Fine particulatematter(PM_(2.5))samples were collected in two neighboring cities,Beijing and Baoding,China.High-concentration events of PM_(2.5) in which the average mass concentration exceeded 75μg/m^(3) were freque...Fine particulatematter(PM_(2.5))samples were collected in two neighboring cities,Beijing and Baoding,China.High-concentration events of PM_(2.5) in which the average mass concentration exceeded 75μg/m^(3) were frequently observed during the heating season.Dispersion Normalized Positive Matrix Factorization was applied for the source apportionment of PM_(2.5) as minimize the dilution effects of meteorology and better reflect the source strengths in these two cities.Secondary nitrate had the highest contribution for Beijing(37.3%),and residential heating/biomass burning was the largest for Baoding(27.1%).Secondary nitrate,mobile,biomass burning,district heating,oil combustion,aged sea salt sources showed significant differences between the heating and non-heating seasons in Beijing for same period(2019.01.10–2019.08.22)(Mann-Whitney Rank Sum Test P<0.05).In case of Baoding,soil,residential heating/biomass burning,incinerator,coal combustion,oil combustion sources showed significant differences.The results of Pearson correlation analysis for the common sources between the two cities showed that long-range transported sources and some sources with seasonal patterns such as oil combustion and soil had high correlation coefficients.Conditional Bivariate Probability Function(CBPF)was used to identify the inflow directions for the sources,and joint-PSCF(Potential Source Contribution Function)was performed to determine the common potential source areas for sources affecting both cities.These models facilitated a more precise verification of city-specific influences on PM_(2.5) sources.The results of this study will aid in prioritizing air pollution mitigation strategies during the heating season and strengthening air quality management to reduce the impact of downwind neighboring cities.展开更多
Over the past decade,biomass burning has emerged as one of the main polluting events in northern India.It is one of the major sources of brown carbon(Br C),the light-absorbing organic carbon component of PM_(2.5).Most...Over the past decade,biomass burning has emerged as one of the main polluting events in northern India.It is one of the major sources of brown carbon(Br C),the light-absorbing organic carbon component of PM_(2.5).Most studies on the impact of biomass burning in India are based on source locations or urban areas;very little is known about its effects on a regional background location.We examine the effect of biomass burning on regional air quality and co-occurring meteorological factors.Year-long PM_(2.5)levels and light absorption by carbonaceous aerosols at 880 nm and 370 nm were measured at Rohtak,a regional background location.Results showed that post-harvest biomass burning in the Punjab-Haryana region affects the regional air quality with a lead of one to two days.A comparison of dispersionnormalized concentrations showed that open-field biomass burning not only affects regional air quality in the post-monsoon season(kharif crops)but is also a dominant source of PM_(2.5)in the post-harvest summer season(rabi crop).A significant(p<0.05)difference is observed in PM_(2.5),b_(abs-880),and b_(abs-370)between biomass burning days and non-biomass burning days during the kharif and rabi harvest seasons.Regression analyses confirm that in summer,regional PM_(2.5)and light absorption by aerosols are influenced more strongly by post-harvest burning of rabi crops.However,adverse meteorology plays a more dominant role in the post-monsoon season than biomass burning.These findings underscore the need for better policy interventions to curb biomass burning and improve air quality during both harvest seasons.展开更多
Substantial effects of photochemical reaction losses of volatile organic compounds(VOCs)on factor profiles can be investigated by comparing the differences between daytime and nighttime dispersion-normalized VOC data ...Substantial effects of photochemical reaction losses of volatile organic compounds(VOCs)on factor profiles can be investigated by comparing the differences between daytime and nighttime dispersion-normalized VOC data resolved profiles.Hourly speciated VOC data measured in Shijiazhuang,China from May to September 2021 were used to conduct study.The mean VOC concentration in the daytime and at nighttime were 32.8 and 36.0 ppbv,respectively.Alkanes and aromatics concentrations in the daytime(12.9 and 3.08 ppbv)were lower than nighttime(15.5 and 3.63 ppbv),whereas that of alkenes showed the opposite tendency.The concentration differences between daytime and nighttime for alkynes and halogenated hydrocarbonswere uniformly small.The reactivities of the dominant species in factor profiles for gasoline emissions,natural gas and diesel vehicles,and liquefied petroleum gas were relatively low and their profiles were less affected by photochemical losses.Photochemical losses produced a substantial impact on the profiles of solvent use,petrochemical industry emissions,combustion sources,and biogenic emissions where the dominant species in these factor profiles had high reactivities.Although the profile of biogenic emissions was substantially affected by photochemical loss of isoprene,the low emissions at nighttime also had an important impact on its profile.Chemical losses of highly active VOC species substantially reduced their concentrations in apportioned factor profiles.This study results were consistent with the analytical results obtained through initial concentration estimation,suggesting that the initial concentration estimation could be the most effective currently availablemethod for the source analyses of active VOCs although with uncertainty.展开更多
We report on the generation of dual-wavelength dissipative solitons in a passively mode-locked fibre laser with a net normal dispersion using the nonlinear polarization rotation （NPR） technique. Taking the intrinsic...We report on the generation of dual-wavelength dissipative solitons in a passively mode-locked fibre laser with a net normal dispersion using the nonlinear polarization rotation （NPR） technique. Taking the intrinsic advantage of the intracavity birefringence-induced spectral filtering effect in the NPR-based ring laser cavity, the dual-wavelength dissipative solitons are obtained. In addition, the wavelength separation and the lasing location of the dual-wavelength solitons can be flexibly tuned by changing the orientation of the polarization controller.展开更多
We use four-level atomic system and control the wave propagation via forbidden decay rate. The Raman gain process becomes dominant on electromagnetically induced transparency (EIT) medium by increasing the forbidden d...We use four-level atomic system and control the wave propagation via forbidden decay rate. The Raman gain process becomes dominant on electromagnetically induced transparency (EIT) medium by increasing the forbidden decay rate via increasing the number of atoms [G.S. Agarwal and T.N. Dey, Phys. Rev. A 74 (2005) 043805 and K. Harada, T. Kanbashi, and M. Mitsunaga, Phys. Rev. A 73 (2006) 013803]. The behavior of wave propagation is dramatically changed from normal (subluminal) to anomalous (superluminal) dispersion by increasing the forbidden decay rate. The system can also give a control over the group velocity of the light propagating through the medium via Kerr field.展开更多
The phase dependence and independence of the response of a trichromatieally driven two-level medium to an arbitrarily intense probe field have been studied. The sum of the relative phases of the sideband components of...The phase dependence and independence of the response of a trichromatieally driven two-level medium to an arbitrarily intense probe field have been studied. The sum of the relative phases of the sideband components of the trichromatic field compared to the central component plays a crucial role in the response of the medium. For a weak probe field, as the sum of the relative phases changes from 0 to π, multiple switching can be achieved, in which switching from normal to anomalous dispersion occurs in multiple separate frequency regimes. The remarkable dependence on the sum phase is also shown for a strong probe field. On the other hand, when the sum of the two relative phases is fixed, the changes in the respective phases have no influence on the response of the medium.展开更多
基金supported by the National Institute of Environmental Research(NIER)funded by the Ministry of Environment(No.NIER-2019-04-02-039)supported by Particulate Matter Management Specialized Graduate Program through the Korea Environmental Industry&Technology Institute(KEITI)funded by the Ministry of Environment(MOE).
文摘Fine particulatematter(PM_(2.5))samples were collected in two neighboring cities,Beijing and Baoding,China.High-concentration events of PM_(2.5) in which the average mass concentration exceeded 75μg/m^(3) were frequently observed during the heating season.Dispersion Normalized Positive Matrix Factorization was applied for the source apportionment of PM_(2.5) as minimize the dilution effects of meteorology and better reflect the source strengths in these two cities.Secondary nitrate had the highest contribution for Beijing(37.3%),and residential heating/biomass burning was the largest for Baoding(27.1%).Secondary nitrate,mobile,biomass burning,district heating,oil combustion,aged sea salt sources showed significant differences between the heating and non-heating seasons in Beijing for same period(2019.01.10–2019.08.22)(Mann-Whitney Rank Sum Test P<0.05).In case of Baoding,soil,residential heating/biomass burning,incinerator,coal combustion,oil combustion sources showed significant differences.The results of Pearson correlation analysis for the common sources between the two cities showed that long-range transported sources and some sources with seasonal patterns such as oil combustion and soil had high correlation coefficients.Conditional Bivariate Probability Function(CBPF)was used to identify the inflow directions for the sources,and joint-PSCF(Potential Source Contribution Function)was performed to determine the common potential source areas for sources affecting both cities.These models facilitated a more precise verification of city-specific influences on PM_(2.5) sources.The results of this study will aid in prioritizing air pollution mitigation strategies during the heating season and strengthening air quality management to reduce the impact of downwind neighboring cities.
基金supported by the Ministry of Environment,Forest and Climate Change(Mo Fand CC),Government of India,under the NCAP-COALESCE project(No.14/10/2014-CC(Vol.II))。
文摘Over the past decade,biomass burning has emerged as one of the main polluting events in northern India.It is one of the major sources of brown carbon(Br C),the light-absorbing organic carbon component of PM_(2.5).Most studies on the impact of biomass burning in India are based on source locations or urban areas;very little is known about its effects on a regional background location.We examine the effect of biomass burning on regional air quality and co-occurring meteorological factors.Year-long PM_(2.5)levels and light absorption by carbonaceous aerosols at 880 nm and 370 nm were measured at Rohtak,a regional background location.Results showed that post-harvest biomass burning in the Punjab-Haryana region affects the regional air quality with a lead of one to two days.A comparison of dispersionnormalized concentrations showed that open-field biomass burning not only affects regional air quality in the post-monsoon season(kharif crops)but is also a dominant source of PM_(2.5)in the post-harvest summer season(rabi crop).A significant(p<0.05)difference is observed in PM_(2.5),b_(abs-880),and b_(abs-370)between biomass burning days and non-biomass burning days during the kharif and rabi harvest seasons.Regression analyses confirm that in summer,regional PM_(2.5)and light absorption by aerosols are influenced more strongly by post-harvest burning of rabi crops.However,adverse meteorology plays a more dominant role in the post-monsoon season than biomass burning.These findings underscore the need for better policy interventions to curb biomass burning and improve air quality during both harvest seasons.
基金supported by the National Key R&D Program of China(No.2023YFC3705801)the National Natural Science Foundation of China(No.42177085).
文摘Substantial effects of photochemical reaction losses of volatile organic compounds(VOCs)on factor profiles can be investigated by comparing the differences between daytime and nighttime dispersion-normalized VOC data resolved profiles.Hourly speciated VOC data measured in Shijiazhuang,China from May to September 2021 were used to conduct study.The mean VOC concentration in the daytime and at nighttime were 32.8 and 36.0 ppbv,respectively.Alkanes and aromatics concentrations in the daytime(12.9 and 3.08 ppbv)were lower than nighttime(15.5 and 3.63 ppbv),whereas that of alkenes showed the opposite tendency.The concentration differences between daytime and nighttime for alkynes and halogenated hydrocarbonswere uniformly small.The reactivities of the dominant species in factor profiles for gasoline emissions,natural gas and diesel vehicles,and liquefied petroleum gas were relatively low and their profiles were less affected by photochemical losses.Photochemical losses produced a substantial impact on the profiles of solvent use,petrochemical industry emissions,combustion sources,and biogenic emissions where the dominant species in these factor profiles had high reactivities.Although the profile of biogenic emissions was substantially affected by photochemical loss of isoprene,the low emissions at nighttime also had an important impact on its profile.Chemical losses of highly active VOC species substantially reduced their concentrations in apportioned factor profiles.This study results were consistent with the analytical results obtained through initial concentration estimation,suggesting that the initial concentration estimation could be the most effective currently availablemethod for the source analyses of active VOCs although with uncertainty.
基金supported by the National Natural Science Foundation of China(Grant No.11074078)the Specialized Research Fund for the Doctoral Program of Higher Education,China(Grant No.20094407110002)+1 种基金the Foundation for Distinguished Young Talents in Higher Education of Guangdong,China(Grant No.C10183)the Key Program for Scientific and Technological Innovations of Higher Education Institutes in Guangdong Province,China(Grant No.cxzdlOll)
文摘We report on the generation of dual-wavelength dissipative solitons in a passively mode-locked fibre laser with a net normal dispersion using the nonlinear polarization rotation （NPR） technique. Taking the intrinsic advantage of the intracavity birefringence-induced spectral filtering effect in the NPR-based ring laser cavity, the dual-wavelength dissipative solitons are obtained. In addition, the wavelength separation and the lasing location of the dual-wavelength solitons can be flexibly tuned by changing the orientation of the polarization controller.
文摘We use four-level atomic system and control the wave propagation via forbidden decay rate. The Raman gain process becomes dominant on electromagnetically induced transparency (EIT) medium by increasing the forbidden decay rate via increasing the number of atoms [G.S. Agarwal and T.N. Dey, Phys. Rev. A 74 (2005) 043805 and K. Harada, T. Kanbashi, and M. Mitsunaga, Phys. Rev. A 73 (2006) 013803]. The behavior of wave propagation is dramatically changed from normal (subluminal) to anomalous (superluminal) dispersion by increasing the forbidden decay rate. The system can also give a control over the group velocity of the light propagating through the medium via Kerr field.
基金Project supported by the National Natural Science Foundation of China （Grant No 60378008）.
文摘The phase dependence and independence of the response of a trichromatieally driven two-level medium to an arbitrarily intense probe field have been studied. The sum of the relative phases of the sideband components of the trichromatic field compared to the central component plays a crucial role in the response of the medium. For a weak probe field, as the sum of the relative phases changes from 0 to π, multiple switching can be achieved, in which switching from normal to anomalous dispersion occurs in multiple separate frequency regimes. The remarkable dependence on the sum phase is also shown for a strong probe field. On the other hand, when the sum of the two relative phases is fixed, the changes in the respective phases have no influence on the response of the medium.
