Ultrafast lasers play an important role in a variety of applications ranging from optical communications to medical diagnostics and industrial materials processing. Graphene and other two-dimensional（2D） noncarbon m...Ultrafast lasers play an important role in a variety of applications ranging from optical communications to medical diagnostics and industrial materials processing. Graphene and other two-dimensional（2D） noncarbon materials, including topological insulators（TIs）, transition metal dichalcogenides（TMDCs）, phosphorene, bismuthene, and antimonene, have witnessed a very fast development of both fundamental and practical aspects in ultrafast photonics since 2009. Their unique nonlinear optical properties enable them to be used as excellent saturable absorbers（SAs） that have fast responses and broadband operation, and can be easily integrated into lasers. Here, we catalog and review recent progress in the exploitation of these 2D noncarbon materials in this emerging field. The fabrication techniques, nonlinear optical properties, and device integration strategies of 2D noncarbon materials are first introduced with a comprehensive view. Then, various mode-locked/Q-switched lasers（e.g., fiber, solid-state, disk, and waveguide lasers） based on 2D noncarbon materials are reviewed. In addition, versatile soliton pulses generated from the mode-locked fiber lasers based on 2D noncarbon materials are also summarized. Finally, future challenges and perspectives of 2D materials-based lasers are addressed.展开更多
We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient second-and third-order nonlinear optical processes in the lattice-matched undoped(GaP)N/(Si 2)M short-period superlattice that...We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient second-and third-order nonlinear optical processes in the lattice-matched undoped(GaP)N/(Si 2)M short-period superlattice that is waveguide-integrated in a microring resonator on an opto-electronic chip.The nonlinear superlattice structures are sit-uated on the optically pumped input area of a heterogeneous“XOI”chip based on silicon.The spectra ofχ(2)zzz(2ω,ω,ω),χ(2)xzx(2ω,ω,ω),χ(3)xxxx(3ω,ω,ω,ω)and the Kerr refractive index(n 2),have been simu-lated as a function of the number of the atomic monolayers for“non-relaxed”heterointerfaces;These nonlinearities are induced by transi-tions between valence and conduction bands.The large obtained val-ues make the(GaP)N/(Si 2)M short-period superlattice a good can-didate for future high-performance XOI photonic integrated chips that may include Si 3 N 4 or SiC or AlGaAs or Si.Near or at the 810-nm and 1550-nm wavelengths,we have made detailed calculations of the efficiency of second-and third-harmonic generation as well as the performances of entangled photon-pair quantum sources that are based upon spontaneous parametric down conversion and sponta-neous four-wave mixing.The results indicate that the(GaP)N/(Si 2)M short-period superlattice is competitive with present technologies and is practical for classical and quantum applications.展开更多
Two-dimensional transition metal dichalcogenides are of great interest for second harmonic generation due to their large second-order susceptibilityx(2),atomically thin structure,and relaxed phase-matching conditions....Two-dimensional transition metal dichalcogenides are of great interest for second harmonic generation due to their large second-order susceptibilityx(2),atomically thin structure,and relaxed phase-matching conditions.Such materials are also promising candidates for miniaturizing nonlinear optical devices for versatile applications in photon manipulation,quantum emission and sensing,and nanophotonic circuits.However,their strong sec-ond harmonic response is limited by nanometer-scale light-matter interaction and material impurities.Although there is considerable work toward engineering these materials for enhancing their nonlinear responses,all-optical methods are still in the exploration stages.We incorporate,to the best of our knowledge,the first experimental demonstration of feedback-based wavefront shaping techniques in atomically thin media to reveal and enhance the weak second harmonic generation of monolayer WS_(2).Phase tuning of the incident wavefront leads to the increase in the intensity of the second harmonic generated in the target regions up to an order of magnitude.We enhance the local nonlinear signal conversion from monolayer WS_(2)up to 41 x using phase-only modulation.Furthermore,by introducing a shift in the transverse phase structure,we achieve observable second harmonic generation at the destructively interfering grain boundaries of polycrystalline monolayers.This method allows for all-optical tuning of transition metal dichalcogenides'nonlinear responses,opening up possibilities for dynamic signal routing and on-demand enhancement in nanoscale photonic systems.展开更多
We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient electric-field-induced three-waves mixing(EFIM)in an undoped lattice-matched short-period superlattice(SL)that integrates quas...We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient electric-field-induced three-waves mixing(EFIM)in an undoped lattice-matched short-period superlattice(SL)that integrates quasi-phase-matched(QPM)SL straight waveguides and SL racetrack resonators on an opto-electronic chip.Periodically reversed DC voltage is applied to electrode segments on each side of the strip waveguide.The spectra ofχ_(xxxx)^((3))and of the linear suscepti-bility have been simulated as a function of the number of the atomic monolayers for“non-relaxed”heterointerfaces,and by considering all the transitions between valence and conduction bands.The large ob-tained values ofχ_(xxxx)^((3))make the(ZnS)3/(Si2)3 short-period SL a good candidate for realizing large effective second-order nonlinearity,en-abling future high-performance of the SLOI PICs and OEICs in the 1000-nm and 2000-nm wavelengths ranges.We have made detailed calculations of the efficiency of second-harmonic generation and of the performances of the optical parametric oscillator(OPO).The re-sults indicate that the(ZnS)N/(Si2)M QPM is competitive with present PPLN technologies and is practical for classical and quantum appli-cations.展开更多
We investigate the mechanisms to realize the Raman laser switching in a silica rod microresonator with mode-interactionassisted excitation.The laser switching can be triggered between two whispering gallery modes[WGMs...We investigate the mechanisms to realize the Raman laser switching in a silica rod microresonator with mode-interactionassisted excitation.The laser switching can be triggered between two whispering gallery modes[WGMs]with either the same or distinct mode families,depending on the pumping conditions.The experimental observations are in excellent agreement with a theoretical analysis based on coupled-mode equations with intermodal interaction terms involved.Additionally,we also demonstrate switching of a single-mode Raman laser and a wideband spectral tuning range up to~32.67 nm by selective excitation of distinct mode sequences.The results contribute to the understanding of Raman lasing formation dynamics via interaction with transverse mode sequences and may extend the microcavity-based Raman microlasers to potential areas in switchable light sources,optical memories,and high sensitivity sensors.展开更多
基金supported by the Program for Equipment Pre-research Field Funds(No.6140414040116CB01012)the National Natural Science Foundation of China(Nos.61575051 and 11704086)the 111 project of the Harbin Engineering University(No.B13015)
文摘Ultrafast lasers play an important role in a variety of applications ranging from optical communications to medical diagnostics and industrial materials processing. Graphene and other two-dimensional（2D） noncarbon materials, including topological insulators（TIs）, transition metal dichalcogenides（TMDCs）, phosphorene, bismuthene, and antimonene, have witnessed a very fast development of both fundamental and practical aspects in ultrafast photonics since 2009. Their unique nonlinear optical properties enable them to be used as excellent saturable absorbers（SAs） that have fast responses and broadband operation, and can be easily integrated into lasers. Here, we catalog and review recent progress in the exploitation of these 2D noncarbon materials in this emerging field. The fabrication techniques, nonlinear optical properties, and device integration strategies of 2D noncarbon materials are first introduced with a comprehensive view. Then, various mode-locked/Q-switched lasers（e.g., fiber, solid-state, disk, and waveguide lasers） based on 2D noncarbon materials are reviewed. In addition, versatile soliton pulses generated from the mode-locked fiber lasers based on 2D noncarbon materials are also summarized. Finally, future challenges and perspectives of 2D materials-based lasers are addressed.
基金The work of Richard Soref is supported by the Air Force Office of Scientific Research under Grant FA9550-21-1-0347.
文摘We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient second-and third-order nonlinear optical processes in the lattice-matched undoped(GaP)N/(Si 2)M short-period superlattice that is waveguide-integrated in a microring resonator on an opto-electronic chip.The nonlinear superlattice structures are sit-uated on the optically pumped input area of a heterogeneous“XOI”chip based on silicon.The spectra ofχ(2)zzz(2ω,ω,ω),χ(2)xzx(2ω,ω,ω),χ(3)xxxx(3ω,ω,ω,ω)and the Kerr refractive index(n 2),have been simu-lated as a function of the number of the atomic monolayers for“non-relaxed”heterointerfaces;These nonlinearities are induced by transi-tions between valence and conduction bands.The large obtained val-ues make the(GaP)N/(Si 2)M short-period superlattice a good can-didate for future high-performance XOI photonic integrated chips that may include Si 3 N 4 or SiC or AlGaAs or Si.Near or at the 810-nm and 1550-nm wavelengths,we have made detailed calculations of the efficiency of second-and third-harmonic generation as well as the performances of entangled photon-pair quantum sources that are based upon spontaneous parametric down conversion and sponta-neous four-wave mixing.The results indicate that the(GaP)N/(Si 2)M short-period superlattice is competitive with present technologies and is practical for classical and quantum applications.
基金Gordon and Betty Moore FoundationU.S.Department of Energy(DE-SC0024676)+2 种基金National Geospatial-Intelligence Agency(HM04762010012)U.S.Department of Energy(DE-SC0023148)Air Force Office of Scientific Research(FA9550-23-1-0325).
文摘Two-dimensional transition metal dichalcogenides are of great interest for second harmonic generation due to their large second-order susceptibilityx(2),atomically thin structure,and relaxed phase-matching conditions.Such materials are also promising candidates for miniaturizing nonlinear optical devices for versatile applications in photon manipulation,quantum emission and sensing,and nanophotonic circuits.However,their strong sec-ond harmonic response is limited by nanometer-scale light-matter interaction and material impurities.Although there is considerable work toward engineering these materials for enhancing their nonlinear responses,all-optical methods are still in the exploration stages.We incorporate,to the best of our knowledge,the first experimental demonstration of feedback-based wavefront shaping techniques in atomically thin media to reveal and enhance the weak second harmonic generation of monolayer WS_(2).Phase tuning of the incident wavefront leads to the increase in the intensity of the second harmonic generated in the target regions up to an order of magnitude.We enhance the local nonlinear signal conversion from monolayer WS_(2)up to 41 x using phase-only modulation.Furthermore,by introducing a shift in the transverse phase structure,we achieve observable second harmonic generation at the destructively interfering grain boundaries of polycrystalline monolayers.This method allows for all-optical tuning of transition metal dichalcogenides'nonlinear responses,opening up possibilities for dynamic signal routing and on-demand enhancement in nanoscale photonic systems.
基金supported by the Air Force Office of Scientific Research under Grant FA9550-21-1-0347.
文摘We present a theoretical investigation,based on the tight-binding Hamiltonian,of efficient electric-field-induced three-waves mixing(EFIM)in an undoped lattice-matched short-period superlattice(SL)that integrates quasi-phase-matched(QPM)SL straight waveguides and SL racetrack resonators on an opto-electronic chip.Periodically reversed DC voltage is applied to electrode segments on each side of the strip waveguide.The spectra ofχ_(xxxx)^((3))and of the linear suscepti-bility have been simulated as a function of the number of the atomic monolayers for“non-relaxed”heterointerfaces,and by considering all the transitions between valence and conduction bands.The large ob-tained values ofχ_(xxxx)^((3))make the(ZnS)3/(Si2)3 short-period SL a good candidate for realizing large effective second-order nonlinearity,en-abling future high-performance of the SLOI PICs and OEICs in the 1000-nm and 2000-nm wavelengths ranges.We have made detailed calculations of the efficiency of second-harmonic generation and of the performances of the optical parametric oscillator(OPO).The re-sults indicate that the(ZnS)N/(Si2)M QPM is competitive with present PPLN technologies and is practical for classical and quantum appli-cations.
基金supported by the National Natural Science Foundation of China(No.62005071)the Natural Science Foundation of Anhui Province(No.2008085QF312)+1 种基金the Fundamental Research Funds for the Central Universities(No.JZ2021HGTB0079)the National Key Research and Development Program of China(No.2019YFE010747)。
文摘We investigate the mechanisms to realize the Raman laser switching in a silica rod microresonator with mode-interactionassisted excitation.The laser switching can be triggered between two whispering gallery modes[WGMs]with either the same or distinct mode families,depending on the pumping conditions.The experimental observations are in excellent agreement with a theoretical analysis based on coupled-mode equations with intermodal interaction terms involved.Additionally,we also demonstrate switching of a single-mode Raman laser and a wideband spectral tuning range up to~32.67 nm by selective excitation of distinct mode sequences.The results contribute to the understanding of Raman lasing formation dynamics via interaction with transverse mode sequences and may extend the microcavity-based Raman microlasers to potential areas in switchable light sources,optical memories,and high sensitivity sensors.
