In recent decades,control performance monitoring(CPM)has experienced remarkable progress in research and industrial applications.While CPM research has been investigated using various benchmarks,the historical data be...In recent decades,control performance monitoring(CPM)has experienced remarkable progress in research and industrial applications.While CPM research has been investigated using various benchmarks,the historical data benchmark(HIS)has garnered the most attention due to its practicality and effectiveness.However,existing CPM reviews usually focus on the theoretical benchmark,and there is a lack of an in-depth review that thoroughly explores HIS-based methods.In this article,a comprehensive overview of HIS-based CPM is provided.First,we provide a novel static-dynamic perspective on data-level manifestations of control performance underlying typical controller capacities including regulation and servo:static and dynamic properties.The static property portrays time-independent variability in system output,and the dynamic property describes temporal behavior driven by closed-loop feedback.Accordingly,existing HIS-based CPM approaches and their intrinsic motivations are classified and analyzed from these two perspectives.Specifically,two mainstream solutions for CPM methods are summarized,including static analysis and dynamic analysis,which match data-driven techniques with actual controlling behavior.Furthermore,this paper also points out various opportunities and challenges faced in CPM for modern industry and provides promising directions in the context of artificial intelligence for inspiring future research.展开更多
In the leakage detection of reservoir dam bodies,traditional geophysical methods can only achieve one-time detection.Meanwhile,due to the non-uniqueness of geophysicalin version,how to improve the fidelity of geophysi...In the leakage detection of reservoir dam bodies,traditional geophysical methods can only achieve one-time detection.Meanwhile,due to the non-uniqueness of geophysicalin version,how to improve the fidelity of geophysical detection inversion profiles has become a key challenge in the industry.This study aims to construct a long-term real-time monitoring system using the time-lapse resistivity method,reveal the spatiotemporal evolution law of dam leakage,and provide technical support for accurate treatment.By integrating the Internet of Things(IoT),5G technology,and AI technology,real-time data acquisition,real-time transmission,and automatic inversionare realized.Through dynamic imaging analysis of the electrical anomaly characteristics of the leakage area and comparison between corresponding rainfall events,the leakage range and resistivity changes,the reliability and efficiency of dam leakagedete ction are significantly improved.This achieves long-termdynamic monitoring of dam leakage and provides a new perspective for the safe operation and maintenance of reservoirs.展开更多
In common practice in the oil fields,the injection of water and gas into reservoirs is a crucial technique to increase production.The control of the waterflooding front in oil/gas exploitation is a matter of great con...In common practice in the oil fields,the injection of water and gas into reservoirs is a crucial technique to increase production.The control of the waterflooding front in oil/gas exploitation is a matter of great concern to reservoir engineers.Monitoring the waterflooding front in oil/gas wells plays a very important role in adjusting the well network and later in production,taking advantage of the remaining oil po-tential and ultimately achieving great success in improving the recovery rate.For a long time,micro-seismic monitoring,numerical simulation,four-dimensional seismic and other methods have been widely used in waterflooding front monitoring.However,reconciling their reliability and cost poses a significant challenge.In order to achieve real-time,reliable and cost-effective monitoring,we propose an innovative method for waterflooding front monitoring through the similarity analysis of passive source time-lapse seismic images.Typically,passive source seismic data collected from oil fields have extremely low signal-to-noise ratio(SNR),which poses a serious problem for obtaining structural images.The proposed method aims to visualize and analyze underground changes by highlighting time-lapse images and provide a strategy for underground monitoring using long-term passive source data under low SNR conditions.First,we verify the feasibility of the proposed method by designing a theoretical model.Then,we conduct an analysis of the correlation coefficient(similarity)on the passive source time-lapse seismic imaging results to enhance the image differences and identify the simulated waterflooding fronts.Finally,the proposed method is applied to the actual waterflooding front monitoring tasks in Shengli Oilfield,China.The research findings indicate that the monitoring results are consistent with the actual devel-opment conditions,which in turn demonstrates that the proposed method has great potential for practical application and is very suitable for monitoring common development tasks in oil fields.展开更多
Addressing the current challenges in transforming pixel displacement into physical displacement in visual monitoring technologies,as well as the inability to achieve precise full-field monitoring,this paper proposes a...Addressing the current challenges in transforming pixel displacement into physical displacement in visual monitoring technologies,as well as the inability to achieve precise full-field monitoring,this paper proposes a method for identifying the structural dynamic characteristics of wind turbines based on visual monitoring data fusion.Firstly,the Lucas-Kanade Tomasi(LKT)optical flow method and a multi-region of interest(ROI)monitoring structure are employed to track pixel displacements,which are subsequently subjected to band pass filtering and resampling operations.Secondly,the actual displacement time history is derived through double integration of the acquired acceleration data and subsequent band pass filtering.The scale factor is obtained by applying the least squares method to compare the visual displacement with the displacement derived from double integration of the acceleration data.Based on this,the multi-point displacement time histories under physical coordinates are obtained using the vision data and the scale factor.Subsequently,when visual monitoring of displacements becomes impossible due to issues such as image blurring or lens occlusion,the structural vibration equation and boundary condition constraints,among other key parameters,are employed to predict the displacements at unknown monitoring points,thereby enabling full-field displacement monitoring and dynamic characteristic testing of the structure.Finally,a small-scale shaking table test was conducted on a simulated wind turbine structure undergoing shutdown to validate the dynamic characteristics of the proposed method through test verification.The research results indicate that the proposed method achieves a time-domain error within the submillimeter range and a frequency-domain accuracy of over 99%,effectively monitoring the full-field structural dynamic characteristics of wind turbines and providing a basis for the condition assessment of wind turbine structures.展开更多
Dynamic stress adjustment in deep-buried high geostress hard rock tunnels frequently triggers catastrophic failures such as rockbursts and collapses.While a comprehensive understanding of this process is critical for ...Dynamic stress adjustment in deep-buried high geostress hard rock tunnels frequently triggers catastrophic failures such as rockbursts and collapses.While a comprehensive understanding of this process is critical for evaluating surrounding rock stability,its dynamic evolution are often overlooked in engineering practice.This study systematically summarizes a novel classification framework for stress adjustment types—stabilizing(two-zoned),shallow failure(three-zoned),and deep failure(four-zoned)—characterized by distinct stress adjustment stages.A dynamic interpretation technology system is developed based on microseismic monitoring,integrating key microseismic parameters(energy index EI,apparent stressσa,microseismic activity S),seismic source parameter space clustering,and microseismic paths.This approach enables precise identification of evolutionary stages,stress adjustment types,and failure precursors,thereby elucidating the intrinsic linkage between geomechanical processes(stress redistribution)and failure risks.The study establishes criteria and procedures for identifying stress adjustment types and their associated failure risks,which were successfully applied in the Grand Canyon Tunnel of the E-han Highway to detect 50 instances of disaster risks.The findings offer invaluable insights into understanding the evolution process of stress adjustment and pinpointing the disaster risks linked to hard rock in comparable high geostress tunnels.展开更多
This study developed a digital twin(DT)and structural health monitoring(SHM)system for a balanced cantilever bridge,utilizing advanced measurement techniques to enhance accuracy.Vibration and dynamic strain measuremen...This study developed a digital twin(DT)and structural health monitoring(SHM)system for a balanced cantilever bridge,utilizing advanced measurement techniques to enhance accuracy.Vibration and dynamic strain measurements were obtained using accelerometers and piezo-resistive strain gauges,capturing low-magnitude dynamic strains during operational vibrations.3D-LiDAR scanning and Ultrasonic Pulse Velocity(UPV)tests captured the bridge's as-is geometry and modulus of elasticity.The resulting detailed 3D point cloud model revealed the structure's true state and highlighted discrepancies between the as-designed and as-built conditions.Dynamic properties,including modal frequencies and shapes,were extracted from the strain and acceleration measurements,providing critical insights into the bridge's structural behavior.The neutral axis depth,indicating stress distribution and potential damage,was accurately determined.Good agreement between vibration measurement data and the as-is model results validated the reliability of the digital twin model.Dynamic strain patterns and neutral axis parameters showed strong correlation with model predictions,serving as sensitive indicators of local damage.The baseline digital twin model and measurement results establish a foundation for future bridge inspections and investigations.This study demonstrates the effectiveness of combining digital twin technology with field measurements for real-time monitoring and predictive maintenance,ensuring the sustainability and safety of the bridge infrastructure,thereby enhancing its overall resilience to operational and environmental stressors.展开更多
Data-driven process monitoring is an effective approach to assure safe operation of modern manufacturing and energy systems,such as thermal power plants being studied in this work.Industrial processes are inherently d...Data-driven process monitoring is an effective approach to assure safe operation of modern manufacturing and energy systems,such as thermal power plants being studied in this work.Industrial processes are inherently dynamic and need to be monitored using dynamic algorithms.Mainstream dynamic algorithms rely on concatenating current measurement with past data.This work proposes a new,alternative dynamic process monitoring algorithm,using dot product feature analysis(DPFA).DPFA computes the dot product of consecutive samples,thus naturally capturing the process dynamics through temporal correlation.At the same time,DPFA's online computational complexity is lower than not just existing dynamic algorithms,but also classical static algorithms(e.g.,principal component analysis and slow feature analysis).The detectability of the new algorithm is analyzed for three types of faults typically seen in process systems:sensor bias,process fault and gain change fault.Through experiments with a numerical example and real data from a thermal power plant,the DPFA algorithm is shown to be superior to the state-of-the-art methods,in terms of better monitoring performance(fault detection rate and false alarm rate)and lower computational complexity.展开更多
Biotite content critically influences rock mechanical behavior and threatens underground engineering stability.Uniaxial compression tests with acoustic emission(AE)monitoring were conducted on granite pegmatite sample...Biotite content critically influences rock mechanical behavior and threatens underground engineering stability.Uniaxial compression tests with acoustic emission(AE)monitoring were conducted on granite pegmatite samples having varying biotite content.Peak frequency distribution analysis,rise angleaverage frequency(RA-AF)analysis,multifractal theory,and a dynamic multifractal algorithm were applied to explore the relationship between damage evolution and AE characteristics.Results indicate that increased biotite content reduces uniaxial compressive strength and elastic modulus,enhances plastic deformation,and increases the proportion of shear cracks.The segmented evolution of the dynamic multifractal parameter Δα_(m) is biotite-dependent.Oscillations during the elastic phase signify localized shear crack initiation and propagation;their attenuation in the plastic phase reflects frictional closure along biotite cleavage planes,promoting elastic energy storage and delaying release.AE-based damage models and time-varying signals characterize rock damage progression.Stress concentrations around biotite minerals foster localized shear band formation,leading to concentrated shear failure at lower damage levels.Higher biotite content accelerates crack propagation,while smooth cleavage planes lower the fracture energy threshold,reducing strength and stiffness.These findings enhance understanding of biotite-influenced progressive rock damage and underpin stability monitoring and early-warning systems for underground engineering.展开更多
Kernel-based slow feature analysis(SFA)methods have been successfully applied in the industrial process fault detection field.However,kernel-based SFA methods have high computational complexity as dealing with nonline...Kernel-based slow feature analysis(SFA)methods have been successfully applied in the industrial process fault detection field.However,kernel-based SFA methods have high computational complexity as dealing with nonlinearity,leading to delays in detecting time-varying data features.Additionally,the uncertain kernel function and kernel parameters limit the ability of the extracted features to express process characteristics,resulting in poor fault detection performance.To alleviate the above problems,a novel randomized auto-regressive dynamic slow feature analysis(RRDSFA)method is proposed to simultaneously monitor the operating point deviations and process dynamic faults,enabling real-time monitoring of data features in industrial processes.Firstly,the proposed Random Fourier mappingbased method achieves more effective nonlinear transformation,contrasting with the current kernelbased RDSFA algorithm that may lead to significant computational complexity.Secondly,a randomized RDSFA model is developed to extract nonlinear dynamic slow features.Furthermore,a Bayesian inference-based overall fault monitoring model including all RRDSFA sub-models is developed to overcome the randomness of random Fourier mapping.Finally,the superiority and effectiveness of the proposed monitoring method are demonstrated through a numerical case and a simulation of continuous stirred tank reactor.展开更多
A rapidly growing field is piezoresistive sensor for accurate respiration rate monitoring to suppress the worldwide respiratory illness.However,a large neglected issue is the sensing durability and accuracy without in...A rapidly growing field is piezoresistive sensor for accurate respiration rate monitoring to suppress the worldwide respiratory illness.However,a large neglected issue is the sensing durability and accuracy without interference since the expiratory pressure always coupled with external humidity and temperature variations,as well as mechanical motion artifacts.Herein,a robust and biodegradable piezoresistive sensor is reported that consists of heterogeneous MXene/cellulose-gelation sensing layer and Ag-based interdigital electrode,featuring customizable cylindrical interface arrangement and compact hierarchical laminated architecture for collectively regulating the piezoresistive response and mechanical robustness,thereby realizing the long-term breath-induced pressure detection.Notably,molecular dynamics simulations reveal the frequent angle inversion and reorientation of MXene/cellulose in vacuum filtration,driven by shear forces and interfacial interactions,which facilitate the establishment of hydrogen bonds and optimize the architecture design in sensing layer.The resultant sensor delivers unprecedented collection features of superior stability for off-axis deformation(0-120°,~2.8×10^(-3) A)and sensing accuracy without crosstalk(humidity 50%-100%and temperature 30-80).Besides,the sensor-embedded mask together with machine learning models is achieved to train and classify the respiration status for volunteers with different ages(average prediction accuracy~90%).It is envisioned that the customizable architecture design and sensor paradigm will shed light on the advanced stability of sustainable electronics and pave the way for the commercial application in respiratory monitory.展开更多
Advanced traffic monitoring systems encounter substantial challenges in vehicle detection and classification due to the limitations of conventional methods,which often demand extensive computational resources and stru...Advanced traffic monitoring systems encounter substantial challenges in vehicle detection and classification due to the limitations of conventional methods,which often demand extensive computational resources and struggle with diverse data acquisition techniques.This research presents a novel approach for vehicle classification and recognition in aerial image sequences,integrating multiple advanced techniques to enhance detection accuracy.The proposed model begins with preprocessing using Multiscale Retinex(MSR)to enhance image quality,followed by Expectation-Maximization(EM)Segmentation for precise foreground object identification.Vehicle detection is performed using the state-of-the-art YOLOv10 framework,while feature extraction incorporates Maximally Stable Extremal Regions(MSER),Dense Scale-Invariant Feature Transform(Dense SIFT),and Zernike Moments Features to capture distinct object characteristics.Feature optimization is further refined through a Hybrid Swarm-based Optimization algorithm,ensuring optimal feature selection for improved classification performance.The final classification is conducted using a Vision Transformer,leveraging its robust learning capabilities for enhanced accuracy.Experimental evaluations on benchmark datasets,including UAVDT and the Unmanned Aerial Vehicle Intruder Dataset(UAVID),demonstrate the superiority of the proposed approach,achieving an accuracy of 94.40%on UAVDT and 93.57%on UAVID.The results highlight the efficacy of the model in significantly enhancing vehicle detection and classification in aerial imagery,outperforming existing methodologies and offering a statistically validated improvement for intelligent traffic monitoring systems compared to existing approaches.展开更多
Diabetes mellitus represents a major global health issue,driving the need for noninvasive alternatives to traditional blood glucose monitoring methods.Recent advancements in wearable technology have introduced skin-in...Diabetes mellitus represents a major global health issue,driving the need for noninvasive alternatives to traditional blood glucose monitoring methods.Recent advancements in wearable technology have introduced skin-interfaced biosensors capable of analyzing sweat and skin biomarkers,providing innovative solutions for diabetes diagnosis and monitoring.This review comprehensively discusses the current developments in noninvasive wearable biosensors,emphasizing simultaneous detection of biochemical biomarkers(such as glucose,cortisol,lactate,branched-chain amino acids,and cytokines)and physiological signals(including heart rate,blood pressure,and sweat rate)for accurate,personalized diabetes management.We explore innovations in multimodal sensor design,materials science,biorecognition elements,and integration techniques,highlighting the importance of advanced data analytics,artificial intelligence-driven predictive algorithms,and closed-loop therapeutic systems.Additionally,the review addresses ongoing challenges in biomarker validation,sensor stability,user compliance,data privacy,and regulatory considerations.A holistic,multimodal approach enabled by these next-generation wearable biosensors holds significant potential for improving patient outcomes and facilitating proactive healthcare interventions in diabetes management.展开更多
Recently,the outbreak and spread of larch caterpillar(Dendrolimus superans)pests have emerged as significant contributors to forest degradation in the Changbai Mountains,China.Understanding the spatiotemporal distribu...Recently,the outbreak and spread of larch caterpillar(Dendrolimus superans)pests have emerged as significant contributors to forest degradation in the Changbai Mountains,China.Understanding the spatiotemporal distribution patterns of these pests is crucial for effective management and protection of forest ecosystems.This study proposes a pest monitoring approach based on Sentinel imagery.Through time-series analysis,we extracted pest-sensitive features and developed a random forest classifier that integrated Sentinel-1,Sentinel-2,and field sampling data from 2019–2023 to monitor larch caterpillar pests in the Changbai Mountains National Nature Reserve(CMNNR),Northeast China.Our findings indicated that bands green(B3),near-infrared(B8),short wave infrared(B11 and B12)from Sentinel-2 remote sensing images exhibited notable discriminative capabilities for identifying larch caterpillar pests.Specifically,the Normalized Difference Vegetation Index(NDVI)at the end of the growing season emerged as the most valuable feature for pest extraction.Incorporating Synthetic Aperture Radar(SAR)features along with optical data marginally enhances model performance.Furthermore,our approach unveiled the outbreak of larch caterpillar pests,achieving classification map with overall accuracy exceeding 85%and Kappa coefficient surpassing 0.8 for five study years.The pest outbreak began in 2019 and progressively intensified over time.In September 2019,the affected area spanned 114.23 km^(2).The infested area exhibited a declining trend from 2020 to 2023.This study introduces a novel method for the high-precision identification of larch caterpillar pests,offering technical advancements and theoretical underpinnings to support forest management strategies.展开更多
The growing prevalence of exercise-induced tibial stress fractures demands wearable sensors capable of monitoring dynamic musculoskeletal loads with medical-grade precision.While flexible pressure-sensing insoles show...The growing prevalence of exercise-induced tibial stress fractures demands wearable sensors capable of monitoring dynamic musculoskeletal loads with medical-grade precision.While flexible pressure-sensing insoles show clinical potential,their development has been hindered by the intrinsic trade-off between high sensitivity and full-range linearity(R^(2)>0.99 up to 1 MPa)in conventional designs.Inspired by the tactile sensing mechanism of human skin,where dermal stratification enables wide-range pressure adaptation and ion-channelregulated signaling maintains linear electrical responses,we developed a dual-mechanism flexible iontronic pressure sensor(FIPS).This innovative design synergistically combines two bioinspired components:interdigitated fabric microstructures enabling pressure-proportional contact area expansion(αP1/3)and iontronic film facilitating self-adaptive ion concentration modulation(αP^(2/3)),which together generate a linear capacitance-pressure response(CαP).The FIPS achieves breakthrough performance:242 kPa^(-1)sensitivity with 0.997linearity across 0-1 MPa,yielding a record linear sensing factor(LSF=242,000).The design is validated across various substrates and ionic materials,demonstrating its versatility.Finally,the FIPS-driven design enables a smart insole demonstrating 1.8%error in tibial load assessment during gait analysis,outperforming nonlinear counterparts(6.5%error)in early fracture-risk prediction.The biomimetic design framework establishes a universal approach for developing high-performance linear sensors,establishing generalized principles for medical-grade wearable devices.展开更多
THE mechanical response and deformation mechanisms of pure nickel under nanoindentation were systematically investigated using molecular dynamics(MD)simulations,with a particular focus on the novel interplay between c...THE mechanical response and deformation mechanisms of pure nickel under nanoindentation were systematically investigated using molecular dynamics(MD)simulations,with a particular focus on the novel interplay between crystallographic orientation,grain boundary(GB)proximity,and pore characteristics(size/location).This study compares single-crystal nickel models along[100],[110],and[111]orientations with equiaxed polycrystalline models containing 0,1,and 2.5 nm pores in surface and subsurface configurations.Our results reveal that crystallographic anisotropy manifests as a 24.4%higher elastic modulus and 22.2%greater hardness in[111]-oriented single crystals compared to[100].Pore-GB synergistic effects are found to dominate the deformation behavior:2.5 nm subsurface pores reduce hardness by 25.2%through stress concentration and dislocation annihilation at GBs,whereas surface pores enable mechanical recovery via accelerated dislocation generation post-collapse.Additionally,size-dependent deformation regimes were identified,with 1 nm pores inducing negligible perturbation due to rapid atomic rearrangement,in contrast with persistent softening in 2.5 nm pores.These findings establish atomic-scale design principles for defect engineering in nickel-based aerospace components,demonstrating how crystallographic orientation,pore configuration,and GB interactions collectively govern nanoindentation behavior.展开更多
Organic electrochemical transistor(OECT)devices demonstrate great promising potential for reservoir computing(RC)systems,but their lack of tunable dynamic characteristics limits their application in multi-temporal sca...Organic electrochemical transistor(OECT)devices demonstrate great promising potential for reservoir computing(RC)systems,but their lack of tunable dynamic characteristics limits their application in multi-temporal scale tasks.In this study,we report an OECT-based neuromorphic device with tunable relaxation time(τ)by introducing an additional vertical back-gate electrode into a planar structure.The dual-gate design enablesτreconfiguration from 93 to 541 ms.The tunable relaxation behaviors can be attributed to the combined effects of planar-gate induced electrochemical doping and back-gateinduced electrostatic coupling,as verified by electrochemical impedance spectroscopy analysis.Furthermore,we used theτ-tunable OECT devices as physical reservoirs in the RC system for intelligent driving trajectory prediction,achieving a significant improvement in prediction accuracy from below 69%to 99%.The results demonstrate that theτ-tunable OECT shows a promising candidate for multi-temporal scale neuromorphic computing applications.展开更多
Photo-assisted lithium–sulfur batteries(PALSBs)offer an eco-friendly solution to address the issue of sluggish reaction kinetics of conventional LSBs.However,designing an efficient photoelectrode for practical implem...Photo-assisted lithium–sulfur batteries(PALSBs)offer an eco-friendly solution to address the issue of sluggish reaction kinetics of conventional LSBs.However,designing an efficient photoelectrode for practical implementation remains a significant challenge.Herein,we construct a free-standing polymer–inorganic hybrid photoelectrode with a direct Z-scheme heterostructure to develop high-efficiency PALSBs.Specifically,polypyrrole(PPy)is in situ vapor-phase polymerized on the surface of N-doped TiO_(2) nanorods supported on carbon cloth(N-TiO_(2)/CC),thereby forming a well-defined p–n heterojunction.This architecture efficiently facilitates the carrier separation of photo-generated electron–hole pairs and significantly enhances carrier transport by creating a built-in electric field.Thus,the PPy@N-TiO_(2)/CC can simultaneously act as a photocatalyst and an electrocatalyst to accelerate the reduction and evolution of sulfur,enabling ultrafast sulfur redox dynamics,as convincingly validated by both theoretical simulations and experimental results.Consequently,the PPy@N-TiO_(2)/CC PALSB achieves a high discharge capacity of 1653 mAh g−1,reaching 98.7%of the theoretical value.Furthermore,5 h of photo-charging without external voltage enables the PALSB to deliver a discharge capacity of 333 mAh g−1,achieving dual-mode energy harvesting capabilities.This work successfully integrates solar energy conversion and storage within a rechargeable battery system,providing a promising strategy for sustainable energy storage technologies.展开更多
Conductive elastomers combining micromechanical sensitivity,lightweight adaptability,and environmental sustainability are critically needed for advanced flexible electronics requiring precise responsiveness and long-t...Conductive elastomers combining micromechanical sensitivity,lightweight adaptability,and environmental sustainability are critically needed for advanced flexible electronics requiring precise responsiveness and long-term wearability;however,the integration of these properties remains a significant challenge.Here,we present a biomass-derived conductive elastomer featuring a rationally engineered dynamic crosslinked network integrated with a tunable microporous architecture.This structural design imparts pronounced micromechanical sensitivity,an ultralow density(~0.25 g cm^(−3)),and superior mechanical compliance for adaptive deformation.Moreover,the unique micro-spring effect derived from the porous architecture ensures exceptional stretchability(>500%elongation at break)and superior resilience,delivering immediate and stable electrical response under both subtle(<1%)and large(>200%)mechanical stimuli.Intrinsic dynamic interactions endow the elastomer with efficient room temperature self-healing and complete recyclability without compromising performance.First-principles simulations clarify the mechanisms behind micropore formation and the resulting functionality.Beyond its facile and mild fabrication process,this work establishes a scalable route toward high-performance,sustainable conductive elastomers tailored for next-generation soft electronics.展开更多
Rheumatoid arthritis(RA)patients face significant psychological challenges alongside physical symptoms,necessitating a comprehensive understanding of how psychological vulnerability and adaptation patterns evolve thro...Rheumatoid arthritis(RA)patients face significant psychological challenges alongside physical symptoms,necessitating a comprehensive understanding of how psychological vulnerability and adaptation patterns evolve throughout the disease course.This review examined 95 studies(2000-2025)from PubMed,Web of Science,and CNKI databases including longitudinal cohorts,randomized controlled trials,and mixed-methods research,to characterize the complex interplay between biological,psychological,and social factors affecting RA patients’mental health.Findings revealed three distinct vulnerability trajectories(45%persistently low,30%fluctuating improvement,25%persistently high)and four adaptation stages,with critical intervention periods occurring 3-6 months postdiagnosis and during disease flares.Multiple factors significantly influence psychological outcomes,including gender(females showing 1.8-fold increased risk),age(younger patients experiencing 42%higher vulnerability),pain intensity,inflammatory markers,and neuroendocrine dysregulation(48%showing cortisol rhythm disruption).Early psychological intervention(within 3 months of diagnosis)demonstrated robust benefits,reducing depression incidence by 42%with effects persisting 24-36 months,while different modalities showed complementary advantages:Cognitive behavioral therapy for depression(Cohen’s d=0.68),mindfulness for pain acceptance(38%improvement),and peer support for meaning reconstruction(25.6%increase).These findings underscore the importance of integrating routine psychological assessment into standard RA care,developing stage-appropriate interventions,and advancing research toward personalized biopsychosocial approaches that address the dynamic psychological dimensions of the disease.展开更多
Pulsed dynamic electrolysis(PDE),driven by renewable energy,has emerged as an innovative electrocatalytic conversion method,demonstrating significant potential in addressing global energy challenges and promoting sust...Pulsed dynamic electrolysis(PDE),driven by renewable energy,has emerged as an innovative electrocatalytic conversion method,demonstrating significant potential in addressing global energy challenges and promoting sustainable development.Despite significant progress in various electrochemical systems,the regulatory mechanisms of PDE in energy and mass transfer and the lifespan extension of electrolysis systems,particularly in water electrolysis(WE)for hydrogen production,remain insufficiently explored.Therefore,there is an urgent need for a deeper understanding of the unique contributions of PDE in mass transfer enhancement,microenvironment regulation,and hydrogen production optimization,aiming to achieve low-energy consumption,high catalytic activity,and long-term stability in the generation of target products.Here,this review critically examines the microenvironmental effects of PDE on energy and mass transfer,the electrode degradation mechanisms in the lifespan extension of electrolysis systems,and the key factors in enhancing WE for hydrogen production,providing a comprehensive summary of current research progress.The review focuses on the complex regulatory mechanisms of frequency,duty cycle,amplitude,and other factors in hydrogen evolution reaction(HER)performance within PDE strategies,revealing the interrelationships among them.Finally,the potential future directions and challenges for transitioning from laboratory studies to industrial applications are proposed.展开更多
基金supported in part by the National Natural Science Foundation of China(62125306)Zhejiang Key Research and Development Project(2024C01163)the State Key Laboratory of Industrial Control Technology,China(ICT2024A06)
文摘In recent decades,control performance monitoring(CPM)has experienced remarkable progress in research and industrial applications.While CPM research has been investigated using various benchmarks,the historical data benchmark(HIS)has garnered the most attention due to its practicality and effectiveness.However,existing CPM reviews usually focus on the theoretical benchmark,and there is a lack of an in-depth review that thoroughly explores HIS-based methods.In this article,a comprehensive overview of HIS-based CPM is provided.First,we provide a novel static-dynamic perspective on data-level manifestations of control performance underlying typical controller capacities including regulation and servo:static and dynamic properties.The static property portrays time-independent variability in system output,and the dynamic property describes temporal behavior driven by closed-loop feedback.Accordingly,existing HIS-based CPM approaches and their intrinsic motivations are classified and analyzed from these two perspectives.Specifically,two mainstream solutions for CPM methods are summarized,including static analysis and dynamic analysis,which match data-driven techniques with actual controlling behavior.Furthermore,this paper also points out various opportunities and challenges faced in CPM for modern industry and provides promising directions in the context of artificial intelligence for inspiring future research.
文摘In the leakage detection of reservoir dam bodies,traditional geophysical methods can only achieve one-time detection.Meanwhile,due to the non-uniqueness of geophysicalin version,how to improve the fidelity of geophysical detection inversion profiles has become a key challenge in the industry.This study aims to construct a long-term real-time monitoring system using the time-lapse resistivity method,reveal the spatiotemporal evolution law of dam leakage,and provide technical support for accurate treatment.By integrating the Internet of Things(IoT),5G technology,and AI technology,real-time data acquisition,real-time transmission,and automatic inversionare realized.Through dynamic imaging analysis of the electrical anomaly characteristics of the leakage area and comparison between corresponding rainfall events,the leakage range and resistivity changes,the reliability and efficiency of dam leakagedete ction are significantly improved.This achieves long-termdynamic monitoring of dam leakage and provides a new perspective for the safe operation and maintenance of reservoirs.
基金supported by the CNPC-SWPU Innovation Alliance Technology Cooperation Project(2020CX020000)the National Natural Science Foundation of China(42022028)+1 种基金the Natural Science Foundation of Sichuan Province(24NSFSC0808)the China Scholarship Council(202306440144)。
文摘In common practice in the oil fields,the injection of water and gas into reservoirs is a crucial technique to increase production.The control of the waterflooding front in oil/gas exploitation is a matter of great concern to reservoir engineers.Monitoring the waterflooding front in oil/gas wells plays a very important role in adjusting the well network and later in production,taking advantage of the remaining oil po-tential and ultimately achieving great success in improving the recovery rate.For a long time,micro-seismic monitoring,numerical simulation,four-dimensional seismic and other methods have been widely used in waterflooding front monitoring.However,reconciling their reliability and cost poses a significant challenge.In order to achieve real-time,reliable and cost-effective monitoring,we propose an innovative method for waterflooding front monitoring through the similarity analysis of passive source time-lapse seismic images.Typically,passive source seismic data collected from oil fields have extremely low signal-to-noise ratio(SNR),which poses a serious problem for obtaining structural images.The proposed method aims to visualize and analyze underground changes by highlighting time-lapse images and provide a strategy for underground monitoring using long-term passive source data under low SNR conditions.First,we verify the feasibility of the proposed method by designing a theoretical model.Then,we conduct an analysis of the correlation coefficient(similarity)on the passive source time-lapse seismic imaging results to enhance the image differences and identify the simulated waterflooding fronts.Finally,the proposed method is applied to the actual waterflooding front monitoring tasks in Shengli Oilfield,China.The research findings indicate that the monitoring results are consistent with the actual devel-opment conditions,which in turn demonstrates that the proposed method has great potential for practical application and is very suitable for monitoring common development tasks in oil fields.
基金supported by the National Science Foundation of China(Grant Nos.52068049 and 51908266)the Science Fund for Distinguished Young Scholars of Gansu Province(No.21JR7RA267)Hongliu Outstanding Young Talents Program of Lanzhou University of Technology.
文摘Addressing the current challenges in transforming pixel displacement into physical displacement in visual monitoring technologies,as well as the inability to achieve precise full-field monitoring,this paper proposes a method for identifying the structural dynamic characteristics of wind turbines based on visual monitoring data fusion.Firstly,the Lucas-Kanade Tomasi(LKT)optical flow method and a multi-region of interest(ROI)monitoring structure are employed to track pixel displacements,which are subsequently subjected to band pass filtering and resampling operations.Secondly,the actual displacement time history is derived through double integration of the acquired acceleration data and subsequent band pass filtering.The scale factor is obtained by applying the least squares method to compare the visual displacement with the displacement derived from double integration of the acceleration data.Based on this,the multi-point displacement time histories under physical coordinates are obtained using the vision data and the scale factor.Subsequently,when visual monitoring of displacements becomes impossible due to issues such as image blurring or lens occlusion,the structural vibration equation and boundary condition constraints,among other key parameters,are employed to predict the displacements at unknown monitoring points,thereby enabling full-field displacement monitoring and dynamic characteristic testing of the structure.Finally,a small-scale shaking table test was conducted on a simulated wind turbine structure undergoing shutdown to validate the dynamic characteristics of the proposed method through test verification.The research results indicate that the proposed method achieves a time-domain error within the submillimeter range and a frequency-domain accuracy of over 99%,effectively monitoring the full-field structural dynamic characteristics of wind turbines and providing a basis for the condition assessment of wind turbine structures.
基金supported by the National Natural Science Foundation of China(Nos.42177173,U23A20651 and 42130719)and the Outstanding Youth Science Fund Project of Sichuan Provincial Natural Science Foundation(No.2025NSFJQ0003)。
文摘Dynamic stress adjustment in deep-buried high geostress hard rock tunnels frequently triggers catastrophic failures such as rockbursts and collapses.While a comprehensive understanding of this process is critical for evaluating surrounding rock stability,its dynamic evolution are often overlooked in engineering practice.This study systematically summarizes a novel classification framework for stress adjustment types—stabilizing(two-zoned),shallow failure(three-zoned),and deep failure(four-zoned)—characterized by distinct stress adjustment stages.A dynamic interpretation technology system is developed based on microseismic monitoring,integrating key microseismic parameters(energy index EI,apparent stressσa,microseismic activity S),seismic source parameter space clustering,and microseismic paths.This approach enables precise identification of evolutionary stages,stress adjustment types,and failure precursors,thereby elucidating the intrinsic linkage between geomechanical processes(stress redistribution)and failure risks.The study establishes criteria and procedures for identifying stress adjustment types and their associated failure risks,which were successfully applied in the Grand Canyon Tunnel of the E-han Highway to detect 50 instances of disaster risks.The findings offer invaluable insights into understanding the evolution process of stress adjustment and pinpointing the disaster risks linked to hard rock in comparable high geostress tunnels.
基金funded by the Thailand Science Research and Innovation Fund,Chulalongkorn University(BCG_FF_68_165_2100_027)The first author(Tidarut Jirawattanasomkul)also gratefully acknowledges support from the Grants for Development of New Faculty Staff,Ratchadaphiseksomphot Fund,Chulalongkorn University.The corresponding author(Supasit Srivaranun)acknowledges the Research and Innovation Funding from National Research Council of Thailand(No.N84A680208)+2 种基金the Research Grant from Faculty of Engineering,Kasetsart University(No.67/05/CE)The fourth author(Suched Likitlersuang)acknowledges Thailand Science Research and Innovation Fund Chulalongkorn University(DISF68210001)the National Research Council of Thailand(NRCT):Grant No.N42A670572.
文摘This study developed a digital twin(DT)and structural health monitoring(SHM)system for a balanced cantilever bridge,utilizing advanced measurement techniques to enhance accuracy.Vibration and dynamic strain measurements were obtained using accelerometers and piezo-resistive strain gauges,capturing low-magnitude dynamic strains during operational vibrations.3D-LiDAR scanning and Ultrasonic Pulse Velocity(UPV)tests captured the bridge's as-is geometry and modulus of elasticity.The resulting detailed 3D point cloud model revealed the structure's true state and highlighted discrepancies between the as-designed and as-built conditions.Dynamic properties,including modal frequencies and shapes,were extracted from the strain and acceleration measurements,providing critical insights into the bridge's structural behavior.The neutral axis depth,indicating stress distribution and potential damage,was accurately determined.Good agreement between vibration measurement data and the as-is model results validated the reliability of the digital twin model.Dynamic strain patterns and neutral axis parameters showed strong correlation with model predictions,serving as sensitive indicators of local damage.The baseline digital twin model and measurement results establish a foundation for future bridge inspections and investigations.This study demonstrates the effectiveness of combining digital twin technology with field measurements for real-time monitoring and predictive maintenance,ensuring the sustainability and safety of the bridge infrastructure,thereby enhancing its overall resilience to operational and environmental stressors.
基金supported in part by the National Science Fund for Distinguished Young Scholars of China(62225303)the National Natural Science Fundation of China(62303039,62433004)+2 种基金the China Postdoctoral Science Foundation(BX20230034,2023M730190)the Fundamental Research Funds for the Central Universities(buctrc202201,QNTD2023-01)the High Performance Computing Platform,College of Information Science and Technology,Beijing University of Chemical Technology
文摘Data-driven process monitoring is an effective approach to assure safe operation of modern manufacturing and energy systems,such as thermal power plants being studied in this work.Industrial processes are inherently dynamic and need to be monitored using dynamic algorithms.Mainstream dynamic algorithms rely on concatenating current measurement with past data.This work proposes a new,alternative dynamic process monitoring algorithm,using dot product feature analysis(DPFA).DPFA computes the dot product of consecutive samples,thus naturally capturing the process dynamics through temporal correlation.At the same time,DPFA's online computational complexity is lower than not just existing dynamic algorithms,but also classical static algorithms(e.g.,principal component analysis and slow feature analysis).The detectability of the new algorithm is analyzed for three types of faults typically seen in process systems:sensor bias,process fault and gain change fault.Through experiments with a numerical example and real data from a thermal power plant,the DPFA algorithm is shown to be superior to the state-of-the-art methods,in terms of better monitoring performance(fault detection rate and false alarm rate)and lower computational complexity.
基金provided by the National Key R&D Program of China(No.2024YFC3012605)the State Key Laboratory of Geohazard Prevention and Geoenvironment Protection Independent Research Project(Nos.SKLGP2022Z001,SKLGP2023Z029 and SKLGP2022K027)。
文摘Biotite content critically influences rock mechanical behavior and threatens underground engineering stability.Uniaxial compression tests with acoustic emission(AE)monitoring were conducted on granite pegmatite samples having varying biotite content.Peak frequency distribution analysis,rise angleaverage frequency(RA-AF)analysis,multifractal theory,and a dynamic multifractal algorithm were applied to explore the relationship between damage evolution and AE characteristics.Results indicate that increased biotite content reduces uniaxial compressive strength and elastic modulus,enhances plastic deformation,and increases the proportion of shear cracks.The segmented evolution of the dynamic multifractal parameter Δα_(m) is biotite-dependent.Oscillations during the elastic phase signify localized shear crack initiation and propagation;their attenuation in the plastic phase reflects frictional closure along biotite cleavage planes,promoting elastic energy storage and delaying release.AE-based damage models and time-varying signals characterize rock damage progression.Stress concentrations around biotite minerals foster localized shear band formation,leading to concentrated shear failure at lower damage levels.Higher biotite content accelerates crack propagation,while smooth cleavage planes lower the fracture energy threshold,reducing strength and stiffness.These findings enhance understanding of biotite-influenced progressive rock damage and underpin stability monitoring and early-warning systems for underground engineering.
基金supported by the Program of National Natural Science Foundation of China(U23A20329,62163036)Youth Academic and Technical Leaders Reserve Talent Training project(202105AC160094)Industrial Innovation Talent Special Project of Xingdian Talent Support Program(XDYC-CYCX-2022-0010).
文摘Kernel-based slow feature analysis(SFA)methods have been successfully applied in the industrial process fault detection field.However,kernel-based SFA methods have high computational complexity as dealing with nonlinearity,leading to delays in detecting time-varying data features.Additionally,the uncertain kernel function and kernel parameters limit the ability of the extracted features to express process characteristics,resulting in poor fault detection performance.To alleviate the above problems,a novel randomized auto-regressive dynamic slow feature analysis(RRDSFA)method is proposed to simultaneously monitor the operating point deviations and process dynamic faults,enabling real-time monitoring of data features in industrial processes.Firstly,the proposed Random Fourier mappingbased method achieves more effective nonlinear transformation,contrasting with the current kernelbased RDSFA algorithm that may lead to significant computational complexity.Secondly,a randomized RDSFA model is developed to extract nonlinear dynamic slow features.Furthermore,a Bayesian inference-based overall fault monitoring model including all RRDSFA sub-models is developed to overcome the randomness of random Fourier mapping.Finally,the superiority and effectiveness of the proposed monitoring method are demonstrated through a numerical case and a simulation of continuous stirred tank reactor.
基金supported by the National Natural Science Foundation of China(22074072,22274083,52376199)the Shandong Provincial Natural Science Foundation(ZR2023LZY005)+1 种基金the Exploration Project of the State Key Laboratory of BioFibers and EcoTextiles of Qingdao University(TSKT202101)the Fundamental Research Funds for the Central Universities(2022BLRD13,2023BLRD01).
文摘A rapidly growing field is piezoresistive sensor for accurate respiration rate monitoring to suppress the worldwide respiratory illness.However,a large neglected issue is the sensing durability and accuracy without interference since the expiratory pressure always coupled with external humidity and temperature variations,as well as mechanical motion artifacts.Herein,a robust and biodegradable piezoresistive sensor is reported that consists of heterogeneous MXene/cellulose-gelation sensing layer and Ag-based interdigital electrode,featuring customizable cylindrical interface arrangement and compact hierarchical laminated architecture for collectively regulating the piezoresistive response and mechanical robustness,thereby realizing the long-term breath-induced pressure detection.Notably,molecular dynamics simulations reveal the frequent angle inversion and reorientation of MXene/cellulose in vacuum filtration,driven by shear forces and interfacial interactions,which facilitate the establishment of hydrogen bonds and optimize the architecture design in sensing layer.The resultant sensor delivers unprecedented collection features of superior stability for off-axis deformation(0-120°,~2.8×10^(-3) A)and sensing accuracy without crosstalk(humidity 50%-100%and temperature 30-80).Besides,the sensor-embedded mask together with machine learning models is achieved to train and classify the respiration status for volunteers with different ages(average prediction accuracy~90%).It is envisioned that the customizable architecture design and sensor paradigm will shed light on the advanced stability of sustainable electronics and pave the way for the commercial application in respiratory monitory.
文摘Advanced traffic monitoring systems encounter substantial challenges in vehicle detection and classification due to the limitations of conventional methods,which often demand extensive computational resources and struggle with diverse data acquisition techniques.This research presents a novel approach for vehicle classification and recognition in aerial image sequences,integrating multiple advanced techniques to enhance detection accuracy.The proposed model begins with preprocessing using Multiscale Retinex(MSR)to enhance image quality,followed by Expectation-Maximization(EM)Segmentation for precise foreground object identification.Vehicle detection is performed using the state-of-the-art YOLOv10 framework,while feature extraction incorporates Maximally Stable Extremal Regions(MSER),Dense Scale-Invariant Feature Transform(Dense SIFT),and Zernike Moments Features to capture distinct object characteristics.Feature optimization is further refined through a Hybrid Swarm-based Optimization algorithm,ensuring optimal feature selection for improved classification performance.The final classification is conducted using a Vision Transformer,leveraging its robust learning capabilities for enhanced accuracy.Experimental evaluations on benchmark datasets,including UAVDT and the Unmanned Aerial Vehicle Intruder Dataset(UAVID),demonstrate the superiority of the proposed approach,achieving an accuracy of 94.40%on UAVDT and 93.57%on UAVID.The results highlight the efficacy of the model in significantly enhancing vehicle detection and classification in aerial imagery,outperforming existing methodologies and offering a statistically validated improvement for intelligent traffic monitoring systems compared to existing approaches.
文摘Diabetes mellitus represents a major global health issue,driving the need for noninvasive alternatives to traditional blood glucose monitoring methods.Recent advancements in wearable technology have introduced skin-interfaced biosensors capable of analyzing sweat and skin biomarkers,providing innovative solutions for diabetes diagnosis and monitoring.This review comprehensively discusses the current developments in noninvasive wearable biosensors,emphasizing simultaneous detection of biochemical biomarkers(such as glucose,cortisol,lactate,branched-chain amino acids,and cytokines)and physiological signals(including heart rate,blood pressure,and sweat rate)for accurate,personalized diabetes management.We explore innovations in multimodal sensor design,materials science,biorecognition elements,and integration techniques,highlighting the importance of advanced data analytics,artificial intelligence-driven predictive algorithms,and closed-loop therapeutic systems.Additionally,the review addresses ongoing challenges in biomarker validation,sensor stability,user compliance,data privacy,and regulatory considerations.A holistic,multimodal approach enabled by these next-generation wearable biosensors holds significant potential for improving patient outcomes and facilitating proactive healthcare interventions in diabetes management.
基金Under the auspices of National Natural Science Foundation of China(No.42171407,42077242)Key Program of National Natural Science Foundation of China(No.42330607)。
文摘Recently,the outbreak and spread of larch caterpillar(Dendrolimus superans)pests have emerged as significant contributors to forest degradation in the Changbai Mountains,China.Understanding the spatiotemporal distribution patterns of these pests is crucial for effective management and protection of forest ecosystems.This study proposes a pest monitoring approach based on Sentinel imagery.Through time-series analysis,we extracted pest-sensitive features and developed a random forest classifier that integrated Sentinel-1,Sentinel-2,and field sampling data from 2019–2023 to monitor larch caterpillar pests in the Changbai Mountains National Nature Reserve(CMNNR),Northeast China.Our findings indicated that bands green(B3),near-infrared(B8),short wave infrared(B11 and B12)from Sentinel-2 remote sensing images exhibited notable discriminative capabilities for identifying larch caterpillar pests.Specifically,the Normalized Difference Vegetation Index(NDVI)at the end of the growing season emerged as the most valuable feature for pest extraction.Incorporating Synthetic Aperture Radar(SAR)features along with optical data marginally enhances model performance.Furthermore,our approach unveiled the outbreak of larch caterpillar pests,achieving classification map with overall accuracy exceeding 85%and Kappa coefficient surpassing 0.8 for five study years.The pest outbreak began in 2019 and progressively intensified over time.In September 2019,the affected area spanned 114.23 km^(2).The infested area exhibited a declining trend from 2020 to 2023.This study introduces a novel method for the high-precision identification of larch caterpillar pests,offering technical advancements and theoretical underpinnings to support forest management strategies.
基金supported by the National Natural Science Foundation of China(NSFC 52175281,52475315)Youth Innovation Promotion Association of CAS(2021382)。
文摘The growing prevalence of exercise-induced tibial stress fractures demands wearable sensors capable of monitoring dynamic musculoskeletal loads with medical-grade precision.While flexible pressure-sensing insoles show clinical potential,their development has been hindered by the intrinsic trade-off between high sensitivity and full-range linearity(R^(2)>0.99 up to 1 MPa)in conventional designs.Inspired by the tactile sensing mechanism of human skin,where dermal stratification enables wide-range pressure adaptation and ion-channelregulated signaling maintains linear electrical responses,we developed a dual-mechanism flexible iontronic pressure sensor(FIPS).This innovative design synergistically combines two bioinspired components:interdigitated fabric microstructures enabling pressure-proportional contact area expansion(αP1/3)and iontronic film facilitating self-adaptive ion concentration modulation(αP^(2/3)),which together generate a linear capacitance-pressure response(CαP).The FIPS achieves breakthrough performance:242 kPa^(-1)sensitivity with 0.997linearity across 0-1 MPa,yielding a record linear sensing factor(LSF=242,000).The design is validated across various substrates and ionic materials,demonstrating its versatility.Finally,the FIPS-driven design enables a smart insole demonstrating 1.8%error in tibial load assessment during gait analysis,outperforming nonlinear counterparts(6.5%error)in early fracture-risk prediction.The biomimetic design framework establishes a universal approach for developing high-performance linear sensors,establishing generalized principles for medical-grade wearable devices.
基金The National Natural Science Foundation of China(Grant No.12462006)Beijing Institute of Structure and Environment Engineering Joint Innovation Fund(No.BQJJ202414).
文摘THE mechanical response and deformation mechanisms of pure nickel under nanoindentation were systematically investigated using molecular dynamics(MD)simulations,with a particular focus on the novel interplay between crystallographic orientation,grain boundary(GB)proximity,and pore characteristics(size/location).This study compares single-crystal nickel models along[100],[110],and[111]orientations with equiaxed polycrystalline models containing 0,1,and 2.5 nm pores in surface and subsurface configurations.Our results reveal that crystallographic anisotropy manifests as a 24.4%higher elastic modulus and 22.2%greater hardness in[111]-oriented single crystals compared to[100].Pore-GB synergistic effects are found to dominate the deformation behavior:2.5 nm subsurface pores reduce hardness by 25.2%through stress concentration and dislocation annihilation at GBs,whereas surface pores enable mechanical recovery via accelerated dislocation generation post-collapse.Additionally,size-dependent deformation regimes were identified,with 1 nm pores inducing negligible perturbation due to rapid atomic rearrangement,in contrast with persistent softening in 2.5 nm pores.These findings establish atomic-scale design principles for defect engineering in nickel-based aerospace components,demonstrating how crystallographic orientation,pore configuration,and GB interactions collectively govern nanoindentation behavior.
基金supported by the National Key Research and Development Program of China under Grant 2022YFB3608300in part by the National Nature Science Foundation of China(NSFC)under Grants 62404050,U2341218,62574056,62204052。
文摘Organic electrochemical transistor(OECT)devices demonstrate great promising potential for reservoir computing(RC)systems,but their lack of tunable dynamic characteristics limits their application in multi-temporal scale tasks.In this study,we report an OECT-based neuromorphic device with tunable relaxation time(τ)by introducing an additional vertical back-gate electrode into a planar structure.The dual-gate design enablesτreconfiguration from 93 to 541 ms.The tunable relaxation behaviors can be attributed to the combined effects of planar-gate induced electrochemical doping and back-gateinduced electrostatic coupling,as verified by electrochemical impedance spectroscopy analysis.Furthermore,we used theτ-tunable OECT devices as physical reservoirs in the RC system for intelligent driving trajectory prediction,achieving a significant improvement in prediction accuracy from below 69%to 99%.The results demonstrate that theτ-tunable OECT shows a promising candidate for multi-temporal scale neuromorphic computing applications.
基金financial support from the National Natural Science Foundation of China(22109127)the Chinese Postdoctoral Science Foundation(2021M702666),+1 种基金he Research Fund of the State Key Laboratory of Solidification Processing(NPU),China(Grant No.2023-TS-02)financial support from the Youth Project of"Shaanxi High-level Talents Introduction Plan"and the Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)are also sincerely appreciated.
文摘Photo-assisted lithium–sulfur batteries(PALSBs)offer an eco-friendly solution to address the issue of sluggish reaction kinetics of conventional LSBs.However,designing an efficient photoelectrode for practical implementation remains a significant challenge.Herein,we construct a free-standing polymer–inorganic hybrid photoelectrode with a direct Z-scheme heterostructure to develop high-efficiency PALSBs.Specifically,polypyrrole(PPy)is in situ vapor-phase polymerized on the surface of N-doped TiO_(2) nanorods supported on carbon cloth(N-TiO_(2)/CC),thereby forming a well-defined p–n heterojunction.This architecture efficiently facilitates the carrier separation of photo-generated electron–hole pairs and significantly enhances carrier transport by creating a built-in electric field.Thus,the PPy@N-TiO_(2)/CC can simultaneously act as a photocatalyst and an electrocatalyst to accelerate the reduction and evolution of sulfur,enabling ultrafast sulfur redox dynamics,as convincingly validated by both theoretical simulations and experimental results.Consequently,the PPy@N-TiO_(2)/CC PALSB achieves a high discharge capacity of 1653 mAh g−1,reaching 98.7%of the theoretical value.Furthermore,5 h of photo-charging without external voltage enables the PALSB to deliver a discharge capacity of 333 mAh g−1,achieving dual-mode energy harvesting capabilities.This work successfully integrates solar energy conversion and storage within a rechargeable battery system,providing a promising strategy for sustainable energy storage technologies.
基金supported by National Natural Science Foundation of China(No.52103044)Double First-Class Initiative University of Science and Technology of China(KY2400000037)the Young Talent Programme(GG2400007009).
文摘Conductive elastomers combining micromechanical sensitivity,lightweight adaptability,and environmental sustainability are critically needed for advanced flexible electronics requiring precise responsiveness and long-term wearability;however,the integration of these properties remains a significant challenge.Here,we present a biomass-derived conductive elastomer featuring a rationally engineered dynamic crosslinked network integrated with a tunable microporous architecture.This structural design imparts pronounced micromechanical sensitivity,an ultralow density(~0.25 g cm^(−3)),and superior mechanical compliance for adaptive deformation.Moreover,the unique micro-spring effect derived from the porous architecture ensures exceptional stretchability(>500%elongation at break)and superior resilience,delivering immediate and stable electrical response under both subtle(<1%)and large(>200%)mechanical stimuli.Intrinsic dynamic interactions endow the elastomer with efficient room temperature self-healing and complete recyclability without compromising performance.First-principles simulations clarify the mechanisms behind micropore formation and the resulting functionality.Beyond its facile and mild fabrication process,this work establishes a scalable route toward high-performance,sustainable conductive elastomers tailored for next-generation soft electronics.
基金Supported by Chongqing Health Commission and Chongqing Science and Technology Bureau,No.2023MSXM182。
文摘Rheumatoid arthritis(RA)patients face significant psychological challenges alongside physical symptoms,necessitating a comprehensive understanding of how psychological vulnerability and adaptation patterns evolve throughout the disease course.This review examined 95 studies(2000-2025)from PubMed,Web of Science,and CNKI databases including longitudinal cohorts,randomized controlled trials,and mixed-methods research,to characterize the complex interplay between biological,psychological,and social factors affecting RA patients’mental health.Findings revealed three distinct vulnerability trajectories(45%persistently low,30%fluctuating improvement,25%persistently high)and four adaptation stages,with critical intervention periods occurring 3-6 months postdiagnosis and during disease flares.Multiple factors significantly influence psychological outcomes,including gender(females showing 1.8-fold increased risk),age(younger patients experiencing 42%higher vulnerability),pain intensity,inflammatory markers,and neuroendocrine dysregulation(48%showing cortisol rhythm disruption).Early psychological intervention(within 3 months of diagnosis)demonstrated robust benefits,reducing depression incidence by 42%with effects persisting 24-36 months,while different modalities showed complementary advantages:Cognitive behavioral therapy for depression(Cohen’s d=0.68),mindfulness for pain acceptance(38%improvement),and peer support for meaning reconstruction(25.6%increase).These findings underscore the importance of integrating routine psychological assessment into standard RA care,developing stage-appropriate interventions,and advancing research toward personalized biopsychosocial approaches that address the dynamic psychological dimensions of the disease.
基金financially supported by the Key Research and Development Program of Heilongjiang Province(No.2024ZXJ03C06)National Natural Science Foundation of China(No.52476192,No.52106237)+1 种基金Natural Science Foundation of Heilongjiang Province(No.YQ2022E027)Technology Project of China Datang Technology Innovation Co.,Ltd(No.DTKC-2024-20610).
文摘Pulsed dynamic electrolysis(PDE),driven by renewable energy,has emerged as an innovative electrocatalytic conversion method,demonstrating significant potential in addressing global energy challenges and promoting sustainable development.Despite significant progress in various electrochemical systems,the regulatory mechanisms of PDE in energy and mass transfer and the lifespan extension of electrolysis systems,particularly in water electrolysis(WE)for hydrogen production,remain insufficiently explored.Therefore,there is an urgent need for a deeper understanding of the unique contributions of PDE in mass transfer enhancement,microenvironment regulation,and hydrogen production optimization,aiming to achieve low-energy consumption,high catalytic activity,and long-term stability in the generation of target products.Here,this review critically examines the microenvironmental effects of PDE on energy and mass transfer,the electrode degradation mechanisms in the lifespan extension of electrolysis systems,and the key factors in enhancing WE for hydrogen production,providing a comprehensive summary of current research progress.The review focuses on the complex regulatory mechanisms of frequency,duty cycle,amplitude,and other factors in hydrogen evolution reaction(HER)performance within PDE strategies,revealing the interrelationships among them.Finally,the potential future directions and challenges for transitioning from laboratory studies to industrial applications are proposed.
