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Release characteristics of arsenic from sediments and its source or sink competition with phosphorus:A case of a great lake with grass-algae alternation
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作者 Shuhang Wang Yongsheng Chang +2 位作者 Wei Huang Dianhai Yang Feifei Che 《Journal of Environmental Sciences》 2025年第3期278-287,共10页
The arsenic(As)release from sediments in great lakes is affected by various factors.In this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sed... The arsenic(As)release from sediments in great lakes is affected by various factors.In this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sediments from different areas(grass-type,algae-type,and grass-algae alternation areas)in great shallow lakes(Taihu Lake,China)were analyzed,and the influence of P competition in the process of As release was also studied.The results showed that changing trend of the values of equilibrium As concentration in sediments were consistent with the regional changes(0 to 28.12μg/L),and the sediments from algaetype areas had the higher values.The sediments from western lake and northwest lake bay were a strong As and a weak P source,and the north lake bay had the opposite trend of these two regions.Intense P source competition with As from the sediments occurred in algae-type areas.The grass-type areas had strong As and P retention capacities,indicating a sink role of sediment with high As and P sorption capacities.The degree of As and P saturation had similar trend in sediments,and the grass-type areas had the higher values,18.3%-21.4%and 15.31%-20.34%,respectively.Contribution analysis results showed that most of As release contribution was from the bottom(30-50 cm)sediments,and the surface(0-10 cm)sediments from algae-type areas contributed more to the overlying water than other region. 展开更多
关键词 ARSENIC PHOSPHORUS Sediment source and sink Contribution
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New alkylbenzene parameters to identify organic matter sources for source rocks of light oils and condensates from the Tarim Basin and Beibuwan Basin
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作者 Bing-Kun Meng Dao-Fu Song +1 位作者 Yuan Chen Sheng-Bao Shi 《Petroleum Science》 2025年第1期76-89,共14页
As an important component of light hydrocarbon compounds,alkylbenzene compounds lack indicators to indicate the source of organic matter of light oils and condensates.Forty-one oil samples from the Tarim Basin and Bei... As an important component of light hydrocarbon compounds,alkylbenzene compounds lack indicators to indicate the source of organic matter of light oils and condensates.Forty-one oil samples from the Tarim Basin and Beibuwan Basin were analyzed by comprehensive two-dimensional gas chromatography time-of-flight mass spectrometry(GC×GC-TOFMS).The concentration distributions of thirteen light hydrocarbon compounds with organic matter source and sedimentary environment indication were studied.There is no significant difference in the concentrations of 1-methylpropylbenzene(MPB)in all studied oils.However,the concentrations of 2-MPB in the Tarim swamp oils are higher than that in the Beibuwan lacustrine oils and Tarim marine oils.Based on the significant concentration difference of 1-and 2-MPB in all studied oils,1-/2-MPB(MPBr)was proposed as an indicator to identify the source of organic matter in crude oils.The MPBr values greater than 1.5 indicate that the crude oil mainly comes from lower aquatic organisms,bacteria,and algae.The MPBr values greater than 1.0 and less than 1.5 indicate that crude oil was derived from the combined contributions of lower aquatic organisms,bacteria and algae,and terrestrial higher plants.The MPBr values less than 1.0 suggest that the crude oil was mainly derived from terrigenous higher plants.The MPBr values in crude oils basically are not or slightly affected by depositional environment and secondary alteration.The MPBr values can be used to infer the organic matter origin in sediments,especially for the lack of biomarkers of light oils and condensates. 展开更多
关键词 2-Methylpropylbenzene GC×GC-TOFMS Organic matter source Light oils and condensates
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A Comparative Study of Williamson Hybrid Nanofluid Flow Consisting of Cu, GaN, and Al2O3 Nanoparticles in Ethylene Glycol over a Stretching Sheet with Suction/Injection and Heat Source/Sink
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作者 Mamidala Jyotshna Vadlakonda Dhanalaxmi 《Journal of Applied Mathematics and Physics》 2022年第12期3864-3897,共34页
Several new techniques in the field of heat transfer in fluids have opened new avenues for studying the heat transfer effects in nanofluids and thermodynamic flow parameters, leading to novel applications. There have ... Several new techniques in the field of heat transfer in fluids have opened new avenues for studying the heat transfer effects in nanofluids and thermodynamic flow parameters, leading to novel applications. There have been studies on nanofluids, including metal, ceramic and magnetic nanoparticles mixed with base fluids such as Water, Kerosene, and Ethylene glycol. However, research on fluids employing semiconductor nanoparticles as supplements to base fluids to generate nanofluids and hybrid nanofluids is limited. For the investigation, Gallium nitrite, a binary semiconductor with excellent heat convection, is together with Cu metal nanoparticles and Al<sub>2</sub>O<sub>3</sub> ceramic nanoparticles separately in the base fluid Ethylene glycol (EG) to form hybrid nanofluids. The effects of convective boundary conditions, thermal radiation, heat source/sink, suction/injection, and activation energy on three-dimensional Williamson MHD hybrid nanofluid flow of Cu + GaN + EG, Al<sub>2</sub>O<sub>3</sub> + GaN + EG, and Cu + Al<sub>2</sub>O<sub>3</sub> + EG are investigated on a stretched sheet with porosity. A similarity transformation is performed on the governing equations to transform them into dimensionless ordinary differential equations ODEs. Numerical analysis is carried out in MATLAB utilizing bvp5c and the shooting technique. The variations of velocity, temperature, and concentration profiles as a function of different physical effects are presented graphically with dimensionless parameters and explained the variations scientifically. As varied with different parameters, the values of the Skin-friction coefficient, Nusselt number, and Sherwood number are mentioned in the table. 展开更多
关键词 Williamson Hybrid Nanofluid Gallium Nitride Heat Transfer Heat source/sink Suction/Injection Solid Volume Fraction
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斯洛文尼亚岩溶区草地生长季土壤CO_(2)变化及其降雨效应 被引量:2
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作者 章程 肖琼 +6 位作者 汪进良 孙平安 苗迎 郭永丽 Mitja PRELOVSEK Martin KNEZ Saša MILANOVIĆ 《地球学报》 北大核心 2025年第2期397-408,共12页
土壤CO_(2)是岩溶作用的核心驱动因子,也是研究土壤呼吸及其与大气CO_(2)源汇关系的核心指标。快速的岩溶动力学和碳循环过程及其对生态系统的敏感性,暗示其在现今全球碳循环中仍在发挥积极作用。本文以斯洛文尼亚第纳尔岩溶区典型草地... 土壤CO_(2)是岩溶作用的核心驱动因子,也是研究土壤呼吸及其与大气CO_(2)源汇关系的核心指标。快速的岩溶动力学和碳循环过程及其对生态系统的敏感性,暗示其在现今全球碳循环中仍在发挥积极作用。本文以斯洛文尼亚第纳尔岩溶区典型草地土壤生态系统为例,开展不同深度土壤温度、水分和土壤CO_(2)含量等指标高分辨率在线监测。监测工作在2021年6—9月草地生长季进行,每10 min记录一组数据。结果表明,土下20 cm、30 cm和50 cm土温均值分别为19.69℃、18.54℃和17.42℃,暗示土温随深度增加逐渐变小。土下20 cm、30 cm和50 cm水分含量均值分别为23.2%、21.7%和24.9%。土壤水分变化主要受降雨控制,降雨强度越大,水分上升幅度越大。土下20 cm、30 cm和50 cm土壤CO_(2)变化范围分别为(1884~6705)×10^(–6)、(2088~5516)×10^(–6)、(2771~3606)×10^(–6),均值分别为3578×10^(–6)、3468×10^(–6)、3174×10^(–6)。无雨期间土壤水分显示出白天下降,夜晚基本保持不变的阶梯状下降趋势,受土壤水分控制,土壤CO_(2)多日总体变化呈现锯齿状持续降低趋势。不同降雨条件下均出现土壤CO_(2)向下迁移现象,从强降雨过程初期产生的土壤CO_(2)含量快速下降看,表明雨水入渗产生的脉冲效应导致CO_(2)快速向下迁移,进一步进入下伏岩溶含水层,可为碳酸盐岩溶蚀提供CO_(2)驱动力,比较下降幅度与雨前CO_(2)含量,暗示降雨过程中12%~33%的土壤CO_(2)进入岩溶含水层并参与碳酸盐岩溶蚀。监测结果暗示岩溶作用是陆地生态系统碳循环的横向延伸,具有土壤CO_(2)汇效应,也就是说,岩溶作用过程具有缓解土壤CO_(2)向大气释放功能,即减源效应。因此,在研究岩溶区碳循环及其碳汇效应时,应把植被-土壤-碳酸盐岩溶蚀作为一个整体,从岩溶关键带角度,系统开展监测与研究,以期获得岩溶区碳循环过程的完整认识,揭示其碳汇效应,进一步评估岩溶区碳循环在全球碳循环的作用和应对气候变化中的地位。 展开更多
关键词 土壤CO_(2) 土壤水分 降雨过程 岩溶作用 减源效应 斯洛文尼亚
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基于宽带光源和悬臂梁光声光谱大气CO_(2)检测
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作者 雒静 牟福生 王松 《淮北师范大学学报(自然科学版)》 2025年第2期19-23,共5页
为研究温室效应和全球变暖等环境问题,需要对温室气体检测方法进行探索和分析。构建基于宽带红外光源和悬臂梁型微音器光声光谱检测系统,利用该系统检测空气中重要大气温室气体之一CO_(2)浓度。为研究系统测量准确性和稳定性,结合不同... 为研究温室效应和全球变暖等环境问题,需要对温室气体检测方法进行探索和分析。构建基于宽带红外光源和悬臂梁型微音器光声光谱检测系统,利用该系统检测空气中重要大气温室气体之一CO_(2)浓度。为研究系统测量准确性和稳定性,结合不同体积分数CO_(2)样气(1.51×10^(-4),2.04×10^(-4),3.58×10^(-4),4.03×10^(-4),4.54×10^(-4),4.95×10^(-4))对系统进行测量和校准,分析不同校准情况的解决方案。利用构建系统与GASERA-ONE光声光谱仪对室外大气进行连续观测,测量结果表明两者具有较好一致性。研究表明,该系统能够实现CO_(2)浓度高精度连续测量,对大气环境监测具有重要意义。 展开更多
关键词 悬臂梁 CO_(2) 光声光谱 环境检测 红外光源
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Interannual Variability of Atmospheric Heat Source/ Sink over the Qinghai-Xizang (Tibetan) Plateau and its Relation to Circulation 被引量:27
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作者 赵平 陈隆勋 +1 位作者 Zhao Ping Chen Longxun 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2001年第1期106-116,共11页
Based on the 1961-1995 atmospheric apparent heat source/sink and the 1961-1990 snow-cover days and depth over the Qinghai-Xizang Plateau (QXP) and the 1961-1995 reanalysis data of NCEP/NCAR and the 1975-1994 OLR data,... Based on the 1961-1995 atmospheric apparent heat source/sink and the 1961-1990 snow-cover days and depth over the Qinghai-Xizang Plateau (QXP) and the 1961-1995 reanalysis data of NCEP/NCAR and the 1975-1994 OLR data, this paper discusses the interannual variability of the heat regime and its relation to atmospheric circulation It is shown that the interannual variability is pronounced, with maximal variability in spring and autumn, and the variability is heterogeneous horizontally. In the years with the weak (or strong) winter cold source, the deep trough over East Asia is to the east (or west) of its normal, which corresponds to strong (or weak) winter monsoon in East Asia. In the years with the strong (or weak) sum mer heat source, there exists an anomalous cyclone (or anticyclone) in the middle and lower troposphere over the QXP and ifs neighborhood and anomalous southwest (or northeast) winds over the Yangtze River valley of China, corresponding to strong (or weak) summer monsoon in East Asia. The summer heat source of the QXP is related to the intensity and position of the South Asia high. The QXP snow cover condition of April has a close relation to the heating intensity of summer. There is a remarkable negative correlation between the summer heat source of the QXP and the convection over the southeastern QXP, the Bay of Bengal, the Indo-China Peninsula, the southeastern Asia, the southwest part of China and the lower reaches of the Yangtze River and in the area from the Yellow Sea of China to the Sea of Japan. 展开更多
关键词 Qinghai-Xizang Plateau apparent heat source/sink snow cover OLR
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严寒地区CO_(2)热泵耦合供热系统改造方案设计及经济性分析
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作者 刘启明 褚赛 +1 位作者 许抗吾 牛笑晨 《制冷与空调(四川)》 2025年第3期406-412,共7页
以内蒙古自治区呼伦贝尔市鄂伦春自治旗内某镇集中供热热源厂为例,对热源厂现状燃煤锅炉供热系统服务规模、收费情况、设备配置、能源消耗、运行状态等进行分析,结合相关政策要求及项目特点,采用CO_(2)空气源热泵+燃煤锅炉耦合系统进行... 以内蒙古自治区呼伦贝尔市鄂伦春自治旗内某镇集中供热热源厂为例,对热源厂现状燃煤锅炉供热系统服务规模、收费情况、设备配置、能源消耗、运行状态等进行分析,结合相关政策要求及项目特点,采用CO_(2)空气源热泵+燃煤锅炉耦合系统进行供热系统替代改造,介绍了耦合系统原理及运行策略,在对CO_(2)空气源热泵机组制热运行特性分析的基础上,详细阐述了耦合系统的经济及环保效益。结果显示,改造后耦合系统采暖季运行费用总计3295.53万元,年均节费1568.45万元,节费率32.25%;CO_(2)排放量共计95234.02t,年均减排CO_(2)达56644.05t,减排率37.30%;静态投资回收期约8.3年,节能环保及经济性较好。 展开更多
关键词 严寒地区 供热改造 CO_(2)空气源热泵 性能系数 运行费用
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Assessing effects of “source-sink” landscape on non-point source pollution based on cell units of a small agricultural catchment 被引量:5
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作者 WANG Jin-liang CHEN Cheng-long +4 位作者 NI Jiu-pai XIE De-ti GUO Xi LUO Zhi-jun ZHAO Yue 《Journal of Mountain Science》 SCIE CSCD 2019年第9期2048-2062,共15页
Ascertaining the relationship between "source-sink" landscape and non-point source(NPS) pollution is crucial for reducing NPS pollution, however, it is not easy to realize this target on cell unit scale. To ... Ascertaining the relationship between "source-sink" landscape and non-point source(NPS) pollution is crucial for reducing NPS pollution, however, it is not easy to realize this target on cell unit scale. To reveal the relationships between "sourcesink" landscape and NPS pollution based on cell units of a small catchment in the Three Gorges Reservoir Region(TGRR), the runoff and nutrient yields were simulated first by rainfall events on a cell unit scale based on the Annualized AGricultural Non-Point Source Pollution Model(AnnAGNPS). Landscape structure and pattern were quantified with "sourcesink" landscape indicators based on cell units including landscape area indices and locationweighted landscape indices. The results showed that:the study case of small Wangjiagou catchment highlighted a good prediction capability of runoff and nutrient export by the AnnAGNPS model. Throughout the catchment, the spatial distribution trends of four location-weighted landscape indices were similar to the trends of simulated total nitrogen(TN) and total phosphorus(TP), which highlighted the importance of spatial arrangement of "source" and "sink" landscape types in a catchment when estimating pollutant loads. Results by Pearson correlation analysis indicated that the location-weighted landscape index provided a more comprehensive account of multiple factors, and can better reflect NPS-related nutrient loss than other landscape indices applied in single-factor analysis. This study provides new findings for applying the "source-sink" landscape indices based on cell units in small catchments to explain the effect of "source-sink" landscape on nutrient export based on cell unit, and helps improve the understanding of the correlation between "source-sink" landscape and NPS pollution. 展开更多
关键词 Nutrient load Non-point source pollution source sink LANDSCAPE index SMALL catchment
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Genetic bases of source-,sink-,and yield-related traits revealed by genome-wide association study in Xian rice 被引量:10
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作者 Yun Wang Yunlong Pang +4 位作者 Kai Chen Laiyuan Zhai Congcong Shen Shu Wang Jianlong Xu 《The Crop Journal》 SCIE CAS CSCD 2020年第1期119-131,共13页
The source-sink relationship determines the ultimate grain yield.We investigated the genetic basis of the relationship between source and sink and yield potential in rice.In two environments,we identified quantitative... The source-sink relationship determines the ultimate grain yield.We investigated the genetic basis of the relationship between source and sink and yield potential in rice.In two environments,we identified quantitative trait loci(QTL)associated with sink capacity(total spikelet number per panicle and thousand-grain weight),source leaf(flag leaf length,flag leaf width and flag leaf area),source-sink relationship(total spikelet number to flag leaf area ratio)and yield-related traits(filled grain number per panicle,panicle number per plant,grain yield per plant,biomass per plant,and harvest index)by genome-wide association analysis using 272 Xian(indica)accessions.The panel showed substantial variation for all traits in the two environments and revealed complex phenotypic correlations.A total of 70 QTL influencing the 11 traits were identified using 469,377 high-quality SNP markers.Five QTL were detected consistently in four chromosomal regions in both environments.Five QTL clusters simultaneously affected source,sink,source–sink relationship,and grain yield traits,probably explaining the genetic basis of significant correlations of grain yield with source and sink traits.We selected 24 candidate genes in the four consistent QTL regions by identifying linkage disequilibrium(LD)blocks associated with significant SNPs and performing haplotype analysis.The genes included one cloned gene(NOG1)and three newly identified QTL(qHI6,qTGW7,and qFLA8).These results provide a theoretical basis for high-yield rice breeding by increasing and balancing source–sink relationships using marker-assisted selection. 展开更多
关键词 RICE GWAS sourcesink relationship Quantitative trait loci/locus(QTL) Candidate gene
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Diagnostic Study of Apparent Heat Sources and Moisture Sinks in the South China Sea and its Adjacent Areas during the Onset of 1998 SCS Monsoon 被引量:7
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作者 王世玉 钱永甫 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2000年第2期285-298,共14页
The apparent heat sources (?Q1 ?) and moisture sinks (?Q2 ?) are calculated based on the reanalyzed data of the South China Sea Monsoon Experiment (SCSMEX) from May 1 to August 31, 1998. It is found that the formation... The apparent heat sources (?Q1 ?) and moisture sinks (?Q2 ?) are calculated based on the reanalyzed data of the South China Sea Monsoon Experiment (SCSMEX) from May 1 to August 31, 1998. It is found that the formation and distribution of the atmospheric heat sources are important for the monsoon onset. The earlier onset of the SCS monsoon is the result of enduring atmospheric heating in the Indo–China Peninsula and South China areas. The atmospheric heating firstly appears in the Indo–China Peninsula area and the sensible heat is the major one. The 30–50 day periodic oscillation of atmospheric heat sources between the SCS area and the western Pacific warm pool has a reverse phase distribution before the middle of July and the low frequency oscillation of heat sources in SCS area has an obvious longitudinal propagation. The 30–50 day low frequency oscillation has vital modificatory effects on the summer monsoon evolution during 1998. Key words Apparent heat sources - Apparent moisture sinks - The South China Sea monsoon - Diagnostic Study Sponsored by the National Key Project of Fundamental Research “ SCSMEX” and the Research Fund for the Doctoral Program of Higher Education: “ Study of the Air-sea Interaction in the SCS Monsoon Region”. 展开更多
关键词 Apparent heat sources Apparent moisture sinks The South China Sea monsoon Diagnostic Study
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Analysis of spatio-temporal features of a carbon source/sink and its relationship to climatic factors in the Inner Mongolia grassland ecosystem 被引量:7
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作者 戴尔阜 黄宇 +1 位作者 吴卓 赵东升 《Journal of Geographical Sciences》 SCIE CSCD 2016年第3期297-312,共16页
Global climate change has become a major concern worldwide. The spatio-temporal characteristics of net ecosystem productivity(NEP), which represents carbon sequestration capacity and directly describes the qualitative... Global climate change has become a major concern worldwide. The spatio-temporal characteristics of net ecosystem productivity(NEP), which represents carbon sequestration capacity and directly describes the qualitative and quantitative characteristics of carbon sources/sinks(C sources/sinks), are crucial for increasing C sinks and reducing C sources. In this study, field sampling data, remote sensing data, and ground meteorological observation data were used to estimate the net primary productivity(NPP) in the Inner Mongolia grassland ecosystem(IMGE) from 2001 to 2012 using a light use efficiency model. The spatio-temporal distribution of the NEP in the IMGE was then determined by estimating the NPP and soil respiration from 2001 to 2012. This research also investigated the response of the NPP and NEP to the main climatic variables at the spatial and temporal scales from 2001 to 2012. The results showed that most of the grassland area in Inner Mongolia has functioned as a C sink since 2001 and that the annual carbon sequestration rate amounts to 0.046 Pg C/a. The total net C sink of the IMGE over the 12-year research period reached 0.557 Pg C. The carbon sink area accounted for 60.28% of the total grassland area and the sequestered 0.692 Pg C, whereas the C source area accounted for 39.72% of the total grassland area and released 0.135 Pg C. The NPP and NEP of the IMGE were more significantly correlated with precipitation than with temperature, showing great potential for C sequestration. 展开更多
关键词 Inner Mongolia grassland ecosystem NPP NEP carbon source carbon sink
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Anomalous Atmospheric Circulation, Heat Sources and Moisture Sinks in Relation to Great Precipitation Anomalies in the Yangtze River Valley 被引量:5
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作者 杨辉 《Advances in Atmospheric Sciences》 SCIE CAS CSCD 2001年第5期972-983,共12页
Using the summer (June to August) monthly mean data of the National Centers for Environmental Predictions (NCEP) - National Center for Atmospheric Research (NCAR) reanalysis from 1980 to 1997, atmospheric heat sources... Using the summer (June to August) monthly mean data of the National Centers for Environmental Predictions (NCEP) - National Center for Atmospheric Research (NCAR) reanalysis from 1980 to 1997, atmospheric heat sources and moisture sinks are calculated. Anomalous circulation and the vertically integrated heat source with the vertical integrated moisture sink and outgoing longwave radiation (OLR) flux are examined based upon monthly composites for 16 great wet-spells and 8 great dry-spells over the middle-lower reaches of the Yangtze River. The wind anomaly exhibits prominent differences between the great wet-spell and the great dry-spell over the Yangtze River Valley. For the great wet-spell, the anomalous southerly from the Bay of Bengal and the South China Sea and the anomalous northerly over North China enhanced low-level convergence toward a narrow latitudinal belt area (the middle-lower reaches of the Yangtze River). The southerly anomaly is connected with an anticyclonic anomalous circulation system centered at 22 degreesN, 140 degreesE and the northerly anomaly is associated with a cyclonic anomalous circulation system centered at the Japan Sea. In the upper level, the anomalous northwesterly between an anticyclonic anomalous system with the center at 23 degreesN, 105 degreesE and a cyclonic anomalous system with the center at Korea diverged over the middle-lower reaches of the Yangtze River. On the contrary, for the great dry-spell, the anomalous northerly over South China and the anomalous southerly over North China diverged from the Yangtze River Valley in the low level. The former formed in the western part of a cyclonic anomalous system centered at 23 degreesN, 135 degreesE. The latter was located in the western ridge of an anticyclonic anomalous system in the northwestern Pacific. The upper troposphere showed easterly anomaly that converged over the middle-lower reaches of the Yangtze River. A cyclonic anomalous system in South China and an anticyclonic system centered in the Japan Sea enhanced the easterly. Large atmospheric heat source anomalies of opposite signs existed over the western Pacific - the South China Sea, with negative in the great wet-spell and positive in the great dry-spell. The analysis of heat source also revealed positive anomalous heat sources during the great wet-spell and negative anomalous heat sources during the great dry-spell over the Yangtze River valley. The changes of the moisture sink and OLR were correspondingly altered, implying the change of heat source anomaly is due to the latent heat releasing of convective activity. Over the southeastern Tibetan Plateau- the Bay of Bengal, the analysis of heat source shows positive anomalous heat sources during the great wet-spell and negative anomalous heat sources during the great dry-spell because of latent heating change. The change of divergent wind coexisted with the change of heat source. In the great wet-spell, southerly divergent wind anomaly in the low level and northerly divergent wind anomaly in high-level are seen over South China. These divergent wind anomalies are helpful to the low-level convergence anomaly and high-level divergence anomaly over the Yangtze River valley. The low-level northerly divergent wind anomaly and high-level southerly divergent wind anomaly over South China reduced the low-level convergence and high-level divergence over the Yangtze River valley during the great dry-spell. 展开更多
关键词 anomalous atmospheric circulation heat sources and moisture sinks anomalies great precipitation anomalies in the Yangtze River valley
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TiO_(2)/石墨烯基复合材料表征及光催化降解VOCs的研究 被引量:1
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作者 齐俊红 徐丽慧 +2 位作者 陈嘉阳 王黎明 潘虹 《功能材料》 北大核心 2025年第3期3134-3142,3164,共10页
研究采用自组装溶剂热法,以二氧化钛(TiO_(2))和氧化石墨烯(GO)为原料,成功制备了TiO_(2)/rGO复合材料。通过对复合材料进行扫描(SEM)观察发现,TiO_(2)颗粒均匀地分散在还原氧化石墨烯(rGO)的片层上,形成了良好的接触界面;X射线衍射(XRD... 研究采用自组装溶剂热法,以二氧化钛(TiO_(2))和氧化石墨烯(GO)为原料,成功制备了TiO_(2)/rGO复合材料。通过对复合材料进行扫描(SEM)观察发现,TiO_(2)颗粒均匀地分散在还原氧化石墨烯(rGO)的片层上,形成了良好的接触界面;X射线衍射(XRD)图谱证实了TiO_(2)具有锐钛矿相结构,并且rGO的存在并未对TiO_(2)的晶型产生显著影响;X射线光电子能谱(XPS)分析揭示了TiO_(2)与rGO之间发生了电子转移,这对于提高复合材料的光催化性能是有利的。为了评估TiO_(2)/rGO复合材料的光催化活性,选择了“五苯三醛”作为挥发性有机化合物(VOCs)的模型污染物,并在模拟的车内环境中进行了实验。实验中使用了不同浓度的VOCs(15~25 mg/m^(3)),并在100 W白炽灯和500 W氙灯两种光源下进行了光催化降解测试。实验结果表明,在100 W白炽灯照射480 min后,15%(质量分数)TiO_(2)/rGO-6h复合材料对VOCs的降解率分别为41.7%、46.6%和65.3%;而在500W氙灯下,降解效率显著提高到了51.33%、72.89%和78.3%。相比之下,纯TiO_(2)在相同条件下的光催化效率较低,TiO_(2)/rGO复合材料在光催化活性方面有显著提升,并且在广泛的VOCs浓度范围内表现出了高效稳定的光催化活性,特别是在氙灯照射下,其光催化性能明显优于纯TiO_(2)。这项工作为解决车内及大气中的VOCs污染问题提供了新思路,并为进一步开发高效的光催化剂材料打下了坚实的基础。 展开更多
关键词 TiO_(2) 还原氧化石墨烯 不同光源 VOCS 光催化活性
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正宁地区楔形前积模式下长7_(1-2)亚段原油地球化学特征及油源分析 被引量:1
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作者 李宗亮 王延山 +4 位作者 杨庆宁 黄双泉 徐建斌 侯拓 邱雯 《地质科学》 北大核心 2025年第5期1329-1341,共13页
鄂尔多斯盆地南缘正宁地区长7段是原油勘探的一个重要领域。本文在新采集三维地震资料基础上,通过岩心的岩石热解、镜鉴,原油的物性、族组成、生物标志化合物等地球化学数据和油源对比指标分析,对鄂尔多斯盆地南部正宁地区长7_(1)、长7_... 鄂尔多斯盆地南缘正宁地区长7段是原油勘探的一个重要领域。本文在新采集三维地震资料基础上,通过岩心的岩石热解、镜鉴,原油的物性、族组成、生物标志化合物等地球化学数据和油源对比指标分析,对鄂尔多斯盆地南部正宁地区长7_(1)、长7_(2)和长7_(3)亚段烃源岩的生烃能力,以及长7_(1-2)原油地球化学特征和来源进行了分析。研究认为,正宁地区延长组长7_(2)—长2段地层呈楔状前积模式,超覆于长7_(3)页岩之上;长7_(3)、长7_(2)和长7_(1)亚段烃源岩都为优质烃源岩,有机质丰度自下而上逐渐变低;长7_(3)亚段有机质类型以Ⅱ_(1)型为主,长7_(1-2)亚段以Ⅱ_(2)型为主,处于成熟生油阶段。长7_(1-2)段原油为成熟轻质原油,Pr/Ph值分布在0.58~0.75,伽马蜡烷指数分布在0.05~0.07,规则甾烷C_(27-28-29)组成呈“V”构型分布,反映母源沉积环境以淡水—微咸水的还原环境为主,生源为低等水生生物、浮游动物和陆生高等植物的混合型母质。长7_(1-2)亚段原油与长7_(1-2)亚段和长7_(3)亚段上部烃源岩对比性较好,表明长7_(1-2)亚段原油来自长7_(1-2)亚段和长7_(3)亚段上部烃源岩。鄂尔多斯正宁地区长7_(1-2)亚段自身具有供烃能力,这极大地拓展了该区原油勘探领域,为该层位发现规模储量提供了坚实的资源保障。 展开更多
关键词 鄂尔多斯盆地 正宁地区 原油地球化学 油源分析 长7_(1-2)亚段
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Ecosystem carbon storage and sink/source of temperate forested wetlands in Xiaoxing’anling, northeast China 被引量:12
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作者 Biao Wang Changcheng Mu +3 位作者 Huicui Lu Na Li Yan Zhang Li Ma 《Journal of Forestry Research》 SCIE CAS CSCD 2022年第3期839-849,共11页
Wetlands play an important role in the global carbon cycle, but there are still considerable uncertainties in the estimation of wetland carbon storage and a dispute on whether wetlands are carbon sources or carbon sin... Wetlands play an important role in the global carbon cycle, but there are still considerable uncertainties in the estimation of wetland carbon storage and a dispute on whether wetlands are carbon sources or carbon sinks. Xiaoxing’anling are one of several concentrated distribution areas of forested wetland in China, but the carbon storage and carbon sink/source of forested wetlands in this area is unclear. We measured the ecosystem carbon storage (vegetation and soil), annual net carbon sequestration of vegetation and annual carbon emissions of soil heterotrophic respiration of five typical forested wetland types (alder swamp, white birch swamp, larch swamp, larch fen, and larch bog) distributed along a moisture gradient in this area in order to reveal the spatial variations of their carbon storage and quantitatively evaluate their position as carbon sink or source according to the net carbon balance of the ecosystems. The results show that the larch fen had high carbon storage (448.8 t ha^(−1)) (6.8% higher than the larch bog and 10.5–30.1% significantly higher than other three wetlands (P < 0.05), the white birch swamp and larch bog were medium carbon storage ecosystems (406.3 and 420.1 t ha^(−1)) (12.4–21.8% significantly higher than the other two types (P < 0.0 5), while the alder swamp and larch swamp were low in carbon storage (345.0 and 361.5 t ha^(−1), respectively). The carbon pools of the five wetlands were dominated by their soil carbon pools (88.5–94.5%), and the vegetation carbon pool was secondary (5.5–11.5%). At the same time, their ecosystem net carbon balances were positive (0.1–0.6 t ha^(−1) a^(−1)) because the annual net carbon sequestration of vegetation (4.0–4.5 t ha^(−1) a^(−1)) were higher than the annual carbon emissions of soil heterotrophic respiration (CO_(2) and CH_(4)) (3.8–4.4 t ha^(−1) a^(−1)) in four wetlands, (the alder swamp being the exception), so all four were carbon sinks while only the alder swamp was a source of carbon emissions (− 2.1 t ha^(−1) a^(−1)) due to a degraded tree layer. Our results demonstrate that these forested wetlands were generally carbon sinks in the Xiaoxing’anling, and there was obvious spatial variation in carbon storage of ecosystems along the moisture gradient. 展开更多
关键词 Temperate forested wetlands Ecosystem carbon storage Carbon sink or source Xiaoxing’anling of China
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Source-Sink Relationship in Intersubspecific Hybrid Rice 被引量:2
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作者 LI Ji-hang XIANG Xun-chao +1 位作者 HE Li-bin LI Ping 《Rice science》 SCIE 2006年第4期250-256,共7页
Three indica restorer lines (Mianhui 725, Shuhui 527, Shuhui 881), an American rice variety Lemont and a javanica rice variety Xiangdali were crossed with japonica Kitaake, and five F1 hybrids were obtained to study... Three indica restorer lines (Mianhui 725, Shuhui 527, Shuhui 881), an American rice variety Lemont and a javanica rice variety Xiangdali were crossed with japonica Kitaake, and five F1 hybrids were obtained to study the photosynthetic and agronomic traits. The data on photosynthetic characteristics indicated that the net photosynthetic rate (Pn) of the five F1 hybrids was significantly higher than that of their parents (or one of them) under high photosynthetic flux density (PFD); while the overall performance of hybrids was better than their respective parents in apparent quantum yield (AQY), carboxylation efficiency (CE) and CO2 compensation point (CCP). Moreover, the photosynthetic performance of the five F1 were different due to the variation in heredity and the typical indica-japonica hybrids, Mianhui 725/Kitaake and Shuhui 527/Kitaake, were better than the others on this aspect. The agronomic traits revealed that the five F1 exhibited different heterosis, with Shuhui 881/Kitaake the largest sink followed by Mianhui 725/Kitaake, Shuhui 527/Kitaake, Lemont/Kitaake and Xiangdali/Kitaake. The production potential of indica-japonica hybrids was higher than that of the other two hybrids, which was consistent with the performance of Pn. However, the superior trait of indica-japonica hybrids on sink size has not been fully turned into high yield because of abnormal seed setting. Therefore, attention should be paid to the proper genome coordination and appropriate genetic distance so as to achieve super high yielding. 展开更多
关键词 RICE intersubspecific hybrid source sink net photosynthetic rate genetic distance HETEROSIS
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A Review of Comminution Age Method and Its Potential Application in the East China Sea to Constrain the Time Scale of Sediment Source-to-Sink Process 被引量:5
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作者 LI Chao YANG Shouye +2 位作者 LIAN Ergang BI Lei ZHANG Zhaofeng 《Journal of Ocean University of China》 SCIE CAS 2015年第3期399-406,共8页
The East China Sea(ECS) is a river-dominated epicontinental sea, linking the Asian continent to the northwestern Pacific via the large rivers originating from Tibetan Plateau. The relevant huge influx of riverine detr... The East China Sea(ECS) is a river-dominated epicontinental sea, linking the Asian continent to the northwestern Pacific via the large rivers originating from Tibetan Plateau. The relevant huge influx of riverine detritus has developed unique sedimentary systems in the ECS during the Quaternary, offering ideal terrestrial archives for reconstructing Quaternary paleoenvironmental changes and studying land-sea interactions. Overall, two characteristic river systems dominate the sedimentary systems and sediment source to sink transport patterns in the ECS, represented by the Changjiang(Yangtze River) and Huanghe(Yellow River) for the large river system and Taiwan rivers for the small river system. Given this, the sediments derived from both river systems bear distinct features in terms of parent rock lithology, provenance weathering and sediment transport. Previous studies mostly focus on either the ‘source' discrimination or the ‘sink' records of the sedimentary system in the ECS, while the source to sink process linking the land and sea, in particular its time scale, has been poorly understood. Here we introduce a newly-developed dating technique, the ‘comminution age' method, which offers a quantitative constraint on the time scale of sediment transfer from its ultimate source to the final depositional sink. This novel method is of great significance for improving our understanding on the earth surface processes including tectonic-climate driven weathering, and sediment recycling in relation to landscape evolution and marine environmental changes. The application of comminution age method in the ECS will provide important constraints on sediment source-to-sink process and more evidences for the construction of late Quaternary paleoenvironmental changes under these unique sedimentary systems. 展开更多
关键词 sediment transport time 234U/238U East China Sea source to sink
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近20年成渝地区双城经济圈植被碳源/汇时空格局演化及其变异性特征 被引量:1
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作者 黄林 汪洋 +3 位作者 李帆 赵俊杰 李培 张珂宁 《贵州师范大学学报(自然科学版)》 北大核心 2025年第3期63-73,共11页
净生态系统生产力(NEP)是陆地生态系统碳源/汇定量评价的重要指标。明晰区域NEP时空演化格局对评估区域碳中和潜力和制定区域“双碳”目标、实现高质量发展具有重要指导意义。以成渝地区双城经济圈为研究区,采用2000、2005、2010、2015... 净生态系统生产力(NEP)是陆地生态系统碳源/汇定量评价的重要指标。明晰区域NEP时空演化格局对评估区域碳中和潜力和制定区域“双碳”目标、实现高质量发展具有重要指导意义。以成渝地区双城经济圈为研究区,采用2000、2005、2010、2015、2020年5期遥感、气象、土地利用空间数据集,基于改进CASA和土壤呼吸模型对2000—2020年的生态系统碳汇进行估算,构建变异性指数探讨其时空格局特征。结果表明:1)成渝地区双城经济圈整体呈碳源属性,但碳源属地比例逐渐降低,上述5年碳源面积占比分别为87.2%、85.0%、75.8%、61.5%、60.5%,多年NEP均值为-53.12 gC·m^(-2)·a^(-1);2)NEP的整体空间格局表现为“边缘高、中间低”,内部呈现“双核多心放射状”的形态,表现出明显的地形因素伴生性和城镇化水平互斥性;3)2000—2020年NEP上升趋势显著,82.1%的区域表现为增长趋势,大-中-小幅度增加、小-中-大幅度减少的区域占比分别为33.7%、27.2%、22.3%、8.9%、5.2%、3.7%;4)NEP的变异格局与地形呈现出一定耦合特征,显著减少区域集中于平原地貌与城镇聚集交叉地带,显著增加区域集中于盆周中低山区及内部低山及中高丘陵区;地形复杂程度整体与变异幅度呈非线性正相关,与变异趋势呈非线性负相关。 展开更多
关键词 植被碳源/汇 空间格局演化 动态趋势 成渝地区双城经济圈 遥感反演
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Convection of Maxwell fluid over stretching porous surface with heat source/sink in presence of nanoparticles:Lie group analysis 被引量:1
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作者 Limei CAO Xinhui SI Liancun ZHENG 《Applied Mathematics and Mechanics(English Edition)》 SCIE EI CSCD 2016年第4期433-442,共10页
The convection of a Maxwell fluid over a stretching porous surface with a heat source/sink in the presence of nanoparticles is investigated. The Lie symmetry group transformations are used to convert the boundary laye... The convection of a Maxwell fluid over a stretching porous surface with a heat source/sink in the presence of nanoparticles is investigated. The Lie symmetry group transformations are used to convert the boundary layer equations into coupled nonlinear ordinary differential equations. The ordinary differential equations are solved numerically by the Bvp4c with MATLAB, which is a collocation method equivalent to the fourth-order mono-implicit Runge-Kutta method. Furthermore, more attention is paid to the effects of the physical parameters, especially the parameters related to nanoparticles, on the temperature and concentration distributions with consideration of permeability and the heat source/sink. 展开更多
关键词 Lie group Maxwell fluid porous stretching surface heat sink or source
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中国燃煤电厂与沉积盆地咸水层CO_(2)封存的源汇匹配研究
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作者 李毅 周凡 +2 位作者 王金生 盖鹏 王浩 《中国地质》 北大核心 2025年第4期1513-1527,共15页
【研究目的】燃煤电厂是中国CO_(2)排放的一个主要集中源,为了完成碳减排的目标,需对其进行碳捕获和封存(CCUS)改造,利用咸水层进行封存是有效手段,两者的源汇匹配评价是推动改造工程的重要一环。但当前缺乏详细和系统地针对全国燃煤电... 【研究目的】燃煤电厂是中国CO_(2)排放的一个主要集中源,为了完成碳减排的目标,需对其进行碳捕获和封存(CCUS)改造,利用咸水层进行封存是有效手段,两者的源汇匹配评价是推动改造工程的重要一环。但当前缺乏详细和系统地针对全国燃煤电厂CO_(2)排放和沉积盆地咸水层封存的源汇匹配研究。【研究方法】本文从盆地一级构造尺度出发,基于全国燃煤电厂CO_(2)排放特征,建立一套考虑全流程的源汇匹配优化模型。【研究结果】99%的电厂均可在唯一的封存地进行封存,陆域盆地作为封存地仍是大多数电厂的首选,海域盆地在沿海地区的匹配中体现出优越性。针对10~40年改造目标年限,2021—2030年电厂到封存地的最大运输距离达到539.28 km,2031—2040年、2041—2050年和2051—2060年的最大运输距离均为660.58 km。【结论】从CO_(2)年捕集量和运输距离来看,在华北、华东、华中和西北地区建立大规模的CO_(2)运输管网进行封存的潜力大于东北和南方。CCUS改造技术成本和运输距离是影响源汇匹配结果的最重要因素,随着改造技术的提高,平均改造成本从500元/t CO_(2)下降到300元/t CO_(2)以内。本研究结果为燃煤电厂的CCUS改造提供了政策决定依据。 展开更多
关键词 燃煤电厂 CO_(2)封存 咸水层 源汇匹配模型 改造成本 地质调查工程
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