Flash Joule heating(FJH),as a high-efficiency and low-energy consumption technology for advanced materials synthesis,has shown significant potential in the synthesis of graphene and other functional carbon materials.B...Flash Joule heating(FJH),as a high-efficiency and low-energy consumption technology for advanced materials synthesis,has shown significant potential in the synthesis of graphene and other functional carbon materials.Based on the Joule effect,the solid carbon sources can be rapidly heated to ultra-high temperatures(>3000 K)through instantaneous high-energy current pulses during FJH,thus driving the rapid rearrangement and graphitization of carbon atoms.This technology demonstrates numerous advantages,such as solvent-and catalyst-free features,high energy conversion efficiency,and a short process cycle.In this review,we have systematically summarized the technology principle and equipment design for FJH,as well as its raw materials selection and pretreatment strategies.The research progress in the FJH synthesis of flash graphene,carbon nanotubes,graphene fibers,and anode hard carbon,as well as its by-products,is also presented.FJH can precisely optimize the microstructures of carbon materials(e.g.,interlayer spacing of turbostratic graphene,defect concentration,and heteroatom doping)by regulating its operation parameters like flash voltage and flash time,thereby enhancing their performances in various applications,such as composite reinforcement,metal-ion battery electrodes,supercapacitors,and electrocatalysts.However,this technology is still challenged by low process yield,macroscopic material uniformity,and green power supply system construction.More research efforts are also required to promote the transition of FJH from laboratory to industrial-scale applications,thus providing innovative solutions for advanced carbon materials manufacturing and waste management toward carbon neutrality.展开更多
Among natural disasters,flash floods are the most destructive events,causing signif-icant damage to the economy and posing a serious threat to human life and property.Comprehensive risk assessment of these sudden floo...Among natural disasters,flash floods are the most destructive events,causing signif-icant damage to the economy and posing a serious threat to human life and property.Comprehensive risk assessment of these sudden floods is a key strategy to mitigate their impact.Accurate analysis of flash flood hazards can greatly enhance prevention efforts and inform critical decision-making processes,ultimately improving our ability to protect communities from these fast-onset disasters.This study analyzed the driving forces of flash flood disaster-causing factors in Heilongjiang Province.Meanwhile,nine different categories of variables affecting the occurrence of flash floods were selected,and the degree of influence of each driving factor on flash floods was quantitatively analyzed,and the driving force analysis of the driving factors of flash floods in Hei-longjiang Province was carried out by using the geographic probe model.This paper employs an uncertainty approach,utilizing a statistical-based interval weight deter-mination technique for evaluation indices and a two-dimensional information-based interval number sorting method.These methodologies are combined to construct a comprehensive flash flood risk assessment model.On this basis,the model was implemented in six regions within China's Heilongjiang province to evaluate and prioritize flash flood risks.The resulting risk ranking for these areas was as follows:Bayan≻Shuangcheng≻Boli≻Suibin≻Hailun≻Yian.The findings demonstrate that the interval number-based evaluation method effectively handles uncertainty,providing a more reliable risk grading system.This approach,by leveraging modern scientific advances and risk quantification techniques,is crucial for improving disaster management and mitigating flash flood impacts.展开更多
基金supported by the National Natural Science Foundation of China(52276196)the Foundation of State Key Laboratory of Coal Combustion(FSKLCCA2508)the High-level Talent Foundation of Anhui Agricultural University(rc412307).
文摘Flash Joule heating(FJH),as a high-efficiency and low-energy consumption technology for advanced materials synthesis,has shown significant potential in the synthesis of graphene and other functional carbon materials.Based on the Joule effect,the solid carbon sources can be rapidly heated to ultra-high temperatures(>3000 K)through instantaneous high-energy current pulses during FJH,thus driving the rapid rearrangement and graphitization of carbon atoms.This technology demonstrates numerous advantages,such as solvent-and catalyst-free features,high energy conversion efficiency,and a short process cycle.In this review,we have systematically summarized the technology principle and equipment design for FJH,as well as its raw materials selection and pretreatment strategies.The research progress in the FJH synthesis of flash graphene,carbon nanotubes,graphene fibers,and anode hard carbon,as well as its by-products,is also presented.FJH can precisely optimize the microstructures of carbon materials(e.g.,interlayer spacing of turbostratic graphene,defect concentration,and heteroatom doping)by regulating its operation parameters like flash voltage and flash time,thereby enhancing their performances in various applications,such as composite reinforcement,metal-ion battery electrodes,supercapacitors,and electrocatalysts.However,this technology is still challenged by low process yield,macroscopic material uniformity,and green power supply system construction.More research efforts are also required to promote the transition of FJH from laboratory to industrial-scale applications,thus providing innovative solutions for advanced carbon materials manufacturing and waste management toward carbon neutrality.
基金Basic Scientific Research Expense Project of IWHR-Extreme rainstorm development trends and prediction techniques,Grant/Award Number:JZ0145B142024National Natural Science Foundation of China,Grant/Award Number:42271095。
文摘Among natural disasters,flash floods are the most destructive events,causing signif-icant damage to the economy and posing a serious threat to human life and property.Comprehensive risk assessment of these sudden floods is a key strategy to mitigate their impact.Accurate analysis of flash flood hazards can greatly enhance prevention efforts and inform critical decision-making processes,ultimately improving our ability to protect communities from these fast-onset disasters.This study analyzed the driving forces of flash flood disaster-causing factors in Heilongjiang Province.Meanwhile,nine different categories of variables affecting the occurrence of flash floods were selected,and the degree of influence of each driving factor on flash floods was quantitatively analyzed,and the driving force analysis of the driving factors of flash floods in Hei-longjiang Province was carried out by using the geographic probe model.This paper employs an uncertainty approach,utilizing a statistical-based interval weight deter-mination technique for evaluation indices and a two-dimensional information-based interval number sorting method.These methodologies are combined to construct a comprehensive flash flood risk assessment model.On this basis,the model was implemented in six regions within China's Heilongjiang province to evaluate and prioritize flash flood risks.The resulting risk ranking for these areas was as follows:Bayan≻Shuangcheng≻Boli≻Suibin≻Hailun≻Yian.The findings demonstrate that the interval number-based evaluation method effectively handles uncertainty,providing a more reliable risk grading system.This approach,by leveraging modern scientific advances and risk quantification techniques,is crucial for improving disaster management and mitigating flash flood impacts.
