In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to ...In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to obtain the maximal positive definite solution of nonlinear matrix equation X+A^(*)X|^(-α)A=Q with the case 0<α≤1.Based on this method,a new iterative algorithm is developed,and its convergence proof is given.Finally,two numerical examples are provided to show the effectiveness of the proposed method.展开更多
The goal of this paper is to investigate the long-time dynamics of solutions to a Kirchhoff type suspension bridge equation with nonlinear damping and memory term.For this problem we establish the well-posedness and e...The goal of this paper is to investigate the long-time dynamics of solutions to a Kirchhoff type suspension bridge equation with nonlinear damping and memory term.For this problem we establish the well-posedness and existence of uniform attractor under some suitable assumptions on the nonlinear term g(u),the nonlinear damping f(u_(t))and the external force h(x,t).Specifically,the asymptotic compactness of the semigroup is verified by the energy reconstruction method.展开更多
In this paper,we present a finite volume trigonometric weighted essentially non-oscillatory(TWENO)scheme to solve nonlinear degenerate parabolic equations that may exhibit non-smooth solutions.The present method is de...In this paper,we present a finite volume trigonometric weighted essentially non-oscillatory(TWENO)scheme to solve nonlinear degenerate parabolic equations that may exhibit non-smooth solutions.The present method is developed using the trigonometric scheme,which is based on zero,first,and second moments,and the direct discontinuous Galerkin(DDG)flux is used to discretize the diffusion term.Moreover,the DDG method directly applies the weak form of the parabolic equation to each computational cell,which can better capture the characteristics of the solution,especially the discontinuous solution.Meanwhile,the third-order TVD-Runge-Kutta method is applied for temporal discretization.Finally,the effectiveness and stability of the method constructed in this paper are evaluated through numerical tests.展开更多
Achieving non-centrosymmetric(NCS) configurations in ABX3-type hybrid halides remains a critical challenge for nonlinear optical(NLO) materials due to the conflicting requirements of high second-harmonic generation(SH...Achieving non-centrosymmetric(NCS) configurations in ABX3-type hybrid halides remains a critical challenge for nonlinear optical(NLO) materials due to the conflicting requirements of high second-harmonic generation(SHG) response,wide bandgap,and phase-matching capabilities.Herein,we propose a triplesite modulation strategy by synergistically tailoring the A-site cations(2-methylimidazole cation/1-ethyl-3-methylimidazole cation),B-site metals(Sn^(2+)/Pb^(2+)),and X-site halogens(Cl/Br),which effectively disrupts lattice symmetry and enables NCS crystallization.Our results demonstrate a strong SHG response,an expanded optical bandgap and increased birefringence.The optimized compound C_(6)H_(11)N_(2)PbCl_(3) exhibits a moderately strong SHG efficiency of 3.8 × KDP,a wide bandgap(3.87 eV),and enhanced birefringence(0.139@1064 nm),surpassing majority hybrid NLO materials.The innovative anionic framework introduced here broadens the scope of hybrid NLO crystals,facilitating the integration of various aromatic heterocyclic cations.This research provides a robust strategic framework for the development of advanced NLO materials.展开更多
Transforming urban spatial structures to promote green and low-carbon development is an effective strategy.Although prior studies have examined the impact of urban polycentricity on carbon emissions and economic devel...Transforming urban spatial structures to promote green and low-carbon development is an effective strategy.Although prior studies have examined the impact of urban polycentricity on carbon emissions and economic development,research on its role in the synergistic relationship between these factors regarding carbon emission efficiency is limited.Furthermore,existing literature often overlooks nonlinear effects and interactions with other urban variables.This paper analyzed data from 295 Chinese cities in 2020,calculating urban population polycentricity,population dispersion indices,and carbon emission efficiency.Utilizing local spatial autocorrelation tools,we reveal interactions among urban population polycentricity,dispersion,carbon emissions,and carbon emission efficiency.We then employ a gradient boosting decision tree model(GBDT)to explore nonlinear and synergistic effects of polycentric urbanization.Key findings include:1)polycentric urbanization in Chinese cities exhibits significant spatial differentiation characteristics.The Polycentricity index is relatively high in economically developed eastern coastal regions with an overall low level,carbon emissions are concentrated in industrialized north-central cities and some Yangtze River Delta hubs,and carbon emission efficiency is the highest in the Yangtze River Delta while relatively low in Northeast China;there are significant spatially heterogeneous interaction characteristics among population polycentricity,population dispersion,carbon emissions,and carbon emission efficiency.2)Urban population polycentricity contributes 9.42%to total carbon emissions and 6.24%to carbon emission efficiency.3)The polycentricity index has a nonlinear impact on carbon emissions and carbon emission efficiency:no significant effect when below 0.50 or above 0.55,increased carbon emissions in 0.50-0.53,and reduced carbon emissions with improved efficiency in 0.53-0.55.4)The polycentricity index has an interaction effect with other variables;specifically,when the polycentricity index is between 0.53 and 0.55,its interaction with urban gross domestic product(GDP),urban population,urban built-up area,green coverage rate in built-up areas,urban technological expenditure,and the proportion of the output value of the secondary industry will reduce carbon emissions and improve carbon emission efficiency.These findings enhance the understanding of urban spatial structures and carbon emissions,providing valuable insights for policymakers in developing green and low-carbon strategies.展开更多
The coupled chemo-mechanical impact of supercritical CO_(2)-H_(2)O(ScCO_(2)-H_(2)O)reactions on fracture geometry and nonlinear flow regimes in deep shale under confining pressures remains inadequately quantified.This...The coupled chemo-mechanical impact of supercritical CO_(2)-H_(2)O(ScCO_(2)-H_(2)O)reactions on fracture geometry and nonlinear flow regimes in deep shale under confining pressures remains inadequately quantified.This study systematically investigates the effects of ScCO_(2)-H_(2)O-shale interactions on fracture morphology and flow properties under confining pressures from 15 MPa to 40 MPa by integrating XRD(X-ray diffraction),micro-CT,3D surface profilometry,and multistage steady-state flow experiments.The results demonstrate that ScCO_(2)-H_(2)O exposure drives pyrite/feldspar dissolution and localized clay precipitation,resulting in fracture branching and macroscopic aperture regularization.Critically,confining pressure dictates the net hydraulic response:under low confining pressure(15-25 MPa),dissolution dominates,enhancing permeability,flow efficiency(Q/VP),and pre-linear flow behavior(n<1).At high confining pressures(30-40 MPa)mechanical compaction and mineral precipitation amplify flow resistance,shifting the flow regime toward quasi-linear behavior,as inertial effects become negligible compared to dominant viscous forces and increased flow resistance.Confining pressure thus critically mediates the dissolution-precipitation balance during ScCO_(2)-H_(2)O treatment,with an optimal window of 15-25 MPa identified for enhancing conductivity while minimizing clogging risk.These findings provide a quantitative framework for predicting stress-dependent flow evolution in chemically altered shale fractures.展开更多
In this work,the Hierarchical Quadrature Element Method(HQEM)formulation of geometrically exact shells is proposed and applied for geometrically nonlinear analyses of both isotropic and laminated shells.The stress res...In this work,the Hierarchical Quadrature Element Method(HQEM)formulation of geometrically exact shells is proposed and applied for geometrically nonlinear analyses of both isotropic and laminated shells.The stress resultant formulation is developed within the HQEM framework,consequently significantly simplifying the computations of residual force and stiffness matrix.The present formulation inherently avoids shear and membrane locking,benefiting from its high-order approximation property.Furthermore,HQEM’s independent nodal distribution capability conveniently supports local p-refinement and flexibly facilitates mesh generation in various structural configurations through the combination of quadrilateral and triangular elements.Remarkably,in lateral buckling analysis,the HQEM outperforms the weak-form quadrilateral element(QEM)in accuracy with identical nodal degrees of freedom(three displacements and two rotations).Under high-load nonlinear response,the QEM exhibits a maximum relative deviation of approximately 9.5%from the reference,while the HQEM remains closely aligned with the benchmark results.In addition,for the cantilever beam under tip moment,HQEM produces virtually no out-of-plane deviation,compared to a slight deviation of 0.00001 with QEM,confirming its superior numerical reliability.In summary,the method demonstrates high accuracy,superior convergence,and robustness in handling large rotations and complex post-buckling behaviors across a series of benchmark problems.展开更多
A nonlinear multi-scale interaction(NMI)model was proposed and developed by the first author for nearly 30 years to represent the evolution of atmospheric blocking.In this review paper,we first review the creation and...A nonlinear multi-scale interaction(NMI)model was proposed and developed by the first author for nearly 30 years to represent the evolution of atmospheric blocking.In this review paper,we first review the creation and development of the NMI model and then emphasize that the NMI model represents a new tool for identifying the basic physics of how climate change influences mid-to-high latitude weather extremes.The building of the NMI model took place over three main periods.In the 1990s,a nonlinear Schr?dinger(NLS)equation model was presented to describe atmospheric blocking as a wave packet;however,it could not depict the lifetime(10-20 days)of atmospheric blocking.In the 2000s,we proposed an NMI model of atmospheric blocking in a uniform basic flow by making a scale-separation assumption and deriving an eddyforced NLS equation.This model succeeded in describing the life cycle of atmospheric blocking.In the 2020s,the NMI model was extended to include the impact of a changing climate mainly by altering the basic zonal winds and the magnitude of the meridional background potential vorticity gradient(PVy).Model results show that when PVy is smaller,blocking has a weaker dispersion and a stronger nonlinearity,so blocking can be more persistent and have a larger zonal scale and weaker eastward movement,thus favoring stronger weather extremes.However,when PVy is much smaller and below a critical threshold under much stronger winter Arctic warming of global warming,atmospheric blocking becomes locally less persistent and shows a much stronger westward movement,which acts to inhibit local cold extremes.Such a case does not happen in summer under global warming because PVy fails to fall below the critical threshold.Thus,our theory indicates that global warming can render summer-blocking anticyclones and mid-to-high latitude heatwaves more persistent,intense,and widespread.展开更多
This paper investigates a multiplayer Pareto game for affine nonlinear stochastic systems disturbed by both external and the internal multiplicative noises.The Pareto cooperative optimal strategies with the H_(∞) con...This paper investigates a multiplayer Pareto game for affine nonlinear stochastic systems disturbed by both external and the internal multiplicative noises.The Pareto cooperative optimal strategies with the H_(∞) constraint are resolved by integrating H_(2)/H_(∞) theory with Pareto game theory.First,a nonlinear stochastic bounded real lemma(SBRL)is derived,explicitly accounting for non-zero initial conditions.Through the analysis of four cross-coupled Hamilton-Jacobi equations(HJEs),we establish necessary and sufficient conditions for the existence of Pareto optimal strategies with the H_(∞) constraint.Secondly,to address the complexity of solving these nonlinear partial differential HJEs,we propose a neural network(NN)framework with synchronous tuning rules for the actor,critic,and disturbance components,based on a reinforcement learning(RL)approach.The designed tuning rules ensure convergence of the actor-critic-disturbance components to the desired values,enabling the realization of robust Pareto control strategies.The convergence of the proposed algorithm is rigorously analyzed using a constructed Lyapunov function for the NN weight errors.Finally,a numerical simulation example is provided to demonstrate the effectiveness of the proposed methods and main results.展开更多
In this paper,we focus on peaked traveling wave solutions of the modified highly nonlinear Novikov equation by dynamical systems approach.We obtain a traveling wave system which is a singular planar dynamical system w...In this paper,we focus on peaked traveling wave solutions of the modified highly nonlinear Novikov equation by dynamical systems approach.We obtain a traveling wave system which is a singular planar dynamical system with three singular straight lines,and derive all possible phase portraits under corresponding parameter conditions.Then we show the existence and dynamics of two types of peaked traveling wave solutions including peakons and periodic cusp wave solutions.The exact explicit expressions of two peakons are given.Besides,we also derive smooth solitary wave solutions,periodic wave solutions,compacton solutions,and kink-like(antikink-like)solutions.Numerical simulations are further performed to verify the correctness of the results.Most importantly,peakons and periodic cusp wave solutions are newly found for the equation,which extends the previous results.展开更多
Due to scale effects,micromechanical resonators offer an excellent platform for investigating the intrinsic mechanisms of nonlinear dynamical phenomena and their potential applications.This review focuses on mode-coup...Due to scale effects,micromechanical resonators offer an excellent platform for investigating the intrinsic mechanisms of nonlinear dynamical phenomena and their potential applications.This review focuses on mode-coupled micromechanical resonators,highlighting the latest advancements in four key areas:internal resonance,synchronization,frequency combs,and mode localization.The origin,development,and potential applications of each of these dynamic phenomena within mode-coupled micromechanical systems are investigated,with the goal of inspiring new ideas and directions for researchers in this field.展开更多
In this paper,we mainly focus on a type of nonlinear Choquard equations with nonconstant potential.Under appropriate hypotheses on potential function and nonlinear terms,we prove that the above Choquard equation with ...In this paper,we mainly focus on a type of nonlinear Choquard equations with nonconstant potential.Under appropriate hypotheses on potential function and nonlinear terms,we prove that the above Choquard equation with prescribed 2-norm has some normalized solutions by introducing variational methods.展开更多
This article studies the existence and uniqueness of the mild solution of a family of control systems with a delay that are governed by the nonlinear fractional evolution differential equations in Banach spaces.Moreov...This article studies the existence and uniqueness of the mild solution of a family of control systems with a delay that are governed by the nonlinear fractional evolution differential equations in Banach spaces.Moreover,we establish the controllability of the considered system.To do so,first,we investigate the approximate controllability of the corresponding linear system.Subsequently,we prove the nonlinear system is approximately controllable if the corresponding linear system is approximately controllable.To reach the conclusions,the theory of resolvent operators,the Banach contraction mapping principle,and fixed point theorems are used.While concluding,some examples are given to demonstrate the efficacy of the proposed results.展开更多
In the modal analysis and control of nonlinear dynamical systems,participation factors(PFs)of state variables with respect to a critical or selected mode serve as a pivotal tool for simplifying stability studies by fo...In the modal analysis and control of nonlinear dynamical systems,participation factors(PFs)of state variables with respect to a critical or selected mode serve as a pivotal tool for simplifying stability studies by focusing on a subset of highly influential state variables.For linear systems,PFs are uniquely determined by the mode’s composition and shape,which are defined by the system’s left and right eigenvectors,respectively.However,the uniqueness of other types of PFs has not been thoroughly addressed in literatures.This paper establishes sufficient conditions for the uniqueness of nonlinear PFs and five other PF variants,taking into account uncertain scaling factors in a mode’s shape and composition.These scaling factors arise from variations in the choice of physical units,which depend on the value ranges of real-world state variables.Understanding these sufficient conditions is essential for the correct application of PFs in practical stability analysis and control design.展开更多
Due to the heterogeneity of rock masses and the variability of in situ stress,the traditional linear inversion method is insufficiently accurate to achieve high accuracy of the in situ stress field.To address this cha...Due to the heterogeneity of rock masses and the variability of in situ stress,the traditional linear inversion method is insufficiently accurate to achieve high accuracy of the in situ stress field.To address this challenge,nonlinear stress boundaries for a numerical model are determined through regression analysis of a series of nonlinear coefficient matrices,which are derived from the bubbling method.Considering the randomness and flexibility of the bubbling method,a parametric study is conducted to determine recommended ranges for these parameters,including the standard deviation(σb)of bubble radii,the non-uniform coefficient matrix number(λ)for nonlinear stress boundaries,and the number(m)and positions of in situ stress measurement points.A model case study provides a reference for the selection of these parameters.Additionally,when the nonlinear in situ stress inversion method is employed,stress distortion inevitably occurs near model boundaries,aligning with the Saint Venant's principle.Two strategies are proposed accordingly:employing a systematic reduction of nonlinear coefficients to achieve high inversion accuracy while minimizing significant stress distortion,and excluding regions with severe stress distortion near the model edges while utilizing the central part of the model for subsequent simulations.These two strategies have been successfully implemented in the nonlinear in situ stress inversion of the Xincheng Gold Mine and have achieved higher inversion accuracy than the linear method.Specifically,the linear and nonlinear inversion methods yield root mean square errors(RMSE)of 4.15 and 3.2,and inversion relative errors(δAve)of 22.08%and 17.55%,respectively.Therefore,the nonlinear inversion method outperforms the traditional multiple linear regression method,even in the presence of a systematic reduction in the nonlinear stress boundaries.展开更多
In this paper,a double-effect DNN-based Digital Back-Propagation(DBP)scheme is proposed and studied to achieve the Integrated Communication and Sensing(ICS)ability,which can not only realize nonlinear damage mitigatio...In this paper,a double-effect DNN-based Digital Back-Propagation(DBP)scheme is proposed and studied to achieve the Integrated Communication and Sensing(ICS)ability,which can not only realize nonlinear damage mitigation but also monitor the optical power and dispersion profile over multi-span links.The link status information can be extracted by the characteristics of the learned optical fiber parameters without any other measuring instruments.The efficiency and feasibility of this method have been investigated in different fiber link conditions,including various launch power,transmission distance,and the location and the amount of the abnormal losses.A good monitoring performance can be obtained while the launch optical power is 2 dBm which does not affect the normal operation of the optical communication system and the step size of DBP is 20 km which can provide a better distance resolution.This scheme successfully detects the location of single or multiple optical attenuators in long-distance multi-span fiber links,including different abnormal losses of 2 dB,4 dB,and 6 dB in 360 km and serval combinations of abnormal losses of(1 dB,5 dB),(3 dB,3 dB),(5 dB,1 dB)in 360 km and 760 km.Meanwhile,the transfer relationship of the estimated coefficient values with different step sizes is further investigated to reduce the complexity of the fiber nonlinear damage compensation.These results provide an attractive approach for precisely sensing the optical fiber link status information and making correct strategies timely to ensure optical communication system operations.展开更多
Herein,we report the synthesis and third-order nonlinear optical(NLO)properties of a novel cage-based 2D metal-organic framework constructed from Ti_(4)L_(6)(L4-=embonate)cage combined with Mg^(2+)and tris[4-(1H-imida...Herein,we report the synthesis and third-order nonlinear optical(NLO)properties of a novel cage-based 2D metal-organic framework constructed from Ti_(4)L_(6)(L4-=embonate)cage combined with Mg^(2+)and tris[4-(1H-imidazol-1-yl)phenyl]amine(tipa)ligand,whose molecular formula is(Me_(2)CH_(2))_(2)[Mg_(3)(Ti_(4)L_(6))(tipa)(H_(2)O)_(12)](PTC‑378).The Ti_(4)L_(6)tetrahedral cages serve as robust building units,while the Mg^(2+)ions and tipa ligands provide structural stability and tunable optical properties.The resulting PTC‑378 film exhibited intriguing third-order NLO property,which was systematically investigated using Z-scan techniques.Our results demonstrate that the synergistic interaction between Ti_(4)L_(6)cages andπ-conjugated ligands significantly enhances the NLO performance of the materials.CCDC:2453909.展开更多
In the near-infrared(NIR)spectroscopic data of complex sample systems,such as tobacco leaves,nonlinearity is fairly significant between the absorbance and concentration.This nonlinearity severely degrades the quantita...In the near-infrared(NIR)spectroscopic data of complex sample systems,such as tobacco leaves,nonlinearity is fairly significant between the absorbance and concentration.This nonlinearity severely degrades the quantitative results of traditional methods,such as partial least squares regression(PLS),which can be used to construct linear models.The problem was addressed in this study by using deep learning(DL).We employed three different DL models:a one-dimensional convolutional neural network(1D CNN),a deep neural network(DNN),and a stacked autoencoder with feedforward neural networks(SAE-FNNs).By carefully selecting and tuning the architectures and parameters of these models,we were able to find the most suitable model for dealing with such nonlinear relationships.Our experimental findings reveal that both the DNN and the SAE-FNN models excel in addressing the nonlinear issues of pectin concentration in tobacco,surpassing the performance of the classic linear model(PLS).Specifically,the DNN model stands out for its low average root mean squared error of prediction(RMSEP)value and small standard deviation(SD)of RMSEPs,leading to a tighter and more centered distribution of residuals in the prediction set.These DL models not only proficiently identify complex patterns within NIR data but also boast high prediction accuracy and fast implementation,demonstrating their effectiveness in analytical applications.展开更多
Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. Whe...Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. When the electromagnetic frequency is close to the cyclotron one, the linear conductivity increases two orders. Under the resonant frequencies nonlinearity becomes essential at low magnitudes of terahertz electric fields. In absence of a bias magnetic field the nonlinear dependences of the surface electric currents on terahertz electric field are practically the same simulated from kinetics and electron hydrodynamics with nonzero “kinetic” electron effective mass. Graphene possesses higher values of nonlinearity of the resonant conductivity, whereas in absence of a bias magnetic field, the electron nonlinearity is higher in silicene.展开更多
With the urgent need to resolve complex behaviors in nonlinear evolution equations,this study makes a contribution by establishing the local existence of solutions for Cauchy problems associated with equations of mixe...With the urgent need to resolve complex behaviors in nonlinear evolution equations,this study makes a contribution by establishing the local existence of solutions for Cauchy problems associated with equations of mixed types.Our primary contribution is the establishment of solution existence,illuminating the dynamics of these complex equations.To tackle this challenging problem,we construct an approximate solution sequence and apply the contraction mapping principle to rigorously prove local solution existence.Our results significantly advance the understanding of nonlinear evolution equations of mixed types.Furthermore,they provide a versatile,powerful approach for tackling analogous challenges across physics,engineering,and applied mathematics,making this work a valuable reference for researchers in these fields.展开更多
基金Supported in part by Natural Science Foundation of Guangxi(2023GXNSFAA026246)in part by the Central Government's Guide to Local Science and Technology Development Fund(GuikeZY23055044)in part by the National Natural Science Foundation of China(62363003)。
文摘In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to obtain the maximal positive definite solution of nonlinear matrix equation X+A^(*)X|^(-α)A=Q with the case 0<α≤1.Based on this method,a new iterative algorithm is developed,and its convergence proof is given.Finally,two numerical examples are provided to show the effectiveness of the proposed method.
基金Supported by the National Natural Science Foundation of China(Grant Nos.11961059,1210502)the University Innovation Project of Gansu Province(Grant No.2023B-062)the Gansu Province Basic Research Innovation Group Project(Grant No.23JRRA684).
文摘The goal of this paper is to investigate the long-time dynamics of solutions to a Kirchhoff type suspension bridge equation with nonlinear damping and memory term.For this problem we establish the well-posedness and existence of uniform attractor under some suitable assumptions on the nonlinear term g(u),the nonlinear damping f(u_(t))and the external force h(x,t).Specifically,the asymptotic compactness of the semigroup is verified by the energy reconstruction method.
基金The Natural Science Foundation of Xinjiang Uygur Autonomous Region of China“RBF-Hermite difference scheme for the time-fractional kdv-Burgers equation”(2024D01C43)。
文摘In this paper,we present a finite volume trigonometric weighted essentially non-oscillatory(TWENO)scheme to solve nonlinear degenerate parabolic equations that may exhibit non-smooth solutions.The present method is developed using the trigonometric scheme,which is based on zero,first,and second moments,and the direct discontinuous Galerkin(DDG)flux is used to discretize the diffusion term.Moreover,the DDG method directly applies the weak form of the parabolic equation to each computational cell,which can better capture the characteristics of the solution,especially the discontinuous solution.Meanwhile,the third-order TVD-Runge-Kutta method is applied for temporal discretization.Finally,the effectiveness and stability of the method constructed in this paper are evaluated through numerical tests.
基金supported by the National Natural Science Foundation of China (No.22275052)Department of Science and Technology of Hubei Province (Nos.2025AFA111 and 2024CSA076)。
文摘Achieving non-centrosymmetric(NCS) configurations in ABX3-type hybrid halides remains a critical challenge for nonlinear optical(NLO) materials due to the conflicting requirements of high second-harmonic generation(SHG) response,wide bandgap,and phase-matching capabilities.Herein,we propose a triplesite modulation strategy by synergistically tailoring the A-site cations(2-methylimidazole cation/1-ethyl-3-methylimidazole cation),B-site metals(Sn^(2+)/Pb^(2+)),and X-site halogens(Cl/Br),which effectively disrupts lattice symmetry and enables NCS crystallization.Our results demonstrate a strong SHG response,an expanded optical bandgap and increased birefringence.The optimized compound C_(6)H_(11)N_(2)PbCl_(3) exhibits a moderately strong SHG efficiency of 3.8 × KDP,a wide bandgap(3.87 eV),and enhanced birefringence(0.139@1064 nm),surpassing majority hybrid NLO materials.The innovative anionic framework introduced here broadens the scope of hybrid NLO crystals,facilitating the integration of various aromatic heterocyclic cations.This research provides a robust strategic framework for the development of advanced NLO materials.
基金Under the auspices of National Natural Science Foundation of China(No.42571300)。
文摘Transforming urban spatial structures to promote green and low-carbon development is an effective strategy.Although prior studies have examined the impact of urban polycentricity on carbon emissions and economic development,research on its role in the synergistic relationship between these factors regarding carbon emission efficiency is limited.Furthermore,existing literature often overlooks nonlinear effects and interactions with other urban variables.This paper analyzed data from 295 Chinese cities in 2020,calculating urban population polycentricity,population dispersion indices,and carbon emission efficiency.Utilizing local spatial autocorrelation tools,we reveal interactions among urban population polycentricity,dispersion,carbon emissions,and carbon emission efficiency.We then employ a gradient boosting decision tree model(GBDT)to explore nonlinear and synergistic effects of polycentric urbanization.Key findings include:1)polycentric urbanization in Chinese cities exhibits significant spatial differentiation characteristics.The Polycentricity index is relatively high in economically developed eastern coastal regions with an overall low level,carbon emissions are concentrated in industrialized north-central cities and some Yangtze River Delta hubs,and carbon emission efficiency is the highest in the Yangtze River Delta while relatively low in Northeast China;there are significant spatially heterogeneous interaction characteristics among population polycentricity,population dispersion,carbon emissions,and carbon emission efficiency.2)Urban population polycentricity contributes 9.42%to total carbon emissions and 6.24%to carbon emission efficiency.3)The polycentricity index has a nonlinear impact on carbon emissions and carbon emission efficiency:no significant effect when below 0.50 or above 0.55,increased carbon emissions in 0.50-0.53,and reduced carbon emissions with improved efficiency in 0.53-0.55.4)The polycentricity index has an interaction effect with other variables;specifically,when the polycentricity index is between 0.53 and 0.55,its interaction with urban gross domestic product(GDP),urban population,urban built-up area,green coverage rate in built-up areas,urban technological expenditure,and the proportion of the output value of the secondary industry will reduce carbon emissions and improve carbon emission efficiency.These findings enhance the understanding of urban spatial structures and carbon emissions,providing valuable insights for policymakers in developing green and low-carbon strategies.
基金support from the Science and Technology Innovation Program of Hunan Province(Grant No.2023RC1021)the Natural Science Foundation of Sichuan Province(Grant No.2025YFHZ0323).-。
文摘The coupled chemo-mechanical impact of supercritical CO_(2)-H_(2)O(ScCO_(2)-H_(2)O)reactions on fracture geometry and nonlinear flow regimes in deep shale under confining pressures remains inadequately quantified.This study systematically investigates the effects of ScCO_(2)-H_(2)O-shale interactions on fracture morphology and flow properties under confining pressures from 15 MPa to 40 MPa by integrating XRD(X-ray diffraction),micro-CT,3D surface profilometry,and multistage steady-state flow experiments.The results demonstrate that ScCO_(2)-H_(2)O exposure drives pyrite/feldspar dissolution and localized clay precipitation,resulting in fracture branching and macroscopic aperture regularization.Critically,confining pressure dictates the net hydraulic response:under low confining pressure(15-25 MPa),dissolution dominates,enhancing permeability,flow efficiency(Q/VP),and pre-linear flow behavior(n<1).At high confining pressures(30-40 MPa)mechanical compaction and mineral precipitation amplify flow resistance,shifting the flow regime toward quasi-linear behavior,as inertial effects become negligible compared to dominant viscous forces and increased flow resistance.Confining pressure thus critically mediates the dissolution-precipitation balance during ScCO_(2)-H_(2)O treatment,with an optimal window of 15-25 MPa identified for enhancing conductivity while minimizing clogging risk.These findings provide a quantitative framework for predicting stress-dependent flow evolution in chemically altered shale fractures.
基金supported by the National Natural Science Foundation of China(Grant Nos.12472194,12002018,11972004,11772031,11402015).
文摘In this work,the Hierarchical Quadrature Element Method(HQEM)formulation of geometrically exact shells is proposed and applied for geometrically nonlinear analyses of both isotropic and laminated shells.The stress resultant formulation is developed within the HQEM framework,consequently significantly simplifying the computations of residual force and stiffness matrix.The present formulation inherently avoids shear and membrane locking,benefiting from its high-order approximation property.Furthermore,HQEM’s independent nodal distribution capability conveniently supports local p-refinement and flexibly facilitates mesh generation in various structural configurations through the combination of quadrilateral and triangular elements.Remarkably,in lateral buckling analysis,the HQEM outperforms the weak-form quadrilateral element(QEM)in accuracy with identical nodal degrees of freedom(three displacements and two rotations).Under high-load nonlinear response,the QEM exhibits a maximum relative deviation of approximately 9.5%from the reference,while the HQEM remains closely aligned with the benchmark results.In addition,for the cantilever beam under tip moment,HQEM produces virtually no out-of-plane deviation,compared to a slight deviation of 0.00001 with QEM,confirming its superior numerical reliability.In summary,the method demonstrates high accuracy,superior convergence,and robustness in handling large rotations and complex post-buckling behaviors across a series of benchmark problems.
基金supported by the National Natural Science Foundation of China(Grant Nos.42150204 and 2288101)supported by the China National Postdoctoral Program for Innovative Talents(BX20230045)the China Postdoctoral Science Foundation(2023M730279)。
文摘A nonlinear multi-scale interaction(NMI)model was proposed and developed by the first author for nearly 30 years to represent the evolution of atmospheric blocking.In this review paper,we first review the creation and development of the NMI model and then emphasize that the NMI model represents a new tool for identifying the basic physics of how climate change influences mid-to-high latitude weather extremes.The building of the NMI model took place over three main periods.In the 1990s,a nonlinear Schr?dinger(NLS)equation model was presented to describe atmospheric blocking as a wave packet;however,it could not depict the lifetime(10-20 days)of atmospheric blocking.In the 2000s,we proposed an NMI model of atmospheric blocking in a uniform basic flow by making a scale-separation assumption and deriving an eddyforced NLS equation.This model succeeded in describing the life cycle of atmospheric blocking.In the 2020s,the NMI model was extended to include the impact of a changing climate mainly by altering the basic zonal winds and the magnitude of the meridional background potential vorticity gradient(PVy).Model results show that when PVy is smaller,blocking has a weaker dispersion and a stronger nonlinearity,so blocking can be more persistent and have a larger zonal scale and weaker eastward movement,thus favoring stronger weather extremes.However,when PVy is much smaller and below a critical threshold under much stronger winter Arctic warming of global warming,atmospheric blocking becomes locally less persistent and shows a much stronger westward movement,which acts to inhibit local cold extremes.Such a case does not happen in summer under global warming because PVy fails to fall below the critical threshold.Thus,our theory indicates that global warming can render summer-blocking anticyclones and mid-to-high latitude heatwaves more persistent,intense,and widespread.
基金supported by the National Natural Science Foundation of China(12426609,62203220,62373229)the Taishan Scholar Project Foundation of Shandong Province(tsqnz20230619,tsqn202408110)+2 种基金the Fundamental Research Foundation of the Central Universities(23Cx06024A)the Natural Science Foundation of Shandong Province(ZR2024QF096)the Outstanding Youth Innovation Team in Shandong Higher Education Institutions(2023KJ061).
文摘This paper investigates a multiplayer Pareto game for affine nonlinear stochastic systems disturbed by both external and the internal multiplicative noises.The Pareto cooperative optimal strategies with the H_(∞) constraint are resolved by integrating H_(2)/H_(∞) theory with Pareto game theory.First,a nonlinear stochastic bounded real lemma(SBRL)is derived,explicitly accounting for non-zero initial conditions.Through the analysis of four cross-coupled Hamilton-Jacobi equations(HJEs),we establish necessary and sufficient conditions for the existence of Pareto optimal strategies with the H_(∞) constraint.Secondly,to address the complexity of solving these nonlinear partial differential HJEs,we propose a neural network(NN)framework with synchronous tuning rules for the actor,critic,and disturbance components,based on a reinforcement learning(RL)approach.The designed tuning rules ensure convergence of the actor-critic-disturbance components to the desired values,enabling the realization of robust Pareto control strategies.The convergence of the proposed algorithm is rigorously analyzed using a constructed Lyapunov function for the NN weight errors.Finally,a numerical simulation example is provided to demonstrate the effectiveness of the proposed methods and main results.
基金Supported by the National Natural Science Foundation of China(12071162)the Natural Science Foundation of Fujian Province(2021J01302)the Fundamental Research Funds for the Central Universities(ZQN-802).
文摘In this paper,we focus on peaked traveling wave solutions of the modified highly nonlinear Novikov equation by dynamical systems approach.We obtain a traveling wave system which is a singular planar dynamical system with three singular straight lines,and derive all possible phase portraits under corresponding parameter conditions.Then we show the existence and dynamics of two types of peaked traveling wave solutions including peakons and periodic cusp wave solutions.The exact explicit expressions of two peakons are given.Besides,we also derive smooth solitary wave solutions,periodic wave solutions,compacton solutions,and kink-like(antikink-like)solutions.Numerical simulations are further performed to verify the correctness of the results.Most importantly,peakons and periodic cusp wave solutions are newly found for the equation,which extends the previous results.
基金supported by the National Key Research and Development Program of China(No.2022YFB3203600)the National Natural Science Foundation of China(Nos.12202355,12132013,and 12172323)the Zhejiang Provincial Natural Science Foundation of China(No.LZ22A020003)。
文摘Due to scale effects,micromechanical resonators offer an excellent platform for investigating the intrinsic mechanisms of nonlinear dynamical phenomena and their potential applications.This review focuses on mode-coupled micromechanical resonators,highlighting the latest advancements in four key areas:internal resonance,synchronization,frequency combs,and mode localization.The origin,development,and potential applications of each of these dynamic phenomena within mode-coupled micromechanical systems are investigated,with the goal of inspiring new ideas and directions for researchers in this field.
基金Supported by the National Natural Science Foundation of China(11671403,11671236,12101192)Henan Provincial General Natural Science Foundation Project(232300420113)。
文摘In this paper,we mainly focus on a type of nonlinear Choquard equations with nonconstant potential.Under appropriate hypotheses on potential function and nonlinear terms,we prove that the above Choquard equation with prescribed 2-norm has some normalized solutions by introducing variational methods.
文摘This article studies the existence and uniqueness of the mild solution of a family of control systems with a delay that are governed by the nonlinear fractional evolution differential equations in Banach spaces.Moreover,we establish the controllability of the considered system.To do so,first,we investigate the approximate controllability of the corresponding linear system.Subsequently,we prove the nonlinear system is approximately controllable if the corresponding linear system is approximately controllable.To reach the conclusions,the theory of resolvent operators,the Banach contraction mapping principle,and fixed point theorems are used.While concluding,some examples are given to demonstrate the efficacy of the proposed results.
文摘In the modal analysis and control of nonlinear dynamical systems,participation factors(PFs)of state variables with respect to a critical or selected mode serve as a pivotal tool for simplifying stability studies by focusing on a subset of highly influential state variables.For linear systems,PFs are uniquely determined by the mode’s composition and shape,which are defined by the system’s left and right eigenvectors,respectively.However,the uniqueness of other types of PFs has not been thoroughly addressed in literatures.This paper establishes sufficient conditions for the uniqueness of nonlinear PFs and five other PF variants,taking into account uncertain scaling factors in a mode’s shape and composition.These scaling factors arise from variations in the choice of physical units,which depend on the value ranges of real-world state variables.Understanding these sufficient conditions is essential for the correct application of PFs in practical stability analysis and control design.
基金funded by the National Key R&D Program of China(Grant No.2022YFC2903904)the National Natural Science Foundation of China(Grant Nos.51904057 and U1906208).
文摘Due to the heterogeneity of rock masses and the variability of in situ stress,the traditional linear inversion method is insufficiently accurate to achieve high accuracy of the in situ stress field.To address this challenge,nonlinear stress boundaries for a numerical model are determined through regression analysis of a series of nonlinear coefficient matrices,which are derived from the bubbling method.Considering the randomness and flexibility of the bubbling method,a parametric study is conducted to determine recommended ranges for these parameters,including the standard deviation(σb)of bubble radii,the non-uniform coefficient matrix number(λ)for nonlinear stress boundaries,and the number(m)and positions of in situ stress measurement points.A model case study provides a reference for the selection of these parameters.Additionally,when the nonlinear in situ stress inversion method is employed,stress distortion inevitably occurs near model boundaries,aligning with the Saint Venant's principle.Two strategies are proposed accordingly:employing a systematic reduction of nonlinear coefficients to achieve high inversion accuracy while minimizing significant stress distortion,and excluding regions with severe stress distortion near the model edges while utilizing the central part of the model for subsequent simulations.These two strategies have been successfully implemented in the nonlinear in situ stress inversion of the Xincheng Gold Mine and have achieved higher inversion accuracy than the linear method.Specifically,the linear and nonlinear inversion methods yield root mean square errors(RMSE)of 4.15 and 3.2,and inversion relative errors(δAve)of 22.08%and 17.55%,respectively.Therefore,the nonlinear inversion method outperforms the traditional multiple linear regression method,even in the presence of a systematic reduction in the nonlinear stress boundaries.
基金supported by the National Key Research and Development Program of China (2019YFB1803905)the National Natural Science Foundation of China (No.62171022)+2 种基金Beijing Natural Science Foundation (4222009)Guangdong Basic and Applied Basic Research Foundation (2021B1515120057)the Scientific and Technological Innovation Foundation of Shunde Graduate School,USTB (No.BK19AF005)。
文摘In this paper,a double-effect DNN-based Digital Back-Propagation(DBP)scheme is proposed and studied to achieve the Integrated Communication and Sensing(ICS)ability,which can not only realize nonlinear damage mitigation but also monitor the optical power and dispersion profile over multi-span links.The link status information can be extracted by the characteristics of the learned optical fiber parameters without any other measuring instruments.The efficiency and feasibility of this method have been investigated in different fiber link conditions,including various launch power,transmission distance,and the location and the amount of the abnormal losses.A good monitoring performance can be obtained while the launch optical power is 2 dBm which does not affect the normal operation of the optical communication system and the step size of DBP is 20 km which can provide a better distance resolution.This scheme successfully detects the location of single or multiple optical attenuators in long-distance multi-span fiber links,including different abnormal losses of 2 dB,4 dB,and 6 dB in 360 km and serval combinations of abnormal losses of(1 dB,5 dB),(3 dB,3 dB),(5 dB,1 dB)in 360 km and 760 km.Meanwhile,the transfer relationship of the estimated coefficient values with different step sizes is further investigated to reduce the complexity of the fiber nonlinear damage compensation.These results provide an attractive approach for precisely sensing the optical fiber link status information and making correct strategies timely to ensure optical communication system operations.
文摘Herein,we report the synthesis and third-order nonlinear optical(NLO)properties of a novel cage-based 2D metal-organic framework constructed from Ti_(4)L_(6)(L4-=embonate)cage combined with Mg^(2+)and tris[4-(1H-imidazol-1-yl)phenyl]amine(tipa)ligand,whose molecular formula is(Me_(2)CH_(2))_(2)[Mg_(3)(Ti_(4)L_(6))(tipa)(H_(2)O)_(12)](PTC‑378).The Ti_(4)L_(6)tetrahedral cages serve as robust building units,while the Mg^(2+)ions and tipa ligands provide structural stability and tunable optical properties.The resulting PTC‑378 film exhibited intriguing third-order NLO property,which was systematically investigated using Z-scan techniques.Our results demonstrate that the synergistic interaction between Ti_(4)L_(6)cages andπ-conjugated ligands significantly enhances the NLO performance of the materials.CCDC:2453909.
基金supported by a joint project with SINOPEC(Dalian)Research Institute of Petroleum and Petrochemicals Co.,Ltd.(Contract No.323061).
文摘In the near-infrared(NIR)spectroscopic data of complex sample systems,such as tobacco leaves,nonlinearity is fairly significant between the absorbance and concentration.This nonlinearity severely degrades the quantitative results of traditional methods,such as partial least squares regression(PLS),which can be used to construct linear models.The problem was addressed in this study by using deep learning(DL).We employed three different DL models:a one-dimensional convolutional neural network(1D CNN),a deep neural network(DNN),and a stacked autoencoder with feedforward neural networks(SAE-FNNs).By carefully selecting and tuning the architectures and parameters of these models,we were able to find the most suitable model for dealing with such nonlinear relationships.Our experimental findings reveal that both the DNN and the SAE-FNN models excel in addressing the nonlinear issues of pectin concentration in tobacco,surpassing the performance of the classic linear model(PLS).Specifically,the DNN model stands out for its low average root mean squared error of prediction(RMSEP)value and small standard deviation(SD)of RMSEPs,leading to a tighter and more centered distribution of residuals in the prediction set.These DL models not only proficiently identify complex patterns within NIR data but also boast high prediction accuracy and fast implementation,demonstrating their effectiveness in analytical applications.
文摘Resonant linear and nonlinear properties in terahertz range of 2D materials graphene and silicene placed into a bias magnetic field are investigated theoretically on the base of the quasi-classical kinetic theory. When the electromagnetic frequency is close to the cyclotron one, the linear conductivity increases two orders. Under the resonant frequencies nonlinearity becomes essential at low magnitudes of terahertz electric fields. In absence of a bias magnetic field the nonlinear dependences of the surface electric currents on terahertz electric field are practically the same simulated from kinetics and electron hydrodynamics with nonzero “kinetic” electron effective mass. Graphene possesses higher values of nonlinearity of the resonant conductivity, whereas in absence of a bias magnetic field, the electron nonlinearity is higher in silicene.
基金Supported by the National Natural Science Foundation of China(12201368,62376252)Key Project of Natural Science Foundation of Zhejiang Province(LZ22F030003)Zhejiang Province Leading Geese Plan(2024C02G1123882,2024C01SA100795).
文摘With the urgent need to resolve complex behaviors in nonlinear evolution equations,this study makes a contribution by establishing the local existence of solutions for Cauchy problems associated with equations of mixed types.Our primary contribution is the establishment of solution existence,illuminating the dynamics of these complex equations.To tackle this challenging problem,we construct an approximate solution sequence and apply the contraction mapping principle to rigorously prove local solution existence.Our results significantly advance the understanding of nonlinear evolution equations of mixed types.Furthermore,they provide a versatile,powerful approach for tackling analogous challenges across physics,engineering,and applied mathematics,making this work a valuable reference for researchers in these fields.
