In this paper, taking its turbulent exchange coefficient as a function of the Lagrangian time scale and standard variance of the turbulence in atmosphere, the atmospheric dispersion PDF models are obtained on the basi...In this paper, taking its turbulent exchange coefficient as a function of the Lagrangian time scale and standard variance of the turbulence in atmosphere, the atmospheric dispersion PDF models are obtained on the basis of atmospheric diffusion K-theory. In the model the statistics of wind speed are directly used as its parameters instead of classic dispersion parameters. The bi- Gaussian PDF is derived in convective boundary layer (CBL), from the statistics of vertical velocity in both of the downdraft and updraft regions that are investigated theoretically in the other part of this paper. Giving the driven parameters of the CBL (including the convective velocity scale w* and the mixing depth h_i) and the time-averaged wind speed at release level, the PDF model is able to simulate the distribution of concentration released at any levels in the CBL. The PDF's simulations are fairly consistent with the measurements in CONDORS experiment or the results brought out by some numerical simulations.展开更多
Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to so...Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to solve this issue that has bothered human society for the last centuries.Scientists have endeavored to figure out the laws of atmospheric pollutant diffusion using various mathematical models and statistical models,and drawn some precious conclusions.This paper explored the basic model of atmospheric diffusion—modeling and solution of Gaussian Diffusion Model,clarify its principles and operation forms,then applied the model into the PM_(2.5) atmospheric diffusion cases,make the program planning base on the results of model calculation,and get the final conclusion.展开更多
To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shan...To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.展开更多
Quantitative real-time retrieval of concentration-lengths (CL) through gaseous plumes is an important tool for environmental monitoring, enabling remote monitoring of emissions from industrial facilities and risk asse...Quantitative real-time retrieval of concentration-lengths (CL) through gaseous plumes is an important tool for environmental monitoring, enabling remote monitoring of emissions from industrial facilities and risk assessment in scenarios of toxic gas releases. The adoption of LWIR (Long Wave InfraRed) hyperspectral imaging as a leading technique for remote gas plume detection paved the way for an introduction of a precise CL estimation and two-dimensional (2D) mapping. A novel methodology for evaluating and characterizing the performance of a retrieval algorithm is presented. The algorithm utilizes state-of-the-art retrieved hyperspectral 2D mapping and is applied on a series of localized atmospheric tracer gas (SF<sub><span style="font-family:Verdana;">6</span></sub><span style="font-family:Verdana;">) releases in monitored environmental conditions. The retrieved CL distributions are compared to a numeric atmospheric T&D (Transport and Diffusion) model. Satisfactory agreement between retrieved and simulated CL prediction is manifested, and the uncertainty involved is quantified. Possible sources for the remained discrepancies between retrieved and simulated CL values are characterized, and methods to minimize them are discussed.</span>展开更多
A global mean ocean model including atmospheric heating, heat capacity of the mixed layer ocean, and vertical thermal diffusivity in the lower ocean, proposed by Cess and Goldenberg (1981), is used in this paper to st...A global mean ocean model including atmospheric heating, heat capacity of the mixed layer ocean, and vertical thermal diffusivity in the lower ocean, proposed by Cess and Goldenberg (1981), is used in this paper to study the sensitivity of global warming to the vertical diffusivity. The results suggest that the behaviour of upper ocean temperature is mainly determined by the magnitude of upper layer diffusivity and an ocean with a larger diffusivity leads to a less increase of sea surface temperature and a longer time delay for the global warming induced by increasing CO2 than that with smaller one. The global warming relative to four scenarios of CO2 emission assumed by Intergovernmental Panel of Climate Change (IPCC) is also estimated by using the model with two kinds of thermal diffusivities. The result shows that for various combinations of the CO2 emission scenarios and the diffusivities, the oceanic time delay to the global warming varies from 15 years to 70 years.展开更多
Haze is a pollution weather phenomenon that has been widely concerned by people in recent years. It has a significant impact on people’s production, life, and health. This study focuses on large-scale haze weather th...Haze is a pollution weather phenomenon that has been widely concerned by people in recent years. It has a significant impact on people’s production, life, and health. This study focuses on large-scale haze weather that happened in eastern China in late January 2021. The research uses multi-party data and synoptic analysis methods to analyze the occurrence, evolution, and end of the haze weather. The polar vortex, the change of the atmospheric circulation, the change of the cold air force, the temperature and humidity, and the rain and snow weather are the important reasons for this weathering process. It can be used for reference in future research on haze weather.展开更多
In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open ...In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open space outside the electrode structure at a lower voltage by constructing a three-dimensional non-uniform spatial electric field using a contact electrode structure.The air purification study is also carried out.Firstly,a contact electrode structure is constructed using a three-dimensional wire electrode.The distribution characteristics of the spatial electric field formed by this electrode structure are analyzed,and the effects of the non-uniform electric field and the different angles of the vertical wire on the generation of three-dimensional spatial diffuse discharge are investigated.Secondly,the copper foam contact electrode structure is constructed using copper foam material,and the effects of different mesh sizes on the electric field distribution are analyzed.The results show that as the mesh size of the copper foam becomes larger,a strong electric field region exists not only on the surface of the insulating layer,but also on the surface of the vertical wires inside the copper foam,i.e.,the strong electric field region shows a three-dimensional distribution.Besides,as the mesh size increases,the area of the vertical strong electric field also increases.However,the electric field strength on the surface of the insulating layer gradually decreases.Therefore,the appropriate mesh size can effectively increase the discharge area,which is conducive to improving the air purification efficiency.Finally,a highly permeable stacked electrode structure of multilayer wire-copper foam is designed.In combination with an ozone treatment catalyst,an air purification device is fabricated,and the air purification experiment is carried out.展开更多
By using the meteorological data in the pollution boundary layer which was observed in two ground observation sites:coast and land in the river outlet area of Grand Liao River during January-February in 2007,the daily...By using the meteorological data in the pollution boundary layer which was observed in two ground observation sites:coast and land in the river outlet area of Grand Liao River during January-February in 2007,the daily change characteristics of pollute boundary layer in winter in the area were discussed. The results showed that the pollute boundary layer in the river outlet area of Grand Liao River was affected by the sea and land. In the certain weather condition,maybe the sea-land breeze appeared in the low altitude which was below 200 m in the coastal zone. The stability change in the different height in the coastal zone was more stable than in the land zone,and the wind field change in the area was mainly in 300 m low altitude. At night,the temperature inversion often appears in the area,and the thickness of temperature inversion layer is stably during 200-300 m. The thermal internal boundary layer penetrated deeply into the land about 10 km,and the height could reach 800 m. The atmospheric diffusion ability in the coastal area was weaker and stronger in the land area.展开更多
In this paper,the circulation background,the characteristics of meteorological elements configuration in the boundary layer and the stable meteorological conditions in two precipitation episodes(during February 19-21,...In this paper,the circulation background,the characteristics of meteorological elements configuration in the boundary layer and the stable meteorological conditions in two precipitation episodes(during February 19-21,2015 and February 10-13,2016,respectively)within the Beijing-Tianjin-Hebei region are compared and analyzed.Data from conventional meteorological observations,air quality monitoring,reanalysis and numerical models are used.The results show that before the two precipitation processes in 2015 and 2016,the circulations in the middle and high latitudes of Asia and Europe demonstrate“two troughs and one ridge”.Besides,the weather is stable and the pollutant concentration is relatively high.During the precipitation,the circulation is relatively stable for the episode in 2015,and no obvious change in the synoptic system is observed.However,during the episode in 2016,the formation of blocking high and the enhancement of the average ridge in western Asia cause obvious change in the circulation.The simulation results show that significant removal can be detected in both cases,and the PM_(2.5) wet deposition fluxes are 647 g/ha and 486 g/ha,respectively,with the removal in 2015 slightly stronger than that in 2016.The removal and dissipation of pollutants is determined by the atmospheric diffusion conditions and the precipitation,especially in the former episode.In the case of February 2016,good diffusion conditions and the precipitation demonstrate obvious PM_(2.5) removal effect.In the case of February 2015,the longstanding calm wind with high humidity and the physical quantity configuration in the lower mixed layer lead to the poor pollutant removal.展开更多
基金This paper supported by the National Natural Science Foundation of China under Grant No.49475247.
文摘In this paper, taking its turbulent exchange coefficient as a function of the Lagrangian time scale and standard variance of the turbulence in atmosphere, the atmospheric dispersion PDF models are obtained on the basis of atmospheric diffusion K-theory. In the model the statistics of wind speed are directly used as its parameters instead of classic dispersion parameters. The bi- Gaussian PDF is derived in convective boundary layer (CBL), from the statistics of vertical velocity in both of the downdraft and updraft regions that are investigated theoretically in the other part of this paper. Giving the driven parameters of the CBL (including the convective velocity scale w* and the mixing depth h_i) and the time-averaged wind speed at release level, the PDF model is able to simulate the distribution of concentration released at any levels in the CBL. The PDF's simulations are fairly consistent with the measurements in CONDORS experiment or the results brought out by some numerical simulations.
基金Program of Regional Tourism Development and Rural Revitalization Coordination Center (2020Z04)。
文摘Air pollution as one of the major environmental issues in modern society,has already brought severe impact to human life and production,thus it is an urgent task for studying environmental and ecological science to solve this issue that has bothered human society for the last centuries.Scientists have endeavored to figure out the laws of atmospheric pollutant diffusion using various mathematical models and statistical models,and drawn some precious conclusions.This paper explored the basic model of atmospheric diffusion—modeling and solution of Gaussian Diffusion Model,clarify its principles and operation forms,then applied the model into the PM_(2.5) atmospheric diffusion cases,make the program planning base on the results of model calculation,and get the final conclusion.
文摘To provide effective environmental management for total amount control of atmospheric pollutants. Methods An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54 279.792 tons per year in 2010. Conclusion The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.
文摘Quantitative real-time retrieval of concentration-lengths (CL) through gaseous plumes is an important tool for environmental monitoring, enabling remote monitoring of emissions from industrial facilities and risk assessment in scenarios of toxic gas releases. The adoption of LWIR (Long Wave InfraRed) hyperspectral imaging as a leading technique for remote gas plume detection paved the way for an introduction of a precise CL estimation and two-dimensional (2D) mapping. A novel methodology for evaluating and characterizing the performance of a retrieval algorithm is presented. The algorithm utilizes state-of-the-art retrieved hyperspectral 2D mapping and is applied on a series of localized atmospheric tracer gas (SF<sub><span style="font-family:Verdana;">6</span></sub><span style="font-family:Verdana;">) releases in monitored environmental conditions. The retrieved CL distributions are compared to a numeric atmospheric T&D (Transport and Diffusion) model. Satisfactory agreement between retrieved and simulated CL prediction is manifested, and the uncertainty involved is quantified. Possible sources for the remained discrepancies between retrieved and simulated CL values are characterized, and methods to minimize them are discussed.</span>
文摘A global mean ocean model including atmospheric heating, heat capacity of the mixed layer ocean, and vertical thermal diffusivity in the lower ocean, proposed by Cess and Goldenberg (1981), is used in this paper to study the sensitivity of global warming to the vertical diffusivity. The results suggest that the behaviour of upper ocean temperature is mainly determined by the magnitude of upper layer diffusivity and an ocean with a larger diffusivity leads to a less increase of sea surface temperature and a longer time delay for the global warming induced by increasing CO2 than that with smaller one. The global warming relative to four scenarios of CO2 emission assumed by Intergovernmental Panel of Climate Change (IPCC) is also estimated by using the model with two kinds of thermal diffusivities. The result shows that for various combinations of the CO2 emission scenarios and the diffusivities, the oceanic time delay to the global warming varies from 15 years to 70 years.
文摘Haze is a pollution weather phenomenon that has been widely concerned by people in recent years. It has a significant impact on people’s production, life, and health. This study focuses on large-scale haze weather that happened in eastern China in late January 2021. The research uses multi-party data and synoptic analysis methods to analyze the occurrence, evolution, and end of the haze weather. The polar vortex, the change of the atmospheric circulation, the change of the cold air force, the temperature and humidity, and the rain and snow weather are the important reasons for this weathering process. It can be used for reference in future research on haze weather.
基金supported by the Fundamental Research Funds for the Central Universities(No.2022YJS094)。
文摘In this work,based on the role of pre-ionization of the non-uniform electric field and its effect of reducing the collisional ionization coefficient,a diffuse dielectric barrier discharge plasma is formed in the open space outside the electrode structure at a lower voltage by constructing a three-dimensional non-uniform spatial electric field using a contact electrode structure.The air purification study is also carried out.Firstly,a contact electrode structure is constructed using a three-dimensional wire electrode.The distribution characteristics of the spatial electric field formed by this electrode structure are analyzed,and the effects of the non-uniform electric field and the different angles of the vertical wire on the generation of three-dimensional spatial diffuse discharge are investigated.Secondly,the copper foam contact electrode structure is constructed using copper foam material,and the effects of different mesh sizes on the electric field distribution are analyzed.The results show that as the mesh size of the copper foam becomes larger,a strong electric field region exists not only on the surface of the insulating layer,but also on the surface of the vertical wires inside the copper foam,i.e.,the strong electric field region shows a three-dimensional distribution.Besides,as the mesh size increases,the area of the vertical strong electric field also increases.However,the electric field strength on the surface of the insulating layer gradually decreases.Therefore,the appropriate mesh size can effectively increase the discharge area,which is conducive to improving the air purification efficiency.Finally,a highly permeable stacked electrode structure of multilayer wire-copper foam is designed.In combination with an ozone treatment catalyst,an air purification device is fabricated,and the air purification experiment is carried out.
基金Supported by The Special Project of Public Welfare Industry(Meteorology)of Science and Technology Ministry(GYHY200806020)The National Natural Science Fund(40975084)The Science Research Fund of Liaoning Meteorological Bureau(2008008)
文摘By using the meteorological data in the pollution boundary layer which was observed in two ground observation sites:coast and land in the river outlet area of Grand Liao River during January-February in 2007,the daily change characteristics of pollute boundary layer in winter in the area were discussed. The results showed that the pollute boundary layer in the river outlet area of Grand Liao River was affected by the sea and land. In the certain weather condition,maybe the sea-land breeze appeared in the low altitude which was below 200 m in the coastal zone. The stability change in the different height in the coastal zone was more stable than in the land zone,and the wind field change in the area was mainly in 300 m low altitude. At night,the temperature inversion often appears in the area,and the thickness of temperature inversion layer is stably during 200-300 m. The thermal internal boundary layer penetrated deeply into the land about 10 km,and the height could reach 800 m. The atmospheric diffusion ability in the coastal area was weaker and stronger in the land area.
基金co-funded by the National Key Research Program of China(Grant No.2016YFC0203301).
文摘In this paper,the circulation background,the characteristics of meteorological elements configuration in the boundary layer and the stable meteorological conditions in two precipitation episodes(during February 19-21,2015 and February 10-13,2016,respectively)within the Beijing-Tianjin-Hebei region are compared and analyzed.Data from conventional meteorological observations,air quality monitoring,reanalysis and numerical models are used.The results show that before the two precipitation processes in 2015 and 2016,the circulations in the middle and high latitudes of Asia and Europe demonstrate“two troughs and one ridge”.Besides,the weather is stable and the pollutant concentration is relatively high.During the precipitation,the circulation is relatively stable for the episode in 2015,and no obvious change in the synoptic system is observed.However,during the episode in 2016,the formation of blocking high and the enhancement of the average ridge in western Asia cause obvious change in the circulation.The simulation results show that significant removal can be detected in both cases,and the PM_(2.5) wet deposition fluxes are 647 g/ha and 486 g/ha,respectively,with the removal in 2015 slightly stronger than that in 2016.The removal and dissipation of pollutants is determined by the atmospheric diffusion conditions and the precipitation,especially in the former episode.In the case of February 2016,good diffusion conditions and the precipitation demonstrate obvious PM_(2.5) removal effect.In the case of February 2015,the longstanding calm wind with high humidity and the physical quantity configuration in the lower mixed layer lead to the poor pollutant removal.
