We investigate the alpha helical protein structure characterized by fourth-order interspine coupling,focusing on a three-coupled fourth-order nonlinear Schr??dinger system.We introduce a generalized Darboux transforma...We investigate the alpha helical protein structure characterized by fourth-order interspine coupling,focusing on a three-coupled fourth-order nonlinear Schr??dinger system.We introduce a generalized Darboux transformation,departing from the classical Darboux transformation.Based on this,we construct the two-and three-degenerate soliton solutions and four-degenerate asymptotic soliton solutions.Based on the asymptotic analysis,we find that the amplitudes of interacting solitons are retained upon the interactions.Elastic interactions between two degenerate solitons exhibiting four curve-type asymptotic solitons are depicted.When the lattice parameterβchanges,the velocities of the two degenerate solitons also change.Elastic interaction among three degenerate solitons comprising four curve-type asymptotic solitons and two line-type solitons is presented.Interaction among one soliton and two degenerate solitons with different velocities is shown.Elastic interaction among four degenerate solitons comprising eight curve-type asymptotic solitons is also presented.Interaction among two two-degenerate solitons with two spectral parameters is shown.The relative distance between two asymptotic solitons exhibits logarithmic growth with|t|,where t represents the retarded time.Acceleration of soliton separation decays exponentially with relative distance,and eventually approaches zero.Phase shifts depend on t.展开更多
Traditional dynamic analysis of mechanical structures,often limited to individual beams or plates,fails to fully capture their dynamic behaviors.In systems where space and mass are constrained,such as the battery supp...Traditional dynamic analysis of mechanical structures,often limited to individual beams or plates,fails to fully capture their dynamic behaviors.In systems where space and mass are constrained,such as the battery support structures in electric aircraft,conventional absorbers and isolators are insufficient for effective vibration control.This study simplifies the battery support structure of electric aircraft as an integrated composite beam consisting of three interconnected beams,and investigated its structural dynamics properties and nonlinear vibration control under thermal conditions caused by battery heat.The nonlinear vibration control is performed using the Nitinol steel wire ropes(Ni Ti-ST),with nonlinear damping properties.The natural frequencies of system are determined using the Rayleigh-Ritz technique.Theoretical results are validated through both Finite Element Method(FEM)and hammer tests.Moreover,the dynamic equations are derived using the Lagrange method and discretized via the Galerkin Truncation Method(GTM).The Harmonic Balance Method(HBM)is used to evaluate the vibration responses of the integrated model,with further verification through the Runge-Kutta Method(RKM).The experiments are conducted to corroborate the theoretical analysis.The results show that the system frequency changes in stages with the increase of the stiffness of the integrated composite beam connection.Especially in the case of varying environments,as the temperature increases,the frequency of system will first increase to a certain maximum value and then gradually decrease.Furthermore,the NiTi-ST effectively reduces vibration in the integrated composite beam,particularly under varying temperatures and external excitations.展开更多
Honeycomb structures of shape memory alloy(SMA)have become one of the most promising materials for flexible skins of morphing aircraft due to their excellent mechanical properties.However,due to the nonlinear material...Honeycomb structures of shape memory alloy(SMA)have become one of the most promising materials for flexible skins of morphing aircraft due to their excellent mechanical properties.However,due to the nonlinear material and geometric large deformation,the SMA honeycomb exhibits significant and complex nonlinearity in the skin and there is a lack of relevant previous research.In this paper,the nonlinear properties of the SMA honeycomb structure with arbitrary geometry are investigated for the first time for large deformation flexible skin applications by theoretical and experimental analysis.Firstly,a novel theoretical model of SMA honeycomb structure considering both material and geometric nonlinearity is proposed,and the corresponding calculation method of nonlinear governing equations is given based upon the shooting method and Runge–Kutta method.Then,the tensile behaviors of four kinds of SMA honeycomb structures,i.e.,U-type,V-type,cosine-type,and trapezoid-type,are analyzed and predicted by the proposed theoretical model and compared with the finite element analysis(FEA)results.Moreover,the tensile experiments were carried out by stretching U-type and V-type honeycomb structures to a global strain of 60%and 40%,respectively,to perform large deformation analysis and verify the theoretical model.Finally,experimental verification and finite element validation show that the curves of the theoretical model results,experimental results,and simulation results are in good agreement,illustrating the generalizability and accuracy of the proposed theoretical model.The theoretical model and experimental investigations in this paper are considered to provide an effective foundation for analyzing and predicting the mechanical behavior of SMA honeycomb flexible skins with large extensional deformations.展开更多
Radial rotating oscillating heat pipes(R-OHPs)have excellent thermal performance and great potential for application in the thermal management of rotatory machinery.However,the heat transport behavior and temperature ...Radial rotating oscillating heat pipes(R-OHPs)have excellent thermal performance and great potential for application in the thermal management of rotatory machinery.However,the heat transport behavior and temperature characteristics of R-OHPs are complex,and their understanding is still limited,hence necessitating further research.In this study,thanks to an experimental investigation involving a copper R-OHP running with acetone and water,its thermal performance is evaluated,and then the temperature characteristics are analyzed by nonlinear dynamic analysis.The study reveals that the effective heat transfer coefficient of R-OHPs undergoes a notable increase with rising rotational speed,exhibiting a peak at a threshold speed value.Such a peak is present irrespectively of the working fluid,and,after exceeding the threshold,higher rotational speeds lead to a lower thermal performance.Based on nonlinear dynamic analysis,the power spectrum density of the evaporator temperature indicates a lack of dominant frequency in temperature signals,suggesting a complex behavior characterized by random oscillations of vapor slugs and liquid plugs.In order to better understand how strong the chaotic behavior is,an autocorrelation analysis was carried out,the OHP at static state has a stronger chaos than R-OHPs.The correlation dimension analysis of the evaporator temperature provides values ranging from 1.2 to 1.6,which together with the Lyapunov exponent calculations,further support an evident chaotic nature of R-OHPs.展开更多
Fatigue failure caused by vibration is the most common type of pipeline failure.The core of this research is to obtain the nonlinear dynamic stress of a pipeline system accurately and efficiently,a topic that needs to...Fatigue failure caused by vibration is the most common type of pipeline failure.The core of this research is to obtain the nonlinear dynamic stress of a pipeline system accurately and efficiently,a topic that needs to be explored in the existing literature.The shell theory can better simulate the circumferential stress distribution,and thus the Mindlin-Reissner shell theory is used to model the pipeline.In this paper,the continuous pipeline system is combined with clamps through modal expansion for the first time,which realizes the coupling problem between a shell and a clamp.While the Bouc-Wen model is used to simulate the nonlinear external force generated by a clamp,the nonlinear coupling characteristics of the system are effectively captured.Then,the dynamic equation of the clamp-pipeline system is established according to the Lagrange energy equation.Based on the resonance frequency and stress amplitude obtained from the experiment,the nonlinear parameters of the clamp are identified with the semi-analytical method(SAM)and particle swarm optimization(PSO)algorithm.This study provides a theoretical basis for the clamp-pipeline system and an efficient and universal solution for stress prediction and analysis of pipelines in engineering.展开更多
In semiconductor precision packaging and other applications involving alignment of automated equipment,the nonlinear motion caused by structural characteristics and friction effects on torque-type rotating motion stag...In semiconductor precision packaging and other applications involving alignment of automated equipment,the nonlinear motion caused by structural characteristics and friction effects on torque-type rotating motion stages seriously affects output accuracy and stability.To solve this problem,the motion characteristics of a rotating stage and the mechanism by which friction nonlinearity influences accuracy are analyzed in detail.In addition,a compound control strategy based on a kinematic model and the Stribeck friction model is designed.A friction disturbance observer based on output position feedback is improved for simple parameter tuning.Finally,an experimental system is constructed to carry out validation tests,including identification of nonlinear characteristics and performance comparisons.The experimental results show that the linear tracking error of the torque-type rotating stage is less than 1.47µm after adoption of the proposed model-based composite control strategy,and the corresponding rotary angle deviation is less than 0.0153°.The linearity of output motion is increased to 97.59%and the error compensation effect is improved by 51.6%compared with the PID control method.The experimental results confirm that the analysis method adopted here and the proposed compensation strategy can effectively reduce frictional nonlinearity and improve motion accuracy.The proposed method can also be applied to other precision electromechanical systems.展开更多
To improve design accuracy and reliability of structures,this study solves the uncertain natural frequencies with consideration for geometric nonlinearity and structural uncertainty.Frequencies of the laminated plate ...To improve design accuracy and reliability of structures,this study solves the uncertain natural frequencies with consideration for geometric nonlinearity and structural uncertainty.Frequencies of the laminated plate with all four edges clamped(CCCC)are derived based on Navier's method and Galerkin's method.The novelty of the current work is that the number of unknowns in the displacement field model of a CCCC plate with free midsurface(CCCC-2 plate)is only three compared with four or five in cases of other exposed methods.The present analytical method is proved to be accurate and reliable by comparing linear natural frequencies and nonlinear natural frequencies with other models available in the open literature.Furthermore,a novel method for analyzing effects of mean values and tolerance zones of uncertain structural parameters on random frequencies is proposed based on a self-developed Multiscale Feature Extraction and Fusion Network(MFEFN)system.Compared with a direct Monte Carlo Simulation(MCS),the MFEFNbased procedure significantly reduces the calculation burden with a guarantee of accuracy.Our research provides a method to calculate nonlinear natural frequencies under two boundary conditions and presentes a surrogate model to predict frequencies for accuracy analysis and optimization design.展开更多
This study investigates the instability of nanofluid thin films flowing down an inclined plane under the influence of a normal electric field.Based on the long-wave approximation and a systematic asymptotic expansion,...This study investigates the instability of nanofluid thin films flowing down an inclined plane under the influence of a normal electric field.Based on the long-wave approximation and a systematic asymptotic expansion,a nonlinear evolution equation is derived to capture the coupled effects of the electric field and nanoparticle properties.Linear stability analysis reveals that the electric field enhances interfacial disturbances and promotes instability,whereas the presence of nanoparticles suppresses this effect by attenuating disturbance amplitudes.A weakly nonlinear analysis further clarifies the interplay among electric field strength,nanoparticle volume fraction,and density difference,enabling a classification of nonlinear stability regimes.Numerical simulations support the analytical predictions,showing that in unstable regimes,perturbations grow over time and eventually destabilize the film.These findings offer theoretical insights into the control of nanofluid film stability via electric field regulation and nanoparticle tuning.展开更多
This study investigates the nonlinear dynamic properties of rotating functionally graded sandwich rectangular plates in a thermal environment.The nonlinear vibration equations for a rotating metal-ceramic functionally...This study investigates the nonlinear dynamic properties of rotating functionally graded sandwich rectangular plates in a thermal environment.The nonlinear vibration equations for a rotating metal-ceramic functionally graded sandwich rectangular plate in a thermal environment are derived using classical thin plate theory and Hamilton’s principle,considering geometric nonlinearity,temperature-dependent material properties,and power law distribution of components through the thickness.With cantilever boundary conditions,the flexural nonlinear differential equations of the rectangular sandwich plate are obtained via the Galerkin method.Since the natural vibration differential equations exhibit nonlinear characteristics,the multiscale method is employed to derive the expression for nonlinear natural frequency.An example analysis reveals how the natural frequency of a functionally graded sandwich rectangular plate varies with rotational speed and temperature.Results show that the nonlinear/linear frequency ratio increases with rotational angular velocity Ω and thickness-to-length ratio h/a,follows a cosine-like periodic pattern with the setting angle,and shows a sharp decrease followed by a rapid increase with increasing width-to-length ratio b/a.The derived analytical solutions for nonlinear frequency provide valuable insights for assessing the dynamic characteristics of functionally graded structures.展开更多
The stability of gaseous detonation waves is crucial for the operation of detonation-based propulsion systems and the assessment of industrial explosion hazards.However,research on the stability of detonation waves in...The stability of gaseous detonation waves is crucial for the operation of detonation-based propulsion systems and the assessment of industrial explosion hazards.However,research on the stability of detonation waves in complex reactive systems that are composed of actual fuels and oxidants and can be described by numerous elementary chemical reactions,has not been fully carried out.To investigate the relationship between linear and nonlinear stabilities in gaseous detonation wave propagation for complex reactive systems,the linear stability analysis and the one-dimensionally nonlinear numerical simulations of H2/O2/Ar(argon)detonations based on the reactive Euler equations and detailed reaction mechanisms are carried out.The results show that in complex reactive systems characterized by elementary chemical reactions,the results of linear stability computation of detonation are consistent with those from one-dimensionally nonlinear oscillations of detonation wave.Utilizing these linear stability results,a neutral stability curve and a perturbation frequency transition curve in the phase plane of initial pressure versus inert gas(Ar)dilution ratio are derived,especially the new frequency transition curve clearly describes the transition of perturbations from low-frequency to high-frequency mode.One-dimensional nonlinear simulations show that near the perturbation frequency transition curve,the oscillations of the detonation wave can also transform between the lowfrequency,high-amplitude oscillation mode and the high-frequency,low-amplitude oscillation mode,with the oscillation frequency corresponding to the mode that exhibits the maximum growth rate identified in the linear stability analysis.This investigation into detonation stability in complex reactive gases offers guidance for selecting appropriate initial conditions and gas compositions in practical applications of detonation.展开更多
This paper analyzes the nonlinear dynamic characteristics and stability of Aero-Engine Dual-Rotor(AEDR)systems under high-frequency excitation,based on the Adaptive Harmonic Balance with the Asymptotic Harmonic Select...This paper analyzes the nonlinear dynamic characteristics and stability of Aero-Engine Dual-Rotor(AEDR)systems under high-frequency excitation,based on the Adaptive Harmonic Balance with the Asymptotic Harmonic Selection(AHB-AHS)method.A finite element dynamic equation for the AEDR system is introduced,considering complex nonlinearities of the intershaft bearing,unbalanced excitations,and high-frequency excitation.A solving strategy combining the AHB-AHS method and improved arclength continuation method is proposed to solve highdimensional dynamic equations containing complex nonlinearities and to track periodic solutions with parameter variations.The Floquet theory is used to analyze the types of bifurcation points in the system and the stability of periodic motions.The results indicate that high-frequency excitation can couple high-order and low-order modes,especially when the system undergoes superharmonic resonance.High-frequency excitation leads to more combination frequency harmonics,among which N_(f)ω_(1)-2ω_(2)dominates.Furthermore,changing the parameters(amplitude and frequency)of high-frequency excitation widens or shifts the unstable regions of the system.These findings contribute to understanding the mechanism of high-frequency excitation on aero-engines and demonstrate that the proposed AHB-AHS method is a powerful tool for analyzing highdimensional complex nonlinear dynamic systems under multi-frequency excitation.展开更多
Border-associated macrophages are located at the interface between the brain and the periphery, including the perivascular spaces, choroid plexus, and meninges. Until recently, the functions of border-associated macro...Border-associated macrophages are located at the interface between the brain and the periphery, including the perivascular spaces, choroid plexus, and meninges. Until recently, the functions of border-associated macrophages have been poorly understood and largely overlooked. However, a recent study reported that border-associated macrophages participate in stroke-induced inflammation, although many details and the underlying mechanisms remain unclear. In this study, we performed a comprehensive single-cell analysis of mouse border-associated macrophages using sequencing data obtained from the Gene Expression Omnibus(GEO) database(GSE174574 and GSE225948). Differentially expressed genes were identified, and enrichment analysis was performed to identify the transcription profile of border-associated macrophages. CellChat analysis was conducted to determine the cell communication network of border-associated macrophages. Transcription factors were predicted using the ‘pySCENIC' tool. We found that, in response to hypoxia, borderassociated macrophages underwent dynamic transcriptional changes and participated in the regulation of inflammatory-related pathways. Notably, the tumor necrosis factor pathway was activated by border-associated macrophages following ischemic stroke. The pySCENIC analysis indicated that the activity of signal transducer and activator of transcription 3(Stat3) was obviously upregulated in stroke, suggesting that Stat3 inhibition may be a promising strategy for treating border-associated macrophages-induced neuroinflammation. Finally, we constructed an animal model to investigate the effects of border-associated macrophages depletion following a stroke. Treatment with liposomes containing clodronate significantly reduced infarct volume in the animals and improved neurological scores compared with untreated animals. Taken together, our results demonstrate comprehensive changes in border-associated macrophages following a stroke, providing a theoretical basis for targeting border-associated macrophages-induced neuroinflammation in stroke treatment.展开更多
Designing,modeling,and analyzing novel nonlinear elastic elements for the nonlinear energy sink(NES)have long been an attractive research topic.Since gravity is difficult to overcome,previous NES research mainly focus...Designing,modeling,and analyzing novel nonlinear elastic elements for the nonlinear energy sink(NES)have long been an attractive research topic.Since gravity is difficult to overcome,previous NES research mainly focused on horizontal vibration suppression.This study proposes an origami-inspired NES.A stacked Miura-origami(SMO)structure,consisting of two Miura-ori sheets,is adopted to construct a nonlinear elastic element.By adjusting the initial angle and the connecting crease torsional stiffness,the quasi-zero stiffness(QZS)and load-bearing capacity can be customized to match the corresponding mass,establishing the vertical SMO-NES.The dynamic model of the SMO-NES coupled with a linear oscillator(LO)is derived for vibrations in the vertical direction.The approximate analytical solutions of the dynamic equation are obtained by the harmonic balance method(HBM),and the solutions are verified numerically.The parameter design principle of the SMO-NES is provided.Finally,the vibration reduction performance of the SMO-NES is studied.The results show that the proposed SMONES can overcome gravity and achieve quasi-zero nonlinear restoring force.Therefore,the SMO-NES has the ability of wide-frequency vibration reduction,and can effectively suppress vertical vibrations.By adjusting the initial angle and connecting the crease torsional stiffness of the SMO,the SMO-NES can be achieved with different loading weights,effectively suppressing the vibrations with different primary system masses and excitation amplitudes.In conclusion,with the help of popular origami structures,this study proposes a novel NES,and starts the research of combining origami and NES.展开更多
Nonlinear energy transfer is represented through eddy viscosity and stochastic forcing within the framework of resolvent analysis.Previous investigations estimate the contribution of eddy-viscosity-enhanced resolvent ...Nonlinear energy transfer is represented through eddy viscosity and stochastic forcing within the framework of resolvent analysis.Previous investigations estimate the contribution of eddy-viscosity-enhanced resolvent opera-tor to nonlinear energy transfer.The present article estimates the contribution of stochastic forcing to nonlinear energy transfer and demonstrates that the contribution of stochastic forcing cannot be ignored.These results are achieved by numerically comparing the eddy-viscosity-enhanced resolvent operator and stochastic forcing with nonlinear energy transfer in turbulent channel flows.Furthermore,the numerical results indicate that composite resolvent operators can improve the prediction of nonlinear energy transfer.展开更多
During strike-slip fault dislocation,multiple fault planes are commonly observed.The resulting permanent ground deformation can lead to profound structural damage to tunnels.However,existing analytical models do not c...During strike-slip fault dislocation,multiple fault planes are commonly observed.The resulting permanent ground deformation can lead to profound structural damage to tunnels.However,existing analytical models do not consider multiple fault planes.Instead,they concentrate the entire fault displacement onto a single fault plane for analysis,thereby giving rise to notable errors in the calculated results.To address this issue,a refined nonlinear theoretical model was established to analyze the mechanical responses of the tunnels subjected to multiple strike-slip fault dislocations.The analytical model considers the number of fault planes,nonlinear soil‒tunnel interactions,geometric nonlinearity,and fault zone width,leading to a significant improvement in its range of applicability and calculation accuracy.The results of the analytical model are in agreement,both qualitatively and quantitatively,with the model test and numerical results.Then,based on the proposed theoretical model,a sensitivity analysis of parameters was conducted,focusing on the variables such as the number of fault planes,fault plane distance(d),fault displacement ratio(η),burial depth(C),crossing angle(β),tunnel diameter(D),fault zone width(Wf),and strike-slip fault displacement(Δfs).The results show that the peak shear force(Vmax),bending moment(Mmax),and axial force(Nmax)decrease with increasing d.The Vmax of the tunnel is found at the fault plane with the largest fault displacement.C,D,andΔfs contribute to the increases in Vmax,Mmax,and Nmax.Additionally,increasing the number of fault planes reduces Vmax and Mmax,whereas the variation in Nmax remains minimal.展开更多
In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to ...In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to obtain the maximal positive definite solution of nonlinear matrix equation X+A^(*)X|^(-α)A=Q with the case 0<α≤1.Based on this method,a new iterative algorithm is developed,and its convergence proof is given.Finally,two numerical examples are provided to show the effectiveness of the proposed method.展开更多
Under investigation is the n-component nonlinear Schrödinger equation with higher-order effects,which describes the ultrashort pulses in the birefringent fiber.Based on the Lax pair,the eigenfunction and generali...Under investigation is the n-component nonlinear Schrödinger equation with higher-order effects,which describes the ultrashort pulses in the birefringent fiber.Based on the Lax pair,the eigenfunction and generalized Darboux transformation are derived.Next,we construct several novel higher-order localized waves and classified them into three categories:(i)higher-order rogue waves interacting with bright/antidark breathers,(ii)higher-order breather fission/fusion,(iii)higherorder breather interacting with soliton.Moreover,we explore the effects of parameters on the structure,collision process and energy distribution of localized waves and these characteristics are significantly different from previous ones.Finally,the dynamical properties of these solutions are discussed in detail.展开更多
Six new lanthanide complexes:[Ln(3,4-DEOBA)3(4,4'-DM-2,2'-bipy)]2·2C_(2)H_(5)OH,[Ln=Dy(1),Eu(2),Tb(3),Sm(4),Ho(5),Gd(6);3,4-DEOBA-=3,4-diethoxybenzoate,4,4'-DM-2,2'-bipy=4,4'-dimethyl-2,2'...Six new lanthanide complexes:[Ln(3,4-DEOBA)3(4,4'-DM-2,2'-bipy)]2·2C_(2)H_(5)OH,[Ln=Dy(1),Eu(2),Tb(3),Sm(4),Ho(5),Gd(6);3,4-DEOBA-=3,4-diethoxybenzoate,4,4'-DM-2,2'-bipy=4,4'-dimethyl-2,2'-bipyridine]were successfully synthesized by the volatilization of the solution at room temperature.The crystal structures of six complexes were determined by single-crystal X-ray diffraction technology.The results showed that the complexes all have a binuclear structure,and the structures contain free ethanol molecules.Moreover,the coordination number of the central metal of each structural unit is eight.Adjacent structural units interact with each other through hydrogen bonds and further expand to form 1D chain-like and 2D planar structures.After conducting a systematic study on the luminescence properties of complexes 1-4,their emission and excitation spectra were obtained.Experimental results indicated that the fluorescence lifetimes of complexes 2 and 3 were 0.807 and 0.845 ms,respectively.The emission spectral data of complexes 1-4 were imported into the CIE chromaticity coordinate system,and their corre sponding luminescent regions cover the yellow light,red light,green light,and orange-red light bands,respectively.Within the temperature range of 299.15-1300 K,the thermal decomposition processes of the six complexes were comprehensively analyzed by using TG-DSC/FTIR/MS technology.The hypothesis of the gradual loss of ligand groups during the decomposition process was verified by detecting the escaped gas,3D infrared spectroscopy,and ion fragment information detected by mass spectrometry.The specific decomposition path is as follows:firstly,free ethanol molecules and neutral ligands are removed,and finally,acidic ligands are released;the final product is the corresponding metal oxide.CCDC:2430420,1;2430422,2;2430419,3;2430424,4;2430421,5;2430423,6.展开更多
The Savitzky-Golay(SG)filter,which employs polynomial least-squares approximations to smooth data and estimate derivatives,is widely used for processing noisy data.However,noise suppression by the SG filter is recogni...The Savitzky-Golay(SG)filter,which employs polynomial least-squares approximations to smooth data and estimate derivatives,is widely used for processing noisy data.However,noise suppression by the SG filter is recognized to be limited at data boundaries and high frequencies,which can significantly reduce the signal-to-noise ratio(SNR).To solve this problem,a novel method synergistically integrating Principal Component Analysis(PCA)with SG filtering is proposed in this paper.This approach avoids the is-sue of excessive smoothing associated with larger window sizes.The proposed PCA-SG filtering algorithm was applied to a CO gas sensing system based on Cavity Ring-Down Spectroscopy(CRDS).The perform-ance of the PCA-SG filtering algorithm is demonstrated through comparison with Moving Average Filtering(MAF),Wavelet Transformation(WT),Kalman Filtering(KF),and the SG filter.The results demonstrate that the proposed algorithm exhibits superior noise reduction capabilities compared to the other algorithms evaluated.The SNR of the ring-down signal was improved from 11.8612 dB to 29.0913 dB,and the stand-ard deviation of the extracted ring-down time constant was reduced from 0.037μs to 0.018μs.These results confirm that the proposed PCA-SG filtering algorithm effectively improves the smoothness of the ring-down curve data,demonstrating its feasibility.展开更多
Objective:To evaluate the global,regional,and national burden and determinants of Acute Respiratory Infections(ARIs)among children and adolescents from 1990 to 2021.Methods:We analysed ARI mortality and disability-adj...Objective:To evaluate the global,regional,and national burden and determinants of Acute Respiratory Infections(ARIs)among children and adolescents from 1990 to 2021.Methods:We analysed ARI mortality and disability-adjusted life years(DALYs),stratified by age,sex,and economic development level based on data retrieved from the Global Burden of Disease study 2021.Decomposition and frontier analyses were employed to identify key drivers of burden variation and visualize potential reductions based on development levels.Results:Between 1990 and 2021,the global burden of ARIs showed a significant decline in both achievable age-standardized DALYs rate and age-standardized mortality rates(EAPC=-3.87 and-3.81,respectively).Different age groups and sex witnessed different levels of ARI burden,males experienced heavier burden than females and the 0-4 years-old group experienced heavier burden than other study age groups.Most of the 204 countries and territories experienced a downward trend of ARI burden,with slight increases observed only in Lesotho and Dominica.A negative correlation was found between the Socio-demographic Index and ARI burden.Decomposition analysis indicated that the significant decreases in deaths and DALYs were primarily driven by epidemiological changes.Conclusions:The global burden of ARIs among children and adolescents has declined over the past three decades,but substantial regional disparities persist.Targeted public health strategies are needed to address the continued ARI burden in high-risk regions and vulnerable age groups.展开更多
基金supported by the Natural Science Foundation of Shandong Province(Grant No.ZR2025QC30)。
文摘We investigate the alpha helical protein structure characterized by fourth-order interspine coupling,focusing on a three-coupled fourth-order nonlinear Schr??dinger system.We introduce a generalized Darboux transformation,departing from the classical Darboux transformation.Based on this,we construct the two-and three-degenerate soliton solutions and four-degenerate asymptotic soliton solutions.Based on the asymptotic analysis,we find that the amplitudes of interacting solitons are retained upon the interactions.Elastic interactions between two degenerate solitons exhibiting four curve-type asymptotic solitons are depicted.When the lattice parameterβchanges,the velocities of the two degenerate solitons also change.Elastic interaction among three degenerate solitons comprising four curve-type asymptotic solitons and two line-type solitons is presented.Interaction among one soliton and two degenerate solitons with different velocities is shown.Elastic interaction among four degenerate solitons comprising eight curve-type asymptotic solitons is also presented.Interaction among two two-degenerate solitons with two spectral parameters is shown.The relative distance between two asymptotic solitons exhibits logarithmic growth with|t|,where t represents the retarded time.Acceleration of soliton separation decays exponentially with relative distance,and eventually approaches zero.Phase shifts depend on t.
基金supported by the National Natural Science Foundation of China(No.12272240)the Liaoning Revitalization Talents Program,China(No.XLYC2203197)。
文摘Traditional dynamic analysis of mechanical structures,often limited to individual beams or plates,fails to fully capture their dynamic behaviors.In systems where space and mass are constrained,such as the battery support structures in electric aircraft,conventional absorbers and isolators are insufficient for effective vibration control.This study simplifies the battery support structure of electric aircraft as an integrated composite beam consisting of three interconnected beams,and investigated its structural dynamics properties and nonlinear vibration control under thermal conditions caused by battery heat.The nonlinear vibration control is performed using the Nitinol steel wire ropes(Ni Ti-ST),with nonlinear damping properties.The natural frequencies of system are determined using the Rayleigh-Ritz technique.Theoretical results are validated through both Finite Element Method(FEM)and hammer tests.Moreover,the dynamic equations are derived using the Lagrange method and discretized via the Galerkin Truncation Method(GTM).The Harmonic Balance Method(HBM)is used to evaluate the vibration responses of the integrated model,with further verification through the Runge-Kutta Method(RKM).The experiments are conducted to corroborate the theoretical analysis.The results show that the system frequency changes in stages with the increase of the stiffness of the integrated composite beam connection.Especially in the case of varying environments,as the temperature increases,the frequency of system will first increase to a certain maximum value and then gradually decrease.Furthermore,the NiTi-ST effectively reduces vibration in the integrated composite beam,particularly under varying temperatures and external excitations.
基金supported by the National Key Research and Development Program of China(No.2020YFB1708303)the National Natural Science Foundation of China(Nos.U1808215 and 12072058)the Fundamental Research Funds for the Central Universities of China(DUT20LK02).
文摘Honeycomb structures of shape memory alloy(SMA)have become one of the most promising materials for flexible skins of morphing aircraft due to their excellent mechanical properties.However,due to the nonlinear material and geometric large deformation,the SMA honeycomb exhibits significant and complex nonlinearity in the skin and there is a lack of relevant previous research.In this paper,the nonlinear properties of the SMA honeycomb structure with arbitrary geometry are investigated for the first time for large deformation flexible skin applications by theoretical and experimental analysis.Firstly,a novel theoretical model of SMA honeycomb structure considering both material and geometric nonlinearity is proposed,and the corresponding calculation method of nonlinear governing equations is given based upon the shooting method and Runge–Kutta method.Then,the tensile behaviors of four kinds of SMA honeycomb structures,i.e.,U-type,V-type,cosine-type,and trapezoid-type,are analyzed and predicted by the proposed theoretical model and compared with the finite element analysis(FEA)results.Moreover,the tensile experiments were carried out by stretching U-type and V-type honeycomb structures to a global strain of 60%and 40%,respectively,to perform large deformation analysis and verify the theoretical model.Finally,experimental verification and finite element validation show that the curves of the theoretical model results,experimental results,and simulation results are in good agreement,illustrating the generalizability and accuracy of the proposed theoretical model.The theoretical model and experimental investigations in this paper are considered to provide an effective foundation for analyzing and predicting the mechanical behavior of SMA honeycomb flexible skins with large extensional deformations.
基金Supported by National Natural Science Foundation of China(Grant No.52205476)Jiangsu Provincial Natural Science Foundation(Grant No.BK20242040)+2 种基金Fundamental Research Funds for the Central Universities(Grant No.NG2024008)the Youth Talent Support Project of CASTthe Fund of Jiangsu Key Laboratory of Precision and Micro-Manufacturing Technology(Grant No.1005-ZAA20003-14)。
文摘Radial rotating oscillating heat pipes(R-OHPs)have excellent thermal performance and great potential for application in the thermal management of rotatory machinery.However,the heat transport behavior and temperature characteristics of R-OHPs are complex,and their understanding is still limited,hence necessitating further research.In this study,thanks to an experimental investigation involving a copper R-OHP running with acetone and water,its thermal performance is evaluated,and then the temperature characteristics are analyzed by nonlinear dynamic analysis.The study reveals that the effective heat transfer coefficient of R-OHPs undergoes a notable increase with rising rotational speed,exhibiting a peak at a threshold speed value.Such a peak is present irrespectively of the working fluid,and,after exceeding the threshold,higher rotational speeds lead to a lower thermal performance.Based on nonlinear dynamic analysis,the power spectrum density of the evaporator temperature indicates a lack of dominant frequency in temperature signals,suggesting a complex behavior characterized by random oscillations of vapor slugs and liquid plugs.In order to better understand how strong the chaotic behavior is,an autocorrelation analysis was carried out,the OHP at static state has a stronger chaos than R-OHPs.The correlation dimension analysis of the evaporator temperature provides values ranging from 1.2 to 1.6,which together with the Lyapunov exponent calculations,further support an evident chaotic nature of R-OHPs.
基金Project supported by the National Science and Technology Major Project(No.J2019-I-0008-0008)the National Natural Science Foundation of China(No.52305096)the Chinese Postdoctoral Science Foundation(No.GZB20230117)。
文摘Fatigue failure caused by vibration is the most common type of pipeline failure.The core of this research is to obtain the nonlinear dynamic stress of a pipeline system accurately and efficiently,a topic that needs to be explored in the existing literature.The shell theory can better simulate the circumferential stress distribution,and thus the Mindlin-Reissner shell theory is used to model the pipeline.In this paper,the continuous pipeline system is combined with clamps through modal expansion for the first time,which realizes the coupling problem between a shell and a clamp.While the Bouc-Wen model is used to simulate the nonlinear external force generated by a clamp,the nonlinear coupling characteristics of the system are effectively captured.Then,the dynamic equation of the clamp-pipeline system is established according to the Lagrange energy equation.Based on the resonance frequency and stress amplitude obtained from the experiment,the nonlinear parameters of the clamp are identified with the semi-analytical method(SAM)and particle swarm optimization(PSO)algorithm.This study provides a theoretical basis for the clamp-pipeline system and an efficient and universal solution for stress prediction and analysis of pipelines in engineering.
基金funded by the European Union’s Horizon 2020 Research and Innovation Program under the Marie Sklodowska-Curie Grant Agreement(Grant No.101026104)by the National Natural Science Foundation of China(Grant No.U20A6004)in part by the State Key Laboratory of Precision Electronics Manufacturing Technology and Equipment(Grant No.JMDZ202314).
文摘In semiconductor precision packaging and other applications involving alignment of automated equipment,the nonlinear motion caused by structural characteristics and friction effects on torque-type rotating motion stages seriously affects output accuracy and stability.To solve this problem,the motion characteristics of a rotating stage and the mechanism by which friction nonlinearity influences accuracy are analyzed in detail.In addition,a compound control strategy based on a kinematic model and the Stribeck friction model is designed.A friction disturbance observer based on output position feedback is improved for simple parameter tuning.Finally,an experimental system is constructed to carry out validation tests,including identification of nonlinear characteristics and performance comparisons.The experimental results show that the linear tracking error of the torque-type rotating stage is less than 1.47µm after adoption of the proposed model-based composite control strategy,and the corresponding rotary angle deviation is less than 0.0153°.The linearity of output motion is increased to 97.59%and the error compensation effect is improved by 51.6%compared with the PID control method.The experimental results confirm that the analysis method adopted here and the proposed compensation strategy can effectively reduce frictional nonlinearity and improve motion accuracy.The proposed method can also be applied to other precision electromechanical systems.
基金the research project funded by the Fundamental Research Funds for the Central Universities(No.HIT.OCEP.2024038)the National Natural Science Foundation of China(No.52372351)the State Key Laboratory of Micro-Spacecraft Rapid Design and Intelligent Cluster,China(No.MS02240107)。
文摘To improve design accuracy and reliability of structures,this study solves the uncertain natural frequencies with consideration for geometric nonlinearity and structural uncertainty.Frequencies of the laminated plate with all four edges clamped(CCCC)are derived based on Navier's method and Galerkin's method.The novelty of the current work is that the number of unknowns in the displacement field model of a CCCC plate with free midsurface(CCCC-2 plate)is only three compared with four or five in cases of other exposed methods.The present analytical method is proved to be accurate and reliable by comparing linear natural frequencies and nonlinear natural frequencies with other models available in the open literature.Furthermore,a novel method for analyzing effects of mean values and tolerance zones of uncertain structural parameters on random frequencies is proposed based on a self-developed Multiscale Feature Extraction and Fusion Network(MFEFN)system.Compared with a direct Monte Carlo Simulation(MCS),the MFEFNbased procedure significantly reduces the calculation burden with a guarantee of accuracy.Our research provides a method to calculate nonlinear natural frequencies under two boundary conditions and presentes a surrogate model to predict frequencies for accuracy analysis and optimization design.
基金supported by the National Natural Science Foundation of China(Grant Nos.11902165,12272188,12102205,and 12262025)the National Science Foundation for Distinguished Young Scholars of the Inner Mongolia Autonomous Region of China(Grant No.2023JQ16)+1 种基金the Program for Young Talents of Science and Technology in Universities of Inner Mongolia Autonomous Region(Grant No.NJYT23098)the Scientific Startin and the Innovative Research Team in Universities of Inner Mongolia Autonomous Region of China(Grant No.NMGIRT2208)。
文摘This study investigates the instability of nanofluid thin films flowing down an inclined plane under the influence of a normal electric field.Based on the long-wave approximation and a systematic asymptotic expansion,a nonlinear evolution equation is derived to capture the coupled effects of the electric field and nanoparticle properties.Linear stability analysis reveals that the electric field enhances interfacial disturbances and promotes instability,whereas the presence of nanoparticles suppresses this effect by attenuating disturbance amplitudes.A weakly nonlinear analysis further clarifies the interplay among electric field strength,nanoparticle volume fraction,and density difference,enabling a classification of nonlinear stability regimes.Numerical simulations support the analytical predictions,showing that in unstable regimes,perturbations grow over time and eventually destabilize the film.These findings offer theoretical insights into the control of nanofluid film stability via electric field regulation and nanoparticle tuning.
基金supported by the National Natural Science Foundation of China(No.11772090).
文摘This study investigates the nonlinear dynamic properties of rotating functionally graded sandwich rectangular plates in a thermal environment.The nonlinear vibration equations for a rotating metal-ceramic functionally graded sandwich rectangular plate in a thermal environment are derived using classical thin plate theory and Hamilton’s principle,considering geometric nonlinearity,temperature-dependent material properties,and power law distribution of components through the thickness.With cantilever boundary conditions,the flexural nonlinear differential equations of the rectangular sandwich plate are obtained via the Galerkin method.Since the natural vibration differential equations exhibit nonlinear characteristics,the multiscale method is employed to derive the expression for nonlinear natural frequency.An example analysis reveals how the natural frequency of a functionally graded sandwich rectangular plate varies with rotational speed and temperature.Results show that the nonlinear/linear frequency ratio increases with rotational angular velocity Ω and thickness-to-length ratio h/a,follows a cosine-like periodic pattern with the setting angle,and shows a sharp decrease followed by a rapid increase with increasing width-to-length ratio b/a.The derived analytical solutions for nonlinear frequency provide valuable insights for assessing the dynamic characteristics of functionally graded structures.
基金supported by the National Natural Science Foundation of China(Grant No.12472335).
文摘The stability of gaseous detonation waves is crucial for the operation of detonation-based propulsion systems and the assessment of industrial explosion hazards.However,research on the stability of detonation waves in complex reactive systems that are composed of actual fuels and oxidants and can be described by numerous elementary chemical reactions,has not been fully carried out.To investigate the relationship between linear and nonlinear stabilities in gaseous detonation wave propagation for complex reactive systems,the linear stability analysis and the one-dimensionally nonlinear numerical simulations of H2/O2/Ar(argon)detonations based on the reactive Euler equations and detailed reaction mechanisms are carried out.The results show that in complex reactive systems characterized by elementary chemical reactions,the results of linear stability computation of detonation are consistent with those from one-dimensionally nonlinear oscillations of detonation wave.Utilizing these linear stability results,a neutral stability curve and a perturbation frequency transition curve in the phase plane of initial pressure versus inert gas(Ar)dilution ratio are derived,especially the new frequency transition curve clearly describes the transition of perturbations from low-frequency to high-frequency mode.One-dimensional nonlinear simulations show that near the perturbation frequency transition curve,the oscillations of the detonation wave can also transform between the lowfrequency,high-amplitude oscillation mode and the high-frequency,low-amplitude oscillation mode,with the oscillation frequency corresponding to the mode that exhibits the maximum growth rate identified in the linear stability analysis.This investigation into detonation stability in complex reactive gases offers guidance for selecting appropriate initial conditions and gas compositions in practical applications of detonation.
基金the financial support from the National Key R&D Program of China(No.2023YFE0125900)National Natural Science Foundation of China(Nos.12372008 and 12102234)+1 种基金Natural Science Foundation of Heilongjiang Province,China(No.YQ2022A008)Taif University,Saudi Arabia,for supporting this work through Project number(TU-DSPP-2024-73).
文摘This paper analyzes the nonlinear dynamic characteristics and stability of Aero-Engine Dual-Rotor(AEDR)systems under high-frequency excitation,based on the Adaptive Harmonic Balance with the Asymptotic Harmonic Selection(AHB-AHS)method.A finite element dynamic equation for the AEDR system is introduced,considering complex nonlinearities of the intershaft bearing,unbalanced excitations,and high-frequency excitation.A solving strategy combining the AHB-AHS method and improved arclength continuation method is proposed to solve highdimensional dynamic equations containing complex nonlinearities and to track periodic solutions with parameter variations.The Floquet theory is used to analyze the types of bifurcation points in the system and the stability of periodic motions.The results indicate that high-frequency excitation can couple high-order and low-order modes,especially when the system undergoes superharmonic resonance.High-frequency excitation leads to more combination frequency harmonics,among which N_(f)ω_(1)-2ω_(2)dominates.Furthermore,changing the parameters(amplitude and frequency)of high-frequency excitation widens or shifts the unstable regions of the system.These findings contribute to understanding the mechanism of high-frequency excitation on aero-engines and demonstrate that the proposed AHB-AHS method is a powerful tool for analyzing highdimensional complex nonlinear dynamic systems under multi-frequency excitation.
基金supported by Qingdao Key Medical and Health Discipline ProjectThe Intramural Research Program of the Affiliated Hospital of Qingdao University,No. 4910Qingdao West Coast New Area Science and Technology Project,No. 2020-55 (all to SW)。
文摘Border-associated macrophages are located at the interface between the brain and the periphery, including the perivascular spaces, choroid plexus, and meninges. Until recently, the functions of border-associated macrophages have been poorly understood and largely overlooked. However, a recent study reported that border-associated macrophages participate in stroke-induced inflammation, although many details and the underlying mechanisms remain unclear. In this study, we performed a comprehensive single-cell analysis of mouse border-associated macrophages using sequencing data obtained from the Gene Expression Omnibus(GEO) database(GSE174574 and GSE225948). Differentially expressed genes were identified, and enrichment analysis was performed to identify the transcription profile of border-associated macrophages. CellChat analysis was conducted to determine the cell communication network of border-associated macrophages. Transcription factors were predicted using the ‘pySCENIC' tool. We found that, in response to hypoxia, borderassociated macrophages underwent dynamic transcriptional changes and participated in the regulation of inflammatory-related pathways. Notably, the tumor necrosis factor pathway was activated by border-associated macrophages following ischemic stroke. The pySCENIC analysis indicated that the activity of signal transducer and activator of transcription 3(Stat3) was obviously upregulated in stroke, suggesting that Stat3 inhibition may be a promising strategy for treating border-associated macrophages-induced neuroinflammation. Finally, we constructed an animal model to investigate the effects of border-associated macrophages depletion following a stroke. Treatment with liposomes containing clodronate significantly reduced infarct volume in the animals and improved neurological scores compared with untreated animals. Taken together, our results demonstrate comprehensive changes in border-associated macrophages following a stroke, providing a theoretical basis for targeting border-associated macrophages-induced neuroinflammation in stroke treatment.
基金Project supported by the National Science Fund for Distinguished Young Scholars(No.12025204)the China Scholarship Council(No.202206890066)。
文摘Designing,modeling,and analyzing novel nonlinear elastic elements for the nonlinear energy sink(NES)have long been an attractive research topic.Since gravity is difficult to overcome,previous NES research mainly focused on horizontal vibration suppression.This study proposes an origami-inspired NES.A stacked Miura-origami(SMO)structure,consisting of two Miura-ori sheets,is adopted to construct a nonlinear elastic element.By adjusting the initial angle and the connecting crease torsional stiffness,the quasi-zero stiffness(QZS)and load-bearing capacity can be customized to match the corresponding mass,establishing the vertical SMO-NES.The dynamic model of the SMO-NES coupled with a linear oscillator(LO)is derived for vibrations in the vertical direction.The approximate analytical solutions of the dynamic equation are obtained by the harmonic balance method(HBM),and the solutions are verified numerically.The parameter design principle of the SMO-NES is provided.Finally,the vibration reduction performance of the SMO-NES is studied.The results show that the proposed SMONES can overcome gravity and achieve quasi-zero nonlinear restoring force.Therefore,the SMO-NES has the ability of wide-frequency vibration reduction,and can effectively suppress vertical vibrations.By adjusting the initial angle and connecting the crease torsional stiffness of the SMO,the SMO-NES can be achieved with different loading weights,effectively suppressing the vibrations with different primary system masses and excitation amplitudes.In conclusion,with the help of popular origami structures,this study proposes a novel NES,and starts the research of combining origami and NES.
基金supported by the National Natural Science Foundation of China(NSFC)Basic Science Center Program for Multiscale Problems in Nonlinear Mechanics(Grant No.11988102).
文摘Nonlinear energy transfer is represented through eddy viscosity and stochastic forcing within the framework of resolvent analysis.Previous investigations estimate the contribution of eddy-viscosity-enhanced resolvent opera-tor to nonlinear energy transfer.The present article estimates the contribution of stochastic forcing to nonlinear energy transfer and demonstrates that the contribution of stochastic forcing cannot be ignored.These results are achieved by numerically comparing the eddy-viscosity-enhanced resolvent operator and stochastic forcing with nonlinear energy transfer in turbulent channel flows.Furthermore,the numerical results indicate that composite resolvent operators can improve the prediction of nonlinear energy transfer.
基金support from the National Natural Science Foundation of China(Grant Nos.52378411,52208404)China National Railway Group Limited Science and Technology Research and Development Program(Grant No.K2023G041).
文摘During strike-slip fault dislocation,multiple fault planes are commonly observed.The resulting permanent ground deformation can lead to profound structural damage to tunnels.However,existing analytical models do not consider multiple fault planes.Instead,they concentrate the entire fault displacement onto a single fault plane for analysis,thereby giving rise to notable errors in the calculated results.To address this issue,a refined nonlinear theoretical model was established to analyze the mechanical responses of the tunnels subjected to multiple strike-slip fault dislocations.The analytical model considers the number of fault planes,nonlinear soil‒tunnel interactions,geometric nonlinearity,and fault zone width,leading to a significant improvement in its range of applicability and calculation accuracy.The results of the analytical model are in agreement,both qualitatively and quantitatively,with the model test and numerical results.Then,based on the proposed theoretical model,a sensitivity analysis of parameters was conducted,focusing on the variables such as the number of fault planes,fault plane distance(d),fault displacement ratio(η),burial depth(C),crossing angle(β),tunnel diameter(D),fault zone width(Wf),and strike-slip fault displacement(Δfs).The results show that the peak shear force(Vmax),bending moment(Mmax),and axial force(Nmax)decrease with increasing d.The Vmax of the tunnel is found at the fault plane with the largest fault displacement.C,D,andΔfs contribute to the increases in Vmax,Mmax,and Nmax.Additionally,increasing the number of fault planes reduces Vmax and Mmax,whereas the variation in Nmax remains minimal.
基金Supported in part by Natural Science Foundation of Guangxi(2023GXNSFAA026246)in part by the Central Government's Guide to Local Science and Technology Development Fund(GuikeZY23055044)in part by the National Natural Science Foundation of China(62363003)。
文摘In this paper,we consider the maximal positive definite solution of the nonlinear matrix equation.By using the idea of Algorithm 2.1 in ZHANG(2013),a new inversion-free method with a stepsize parameter is proposed to obtain the maximal positive definite solution of nonlinear matrix equation X+A^(*)X|^(-α)A=Q with the case 0<α≤1.Based on this method,a new iterative algorithm is developed,and its convergence proof is given.Finally,two numerical examples are provided to show the effectiveness of the proposed method.
基金Project supported by the National Natural Science Foundation of China(Grant No.12271096)the Natural Science Foundation of Fujian Province(Grant No.2021J01302)。
文摘Under investigation is the n-component nonlinear Schrödinger equation with higher-order effects,which describes the ultrashort pulses in the birefringent fiber.Based on the Lax pair,the eigenfunction and generalized Darboux transformation are derived.Next,we construct several novel higher-order localized waves and classified them into three categories:(i)higher-order rogue waves interacting with bright/antidark breathers,(ii)higher-order breather fission/fusion,(iii)higherorder breather interacting with soliton.Moreover,we explore the effects of parameters on the structure,collision process and energy distribution of localized waves and these characteristics are significantly different from previous ones.Finally,the dynamical properties of these solutions are discussed in detail.
文摘Six new lanthanide complexes:[Ln(3,4-DEOBA)3(4,4'-DM-2,2'-bipy)]2·2C_(2)H_(5)OH,[Ln=Dy(1),Eu(2),Tb(3),Sm(4),Ho(5),Gd(6);3,4-DEOBA-=3,4-diethoxybenzoate,4,4'-DM-2,2'-bipy=4,4'-dimethyl-2,2'-bipyridine]were successfully synthesized by the volatilization of the solution at room temperature.The crystal structures of six complexes were determined by single-crystal X-ray diffraction technology.The results showed that the complexes all have a binuclear structure,and the structures contain free ethanol molecules.Moreover,the coordination number of the central metal of each structural unit is eight.Adjacent structural units interact with each other through hydrogen bonds and further expand to form 1D chain-like and 2D planar structures.After conducting a systematic study on the luminescence properties of complexes 1-4,their emission and excitation spectra were obtained.Experimental results indicated that the fluorescence lifetimes of complexes 2 and 3 were 0.807 and 0.845 ms,respectively.The emission spectral data of complexes 1-4 were imported into the CIE chromaticity coordinate system,and their corre sponding luminescent regions cover the yellow light,red light,green light,and orange-red light bands,respectively.Within the temperature range of 299.15-1300 K,the thermal decomposition processes of the six complexes were comprehensively analyzed by using TG-DSC/FTIR/MS technology.The hypothesis of the gradual loss of ligand groups during the decomposition process was verified by detecting the escaped gas,3D infrared spectroscopy,and ion fragment information detected by mass spectrometry.The specific decomposition path is as follows:firstly,free ethanol molecules and neutral ligands are removed,and finally,acidic ligands are released;the final product is the corresponding metal oxide.CCDC:2430420,1;2430422,2;2430419,3;2430424,4;2430421,5;2430423,6.
文摘The Savitzky-Golay(SG)filter,which employs polynomial least-squares approximations to smooth data and estimate derivatives,is widely used for processing noisy data.However,noise suppression by the SG filter is recognized to be limited at data boundaries and high frequencies,which can significantly reduce the signal-to-noise ratio(SNR).To solve this problem,a novel method synergistically integrating Principal Component Analysis(PCA)with SG filtering is proposed in this paper.This approach avoids the is-sue of excessive smoothing associated with larger window sizes.The proposed PCA-SG filtering algorithm was applied to a CO gas sensing system based on Cavity Ring-Down Spectroscopy(CRDS).The perform-ance of the PCA-SG filtering algorithm is demonstrated through comparison with Moving Average Filtering(MAF),Wavelet Transformation(WT),Kalman Filtering(KF),and the SG filter.The results demonstrate that the proposed algorithm exhibits superior noise reduction capabilities compared to the other algorithms evaluated.The SNR of the ring-down signal was improved from 11.8612 dB to 29.0913 dB,and the stand-ard deviation of the extracted ring-down time constant was reduced from 0.037μs to 0.018μs.These results confirm that the proposed PCA-SG filtering algorithm effectively improves the smoothness of the ring-down curve data,demonstrating its feasibility.
文摘Objective:To evaluate the global,regional,and national burden and determinants of Acute Respiratory Infections(ARIs)among children and adolescents from 1990 to 2021.Methods:We analysed ARI mortality and disability-adjusted life years(DALYs),stratified by age,sex,and economic development level based on data retrieved from the Global Burden of Disease study 2021.Decomposition and frontier analyses were employed to identify key drivers of burden variation and visualize potential reductions based on development levels.Results:Between 1990 and 2021,the global burden of ARIs showed a significant decline in both achievable age-standardized DALYs rate and age-standardized mortality rates(EAPC=-3.87 and-3.81,respectively).Different age groups and sex witnessed different levels of ARI burden,males experienced heavier burden than females and the 0-4 years-old group experienced heavier burden than other study age groups.Most of the 204 countries and territories experienced a downward trend of ARI burden,with slight increases observed only in Lesotho and Dominica.A negative correlation was found between the Socio-demographic Index and ARI burden.Decomposition analysis indicated that the significant decreases in deaths and DALYs were primarily driven by epidemiological changes.Conclusions:The global burden of ARIs among children and adolescents has declined over the past three decades,but substantial regional disparities persist.Targeted public health strategies are needed to address the continued ARI burden in high-risk regions and vulnerable age groups.
