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Conceptual design of an ultra-high flux fast reactor with strong irradiation capability
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作者 Qingquan PAN Lianjie WANG +2 位作者 Bangyang XIA Yun CAI Xiaojing LIU 《Science China(Technological Sciences)》 2026年第3期44-57,共14页
From an engineering feasibility standpoint, what level of performance metrics can be ultimately achieved when designing a reactor using well-established nuclear fuels and structural materials that have already undergo... From an engineering feasibility standpoint, what level of performance metrics can be ultimately achieved when designing a reactor using well-established nuclear fuels and structural materials that have already undergone irradiation testing? The irradiation capability, which hinges on parameters like neutron flux level, irradiation channels' volume, and fuel cycle duration, is a core indicator for high-flux reactors. We propose a conceptual design of an ultra-high flux fast reactor(UFFR) with strong irradiation capability, which utilizes U-20Pu-10Zr alloy fuel and employs lead-bismuth as the coolant. The maximum neutron flux in the core reaches 1.32×10^(16) cm^(-2)s^(-1), while the average neutron flux in the irradiation channels attains 1.19×10^(16) cm^(-2)s^(-1). The volume of the central irradiation channel exceeds 10000 cm^(3), and the fuel cycle duration is 165 d, placing all its performance indicators among the top in the world. Based on the analyses of reactor physics and thermalhydraulics, it has been demonstrated that all reactivity coefficients are negative and all physical parameters meet the design criteria, ensuring the inherent safety of UFFR. An assessment of the irradiation capability has been carried out based on californium-252(^(252)Cf) production, indicating that the irradiation capability of UFFR surpasses that of the high flux isotope reactor(HFIR). The yield of ^(252)Cf from UFFR is 14.39 times that of HFIR, and its nuclei conversion rate is 3.21 times that of HFIR. 展开更多
关键词 high-flux reactor conceptual design neutron flux irradiation capability californium-252
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Conceptual design and preliminary feasibility study of fluid‑driven suspended control rods for molten salt reactors
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作者 Jin‑Tong Cao Gui‑Feng Zhu +4 位作者 Chang‑Qing Yu Ya‑Fen Liu Yang Zou Rui Yan Hong‑Jie Xu 《Nuclear Science and Techniques》 2026年第1期225-243,共19页
Molten salt reactors,being the only reactor type among Generation Ⅳ advanced nuclear reactors that utilize liquid fuels,offer inherent safety,high-temperature,and low-pressure operation,as well as the capability for ... Molten salt reactors,being the only reactor type among Generation Ⅳ advanced nuclear reactors that utilize liquid fuels,offer inherent safety,high-temperature,and low-pressure operation,as well as the capability for online fuel reprocessing.However,the fuel-salt flow results in the decay of delayed neutron precursors(DNPs)outside the core,causing fluctuations in the effective delayed neutron fraction and consequently impacting the reactor reactivity.Particularly in accident scenarios—such as a combined pump shutdown and the inability to rapidly scram the reactor—the sole reliance on negative temperature feedback may cause a significant increase in core temperature,posing a threat to reactor safety.To address these problems,this paper introduces an innovative design for a passive fluid-driven suspended control rod(SCR)to dynamically compensate for reactivity fluctuations caused by DNPs flowing with the fuel.The control rod operates passively by leveraging the combined effects of gravity,buoyancy,and fluid dynamic forces,thereby eliminating the need for an external drive mechanism and enabling direct integration within the active region of the core.Using a 150 MWt thorium-based molten salt reactor as the reference design,we develop a mathematical model to systematically analyze the effects of key parameters—including the geometric dimensions and density of the SCR—on its performance.We examine its motion characteristics under different core flow conditions and assess its feasibility for the dynamic compensation of reactivity changes caused by fuel flow.The results of this study demonstrate that the SCR can effectively counteract reactivity fluctuations induced by fuel flow within molten salt reactors.A sensitivity analysis reveals that the SCR’s average density exerts a profound impact on its start-up flow threshold,channel flow rate,resistance to fuel density fluctuations,and response characteristics.This underscores the critical need to optimize this parameter.Moreover,by judiciously selecting the SCR’s length,number of deployed units,and the placement we can achieve the necessary reactivity control while maintaining a favorable balance between neutron economy and heat transfer performance.Ultimately,this paper provides an innovative solution for the passive reactivity control in molten salt reactors,offering significant potential for practical engineering applications. 展开更多
关键词 Molten salt reactor DNP flow-induced reactivity Passive control Suspended control rod
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Efficient control and removal of laser‑generated aerosol particles by combining water spray with pre‑injection of electrical charged mist for nuclear reactor decommissioning
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作者 Ruicong Xu Avadhesh Kumar Sharma +6 位作者 Zeeshan Ahmed Ravinder Kumar Laffolley Hugo Ryo Yokoyama Shuichiro Miwa Shunichi Suzuki Atsushi Kosuge 《Nuclear Science and Techniques》 2026年第1期244-262,共19页
Laser-induced aerosols,predominantly submicron in size,pose significant environmental and health risks during the decommissioning of nuclear reactors.This study experimentally investigated the removal of laser-generat... Laser-induced aerosols,predominantly submicron in size,pose significant environmental and health risks during the decommissioning of nuclear reactors.This study experimentally investigated the removal of laser-generated aerosol particles using a water spray system integrated with an innovative system for pre-injecting electrically charged mist in our facility.To simulate aerosol generation in reactor decommissioning,a high-power laser was used to irradiate various materials(including stainless steel,carbon steel,and concrete),generating aerosol particles that were agglomerated with injected water mist and subsequently scavenged by water spray.Experimental results demonstrate enhanced aerosol removal via aerosol-mist agglomeration,with charged mist significantly improving particle capture by increasing wettability and size.The average improvements for the stainless steel,carbon steel,and concrete were 40%,44%,and 21%,respectively.The results of experiments using charged mist with different polarities(both positive and negative)and different surface coatings reveal that the dominant polarity of aerosols varies with the irradiated materials,influenced by their crystal structure and electron emission properties.Notably,surface coatings such as ZrO_(2)and CeO_(2)were found to possibly alter aerosol charging characteristics,thereby affecting aerosol removal efficiency with charged mist configurations.The innovative aerosol-mist agglomeration approach shows promise in mitigating radiation exposure,ensuring environmental safety,and reducing contaminated water during reactor dismantling.This study contributes critical knowledge for the development of advanced aerosol management strategies for nuclear reactor decommissioning.The understanding obtained in this work is also expected to be useful for various environmental and chemical engineering applications such as gas decontamination,air purification,and pollution control. 展开更多
关键词 Laser-induced aerosol generation Aerosol removal Electrically charging mist AGGLOMERATION Water spray scavenging reactor decommissioning
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Comparing of small and large optimal tapered cascades for supplying enriched uranium for fresh fuel production in the equilibrium cycle of a nuclear power reactor
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作者 S.L.Mirmohammadi J.Safdari A.A.Ghorbanpour Khamseh 《Nuclear Science and Techniques》 2026年第3期208-234,共27页
One of the main issues in designing optimum tapered cascades for uranium enrichment for annual fuel production in a power reactor is whether to employ large(fat)or small(thin)cascades.What will be the permissible and ... One of the main issues in designing optimum tapered cascades for uranium enrichment for annual fuel production in a power reactor is whether to employ large(fat)or small(thin)cascades.What will be the permissible and optimal ranges of the number of machines that can be used in a cascade?For the first time,the permissible and optimal ranges of the number of gas centrifuges that can be utilized in a cascade were investigated using two types of centrifuges,and the performance of small and large tapered cascades was discussed.The particle swarm optimization algorithm(PSO)has been used to optimize tapered cascades.The results show:(1)For the first centrifuge,41 cascades(91≤n≤4897)and for the second centrifuge,49 cascades(18≤n≤3839)with small and large sizes can be used in enrichment facilities,and the best cascade for them has 530(with 23 stages)and 39(with 7 stages)centrifuges,respectively.(2)For both centrifuges,when 600≤n(number of centrifuges=n),the large cascade performance changes are relatively insignificant.(3)For both types of gas centrifuges,the annual los s of separation power in enrichment facilities is approximately 1.25%-4.82%of the total separation work required. 展开更多
关键词 Small tapered cascade(thin) Large tapered cascade(fat) Enriched uranium fuel Power reactor PSO algorithm
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Single-phase-to-ground fault protection based on zero-sequence current ratio coefficient for low-resistance grounding distribution network 被引量:4
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作者 Jianrui Li Yongli Li +1 位作者 Yonghuan Wang Jinzhao Song 《Global Energy Interconnection》 EI CAS CSCD 2021年第6期564-575,共12页
Definite-time zero-sequence over-current protection is presently used in systems whose neutral point is grounded by a low resistance(low-resistance grounding systems).These systems frequently malfunction owing to thei... Definite-time zero-sequence over-current protection is presently used in systems whose neutral point is grounded by a low resistance(low-resistance grounding systems).These systems frequently malfunction owing to their high settings of the action value when a high-impedance grounding fault occurs.In this study,the relationship between the zero-sequence currents of each feeder and the neutral branch was analyzed.Then,a grounding protection method was proposed on the basis of the zero-sequence current ratio coefficient.It is defined as the ratio of the zero-sequence current of the feeder to that of the neutral branch.Nonetheless,both zero-sequence voltage and zero-sequence current are affected by the transition resistance,The influence of transition resistance can be eliminated by calculating this coefficient.Therefore,a method based on the zero-sequence current ratio coefficient was proposed considering the significant difference between the faulty feeder and healthy feeder.Furthermore,unbalanced current can be prevented by setting the starting current.PSCAD simulation results reveal that the proposed method shows high reliability and sensitivity when a high-resistance grounding fault occurs. 展开更多
关键词 Low-resistance grounding system High-impedance grounding fault Grounding protection zero-sequence current ratio coefficient
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Zero-sequence Current Suppressing Strategy for Dual Three-phase Permanent Magnet Synchronous Machines Connected with Single Neutral Point 被引量:3
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作者 Zongwang Li Yuxuan Du +2 位作者 Jinghua Ji Tao Tao Wenxiang Zhao 《CES Transactions on Electrical Machines and Systems》 CSCD 2022年第4期465-472,共8页
Dual three-phase permanent-magnet synchronous machines(DTP-PMSM)connected with a single neutral point provide a loop for zero-sequence current(ZSC).This paper proposes a novel space vector pulse width modulation(SVPWM... Dual three-phase permanent-magnet synchronous machines(DTP-PMSM)connected with a single neutral point provide a loop for zero-sequence current(ZSC).This paper proposes a novel space vector pulse width modulation(SVPWM)strategy to suppress the ZSC.Five vectors are selected as basic voltage vectors in one switching period.The fundamental and harmonic planes and the zero-sequence plane are taken into consideration to synthesis the reference voltage vector.To suppress the ZSC,a non-zero zero-sequence voltage(ZSV)is generated to compensate the third harmonic back-EMF.Rather than triangular carrier modulation,the sawtooth carrier modulation strategy is used to generate asymmetric PWM signals.The modulation range is investigated to explore the variation of modulation range caused by considering the zero-sequence plane.With the proposed method,the ZSC can be considerably reduced.The simulated and experimental results are presented to validate the effectiveness of the proposed modulation strategy. 展开更多
关键词 zero-sequence current a single neutral point dual three-phase permanent-magnet synchronous machine third harmonic back-EMF
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Protection of Zero-Sequence Power Variation in Mountain Wind Farm Collector Lines Based on Multi-Mode Grounding
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作者 Hongchun Shu Yaqi Deng +3 位作者 Pulin Cao Jun Dong Hongjiang Rao Zhiqian Bo 《Energy Engineering》 EI 2022年第2期523-538,共16页
The arc-suppression coil(ASC)in parallel low resistance(LR)multi-mode grounding is adopted in the mountain wind farm to cope with the phenomenon that is misoperation or refusal of zero-sequence protection in LR ground... The arc-suppression coil(ASC)in parallel low resistance(LR)multi-mode grounding is adopted in the mountain wind farm to cope with the phenomenon that is misoperation or refusal of zero-sequence protection in LR grounding wind farm.If the fault disappears before LR is put into the system,it is judged as an instantaneous fault;while the fault does not disappear after LR is put into the system,it is judged as a permanent fault;the single-phase grounding fault(SLG)protection criterion based on zerosequence power variation is proposed to identify the instantaneous-permanent fault.Firstly,the distribution characteristic of zero-sequence voltage(ZSV)and zero-sequence current(ZSC)are analyzed after SLGfault occurs in multi-mode grounding.Then,according to the characteristics that zero-sequence power variation of non-fault collector line is small,while the zero-sequence power variation of fault collector line can reflect the active power component of fault resistance,the protection criterion based on zero-sequence power variation is constructed.The theoretical analysis and simulation results show that the protection criterion can distinguish the property of fault only by using the single terminal information,which has high reliability. 展开更多
关键词 Mountain wind farm multi-mode grounding collector line single-phase grounding fault zero-sequence power variation
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Zero-Sequence Current Suppression Strategy for Open-End Winding Permanent Magnet Synchronous Motor Based on Model Predictive Control
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作者 LIU Huashan LI Jie YAO Fei 《Journal of Donghua University(English Edition)》 EI CAS 2020年第4期286-292,共7页
Compared with the traditional three-phase star connection winding,the open-end winding permanent magnet synchronous motor(OW-PMSM)system with a common direct current(DC)bus has a zero-sequence circuit,which makes the ... Compared with the traditional three-phase star connection winding,the open-end winding permanent magnet synchronous motor(OW-PMSM)system with a common direct current(DC)bus has a zero-sequence circuit,which makes the common-mode voltage and the back electromotive force(EMF)harmonic generated by the inverters produce the zero-sequence current in the zero-sequence circuit,and the zero-sequence current has great influence on the operation efficiency and stability of the motor control system.A zero-sequence current suppression strategy is presented based on model predictive current control for OW-PMSM.Through the mathematical model of OW-PMSM to establish the predictive model and the zero-sequence circuit model,the common-mode voltage under different voltage vector combinations is fully considered during vector selection and action time calculation.Then zero-sequence loop constraints are established,so as to suppress the zero-sequence current.In the end,the control strategy proposed in this paper is verified by simulation experiments. 展开更多
关键词 open-end winding permanent magnet synchronous motor(OW-PMSM) zero-sequence current HARMONIC model predictive current control common-mode voltage
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Electromagnetic Zero-Sequence Harmonics Blocker: Modeling and Experimental Analysis
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作者 Luis C. Origa de Oliveira Rodrigo N. de Oliveira +1 位作者 Julio B. de Souza Stefani C. L. de Freitas 《Journal of Energy and Power Engineering》 2014年第8期1425-1431,共7页
This paper reveals new contributions to the analysis and development of devices for harmonic distortion mitigation. Considering the sequential distribution of harmonic currents, zero-sequence components could be dimin... This paper reveals new contributions to the analysis and development of devices for harmonic distortion mitigation. Considering the sequential distribution of harmonic currents, zero-sequence components could be diminished using electromagnetic devices, particularly the eZSB (electromagnetic zero-sequence blocking). One important characteristic of this device, which has received particular attention on this research, is its robustness and low cost of construction. Theoretical and experimental results related to the behavior of the electromagnetic blocking devices are presented. The results illustrate the consistence of the theoretical aspects related with the model in the frequency domain, as well as the performance of the blocking devices, reducing zero-sequence harmonic currents, mainly by the conjunct action of the eZSF (electromagnetic zero-sequence harmonic filter), working as a impedance coupler. In this context, aiming the evaluation of the reliability of the results obtained through mathematical modeling, experimental tests have been carried out using a low-power prototype, highlighting particular aspects related to its function as a zero-sequence harmonic blocker. 展开更多
关键词 Electromagnetic blocker zero-sequence harmonics triplens harmonics power quality
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Dataset of neutron energy region values for the in-reactor production of medical isotopes 被引量:1
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作者 Qing-Quan Pan Guo Lv +1 位作者 Sheng-Dian Zou Xiao-Jing Liu 《Nuclear Science and Techniques》 2025年第8期18-25,共8页
Medical isotopes are the foundation material for nuclear medicine and are primarily produced through in-reactor irradia-tion.Neutron spectrum regulation is the main technical approach for enhancing the production of m... Medical isotopes are the foundation material for nuclear medicine and are primarily produced through in-reactor irradia-tion.Neutron spectrum regulation is the main technical approach for enhancing the production of medical isotopes,and it requires determining the optimal neutron spectrum and quantifying the values of neutrons in different energy regions.We calculated the neutron energy region values for 20 medical isotopes(^(14)C,^(32)P,^(47)Sc,^(60)Co,^(64)Cu,^(67)Cu,^(89)Sr,^(90)Y,^(99)Mo,^(125)I,^(131)I,^(153)Sm,^(161)Tb,^(166)Ho,^(177)Lu,^(186)Re,^(188)Re,^(92)Ir,^(225)Ac,and ^(252)Cf).The entire energy range was divided into 238 energy regions to improve the energy spectrum resolution,and both fast and thermal reactors were simulated to enhance universal applicability.A dataset of neutron energy region values across the entire energy range was built,which identifies the positive and negative-energy regions and guides the neutron spectrum regulation process during in-reactor medical isotope produc-tion.We conducted neutron spectrum regulation based on this dataset,which effectively improved the production efficiency of medical isotopes and demonstrated the correctness and feasibility of the dataset. 展开更多
关键词 Medical isotopes High-flux isotope reactor Neutron energy region value Spectrum regulation
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Intelligent path planning for small modular reactors based on improved reinforcement learning
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作者 DONG Yun-Feng ZHOU Wei-Zheng +1 位作者 WANG Zhe-Zheng ZHANG Xiao 《四川大学学报(自然科学版)》 北大核心 2025年第4期1006-1014,共9页
Small modular reactor(SMR)belongs to the research forefront of nuclear reactor technology.Nowadays,advancement of intelligent control technologies paves a new way to the design and build of unmanned SMR.The autonomous... Small modular reactor(SMR)belongs to the research forefront of nuclear reactor technology.Nowadays,advancement of intelligent control technologies paves a new way to the design and build of unmanned SMR.The autonomous control process of SMR can be divided into three stages,say,state diagnosis,autonomous decision-making and coordinated control.In this paper,the autonomous state recognition and task planning of unmanned SMR are investigated.An operating condition recognition method based on the knowledge base of SMR operation is proposed by using the artificial neural network(ANN)technology,which constructs a basis for the state judgment of intelligent reactor control path planning.An improved reinforcement learning path planning algorithm is utilized to implement the path transfer decision-makingThis algorithm performs condition transitions with minimal cost under specified modes.In summary,the full range control path intelligent decision-planning technology of SMR is realized,thus provides some theoretical basis for the design and build of unmanned SMR in the future. 展开更多
关键词 Small modular reactor Operating condition recognition Path planning Reinforcement learning
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A composite controller for reactor core combining artificial neural network and fractional-order PID controller
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作者 WANG Zhe-Zheng ZHANG Xiao DENG Ke 《四川大学学报(自然科学版)》 北大核心 2025年第4期1015-1024,共10页
Core power is a key parameter of nuclear reactor.Traditionally,the proportional-integralderivative(PID)controllers are used to control the core power.Fractional-order PID(FOPID)controller represents the cutting edge i... Core power is a key parameter of nuclear reactor.Traditionally,the proportional-integralderivative(PID)controllers are used to control the core power.Fractional-order PID(FOPID)controller represents the cutting edge in core power control research.In comparing with the integer-order models,fractional-order models describe the variation of core power more accurately,thus provide a comprehensive and realistic depiction for the power and state changes of reactor core.However,current fractional-order controllers cannot adjust their parameters dynamically to response the environmental changes or demands.In this paper,we aim at the stable control and dynamic responsiveness of core power.Based on the strong selflearning ability of artificial neural network(ANN),we propose a composite controller combining the ANN and FOPID controller.The FOPID controller is firstly designed and a back propagation neural network(BPNN)is then utilized to optimize the parameters of FOPID.It is shown by simulation that the composite controller enables the real-time parameter tuning via ANN and retains the advantage of FOPID controller. 展开更多
关键词 Nuclear reactor Core power Fractional PID controller Artificial neural network
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Photocatalytic C−C coupling of acetonitrile into succinonitrile over hydrophobic TiO_(2) in a flow reactor
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作者 GONG Kun HUANG Min +4 位作者 LI Ruitao DAI Yuanyuan NIU Qiang LIN Tiejun ZHONG Liangshu 《燃料化学学报(中英文)》 北大核心 2025年第12期1807-1816,共10页
A radical C−C-coupling reaction of acetonitrile into succinonitrile over hydrophobic TiO_(2) photocatalyst with enhanced catalytic activity was developed.In addition,the usage of a flow reactor further improved the ph... A radical C−C-coupling reaction of acetonitrile into succinonitrile over hydrophobic TiO_(2) photocatalyst with enhanced catalytic activity was developed.In addition,the usage of a flow reactor further improved the photon utilization efficiency for succinonitrile synthesis at room temperature.The space time yield of succinonitrile reached 55.59μmol/(g·h)over hydrophobic TiO_(2) catalyst,which was much higher than that of pristine TiO_(2)(4.23μmol/(g·h)).Mechanistic studies revealed that the hydrophobic modification of TiO_(2) promoted the separation and transfer of photogenerated carriers,as well as suppressed their recombination.Hydrophobic TiO_(2) also enhanced the adsorption of−CH3 of acetonitrile,thus facilitating the activation of C−H bond and the utilization efficiency of photocarriers. 展开更多
关键词 photocatalysis SUCCINONITRILE C−C coupling hydrophobic TiO_(2) flow reactor
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Densification and thermal properties of cylindrical graphite-based fuel elements used in a molten salt reactor
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作者 WANG Gan WANG Hao-ran +5 位作者 LU Lin-yuan LI Wan-lin CHEN Nan-nan HE Yun ZHONG Ya-juan LIN Jun 《新型炭材料(中英文)》 北大核心 2025年第6期1362-1376,I0059,共16页
Based on the service characteristics of fuel elements for molten salt reactors,they need to have a high power density,resistance to coolant infiltration,and excellent thermodynamic properties.To solve the problem of t... Based on the service characteristics of fuel elements for molten salt reactors,they need to have a high power density,resistance to coolant infiltration,and excellent thermodynamic properties.To solve the problem of the graphite used in the fuel element for these reactors being susceptible to molten salt infiltration,carbon black(CB)was added to increase the density of the graphite,and a fuel element(TRISO(tri-structural isotropic)fuel particles were randomly distributed in the modified graphite matrix)was prepared by cold isostatic pressing process.An out-of-pile performance study shows that the densification and pore structure of the modified graphite matrix were improved,as was the resistance to molten salt infiltration.The median pore size of the modified graphite was reduced from 673 to 433 nm and the threshold pressure for molten salt(FLiBe,66%(molar fraction)LiF and 34%BeF_(2))infiltration was increased from 0.88 to 1.37 MPa.The isotropic CB made the graphite matrix less anisotropic,while its thermal conductivity and compressive strength were reduced due to the difficult graphitization of CB.Fuel elements containing 20%(volume fraction)TRISO particles were prepared.Numerical simulations show that the power and temperature distribution of the fuel were in line with the design requirements.The modified graphite matrix had a higher density,smaller pores,a lower anisotropy and a greater resistance to FLiBe infiltration. 展开更多
关键词 Molten salt reactor Cylindrical fuel element Graphite matrix Thermal properties Molten salt infiltration
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Ambient CO_(2) Capture and Valorization Enabled by Tandem Electrolysis Using Solid-State Electrolyte Reactor
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作者 Yan-Bo Hua Bao-Xin Ni Kun Jiang 《电化学(中英文)》 北大核心 2025年第6期38-50,共13页
Electrocatalytic carbon dioxide reduction is a promising technology for addressing global energy and environmental crises. However, its practical application faces two critical challenges: the complex and energy-inten... Electrocatalytic carbon dioxide reduction is a promising technology for addressing global energy and environmental crises. However, its practical application faces two critical challenges: the complex and energy-intensive process of separat-ing mixed reduction products and the economic viability of the carbon sources (reactants) used. To tackle these challenges simultaneously, solid-state electrolyte (SSE) reactors are emerging as a promising solution. In this review, we focus on the feasibility of applying SSE for tandem electrochemical CO_(2) capture and conversion. The configurations and fundamental principles of SSE reactors are first discussed, followed by an introduction to its applications in these two specific areas, along with case studies on the implementation of tandem electrolysis. In comparison to conventional H-type cell, flow cell and membrane electrode assembly cell reactors, SSE reactors incorporate gas diffusion electrodes and utilize a solid electro-lyte layer positioned between an anion exchange membrane (AEM) and a cation exchange membrane (CEM). A key inno-vation of this design is the sandwiched SSE layer, which enhances efficient ion transport and facilitates continuous product extraction through a stream of deionized water or humidified nitrogen, effectively separating ion conduction from product collection. During electrolysis, driven by an electric field and concentration gradient, electrochemically generated ions (e.g., HCOO- and CH3COO-) migrate through the AEM into the SSE layer, while protons produced from water oxidation at the anode traverse the CEM into the central chamber to maintain charge balance. Targeted products like HCOOH can form in the middle layer through ionic recombination and are efficiently carried away by the flowing medium through the porous SSE layer, in the absence of electrolyte salt impurities. As CO_(2)RR can generate a series of liquid products, advancements in catalyst discovery over the past several years have facilitated the industrial application of SSE for more efficient chemicals production. Also noteworthy, the cathode reduction reaction can readily consume protons from water, creating a highly al-kaline local environment. SSE reactors are thereby employed to capture acidic CO_(2), forming CO_(3)^(2-) from various gas sources including flue gases. Driven by the electric field, the formed CO_(3)^(2-) can traverse through the AEM and react with protons originating from the anode, thereby regenerating CO_(2). This CO_(2) can then be collected and utilized as a low-cost feedstock for downstream CO_(2) electrolysis. Based on this principle, several cell configurations have been proposed to enhance CO_(2) capture from diverse gas sources. Through the collaboration of two SSE units, tandem electrochemical CO_(2) capture and con-version has been successfully implemented. Finally, we offer insights into the future development of SSE reactors for prac-tical applications aimed at achieving carbon neutrality. We recommend that greater attention be focused on specific aspects, including the fundamental physicochemical properties of the SSE layer, the electrochemical engineering perspective related to ion and species fluxes and selectivity, and the systematic pairing of consecutive CO_(2) capture and conversion units. These efforts aim to further enhance the practical application of SSE reactors within the broader electrochemistry community. 展开更多
关键词 ELECTROCATALYSIS ELECTROLYSIS CO_(2)capture CO_(2)reduction Solid-state electrolyte reactor
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Validation and application of a coupled xenon-transport and reactor dynamic model of Molten-salt reactor experiment
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作者 Jia-Qi Chen Caleb S.Brooks 《Nuclear Science and Techniques》 2025年第6期156-175,共20页
Liquid-fueled molten-salt reactors have dynamic features that distinguish them from solid-fueled reactors,such that conventional system-analysis codes are not directly applicable.In this study,a coupled dynamic model ... Liquid-fueled molten-salt reactors have dynamic features that distinguish them from solid-fueled reactors,such that conventional system-analysis codes are not directly applicable.In this study,a coupled dynamic model of the Molten-Salt Reactor Experiment(MSRE)is developed.The coupled model includes the neutronics and single-phase thermal-hydraulics modeling of the reactor and validated xenon-transport modeling from previous studies.The coupled dynamic model is validated against the frequency-response and transient-response data from the MSRE.The validated model is then applied to study the effects of xenon and void transport on the dynamic behaviors of the reactor.Plant responses during the unique initiating events such as off-gas system blockages and loss of circulating voids are investigated. 展开更多
关键词 Nuclear-reactor dynamics Molten-salt reactor experiment Frequency response Molten-salt reactor XENON
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CFD-ML integrated multi-objective optimization for n-butane partial oxidation reactor
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作者 Xiangkun Liu Qihuan Qiu +4 位作者 Bingxu Chen Yao Shi Longqin Gu Xinggui Zhou Xuezhi Duan 《Chinese Journal of Chemical Engineering》 2025年第12期53-64,共12页
This study develops a CFD-ML integrated framework to achieve multi-objective optimization for the partial oxidation of n-butane to maleic anhydride(MA).A reactor-pellet coupled model was established to investigate the... This study develops a CFD-ML integrated framework to achieve multi-objective optimization for the partial oxidation of n-butane to maleic anhydride(MA).A reactor-pellet coupled model was established to investigate the effects of four key operating parameters,revealing that inlet temperature dominates reactor performance by increasing MA yield from 35.0%to 37.6%while sharply raising hotspot temperatures by 42 K.The coupled model was then employed to generate 621 cases for training machine learning models,among which the Gaussian Process Regression(GPR)model exhibits superior accuracy.The GPR model was further integrated with the genetic algorithm to generate Pareto-optimal sets.The results indicate that a critical inflection point is identified on the Pareto front,and once this point is exceeded,even a slight increase in MA yield could lead to a sharp rise in the reactor hotspot temperature,thereby increasing the risk of thermal runaway. 展开更多
关键词 n-Butane partial oxidation reactor operating conditions reactor simulation Machine learning Pareto optimization
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Uncertainty and sensibility analysis of loss-of-forced-cooling accidents for 150-MWt molten salt reactors
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作者 Kai Wang Chao-Qun Wang +2 位作者 Qun Yang Zhao-Zhong He Na-Xiu Wang 《Nuclear Science and Techniques》 2025年第6期228-239,共12页
Molten salt reactors(MSRs)are a promising candidate for Generation IV reactor technologies,and the small modular molten salt reactor(SM-MSR),which utilizes low-enriched uranium and thorium fuels,is regarded as a wise ... Molten salt reactors(MSRs)are a promising candidate for Generation IV reactor technologies,and the small modular molten salt reactor(SM-MSR),which utilizes low-enriched uranium and thorium fuels,is regarded as a wise development path to accelerate deployment time.Uncertainty and sensitivity analyses of accidents guide nuclear reactor design and safety analyses.Uncertainty analysis can ascertain the safety margin,and sensitivity analysis can reveal the correlation between accident consequences and input parameters.Loss of forced cooling(LOFC)represents an accident scenario of the SM-MSR,and the study of LOFC could offer useful information to improve physical thermohydraulic and structural designs.Therefore,this study investigates the uncertainty of LOFC consequences and the sensitivity of related parameters.The uncertainty of the LOFC consequences was analyzed using the Monte Carlo method,and multiple linear regression was employed to analyze the sensitivity of the input parameters.The uncertainty and sensitivity analyses showed that the maximum reactor outlet fuel salt temperature was 725.5℃,which is lower than the acceptable criterion,and five important parameters influencing LOFC consequences were identified. 展开更多
关键词 Molten salt reactor LOFC Uncertainty analysis Sensibility analysis
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Microfluidic reactors for paired electrosynthesis:Fundamentals,applications and future prospects
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作者 Hao Xue Zhi-Hao Zhao +1 位作者 Menglei Yuan Guangjin Zhang 《Green Energy & Environment》 2025年第3期471-499,共29页
Paired electrosynthesis has received considerable attention as a consequence of simultaneously synthesizing target products at both cathode and anode,whereas the related synthetic efficiency in batch reactors is still... Paired electrosynthesis has received considerable attention as a consequence of simultaneously synthesizing target products at both cathode and anode,whereas the related synthetic efficiency in batch reactors is still undesirable under certain circumstances.Encouragingly,laminar microfluidic reactor offers prospective options that possess controllable flow characteristics such as enhanced mass transport,precise laminar flow control and the ability to expand production scale progressively.In this comprehensive review,the underlying fundamentals of the paired electrosynthesis are initially summarized,followed by categorizing the paired electrosynthesis including parallel paired electrosynthesis,divergent paired electrosynthesis,convergent paired electrosynthesis,sequential paired electrosynthesis and linear paired electrosynthesis.Thereafter,a holistic overview of microfluidic reactor equipment,integral fundamentals and research methodology as well as channel extension and scale-up strategies is proposed.The established fundamentals and evaluated metrics further inspired the applications of microfluidic reactors in paired electrosynthesis.This work stimulated the overwhelming investigation of mechanism discovery,material screening strategies,and device assemblies. 展开更多
关键词 Paired electrosynthesis Microfluidic reactor Laminar flow Scaling-up strategy
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Ray-tracing analysis of Doppler backscattering diagnostic for tokamak with reactor technologies
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作者 Alexander YASHIN Anna PONOMARENKO +1 位作者 Arseny TOKAREV Eugeniy KISELEV 《Plasma Science and Technology》 2025年第5期72-80,共9页
This study discusses the scope of application of the Doppler backscattering(DBS)diagnostic for the tokamak with reactor technologies(TRT)project.This involved numerical modeling of the three-dimensional(3D)beam trajec... This study discusses the scope of application of the Doppler backscattering(DBS)diagnostic for the tokamak with reactor technologies(TRT)project.This involved numerical modeling of the three-dimensional(3D)beam trajectories.Calculations were performed to investigate the propagation of microwaves in the V(40–75 GHz)and W(75–110 GHz)frequency ranges with O-mode polarization for the density profile of the base TRT scenario.Our analysis showed that the DBS system antenna on the TRT would need to be tilted in both the poloidal and toroidal directions in order to meet the condition Kperp/Kpar<10%..For the DBS system located in the equatorial plane it was shown that a wide range of poloidal and toroidal angles is available for the successful implementation of the diagnostic to study the core,pedestal and scrape-off layer(SOL)regions.The DBS system located at 35 cm above the equatorial plane would be more limited in measurements only covering the SOL and pedestal regions.A shift of the cut-offs in the toroidal direction highlighted the need for 3D analysis of the DBS data. 展开更多
关键词 plasma diagnostics Doppler backscattering Doppler reflectometry reactor tokamak TRT
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