Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory a...Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory and cardiovascular diseases.In this study,we assessed the oxidative potential(OP)of fresh and O_(3)-aged PM_(2.5)particles from various urban and rural emission sources using the dithiothreitol(DTT)method.Our results revealed variations in the OP of fresh PM_(2.5)among different emission sources,with biomass burning sources exhibiting the highest OP,followed by industrial areas,vehicular emissions,cooking emissions,and suburban areas,respectively.Water-soluble organics and transition metals might potentially exert significant influence on particle OP.O_(3)aging notably decreased the OP of PM_(2.5)particles,possibly due to the oxidation of highly DTT-active components into low redox-active small molecules.Moreover,the evolution of OP in different PM_(2.5)components,including methanol-soluble and insoluble fractions,exhibited distinct responses to O_(3)aging for source-oriented PM_(2.5).Additionally,differences in chemical composition between fresh and aged PM_(2.5)were further elucidated through measurements of component-dependent hygroscopic behaviors and phase transitions.This study systematically delineates variances in the toxic potential of fresh and O_(3)-aged PM_(2.5)from various anthropogenic sources.The findings highlight the intrinsic compositional dependence of particle OP and provide essential insights for assessing the health effects of source-oriented PM_(2.5),as well as for formulating human health protection policies.展开更多
The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental result...The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental results have shown that in pp collisions,the size of the one-dimensional primordial source depends on the transverse mass(m_(T))of the hadron pairs,following a common scaling behavior similar to that observed in Pb-Pb collisions.In this study,a systematic analysis of the π-π source and correlation functions was performed using the multiphase transport model(AMPT)to understand the properties of the emitting source created in high-multiplicity pp collisions at√s=13 TeV.The mT-scaling behavior and pion emission source radii measured by the ALICE experiment can be described well by a model with a subnucleon structure.This work sheds new light on the effective size of the π-π emission source and the study of intensity interferometry in small systems using a transport model.展开更多
To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and...To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and plane location tests were carried out in the granite rod using two sensors and the cube of marble using four sensors, respectively. To compare the position accuracy between line and plane positions, the line poison test was also carried out on the marble surface. The results show that for line positioning, the maximum error of absolute distance is about 0.8 cm. With the speed difference of 200 m/s, the average value of absolute difference from the position error is about 0.4 cm. For the plane positioning, in the case of the sensor array of 30 cm, the absolute positioning distance is up to 8.7 cm. It can be seen that the sonic speed seriously impacts on the plane positioning accuracy. The plane positioning error is lager than the line positioning error, which means that when the line position can satisfy the need in practical engineering, it is better to use the line position instead of the plane location. The plane positioning error with the diagonal speed is the minimum one.展开更多
In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature...In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature extraction and the hierarchy support vector machine （H-SVM） classifier is proposed. After a four-level decomposition of the HWPT, the energy feature of AE signals in different frequency bands is extracted, which overcomes the shortcomings of the traditional wavelet packet including energy leakage, and inflexible frequency band selection and different frequency resolutions on different levels. The H-SVM classifier is trained with a subset of the experimental data for known AE source types and tested using the remaining set of data. The results of pressure-off experiments on the specimens of carbon fiber materials indicate that the proposed approach can effectively implement the AE source type identification, and has a better performance in terms of computational efficiency and identification accuracy than the wavelet packet （WPT） feature extraction.展开更多
The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of ...The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of 2007 were examined in a modeling study.The modeling system consisted of the Weather Research and Forecasting （WRF） model and the photochemical dispersion model,CAMx.The factor separation technique （FST） was used to quantify the effect of individual emission source types and the synergistic interactions among two or more types.Additionally,the effectiveness of emission reduction scenarios was explored.The industry,power plant,and transportation emission source types were found to be the most important in terms of their individual effects on O3DM.The key contributor to high surface O3 was power plant emissions,with a peak individual effect of 40 ppbv in the southwestern BTH area.The individual effect from the biogenic emission category was quite low.The synergistic effects from the combinations of each pair of anthropogenic emission types suppressed O3 formation,while the synergistic effects for combinations of three were favorable for O3 formation when the industrial and power plant emission source types coexisted.The quadruple synergistic effects were positive only with the combination of power plant,transportation,residential,and biogenic sources,while the quintuple synergistic effect showed only minor impacts on O3DM concentrations.A 30％ reduction in industrial and transportation sources produced the most effective impacts on O3 concentrations,with a maximum decrease of 20 ppbv.These results suggested that the synergistic impacts among emission source types should be considered when formulating emission control strategies for O3 reduction.展开更多
The soil type is a key factor influencing N(nitrogen)cycling in soil;however,gross N transformations and N_(2)O emission sources are still poorly understood.In this study,a laboratory 15N tracing experiment was carrie...The soil type is a key factor influencing N(nitrogen)cycling in soil;however,gross N transformations and N_(2)O emission sources are still poorly understood.In this study,a laboratory 15N tracing experiment was carried out at 60%WHC(water holding capacity)and 25℃to evaluate the gross N transformation rates and N_(2)O emission pathways in sandy loam and silt loam soils in a semi-arid region of Heilongjiang Province,China.The results showed that the gross rates of N mineralization,immobilization,and nitrification were 3.60,1.90,and 5.63 mg N/(kg·d)in silt loam soil,respectively,which were 3.62,4.26,and 3.13 times those in sandy loam soil,respectively.The ratios of the gross nitrification rate to the ammonium immobilization rate(n/ia)in sandy loam soil and silt loam soil were all higher than 1.00,whereas the n/ia in sandy loam soil(4.36)was significantly higher than that in silt loam soil(3.08).This result indicated that the ability of sandy loam soil to release and conserve the available N was relatively poor in comparison with silt loam soil,and the relatively strong nitrification rate compared to the immobilization rate may lead to N loss through NO_(3)–leaching.Under aerobic conditions,both nitrification and denitrification made contributions to N_(2)O emissions.Nitrification was the dominant pathway leading to N_(2)O production in soils and was responsible for 82.0%of the total emitted N_(2)O in sandy loam soil,which was significantly higher than that in silt loam soil(71.7%).However,the average contribution of denitrification to total N_(2)O production in sandy loam soil was 17.9%,which was significantly lower than that in silt loam soil(28.3%).These results are valuable for developing reasonable fertilization management and proposing effective greenhouse gas mitigation strategies in different soil types in semiarid regions.展开更多
The azimuthal distributions of final-state particles and fragments produced in high-energy nucleus-nucleus collisions are described by a modified multisource ideal gas model which contains the expansions and movements...The azimuthal distributions of final-state particles and fragments produced in high-energy nucleus-nucleus collisions are described by a modified multisource ideal gas model which contains the expansions and movements of the emission sources. The transverse structures of the sources are given in the transverse plane by momentum components Px and Py, and described by parameters in the model. The results of the azimuthal distributions, calculated by the Monte Carlo method, are in good agreement with the experimental data in nucleus-nucleus collisions at high energies.展开更多
Emissions derived from the consumption of organic solvents have been proven to be the primary industrial source of volatile organic compounds(VOCs).In conjunction with epidemiologic studies, water-based paints(WBPs) a...Emissions derived from the consumption of organic solvents have been proven to be the primary industrial source of volatile organic compounds(VOCs).In conjunction with epidemiologic studies, water-based paints(WBPs) and solvent-based paints(SBPs) were selected as representatives of newly developed solvents and traditional solvents, respectively,to simulate the effects of consuming solvents emitted during industrial production.And non-carcinogenic and carcinogenic risks to residents near emission sources were studied in detail.The results showed that the spatial distribution of health risks varied with meteorological conditions and type of emission source, and the prevailing wind direction strongly affected the distribution range and shape of the influenced area.The areas of influence maximized on heavy-polluting days for both WBP and SBP emission sources with the total span reaching 804 m and 16 km, respectively;meanwhile, the areas of influence for carcinogenic risk resulting from WBP emission sources were 1.2 and 2.3 times greater than those measured on fine and rainy days, respectively, and 1.8 and 2.9 times greater for SBP emission sources.Compared with WBPs, the total spans of negatively influenced regions resulting from SBP emission sources were 10.4, 12.5 and 19.9 times greater on fine, rainy and heavypolluting days, respectively.Therefore, carcinogenic risk was the dominant health threat for populations residing close to solvent-consuming industrial emission sources.The findings suggest that newly developed solvents are capable of significantly reducing consequent health threats, nevertheless, they could still pose occasional threats to nearby residents under specific meteorological conditions.展开更多
Monitoring sensors in complex engineering environments often record abnormal data,leading to significant positioning errors.To reduce the influence of abnormal arrival times,we introduce an innovative,outlier-robust l...Monitoring sensors in complex engineering environments often record abnormal data,leading to significant positioning errors.To reduce the influence of abnormal arrival times,we introduce an innovative,outlier-robust localization method that integrates kernel density estimation(KDE)with damping linear correction to enhance the precision of microseismic/acoustic emission(MS/AE)source positioning.Our approach systematically addresses abnormal arrival times through a three-step process:initial location by 4-arrival combinations,elimination of outliers based on three-dimensional KDE,and refinement using a linear correction with an adaptive damping factor.We validate our method through lead-breaking experiments,demonstrating over a 23%improvement in positioning accuracy with a maximum error of 9.12 mm(relative error of 15.80%)—outperforming 4 existing methods.Simulations under various system errors,outlier scales,and ratios substantiate our method’s superior performance.Field blasting experiments also confirm the practical applicability,with an average positioning error of 11.71 m(relative error of 7.59%),compared to 23.56,66.09,16.95,and 28.52 m for other methods.This research is significant as it enhances the robustness of MS/AE source localization when confronted with data anomalies.It also provides a practical solution for real-world engineering and safety monitoring applications.展开更多
A model of three-level amplified spontaneous emission(ASE)sources,considering radiation effect,is proposed to predict radiation induced loss of output power in radiation environment.Radiation absorption parameters of ...A model of three-level amplified spontaneous emission(ASE)sources,considering radiation effect,is proposed to predict radiation induced loss of output power in radiation environment.Radiation absorption parameters of ASE sources model are obtained by the fitting of color centers generation and recovery process of gain loss data at lower dose rate.Gain loss data at higher dose is applied for self-validating.This model takes both the influence of erbium ions absorption and photon bleaching effect into consideration,which makes the prediction of different dose and dose rate more accurate and flexible.The fitness value between ASE model and gain loss data is 99.98%,which also satisfies the extrapolation at the low dose rate.The method and model may serve as a valuable tool to predict ASE performance in harsh environment.展开更多
In order to evaluate the impacts of volatile organic compounds(VOCs)emissions from building materials on the indoor air quality beyond the standard chamber test conditions and test period,mechanistic emission source m...In order to evaluate the impacts of volatile organic compounds(VOCs)emissions from building materials on the indoor air quality beyond the standard chamber test conditions and test period,mechanistic emission source models have been developed in the past.However,very limited data are available for the required model parameters including the initial concentration(C_(m0)),in-material diffusion coefficient(D_(m)),partition coefficient(Kma),and convective mass transfer coefficient(k_(m)).In this study,a procedure was developed for estimating the model parameters by using VOC emission data from standard small chamber tests.In the procedure,initial values of the model parameters were refined by multivariate regression analysis of the measured emission data.To verify the procedure and estimate its uncertainty,simulated chamber test data were generated by adding 10% experimental uncertainties on the theoretical curve from the analytical solution to a mechanistic emission model.Then the procedure was applied to the generated data to estimate the model parameters.Results indicated that estimates converged to the original parameter values used for the data generation and the error of estimated parameters D_(m1)C_(m0) and K_(ma) were within±10%,±23%,and±25%of the true values,respectively.The procedure was further demonstrated by applying it to estimate the model parameters from real chamber test data.Wide application of the procedure would result in a database of mechanistic source model parameters for assessing the impact of VOC emissions on indoor pollution load,which are essential input data for evaluating the effectiveness of various indoor air quality(IAQ)design and control strategies as well as the energy required for meeting given IAQ requirements.展开更多
High-rise buildings form deep urban street canyons and restrict the dispersion of vehicle emissions,posing severe health risks to the public by aggravating roadside air quality.Field measurements are important for und...High-rise buildings form deep urban street canyons and restrict the dispersion of vehicle emissions,posing severe health risks to the public by aggravating roadside air quality.Field measurements are important for understanding the dispersion process of tailpipe emissions in street canyons,while a major challenge is the lack of a suitable tracer gas.Carbon dioxide(CO_(2)),which is safe to the public and inexpensive to obtain,can be reliably measured by existing gas analysers.This study investigated the suitability of using CO_(2)as a tracer gas for characterising vehicle emission dispersion in a real-world street canyon.The tracer gas was released via a line or point source,whose dispersion was characterised by a sensors network comprising low-cost air quality sensors.The results showed that the CO_(2)contained in the exhaust gas of a test vehicle itself had unmeasurable effect at roadsides.Both the line and point sources produced obvious CO_(2)level elevations at approximately 30 s after the test vehicle passed by.In addition,for both line and point sources,the CO_(2)elevations were much more distinct at the roadside next to tailpipe exit than the opposite side,and were higher at 0.8 m than 1.6 m above the ground.The present study demonstrated that using CO_(2)as a tracer gas is feasible for investigating vehicle emission dispersion in real-world street canyons.Future studies are needed to improve the gas release rate of the developed tracer gas systems for more reliable measurements and larger street canyons.展开更多
The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission （AE） sour...The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission （AE） sources of inner cracks in rail, AE sources with different types, depths and propagation distances are examined for crack in rail. The finite element method is utilized to model the rail with cracks and the results of experiment demonstrate the effectiveness of this model. Wavelet transform and Rayleigh-Lamb equations are utilized to extract the features of crack AE sources. The results illustrate that the intensity ratio among AE modes can identify the AE source types and the AE sources with different frequencies in rail. There are uniform AE mode features existing in the AE signals from AE sources in rail web, however AE signals from AE sources in rail head and rail base have the complex and unstable AE modes. Different AE source types have the different propagation features in rail. It is helpful to understand the rail cracks and detect the rail cracks based on the AE technique.展开更多
By establishing emission inventory of air pollution sources in Beijing,and classifying and compiling the pollutant types and corresponding pollution source data in more detail,it could provide the reference for studyi...By establishing emission inventory of air pollution sources in Beijing,and classifying and compiling the pollutant types and corresponding pollution source data in more detail,it could provide the reference for studying causes of haze and related policy impact assessment in Beijing.In this paper,selecting relevant data published in the Beijing Statistical Yearbook,referring to emission coefficients in the technical guidelines for the preparation of various pollution sources,and combining characteristics of energy consumption in Beijing,emission inventory of air pollution sources in six parts is established:thermal power plant,industrial combustion source(by industry),technological process source(by product variety),motor vehicle,building construction and residents life,and the contribution rate of each part to air pollutants is given.Finally,policy suggestions for haze control in Beijing are put forward.展开更多
Using the incomplete adjoint operator method in part I of this series of papers,the total emission source S can be retrieved from the pollutant concentrationsρob obtained from the air pollution monitoring network.Thi...Using the incomplete adjoint operator method in part I of this series of papers,the total emission source S can be retrieved from the pollutant concentrationsρob obtained from the air pollution monitoring network.This paper studies the problem of retrieving anthropogenic emission sources from S.Assuming that the natural source Sn is known,and as the internal source Sc due to chemical reactions is a function of pollutant concentrations,if the chemical reaction equations are complete and the parameters are accurate,Sc can be calculated directly fromρob,and then Sa can be obtained from S.However,if the chemical reaction parameters(denoted asγ)are insufficiently accurate,bothγand Sc should be corrected.This article proposes a"double correction iterative method"to retrieve Sc and correctγand proves that this iterative method converges.展开更多
Fine particulate matter(particulate matter with a diameter of 2.5μm or less;PM2.5)causes millions of premature deaths globally1,but not all particles are equally harmful2-4.Current air-pollution control strategies,pr...Fine particulate matter(particulate matter with a diameter of 2.5μm or less;PM2.5)causes millions of premature deaths globally1,but not all particles are equally harmful2-4.Current air-pollution control strategies,prioritizing PM2.5 mass reduction,have provided considerable health benefits but further refinements based on differences in the toxicity of various emission sources may provide greater benefits5-7.Here we integrated field measurements with air-quality modelling to assess the unequal toxicities of PM2.5 from various anthropogenic sources.展开更多
The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire ...The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire more accurate results.First,the SEI of secondary component precursors(SO2,NOx,NH3,and VOCs)was compiled to acquire the emission ratios of these sources for the precursors.Then,a regular CMB simulation was executed to obtain the contributions of primary particle sources and secondary components(SO4^2-,NO3^-3,NH4^+,and SOC).Afterwards,the contributions of secondary components were apportioned into primary sources according to the source emission ratios.The final source apportionment results combined the contributions of primary sources by CMB and SEI.This integrated approach was carried out via a case study of three coastal cities(Zhoushan,Taizhou,and Wenzhou;abbreviated WZ,TZ,and ZS)in Zhejiang Province,China.The regular CMB simulation results showed that PM2.5 pollution was mainly affected by secondary components and mobile sources.The SEI results indicated that electricity,industrial production and mobile sources were the largest contributors to the emission of PM2.5 gaseous precursors.The simulation results of the CMB-SEI model showed that PM2.5 pollution in the coastal areas of Zhejiang Province presented complex pollution characteristics dominated by mobile sources,electricity production sources and industrial production sources.Compared to the results of the CMB and SEI models alone,the CMB-SEI model completely apportioned PM2.5 to primary sources and simultaneously made the results more accurate and reliable in accordance with local industrial characteristics.展开更多
Although atmospheric CO_(2) observations are becoming increasingly widespread in China,the identification of CO_(2) emission sources is still scarce,especially in undeveloped Central China.To effectively address this ...Although atmospheric CO_(2) observations are becoming increasingly widespread in China,the identification of CO_(2) emission sources is still scarce,especially in undeveloped Central China.To effectively address this issue,in a typical site in Central China,the simultaneous measurements of atmospheric CO_(2),CO,andδ^(13)C were conducted,and the characteristics of CO_(2) emission sources were systematically investigated based on the relationships among CO_(2),CO,andδ^(13)C.The average CO_(2)/CO ratio of winter increased from 52.4 ppm/ppm during 2018–2020 to 65.1 ppm/ppm during 2021–2022,which confirmed the improvement of energy consumption efficiency in China.Air-mass transportation from central China and Yangtze River Delta regions contributed largely to higher CO_(2)/CO ratios in 2021–2022.A highermean CO_(2)/CO ratio appeared during the morning rush hours(60.3 ppm/ppm)than in the afternoon rush hours(51.4 ppm/ppm)in winter.In addition,the meanδ^(13)C value of CO_(2) sources(δ^(13)Cs)also displayed more negative values during the morning rush hours(-28.3‰)than the afternoon rush hours(-22.2‰),suggesting the significant influence of vehicle and natural gas usage at themorning rush hours and the impact of straw burning in the afternoon rush hours.The meanδ^(13)Cs was-24.7‰for winter and-21.9‰for vegetation season,implying the main contribution of coal in winter and the impact of C4 plants during the vegetation season.The contribution of biogenic respiration CO_(2) was inferred to exceed 50%during the nighttime of summer according to the obtained meanδ^(13)C value of biogenic respiration CO_(2),which was calculated to be-21.4‰.展开更多
To obtain a stable amplified spontaneous emission（ASE） source for complex environment applications, we design an ASE source and study the output power and spectral characteristics under different ambient temperature...To obtain a stable amplified spontaneous emission（ASE） source for complex environment applications, we design an ASE source and study the output power and spectral characteristics under different ambient temperatures.We optimize the structure of the ASE source to flatten the ASE spectrum, and study the output characteristics in terms of output power and optical spectrum under different pump powers. Then the performance of the ASE source is investigated in the temperature range from-18.9°C to 50°C. A stable-power and flat-spectrum ASE source can be obtained by structural optimization and pump control.展开更多
To study the pollution features and underlying mechanism of PM_(2.5) in Luoyang, a typical developing urban site in the central plain of China, 303 PM_(2.5) samples were collected from April 16 to December 29, 2015 to...To study the pollution features and underlying mechanism of PM_(2.5) in Luoyang, a typical developing urban site in the central plain of China, 303 PM_(2.5) samples were collected from April 16 to December 29, 2015 to analyze the elements, water soluble inorganic ions, organic carbon and elemental carbon. The annual mean concentration of PM_(2.5) was 142.3 μg/m^(3), and 75% of the daily PM_(2.5) concentrations exceeded the 75 μg/m^(3). The secondary inorganic ions, organic matter and mineral dust were the most abundant species, accounting for 39.6%, 19.2% and 9.3% of the total mass concentration, respectively. But the major chemical components showed clear seasonal dependence. SO_(4)^(2-) was most abundant specie in spring and summer, which related to intensive photochemical reaction under high O_3 concentration. In contrast, the secondary organic carbon and ammonium while primary organic carbon and ammonium significantly contributed to haze formation in autumn and winter, respectively. This indicated that the collaboration effect of secondary inorganic aerosols and carbonaceous matters result in heavy haze in autumn and winter. Six main sources were identified by positive matrix factorization model: industrial emission, combustion sources, traffic emission, mineral dust, oil combustion and secondary sulfate, with the annual contribution of 24%, 20%, 24%, 4%, 5% and 23%, respectively. The potential source contribution function analysis pointed that the contribution of the local and short-range regional transportation had significant impact. This result highlighted that local primary carbonaceous and precursor of secondary carbonaceous mitigation would be key to reduce PM_(2.5) and O_3 during heavy haze episodes in winter and autumn.展开更多
基金supported by the National Natural Science Foundation of China(No.42305109)Quzhou Municipal Science and Technology Bureau(No.2023K222).
文摘Inhalation of atmospheric PM_(2.5)can induce the generation of excessive reactive oxygen species(ROS)in human alveoli,triggering local and systemic inflammation,which can directly or indirectly result in respiratory and cardiovascular diseases.In this study,we assessed the oxidative potential(OP)of fresh and O_(3)-aged PM_(2.5)particles from various urban and rural emission sources using the dithiothreitol(DTT)method.Our results revealed variations in the OP of fresh PM_(2.5)among different emission sources,with biomass burning sources exhibiting the highest OP,followed by industrial areas,vehicular emissions,cooking emissions,and suburban areas,respectively.Water-soluble organics and transition metals might potentially exert significant influence on particle OP.O_(3)aging notably decreased the OP of PM_(2.5)particles,possibly due to the oxidation of highly DTT-active components into low redox-active small molecules.Moreover,the evolution of OP in different PM_(2.5)components,including methanol-soluble and insoluble fractions,exhibited distinct responses to O_(3)aging for source-oriented PM_(2.5).Additionally,differences in chemical composition between fresh and aged PM_(2.5)were further elucidated through measurements of component-dependent hygroscopic behaviors and phase transitions.This study systematically delineates variances in the toxic potential of fresh and O_(3)-aged PM_(2.5)from various anthropogenic sources.The findings highlight the intrinsic compositional dependence of particle OP and provide essential insights for assessing the health effects of source-oriented PM_(2.5),as well as for formulating human health protection policies.
基金the National Natural Science Foundation of China(Nos.12061141008,12147101,and 12322508)the Science and Technology Commission of Shanghai Municipality(23590780100)+1 种基金LZ acknowledges the support of the Fundamental Research Funds for the Central UniversitiesChina University of Geosciences(Wuhan),with No.G1323523064.
文摘The measurement of momentum correlations of identical pions serves as a fundamental tool for probing the space-time properties of a particle-emitting source created in high-energy collisions.Recent experimental results have shown that in pp collisions,the size of the one-dimensional primordial source depends on the transverse mass(m_(T))of the hadron pairs,following a common scaling behavior similar to that observed in Pb-Pb collisions.In this study,a systematic analysis of the π-π source and correlation functions was performed using the multiphase transport model(AMPT)to understand the properties of the emitting source created in high-multiplicity pp collisions at√s=13 TeV.The mT-scaling behavior and pion emission source radii measured by the ALICE experiment can be described well by a model with a subnucleon structure.This work sheds new light on the effective size of the π-π emission source and the study of intensity interferometry in small systems using a transport model.
基金Projects (50934006, 10872218) supported by the National Natural Science Foundation of ChinaProject (2010CB732004) supported by the National Basic Research Program of ChinaProject (kjdb2010-6) supported by Doctoral Candidate Innovation Research Support Program of Science & Technology Review, China
文摘To quantitatively study the location errors induced by deviation of sonic speed, the line and plane location tests were carried out. A broken pencil was simulated as acoustic emission source in the rocks. The line and plane location tests were carried out in the granite rod using two sensors and the cube of marble using four sensors, respectively. To compare the position accuracy between line and plane positions, the line poison test was also carried out on the marble surface. The results show that for line positioning, the maximum error of absolute distance is about 0.8 cm. With the speed difference of 200 m/s, the average value of absolute difference from the position error is about 0.4 cm. For the plane positioning, in the case of the sensor array of 30 cm, the absolute positioning distance is up to 8.7 cm. It can be seen that the sonic speed seriously impacts on the plane positioning accuracy. The plane positioning error is lager than the line positioning error, which means that when the line position can satisfy the need in practical engineering, it is better to use the line position instead of the plane location. The plane positioning error with the diagonal speed is the minimum one.
基金The Natural Science Foundation of Heilongjiang Province ( No. F201018)the National Natural Science Foundation of China( No. 60901042)
文摘In order to solve the fatigue damage identification problem of helicopter moving components, a new approach for acoustic emission （AE） source type identification based on the harmonic wavelet packet （HWPT） feature extraction and the hierarchy support vector machine （H-SVM） classifier is proposed. After a four-level decomposition of the HWPT, the energy feature of AE signals in different frequency bands is extracted, which overcomes the shortcomings of the traditional wavelet packet including energy leakage, and inflexible frequency band selection and different frequency resolutions on different levels. The H-SVM classifier is trained with a subset of the experimental data for known AE source types and tested using the remaining set of data. The results of pressure-off experiments on the specimens of carbon fiber materials indicate that the proposed approach can effectively implement the AE source type identification, and has a better performance in terms of computational efficiency and identification accuracy than the wavelet packet （WPT） feature extraction.
基金jointly supported by a key project of the Chinese Academy of Sciences (Grant No. XDB05030301)the National Natural Science Foundation of China (Grant Nos. 40905055 and 41175105)the special fund of the State Key Joint Laboratory of Environment Simulation and Pollution Control (Grant No. 13K04ESPCP)
文摘The impacts of emissions from industry,power plant,transportation,residential,and biogenic sources on daily maximum surface ozone （O3DM） over the Beijing-Tianjin-Hebei （BTH） region in North China in the summer of 2007 were examined in a modeling study.The modeling system consisted of the Weather Research and Forecasting （WRF） model and the photochemical dispersion model,CAMx.The factor separation technique （FST） was used to quantify the effect of individual emission source types and the synergistic interactions among two or more types.Additionally,the effectiveness of emission reduction scenarios was explored.The industry,power plant,and transportation emission source types were found to be the most important in terms of their individual effects on O3DM.The key contributor to high surface O3 was power plant emissions,with a peak individual effect of 40 ppbv in the southwestern BTH area.The individual effect from the biogenic emission category was quite low.The synergistic effects from the combinations of each pair of anthropogenic emission types suppressed O3 formation,while the synergistic effects for combinations of three were favorable for O3 formation when the industrial and power plant emission source types coexisted.The quadruple synergistic effects were positive only with the combination of power plant,transportation,residential,and biogenic sources,while the quintuple synergistic effect showed only minor impacts on O3DM concentrations.A 30％ reduction in industrial and transportation sources produced the most effective impacts on O3 concentrations,with a maximum decrease of 20 ppbv.These results suggested that the synergistic impacts among emission source types should be considered when formulating emission control strategies for O3 reduction.
基金financed by the National Natural Science Foundation of China(41301345,41101284)。
文摘The soil type is a key factor influencing N(nitrogen)cycling in soil;however,gross N transformations and N_(2)O emission sources are still poorly understood.In this study,a laboratory 15N tracing experiment was carried out at 60%WHC(water holding capacity)and 25℃to evaluate the gross N transformation rates and N_(2)O emission pathways in sandy loam and silt loam soils in a semi-arid region of Heilongjiang Province,China.The results showed that the gross rates of N mineralization,immobilization,and nitrification were 3.60,1.90,and 5.63 mg N/(kg·d)in silt loam soil,respectively,which were 3.62,4.26,and 3.13 times those in sandy loam soil,respectively.The ratios of the gross nitrification rate to the ammonium immobilization rate(n/ia)in sandy loam soil and silt loam soil were all higher than 1.00,whereas the n/ia in sandy loam soil(4.36)was significantly higher than that in silt loam soil(3.08).This result indicated that the ability of sandy loam soil to release and conserve the available N was relatively poor in comparison with silt loam soil,and the relatively strong nitrification rate compared to the immobilization rate may lead to N loss through NO_(3)–leaching.Under aerobic conditions,both nitrification and denitrification made contributions to N_(2)O emissions.Nitrification was the dominant pathway leading to N_(2)O production in soils and was responsible for 82.0%of the total emitted N_(2)O in sandy loam soil,which was significantly higher than that in silt loam soil(71.7%).However,the average contribution of denitrification to total N_(2)O production in sandy loam soil was 17.9%,which was significantly lower than that in silt loam soil(28.3%).These results are valuable for developing reasonable fertilization management and proposing effective greenhouse gas mitigation strategies in different soil types in semiarid regions.
基金Project supported by the National Natural Science Foundation of China （Grant Nos 10275042 and 10475054）, the Shanxi Provincial Natural Science Foundation （Grant No 20021006）, and the Shanxi Provincial 1Foundation for Returned 0verseas Scholars.
文摘The azimuthal distributions of final-state particles and fragments produced in high-energy nucleus-nucleus collisions are described by a modified multisource ideal gas model which contains the expansions and movements of the emission sources. The transverse structures of the sources are given in the transverse plane by momentum components Px and Py, and described by parameters in the model. The results of the azimuthal distributions, calculated by the Monte Carlo method, are in good agreement with the experimental data in nucleus-nucleus collisions at high energies.
基金supported by the Ministry of Science and Technology of the People’s Republic of China (No.2020YFC1806303)the Beijing Municipal Science & Technology Commission (No.Z171100004417029)。
文摘Emissions derived from the consumption of organic solvents have been proven to be the primary industrial source of volatile organic compounds(VOCs).In conjunction with epidemiologic studies, water-based paints(WBPs) and solvent-based paints(SBPs) were selected as representatives of newly developed solvents and traditional solvents, respectively,to simulate the effects of consuming solvents emitted during industrial production.And non-carcinogenic and carcinogenic risks to residents near emission sources were studied in detail.The results showed that the spatial distribution of health risks varied with meteorological conditions and type of emission source, and the prevailing wind direction strongly affected the distribution range and shape of the influenced area.The areas of influence maximized on heavy-polluting days for both WBP and SBP emission sources with the total span reaching 804 m and 16 km, respectively;meanwhile, the areas of influence for carcinogenic risk resulting from WBP emission sources were 1.2 and 2.3 times greater than those measured on fine and rainy days, respectively, and 1.8 and 2.9 times greater for SBP emission sources.Compared with WBPs, the total spans of negatively influenced regions resulting from SBP emission sources were 10.4, 12.5 and 19.9 times greater on fine, rainy and heavypolluting days, respectively.Therefore, carcinogenic risk was the dominant health threat for populations residing close to solvent-consuming industrial emission sources.The findings suggest that newly developed solvents are capable of significantly reducing consequent health threats, nevertheless, they could still pose occasional threats to nearby residents under specific meteorological conditions.
基金the financial support provided by the National Key Research and Development Program for Young Scientists(No.2021YFC2900400)Postdoctoral Fellowship Program of China Postdoctoral Science Foundation(CPSF)(No.GZB20230914)+2 种基金National Natural Science Foundation of China(No.52304123)China Postdoctoral Science Foundation(No.2023M730412)Chongqing Outstanding Youth Science Foundation Program(No.CSTB2023NSCQ-JQX0027).
文摘Monitoring sensors in complex engineering environments often record abnormal data,leading to significant positioning errors.To reduce the influence of abnormal arrival times,we introduce an innovative,outlier-robust localization method that integrates kernel density estimation(KDE)with damping linear correction to enhance the precision of microseismic/acoustic emission(MS/AE)source positioning.Our approach systematically addresses abnormal arrival times through a three-step process:initial location by 4-arrival combinations,elimination of outliers based on three-dimensional KDE,and refinement using a linear correction with an adaptive damping factor.We validate our method through lead-breaking experiments,demonstrating over a 23%improvement in positioning accuracy with a maximum error of 9.12 mm(relative error of 15.80%)—outperforming 4 existing methods.Simulations under various system errors,outlier scales,and ratios substantiate our method’s superior performance.Field blasting experiments also confirm the practical applicability,with an average positioning error of 11.71 m(relative error of 7.59%),compared to 23.56,66.09,16.95,and 28.52 m for other methods.This research is significant as it enhances the robustness of MS/AE source localization when confronted with data anomalies.It also provides a practical solution for real-world engineering and safety monitoring applications.
基金supported by the Aeronautical Science Foundation of China(Grant No.20170851007)。
文摘A model of three-level amplified spontaneous emission(ASE)sources,considering radiation effect,is proposed to predict radiation induced loss of output power in radiation environment.Radiation absorption parameters of ASE sources model are obtained by the fitting of color centers generation and recovery process of gain loss data at lower dose rate.Gain loss data at higher dose is applied for self-validating.This model takes both the influence of erbium ions absorption and photon bleaching effect into consideration,which makes the prediction of different dose and dose rate more accurate and flexible.The fitness value between ASE model and gain loss data is 99.98%,which also satisfies the extrapolation at the low dose rate.The method and model may serve as a valuable tool to predict ASE performance in harsh environment.
文摘In order to evaluate the impacts of volatile organic compounds(VOCs)emissions from building materials on the indoor air quality beyond the standard chamber test conditions and test period,mechanistic emission source models have been developed in the past.However,very limited data are available for the required model parameters including the initial concentration(C_(m0)),in-material diffusion coefficient(D_(m)),partition coefficient(Kma),and convective mass transfer coefficient(k_(m)).In this study,a procedure was developed for estimating the model parameters by using VOC emission data from standard small chamber tests.In the procedure,initial values of the model parameters were refined by multivariate regression analysis of the measured emission data.To verify the procedure and estimate its uncertainty,simulated chamber test data were generated by adding 10% experimental uncertainties on the theoretical curve from the analytical solution to a mechanistic emission model.Then the procedure was applied to the generated data to estimate the model parameters.Results indicated that estimates converged to the original parameter values used for the data generation and the error of estimated parameters D_(m1)C_(m0) and K_(ma) were within±10%,±23%,and±25%of the true values,respectively.The procedure was further demonstrated by applying it to estimate the model parameters from real chamber test data.Wide application of the procedure would result in a database of mechanistic source model parameters for assessing the impact of VOC emissions on indoor pollution load,which are essential input data for evaluating the effectiveness of various indoor air quality(IAQ)design and control strategies as well as the energy required for meeting given IAQ requirements.
基金supported by the Environment and Conservation Fund(No.ECF 14/2018)of the Hong Kong SAR Government,China.
文摘High-rise buildings form deep urban street canyons and restrict the dispersion of vehicle emissions,posing severe health risks to the public by aggravating roadside air quality.Field measurements are important for understanding the dispersion process of tailpipe emissions in street canyons,while a major challenge is the lack of a suitable tracer gas.Carbon dioxide(CO_(2)),which is safe to the public and inexpensive to obtain,can be reliably measured by existing gas analysers.This study investigated the suitability of using CO_(2)as a tracer gas for characterising vehicle emission dispersion in a real-world street canyon.The tracer gas was released via a line or point source,whose dispersion was characterised by a sensors network comprising low-cost air quality sensors.The results showed that the CO_(2)contained in the exhaust gas of a test vehicle itself had unmeasurable effect at roadsides.Both the line and point sources produced obvious CO_(2)level elevations at approximately 30 s after the test vehicle passed by.In addition,for both line and point sources,the CO_(2)elevations were much more distinct at the roadside next to tailpipe exit than the opposite side,and were higher at 0.8 m than 1.6 m above the ground.The present study demonstrated that using CO_(2)as a tracer gas is feasible for investigating vehicle emission dispersion in real-world street canyons.Future studies are needed to improve the gas release rate of the developed tracer gas systems for more reliable measurements and larger street canyons.
基金supported by the China Scholarship Council,the National Natural Science Foundation of China(61171197,61201307,61371045)the Innovation Funds of Harbin Institute of Technology(Grant IDGA18102011)the Promotive Research Fund for Excellent Young and Middle-Aged Scientisits of Shandong Province(BS2010DX001)
文摘The safety of rail is very important for the development of high speed railway, and it is necessary to investigate the features of inner cracks in rail. In order to obtain the features of Acoustic Emission （AE） sources of inner cracks in rail, AE sources with different types, depths and propagation distances are examined for crack in rail. The finite element method is utilized to model the rail with cracks and the results of experiment demonstrate the effectiveness of this model. Wavelet transform and Rayleigh-Lamb equations are utilized to extract the features of crack AE sources. The results illustrate that the intensity ratio among AE modes can identify the AE source types and the AE sources with different frequencies in rail. There are uniform AE mode features existing in the AE signals from AE sources in rail web, however AE signals from AE sources in rail head and rail base have the complex and unstable AE modes. Different AE source types have the different propagation features in rail. It is helpful to understand the rail cracks and detect the rail cracks based on the AE technique.
基金Supported by Beijing Natural Science Foundation Project(9192002)Key Project of Beijing Social Science Foundation(19YJA002).
文摘By establishing emission inventory of air pollution sources in Beijing,and classifying and compiling the pollutant types and corresponding pollution source data in more detail,it could provide the reference for studying causes of haze and related policy impact assessment in Beijing.In this paper,selecting relevant data published in the Beijing Statistical Yearbook,referring to emission coefficients in the technical guidelines for the preparation of various pollution sources,and combining characteristics of energy consumption in Beijing,emission inventory of air pollution sources in six parts is established:thermal power plant,industrial combustion source(by industry),technological process source(by product variety),motor vehicle,building construction and residents life,and the contribution rate of each part to air pollutants is given.Finally,policy suggestions for haze control in Beijing are put forward.
基金supported by the National Natural Science Foundation of China(Grant Nos.41630530&41877316)the Key Research Program of Frontier Sciences,Chinese Academy of Sciences(Grant No.QYZDY-SSW-DQC002)the Youth Innovation Promotion Association,Chinese Academy of Sciences(Grant No.2019079)。
文摘Using the incomplete adjoint operator method in part I of this series of papers,the total emission source S can be retrieved from the pollutant concentrationsρob obtained from the air pollution monitoring network.This paper studies the problem of retrieving anthropogenic emission sources from S.Assuming that the natural source Sn is known,and as the internal source Sc due to chemical reactions is a function of pollutant concentrations,if the chemical reaction equations are complete and the parameters are accurate,Sc can be calculated directly fromρob,and then Sa can be obtained from S.However,if the chemical reaction parameters(denoted asγ)are insufficiently accurate,bothγand Sc should be corrected.This article proposes a"double correction iterative method"to retrieve Sc and correctγand proves that this iterative method converges.
文摘Fine particulate matter(particulate matter with a diameter of 2.5μm or less;PM2.5)causes millions of premature deaths globally1,but not all particles are equally harmful2-4.Current air-pollution control strategies,prioritizing PM2.5 mass reduction,have provided considerable health benefits but further refinements based on differences in the toxicity of various emission sources may provide greater benefits5-7.Here we integrated field measurements with air-quality modelling to assess the unequal toxicities of PM2.5 from various anthropogenic sources.
基金supported by the National Key Research and Development Program of China(No.2018YFC0214102)。
文摘The source apportionment of PM2.5 is essential for pollution prevention.In view of the weaknesses of individual models,we proposed an integrated chemical mass balancesource emission inventory(CMB-SEI)model to acquire more accurate results.First,the SEI of secondary component precursors(SO2,NOx,NH3,and VOCs)was compiled to acquire the emission ratios of these sources for the precursors.Then,a regular CMB simulation was executed to obtain the contributions of primary particle sources and secondary components(SO4^2-,NO3^-3,NH4^+,and SOC).Afterwards,the contributions of secondary components were apportioned into primary sources according to the source emission ratios.The final source apportionment results combined the contributions of primary sources by CMB and SEI.This integrated approach was carried out via a case study of three coastal cities(Zhoushan,Taizhou,and Wenzhou;abbreviated WZ,TZ,and ZS)in Zhejiang Province,China.The regular CMB simulation results showed that PM2.5 pollution was mainly affected by secondary components and mobile sources.The SEI results indicated that electricity,industrial production and mobile sources were the largest contributors to the emission of PM2.5 gaseous precursors.The simulation results of the CMB-SEI model showed that PM2.5 pollution in the coastal areas of Zhejiang Province presented complex pollution characteristics dominated by mobile sources,electricity production sources and industrial production sources.Compared to the results of the CMB and SEI models alone,the CMB-SEI model completely apportioned PM2.5 to primary sources and simultaneously made the results more accurate and reliable in accordance with local industrial characteristics.
基金supported by the National Natural Science Foundation of China(No.42105159)the Key Technologies Research and Development Program(No.2022YFF0606400)+2 种基金China Meteorological Administration“Research on value realization of climate ecological products”Youth Innovation Team Project(No.CMA2024QN15)Jiangxi Meteorological Technology Project(Nos.JX2021Z06,JX2022Z03,and JX2023Z03)the Joint Open Fund of the Institute of Atmospheric Environment,China Meteorological Administration,Shenyang and Key Laboratory of Agro-Meteorological Disasters of Liaoning Province(No.2024SYIAEKFZD05)。
文摘Although atmospheric CO_(2) observations are becoming increasingly widespread in China,the identification of CO_(2) emission sources is still scarce,especially in undeveloped Central China.To effectively address this issue,in a typical site in Central China,the simultaneous measurements of atmospheric CO_(2),CO,andδ^(13)C were conducted,and the characteristics of CO_(2) emission sources were systematically investigated based on the relationships among CO_(2),CO,andδ^(13)C.The average CO_(2)/CO ratio of winter increased from 52.4 ppm/ppm during 2018–2020 to 65.1 ppm/ppm during 2021–2022,which confirmed the improvement of energy consumption efficiency in China.Air-mass transportation from central China and Yangtze River Delta regions contributed largely to higher CO_(2)/CO ratios in 2021–2022.A highermean CO_(2)/CO ratio appeared during the morning rush hours(60.3 ppm/ppm)than in the afternoon rush hours(51.4 ppm/ppm)in winter.In addition,the meanδ^(13)C value of CO_(2) sources(δ^(13)Cs)also displayed more negative values during the morning rush hours(-28.3‰)than the afternoon rush hours(-22.2‰),suggesting the significant influence of vehicle and natural gas usage at themorning rush hours and the impact of straw burning in the afternoon rush hours.The meanδ^(13)Cs was-24.7‰for winter and-21.9‰for vegetation season,implying the main contribution of coal in winter and the impact of C4 plants during the vegetation season.The contribution of biogenic respiration CO_(2) was inferred to exceed 50%during the nighttime of summer according to the obtained meanδ^(13)C value of biogenic respiration CO_(2),which was calculated to be-21.4‰.
基金Supported by the National Natural Science Foundation of China under Grant No 11504320
文摘To obtain a stable amplified spontaneous emission（ASE） source for complex environment applications, we design an ASE source and study the output power and spectral characteristics under different ambient temperatures.We optimize the structure of the ASE source to flatten the ASE spectrum, and study the output characteristics in terms of output power and optical spectrum under different pump powers. Then the performance of the ASE source is investigated in the temperature range from-18.9°C to 50°C. A stable-power and flat-spectrum ASE source can be obtained by structural optimization and pump control.
基金supported by the Ministry of Science and Technology of China(No.2017YFC0210000)the National Natural Science Foundation of China(No.41807327)the Program for Innovative Research Team in Science and Technology in University of Henan Province(No.20 IRTSTHN011)。
文摘To study the pollution features and underlying mechanism of PM_(2.5) in Luoyang, a typical developing urban site in the central plain of China, 303 PM_(2.5) samples were collected from April 16 to December 29, 2015 to analyze the elements, water soluble inorganic ions, organic carbon and elemental carbon. The annual mean concentration of PM_(2.5) was 142.3 μg/m^(3), and 75% of the daily PM_(2.5) concentrations exceeded the 75 μg/m^(3). The secondary inorganic ions, organic matter and mineral dust were the most abundant species, accounting for 39.6%, 19.2% and 9.3% of the total mass concentration, respectively. But the major chemical components showed clear seasonal dependence. SO_(4)^(2-) was most abundant specie in spring and summer, which related to intensive photochemical reaction under high O_3 concentration. In contrast, the secondary organic carbon and ammonium while primary organic carbon and ammonium significantly contributed to haze formation in autumn and winter, respectively. This indicated that the collaboration effect of secondary inorganic aerosols and carbonaceous matters result in heavy haze in autumn and winter. Six main sources were identified by positive matrix factorization model: industrial emission, combustion sources, traffic emission, mineral dust, oil combustion and secondary sulfate, with the annual contribution of 24%, 20%, 24%, 4%, 5% and 23%, respectively. The potential source contribution function analysis pointed that the contribution of the local and short-range regional transportation had significant impact. This result highlighted that local primary carbonaceous and precursor of secondary carbonaceous mitigation would be key to reduce PM_(2.5) and O_3 during heavy haze episodes in winter and autumn.
