To overcome the difficulty and high cost of some specific isotopic targets,a substitution method was proposed to measure the cross section of the(γ,n)reactions.Considering that the natural copper element(^(nat)Cu)onl...To overcome the difficulty and high cost of some specific isotopic targets,a substitution method was proposed to measure the cross section of the(γ,n)reactions.Considering that the natural copper element(^(nat)Cu)only has^(63)Cu and^(65)Cu isotopes,the^(65)Cu(γ,n)^(64)Cu reaction was taken as an example to test the substitution method.Using quasi-monoenergeticγbeams provided by the Shanghai Laser Electron Gamma Source(SLEGS)of the Shanghai Synchrotron Radiation Facility(SSRF),^(nat)Cu(γ,n)was measured from E_(γ)=11.09 MeV to 17.87 MeV.Furthermore,based on the^(63)Cu(γ,n)reaction measured using the same experimental setup at SLEGS,^(65)Cu(γ,n)^(64)Cu was extracted using the substitution method.The abundance variation of natural copper,showing a significant influence on the cross section,was also investigated.The results were compared to the existing experimental data measured by bremsstrahlung and positron annihilation in-flight sources,and the TALYS 2.0 predictions.Theγstrength function(γSF)of^(65)Cu was obtained from the^(65)Cu(γ,n)data,and the reaction cross section of^(64)Cu(n,γ)was further calculated.展开更多
The accurate photoneutron cross section of the^(27)Al nucleus has a significant impact on resolving differences in existing experimental data and enhancing the precision of nuclear reaction rate calculations for^(26)A...The accurate photoneutron cross section of the^(27)Al nucleus has a significant impact on resolving differences in existing experimental data and enhancing the precision of nuclear reaction rate calculations for^(26)Al in nuclear astrophysics.The photoneutron cross sections for the^(27)Al(γ,n)^(26)Al reaction,within the neutron separation energy range of 13.2-21.7 MeV,were meticulously measured using a new flat efficiency detector array at the Shanghai Laser-Electron Gamma Source.The uncertainty of the data was controlled to below 4%throughout the process,and inconsistencies between the present data and existing data from different gamma sources,as well as the TENDL-2021 data,are discussed in detail.These discussions provide a valuable reference for addressing discrepancies in the^(27)Al(γ,n)^(26)Al cross-section data and improving related theoretical calculations.展开更多
A reasonable prediction of photofission observables plays a paramount role in understanding the photofission process and guiding various photofission-induced applications,such as short-lived isotope production,nuclear...A reasonable prediction of photofission observables plays a paramount role in understanding the photofission process and guiding various photofission-induced applications,such as short-lived isotope production,nuclear waste disposal,and nuclear safeguards.However,the available experimental data for photofission observables are limited,and the existing models and programs have mainly been developed for neutron-induced fission processes.In this study,a general framework is proposed for characterizing the photofission observables of actinides,including the mass yield distributions(MYD) and isobaric charge distributions(ICD) of fission fragments and the multiplicity and energy distributions of prompt neutrons(n_(p)) and prompt γ rays(γ_(p)).The framework encompasses various systematic neutron models and empirical models considering the Bohr hypothesis and does not rely on the experimental data as input.These models are then validated individually against experimental data at an average excitation energy below 30 MeV,which shows the reliability and robustness of the general framework.Finally,we employ this framework to predict the characteristics of photofission fragments and the emissions of prompt particles for typical actinides including ^(232)Th,^(235,238)U and ^(240)Pu.It is found that the ^(238)U(γ,f) reaction is more suitable for producing neutron-rich nuclei compared to the ^(232)Th(γ,f) reaction.In addition,the average multiplicity number of both n_(p) and yp increases with the average excitation energy.展开更多
基金supported by the National key R&D program(Nos.2022YFA1602404 and 2023YFA1606901)the National Natural Science Foundation of China(Nos.12375123 and 12388102)the Natural Science Foundation of Henan Province(No.242300422048).
文摘To overcome the difficulty and high cost of some specific isotopic targets,a substitution method was proposed to measure the cross section of the(γ,n)reactions.Considering that the natural copper element(^(nat)Cu)only has^(63)Cu and^(65)Cu isotopes,the^(65)Cu(γ,n)^(64)Cu reaction was taken as an example to test the substitution method.Using quasi-monoenergeticγbeams provided by the Shanghai Laser Electron Gamma Source(SLEGS)of the Shanghai Synchrotron Radiation Facility(SSRF),^(nat)Cu(γ,n)was measured from E_(γ)=11.09 MeV to 17.87 MeV.Furthermore,based on the^(63)Cu(γ,n)reaction measured using the same experimental setup at SLEGS,^(65)Cu(γ,n)^(64)Cu was extracted using the substitution method.The abundance variation of natural copper,showing a significant influence on the cross section,was also investigated.The results were compared to the existing experimental data measured by bremsstrahlung and positron annihilation in-flight sources,and the TALYS 2.0 predictions.Theγstrength function(γSF)of^(65)Cu was obtained from the^(65)Cu(γ,n)data,and the reaction cross section of^(64)Cu(n,γ)was further calculated.
基金supported by the National key R&D program(Nos.2023YFA1606901 and 2022YFA1602404)the National Natural Science Foundation of China(Nos.12375123 and 12388102)the Natural Science Foundation of Henan Province(No.242300422048)。
文摘The accurate photoneutron cross section of the^(27)Al nucleus has a significant impact on resolving differences in existing experimental data and enhancing the precision of nuclear reaction rate calculations for^(26)Al in nuclear astrophysics.The photoneutron cross sections for the^(27)Al(γ,n)^(26)Al reaction,within the neutron separation energy range of 13.2-21.7 MeV,were meticulously measured using a new flat efficiency detector array at the Shanghai Laser-Electron Gamma Source.The uncertainty of the data was controlled to below 4%throughout the process,and inconsistencies between the present data and existing data from different gamma sources,as well as the TENDL-2021 data,are discussed in detail.These discussions provide a valuable reference for addressing discrepancies in the^(27)Al(γ,n)^(26)Al cross-section data and improving related theoretical calculations.
基金Supported by the National Natural Science Foundation of China (11675075)Independent research project of key laboratory of plasma physics,CAEP(JCKYS2021212009)Hengyang Municipal Science and Technology Project (202150054076)。
文摘A reasonable prediction of photofission observables plays a paramount role in understanding the photofission process and guiding various photofission-induced applications,such as short-lived isotope production,nuclear waste disposal,and nuclear safeguards.However,the available experimental data for photofission observables are limited,and the existing models and programs have mainly been developed for neutron-induced fission processes.In this study,a general framework is proposed for characterizing the photofission observables of actinides,including the mass yield distributions(MYD) and isobaric charge distributions(ICD) of fission fragments and the multiplicity and energy distributions of prompt neutrons(n_(p)) and prompt γ rays(γ_(p)).The framework encompasses various systematic neutron models and empirical models considering the Bohr hypothesis and does not rely on the experimental data as input.These models are then validated individually against experimental data at an average excitation energy below 30 MeV,which shows the reliability and robustness of the general framework.Finally,we employ this framework to predict the characteristics of photofission fragments and the emissions of prompt particles for typical actinides including ^(232)Th,^(235,238)U and ^(240)Pu.It is found that the ^(238)U(γ,f) reaction is more suitable for producing neutron-rich nuclei compared to the ^(232)Th(γ,f) reaction.In addition,the average multiplicity number of both n_(p) and yp increases with the average excitation energy.
