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Source term estimation of hazardous gas leakages under turbulent atmospheric transport dispersion scenarios
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作者 Chuantao Ni Ziqiang Lang +4 位作者 Bing Wang Ang Li Chenxi Cao Wenli Du Feng Qian 《Chinese Journal of Chemical Engineering》 2025年第12期222-238,共17页
Source term estimation(STE)of hazardous gas leakages in chemical industrial parks(CIPs)is important for addressing environmental pollution and improving safety and reliability in engineering practice.To achieve real-t... Source term estimation(STE)of hazardous gas leakages in chemical industrial parks(CIPs)is important for addressing environmental pollution and improving safety and reliability in engineering practice.To achieve real-time STE,least squares-based STE methods have recently been developed.However,these methods require the number and locations of potential hazardous gas leakage sources are known as a priori,which is difficult in many practical scenarios.To address this limitation,we propose a new datadriven STE approach,which enables the STE to be implemented in real time and applicable to complicated turbulent dispersion scenarios.The linear independent analysis in data science is applied to historically collected concentration data of a hazardous gas of concern from a network of sensors to extract the sensor data which represent independent hazardous gas leakage scenarios(IHGLSs).An appropriate Gaussian model approximation to a high-fidelity computational fluid dynamics(CFD)model that must be used to represent the hazardous gas leakage scenarios of concern is built,and the off-line STE of IHGLSs using the approximating Gaussian model is then performed to build the datadriven STE model.The performance of the proposed approach is evaluated by using data that are generated by simulating ethane leakage scenarios in a CIP using a CFD model.Results indicate that the leakage localization accuracy is 100%and the mean relative estimation error for the leakage strength is6.76%.Moreover,the proposed approach is validated with real data in Prairie Grass field dispersion experiments,demonstrating the practical applicability of the proposed approach. 展开更多
关键词 Computation fluiddynamics Hazardous gas leakage OPTIMIZATION source term estimation Turbulent flow
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MULTIPLICITY OF SOLUTIONS AND SOURCE TERMS IN A FOURTH ORDER NONLINEAR ELLIPTIC EQUATION 被引量:3
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作者 Choi Q-Heung Jung Tacksun(Departmctzt of Mathematics, Inha University, Incheon 402-751, KoreaDepartment of Mathematics, Kunsan National University, Kunsan 573-701, Korea) 《Acta Mathematica Scientia》 SCIE CSCD 1999年第4期361-374,共14页
The authors investigatc relations between multiplicity of solutions and sourceterms of the fourth order nonlinear elliptic boundary value problem under Dirichlet boundary condition △2u+c△u = bu++f inΩ, wherc Ω i... The authors investigatc relations between multiplicity of solutions and sourceterms of the fourth order nonlinear elliptic boundary value problem under Dirichlet boundary condition △2u+c△u = bu++f inΩ, wherc Ω is a bounded open set in Rn with smoothbonndary and the nonlinearity bu+ crosses eigenvalues of △2 +c△. They investigate therelatiolls when the source term is constant and when it is generated by two eigenfuntions. 展开更多
关键词 Nonlinear elliptic equation SOLUTION source terms boundary value problem
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Least-squares finite-element method for shallow-water equations with source terms 被引量:2
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作者 Shin-Jye Liang Tai-Wen Hsu 《Acta Mechanica Sinica》 SCIE EI CAS CSCD 2009年第5期597-610,共14页
Numerical solution of shallow-water equations (SWE) has been a challenging task because of its nonlinear hyperbolic nature, admitting discontinuous solution, and the need to satisfy the C-property. The presence of s... Numerical solution of shallow-water equations (SWE) has been a challenging task because of its nonlinear hyperbolic nature, admitting discontinuous solution, and the need to satisfy the C-property. The presence of source terms in momentum equations, such as the bottom slope and friction of bed, compounds the difficulties further. In this paper, a least-squares finite-element method for the space discretization and θ-method for the time integration is developed for the 2D non-conservative SWE including the source terms. Advantages of the method include: the source terms can be approximated easily with interpolation functions, no upwind scheme is needed, as well as the resulting system equations is symmetric and positive-definite, therefore, can be solved efficiently with the conjugate gradient method. The method is applied to steady and unsteady flows, subcritical and transcritical flow over a bump, 1D and 2D circular dam-break, wave past a circular cylinder, as well as wave past a hump. Computed results show good C-property, conservation property and compare well with exact solutions and other numerical results for flows with weak and mild gradient changes, but lead to inaccurate predictions for flows with strong gradient changes and discontinuities. 展开更多
关键词 Shallow-water equations source terms Least-squares finite-element method DAM-BREAK C-property
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Forest Canopy Flow Analysis Using Turbulence Model with Source/Sink Terms
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作者 杨会 付海明 《Journal of Donghua University(English Edition)》 EI CAS 2015年第4期588-593,共6页
A computational fluid dynamics( CFD) model was presented to simulate wind flow over a forest canopy for analyzing the wind flow within and above forest canopies. Unlike previous studies on the canopy flow,the effect o... A computational fluid dynamics( CFD) model was presented to simulate wind flow over a forest canopy for analyzing the wind flow within and above forest canopies. Unlike previous studies on the canopy flow,the effect of canopy contour on the canopy was considered to develop the simulation method into a more general but complex case of wind flow over a forest canopy,using cedrus deodara and cinnamomum camphora. The desire of this work is mainly motivated to provide a rational way for predicting the wind flow within and above vegetation canopies. The model of canopy is not incorporated in the geometrical model,and it uses a porous domain combined with k-ε two-equation turbulence model with source / sink terms. The objectives of this paper are to analyze the contour of pressure and velocity and compare the simulation results with other works and field measurements. Results are encouraging,as the model profiles of mean velocity( u) qualitatively agree well with other works compared with and quantitatively have similar explanations as several authors. In conclusion, it is demonstrated that the adoption turbulence model with source / sink terms for forest canopies is proved to be a physically accurate and numerically robust method. The model and method are recommended for future use in simulating turbulent flows in forest canopies. 展开更多
关键词 k-ε source / sink terms mean velocity forest canopy
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On Steady States and Its Capturing Schemes for Shallow-Water Equations with Source Terms
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作者 尹丽 黄明游 尹景学 《Northeastern Mathematical Journal》 CSCD 2004年第3期257-260,共4页
关键词 shallow-water equation source term hydraulic jump balance condition difference scheme
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Exact Solution of Fractional Diffusion Model with Source Term used in Study of Concentration of Fission Product in Uranium Dioxide Particle 被引量:2
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作者 房超 曹建主 孙立风 《Communications in Theoretical Physics》 SCIE CAS CSCD 2011年第5期863-867,共5页
The exact solution of fractional diffusion model with a location-independent source term used in the study of the concentration of fission product in spherical uranium dioxide (U02) particle is built. The adsorption... The exact solution of fractional diffusion model with a location-independent source term used in the study of the concentration of fission product in spherical uranium dioxide (U02) particle is built. The adsorption effect of the fission product on the surface of the U02 particle and the delayed decay effect are also considered. The solution is given in terms of Mittag-Leffler function with finite Hankel integral transformation and Laplace transformation. At last, the reduced forms of the solution under some special physical conditions, which is used in nuclear engineering, are obtained and corresponding remarks are given to provide significant exact results to the concentration analysis of nuclear fission products in nuclear reactor. 展开更多
关键词 fractional diffusion Fick's law source term finite Hankel transformation Laplace transformation
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Optimization of sensor deployment sequences for hazardous gas leakage monitoring and source term estimation 被引量:1
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作者 Jikai Dong Bing Wang +3 位作者 Xinjie Wang Chenxi Cao Shikuan Chen Wenli Du 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2023年第4期169-179,共11页
Nowadays, chemical safety has attracted considerable attention, and chemical gas leakage monitoring and source term estimation(STE) have become hot spots. However, few studies have focused on sensor layouts in scenari... Nowadays, chemical safety has attracted considerable attention, and chemical gas leakage monitoring and source term estimation(STE) have become hot spots. However, few studies have focused on sensor layouts in scenarios with multiple potential leakage sources and wind conditions, and studies on the risk information(RI) detection and prioritization order of sensors have not been performed. In this work, the monitoring area of a chemical factory is divided into multiple rectangles with a uniform mesh. The RI value of each grid node is calculated on the basis of the occurrence probability and normalized concentrations of each leakage scenario. A high RI value indicates that a sensor at a grid node has a high chance of detecting gas concentrations in different leakage scenarios. This situation is beneficial for leakage monitoring and STE. The methods of similarity redundancy detection and the maximization of sensor RI detection are applied to determine the sequence of sensor locations. This study reveals that the RI detection of the optimal sensor layout with eight sensors exceeds that of the typical layout with 12 sensors. In addition, STE with the optimized placement sequence of the sensor layout is numerically simulated. The statistical results of each scenario with various numbers of sensors reveal that STE is affected by sensor number and scenarios(leakage locations and winds). In most scenarios, appropriate STE results can be retained under the optimal sensor layout even with four sensors. Eight or more sensors are advised to improve the performance of STE in all scenarios. Moreover, the reliability of the STE results in each scenario can be known in advance with a specific number of sensors. Such information thus provides a reference for emergency rescue. 展开更多
关键词 Gas leakage source term estimation Sensor layout Risk information Numerical simulation OPTIMIZATION
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Well-posedness for A Plate Equation with Nonlocal Source term
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作者 LIU Gong-wei ZHAO Rui-min ZHANG Hong-wei 《Chinese Quarterly Journal of Mathematics》 2019年第4期331-342,共12页
In this paper,we investigate the initial boundary value problem for a plate equation with nonlocal source term.The local,global existence and exponential decay result are established under certain conditions.Moreover,... In this paper,we investigate the initial boundary value problem for a plate equation with nonlocal source term.The local,global existence and exponential decay result are established under certain conditions.Moreover,we also prove the blow-up in finite time and the lifespan of solution under certain conditions. 展开更多
关键词 Plate equation Nonlocal source term Decay estimate BLOW-UP
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Research on inversion method for complex source-term distributions based on deep neural networks
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作者 Yi‑Sheng Hao Zhen Wu +3 位作者 Yan‑Heng Pu Rui Qiu Hui Zhang Jun‑Li Li 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2023年第12期159-176,共18页
This study proposes a source distribution inversion convolutional neural network (SDICNN), which is deep neural network model for the inversion of complex source distributions, to solve inversion problems involving fi... This study proposes a source distribution inversion convolutional neural network (SDICNN), which is deep neural network model for the inversion of complex source distributions, to solve inversion problems involving fixed-source distributions. A function is developed to obtain the distribution information of complex source terms from radiation parameters at individual sampling points in space. The SDICNN comprises two components:a fully connected network and a convolutional neural network. The fully connected network mainly extracts the parameter measurement information from the sampling points,whereas the convolutional neural network mainly completes the fine inversion of the source-term distribution. Finally, the SDICNN obtains a high-resolution source-term distribution image. In this study, the proposed source-term inversion method is evaluated based on typical geometric scenarios. The results show that, unlike the conventional fully connected neural network, the SDICNN model can extract the two-dimensional distribution features of the source terms, and its inversion results are better. In addition, the effects of the shielding mechanism and number of sampling points on the inversion process are examined. In summary, the result of this study can facilitate the accurate assessment of dose distributions in nuclear facilities. 展开更多
关键词 source term inversion Monte Carlo Artificial intelligence Neural network
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Accident source term and radiological consequences of a small modular reactor
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作者 Hai-Ying Chen Fu-Dong Liu +3 位作者 Shao-Wei Wang Yi-Chuan Wang Chao Xu Qiao-Feng Liu 《Nuclear Science and Techniques》 SCIE EI CAS CSCD 2023年第3期82-92,共11页
Considering the growing global demand for energy and the need for countries to achieve climate goals,there is an increasing global interest in small modular reactors(SMRs)and their applications.Accident source term an... Considering the growing global demand for energy and the need for countries to achieve climate goals,there is an increasing global interest in small modular reactors(SMRs)and their applications.Accident source term and radiological consequence evaluations of SMRs are key components of nuclear and radiation safety reviews,which affect the site,exclusion area(EAB),and low population zone outer boundaries.Based on the design characteristics of the SMR and accident analysis results,a theoretical model of a whole-core fuel cladding damage accident was constructed to study the radioactivity released into the environment and its consequences.The accident source term and radiation dose calculation models were established to analyze the released amounts of radionuclides and the total effective dose affecting individuals at the site boundary.The results showed that the amount of radionuclides released into the environment after a whole-core fuel cladding damage accident reached 10^(14) Bq,among which the release amount of ^(133)Xe was the largest.The total effective dose at the site boundary 30 days after the accident was 8.65 mSv.The highest total effective dose affecting individuals occurred to the east-north-east.The results of the accident source term and radiological consequence provide technical support for site boundary dose assessments and reviews of SMRs. 展开更多
关键词 Small modular reactor ACCIDENT source term Radiological consequence Total effective dose
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An improved four-dimensional variation source term inversion model with observation error regularization
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作者 Chao-shuai Han Xue-zheng Zhu +3 位作者 Jin Gu Guo-hui Yan Xiao-hui Gao Qin-wen Zuo 《Defence Technology(防务技术)》 SCIE EI CAS CSCD 2023年第6期349-360,共12页
Aiming at the Four-Dimensional Variation source term inversion algorithm proposed earlier,the observation error regularization factor is introduced to improve the prediction accuracy of the diffusion model,and an impr... Aiming at the Four-Dimensional Variation source term inversion algorithm proposed earlier,the observation error regularization factor is introduced to improve the prediction accuracy of the diffusion model,and an improved Four-Dimensional Variation source term inversion algorithm with observation error regularization(OER-4DVAR STI model)is formed.Firstly,by constructing the inversion process and basic model of OER-4DVAR STI model,its basic principle and logical structure are studied.Secondly,the observation error regularization factor estimation method based on Bayesian optimization is proposed,and the error factor is separated and optimized by two parameters:error statistical time and deviation degree.Finally,the scientific,feasible and advanced nature of the OER-4DVAR STI model are verified by numerical simulation and tracer test data.The experimental results show that OER-4DVAR STI model can better reverse calculate the hazard source term information under the conditions of high atmospheric stability and flat underlying surface.Compared with the previous inversion algorithm,the source intensity estimation accuracy of OER-4DVAR STI model is improved by about 46.97%,and the source location estimation accuracy is improved by about 26.72%. 展开更多
关键词 source term inversion Four dimensional variation Observation error regularization factor Bayesian optimization SF6 tracer test
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TWO REGULARIZATION METHODS FOR IDENTIFYING THE SOURCE TERM PROBLEM ON THE TIME-FRACTIONAL DIFFUSION EQUATION WITH A HYPER-BESSEL OPERATOR
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作者 Fan YANG Qiaoxi SUN Xiaoxiao LI 《Acta Mathematica Scientia》 SCIE CSCD 2022年第4期1485-1518,共34页
In this paper,we consider the inverse problem for identifying the source term of the time-fractional equation with a hyper-Bessel operator.First,we prove that this inverse problem is ill-posed,and give the conditional... In this paper,we consider the inverse problem for identifying the source term of the time-fractional equation with a hyper-Bessel operator.First,we prove that this inverse problem is ill-posed,and give the conditional stability.Then,we give the optimal error bound for this inverse problem.Next,we use the fractional Tikhonov regularization method and the fractional Landweber iterative regularization method to restore the stability of the ill-posed problem,and give corresponding error estimates under different regularization parameter selection rules.Finally,we verify the effectiveness of the method through numerical examples. 展开更多
关键词 Time-fractional diffusion equation source term problem fractional Landweber regularization method Hyper-Bessel operator fractional Tikhonov regularization method
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Approximation of Derivative for a Singularly Perturbed Second-Order ODE of Robin Type with Discontinuous Convection Coefficient and Source Term
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作者 R.Mythili Priyadharshini N.Ramanujam 《Numerical Mathematics(Theory,Methods and Applications)》 SCIE 2009年第1期100-118,共19页
In this paper, a singularly perturbed Robin type boundary value problem for second-order ordinary differential equation with discontinuous convection coefficient and source term is considered. A robust-layer-resolving... In this paper, a singularly perturbed Robin type boundary value problem for second-order ordinary differential equation with discontinuous convection coefficient and source term is considered. A robust-layer-resolving numerical method is proposed. An e-uniform global error estimate for the numerical solution and also to the numerical derivative are established. Numerical results are presented, which are in agreement with the theoretical predictions. 展开更多
关键词 Singular perturbation problem piecewise uniform mesh discrete derivative discontinuous convection coefficient Robin boundary conditions discontinuous source term.
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Burial fluxes and sources of organic carbon in sediments of the central Yellow Sea mud area over the past 200 years 被引量:4
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作者 YANG Shu YANG Qian +3 位作者 LIU Sai CAI Deling QU Keming SUN Yao 《Acta Oceanologica Sinica》 SCIE CAS CSCD 2015年第10期13-22,共10页
Long-term changes of composition, sources and burial fluxes of TOC (total organic carbon) in sediments of the central Yellow Sea mud area and their possible affecting factors are discussed in this paper. Firstly, si... Long-term changes of composition, sources and burial fluxes of TOC (total organic carbon) in sediments of the central Yellow Sea mud area and their possible affecting factors are discussed in this paper. Firstly, similarity analysis is employed to confirm that the carbon burial features resulted from two collected cores are typical in the central Yellow Sea mud area where YSWC (Yellow Sea Warm Current) is prevalent. On this basis, the burial flux of TOC here was considered to be 235.5-488.4 pmol/(cm^2.a) since the first industrial revolution, accounting for about 70%-90% among burial fluxes of TC (total carbon) in the sediments. Compared TOC/TC ratio in the two cores with that in other marine sediments worldwide, we suggest that the growth of calcareous/non-calcareous organisms and dissolution of IC (inorganic carbon) are important factors controlling the TOC/TC ratio in sediment. Results of two-end mixed model based on fi13C data indicate that marine-derived organic carbon (OCa) is the main part among total burial organic carbon which accounts for a ratio over 85%. Due to the high TOC/TC ratio in the two cores, TC in the sediments also mainly exists as OCa, and the proportion of OCa is about 60%-80%. Away from the shore and relatively high primary production in upper waters are the main reasons that OCa is predominant among all burial OC in sediments of the central Yellow Sea mud area. Burial of OC in this mud area is probably mainly influenced by the human activities. Although the economic development during the late 19th century caused by the first industrial revolution in China did not obviously increase the TOC burial fluxes in the sediments, the rise of industry and agriculture after the founding of new China has clearly increased the TOC burial flux since 1950s. Otherwise, we also realize that among TC burial fluxes, TIC account for about 10%-30% in sediments of the central Yellow Sea mud area, so its burial could not be simply ignored here. Distinct from TOC burial, long-term TIC burial fluxes variations relate with climate changes more closely: the East Asian summer monsoon may influence the strength of the Huanghe River (Yellow River) flood, which could further affect the transport of terrestrial IC from land to the central Yellow Sea as well as the burial of these IC in the sediments. 展开更多
关键词 the central Yellow Sea mud area organic carbon burial flux source long-term changes human activities
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Neural network-based source tracking of chemical leaks with obstacles
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作者 Qiaoyi Xu Wenli Du +1 位作者 Jinjin Xu Jikai Dong 《Chinese Journal of Chemical Engineering》 SCIE EI CAS CSCD 2021年第5期211-220,共10页
The leakage of hazardous gases poses a significant threat to public security and causes environmental damage.The effective and accurate source term estimation(STE)is necessary when a leakage accident occurs.However,mo... The leakage of hazardous gases poses a significant threat to public security and causes environmental damage.The effective and accurate source term estimation(STE)is necessary when a leakage accident occurs.However,most research generally assumes that no obstacles exist near the leak source,which is inappropriate in practical applications.To solve this problem,we propose two different frameworks to emphasize STE with obstacles based on artificial neural network(ANN)and convolutional neural network(CNN).Firstly,we build a CFD model to simulate the gas diffusion in obstacle scenarios and construct a benchmark dataset.Secondly,we define the structure of ANN by searching,then predict the concentration distribution of gas using the searched model,and optimize source term parameters by particle swarm optimization(PSO)with well-performed cost functions.Thirdly,we propose a one-step STE method based on CNN,which establishes a link between the concentration distribution and the location of obstacles.Finally,we propose a novel data processing method to process sensor data,which maps the concentration information into feature channels.The comprehensive experiments illustrate the performance and efficiency of the proposed methods. 展开更多
关键词 OBSTACLE Optimization NEURAL networks FEATURE extraction source term estimation COMPUTATIONAL fluid dynamics (CFD)
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基于二级PSA的应急计划区事故源项选取方法
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作者 王海峰 赵锋 +1 位作者 张启明 殷煜皓 《核动力工程》 北大核心 2026年第1期274-279,共6页
为建立包括大型堆、小型堆和其他类型核电厂用于应急计划区测算的事故源项选取方法,本研究参考国内外现行应急事故源项选取方法,特别是美国核管理委员会(NRC)最新批准的NuScale小型模块化反应堆应急源项的筛选方法,梳理国内二代改进型... 为建立包括大型堆、小型堆和其他类型核电厂用于应急计划区测算的事故源项选取方法,本研究参考国内外现行应急事故源项选取方法,特别是美国核管理委员会(NRC)最新批准的NuScale小型模块化反应堆应急源项的筛选方法,梳理国内二代改进型和三代大型压水堆核电厂现行事故源项选取并分析其共性和不足,在考虑事故机理和应急流程后,推荐基于二级概率安全评价(PSA)的应急计划区事故源项选取方法,并特别考虑地震引发的事故序列,同时分析多机组应急的影响。此方法契合NUREG-0396报告应急源项选取原则,通过实例分析表明,与目前国内大型压水堆核电厂现行事故源项选取具有一致性。本研究源项选取方法有利于不同类型机组统一应急基准,基于机组安全性和厂址应急特征开展应急准备和响应,并可用于各类堆型核电厂应急计划区事故源项的选取。 展开更多
关键词 二级概率安全评价(PSA) 源项 应急计划区 核应急
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基于蒸发法试验的铅铋快堆挥发性核素源项计算方法研究
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作者 黄丽萍 王凤龙 +3 位作者 张强 王事喜 朱润 杨勇 《原子能科学技术》 北大核心 2026年第1期185-194,共10页
针对轻水堆与钠冷快堆源项计算方法无法直接用于铅铋快堆的问题,为研究挥发性核素从铅铋冷却剂向覆盖气腔、安全壳的迁移行为并获取迁移数据,建立了一套适用于铅铋堆的源项计算方法,以蒸发平衡模型为基础,进行了蒸发法试验,对300~1000... 针对轻水堆与钠冷快堆源项计算方法无法直接用于铅铋快堆的问题,为研究挥发性核素从铅铋冷却剂向覆盖气腔、安全壳的迁移行为并获取迁移数据,建立了一套适用于铅铋堆的源项计算方法,以蒸发平衡模型为基础,进行了蒸发法试验,对300~1000℃下不同气氛(纯Ar、Ar+5%H_(2)、Ar+2%H_(2)O)LBE中钋的蒸发行为及其亨利常数、300~600℃下LBE-3%CsI和LBE-1%Te合金气溶胶的粒径分布进行了研究。结果表明,钋的亨利常数在高温下具有较好的一致性,低温下钋的蒸发更容易受到氧化还原与表面富集的影响,造成亨利常数测量值偏大;铅铋合金气溶胶粒径在几百纳米至微米量级。基于试验结果建立的铅铋快堆覆盖气腔、安全壳及环境释放的源项计算方法,可有效评估铅铋快堆在不同工况下的挥发性核素释放量,能为铅铋快堆安全分析提供参考。 展开更多
关键词 铅铋快堆 挥发性核素 蒸发法试验 源项计算方法
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具黏弹性项的四阶变系数波方程解的衰减估计
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作者 张帅 高云柱 《吉林大学学报(理学版)》 北大核心 2026年第2期221-226,共6页
考虑一类具有对数源项和黏弹性项的变系数波方程的初边值问题.首先,讨论非均匀介质中对数源项与黏弹性项对该问题解的长时间动力学行为的影响.其次,通过构造一类特殊乘子并结合对数型Sobolev不等式,证明当初始能量满足0<E(0)<d(d... 考虑一类具有对数源项和黏弹性项的变系数波方程的初边值问题.首先,讨论非均匀介质中对数源项与黏弹性项对该问题解的长时间动力学行为的影响.其次,通过构造一类特殊乘子并结合对数型Sobolev不等式,证明当初始能量满足0<E(0)<d(d为阱深)时,系统能量泛函具有指数衰减性. 展开更多
关键词 波方程 对数源项 黏弹性项 变系数
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石墨孔隙动态变化对球床式高温气冷堆^(14)C源项影响研究
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作者 曹成昊 王雯毅 +3 位作者 梁金刚 陈俊逸 李川 曹建主 《核动力工程》 北大核心 2026年第1期142-150,共9页
高温气冷堆石墨孔隙内^(14)N的活化及粉尘磨损等现象,使得^(14)C在一回路中的产生与释放分析面临挑战。为了提高^(14)C活化源项分析精度,本文基于石墨孔隙动态变化模型,研究了孔隙打开速率对^(14)N活化及孔隙表面^(14)C腐蚀的影响。此外... 高温气冷堆石墨孔隙内^(14)N的活化及粉尘磨损等现象,使得^(14)C在一回路中的产生与释放分析面临挑战。为了提高^(14)C活化源项分析精度,本文基于石墨孔隙动态变化模型,研究了孔隙打开速率对^(14)N活化及孔隙表面^(14)C腐蚀的影响。此外,以10 MW高温气冷堆(HTR-10)为研究对象,系统分析^(14)C的产生与释放特征,并将理论计算结果与堆内实测数据进行对比。结果表明,堆内^(14)C主要由^(14)N的活化产生,孔隙动态变化影响可腐蚀表面^(14)C的盘存量和^(14)CO的释放率;在寿期初,^(14)C集中于堆芯燃料元件,而在寿期末,反射层中的^(14)C占比更高;冷却剂中的^(14)C主要以^(14)CO的形式存在;粉尘载带的^(14)C沉积在一回路表面,且反射层磨损对寿期末粉尘中^(14)C比活度的增加有贡献。本文计算得到的一回路^(14)CO浓度比传统模型更接近堆内实测值,验证了模型的有效性,研究结果对提升高温气冷堆安全分析精度具有重要意义。 展开更多
关键词 高温气冷堆 ^(14)C 源项分析 活化产物
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武汉城区大气PM2.5中多环芳烃污染特征、来源及健康风险评价
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作者 宋华英 唐娇 +2 位作者 杨一凡 邓萌杰 成海容 《环境科学研究》 北大核心 2026年第3期614-624,共11页
多环芳烃(Polycyclic aromatic hydrocarbons,PAHs)是大气细颗粒物(PM2.5)的关键有毒成分,其危害不容小觑,但目前关于武汉市大气PM2.5中PAHs污染特征和来源年际变化趋势的研究较为匮乏。本研究于2018年和2023年在武汉城区站点采集PM2.5... 多环芳烃(Polycyclic aromatic hydrocarbons,PAHs)是大气细颗粒物(PM2.5)的关键有毒成分,其危害不容小觑,但目前关于武汉市大气PM2.5中PAHs污染特征和来源年际变化趋势的研究较为匮乏。本研究于2018年和2023年在武汉城区站点采集PM2.5样品,并运用气相色谱-质谱联用仪(GC-MS)对PM2.5样品中18种PAHs的浓度进行测定,分析了2018年和2023年武汉市城区大气PM2.5中PAHs的污染水平、来源及健康风险。结果表明:(1)2018年和2023年武汉市城区大气PM2.5中∑18PAHs的平均浓度分别为19.82和15.76 ng/m3,2023年相比2018年有所下降。(2)机动车排放源、化石燃料燃烧对2018年和2023年武汉市城区大气PM2.5中PAHs的贡献较大,相比2018年,2023年机动车排放源的相对贡献率有所增加,而化石燃料燃烧源的相对贡献率有所下降,二者对PAHs浓度的贡献率均有所下降。(3)2018年和2023年儿童、青少年吸入PAHs的致癌风险可以忽略,而2023年成年人的致癌风险虽相比2018年有所下降,但仍有潜在的较低致癌风险。研究显示,武汉市城区PM2.5中PAHs污染得到改善,但机动车源的相对贡献增加,且成年人仍存在潜在的低致癌风险。 展开更多
关键词 多环芳烃(PAHs) 年际变化趋势 污染来源 健康风险
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