Plasmonic nanoantennas provide unique opportunities for precise control of light–matter coupling in surface-enhanced infrared absorption(SEIRA)spectroscopy,but most of the resonant systems realized so far suffer from...Plasmonic nanoantennas provide unique opportunities for precise control of light–matter coupling in surface-enhanced infrared absorption(SEIRA)spectroscopy,but most of the resonant systems realized so far suffer from the obstacles of low sensitivity,narrow bandwidth,and asymmetric Fano resonance perturbations.Here,we demonstrated an overcoupled resonator with a high plasmon-molecule coupling coefficient(μ)(OC-Hμresonator)by precisely controlling the radiation loss channel,the resonator-oscillator coupling channel,and the frequency detuning channel.We observed a strong dependence of the sensing performance on the coupling state,and demonstrated that OC-Hμresonator has excellent sensing properties of ultra-sensitive(7.25%nm^(−1)),ultra-broadband(3–10μm),and immune asymmetric Fano lineshapes.These characteristics represent a breakthrough in SEIRA technology and lay the foundation for specific recognition of biomolecules,trace detection,and protein secondary structure analysis using a single array(array size is 100×100μm^(2)).In addition,with the assistance of machine learning,mixture classification,concentration prediction and spectral reconstruction were achieved with the highest accuracy of 100%.Finally,we demonstrated the potential of OC-Hμresonator for SARS-CoV-2 detection.These findings will promote the wider application of SEIRA technology,while providing new ideas for other enhanced spectroscopy technologies,quantum photonics and studying light–matter interactions.展开更多
提出一种人体植入式医学装置电能传输新方法,该方法以人体组织作为耦合介质,通过体内、外耦合极板构建耦合电容,以耦合电场实现电能的无线传输。分析了人体组织的电学特性,设计了电能传输系统,并通过实验验证了该方法的可行性。实验中,...提出一种人体植入式医学装置电能传输新方法,该方法以人体组织作为耦合介质,通过体内、外耦合极板构建耦合电容,以耦合电场实现电能的无线传输。分析了人体组织的电学特性,设计了电能传输系统,并通过实验验证了该方法的可行性。实验中,通过36 cm2的耦合面积,穿越2 cm厚度的生物组织,可传输100 m W的可用电能,传输效率为35%~40%。该电能传输方式具有无电涡流致热、电磁干扰小、易于与医学仪器集成的优点,是人体植入式医学装置无线电能供给的新思路。展开更多
Understanding the relationship between plasmon near-field enhancement and lifetime is crucial for various applications,yet their inverse correlation in single-element nanoresonators remains underexplored.Here,we exper...Understanding the relationship between plasmon near-field enhancement and lifetime is crucial for various applications,yet their inverse correlation in single-element nanoresonators remains underexplored.Here,we experimentally demonstrate an inverse correlation between these two parameters in single-element gold lateral V-shaped nanoresonators under different light polarization conditions by tuning the opening angle,through femtosecond time-resolved photoemission electron microscopy.Specifically,under p-polarized light irradiation,as the opening angle of V-shaped nanoresonators decreases,the plasmon near-field enhancement increases while the lifetime shortens simultaneously.展开更多
Photonic hardware implementation of spiking neural networks,regarded as a viable potential paradigm for ultra-high speed and energy efficiency computing,leverages spatiotemporal spike encoding and event-driven dynamic...Photonic hardware implementation of spiking neural networks,regarded as a viable potential paradigm for ultra-high speed and energy efficiency computing,leverages spatiotemporal spike encoding and event-driven dynamics to simulate brain-like parallel information processing.Silicon-based microring resonators(MRRs)offer a power efficiency and ultrahigh flexibility scheme to mimic biological neuron,however,their substantial potential for integrated neuromorphic systems remains limited by insufficient exploration of MRR-based spiking digital and analog computation.Here,an all-optical neural dynamics framework,encompassing both excitatory and inhibitory behaviors based on multi-wavelength auxiliary and competition mechanism in an MRR,is proposed numerically.Leveraging multi-wavelength resonance characteristics and wavelength division multiplexing(WDM)technology,a single MRR implements the five fundamental optical digital logic gates:AND,OR,NOT,XNOR and XOR.Besides,the cascading capabilities of MRR-based spiking neurons are demonstrated through multi-level digital logic gates including NAND,NOR,4-input AND,8-input AND,and a full adder,emphasizing their promise for large-scale digital logic networks.Furthermore,an exemplary binary convolution has been achieved by utilizing the proposed MRR-based digital logic operation,illustrating the potential of all-optical binary convolution to compute image gradient magnitudes for edge detection.Such passive photonic neurons and networks promise access to the high transmission speed and low power consumption inherent to optical systems,thus enabling direct hardware-algorithm co-computation and accelerating artificial intelligence.展开更多
基金supported by A*STAR under the“Nanosystems at the Edge”program(Grant No.A18A4b0055)Ministry of Education(MOE)under the research grant of R-263-000-F18-112/A-0009520-01-00+1 种基金National Research Foundation Singapore grant CRP28-2022-0038the Reimagine Re-search Scheme(RRSC)Project(Grant A-0009037-02-00&A0009037-03-00)at National University of Singapore.
文摘Plasmonic nanoantennas provide unique opportunities for precise control of light–matter coupling in surface-enhanced infrared absorption(SEIRA)spectroscopy,but most of the resonant systems realized so far suffer from the obstacles of low sensitivity,narrow bandwidth,and asymmetric Fano resonance perturbations.Here,we demonstrated an overcoupled resonator with a high plasmon-molecule coupling coefficient(μ)(OC-Hμresonator)by precisely controlling the radiation loss channel,the resonator-oscillator coupling channel,and the frequency detuning channel.We observed a strong dependence of the sensing performance on the coupling state,and demonstrated that OC-Hμresonator has excellent sensing properties of ultra-sensitive(7.25%nm^(−1)),ultra-broadband(3–10μm),and immune asymmetric Fano lineshapes.These characteristics represent a breakthrough in SEIRA technology and lay the foundation for specific recognition of biomolecules,trace detection,and protein secondary structure analysis using a single array(array size is 100×100μm^(2)).In addition,with the assistance of machine learning,mixture classification,concentration prediction and spectral reconstruction were achieved with the highest accuracy of 100%.Finally,we demonstrated the potential of OC-Hμresonator for SARS-CoV-2 detection.These findings will promote the wider application of SEIRA technology,while providing new ideas for other enhanced spectroscopy technologies,quantum photonics and studying light–matter interactions.
文摘提出一种人体植入式医学装置电能传输新方法,该方法以人体组织作为耦合介质,通过体内、外耦合极板构建耦合电容,以耦合电场实现电能的无线传输。分析了人体组织的电学特性,设计了电能传输系统,并通过实验验证了该方法的可行性。实验中,通过36 cm2的耦合面积,穿越2 cm厚度的生物组织,可传输100 m W的可用电能,传输效率为35%~40%。该电能传输方式具有无电涡流致热、电磁干扰小、易于与医学仪器集成的优点,是人体植入式医学装置无线电能供给的新思路。
基金National Key Research and Development Program of China(2022YFA1604304,2022YFA1604303)National Natural Science Foundation of China(12404356,12374341)+2 种基金Department of Science and Technology of Jilin Province(YDZJ202401607ZYTS)Natural Science Foundation of Chongqing Municipality(CSTB2023NSCQMSX1026,CSTB2023NSCQ-MSX0302,CSTB2023NSCQMSX0708)111 Project(D17017)。
文摘Understanding the relationship between plasmon near-field enhancement and lifetime is crucial for various applications,yet their inverse correlation in single-element nanoresonators remains underexplored.Here,we experimentally demonstrate an inverse correlation between these two parameters in single-element gold lateral V-shaped nanoresonators under different light polarization conditions by tuning the opening angle,through femtosecond time-resolved photoemission electron microscopy.Specifically,under p-polarized light irradiation,as the opening angle of V-shaped nanoresonators decreases,the plasmon near-field enhancement increases while the lifetime shortens simultaneously.
基金supports from National Natural Science Foundation of China(62171087,62475036).
文摘Photonic hardware implementation of spiking neural networks,regarded as a viable potential paradigm for ultra-high speed and energy efficiency computing,leverages spatiotemporal spike encoding and event-driven dynamics to simulate brain-like parallel information processing.Silicon-based microring resonators(MRRs)offer a power efficiency and ultrahigh flexibility scheme to mimic biological neuron,however,their substantial potential for integrated neuromorphic systems remains limited by insufficient exploration of MRR-based spiking digital and analog computation.Here,an all-optical neural dynamics framework,encompassing both excitatory and inhibitory behaviors based on multi-wavelength auxiliary and competition mechanism in an MRR,is proposed numerically.Leveraging multi-wavelength resonance characteristics and wavelength division multiplexing(WDM)technology,a single MRR implements the five fundamental optical digital logic gates:AND,OR,NOT,XNOR and XOR.Besides,the cascading capabilities of MRR-based spiking neurons are demonstrated through multi-level digital logic gates including NAND,NOR,4-input AND,8-input AND,and a full adder,emphasizing their promise for large-scale digital logic networks.Furthermore,an exemplary binary convolution has been achieved by utilizing the proposed MRR-based digital logic operation,illustrating the potential of all-optical binary convolution to compute image gradient magnitudes for edge detection.Such passive photonic neurons and networks promise access to the high transmission speed and low power consumption inherent to optical systems,thus enabling direct hardware-algorithm co-computation and accelerating artificial intelligence.
