this new algorithm architecture, taking the broadband scattering of plane SV waves by a large-scale Gaussian-shaped hill of thousands-meters height as an example, the influence of several important parameters is investigated, including the incident frequency, the incident angle and the height-width and length-width ratio of the hill. The numerical results illustrate that the amplification effect on the ground motion by a near-hemispherical hill is more significant than the narrow hill. For low-frequency waves, the scattering effect of the higher hill is more pronounced, and there is only a single peak near the top of the hill. However, for high-frequency waves, rapid spatial variation of displacement amplitude appears on the hill surface.展开更多
This is a short report of a recently uncovered resonant phenomenon. The modified Faddeev equation that correctly includes all six open channels is used. The calculation is carried out in s-partial wave. We report a nu...This is a short report of a recently uncovered resonant phenomenon. The modified Faddeev equation that correctly includes all six open channels is used. The calculation is carried out in s-partial wave. We report a number of resonant peaks in the elastic cross sections as well as the wave amplitudes involved. This is the energy region where the Stark-effect induced electric dipole energy split in the target dominates the physics and the Long-Range behavior of the 3-body scattering system. It is found that when the center of mass collision energy in the new channels is in integer proportion to the corresponding electric dipole energy split, Bremsstrahlung photon mediated resonant scattering occurs. The corresponding wave amplitudes deform into wave-packets hundreds to thousands of Bohr radii in width. The physical implication of this phenomenon will be discussed.展开更多
Obtaining phase information for the solution of macromolecular structures is a bottleneck in X-ray crystallography. Anomalous dispersion was recognized as a powerful tool for phasing macromolecular structures. It was ...Obtaining phase information for the solution of macromolecular structures is a bottleneck in X-ray crystallography. Anomalous dispersion was recognized as a powerful tool for phasing macromolecular structures. It was used mainly to supplement the isomorphous replacement or to locate the anomalous scatterer itself. The first step in solving macromolecular structures by SAD (single-wavelength anomalous diffraction) is the location of the anomalous scatterers. The SAD method for experimental phasing has evolved substantially in the recent years. A phasing tool, 5-amino-2,4,6- triiodoisophthalic acid (I3C—magic triangle), was incorporated into three proteins, lysozyme, glucose isomerase and thermolysin using quick-soaking and co-crystallization method in order to understand the binding of metal ion with proteins. The high quality of the diffraction data, the use of chromium anode X-ray radiation and the required amount of anomalous signal enabled way for successful structure determination and automated model building. An analysis and/or comparison of the sulfur and iodine anomalous signals at the Cr Kα wavelength are discussed.展开更多
Raman spectrum of molten cryolite was recorded. Based on the new understanding of the scattering coefficients, contents of various structural entities in acidic NaF-AlF3 melts at 942-1 024 ℃ in previous research were...Raman spectrum of molten cryolite was recorded. Based on the new understanding of the scattering coefficients, contents of various structural entities in acidic NaF-AlF3 melts at 942-1 024 ℃ in previous research were reanalyzed. The new quantitative analysis results show that when cryolite ratio(CR) is less than 2, AlF4- is the dominant anion in the melts, and its mole fraction is about 0.70 for melts with CR=1.5 and 0.50 for melts with CR=2. When CR is more than 2.5, the mole fraction of AlF6^3- is relatively large, which is around 0.45 for melts with CR=2.5. Ionic structure of Na3AlF6-Al2O3 melts was investigated by UV-Raman spectroscopy. Octahedral AlF6^3- and tetrahedral AlF4- are proved to exist with possible partial replacement of F- by O^2-. Al2O2F4^2- with a large scattering coefficient also exists in the melts in which alumina concentration is more than 4% (mass fraction). The increase of temperature causes blue-shift of the bands in the Raman spectra.展开更多
基金supported by the National Natural Science Foundation of China(Grant Nos.62275188 and 62505216)the Central Guidance on Local Science and Technology Development Fund(Grant No.YDZJSX2024D019)+1 种基金the International Scientific and Technological Cooperative Project in Shanxi Province(Grant No.202104041101009)the Natural Science Foundation of Shanxi Province of China through Research Project(Grant No.20210302123195).
文摘Transforming a scattering medium into a lens for imaging very simple binary objects is possible;however,it remains challenging to image complex grayscale objects,let alone measure 3D continuous distribution objects.Here,we propose and demonstrate the use of a ground glass diffuser as a scattering lens for imaging complex grayscale fringes,and we employ it to achieve microscopic structured light 3D imaging(MSL3DI).The ubiquitous property of the speckle patterns permits the exploitation of the scattering medium as an ultra-thin scattering lens with a variable focal length and a flexible working distance for microscale object measurement.The method provides a light,flexible,and cost-effective imaging device as an alternative to microscope objectives or telecentric lenses in conventional MSL3DI systems.We experimentally demonstrate that employing a scattering lens allows us to achieve relatively good phase information and robust 3D imaging from depth measurements,yielding measurement accuracy only marginally lower than that of a telecentric lens,typically within approximately 10μm.Furthermore,the scattering lens demonstrates robust performance even when the imaging distance exceeds the typical working distance of a telecentric lens.The proposed method facilitates the application of scattering imaging techniques,providing a more flexible solution for MSL3DI.
基金supported by the National Natural Science Foundation of China (50908156,50978183)Tianjin Research Program of Application Foundation and Advanced Technology (12JCQNJC04700)
文摘The indirect boundary element method is used to study the 3D dynamic response of an infinitely long alluvial valley embedded in a saturated layered half-space for obli- quely incident SV waves. A wave-number transform is first applied along the valley's axis to reduce a 3D problem to a 2D plane strain problem. The problem is then solved in the section perpendicular to the axis of the valley. Finally, the 3D dynamic responses of the valley are obtained by an inverse wave-number transform. The validity of the method is con- firmed by comparison with relevant results. The differences between the responses around the valley embedded in dry and in saturated poroelastic medium are studied, and the effects of drainage conditions, porosity, soil layer stiffness, and soil layer thickness on the dynamic response are dis- cussed in detail resulting in some conclusions.
基金Prof.Dao T.Khoa of the Institute for Nuclear Science and Technology(INST),Vietnam,is specially and gratefully acknowledged for providing helpful academic materials and excellent guidance in this work.
文摘In this paper,a new M3Y-type effective nucleon–nucleon interaction,derived based on the lowest order constrained variational approach(LOCV)and termed B3Y-Fetal,has been used in DDM3Y1,BDM3Y1,BDM3Y2,and BDM3Y3 density-dependent versions in a heavy ion(HI)optical potential based on four types of a real folded potential and a phenomenological Woods–Saxon imaginary potential to study the elastic scattering of the^(16)O+^(16)O nuclear system within the framework of the optical model(OM)by computing the associated differential cross sections at various incident energies.The results of the folding analyses have shown the DDB3Y1-Fetal and BDB3Y1-Fetal,out of the four folded potentials,give a reasonably better description of the elastic data of the nuclear system.These best-fit folded potentials are followed,in performance,by the BDB3Y2-Fetal,with the BDB3Y3-Fetal potential coming last.This performance trend was also demonstrated by the optical potentials based on the M3Y-Reid interaction.Furthermore,the best-fit folded potentials,renormalized by a factor NRof approximately 0.9,have been shown to reproduce the energy dependence of the real optical potential for^(16)O scattering found in previous optical model analyses creditably well.In excellent agreement with previous works,they have also been identified in this work to belong to the family of deep refractive potentials because they have been able to reproduce and consistently describe the evolution of Airylike structures,at large scattering angles,observed in the^(16)O scattering data at different energies.Finally,a comparison of the performances of B3Y-Fetal and M3Y-Reid effective interactions undertaken in this work has shown impressive agreement between them.
基金supported by the National Nature Science Foundation of China (No.61471153)the Scientific and Technological Support Project (Industry) of Jiangsu Province (No. BE2011195)the Major Program of the Natural Science Foundation of Institution of Higher Education of Jiangsu Province (No. 14KJA510001)
文摘In this paper, a generalized three-dimensional(3D) scattering channel model for macrocellular land mobile environments is considered. This model simultaneously describes angular arrival of multi-path signals in the azimuth and elevation planes in an environment where uniformly distributed scatterers are assumed to be present in hemispheroids around the base station(BS) and mobile station(MS). Using this channel model, we first derive the closed-form expression for the joint and marginal probability density functions of the angle-of-arrival and time-of-arrival measured at the BS and the MS corresponding to the azimuth and elevation angles. Next, we derive an expression for the Doppler spectral distribution caused by motion of the MSs. Furthermore, we analyze the performance of multiple-input multiple-output antenna systems numerically. The results show that the proposed 3D scattering channel model performs better than previously proposed two-dimensional(2D) models for indoor and outdoor environments. We compare the results with previous scattering channel models and measurement results to validate the generalizability of our model.
基金Supported by National Natural Science Foundation of China (No. 50978156 and 50908183)Tianjin Research Programof Application Foundation and Advanced Technology(12JCQNJC04700)
文摘The indirect boundary element method(IBEM) was established to solve the problem of 3-D seismic responses of 2-D topographies,by calculating the free-field responses with the direct-stiffness method and simulating the scattering wave fields with the dynamic Green's functions of moving distributed loads.The proposed method yields accurate results,because the 3-D dynamic stiffness matrixes used are exact and the fictitious moving distributed loads can be acted directly on the interface between the alluvial valley and the layered half-space without singularity.The comparison with the published methods verifies the validity of the proposed method.And the numerical analyses are performed to give some beneficial conclusions.The study shows that 3-D scattering by an alluvial valley is essentially different from the 2-D case,and that the presence of soil layer affects not only the amplitude value of surface displacements but also the distribution of surface displacements.
基金supported by the National Key Research and Development Program of China(Grant Nos.2022YFB2804300 and 2023YFB3611500)the National Natural Science Foundation of China(Grant No.62275218)+1 种基金the China Postdoctoral Science Foundation(Grant No.2022M712586)the Guangdong Basic and Applied Basic Research Foundation(Grant No.2023A1515011335).
文摘Obtaining the ground truth for imaging through the scattering objects is always a challenging task.Furthermore,the scattering process caused by complex media is too intricate to be accurately modeled by either traditional physical models or neural networks.To address this issue,we present a learning from better simulation(LBS)method.Utilizing the physical information from a single experimentally captured image through an optimization-based approach,the LBS method bypasses the multiple-scattering process and directly creates highly realistic synthetic data.The data can then be used to train downstream models.As a proof of concept,we train a simple U-Net solely on the synthetic data and demonstrate that it generalizes well to experimental data without requiring any manual labeling.3D holographic particle field monitoring is chosen as the testing bed,and simulation and experimental results are presented to demonstrate the effectiveness and robustness of the proposed technique for imaging of complex scattering media.The proposed method lays the groundwork for reliable particle field imaging in high concentration.The concept of utilizing realistic synthetic data for training can be significantly beneficial in various deep learningbased imaging tasks,especially those involving complex scattering media.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 10674171 and 10874236)
文摘This paper reports that La-doped BiFeO3 (Bil-xLaxFeO3, x = 0, 0.1, 0.2, 0.3, 0.6, 0.8 and 1.0) were studied by using micro-Raman spectroscopy and x-ray diffraction (XRD). The XRD patterns indicate that the structure of Bi1-xLaxFeO3 changes from rhombohedral BiFeO3 to orthorhombic LaFeO3. The results of Raman spectroscopy show good agreement with the XRD results. Strikingly, the phonon peak at around 610 cm^-1 and the two-phonon peaks in the high frequency range exist in all compounds and enhance with increasing La substitution. The increasing intensity of the 610 cm-1 peak is attributed to the changes in the FeO6 octahedron during the rhombohedral-orthorhombic phase transition. The enhancements of the two-phonon peaks are associated with the breakdown of the cycloid spin configuration with the appearance of the orthorhombic structure. These results indicate the existence of strong spin phonon coupling in Bi1-xLaxFeO3, which may provide useful information for understanding the effects of La content on the structural and magnetic properties of Bi1 -xLaxFeO3.
文摘A combined study examining the temperature dependencies of Raman scattering and photoluminescence(PL)of a YBa2 Cu3 O7(YBCO)matrix doped with SiO2(12 nm;0.01 wt%.,0.10 wt%)and Zn0.95Mn0.05O(20 nm;0.02 wt%,0.10 wt%)nanoparticles was presented.X-ray diffraction(XRD)analysis confirms that both YBCO types exhibit aperovskite structure with the orthorhombic Pmmm phase.The microstructure was examined using environmental scanning electron microscopy(ESEM).Raman scattering and photoluminescence measurements as functions of temperature were conducted in the 77-837 K range.The photoluminescence intensity is observed to decrease for the doped YBCO than for the pure YBCO,because of localized defects.The photoluminescence spectrum is primarily composed of three bands at 1.60,1.88,and 2.40 eV.A clearly pronounced correlation is observed between electronic and structural changes in the doped YBCO,which is due to the temperature,illumination,added oxygen or metal ions,and spectral parameters.The PL integrated intensity as a function of the inverse temperature was simulated using the Arrhenius model.This analysis reveals that the energy exchange between the different levels in the pure and doped YBCO was conducted via two vibration modes only,which are strongly linked to the oxygen and copper atoms in the YBCO matrix.The temperature dependencies of the modes at 340 and 500 cm-1 exhibit softening with temperature increase,resulting from microstructure control,which may be due to small concentrations of Si,Zn,and Mn substitutions at the chain Cu(1)and plane Cu(2)sites.
基金Project supported by the National Natural Science Foundation of China (Grant Nos. 10874236 and 60808010)
文摘From the sound velocity measured using the Brillouin scattering technique, the elastic, piezoelectric, and dielectric constants of a high-quality monodomain tetragonal Rh:BaTiO3 single crystal are determined at room temperature. The elastic constants are in fairly good agreement with those of the BaTiO3 single crystal, measured previously by Brillouin scattering and the low-frequency equivalent circuit methods. However, their electromeehanical properties are significantly different. Based on the sound propagation equations and these results, the directional dependence of the compressional modulus and the shear modulus of Rh:BaTiO3 in the (010) plane is investigated. Some properties of sound propagation and electromechanical coupling in the crystal are discussed.
基金Supported by the National Natural Science Foundation of China under Grant Nos 61264008 and 61274121the Natural Science Foundation of Jiangsu Province under Grant No BK2012829
文摘Regulation of optical properties and electronic structure of graphitic carbon nitride (g-C3N4 ) via external strain has attracted much attention due to its potential in photocatalyst and electronic devices. However, the identifi- cation of g-C3N4 structure transformation induced by strain is greatly lacking. In this work, the Raman spectra of g-C3N4 with external strain are determined theoretically based on the density function theory. Deformation induced by external strain not only regulates the Raman mode positions but also leads to a I^aman mode split- ting, which can be ascribed to crystal symmetry destruction by strain engineering. Our results suggest the use of Raman scattering in structural identification in deformed 9-C3N4 structure.
基金Project Supported by National Nature Science Foundation of China (50578034) Science and Technology Development Foundation ofDonghua University
文摘The soft measurement technology of flame temperature field is an efficient method to learn the combustion status in furnace. Generally, it reconstructs the temperature field in furnace through the image of flame, which is a process to solve radiative inverse problem. In this paper, the flame of pulverized coal is considered as 3-D, absorbing, emitting, and anisotropically scattering non-gray medium. Through the study on inverse problem of radiative heat transfer, the temperature field in this kind of medium has been reconstructed. The mechanism of 3-D radiative heat transfer in a rectangular media, which is 2 m×3 m× 5 m and full of CO2, N2 and carbon particles, is studied with Monte Carlo method. The 3-D temperature field in this rectangular space is reconstructed and the influence of particles density profile is discussed.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11474195,11274226 and 61171145
文摘We present a theoretical investigation of the scattering of high frequency S0 Lamb mode from a circular blind hole defect in a plate based on the 3D theory. The SO wave is incident at the frequency above the A1 mode cut-off frequency, in which the popular approximate plate theories are inapplicable. Due to the non-symmetric blind hole defect, the scattered fields will contain higher order converted modes in addition to the fundamental SO and AO modes. The far-field scattering amplitudes of various propagating Lamb modes for different hole sizes are inspected. The results are compared with those of lower frequencies and some different phenomena are found. Two-dimensional Fourier transform (2DFT) results of transient scattered Lamb and SH wave signals agree well with the analytical dispersion curves, which check the validity of the solutions from another point of view.
基金financially supported by the Framework Programme 7 Project NANOGOLD (No.ERAS-989409)。
文摘Gold nanoparticle arrays fabricated via layerby-layer technique were investigated using grazing-incidence small-angle X-ray scattering(GISAXS) method.Samples containing two gold nanoparticle layers that were separated by 5,11,15 and 21 poly electrolyte(PE) interlayers were studied.By using different X-ray incident angles,correlations of gold nanoparticles(GNPs) in the same layer and in two different layers were investigated.It is found that both sideway correlations between GNPs in the same layer and vertical correlation between two gold nanoparticle layers depend on the thickness of PE interlayers.According to sideway correlation,the size of GNPs is determined to be(13.0±0.5) nm in all of the four samples,which was also proved by scanning electron microscopy(SEM) and theoretical calculation of form factor of spherical particles.From vertical correlation,distance between two gold nanoparticle layers was determined for sample with 11,15 and 21 PE layers.These distances can be reasonably explained with the number of PE layers and the thickness of single PE layer.These results indicate that by repeated depositing of oppositely charged PE layers,a true three-dimensional(3 D) nanostructure can eventually be designed.
基金National Natural Science Foundation of China under Grant No. 51678390National Natural Science Foundation of China under Grant No. 51708391the Major Science and Technology Projects in Tianjin under Grant No. 18ZXAQSF00110。
文摘To solve seismic wave scattering by a large-scale three-dimensional(3-D) hill topography, a fast parallel indirect boundary element method(IBEM) is developed by proposing a new construction method for the wave field, modifying the generalized minimum residual(GMRES) algorithm and constructing an Open MP plus MPI parallel model. The validations of accuracy and efficiency show that this method can solve 3-D seismic response of a large-scale hill topography for broadband waves, and overcome the weakness of large storage and low efficiency of the traditional IBEM. Based on this new algorithm architecture, taking the broadband scattering of plane SV waves by a large-scale Gaussian-shaped hill of thousands-meters height as an example, the influence of several important parameters is investigated, including the incident frequency, the incident angle and the height-width and length-width ratio of the hill. The numerical results illustrate that the amplification effect on the ground motion by a near-hemispherical hill is more significant than the narrow hill. For low-frequency waves, the scattering effect of the higher hill is more pronounced, and there is only a single peak near the top of the hill. However, for high-frequency waves, rapid spatial variation of displacement amplitude appears on the hill surface.
文摘This is a short report of a recently uncovered resonant phenomenon. The modified Faddeev equation that correctly includes all six open channels is used. The calculation is carried out in s-partial wave. We report a number of resonant peaks in the elastic cross sections as well as the wave amplitudes involved. This is the energy region where the Stark-effect induced electric dipole energy split in the target dominates the physics and the Long-Range behavior of the 3-body scattering system. It is found that when the center of mass collision energy in the new channels is in integer proportion to the corresponding electric dipole energy split, Bremsstrahlung photon mediated resonant scattering occurs. The corresponding wave amplitudes deform into wave-packets hundreds to thousands of Bohr radii in width. The physical implication of this phenomenon will be discussed.
文摘Obtaining phase information for the solution of macromolecular structures is a bottleneck in X-ray crystallography. Anomalous dispersion was recognized as a powerful tool for phasing macromolecular structures. It was used mainly to supplement the isomorphous replacement or to locate the anomalous scatterer itself. The first step in solving macromolecular structures by SAD (single-wavelength anomalous diffraction) is the location of the anomalous scatterers. The SAD method for experimental phasing has evolved substantially in the recent years. A phasing tool, 5-amino-2,4,6- triiodoisophthalic acid (I3C—magic triangle), was incorporated into three proteins, lysozyme, glucose isomerase and thermolysin using quick-soaking and co-crystallization method in order to understand the binding of metal ion with proteins. The high quality of the diffraction data, the use of chromium anode X-ray radiation and the required amount of anomalous signal enabled way for successful structure determination and automated model building. An analysis and/or comparison of the sulfur and iodine anomalous signals at the Cr Kα wavelength are discussed.
基金Project (51004034) supported by the National Natural Science, ChinaProject(N090302009) supported by the Fundamental Research Funds for the Central Universities, China
文摘Raman spectrum of molten cryolite was recorded. Based on the new understanding of the scattering coefficients, contents of various structural entities in acidic NaF-AlF3 melts at 942-1 024 ℃ in previous research were reanalyzed. The new quantitative analysis results show that when cryolite ratio(CR) is less than 2, AlF4- is the dominant anion in the melts, and its mole fraction is about 0.70 for melts with CR=1.5 and 0.50 for melts with CR=2. When CR is more than 2.5, the mole fraction of AlF6^3- is relatively large, which is around 0.45 for melts with CR=2.5. Ionic structure of Na3AlF6-Al2O3 melts was investigated by UV-Raman spectroscopy. Octahedral AlF6^3- and tetrahedral AlF4- are proved to exist with possible partial replacement of F- by O^2-. Al2O2F4^2- with a large scattering coefficient also exists in the melts in which alumina concentration is more than 4% (mass fraction). The increase of temperature causes blue-shift of the bands in the Raman spectra.