As part of the development work of the Chinese new regional climate model (RIEMS), the radiative process of black carbon (BC) aerosols has been introduced into the original radiative procedures of RIEMS, and the trans...As part of the development work of the Chinese new regional climate model (RIEMS), the radiative process of black carbon (BC) aerosols has been introduced into the original radiative procedures of RIEMS, and the transport model of BC aerosols has also been established and combined with the RIEMS model. Using the new model system, the distribution of black carbon aerosols and their radiative effect over the China region are investigated. The influences of BC aerosole on the atmospheric radiative transfer and on the air temperature, land surface temperature, and total rainfall are analyzed. It is found that BC aerosols induce a positive radiative forcing at the top of the atmosphere (TOA), which is dominated by shortwave radiative forcing. The maximum radiative forcing occurs in North China in July and in South China in April. At the same time, negative radiative forcing is observed on the surface. Based on the radiative forcing comparison between clear sky and cloudy sky, it is found that cloud can enforce the TOA positive radiative forcing and decrease the negative surface radiative forcing. The responses of the climate system in July to the radiative forcing due to BC aerosols are the decrease in the air temperature in the middle and lower reaches of the Changjiang River and Huaihe area and most areas of South China, and the weak increase or decrease in air temperature over North China. The total rainfall in the middle and lower reaches of the Changjiang River area is increased, but it decreased in North China in July.展开更多
Cloud microphysical and rainfall responses to radiative processes are examined through analysis of cloud-resolving model sensitivity experiments of Typhoon Fitow（2013） during landfall.The budget analysis shows that ...Cloud microphysical and rainfall responses to radiative processes are examined through analysis of cloud-resolving model sensitivity experiments of Typhoon Fitow（2013） during landfall.The budget analysis shows that the increase in the mean rainfall caused by the exclusion of radiative effects of water clouds corresponds to the decrease in accretion of raindrops by cloud ice in the presence of radiative effects of ice clouds,but the rainfall is insensitive to radiative effects of water clouds in the absence of radiative effects of ice clouds.The increases in the mean rainfall resulting from the removal of radiative effects of ice clouds correspond to the enhanced net condensation.The increases（decreases） in maximum rainfall caused by the exclusion of radiative effects of water clouds in the presence（absence） of radiative effects of ice clouds,or the removal of radiative effects of ice clouds in the presence（absence） of radiative effects of water clouds,correspond mainly to the enhancements（reductions） in net condensation.The mean rain rate is a product of rain intensity and fractional rainfall coverage.The radiation-induced difference in the mean rain rate is related to the difference in rain intensity.The radiation-induced difference in the maximum rain rate is associated with the difference in the fractional coverage of maximum rainfall.展开更多
Intensive measurements were conducted in Xi’an,China before and during a COVID-19 lockdown period to investigate how changes in anthropogenic emissions affected the optical properties and radiative effects of brown c...Intensive measurements were conducted in Xi’an,China before and during a COVID-19 lockdown period to investigate how changes in anthropogenic emissions affected the optical properties and radiative effects of brown carbon(BrC)aerosol.The contribution of BrC to total aerosol light absorption during the lockdown(13%-49%)was higher compared with the normal period(4%-29%).Mass absorption cross-sections(MACs)of specific organic aerosol(OA)factors were calculated from a ridge regression model.Of the primary OA(POA),coal combustion OA(CCOA)had the largest MACs at all tested wave-lengths during both periods due to high molecular-weight BrC chromophores;that was followed by biomass burning OA(BBOA)and hydrocarbon-like OA(HOA).For secondary OA(SOA),the MACs of the lessoxidized oxygenated OA(OOA)species(LO-OOA)atλ=370-590 nm were higher than those of more-oxidized OOA(MO-OOA)during both periods,presumably due to chromophore bleaching.The largest contributor to BrC absorption at the short wavelengths was CCOA during both periods,but BrC absorption by LO-OOA and MO-OOA became dominant at longer wavelengths during the lockdown.The estimated radiation forcing efficiency of BrC over 370-600 nm increased from 37.5 W·gduring the normal period to 50.2 W·gduring the lockdown,and that enhancement was mainly caused by higher MACs for both LO-OOA and MO-OOA.This study provides insights into the optical properties and radiative effects of source-specific BrC aerosol when pollution emissions are reduced.展开更多
The authors examine the equilibrium climatic response to the direct radiative effect （DRE） of mineral dust and sea salt aerosols in a doubled-CO2 climate with two-way coupling of aerosol-climate interactions.In resp...The authors examine the equilibrium climatic response to the direct radiative effect （DRE） of mineral dust and sea salt aerosols in a doubled-CO2 climate with two-way coupling of aerosol-climate interactions.In response to the drier and windier conditions,dust emissions increase by 26％ in the Sahara Desert and by 18％ on the global scale relative to present day.Sea salt emissions increase in high latitudes （＞60°） but decrease in middle latitudes （30°-60°） of both hemispheres due to the poleward shift of westerlies,leading to a 3％ decrease in global emissions.The burdens of dust and sea salt increase by 31％ and 7％ respectively,because reductions in rainfall over the tropical oceans increase the lifetime of particles in the warmer climate.The higher aerosol loading in the doubled-CO2 climate reinforces aerosol DRE by -0.2 W m-2,leading to an additional cooling of 0.1℃ at the surface compared with the climatic effects of aerosols in present day.The additional cooling from changes in natural aerosols compensates for up to 15％ of the regional warming induced by doubled CO2.展开更多
Cloud radiative effects （CREs） at the top of the atmosphere （TOA） in three reanalysis datasets （the Eur- opean Center for Medium-Range Weather Forecasts In- terim Reanalysis （ERA-Interim）, the Japanese 55-yr Re...Cloud radiative effects （CREs） at the top of the atmosphere （TOA） in three reanalysis datasets （the Eur- opean Center for Medium-Range Weather Forecasts In- terim Reanalysis （ERA-Interim）, the Japanese 55-yr Re- analysis Project （JRA-55）, and the Modem-Era Retro- spective Analysis for Research and Applications （MERRA）） are evaluated using recent satellite-based observations. The reanalyses can basically capture the spatial pattern of the annual mean shortwave CRE, but the global mean longwave CRE in ERA-interim and JRA55 is weaker than observed, leading to overestimations of the net CRE. Moreover, distinct CRE biases of the reanalyses occur in the Intertropical Convergence Zone （ITCZ）, coastal Pa- cific and Atlantic regions, and East Asia. Quantitative examination further indicates that the spatial correlations of CREs and TOA upward radiation fluxes with corre- sponding observations in ERA-Interim are better than in the other two reanalyses. Although MERRA has certain abilities in producing the magnitudes of global mean CREs, its performance in terms of spatial correlations in winter and summer are worse than for the other two re- analyses. The ability of JRA55 in reflecting CREs lies between the other two datasets. Compared to the global mean results, the spatial correlations of shortwave CRE in East Asia decrease and the biases of regional mean CREs increase in the three reanalyses. This implies that, cur- rently, it is still difficult to reproduce East Asian CREs based on these reanalyses. Relatively, ERA-Interim de- scribes the seasonal variation of East Asian CREs well, albeit weaker than observed. The present study also sug- gests that in-depth exploration of the ability of reanalysis data to describe aspects relating to cloud properties and rad- iation is needed usin~ more comprehensive observations.展开更多
The Regional Integrated Environmental Model System （RIEMS 2.0） coupled with a chemistry-aerosol model and the Princeton Ocean Model （POM） is employed to simulate regional oceanic impact on atmospheric circulation ...The Regional Integrated Environmental Model System （RIEMS 2.0） coupled with a chemistry-aerosol model and the Princeton Ocean Model （POM） is employed to simulate regional oceanic impact on atmospheric circulation and the direct radiative effect （DRE） of aerosol over East Asia. The aerosols considered in this study include both major anthropogenic aerosols （e.g., sulfate, black carbon, and organic carbon） and natural aerosols （e.g., soil dust and sea salt）. The RIEMS 2.0 is driven by NCEP/NCAR reanalysis II, and the simulated period is from 1 January to 31 December 2006. The results show the following： （1） The simulated annual mean sea-level pressure by RIEMS 2.0 with POM is lower than without POM over the mainland and higher without POM over the ocean. （2） In summer, the subtropical high simulated by RIEMS 2.0 with POM is stronger and extends further westward, and the continental low is stronger than without POM in summer. （3） The aerosol optical depth （AOD） simulated by RIEMS 2.0 with POM is larger in the middle and lower reaches of the Yangtze River than without POM. （4） The direct radiative effect with POM is stronger than that without POM in the middle and lower reaches of the Yangtze River and parts of southern China. Therefore, the authors should take account of the impact of the regional ocean model on studying the direct climate effect ＆aerosols in long term simulation.展开更多
In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced ...In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m^3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m^3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m^2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols.展开更多
Current global climate models cannot resolve the complex topography over the Tibetan Plateau(TP)due to their coarse resolution.This study investigates the impacts of horizontal resolution on simulating aerosol and its...Current global climate models cannot resolve the complex topography over the Tibetan Plateau(TP)due to their coarse resolution.This study investigates the impacts of horizontal resolution on simulating aerosol and its direct radiative effect(DRE)over the TP by applying two horizontal resolutions of about 100 km and 25 km to the Chinese Academy of Sciences Flexible Global Ocean-Atmosphere Land System(CAS FGOALS-f3)over a 10-year period.Compared to the AErosol RObotic NETwork observations,a high-resolution model(HRM)can better reproduce the spatial distribution and seasonal cycles of aerosol optical depth(AOD)compared to a low-resolution model(LRM).The HRM bias and RMSE of AOD decreased by 0.08 and 0.12,and the correlation coefficient increased by 0.22 compared to the LRM.An LRM is not sufficient to reproduce the aerosol variations associated with fine-scale topographic forcing,such as in the eastern marginal region of the TP.The difference between hydrophilic aerosols in an HRM and LRM is caused by the divergence of the simulated relative humidity(RH).More reasonable distributions and variations of RH are conducive to simulating hydrophilic aerosols.An increase of the 10-m wind speed in winter by an HRM leads to increased dust emissions.The simulated aerosol DREs at the top of the atmosphere(TOA)and at the surface by the HRM are–0.76 W m^(–2)and–8.72 W m^(–2)over the TP,respectively.Both resolution models can capture the key feature that dust TOA DRE transitions from positive in spring to negative in the other seasons.展开更多
To assess individual direct radiative effects of diverse aerosol species on a regional scale, the air quality modeling system RAMS-CMAQ （Regional Atmospheric Modeling System and Community Multiscale Air Quality） cou...To assess individual direct radiative effects of diverse aerosol species on a regional scale, the air quality modeling system RAMS-CMAQ （Regional Atmospheric Modeling System and Community Multiscale Air Quality） coupled with an aerosol optical properties/radiative transfer module was used to simulate the temporal and spatial distributions of their optical and radiative properties over East Asia throughout 2005. Annual and seasonal averaged aerosol direct radiative forcing （ADRF） of all important aerosols and individual components, such as sulfate, nitrate, ammonium, black carbon （BC）, organic carbon （OC）, and dust at top-of-atmosphere （TOA） in clear sky are analyzed. Analysis of the model results shows that the annual average ADRF of all important aerosols was in the range of 0 to -18 W m-z, with the maximum values mainly distributed over the Sichuan Basin. The direct radiative effects of sulfate, nitrate, and ammonium make up most of the total ADRF in East Asia, being concentrated mainly over North and Southeast China. The model domain is also divided into seven regions based on different administrative regions or countries to investigate detailed information about regional ADRF variations over East Asia. The model results show that the ADRFs of sulfate, ammonium, BC, and OC were stronger in summer and weaker in winter over most regions of East Asia, except over Southeast Asia. The seasonal variation in the ADRF of nitrate exhibited the opposite trend. A strong ADRF of dust mainly appeared in spring over Northwest China and Mongolia.展开更多
The study of shortwave(SW) radiation and its interactions with our planet has proven critical for advancing the understanding of the Earth–atmosphere system. Here, the author shares an accessible and high-level persp...The study of shortwave(SW) radiation and its interactions with our planet has proven critical for advancing the understanding of the Earth–atmosphere system. Here, the author shares an accessible and high-level perspective on recent progress, surprises encountered, and promising future research directionsa. A brief context for the study of SW radiation is provided, after which three specific aspects are focused upon that the author considers particularly important. First, the significance of three-dimensional(3D) SW radiative effects is highlighted via impacts on surface downward SW radiation in complex cloud fields. Crucially, it is shown that probability distributions of surface radiation can only be reliably simulated when accounting for 3D effects, which has implications for various applications and next-generation atmospheric modeling. Second, the significance of the often overlooked diurnal cycle in global top-of-atmosphere upward SW radiation is underscored by quantifying the controlling properties and processes. Opportunities for improved future satellite observations of the global diurnal cycle are noted. Third, the wealth of information provided by the spectral dimension of SW radiation is demonstrated through the extraction and attribution of SW spectral signatures. It is argued that further exploration of the spectral dimension, aided by the recently launched and upcoming suite of spectrally resolved SW satellite observations, promises a new era of SW radiation research.展开更多
Due to increased aerosol emissions and unfavorable weather conditions, severe haze events have occurred fre- quently in China in the last 10 years. In addition, the interaction between the boundary layer and the aeros...Due to increased aerosol emissions and unfavorable weather conditions, severe haze events have occurred fre- quently in China in the last 10 years. In addition, the interaction between the boundary layer and the aerosol radiative effect may be another important factor in haze formation. To better understand the effect of this interaction, the aero- sol radiative effect on a severe haze episode that took place in December 2013 was investigated by using two WRF- Chem model simulations with different aerosol configurations. The results showed that the maximal reduction of re- gional average surface shortwave radiation, latent heat, and sensible heat during this event were 88, 12, and 37 W m2, respectively. The planetary boundary layer height, daytime temperature, and wind speed dropped by 276 m, I^C, and 0.33 m s-l, respectively. The ventilation coefficient dropped by 8%-24% for in the central and northwestern Yangtze River Delta （YRD）. The upper level of the atmosphere was warmed and the lower level was cooled, which stabilized the stratification. In a word, the dispersion ability of the atmosphere was weakened due to the aerosol radi- ative feedback. Additional results showed that the PM2.5 concentration in the central and northwestern YRD in- creased by 6-18 p.g m3, which is less than 15% of the average PM2.5 concentration during the severely polluted peri- od in this area. The vertical profile showed that the PM2.5 and PM10 concentrations increased below 950 hPa, with a maximum increase of 7 and 8 gg m-3, respectively. Concentrations reduced between 950 and 800 hPa, however, with a maximum reduction of 3.5 and 4.5 p.g rn-3, respectively. Generally, the aerosol radiative effect aggravated the level of pollution, but the effect was limited, and this haze event was mainly caused by the stagnant meteorological condi- tions. The interaction between the boundary layer and the aerosol radiative effect may have been less important than the large-scale static weather conditions for the formation of this haze episode.展开更多
Based on the CALIPSO （Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation） Version 4.10 products released on 8 November 2016, the Level 2 （L2） aerosol product over the Tibetan Plateau （TP） is evalu...Based on the CALIPSO （Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation） Version 4.10 products released on 8 November 2016, the Level 2 （L2） aerosol product over the Tibetan Plateau （TP） is evaluated and the aerosol radiative effect is also estimated in this study. As there are still some missing aerosol data points in the day-time CALIPSO Version 4.10 L2 product, this study re-calculated the aerosol extinction coefficient to explore the aer-osol radiative effect over the TP based on the CALIPSO Level 1 （L1） and CloudSat 2B-CLDCLASS-LIDAR products. The energy budget estimation obtained by using the AODs （aerosol optical depths） from calculated aerosol extinction coefficient as an input to a radiative transfer model shows better agreement with the Earth＇s Radiant En- ergy System （CERES） and CloudSat 2B-FLXHR-LIDAR observations than that with the input of AODs from aero- sol extinction coefficient from CALIPSO Version 4.10 L2 product. The radiative effect and heating rate of aerosols over the TP are further simulated by using the calculated aerosol extinction coefficient. The dust aerosols may heat the atmosphere by retaining the energy in the layer. The instantaneous heating rate can be as high as 5.5 K day^-1 de-pending on the density of the dust layers. Overall, the dust aerosols significantly affect the radiative energy budget and thermodynamic structure of the air over the TP, mainly by altering the shortwave radiation budget. The signific-ant influence of dust aerosols over the TP on the radiation budget may have important implications for investigating the atmospheric circulation and future regional and global climate.展开更多
The South China Sea summer monsoon(SCSSM)onset is characterized by rapid thermodynamical changes in the atmosphere that are critical to regional weather and climate processes.So far,few studies have focused on the cha...The South China Sea summer monsoon(SCSSM)onset is characterized by rapid thermodynamical changes in the atmosphere that are critical to regional weather and climate processes.So far,few studies have focused on the changes in the associated cloud and radiative features.This study investigates spatiotemporal characteristics of topof-atmosphere(TOA)cloud radiative effects(CREs)before and after the SCSSM onset over the South China Sea(SCS)and South China(SC),based on the 2001–2016 Clouds and the Earth’s Radiant Energy System(CERES)Energy Balanced and Filled(EBAF)satellite data and ERA-Interim reanalysis data.Before the SCSSM onset,strong net CRE(NCRE)dominated by its cooling shortwave component occurs over SC,while descending motion and weak NCRE prevail over the SCS.In the SCSSM onset pentad,convection,high clouds,and longwave and shortwave CREs(LWCRE and SWCRE)abruptly increase over the southern and central SCS,and their high-value centers subsequently move northeastward and are strongly affected by the western Pacific subtropical high.The strong offset between LWCRE and SWCRE enables the NCRE intensity(TOA radiation budget)to be quite small(large)between the SCS and the western North Pacific after the SCSSM onset.In contrast,low–middle-level clouds and strong cooling SWCRE remain over SC after the SCSSM onset,but the increasing high clouds and LWCRE weaken(intensify)the regional NCRE(TOA radiation budget)intensity.These marked latitudinal differences in CREs between the SCS and SC primarily arise from their respective dominant cloud types and circulation conditions,which manifest the differences between the tropical SCSSM and subtropical East Asian monsoon processes.The results indicate that regional cloud fractions and CREs before and after the SCSSM onset are strongly modulated by quickly changed largescale circulation over the East Asian monsoon regions,and the spatiotemporal variation of CREs is a response to the monsoonal circulation adjustment to a large extent.展开更多
Atmospheric aerosols influence the earth＇s radiative balance directly through scattering and absorbing solar radiation,and indirectly through affecting cloud properties.An understanding of aerosol optical properties ...Atmospheric aerosols influence the earth＇s radiative balance directly through scattering and absorbing solar radiation,and indirectly through affecting cloud properties.An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate.Although many such studies have been undertaken,large uncertainties in describing aerosol optical characteristics remain,especially regarding the absorption properties of different aerosols.Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance,and they include direct,indirect（albedo effect and cloud lifetime effect）,and semi-direct effects.The total direct effect of anthropogenic aerosols is negative（cooling）,although some components may contribute a positive effect（warming）.Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover,respectively.Absorbing aerosols,such as carbonaceous aerosols and dust,exert a positive forcing at the top of atmosphere and a negative forcing at the surface,and they can directly warm the atmosphere.Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do.The semidirect effect of absorbing aerosols could amplify this warming effect.Based on observational（ground- and satellite-based） and simulation studies,this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.展开更多
Cloud–radiation processes play an important role in regional energy budgets and surface temperature changes over arid regions. Cloud radiative effects（CREs） are used to quantitatively measure the aforementioned cli...Cloud–radiation processes play an important role in regional energy budgets and surface temperature changes over arid regions. Cloud radiative effects（CREs） are used to quantitatively measure the aforementioned climatic role. This study investigates the characteristics of CREs and their temporal variations over three arid regions in central Asia（CA）, East Asia（EA）, and North America（NA）, based on recent satellite datasets. Our results show that the annual mean shortwave（SW） and net CREs（SWCRE and NCRE） over the three arid regions are weaker than those in the same latitudinal zone of the Northern Hemisphere. In most cold months（November–March）, the longwave（LW）CRE is stronger than the SWCRE over the three arid regions, leading to a positive NCRE and radiative warming in the regional atmosphere–land surface system. The cold-season mean NCRE at the top of the atmosphere（TOA） averaged over EA is 4.1 W m^-2, with a positive NCRE from November to March, and the intensity and duration of the positive NCRE is larger than that over CA and NA. The CREs over the arid regions of EA exhibit remarkable annual cycles due to the influence of the monsoon in the south. The TOA LWCRE over arid regions is closely related to the high-cloud fraction, and the SWCRE relates well to the total cloud fraction. In addition, the relationship between the SWCRE and the low-cloud fraction is good over NA because of the considerable occurrence of low cloud. Further results show that the interannual variation of TOA CREs is small over the arid regions of CA and EA, but their surface LWCREs show certain decreasing trends that correspond well to their decreasing total cloud fraction. It is suggested that combined studies of more observational cloud properties and meteorological elements are needed for indepth understanding of cloud–radiation processes over arid regions of the Northern Hemisphere.展开更多
Cloud radiative and microphysical effects on the relation between spatial mean rain rate, rain intensity and fractional rainfall coverage are investigated in this study by conducting and analyzing a series of two-dime...Cloud radiative and microphysical effects on the relation between spatial mean rain rate, rain intensity and fractional rainfall coverage are investigated in this study by conducting and analyzing a series of two-dimensional cloud resolving model sensitivity experiments of pre-summer torrential rainfall in June 2008. The analysis of time-mean data shows that the exclusion of radiative effects of liquid clouds reduces domain mean rain rate by decreasing convective rain rate mainly through the reduced convective-rainfall area associated with the strengthened hydrometeor gain in the presence of radiative effects of ice clouds, whereas it increases domain mean rain rate by enhancing convective rain rate mainly via the intensified convective rain intensity associated with the enhanced net condensation in the absence of radiative effects of ice clouds. The removal of radiative effects of ice clouds decreases domain mean rain rate by reducing stratiform rain rate through the suppressed stratiform rain intensity related to the suppressed net condensation in the presence of radiative effects of liquid clouds, whereas it increases domain mean rain rate by strengthening convective rain rate mainly via the enhanced convective rain intensity in response to the enhanced net condensation in the absence of radiative effects of liquid clouds. The elimination of microphysical effects of ice clouds suppresses domain mean rain rate by reducing stratiform rain rate through the reduced stratiform-rainfall area associated with severely reduced hydrometeor loss.展开更多
On the basis of the emission data of the industrial sulphur dioxide (SO_2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol(SO_4~2-) with seasonal variation in the troposph...On the basis of the emission data of the industrial sulphur dioxide (SO_2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol(SO_4~2-) with seasonal variation in the troposphere is simulated and analyzed by a regional sulfur transport model, and the direct radiative effects of SO_4~2- under different weather conditions are also calculated using the discrete ordinate method. The results show that the concentration of SO_4~2- has significant seasonal and spatial variations resulting from the effects of SO_2 emission source and precipitation and wind fields. Both the concentration of SO_2 and its radiative forcing have the largest values in October and the lowest in July. SO_4~2- causes the decrease of the radiation flux absorbed by earth-atmosphere and the cooling of air temperature by scattering more solar radiation back into space. Besides, the radiative and climatic effects of SO_4~2- are related to the types and height and optical thickness, etc., of the clouds.展开更多
Northwest China is recognized as a main source and a major transport channel of dust aerosols in East Asia.With a fragile ecological environment,this region is quite sensitive to global climate change.Based on the sat...Northwest China is recognized as a main source and a major transport channel of dust aerosols in East Asia.With a fragile ecological environment,this region is quite sensitive to global climate change.Based on the satellite-derived aerosol three-dimensional distribution,the direct radiative effects of dust aerosols over Northwest China are evaluated.Aerosols over Northwest China are mainly distributed in the Tarim Basin,Junggar Basin,Gobi Desert,and Loess Plateau.The aerosol extinction coefficients are greater than 0.36 km-1 over the Tarim Basin and 0.16 km^(-1) over the Gobi Desert and Loess Plateau,decreasing with height.Aerosols over Northwest China are mainly composed of pure dust and polluted dust.These dust aerosols can modify the horizontal temperature gradient,vertical thermodynamic structure,and diurnal temperature range by absorbing and scattering shortwave radiation and emitting longwave radiation.For the column atmosphere,the radiative effect of dust aerosols shows heating effect of approximately 0.3 K day^(-1) during the daytime and cooling effect of approximately-0.4 K day^(-1) at night.In the vertical direction,dust aerosols can heat up the lower atmosphere(0.5–1.5 K day^(-1))and cool down the upper atmosphere(about-1.0 K day^(-1))during the daytime,while they cool down the lower atmosphere(-3 to-1.5 K day^(-1))and heat up the upper atmosphere(1–1.5 K day^(-1))at night.There are also significant lateral and vertical variations in the dust radiative effects corresponding to their spatial distributions.This study provides some scientific basis for reducing uncertainty in the investigation of aerosol radiative effects and provides observation evidence for simulation studies.展开更多
Fluids engineering is extremely important in a wide variety of materials processing systems,such as soldering,welding,extrusion of plastics and other polymeric materials,Chemical Vapor Deposition(CVD),composite materi...Fluids engineering is extremely important in a wide variety of materials processing systems,such as soldering,welding,extrusion of plastics and other polymeric materials,Chemical Vapor Deposition(CVD),composite materials manufacturing.In particular,mixed convection due to moving surfaces is very important in these applications.Mixed convection in a channel,as a result of buoyancy and motion of one of its walls has received little research attention and few guidelines are available for choosing the best performing channel configuration,particularly when radiative effects are significant.In this study a numerical investigation of the effect of radiation on mixed convection in air due to the interaction between a buoyancy flow and an unheated moving plate induced flow in a uniformly heated convergent vertical channel is carried out.The moving plate has a constant velocity and moves in the buoyancy force direction.The principal walls of the channel are heated at uniform heat flux.The numerical analysis is accomplished by means of the commercial code Fluent.The effects of the wall emissivity,the minimum channel spacing,the converging angle and the moving plate velocity are investigated and results in terms of air velocity and temperature fields inside the channel and wall temperature profiles,both of the moving and the heated plates,are given.Nusselt numbers,both accounting and not for the radiative contribution to heat removal,are also presented.展开更多
The impact of haze radiative effect on summertime 24-h convective precipitation over North China was investigated using WRF model （version 3.3） through model sensitivity studies between scenarios with and without ae...The impact of haze radiative effect on summertime 24-h convective precipitation over North China was investigated using WRF model （version 3.3） through model sensitivity studies between scenarios with and without aerosol radiative effects. The haze radiative effect was represented by incorporating an idealized aerosol optical profile, with AOD values around 1, derived from the aircraft measurement into the WRF shortwave scheme. We found that the shortwave heating induced by aerosol radiative effects would significantly reduce heavy rainfalls, although its effect on the post-frontal localized thunderstorm precipitation was more diverse. To capture the key factors that determine whether precipitation is enhanced or suppressed, model grids with 24-h precipitation difference between the ：two scenarios exceeding certain threshold （〉30 mm or〈 -30 mm） were separated into two sets. Analyses of key meteorological variables between the enhanced and suppressed regimes suggested that atmospheric convection was the most important factor that determined whether precipitation was enhanced or suppressed during summertime over North China. The convection was stronger over places with precipitation enhancement over 30 mm. Haze weakened the convection over places with precipitation suppression exceeding 30 mm and caused less water vapor to rise to a higher level and thus further suppressed precipitation. The suppression of precipitation was often accompanied with relatively high convective available potential energy （CAPE）, relative humidity （RH） and updraft velocities.展开更多
基金This research was sponsored by the National Key Program for Developing Basic Sciences of China(No.G1999043400)the National Natural Science Foundation of China(Grant Nos.40205016 and 40165001).
文摘As part of the development work of the Chinese new regional climate model (RIEMS), the radiative process of black carbon (BC) aerosols has been introduced into the original radiative procedures of RIEMS, and the transport model of BC aerosols has also been established and combined with the RIEMS model. Using the new model system, the distribution of black carbon aerosols and their radiative effect over the China region are investigated. The influences of BC aerosole on the atmospheric radiative transfer and on the air temperature, land surface temperature, and total rainfall are analyzed. It is found that BC aerosols induce a positive radiative forcing at the top of the atmosphere (TOA), which is dominated by shortwave radiative forcing. The maximum radiative forcing occurs in North China in July and in South China in April. At the same time, negative radiative forcing is observed on the surface. Based on the radiative forcing comparison between clear sky and cloudy sky, it is found that cloud can enforce the TOA positive radiative forcing and decrease the negative surface radiative forcing. The responses of the climate system in July to the radiative forcing due to BC aerosols are the decrease in the air temperature in the middle and lower reaches of the Changjiang River and Huaihe area and most areas of South China, and the weak increase or decrease in air temperature over North China. The total rainfall in the middle and lower reaches of the Changjiang River area is increased, but it decreased in North China in July.
基金supported by the National Natural Science Foundation of China (Grant No. 41475039)the National Key Basic Research and Development Project of China (Grant No. 2015CB953601)
文摘Cloud microphysical and rainfall responses to radiative processes are examined through analysis of cloud-resolving model sensitivity experiments of Typhoon Fitow（2013） during landfall.The budget analysis shows that the increase in the mean rainfall caused by the exclusion of radiative effects of water clouds corresponds to the decrease in accretion of raindrops by cloud ice in the presence of radiative effects of ice clouds,but the rainfall is insensitive to radiative effects of water clouds in the absence of radiative effects of ice clouds.The increases in the mean rainfall resulting from the removal of radiative effects of ice clouds correspond to the enhanced net condensation.The increases（decreases） in maximum rainfall caused by the exclusion of radiative effects of water clouds in the presence（absence） of radiative effects of ice clouds,or the removal of radiative effects of ice clouds in the presence（absence） of radiative effects of water clouds,correspond mainly to the enhancements（reductions） in net condensation.The mean rain rate is a product of rain intensity and fractional rainfall coverage.The radiation-induced difference in the mean rain rate is related to the difference in rain intensity.The radiation-induced difference in the maximum rain rate is associated with the difference in the fractional coverage of maximum rainfall.
基金financially supported by the Key Research and Development Program of Shaanxi Province(2018-ZDXM3-01)the Strategic Priority Research Program of Chinese Academy of Sciences(XDB40000000)+3 种基金the Sino-Swiss Cooperation on Air Pollution for Better Air(7F-09802.01.02)the Youth Innovation Promotion Association of the Chinese Academy of Sciences(2019402)the Sino-Swiss Science and Technology Cooperation(SSSTC)project HAZECHINA(IZLCZ2_169986)the SDC Clean-Air-China Program(7F-09802.01.03)。
文摘Intensive measurements were conducted in Xi’an,China before and during a COVID-19 lockdown period to investigate how changes in anthropogenic emissions affected the optical properties and radiative effects of brown carbon(BrC)aerosol.The contribution of BrC to total aerosol light absorption during the lockdown(13%-49%)was higher compared with the normal period(4%-29%).Mass absorption cross-sections(MACs)of specific organic aerosol(OA)factors were calculated from a ridge regression model.Of the primary OA(POA),coal combustion OA(CCOA)had the largest MACs at all tested wave-lengths during both periods due to high molecular-weight BrC chromophores;that was followed by biomass burning OA(BBOA)and hydrocarbon-like OA(HOA).For secondary OA(SOA),the MACs of the lessoxidized oxygenated OA(OOA)species(LO-OOA)atλ=370-590 nm were higher than those of more-oxidized OOA(MO-OOA)during both periods,presumably due to chromophore bleaching.The largest contributor to BrC absorption at the short wavelengths was CCOA during both periods,but BrC absorption by LO-OOA and MO-OOA became dominant at longer wavelengths during the lockdown.The estimated radiation forcing efficiency of BrC over 370-600 nm increased from 37.5 W·gduring the normal period to 50.2 W·gduring the lockdown,and that enhancement was mainly caused by higher MACs for both LO-OOA and MO-OOA.This study provides insights into the optical properties and radiative effects of source-specific BrC aerosol when pollution emissions are reduced.
基金supported by the National Basic Research Program of China(973 program,Grant 2010CB951901)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant XDA05100503)
文摘The authors examine the equilibrium climatic response to the direct radiative effect （DRE） of mineral dust and sea salt aerosols in a doubled-CO2 climate with two-way coupling of aerosol-climate interactions.In response to the drier and windier conditions,dust emissions increase by 26％ in the Sahara Desert and by 18％ on the global scale relative to present day.Sea salt emissions increase in high latitudes （＞60°） but decrease in middle latitudes （30°-60°） of both hemispheres due to the poleward shift of westerlies,leading to a 3％ decrease in global emissions.The burdens of dust and sea salt increase by 31％ and 7％ respectively,because reductions in rainfall over the tropical oceans increase the lifetime of particles in the warmer climate.The higher aerosol loading in the doubled-CO2 climate reinforces aerosol DRE by -0.2 W m-2,leading to an additional cooling of 0.1℃ at the surface compared with the climatic effects of aerosols in present day.The additional cooling from changes in natural aerosols compensates for up to 15％ of the regional warming induced by doubled CO2.
基金supported jointly by the National Basic Research Program of China(Grant Nos.2012CB955303 and 2013CB955803)the Chinese Academy of Sciences Ocean Project(Grant No.XDA11010402)+1 种基金the National Natural Science Foundation of China(Grant Nos.41175059 and 41375087)the Key Laboratory of Meteorological Disaster of Ministry of Education(Nanjing University of Information Science and Technology)(Grant No.KLME1409)
文摘Cloud radiative effects （CREs） at the top of the atmosphere （TOA） in three reanalysis datasets （the Eur- opean Center for Medium-Range Weather Forecasts In- terim Reanalysis （ERA-Interim）, the Japanese 55-yr Re- analysis Project （JRA-55）, and the Modem-Era Retro- spective Analysis for Research and Applications （MERRA）） are evaluated using recent satellite-based observations. The reanalyses can basically capture the spatial pattern of the annual mean shortwave CRE, but the global mean longwave CRE in ERA-interim and JRA55 is weaker than observed, leading to overestimations of the net CRE. Moreover, distinct CRE biases of the reanalyses occur in the Intertropical Convergence Zone （ITCZ）, coastal Pa- cific and Atlantic regions, and East Asia. Quantitative examination further indicates that the spatial correlations of CREs and TOA upward radiation fluxes with corre- sponding observations in ERA-Interim are better than in the other two reanalyses. Although MERRA has certain abilities in producing the magnitudes of global mean CREs, its performance in terms of spatial correlations in winter and summer are worse than for the other two re- analyses. The ability of JRA55 in reflecting CREs lies between the other two datasets. Compared to the global mean results, the spatial correlations of shortwave CRE in East Asia decrease and the biases of regional mean CREs increase in the three reanalyses. This implies that, cur- rently, it is still difficult to reproduce East Asian CREs based on these reanalyses. Relatively, ERA-Interim de- scribes the seasonal variation of East Asian CREs well, albeit weaker than observed. The present study also sug- gests that in-depth exploration of the ability of reanalysis data to describe aspects relating to cloud properties and rad- iation is needed usin~ more comprehensive observations.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences (Grant No.KZCX2-YW-Q11-03)the National Basic Research Program of China(Grant Nos.2010CB950900 and 2009CB421100)+1 种基金the National Natural Science Foundation of China(Grant No. 91025003)the R&D Special Fund for Public Welfare Industry (Meteorology)(Grant No.GYHY200906020)
文摘The Regional Integrated Environmental Model System （RIEMS 2.0） coupled with a chemistry-aerosol model and the Princeton Ocean Model （POM） is employed to simulate regional oceanic impact on atmospheric circulation and the direct radiative effect （DRE） of aerosol over East Asia. The aerosols considered in this study include both major anthropogenic aerosols （e.g., sulfate, black carbon, and organic carbon） and natural aerosols （e.g., soil dust and sea salt）. The RIEMS 2.0 is driven by NCEP/NCAR reanalysis II, and the simulated period is from 1 January to 31 December 2006. The results show the following： （1） The simulated annual mean sea-level pressure by RIEMS 2.0 with POM is lower than without POM over the mainland and higher without POM over the ocean. （2） In summer, the subtropical high simulated by RIEMS 2.0 with POM is stronger and extends further westward, and the continental low is stronger than without POM in summer. （3） The aerosol optical depth （AOD） simulated by RIEMS 2.0 with POM is larger in the middle and lower reaches of the Yangtze River than without POM. （4） The direct radiative effect with POM is stronger than that without POM in the middle and lower reaches of the Yangtze River and parts of southern China. Therefore, the authors should take account of the impact of the regional ocean model on studying the direct climate effect ＆aerosols in long term simulation.
基金National Key Basic Research and Development Planning Program of China(Program 973)(2014CB441203)Special Research Program for Public Welfare Industries(GYHY201206011)
文摘In this paper,the RIEMS 2.0 model,source emission in 2006 and 2010 are used to simulate the distributions and radiative effects of different anthropogenic aerosols over China.The comparison between the results forced by source emissions in 2006 and 2010 also reveals the sensitivity of the radiative effects to source emission.The results are shown as follows:(1) Compared with those in 2006,the annual average surface concentration of sulfate in 2010 decreased over central and eastern China with a range of-5 to 0 μg/m^3;the decrease of annual average aerosol optical depth of sulfate over East China varied from 0.04 to 0.08;the annual average surface concentrations of BC,OC and nitrate increased over central and eastern China with maximums of 10.90,11.52 and 12.50μg/m^3,respectively;the annual aerosol optical depths of BC,OC and nitrate increased over some areas of East China with extremes of 0.006,0.007 and 0.008,respectively.(2)For the regional average results in 2010,the radiative forcings of sulfate,BC,OC,nitrate and their total net radiative forcing at the top of the atmosphere over central and eastern China were-0.64,0.29,-0.41,-0.33 and-1.1 W/m^2,respectively.Compared with those in 2006,the radiative forcings of BC and OC in 2010 were both enhanced,while that of sulfate and the net radiative forcing were both weakened over East China mostly.(3)The reduction of the cooling effect of sulfate in 2010 produced a warmer surface air temperature over central and eastern China;the maximum value was 0.25 K.The cooling effect of nitrate was also slightly weakened.The warming effect of BC was enhanced over most of the areas in China,while the cooling effect of OC was enhanced over the similar area,particularly the area between Yangtze and Huanghe Rivers.The net radiative effect of the four anthropogenic aerosols generated the annual average reduction and the maximum reduction were-0.096 and-0.285 K,respectively,for the surface temperature in 2006,while in 2010 they were-0.063 and-0.256 K,respectively.In summary,the change in source emission lowered the cooling effect of anthropogenic aerosols,mainly because of the enhanced warming effect of BC and weakened cooling effect of scattering aerosols.
基金supported by the National Natural Science Funds of China(Grant Nos.41875133,91937302)the Strategic Priority Research Program of the Chinese Academy of Sciences(Grant No.XDA2006010302)+2 种基金the Second Tibetan Plateau Scientific Expedition and Research Program(STEP,Grant No.2019QZKK0206)the Youth Innovation Promotion Association CAS(2020078)the International Partnership Program of Chinese Academy of Sciences(Grant No.134111KYSB20200006).
文摘Current global climate models cannot resolve the complex topography over the Tibetan Plateau(TP)due to their coarse resolution.This study investigates the impacts of horizontal resolution on simulating aerosol and its direct radiative effect(DRE)over the TP by applying two horizontal resolutions of about 100 km and 25 km to the Chinese Academy of Sciences Flexible Global Ocean-Atmosphere Land System(CAS FGOALS-f3)over a 10-year period.Compared to the AErosol RObotic NETwork observations,a high-resolution model(HRM)can better reproduce the spatial distribution and seasonal cycles of aerosol optical depth(AOD)compared to a low-resolution model(LRM).The HRM bias and RMSE of AOD decreased by 0.08 and 0.12,and the correlation coefficient increased by 0.22 compared to the LRM.An LRM is not sufficient to reproduce the aerosol variations associated with fine-scale topographic forcing,such as in the eastern marginal region of the TP.The difference between hydrophilic aerosols in an HRM and LRM is caused by the divergence of the simulated relative humidity(RH).More reasonable distributions and variations of RH are conducive to simulating hydrophilic aerosols.An increase of the 10-m wind speed in winter by an HRM leads to increased dust emissions.The simulated aerosol DREs at the top of the atmosphere(TOA)and at the surface by the HRM are–0.76 W m^(–2)and–8.72 W m^(–2)over the TP,respectively.Both resolution models can capture the key feature that dust TOA DRE transitions from positive in spring to negative in the other seasons.
基金supported by the Knowledge Innovation Program of the Chinese Academy of Sciences(KZCX2-YW-Q11-04)the "Strategic Priority Research Program" of the Chinese Academy of Sciences (XDA05100502)
文摘To assess individual direct radiative effects of diverse aerosol species on a regional scale, the air quality modeling system RAMS-CMAQ （Regional Atmospheric Modeling System and Community Multiscale Air Quality） coupled with an aerosol optical properties/radiative transfer module was used to simulate the temporal and spatial distributions of their optical and radiative properties over East Asia throughout 2005. Annual and seasonal averaged aerosol direct radiative forcing （ADRF） of all important aerosols and individual components, such as sulfate, nitrate, ammonium, black carbon （BC）, organic carbon （OC）, and dust at top-of-atmosphere （TOA） in clear sky are analyzed. Analysis of the model results shows that the annual average ADRF of all important aerosols was in the range of 0 to -18 W m-z, with the maximum values mainly distributed over the Sichuan Basin. The direct radiative effects of sulfate, nitrate, and ammonium make up most of the total ADRF in East Asia, being concentrated mainly over North and Southeast China. The model domain is also divided into seven regions based on different administrative regions or countries to investigate detailed information about regional ADRF variations over East Asia. The model results show that the ADRFs of sulfate, ammonium, BC, and OC were stronger in summer and weaker in winter over most regions of East Asia, except over Southeast Asia. The seasonal variation in the ADRF of nitrate exhibited the opposite trend. A strong ADRF of dust mainly appeared in spring over Northwest China and Mongolia.
基金the NOAA Atmospheric Science for Renewable Energy (ASRE) programthe Earth Venture Continuity 1 (EVC-1) Libera project under NASA Contract 80LARC20D0006the NOAA cooperative agreement with CIRES,NA22OAR4320151。
文摘The study of shortwave(SW) radiation and its interactions with our planet has proven critical for advancing the understanding of the Earth–atmosphere system. Here, the author shares an accessible and high-level perspective on recent progress, surprises encountered, and promising future research directionsa. A brief context for the study of SW radiation is provided, after which three specific aspects are focused upon that the author considers particularly important. First, the significance of three-dimensional(3D) SW radiative effects is highlighted via impacts on surface downward SW radiation in complex cloud fields. Crucially, it is shown that probability distributions of surface radiation can only be reliably simulated when accounting for 3D effects, which has implications for various applications and next-generation atmospheric modeling. Second, the significance of the often overlooked diurnal cycle in global top-of-atmosphere upward SW radiation is underscored by quantifying the controlling properties and processes. Opportunities for improved future satellite observations of the global diurnal cycle are noted. Third, the wealth of information provided by the spectral dimension of SW radiation is demonstrated through the extraction and attribution of SW spectral signatures. It is argued that further exploration of the spectral dimension, aided by the recently launched and upcoming suite of spectrally resolved SW satellite observations, promises a new era of SW radiation research.
基金Supported by the National Key Research and Development(973)Program(2014CB441203)National Natural Science Foundation of China(41575141 and 41305006)Collaborative Innovation Center of Climate Change in Jiangsu Province
文摘Due to increased aerosol emissions and unfavorable weather conditions, severe haze events have occurred fre- quently in China in the last 10 years. In addition, the interaction between the boundary layer and the aerosol radiative effect may be another important factor in haze formation. To better understand the effect of this interaction, the aero- sol radiative effect on a severe haze episode that took place in December 2013 was investigated by using two WRF- Chem model simulations with different aerosol configurations. The results showed that the maximal reduction of re- gional average surface shortwave radiation, latent heat, and sensible heat during this event were 88, 12, and 37 W m2, respectively. The planetary boundary layer height, daytime temperature, and wind speed dropped by 276 m, I^C, and 0.33 m s-l, respectively. The ventilation coefficient dropped by 8%-24% for in the central and northwestern Yangtze River Delta （YRD）. The upper level of the atmosphere was warmed and the lower level was cooled, which stabilized the stratification. In a word, the dispersion ability of the atmosphere was weakened due to the aerosol radi- ative feedback. Additional results showed that the PM2.5 concentration in the central and northwestern YRD in- creased by 6-18 p.g m3, which is less than 15% of the average PM2.5 concentration during the severely polluted peri- od in this area. The vertical profile showed that the PM2.5 and PM10 concentrations increased below 950 hPa, with a maximum increase of 7 and 8 gg m-3, respectively. Concentrations reduced between 950 and 800 hPa, however, with a maximum reduction of 3.5 and 4.5 p.g rn-3, respectively. Generally, the aerosol radiative effect aggravated the level of pollution, but the effect was limited, and this haze event was mainly caused by the stagnant meteorological condi- tions. The interaction between the boundary layer and the aerosol radiative effect may have been less important than the large-scale static weather conditions for the formation of this haze episode.
基金Supported by the Strategic Priority Research Program of Chinese Academy of Sciences(XDA2006010301)National Natural Science Foundation of China(91737101,41475095,and 41405010)+1 种基金Fundamental Research Funds for Central Universities(lzujbky-2017-63)China 111 Project(B13045)
文摘Based on the CALIPSO （Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation） Version 4.10 products released on 8 November 2016, the Level 2 （L2） aerosol product over the Tibetan Plateau （TP） is evaluated and the aerosol radiative effect is also estimated in this study. As there are still some missing aerosol data points in the day-time CALIPSO Version 4.10 L2 product, this study re-calculated the aerosol extinction coefficient to explore the aer-osol radiative effect over the TP based on the CALIPSO Level 1 （L1） and CloudSat 2B-CLDCLASS-LIDAR products. The energy budget estimation obtained by using the AODs （aerosol optical depths） from calculated aerosol extinction coefficient as an input to a radiative transfer model shows better agreement with the Earth＇s Radiant En- ergy System （CERES） and CloudSat 2B-FLXHR-LIDAR observations than that with the input of AODs from aero- sol extinction coefficient from CALIPSO Version 4.10 L2 product. The radiative effect and heating rate of aerosols over the TP are further simulated by using the calculated aerosol extinction coefficient. The dust aerosols may heat the atmosphere by retaining the energy in the layer. The instantaneous heating rate can be as high as 5.5 K day^-1 de-pending on the density of the dust layers. Overall, the dust aerosols significantly affect the radiative energy budget and thermodynamic structure of the air over the TP, mainly by altering the shortwave radiation budget. The signific-ant influence of dust aerosols over the TP on the radiation budget may have important implications for investigating the atmospheric circulation and future regional and global climate.
基金Supported by the National Key Research and Development Program of China(2017YFA0603503 and 2017YFA0603804)National Natural Science Foundation of China(41831174,41975109,and 41730963)UK–China Research and Innovation Partnership Fund through the Met Office Climate Science for Service Partnership(CSSP)China as part of the Newton Fund。
文摘The South China Sea summer monsoon(SCSSM)onset is characterized by rapid thermodynamical changes in the atmosphere that are critical to regional weather and climate processes.So far,few studies have focused on the changes in the associated cloud and radiative features.This study investigates spatiotemporal characteristics of topof-atmosphere(TOA)cloud radiative effects(CREs)before and after the SCSSM onset over the South China Sea(SCS)and South China(SC),based on the 2001–2016 Clouds and the Earth’s Radiant Energy System(CERES)Energy Balanced and Filled(EBAF)satellite data and ERA-Interim reanalysis data.Before the SCSSM onset,strong net CRE(NCRE)dominated by its cooling shortwave component occurs over SC,while descending motion and weak NCRE prevail over the SCS.In the SCSSM onset pentad,convection,high clouds,and longwave and shortwave CREs(LWCRE and SWCRE)abruptly increase over the southern and central SCS,and their high-value centers subsequently move northeastward and are strongly affected by the western Pacific subtropical high.The strong offset between LWCRE and SWCRE enables the NCRE intensity(TOA radiation budget)to be quite small(large)between the SCS and the western North Pacific after the SCSSM onset.In contrast,low–middle-level clouds and strong cooling SWCRE remain over SC after the SCSSM onset,but the increasing high clouds and LWCRE weaken(intensify)the regional NCRE(TOA radiation budget)intensity.These marked latitudinal differences in CREs between the SCS and SC primarily arise from their respective dominant cloud types and circulation conditions,which manifest the differences between the tropical SCSSM and subtropical East Asian monsoon processes.The results indicate that regional cloud fractions and CREs before and after the SCSSM onset are strongly modulated by quickly changed largescale circulation over the East Asian monsoon regions,and the spatiotemporal variation of CREs is a response to the monsoonal circulation adjustment to a large extent.
基金Supported by the National Basic Research and Development (973) Program of China(2012CB955301)National Natural Science Foundation of China(41475095 and 41275006)+1 种基金China 111 Project(B13045)Fundamental Research Fund for Central Universities of China(lzujbky-2013-ct05 and lzujbky-2014-109)
文摘Atmospheric aerosols influence the earth＇s radiative balance directly through scattering and absorbing solar radiation,and indirectly through affecting cloud properties.An understanding of aerosol optical properties is fundamental to studies of aerosol effects on climate.Although many such studies have been undertaken,large uncertainties in describing aerosol optical characteristics remain,especially regarding the absorption properties of different aerosols.Aerosol radiative effects are considered as either positive or negative perturbations to the radiation balance,and they include direct,indirect（albedo effect and cloud lifetime effect）,and semi-direct effects.The total direct effect of anthropogenic aerosols is negative（cooling）,although some components may contribute a positive effect（warming）.Both the albedo effect and cloud lifetime effect cool the atmosphere by increasing cloud optical depth and cloud cover,respectively.Absorbing aerosols,such as carbonaceous aerosols and dust,exert a positive forcing at the top of atmosphere and a negative forcing at the surface,and they can directly warm the atmosphere.Internally mixed black carbon aerosols produce a stronger warming effect than externally mixed black carbon particles do.The semidirect effect of absorbing aerosols could amplify this warming effect.Based on observational（ground- and satellite-based） and simulation studies,this paper reviews current progress in research regarding the optical properties and radiative effects of aerosols and also discusses several important issues to be addressed in future studies.
基金National Basic Research Program of China(2012CB955303)National Natural Science Foundation of China(41430425,41375031,and 41505130)State Key Laboratory of Loess and Quaternary Geology,Institute of Earth Environment,Chinese Academy of Sciences(SKLLQG1407)
文摘Cloud–radiation processes play an important role in regional energy budgets and surface temperature changes over arid regions. Cloud radiative effects（CREs） are used to quantitatively measure the aforementioned climatic role. This study investigates the characteristics of CREs and their temporal variations over three arid regions in central Asia（CA）, East Asia（EA）, and North America（NA）, based on recent satellite datasets. Our results show that the annual mean shortwave（SW） and net CREs（SWCRE and NCRE） over the three arid regions are weaker than those in the same latitudinal zone of the Northern Hemisphere. In most cold months（November–March）, the longwave（LW）CRE is stronger than the SWCRE over the three arid regions, leading to a positive NCRE and radiative warming in the regional atmosphere–land surface system. The cold-season mean NCRE at the top of the atmosphere（TOA） averaged over EA is 4.1 W m^-2, with a positive NCRE from November to March, and the intensity and duration of the positive NCRE is larger than that over CA and NA. The CREs over the arid regions of EA exhibit remarkable annual cycles due to the influence of the monsoon in the south. The TOA LWCRE over arid regions is closely related to the high-cloud fraction, and the SWCRE relates well to the total cloud fraction. In addition, the relationship between the SWCRE and the low-cloud fraction is good over NA because of the considerable occurrence of low cloud. Further results show that the interannual variation of TOA CREs is small over the arid regions of CA and EA, but their surface LWCREs show certain decreasing trends that correspond well to their decreasing total cloud fraction. It is suggested that combined studies of more observational cloud properties and meteorological elements are needed for indepth understanding of cloud–radiation processes over arid regions of the Northern Hemisphere.
基金National Natural Science Foundation of China(41475039,41775040)National Key Basic Research and Development Project of China(2015CB953601)
文摘Cloud radiative and microphysical effects on the relation between spatial mean rain rate, rain intensity and fractional rainfall coverage are investigated in this study by conducting and analyzing a series of two-dimensional cloud resolving model sensitivity experiments of pre-summer torrential rainfall in June 2008. The analysis of time-mean data shows that the exclusion of radiative effects of liquid clouds reduces domain mean rain rate by decreasing convective rain rate mainly through the reduced convective-rainfall area associated with the strengthened hydrometeor gain in the presence of radiative effects of ice clouds, whereas it increases domain mean rain rate by enhancing convective rain rate mainly via the intensified convective rain intensity associated with the enhanced net condensation in the absence of radiative effects of ice clouds. The removal of radiative effects of ice clouds decreases domain mean rain rate by reducing stratiform rain rate through the suppressed stratiform rain intensity related to the suppressed net condensation in the presence of radiative effects of liquid clouds, whereas it increases domain mean rain rate by strengthening convective rain rate mainly via the enhanced convective rain intensity in response to the enhanced net condensation in the absence of radiative effects of liquid clouds. The elimination of microphysical effects of ice clouds suppresses domain mean rain rate by reducing stratiform rain rate through the reduced stratiform-rainfall area associated with severely reduced hydrometeor loss.
文摘On the basis of the emission data of the industrial sulphur dioxide (SO_2) and observed climate fields over East Asia, the distribution of anthropogenic sulfate aerosol(SO_4~2-) with seasonal variation in the troposphere is simulated and analyzed by a regional sulfur transport model, and the direct radiative effects of SO_4~2- under different weather conditions are also calculated using the discrete ordinate method. The results show that the concentration of SO_4~2- has significant seasonal and spatial variations resulting from the effects of SO_2 emission source and precipitation and wind fields. Both the concentration of SO_2 and its radiative forcing have the largest values in October and the lowest in July. SO_4~2- causes the decrease of the radiation flux absorbed by earth-atmosphere and the cooling of air temperature by scattering more solar radiation back into space. Besides, the radiative and climatic effects of SO_4~2- are related to the types and height and optical thickness, etc., of the clouds.
基金Supported by the Gansu Provincial Special Fund for Scientific and Technological Innovation and Development(2019ZX-06)Fundamental Research Funds for the Central Universities(lzujbky-2020-kb31)Meteorological Science and Technology Research Project of Shandong Meteorological Bureau(2019sdqxm14)。
文摘Northwest China is recognized as a main source and a major transport channel of dust aerosols in East Asia.With a fragile ecological environment,this region is quite sensitive to global climate change.Based on the satellite-derived aerosol three-dimensional distribution,the direct radiative effects of dust aerosols over Northwest China are evaluated.Aerosols over Northwest China are mainly distributed in the Tarim Basin,Junggar Basin,Gobi Desert,and Loess Plateau.The aerosol extinction coefficients are greater than 0.36 km-1 over the Tarim Basin and 0.16 km^(-1) over the Gobi Desert and Loess Plateau,decreasing with height.Aerosols over Northwest China are mainly composed of pure dust and polluted dust.These dust aerosols can modify the horizontal temperature gradient,vertical thermodynamic structure,and diurnal temperature range by absorbing and scattering shortwave radiation and emitting longwave radiation.For the column atmosphere,the radiative effect of dust aerosols shows heating effect of approximately 0.3 K day^(-1) during the daytime and cooling effect of approximately-0.4 K day^(-1) at night.In the vertical direction,dust aerosols can heat up the lower atmosphere(0.5–1.5 K day^(-1))and cool down the upper atmosphere(about-1.0 K day^(-1))during the daytime,while they cool down the lower atmosphere(-3 to-1.5 K day^(-1))and heat up the upper atmosphere(1–1.5 K day^(-1))at night.There are also significant lateral and vertical variations in the dust radiative effects corresponding to their spatial distributions.This study provides some scientific basis for reducing uncertainty in the investigation of aerosol radiative effects and provides observation evidence for simulation studies.
文摘Fluids engineering is extremely important in a wide variety of materials processing systems,such as soldering,welding,extrusion of plastics and other polymeric materials,Chemical Vapor Deposition(CVD),composite materials manufacturing.In particular,mixed convection due to moving surfaces is very important in these applications.Mixed convection in a channel,as a result of buoyancy and motion of one of its walls has received little research attention and few guidelines are available for choosing the best performing channel configuration,particularly when radiative effects are significant.In this study a numerical investigation of the effect of radiation on mixed convection in air due to the interaction between a buoyancy flow and an unheated moving plate induced flow in a uniformly heated convergent vertical channel is carried out.The moving plate has a constant velocity and moves in the buoyancy force direction.The principal walls of the channel are heated at uniform heat flux.The numerical analysis is accomplished by means of the commercial code Fluent.The effects of the wall emissivity,the minimum channel spacing,the converging angle and the moving plate velocity are investigated and results in terms of air velocity and temperature fields inside the channel and wall temperature profiles,both of the moving and the heated plates,are given.Nusselt numbers,both accounting and not for the radiative contribution to heat removal,are also presented.
文摘The impact of haze radiative effect on summertime 24-h convective precipitation over North China was investigated using WRF model （version 3.3） through model sensitivity studies between scenarios with and without aerosol radiative effects. The haze radiative effect was represented by incorporating an idealized aerosol optical profile, with AOD values around 1, derived from the aircraft measurement into the WRF shortwave scheme. We found that the shortwave heating induced by aerosol radiative effects would significantly reduce heavy rainfalls, although its effect on the post-frontal localized thunderstorm precipitation was more diverse. To capture the key factors that determine whether precipitation is enhanced or suppressed, model grids with 24-h precipitation difference between the ：two scenarios exceeding certain threshold （〉30 mm or〈 -30 mm） were separated into two sets. Analyses of key meteorological variables between the enhanced and suppressed regimes suggested that atmospheric convection was the most important factor that determined whether precipitation was enhanced or suppressed during summertime over North China. The convection was stronger over places with precipitation enhancement over 30 mm. Haze weakened the convection over places with precipitation suppression exceeding 30 mm and caused less water vapor to rise to a higher level and thus further suppressed precipitation. The suppression of precipitation was often accompanied with relatively high convective available potential energy （CAPE）, relative humidity （RH） and updraft velocities.
